Paper:
The Unreasonable Effectiveness of Structured Random Orthogonal Embeddings
We examine a class of embeddings based on structured random matrices with orthogonal rows which can be applied in many machine learning applications including dimensionality reduction and kernel approximation. For both the JohnsonLindenstrauss transform and the angular kernel, we show that we can select matrices yielding guaranteed improved performance in accuracy and/or speed compared to earlier methods. We introduce matrices with complex entries which give significant further accuracy improvement. We provide geometric and Markov chain-based perspectives to help understand the benefits, and empirical results which suggest that the approach is helpful in a wider range of applications.

Review:
The paper analyses the theoretical properties of a family random projections approaches to approximate inner products in high dimensional spaces. In particular the authors focus on methods based on random structured matrices, namely Gaussian orthogonal matrices and SD-matrices. The latter are indeed appealing since they require significantly less computations to perform the projections thanks to their underlying structure. The authors show that the methods considered perform comparably well (or better) with respect to the Johnson-Lindenstrauss transform (baseline based on unstructured Gaussian matrices). Moreover they show that further improvements can be achieved by extending SD-matrices to the complex domain. The authors extend their analysis to the case random feature based approximation of angular kernels. 
The paper is well written and clear to read, however the discussion of some of the results could be elaborated more. For instance after Thm 3.3, which characterizes the MSE of the orthogonal JL transform based on SD-matrices, it is not discussed in much detail how this compares to the standard JL baseline. Cor. 3.4 does not really help much since it simply states that Thm 3.3 yields to lower MSE, without clarifying the entity of such improvement. In particular it appears that the improvement in performance of the OJLT over JLT is only in terms of constants (w.r.t. the number of sub-sampled dimensions m). 
I found it a bit misleading in Sec. 4, to introduce a general family of kernels, namely the pointwise nonlinear Gaussian kernels, but then immediately focus on a specific instance of such class. The reader expects the following results to apply to the whole family but this is not the case. Reversing the order, and discussing PNG kernels only at the end of the section would probably help the discussion.
I found the term 'Unreasonable' in the title not explained in the text. Is it not reasonable to expect that adding structure to an estimator could make it more effective?
The Mean Squared Error (MSE) is never defined. Although being a standard concept, it is also critical to the theoretical analysis presented in the paper, so it should be defined nevertheless.