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It's a blue icon with a white "F," typically found on the home screen. If you're not signed in, type your account information and tap Log In. It's at the top of the screen. The search key is the magnifying glass key on your keyboard. It's the first option in the search results. Be sure to choose this first option instead of "close friends list" or something like it. This opens that person's profile. It's beneath the person's name on their profile. If this person is a member of the Close Friends list, you'll see a blue check mark next to the list's name. This removes the blue check mark from the list's name. It's at the top-right corner of the screen. You've now removed your friend from the Close Friends list.
Open Facebook. Tap the Search box. Type close friends and tap the search key. Select Close Friends. Select the friend you want to remove from the list. Tap Friends. Tap Edit Friend Lists. Tap Close Friends. Tap Done.