Indeed you can! Here's how: put the coconut shrimp on a cookie sheet lined with waxed paper or parchment paper. Make sure they are in a single layer so they don't stick together. Then pop them into the freezer. After a few hours, you can put them into a zip top baggie. When you are ready to fix them, grab them out of the freezer and fry or bake following the instructions above. Oh. And don't let them thaw, or the coating will come off. And that will make you cry...