Patent Number: 047822317
Section: claims

1. A method of preparation of .sup.99m Tc elution comprising the steps of, filling a main column composed of a material selected from the group consisting of aluminum, zirconium, quartz, carbon and oxides thereof with a target material comprising at least 10% by weight of molybdenum;  plugging the ends of the main column with a porous material;  closing the ends of the main column;  wrapping the ends of the main column to protect against secondary bacterial contamination;  activating the target material to form a .sup.99 Mo containing sorption matrix accompanied simultaneously by radiation sterilization of the main generator column and its contents by exposure to neutron and accompanied gamma radiation in a reactor;  opening the ends of the main generator column in sterile environment under aseptic conditions of manipulation;  connecting a supply tube to one end of the main column and a discharge tube to the other end in a sterile manner;  placing the main column, supply tube, and discharge tube in a transport container composed of a material selected from the group consisting of lead or depleted uranium;  placing the transport container in a laboratory container, the laboratory container also housing an elution vessel, a protective column, and at least one eluate collection bottle;  connecting the supply tube to an elution vessel in a sterile manner, the elution vessel containing an elution solution;  connecting the discharge tube to one end of a protective column in a sterile manner, the other end having a piercing head;  piercing the seal of an evacuated eluate collection bottle with the piercing head;  drawing the eluation solution through the supply tube, main column containing the sorption matrix, discharge tube, and protective column, and into the eluate collection bottle, the eluate containing .sup.99m Tc. 2. A method as in claim 1 wherein the ratio of the diameter of the main column to its height is 1:2-5; the target material is selected from the group consisting of molybdates and polymolybdates of titanium and zirconium having a molybdenum content of from 20 to 40% by weight; the porous plug is composed of a material selected from the group consisting of aluminum, zirconium, quartz, carbon, oxides and composites thereof, and felt, the elution solution is a 0.9% solution of NaCl by weight; the protective column contains a sorbent selected from the group consisting of zirconium oxide and aluminum oxide; and the transport container is a material selected from the group consisting of lead and depleted uranium. 3. A method as in claim 1 additionally comprising the steps of placing the transport container in a protective container; shipping the protective container to the user, and removing the transport container from the protective container prior to the step of placing the transport container in the laboratory container. 4. A method as in claim 2 additionally comprising the steps of placing the transport container in a protective container; shipping the protective container to the user, and removing the transport container from the protective container prior to the step of placing the transport container in the laboratory container. 5. A method as in claim 1, wherein the target material is selected from the group consisting of molybdates and polymolybdates of zirconium titanium and other elements, the specific activity thereof, expressed in Bq/g of the corresponding element 25 hours after reactor irradiation end, is lower than twice the specific activity of .sup.99 Mo reached irradiating under the same conditions molybdenum in its natural isotopic mixture; the content of molybdenum in the target plugs, covers and other parts of the main generator column are made from elements and their oxides, the specific activity thereof, 24 hours after reactor irradiation end, is lower than twice the specific activity of .sup.99 Mo reached by irradiating under the same conditions molybdenum in its natural isotopic abundance, the specific activity is evaluated by Bq/g of the corresponding element; wherein the elements used are selected from the group consisting of zirconium, titanium, aluminum, carbon, silicon and their oxides; the porous plugs are made from the above mentioned materials formed into fibers, composites, felt or wool. 6. A method as in claim 5 additionally comprising the steps of placing the transport container in a protective container; shipping the protective container to the user, and removing the transport container from the protective container prior to the step of placing the transport container in the laboratory container.