Yes, you can use the shampoo for babies as a face wash. Now, this is mainly because most shampoos for babies come with a hypoallergenic formula that cleanses skin without irritation. In fact, most shampoos are gentle enough to cleanse your baby’s face without any irritation. In fact, even you could use it to remove your eye makeup. In short, the shampoos for babies surely make up for a good babyface wash too.