Behavioral Reprogramming of Open-Weights Models: Cognitive Plasticity and Alignment Bounds

Large language models (LLMs) are predominantly aligned to function as passive, sycophantic assistants. We challenge this default paradigm by empirically evaluating the cognitive plasticity of open-weight architectures when subjected to rigorous behavioral reprogramming. Our objective is to induce a proactive, Socratic conversational framework, characterized by high-frequency question generation under strictly constrained high-performance computing (HPC) conditions. Through a massively parallelized hyperparameter sweep comprising 405 HPC jobs, we define precise mathematical bounds for parameter-efficient fine-tuning (PEFT). We identify an architectural threshold at LoRA rank r=16 and demonstrate via extensive epoch ablation that generalization capacity strictly reaches its optimal convergence within an optimized training window of e in [2, 3] depending on dataset density (minimum validation loss of 0.919). Furthermore, scaling model capacity to 14B parameters yielded a lower localized evaluation perplexity (1.414). Subsequent Direct Preference Optimization (DPO) successfully decoupled the underlying assertive behavior from localized syntax, while rigorous cross-lingual stress testing reveals both the capabilities and the structural boundaries of zero-shot persona transfer, demonstrating robust alignment in closely related linguistic families alongside identifiable degradation pathways in morphologically distant targets. These findings establish a rigorous empirical framework for compute-efficient, cross-lingual behavioral modification.