Yes, as long as the ingredients you choose do not have any added sugars. I would use yogurt or peanut butter (or nut or seed butter if there is an allergy) for the coating. If using nuts as a topping, be sure to finely ground. For babies, I recommend slicing the halved banana into 3 spears and leaving out the popsicle sticks. These banana popsicles are great for teething too.