  Manipulation of the intersublattice interaction strengh (JRE-TM) in rare
earth (RE)-transition metal (TM) alloys is a key issue to understand how
efficiently the laser-induced angular momentum transfers from 3d to 4f spins
and to have a better control of the ultrafast spin dynamics. In this work, the
relationships between laser-induced demagnetization process and the
intersublattice 3d-4f interaction for the GdCoFe alloys were systematically
studied. The ultrafast two-stage demagnetization process could change into a
one-stage mode as the angular momentum transferring channel between 3d and 4f
spins is switched off, which could be modulated by JRE-TM. Furthermore, both
the effective g-factor and damping constant deduced by the subsequently
laser-induced magnetization precession process diverge at the angular momentum
compensation point based on the ferromagnetic resonance method with the LLG
equations. The results provide an alternative way to efficiently manipulate the
ultrafast demagnetization time for practical applications.
