# Laser-Driven Proton-Boron Fusions: Influences of the Boron State

Authors: Xiaochuan Ning; Tianyi Liang; Dong Wu; Shujun Liu; Yangchun Liu; Tianxing Hu; Zhengmao Sheng; Jieru Ren; Bowen Jiang; Yongtao Zhao; Dieter H. H. Hoffmann; X.T. He
Journal: Laser and Particle Beams
 (2022)

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## Abstract

The proton-boron (p11 B) reaction is regarded as the holy grail of advanced fusion fuels, where the primary reaction produces 3 energetic α particles. However, due to the high nuclear bounding energy and bremsstrahlung energy losses, energy gain from the p 11 B fusion is hard to achieve in thermal fusion conditions. Owing to advances in intense laser technology, the p11 B fusion has drawn renewed attention by using an intense laser-accelerated proton beam to impact a boron-11 target. As one of the most influential works in this field, Labaune et al. first experimentally found that states of boron (solid or plasma) play an important role in the yield of α particles. This exciting experimental finding rouses an attempt to measure the nuclear fusion cross section in a plasma environment. However, up to now, there is still no quantitative explanation. Based on large-scale, fully kinetic computer simulations, the inner physical mechanism of yield increment is uncovered, and a quantitative explanation is given. Our results indicate the yield increment is attributed to the reduced energy loss of the protons under the synergetic influences of degeneracy effects and collective electromagnetic effects. Our work may serve as a reference for not only analyzing or improving further experiments of the p 11 B fusion but also investigating other beam-plasma systems, such as ion-driven inertial confinement fusions.


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## Body

## 1. Introduction

Progress in fusion experiments has been continuously made towards the final goal of contributing to the world’s energy supply. Both the magnetic confinement fusion (MCF) experiments and the inertial confinement fusion (ICF) experiments have achieved significant milestones in recent years. The Experimental Advanced Superconducting Tokamak (EAST) at Hefei has made a world record for realizing a 101-second H-mode discharge [1], and the most advanced ICF experiments at the Livermore National Ignition Facility (NIF) have obtained a 1.35-MJ fusion energy output recently, which is about 70% of the laser input energy [2]. Despite the great achievements, there remains a long way to go to solve the energy crisis. For the magnetic confinement approach, adequate plasma confinement time and qualified materials for the first wall of the reactor, which can bear the tough conditions, are still two main issues to be addressed. As for the inertial confinement approach, in the case of the NIF, though it obtains 1.35-MJ energy, it starts with more than 400 MJ of total stored energy. From this perspective, the ratio of the total output energy to the total input energy is quite low and far from the envisioned goal of achieving a gain of 10. Moreover, 14-MeV neutrons produced by deuterium-tritium (D-T) fusion also raise some concerns about induced radioactivity, and it is still a challenging problem to efficiently convert neutron energy into useful electricity.While we are convinced that nuclear fusion is the world energy source of the future, it is obvious that even if, from now on, all fusion scenarios based on the ITER technology or similar technology proceed on schedule, fusion will not contribute significantly to eliminating the problems associated with climate change in a short time. Having said that, we believe that it makes sense to investigate fusion scenarios that use fusion fuel that is not radioactive and is available in abundant quantities. The holy grail of advanced fusion fuels, therefore, is considered to be the p11 B reaction, where the primary reaction produces 3 energetic α particles.(1)11B+p⟶3α+8.7MeV.Only secondary reactions produce neutrons and induce radioactivity. Although the peak fusion cross section is comparable to the D-T fusion, due to the much higher nuclear bounding energy and bremsstrahlung energy losses, energy gain from the p 11 B fusion is hard to achieve in thermal fusion conditions.Owing to advances in laser technology [3, 4], it has becomes easier to obtain high-intensity ion beams [5, 6] and explore warm-dense-matter physics [7, 8] or high-energy-density physics [9, 10], and the p 11 B fusion has also drawn renewed attention [11–13]. The proposal of using intense laser beams or intense laser-accelerated proton beams to impact a boron target so as to generate the p 11 B fusion is becoming increasingly attractive. Based on this method, a number of groups [14–20] have performed a series of experiments on the p 11 B fusion reaction and measured the yields of α particles. Meanwhile, significant progress has also continuously been made in this field. The record yield of α particles has increased from 105/sr in 2005 [14, 21] to 1010/sr in 2020 [18]. However, there still remain unclear physical mechanisms in the interaction of a proton beam and a boron target, which strongly depends on the intensity of the proton beam as well as the conditions of the boron target, including temperature, density, ingredients, and so on, and potentially has a large influence on the possibility of the p 11 B fusion reaction and the α-particle yield. Labaune et al. [15] first experimentally found that states of boron (solid or plasma) play an important role in the yield of α particles produced by the p 11 B fusion reaction. In their experiments, compared with boron solid, a boron plasma ablated by a nanosecond laser can produce many more (nearly two orders of magnitude more) α particles under the impact of a proton beam accelerated by a picosecond laser. As the inner physical mechanism of their experiments is still not clear, in order to figure out the issue, we have recently performed a set of simulations according to their experiments.


## 2. The Interaction between a Nanosecond Laser and a Boron Solid

To ascertain the specific state of the boron target after it is ablated, we have performed a one-dimensional radiation-hydrodynamic simulation with the MULTI-1D code [22] on the interaction of a nanosecond laser pulse and a boron solid, which is the first step in the experiment of Labaune et al. The MULTI-1D code has been widely used by various authors [23–27]. Readers are suggested to refer to Ref. [22] for more detailed information. In our simulation, the grid size is 8 μm and the time step is 0.02 ns. To be consistent with the experiments, the laser duration time is 1.5 ns with a 0.53μm wavelength and an intensity of 6×1014Wcm−2. The initial mass density of the boron solid is set to 2.34 g/cm3. The simulation results of the mass density distributions and the temperature distributions of the boron target at different moments are displayed in Figures 1(a) and 1(c). For the purpose of further analysis, we have extracted the data at t = 1.2 ns, as shown in Figures 1(b) and 1(d). A low-density boron plasma is widely formed in the region away from the boron solid, whereas, on the surface of the boron solid, there actually exists a high-density boron plasma that is driven by shocks. To the best of our knowledge, this high-density boron plasma was not considered seriously in previous studies. It can also be seen in Figures 1(b) and 1(d) that the surface high-density boron plasma is about 5 times denser than the boron solid, its range is about tens of microns, and its temperature is about 10 eV. Under this condition, the ionization degree of the boron target is about two [28]. To quantitatively evaluate the impact of degeneracy effects, we can define the degeneracy degree of plasma electrons as θ=kBTe/EF, where kBTe is the thermal energy and EF=3π2ne2/3ℏ2/2me is the Fermi energy. Here, ne is the density of plasma electrons, ℏ is the reduced Planck’s constant and me is the electron mass. By using the above parameters of the boron target, we can obtain.(2)θ=kBTeEF=0.23<1.This indicates that after the laser ablated the boron solid, degeneracy effects indeed should be taken into account.Figure 1
Evolution of the mass density distribution in (a) and the temperature distribution in (c) of boron ions with time. (b) and (d) correspond to the mass density distribution and the temperature distribution att = 1.2 ns, respectively.


## 3. The Interaction Between a Proton Beam and a Boron Target under the Different States

Next, we further performed another set of simulations with the LAPINS code [29–33] on the p11B fusion by injecting proton beams into a boron solid and a boron plasma, respectively. To make the simulations more credible and closer to the real experimental situation, modules of collisional effects [30], degeneracy effects [31] and nuclear reactions [32] are contained in the LAPINS code. Detailed information on these modules can be found in the relevant references. Moreover, to deal with the self-generated electromagnetic fields of the beam-target system, collective electromagnetic effects are also considered in the LAPINS code. As a hybrid PIC code, the LAPINS code treats plasma ions and the injected beam particles by using the traditional PIC method, while plasma electrons are treated as a fluid, of which the current density is solved by applying Ampere’s law as follows [34]:(3)Je=12π∇×B−12π∂E∂t−Jb−Ji,where B is the magnetic field, E is the electric field, Jb is the beam current density and Ji is the plasma ion current density. Applying the continuity equation∇⋅J+∂ρ/∂t=0, where J=Jb+Je+Ji is the total current density, and ρ is the charge density, we can see that the Poisson’s equation ∇⋅E=2πρ is rigorously satisfied, which indicates the charge separation electric field is naturally contained in the LAPINS code.When a charged particle beam is injected into a target, target electrons will quickly respond to the electromagnetic fields generated by the beam and neutralize the beam’s charge and current. The fields generated by the beam-target system depend on not only the quality of the beam but also the target’s ability to cancel the beam charge and current [34]. A widely used model to calculate the electric field is the basic Ohm’s law [34–38], E=ηJe, where η is the resistivity, which is obtained by averaging over all binary collisions at each time step for each simulation cell in a natural manner. The LAPINS code applies to a more general form as follows:(4)E=ηJe−ve×B−1ene∇pe,where ve is the flow velocity of plasma electrons, pe is the plasma electron thermal pressure, ne is the plasma electron density, and e is the elementary charge. The magnetic field is finally derived from Faraday’s law,∂B/∂t=−∇×E. As only a part of Maxwell’s equations needs to be solved, this method is of high speed and particularly useful for large-scale simulations.As mentioned above, degeneracy effects and collective electromagnetic effects are important in our cases. To evaluate the influences of these two effects on the p11 B fusion, we have performed four simulations. With the module of collective electromagnetic effects on/off, a proton beam interacts with a boron solid/plasma. These simulations are based on a two-dimensional Z–Y Cartesian geometry. The grid size is 0.1 μm× 0.2 μm, and the time step is 1.6 fs. To make the proton beam possess a wide energy spectrum similar to the experimental result obtained by Labaune et al., we set both the kinetic energy and the temperature of the proton beam to 1 MeV. The duration time of the proton beam is 1 ps. The parameters of the boron targets are extracted from the results of the MULTI-1D simulation in Section 2. The density of the boron solid and the boron plasma is 2.34 g/cm 3 and 11.4 g/cm 3, respectively. The temperature of the boron solid is set to 0.0243 eV (room temperature), and the temperature of the boron plasma is set to 10 eV. The simulation results of the proton mass density distributions and the electric field distributions at t = 1.3 ps are displayed in Figure 2.Figure 2
Mass density distributions of the proton beam and the electric field distributions att = 1.3 ps for the boron solid in (a) and (c) and for the laser-ablated boron solid (boron plasma) in (b) and (d), respectively. The boron targets are located on the right side of the white dashed lines in (a) and (b). The black arrows in (a) and (b) indicate the incident direction of the proton beams, of which the angle is 45° to the z-axis. The white arrows in (c) and (d) are the directions of the electric fields. In (d), the white ‘×100’ means the electric field is magnified by a factor of 100, which generally suggests the real electric field in (d) is at least 100 times weaker than that in (c).


## 4. Results and Discussion

Comparing Figures2a and 2b, we can see that for the boron solid, the proton beam can only penetrate to the surface, whereas for the boron plasma, it can penetrate to a longer distance. This difference can be explained as follows. The boron solid has a large resistivity, and the boron plasma, with abundant free electrons, has a much lower resistivity. Ohm’s law (4) reveals the fact that the large difference in resistivity will lead to a significant difference in the electric field generation. As shown in Figure. 2c and 2d, the maximum value of the electric field in the boron solid is more than 100 times stronger than that in the boron plasma. Such a strong electric field in the boron solid will greatly prevent the beam from penetrating deeper into the target.Imitating the experimental measurement method, we have recorded the energy spectra ofα particles escaping from the left simulation boundary in the range of 0 to 6.5 MeV, which are plotted in Figure 3. Comparing the cases of the boron plasma without electromagnetic fields (5N-noEB) and the boron solid without electromagnetic fields (N-noEB), we find that when electromagnetic fields are not calculated in the simulations, there are about 40% more α particles produced by the p11B fusion reactions in the laser-ablated boron solid (boron plasma). This difference is attributed to degeneracy effects, which do not play a role in the solid boron target but become non-negligible after laser ablation, as mentioned above. A theoretical explanation can be given here. For degenerate electrons, their velocity distribution is governed by the Fermi ̶Dirac (FD) statistics as follows:(5)fFDve=2me32πℏ3ne1expβEe−μ+1,where me is the electron mass, β=1/kBTe, Ee is the electron energy, and μ is the chemical potential. The dielectric function of degenerate electrons can be expressed as [39].(6)εk,ω=1+14πkFa02z3gu+z−gu−z.Here, a0 is the Bohr radius, kF=mevFℏ=3π2ne1/3, u=ω/kvF, z=k/2kF, and(7)gx=∫0∞ydyexpDy2−βμ+1lnx+yx−y,where D=EFβ is the degeneracy parameter. Finally, the stopping power of degenerate electrons can be obtained by the widely used dielectric formalism [40–43].(8)sp=−dEdz=2Ze2πv2∫0∞dkk∫0kvdωωIm−1εk,ω.For the convenience of analysis, it is instructive to take advantage of the stopping power per unit density (SPPUD) to evaluate the influence of degeneracy effects(9)sp′=−spne.Figure 4 shows the numerical results of (9) for different electron densities. It can be seen that if the electron density is increased from 2.52×1023 cm −3 (density of the boron solid) to 1.26×1024 cm −3 (density of the boron plasma), SPPUD of the electrons is decreased. In our cases, the yield of α particles produced by the p 11 B fusion can be expressed as [18].(10)Nα=3NpneZi∫0E0σEdEdz−1dE=3NpZi∫0E0σEsp′dE,where Np is the number of protons, Zi is the charge number of the boron ion, andσE is the cross section of the p 11 B fusion. (10) reveals the relation between the yield of α particles and the SPPUD of the electrons and implies that the proton beam propagating in the high-density boron plasma will have more chances to collide with boron nuclei, generate the p 11 B fusion and produce α particles, which is consistent with our simulation results about the gap between the cases of the boron plasma without electromagnetic fields (5N-noEB) and the boron solid without electromagnetic fields (N-noEB) in Figure 3. Both the theory and the simulations indicate that degeneracy effects have an influence on the p 11 B fusion. Nonetheless, quantitatively speaking, they are not the primary factor that causes the significant difference in the yield of α particles in the experiments of Labaune et al. since, as shown in Figure 3, they can only increase the yield by about 40%.Figure 3
The energy spectra ofα particles escaping from the left simulation boundary in the range of 0 MeV to 6.5 MeV: (1) the blue line (N-noEB), the boron solid without electromagnetic fields; (2) the red line (5N-noEB), the boron plasma without electromagnetic fields; (3) the blue triangle line (N-EB), the boron solid with electromagnetic fields; (4) the red square line (5N-EB), the boron plasma with electromagnetic fields. The yellow patch corresponds to where it cannot be measured in the experiments.Figure 4
SPPUD as a function of the proton energy. For the blue solid line, the electron density isne=2.52×1023 cm −3, corresponding to the density of the boron solid, and for the red dotted line, the electron density is ne=1.26×1024 cm −3, corresponding to the density of boron plasma.It can be seen in Figure3 that there is a large gap between the cases of the boron solid without electromagnetic fields (N-noEB) and the boron solid with electromagnetic fields (N-EB), which indicates that in terms of the boron solid, collective electromagnetic effects have a huge influence on the number of fusion reactions and the yield of α particles. As mentioned above and shown in Figure 2c, when the proton beam is injected into the boron solid, a strong stopping electric field will be generated. On the one hand, it can greatly increase the energy loss of the proton beam and prevent the beam from penetrating. Recently, Ren et al. presented a piece of experimental evidence on the significantly enhanced energy loss of a laser-accelerated proton beam in the dense ionized matter [44], which is similar to the case we are describing. On the other hand, (10) shows that if the energy loss of the beam increases, the number of fusion reactions and the yield of α particles will decrease accordingly. For the boron plasma, the gap between the cases of the boron plasma without electromagnetic fields (5N-noEB) and the boron plasma with electromagnetic fields (5N-EB) is not that large because, compared with the boron solid, the boron plasma has a much lower resistivity and, according to Ohm’s law Eq. (4), the generated electric field will also be smaller, as displayed in Figure 2c and 2d. Therefore, collective electromagnetic effects in the boron plasma are not as significant as in the boron solid. Collective electromagnetic effects described in this paper are a kind of nonlinear effects caused by a large number of injected ions. Previously commonly used single-particle theories and simulation models cannot be used here. Collective electromagnetic effects depend on many factors, such as the current density of the proton beam, the resistivity of the boron target, and the flow velocity of plasma electrons.For the cases of the boron solid without electromagnetic fields (N-EB) and the boron plasma with electromagnetic fields (5N-EB), both degeneracy effects and collective electromagnetic effects are taken into account. The gap in the yields ofα particles between these two cases is about a tenth of a second, which is in good agreement with the results at dt = 1.2 ns in the experiments of Labaune et al. As we have discussed above separately, the gap here originates from two aspects: degeneracy effects and collective electromagnetic effects. They exert influences on the number of fusion reactions by changing the energy loss of the proton beam. To be specific, the more energy the proton beam losses during its transport in boron targets, the smaller the number of fusion reactions between protons and boron atomic nuclei will be. Readers may notice that the specific numbers of recorded α particles in our simulations are greater than those in the experiments. Actually, it is caused by the difference in the total number of injected protons between our simulations and their experiments. As shown in Eq. (10), the yield of α particles produced by the p 11 B fusion is proportional to the number of protons. If the total numbers of protons in our simulations is greater than that in the experiments, then there will be an equal multiple difference in the yields of α particles. In this work, we are concerned with the difference in the α-particle yields produced in different states of boron targets rather than the specific numbers. From this perspective, our simulations are indeed in good agreement with the experiments.Eventually, it should be mentioned that whileα particles produced by the p 11 B fusion are propagating in boron targets, they are simultaneously heated and being stopped by the background particles [45–47], which, as a matter of fact, will alter the initial energy spectrum of α particles. This indicates that degeneracy effects and collective electromagnetic effects influence not only the yield of α particles but also their energy spectrum or velocity distributions. Degeneracy effects can be considered to be isotropic if local fluctuations of the boron density and temperature are ignored, but it is not the case with collective electromagnetic effects. For the α particles moving forward (the opposite direction of the electric field), their energy loss will be increased, whereas for the α particles moving backward (the same direction as the electric field), they will be accelerated by the electric field and gain energy. Whether one tries to use the p 11 B fusion to obtain a net energy output to solve the energy crisis or view the p11 B fusion as α-particle source, the influences of degeneracy effects and collective electromagnetic effects on the energy evolution of α particles could be a topic worthy of in-depth study in future work.


## 5. Conclusion

The influences of the boron state on the yield ofα particles produced by the p 11 B fusion have been studied. It is found that compared with a boron solid, a boron plasma can produce much more α particles under the impact of a proton beam, which in this paper is proved to be attributed to degeneracy effects and collective electromagnetic effects. First, when a boron solid is ablated into a boron plasma by a nanosecond laser, degeneracy effects become non-negligible and can increase the yield of α particles by about 40%. Besides, a boron solid, as a poor conductor of electricity, has a large resistivity, while a boron plasma with abundant free electrons has a much lower resistivity. Ohm’s law (4) indicates that such a transition from boron solid to a boron plasma will lead to a reduction in the generation of electromagnetic fields. Simulation results show that the reduction of collective electromagnetic effects can significantly increase the yield of α particles by one to two orders of magnitude. Degeneracy effects and collective electromagnetic effects exert influences on the number of fusion reactions by changing the energy loss of the proton beam. To be specific, if the energy loss of the proton beam is decreased during its transporting in boron targets, the protons will have more chances to collide with boron nuclei, generate the p 11 B fusion, and produce α particles.Our results are in good agreement with the experiments of Labaune et al., and we believe that for future experiments of the p11 B fusion, a promising method to improve the yield of α particles is to heat and compress boron solid into a high-density plasma before injecting a proton beam, because in doing so, the energy loss of the proton beam will be reduced and, accordingly, more fusion reactions are expected to occur. Moreover, our findings may also be able to serve as a reference for investigating other beam-plasma systems, such as ion-driven inertial confinement fusions.



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