Kind of. It isn't as straightforward as you hope, but there is a workaround. When you go through Zelle and are trying to connect to Chime, you'll want to skip the initial "Where do you bank" question. Instead, go to the app's "Move Money" section, then go to add a bank, and click on the "don't see your bank" link. This will allow you to input your Chime account's debit card info into Zelle. That's it; you're done.