# Modeling and Analysis of Mechanical Properties of Aluminium Alloy (A413) Processed through Squeeze Casting Route Using Artificial Neural Network Model and Statistical Technique

Authors: R. Soundararajan; A. Ramesh; S. Sivasankaran; A. Sathishkumar
Journal: Advances in Materials Science and Engineering
 (2015)

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## Abstract

Artificial Neural Network (ANN) approach was used for predicting and analyzing the mechanical properties of A413 aluminum alloy produced by squeeze casting route. The experiments are carried out with different controlled input variables such as squeeze pressure, die preheating temperature, and melt temperature as per Full Factorial Design (FFD). The accounted absolute process variables produce a casting with pore-free and ideal fine grain dendritic structure resulting in good mechanical properties such as hardness, ultimate tensile strength, and yield strength. As a primary objective, a feed forward back propagation ANN model has been developed with different architectures for ensuring the definiteness of the values. The developed model along with its predicted data was in good agreement with the experimental data, inferring the valuable performance of the optimal model. From the work it was ascertained that, for castings produced by squeeze casting route, the ANN is an alternative method for predicting the mechanical properties and appropriate results can be estimated rather than measured, thereby reducing the testing time and cost. As a secondary objective, quantitative and statistical analysis was performed in order to evaluate the effect of process parameters on the mechanical properties of the castings.


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## Body

## 1. Introduction

The automobile industries are focusing their concentration on light weight vehicles due to market demand and governing regulations. Weight reduction in vehicles can be achieved by new engineering design and application of lightweight materials such as aluminium alloys and magnesium alloys. Among the lightweight materials a large amount of castings are made from Al-Si alloys. This alloy is one of the most popular alloys used in aerospace, automobile, marine, and mining industries due to excellent properties [1, 2].The silicon based aluminium alloy A413, which was chosen for this work, is associated with the theoretical density of 2.66 g/cm3. This alloy has been selected because of its good fluidity due to the presence of silicon content [1–5]. Also it is associated with excellent pressure tightness, good hot tear resistance, good castability, good machinability, high specific strength, and high corrosion resistance. Due to these properties, it finds use in numerous applications such as engine cylinder, piston, manifolds, and motor casings [6, 7]. The chemical composition of A413 aluminium alloy is represented in Table 1.Table 1
Chemical composition of A413 aluminium alloy in wt. %.
Cu
Mg
Si
Fe
Mn
Ni
Zn
Pb
Sn
Ti
Al
Standard
0.25 max
0.15 max
10.0–13.0
0.60 max
0.50 max
0.10 max
0.30 max
0.10 max
0.10 max
0.20 max
Reminder
Tested
0.1
0.1
11.81
0.56
0.5
0.1
0.1
0.1
0.05
0.1
ReminderMetal casting is the most economical route to produce metallic components in which the liquid metal is directly poured into the mould cavity of the required size and shape. The major drawback of casting processes is the formation of casting defects such as porosity, segregation, and hot tears [7, 8]. Further, the conventional casting processes cannot achieve the defect-free castings and desirable properties that satisfy the current demand.Squeeze casting is one of the modern casting techniques that respond best to the current demand. It is a hybrid metal casting/liquid-metal forging process, in which the molten metal solidifies under pressure within the closed die cavity, positioned between the plates of a hydraulic unit. The castings produced through squeeze casting route eliminate the defects with superior properties over the conventional castings due to fast heat transfer rate [9–11].To achieve a sound casting in squeeze casting route, the most dominant process parameter is level of applied pressure, although die preheating temperature, pouring temperature, and superheat are also important [9]. The die temperature is usually held between 200 and 300°C for aluminium alloy while the applied pressure varies between 70 and 210 MPa [12]. The process parameters in squeeze casting technique were studied and reported that the squeeze pressure and pouring temperature of 125 MPa and 700°C, respectively, gave good combination of hardness and tensile properties in Al-8% Si alloys having an aspect ratio not greater than 2.5 : 1 [13]. Squeeze pressure variation plays a major role in the formation of finer microstructure leading to good mechanical properties. Further, higher pressure decreases the percentage of porosity and increases the density of the cast alloy [14, 15]. Squeeze casting accounted for 15–40% improvement of mechanical properties than gravity die casting process [16]. The effect of applied pressure (1–75 MPa) on A413 Al-Si alloy was studied and reported that increasing the applied pressure results in increase of about 3.4% in density, 63% in UTS, 2.6% in percentage elongation, and 50% in hardness [17].In recent years, Artificial Neural Networks (ANNs) approach is one of the most powerful computing modeling facilities, based on statistical approach. This is currently being used in many fields of engineering for modeling complex relationships which are arduous to describe with physical models. Neural networks, as used in artificial intelligence, have traditionally been viewed as simplified models of neural processing in the human brain. The origins of neural networks are based on efforts to model information processing in biological systems, which may rely largely on parallel processing as well as implicit instructions based on recognition of patterns of “sensory” input from external sources. Artificial Neural Network (ANN) is a potent technique in the prediction of the properties and quite useful instead of time-consuming experimental processes and avoids costly manufacturing in analyzing the effects. To avoid cost incurred in manufacturing, ANN simulation model using Levenberg-Marquardt (LM) algorithm was developed and the performance in predictions was contemplated with experimentally measured values [18–21].Determination of the optimum squeeze cast process parameters of A413 aluminum alloy castings depending upon several factors and having subjected to many performance constraints is often complex and prolonged. This complexity could be made simple with the utilization of quantitative and statistical analysis, as the mechanical properties of the castings are dependent upon the relative process parameters. Several authors have optimized the squeeze casting process parameters for various Aluminum alloy grades using Taguchi method, Grey relational analysis, and genetic algorithm. It was reported that squeeze pressure, die preheating temperature, and melt temperature were found to be the major contributing factors on the mechanical properties of the castings and evaluated the optimal solutions for each factor [22–29]. Among all the available methods of Design of Experiments (DOE), Full Factorial Design (FFD) is a strong candidate in evaluating significant process parameters that can be employed to develop the casting process by evaluation of combined independent factors [30]. Analysis of Variance (ANOVA) is one of the proficient tools that allow the simultaneous study of the effects of all the input parameters and determines the significant parameters by carrying out a single analysis [30, 31].Antecedent research works annotated that the hardness, ultimate tensile strength, and yield strength of A413 Al alloy, processed by various casting processes, had exhibited considerable improvement in mechanical properties. Among several casting techniques, squeeze casting route shows better properties due to the application of various influenced process parameters. The process parameters vary with volume and shape (symmetrical/nonsymmetrical and aspect ratio) of the castings [13, 23–29] and also with different grades of aluminium alloy which are tabulated in Table 2. However, optimization of mechanical properties of A413 aluminium alloy (cylindrical castings of dia 50 mm and height 200 mm size) produced through squeeze casting route using FFD for varying squeeze pressure, die preheating temperature, and molten metal temperature modeled with artificial neural network had not been reported in the scientific community. The controlled and uncontrolled parameters during the process of experimentation may affect the truthfulness of the results. These discrepancies are sorted out by the usage of ANN, by means of modelling and predicting the responses. Also it is an attractive processing method since it is relatively inexpensive and offers a wide selection of input and output data conditions. This helps us in meeting with the botherations of time and cost. This work also focuses on the application of statistical technique to determine the precise influence of process parameters on the mechanical properties of the castings. The inquisition is enumerated and presented.Table 2
Comparison of antecedent research works.
Process
Metal/reinforcement
Input process parameters
UTS
Hardness
Reference
Pressure die casting
LM6 + 15 wt. %, size 44μm Al2O3
100 Mpa pressure 250  die temperature and 700 melt temperature
145 MPa
129 HBN
[9]
Squeeze casting
Al-8% Si
125 Mpa  pressure 250  die temperature and 700 pouring temperature
232 Mpa
58.0 HRF
[13]
Squeeze casting
2024 Al alloy
70 Mpa pressure 250  die temperature, and750 pouring temperature
<250 Mpa
—
[14]
Squeeze casting
7075 + SiC
10% Wt SiC, 70 TON pressure, 300 die temperature, and 780 pouring temperature
210 Mpa
138 VHN
[15]
Squeeze casting
AC2A-Ni coated SiC alloy
10% Wt SiC, 100 Mpa pressure, 250  die temperature, 725 melt temperature, and 45 sec pressure duration
402–419 Mpa
141–147 BHN
[23]
Squeeze casting
LM 24
106 Mpa pressure, 150  die temperature, 45 sec pressure duration, 750 melt temperature.
258 Mpa
93 BHN
[24]
Squeeze casting
AC2A alloy
100 Mpa pressure, 200  die temperature, 725 melt temperature, hot die steel die, and 45 sec pressure duration
328 Mpa
115 BHN
[27]
Squeeze casting
LM24
105.901 Mpa  pressure, 35.103  die temperature, pressure duration 15.124 sec, and 750 pouring temperature
272.258 Mpa
98.013 BHN
[29]


## 2. Experimental Technique

### 2.1. Materials and Methods

The metallic H13 die steel die was firmly seated over the 250 MPa (50 Ton) capacity hydraulic unit base plates. The punch was firmly fitted in a hydraulic unit to apply the required squeeze pressure. The preheater with maximum range of 500°C capacity has thermocouple arrangements to control the temperature of the die accurately. A bottom pouring red hot electric furnace (maximum range of 1200°C) with 2-liter capacity has been used to melt the metal. A preheated pathway unit with 400°C capacity is inbuilt in this setup. Standard hexachloroethylene (C2Cl6) degasser was used to remove the entrapped gases and other impurities/slag in the molten metal. The entire squeeze casting setup is shown in Figure 1.Figure 1
Squeeze casting setup.The experimentation was carried out by varying the influencing input parameters such as squeeze pressure, die preheating temperature, and melt temperature. The molten metal from the bottom pouring furnace was transferred into the preheated die through preheated pathway within few seconds, so as to avoid melt temperature loss and turbulence of molten metal flow.The squeeze pressure was applied on the molten metal by lowering the punch which is attached to the hydraulic unit with varying squeeze pressure (70, 105, and 140 MPa), die preheating temperatures (150°C, 225°C, and 300°C), and melt temperatures (650°C, 725°C, and 800°C) [12]. The compression loads were applied at a delay time of about five seconds after pouring molten metal and retained on the solidifying molten metal for a period of 60 seconds to produce sound castings (diameter 50 mm × height 200 mm). The castings were performed as per design of experiments (DOE) approach using L27 orthogonal array.


### 2.2. Full Factorial Design

The structure of the selected design of experiments should be such that the experimental investigation is completely factorial. This means that every possible combination between the levels of the various factors is analyzed. For the 33 full factorial design, squeeze pressure, die preheating temperature, and melt temperature were selected as factors and each was run at three levels as represented in Table 3. The 27 different combinations determined by Minitab 16 statistical software were evaluated. The preliminary investigation of the factors was performed to evaluate the effects of each parameter on the response by using P value and F test. The P value for each factor tests the null hypothesis that the coefficient is equal to zero (no effect). A low P value (<0.05) indicates that you can reject the null hypothesis; that is, the factor has a meaningful addition towards the response variable. Conversely, a larger (insignificant) P value suggests that the factor is not associated with changes in the response. The Analysis of Variance (ANOVA) was adopted for testing the significance of main effects on response [32–35].Table 3
Factors and their levels adopted for the 33 (L27) full factorial design used.
Factors
Level 1
Level 2
Level 3
Squeeze pressure (MPa)
70
105
140
Die preheating temperature (°C)
150
225
300
Molten metal temperature (°C)
650
725
800


### 2.3. Hardness Test and Tensile Test

Cast samples were machined to the testing conditions and for each type of test, three specimens were prepared. For Brinell hardness (BHN) test, 250 kg load for 10 to 15 seconds was applied through a ball indenter of 10 mm on the polished specimen surface and hardness values were measured in three spots of the cast specimen areas. Universal testing machine was employed for performing tensile test on the specimens. Three tensile test specimens were prepared as per the ASTM standard [36]. From the tensile test conducted, the UTS and yield strength readings for all the specimens were noted for each set. The average value is taken for further processing, it was shown in Table 4.Table 4
Assigned orthogonal L27 with the acquired data.
S. number
Squeeze pressure (MPa)
Die preheating temperature    (°C)
Melt temperature (°C)
Hardness (BHN)
UTS (MPa)
YS (MPa)
1
70
150
650
72
252
149
2
70
225
650
76
266
147
3
70
300
650
65
236
136
4
70
150
725
71
249
146
5
70
225
725
78
269
152
6
70
300
725
66
237
135
7
70
150
800
72
239
135
8
70
225
800
75
248
141
9
70
300
800
62
232
131
10
105
150
650
84
285
158
11
105
225
650
87
289
167
12
105
300
650
79
258
142
13
105
150
725
89
284
166
14
105
225
725
88
293
167
15
105
300
725
81
274
158
16
105
150
800
78
265
156
17
105
225
800
87
291
161
18
105
300
800
79
258
149
19
140
150
650
94
298
171
20
140
225
650
92
299
174
21
140
300
650
87
286
162
22
140
150
725
94
301
167
23
140
225
725
95
305
176
24
140
300
725
87
287
169
25
140
150
800
91
285
166
26
140
225
800
92
299
171
27
140
300
800
83
284
162


### 2.4. Microscopy

For microscopic examination, specimens of cast samples of 15 mm diameter and 10 mm thickness were first grinded through emery papers (320, 400, 600, 800, 1200, and 1500 grit emery papers) followed by polishing by 6-micrometer diamond paste. The samples were then etched with Keller’s reagent to obtain better contrast (2.5 mL HNO3, 1.5 mL HCl, 1.0 mL HF, and 95.0 mL Water) and dried by an electric drier. Well-formed grain boundaries were observed by a metallurgical microscope having 100x magnification. All the specimens were prepared and responses were tested as per ASTM Standard [36]. Cast samples and tested specimens are shown in Figures 2, 3(a), and 3(b).Figure 2
Cast samples made from squeeze casting process.Figure 3
Tested specimens (a) UTS and YS (b) hardness and microstructure.
(a)
(b)


### 2.5. Modeling of Process Variables

To ensure the definiteness of the experimental results an ANN model was developed with which all the responses were predicted. ANN with Back Propagation (BP) algorithm has been adopted in this model. There are several algorithms available among which the Levenberg-Marquardt algorithm (TRAINLM) will have the fastest convergence. This BP neural network is a multilayer of the network architecture including the input layer, the hidden layer(s), and the output layer. In the BP neural network, initially the weights of the outputs are calculated randomly. However, the outputs so calculated are compared with the actual/desired outputs by the network and the error is transmitted to the initial layer, which results in correction of the weights. The training iteration process may be terminated either by attaining a convergence limit or simply by limiting the total number of iterations [37–39]. Squeeze casting parameters such as squeeze pressure, die preheating temperature, and melt temperature were given as input parameters to ANN model. Mechanical properties such as hardness, ultimate tensile strength, and yield strength were given as output parameters. The input/output dataset of the model is illustrated schematically in Figure 4.Figure 4
ANN model.The networks consist of three layers: the input layer, the hidden layer, and the output layer. Now, the designed network has three input neurons and three output neurons. Then the problem of determining the optimal number of hidden neurons is a crucial one. The number of hidden neurons must be sufficiently large to realize a certain function. Several structures have to be considered with different numbers of hidden neurons to determine the best configuration [37–40].


#### 2.5.1. Designing, Training, and Testing of Neural Network

In ANN model, the three input parameters, namely, squeeze pressure, die preheating temperature, and melt temperature which has a major influence on mechanical properties of casting, and the output parameters were constrained to hardness, ultimate tensile strength, and yield strength. The data for training and testing have been taken from experiments conducted as per DOE. From the data of 27 experiments, 18 experiments (two-third) were selected for training and 9 experiments (one-third) were selected for testing. Both input dataset and output dataset were fed into neural network toolbox. Before training and testing the network, the input and output dataset were normalized to avoid suppressing. Three neurons corresponding to three inputs were fixed in input layer, three neurons corresponding to three outputs were fixed in output layer, and one/two neurons were fixed in hidden layer. After designing the network, selected training data of both input data and output data (18 dataset) was fed into the 3-1-3 ANN architecture initially. Then, the test input data (9-input data only) was fed into the same trained architecture and the performance was checked in terms of correlation coefficient and percentage of prediction error. Similarly the performance of other various architectures was checked in the same manner as shown in Table5 [37–41].Table 5
ANN architecture.
S. number
Architecture
Number of epochs
Performance: MSE
Correlation
Mean error
Test/entire data
H (BHN)
UTS (MPa)
YS   (MPa)
H   (BHN)
UTS (MPa)
YS (MPa)
1
3-1-3
19
0.0153
Test data
0.327603
−0.52923
0.2819692
6.4070304
0.6680727
9.931497
Entire data
−0.02037
0.017747
0.0346113
2
3-2-3
76
0.0168
Test data
0.94322
0.954007
0.9677214
−5.152297
−1.085981
−1.38332
Entire data
0.809566
0.809297
0.7972548
3
3-3-3
18
0.0125
Test data
0.780081
0.907185
0.7789159
−4.302875
1.2958169
−0.59547
Entire data
0.848023
0.857453
0.8640303
4
3-4-3
6
0.0118
Test data
0.934155
0.907692
0.9122967
−4.275792
−1.165425
−0.62814
Entire data
0.943153
0.908484
0.9054783
5
3-5-3
12
0.0158
Test data
0.839814
0.690353
0.7600678
−110.4625
5.5196954
−10.6531
Entire data
0.791315
0.807815
0.8151711
6
3-6-3
12
0.0143
Test data
0.390528
0.347113
0.345408
−8.036783
−3.622216
−4.14339
Entire data
0.604023
0.614535
0.6054474
7
3-7-3
8
0.016
Test data
0.953263
−0.01524
0.9097742
−4.071106
−3.822994
−0.46965
Entire data
0.87159
0.385303
0.8262986
8
3-8-3
14
0.0157
Test data
0.788937
0.913911
0.8342317
−6.298363
−4.394251
−2.46758
Entire data
0.754908
0.858456
0.8069087
9
3-9-3
14
0.0133
Test data
0.805992
0.760128
0.7849734
−2.171933
−0.727916
1.404604
Entire data
0.836876
0.575532
0.8616371
10
3-10-3
14
0.011
Test data
0.632409
0.420896
0.560555
−2.060248
2.5579382
1.594802
Entire data
0.649051
0.699587
0.6760219
11
3-11-3
12
0.0177
Test data
0.659561
0.584633
0.6891394
−4.41507
0.9423024
−0.76729
Entire data
0.742866
0.717644
0.6901495
12
3-12-3
6
0.0427
Test data
0.93661
0.955082
0.966098
−5.407939
−1.006904
−1.70824
Entire data
0.863574
0.903328
0.9145165
13
3-13-3
8
0.0189
Test data
0.861302
0.68761
0.8270757
−3.423997
0.1655911
0.209299
Entire data
0.80392
0.731365
0.8195485
14
3-14-3
10
0.0179
Test data
0.734746
0.479647
0.7634393
−3.981211
2.7269592
−0.32946
Entire data
0.599238
0.605336
0.5712369
15
3-15-3
13
0.00411
Test data
0.676342
0.953195
0.5946501
−5.790492
−1.623646
−2.05908
Entire data
0.747591
0.742622
0.6952719
16
3-16-3
10
0.0114
Test data
0.689947
0.867599
0.673677
−6.676086
−7.674145
−2.79686
Entire data
0.523877
0.417702
0.5356747
17
3-17-3
9
0.0209
Test data
0.156265
0.651166
0.1065115
−7.384365
5.5971769
−3.46927
Entire data
0.323953
0.505014
0.3186462
18
3-18-3
11
0.0984
Test data
0.403611
0.215978
0.249155
−5.303702
−2.487303
−1.50279
Entire data
0.698538
0.517436
0.7220452
19
3-19-3
8
0.0115
Test data
0.279565
0.964118
0.1682354
−3.403389
−1.713562
0.372705
Entire data
0.636981
0.907228
0.6774376
20
3-20-3
9
0.0101
Test data
0.80951
0.440466
0.7587061
−5.093201
0.2234417
−1.44388
Entire data
0.820222
0.680731
0.8224538
21
3-21-3
19
0.0153
Test data
0.82207
0.735911
0.7792016
−3.23522
−5.201905
0.376968
Entire data
0.779545
0.562689
0.7843417
22
3-22-3
19
0.0033
Test data
0.801136
0.921609
0.8114929
−7.751205
−2.592206
−3.94691
Entire data
0.826023
0.896124
0.8486225
23
3-23-3
19
0.0033
Test data
0.902197
0.669849
0.9400662
−6.302445
0.0397876
−2.65069
Entire data
0.815188
0.748771
0.8190763
24
3-24-3
7
0.0141
Test data
0.896778
0.918436
0.9329285
−4.152075
1.861485
−0.58482
Entire data
0.838781
0.752487
0.8235012
25
3-25-3
20
0.0177
Test data
0.810949
0.942861
0.770819
−4.811529
−1.148135
−1.06377
Entire data
0.714298
0.956582
0.7584142
26
3-26-3
8
0.0197
Test data
0.760178
0.912027
0.8164788
−4.569494
−3.024534
−0.95131
Entire data
0.774651
0.835861
0.7968075
27
3-27-3
6
0.0485
Test data
0.586688
0.954093
0.5396927
−0.729404
−3.985483
2.890374
Entire data
0.503455
0.889756
0.5307252
28
3-28-3
16
0.00141
Test data
0.88813
0.707645
0.9106447
−5.604047
−0.933052
−1.90122
Entire data
0.894371
0.802735
0.9359015
29
3-29-3
6
0.000397
Test data
0.507564
0.709963
0.45177
−5.865029
−1.351596
−2.10801
Entire data
0.7348
0.84627
0.7248776
30
3-30-3
6
0.0241
Test data
0.839443
0.792214
0.8946843
−7.977714
−0.504186
−4.21865
Entire data
0.752873
0.612031
0.7235352
31
3-31-3
7
0.0121
Test data
0.619047
−0.24167
0.5628295
2.3735194
−4.250233
5.776631
Entire data
0.685724
0.237457
0.6503848
32
3-32-3
12
0.00525
Test data
0.676626
0.547831
0.6692496
0.4171497
1.1120063
3.866985
Entire data
0.712427
0.738399
0.7062675
33
3-33-3
12
0.00777
Test data
0.903874
0.918511
0.9345398
−4.670028
−3.996412
−1.05047
Entire data
0.861108
0.822352
0.8848927
34
3-34-3
19
0.0281
Test data
0.365745
0.480003
0.421164
−8.402186
−3.453508
−4.62887
Entire data
0.622373
0.562207
0.5819972
35
3-35-3
6
0.00566
Test data
−0.70867
0.903043
−0.591856
−3.106763
0.4439772
0.795056
Entire data
0.097941
0.859707
0.1652056
36
3-38-3
6
0.0131
Test data
−0.59412
0.135391
−0.479609
−10.66344
4.3551262
−6.47462
Entire data
−0.35247
0.263477
−0.36004
37
3-1-1-3
28
0.0179
Test data
0.884277
0.910968
0.8426251
−4.867553
−0.956848
−1.04493
Entire data
0.667791
0.667375
0.6602249
38
3-2-2-3
18
0.0171
Test data
0.878881
0.893853
0.874913
−5.63957
−1.887107
−1.94438
Entire data
0.893016
0.899124
0.8916044
39
3-3-3-3
11
0.00861
Test data
0.85698
0.924045
0.8330365
−4.762418
−0.929011
−1.09533
Entire data
0.850919
0.889318
0.8531049
40
3-4-4-3
6
0.000236
Test data
0.936266
0.969176
0.9508616
−1.857168
−0.245293
−0.66882
Entire data
0.952932
0.978929
0.9696032Then the data were trained and tested as shown in the flow diagram of Figure5 and the percentage of error is calculated using the following formulae: (1)Percentageoferror%=ActualValue-PredictedValueActualValue∗100.Figure 5
Flow Diagram for training and testing of ANN model.Table6 shows the experimental and predicted results with the predicted error percentage. Similarly predictions were done and graphs were plotted as shown in Figures 6–8.Table 6
Experimental and ANN results of training and testing data.
S. number
Experimental results
ANN results
Predicted error
H
UTS
YS
H
UTS
YS
H
UTS
YS
Training set
1
72
252
149
74.17924
255.3464
150.7671
−3.02672
−1.32792
−1.18595
2
76
266
147
78.15725
255.9242
142.0319
−2.83849
3.787894
3.379629
3
65
236
136
70.89582
238.4725
135.2735
−9.07049
−1.04765
0.534189
4
71
249
146
71.6759
247.9369
147.3548
−0.95197
0.426944
−0.92793
5
78
269
152
81.66384
271.4753
153.9232
−4.69723
−0.92017
−1.26526
6
72
239
135
71.65555
240.363
139.2488
0.478404
−0.57029
−3.14725
7
75
248
141
75.12859
247.1022
141.6824
−0.17145
0.362011
−0.48396
8
87
289
167
85.63843
285.8119
164.3899
1.565027
1.103139
1.562942
9
79
258
142
78.52493
257.8554
143.3112
0.601349
0.056062
−0.92335
10
88
293
167
88.26898
291.553
167.574
−0.30566
0.493862
−0.34373
11
81
274
158
82.02498
274.0065
155.8774
−1.26541
−0.00239
1.343432
12
87
291
161
89.01555
286.0511
163.069
−2.31672
1.70066
−1.28508
13
79
258
149
78.54525
258.7912
148.6646
0.575627
−0.30668
0.225122
14
92
299
174
92.93316
300.7147
172.4506
−1.0143
−0.57348
0.89045
15
95
305
176
94.58353
304.0236
174.8126
0.438389
0.320127
0.674637
16
91
285
166
90.14581
286.8076
166.1176
0.938668
−0.63424
−0.07087
17
92
299
171
94.87449
304.6269
175.3976
−3.12444
−1.8819
−2.57167
18
83
284
162
84.7705
283.1482
163.473
−2.13314
0.299932
−0.90924
Testing set
19
66
237
135
72.33027
240.346
135.6869
−9.59132
−1.41181
−0.50878
20
62
232
131
60.56261
237.9408
135.5271
2.318365
−2.56069
−3.45579
21
84
285
158
92.38562
296.7993
170.5431
−9.98288
−4.14011
−7.93869
22
89
284
166
89.62359
286.8772
166.2851
−0.70067
−1.01309
−0.17177
23
78
265
156
77.80651
272.6354
158.4703
0.248062
−2.88128
−1.58353
24
94
298
171
93.83024
300.7667
172.6961
0.180592
−0.92844
−0.99188
25
87
286
162
83.94891
282.625
163.0893
3.507002
1.180066
−0.67239
26
94
301
167
91.36167
291.7642
168.4075
2.806739
3.068358
−0.84281
27
87
287
169
84.6408
284.7666
164.5869
2.71172
0.778174
2.611294
Correlation coefficient (R): for hardness R = 0.95, for UTS R=0.95, and for YS R=0.96.Figure 6
Actual versus ANN predicted results for hardness.Figure 7
Actual versus ANN predicted results for UTS.Figure 8
Actual versus ANN predicted results for YS.


## 2.1. Materials and Methods

The metallic H13 die steel die was firmly seated over the 250 MPa (50 Ton) capacity hydraulic unit base plates. The punch was firmly fitted in a hydraulic unit to apply the required squeeze pressure. The preheater with maximum range of 500°C capacity has thermocouple arrangements to control the temperature of the die accurately. A bottom pouring red hot electric furnace (maximum range of 1200°C) with 2-liter capacity has been used to melt the metal. A preheated pathway unit with 400°C capacity is inbuilt in this setup. Standard hexachloroethylene (C2Cl6) degasser was used to remove the entrapped gases and other impurities/slag in the molten metal. The entire squeeze casting setup is shown in Figure 1.Figure 1
Squeeze casting setup.The experimentation was carried out by varying the influencing input parameters such as squeeze pressure, die preheating temperature, and melt temperature. The molten metal from the bottom pouring furnace was transferred into the preheated die through preheated pathway within few seconds, so as to avoid melt temperature loss and turbulence of molten metal flow.The squeeze pressure was applied on the molten metal by lowering the punch which is attached to the hydraulic unit with varying squeeze pressure (70, 105, and 140 MPa), die preheating temperatures (150°C, 225°C, and 300°C), and melt temperatures (650°C, 725°C, and 800°C) [12]. The compression loads were applied at a delay time of about five seconds after pouring molten metal and retained on the solidifying molten metal for a period of 60 seconds to produce sound castings (diameter 50 mm × height 200 mm). The castings were performed as per design of experiments (DOE) approach using L27 orthogonal array.


## 2.2. Full Factorial Design

The structure of the selected design of experiments should be such that the experimental investigation is completely factorial. This means that every possible combination between the levels of the various factors is analyzed. For the 33 full factorial design, squeeze pressure, die preheating temperature, and melt temperature were selected as factors and each was run at three levels as represented in Table 3. The 27 different combinations determined by Minitab 16 statistical software were evaluated. The preliminary investigation of the factors was performed to evaluate the effects of each parameter on the response by using P value and F test. The P value for each factor tests the null hypothesis that the coefficient is equal to zero (no effect). A low P value (<0.05) indicates that you can reject the null hypothesis; that is, the factor has a meaningful addition towards the response variable. Conversely, a larger (insignificant) P value suggests that the factor is not associated with changes in the response. The Analysis of Variance (ANOVA) was adopted for testing the significance of main effects on response [32–35].Table 3
Factors and their levels adopted for the 33 (L27) full factorial design used.
Factors
Level 1
Level 2
Level 3
Squeeze pressure (MPa)
70
105
140
Die preheating temperature (°C)
150
225
300
Molten metal temperature (°C)
650
725
800


## 2.3. Hardness Test and Tensile Test

Cast samples were machined to the testing conditions and for each type of test, three specimens were prepared. For Brinell hardness (BHN) test, 250 kg load for 10 to 15 seconds was applied through a ball indenter of 10 mm on the polished specimen surface and hardness values were measured in three spots of the cast specimen areas. Universal testing machine was employed for performing tensile test on the specimens. Three tensile test specimens were prepared as per the ASTM standard [36]. From the tensile test conducted, the UTS and yield strength readings for all the specimens were noted for each set. The average value is taken for further processing, it was shown in Table 4.Table 4
Assigned orthogonal L27 with the acquired data.
S. number
Squeeze pressure (MPa)
Die preheating temperature    (°C)
Melt temperature (°C)
Hardness (BHN)
UTS (MPa)
YS (MPa)
1
70
150
650
72
252
149
2
70
225
650
76
266
147
3
70
300
650
65
236
136
4
70
150
725
71
249
146
5
70
225
725
78
269
152
6
70
300
725
66
237
135
7
70
150
800
72
239
135
8
70
225
800
75
248
141
9
70
300
800
62
232
131
10
105
150
650
84
285
158
11
105
225
650
87
289
167
12
105
300
650
79
258
142
13
105
150
725
89
284
166
14
105
225
725
88
293
167
15
105
300
725
81
274
158
16
105
150
800
78
265
156
17
105
225
800
87
291
161
18
105
300
800
79
258
149
19
140
150
650
94
298
171
20
140
225
650
92
299
174
21
140
300
650
87
286
162
22
140
150
725
94
301
167
23
140
225
725
95
305
176
24
140
300
725
87
287
169
25
140
150
800
91
285
166
26
140
225
800
92
299
171
27
140
300
800
83
284
162


## 2.4. Microscopy

For microscopic examination, specimens of cast samples of 15 mm diameter and 10 mm thickness were first grinded through emery papers (320, 400, 600, 800, 1200, and 1500 grit emery papers) followed by polishing by 6-micrometer diamond paste. The samples were then etched with Keller’s reagent to obtain better contrast (2.5 mL HNO3, 1.5 mL HCl, 1.0 mL HF, and 95.0 mL Water) and dried by an electric drier. Well-formed grain boundaries were observed by a metallurgical microscope having 100x magnification. All the specimens were prepared and responses were tested as per ASTM Standard [36]. Cast samples and tested specimens are shown in Figures 2, 3(a), and 3(b).Figure 2
Cast samples made from squeeze casting process.Figure 3
Tested specimens (a) UTS and YS (b) hardness and microstructure.
(a)
(b)


## 2.5. Modeling of Process Variables

To ensure the definiteness of the experimental results an ANN model was developed with which all the responses were predicted. ANN with Back Propagation (BP) algorithm has been adopted in this model. There are several algorithms available among which the Levenberg-Marquardt algorithm (TRAINLM) will have the fastest convergence. This BP neural network is a multilayer of the network architecture including the input layer, the hidden layer(s), and the output layer. In the BP neural network, initially the weights of the outputs are calculated randomly. However, the outputs so calculated are compared with the actual/desired outputs by the network and the error is transmitted to the initial layer, which results in correction of the weights. The training iteration process may be terminated either by attaining a convergence limit or simply by limiting the total number of iterations [37–39]. Squeeze casting parameters such as squeeze pressure, die preheating temperature, and melt temperature were given as input parameters to ANN model. Mechanical properties such as hardness, ultimate tensile strength, and yield strength were given as output parameters. The input/output dataset of the model is illustrated schematically in Figure 4.Figure 4
ANN model.The networks consist of three layers: the input layer, the hidden layer, and the output layer. Now, the designed network has three input neurons and three output neurons. Then the problem of determining the optimal number of hidden neurons is a crucial one. The number of hidden neurons must be sufficiently large to realize a certain function. Several structures have to be considered with different numbers of hidden neurons to determine the best configuration [37–40].


### 2.5.1. Designing, Training, and Testing of Neural Network

In ANN model, the three input parameters, namely, squeeze pressure, die preheating temperature, and melt temperature which has a major influence on mechanical properties of casting, and the output parameters were constrained to hardness, ultimate tensile strength, and yield strength. The data for training and testing have been taken from experiments conducted as per DOE. From the data of 27 experiments, 18 experiments (two-third) were selected for training and 9 experiments (one-third) were selected for testing. Both input dataset and output dataset were fed into neural network toolbox. Before training and testing the network, the input and output dataset were normalized to avoid suppressing. Three neurons corresponding to three inputs were fixed in input layer, three neurons corresponding to three outputs were fixed in output layer, and one/two neurons were fixed in hidden layer. After designing the network, selected training data of both input data and output data (18 dataset) was fed into the 3-1-3 ANN architecture initially. Then, the test input data (9-input data only) was fed into the same trained architecture and the performance was checked in terms of correlation coefficient and percentage of prediction error. Similarly the performance of other various architectures was checked in the same manner as shown in Table5 [37–41].Table 5
ANN architecture.
S. number
Architecture
Number of epochs
Performance: MSE
Correlation
Mean error
Test/entire data
H (BHN)
UTS (MPa)
YS   (MPa)
H   (BHN)
UTS (MPa)
YS (MPa)
1
3-1-3
19
0.0153
Test data
0.327603
−0.52923
0.2819692
6.4070304
0.6680727
9.931497
Entire data
−0.02037
0.017747
0.0346113
2
3-2-3
76
0.0168
Test data
0.94322
0.954007
0.9677214
−5.152297
−1.085981
−1.38332
Entire data
0.809566
0.809297
0.7972548
3
3-3-3
18
0.0125
Test data
0.780081
0.907185
0.7789159
−4.302875
1.2958169
−0.59547
Entire data
0.848023
0.857453
0.8640303
4
3-4-3
6
0.0118
Test data
0.934155
0.907692
0.9122967
−4.275792
−1.165425
−0.62814
Entire data
0.943153
0.908484
0.9054783
5
3-5-3
12
0.0158
Test data
0.839814
0.690353
0.7600678
−110.4625
5.5196954
−10.6531
Entire data
0.791315
0.807815
0.8151711
6
3-6-3
12
0.0143
Test data
0.390528
0.347113
0.345408
−8.036783
−3.622216
−4.14339
Entire data
0.604023
0.614535
0.6054474
7
3-7-3
8
0.016
Test data
0.953263
−0.01524
0.9097742
−4.071106
−3.822994
−0.46965
Entire data
0.87159
0.385303
0.8262986
8
3-8-3
14
0.0157
Test data
0.788937
0.913911
0.8342317
−6.298363
−4.394251
−2.46758
Entire data
0.754908
0.858456
0.8069087
9
3-9-3
14
0.0133
Test data
0.805992
0.760128
0.7849734
−2.171933
−0.727916
1.404604
Entire data
0.836876
0.575532
0.8616371
10
3-10-3
14
0.011
Test data
0.632409
0.420896
0.560555
−2.060248
2.5579382
1.594802
Entire data
0.649051
0.699587
0.6760219
11
3-11-3
12
0.0177
Test data
0.659561
0.584633
0.6891394
−4.41507
0.9423024
−0.76729
Entire data
0.742866
0.717644
0.6901495
12
3-12-3
6
0.0427
Test data
0.93661
0.955082
0.966098
−5.407939
−1.006904
−1.70824
Entire data
0.863574
0.903328
0.9145165
13
3-13-3
8
0.0189
Test data
0.861302
0.68761
0.8270757
−3.423997
0.1655911
0.209299
Entire data
0.80392
0.731365
0.8195485
14
3-14-3
10
0.0179
Test data
0.734746
0.479647
0.7634393
−3.981211
2.7269592
−0.32946
Entire data
0.599238
0.605336
0.5712369
15
3-15-3
13
0.00411
Test data
0.676342
0.953195
0.5946501
−5.790492
−1.623646
−2.05908
Entire data
0.747591
0.742622
0.6952719
16
3-16-3
10
0.0114
Test data
0.689947
0.867599
0.673677
−6.676086
−7.674145
−2.79686
Entire data
0.523877
0.417702
0.5356747
17
3-17-3
9
0.0209
Test data
0.156265
0.651166
0.1065115
−7.384365
5.5971769
−3.46927
Entire data
0.323953
0.505014
0.3186462
18
3-18-3
11
0.0984
Test data
0.403611
0.215978
0.249155
−5.303702
−2.487303
−1.50279
Entire data
0.698538
0.517436
0.7220452
19
3-19-3
8
0.0115
Test data
0.279565
0.964118
0.1682354
−3.403389
−1.713562
0.372705
Entire data
0.636981
0.907228
0.6774376
20
3-20-3
9
0.0101
Test data
0.80951
0.440466
0.7587061
−5.093201
0.2234417
−1.44388
Entire data
0.820222
0.680731
0.8224538
21
3-21-3
19
0.0153
Test data
0.82207
0.735911
0.7792016
−3.23522
−5.201905
0.376968
Entire data
0.779545
0.562689
0.7843417
22
3-22-3
19
0.0033
Test data
0.801136
0.921609
0.8114929
−7.751205
−2.592206
−3.94691
Entire data
0.826023
0.896124
0.8486225
23
3-23-3
19
0.0033
Test data
0.902197
0.669849
0.9400662
−6.302445
0.0397876
−2.65069
Entire data
0.815188
0.748771
0.8190763
24
3-24-3
7
0.0141
Test data
0.896778
0.918436
0.9329285
−4.152075
1.861485
−0.58482
Entire data
0.838781
0.752487
0.8235012
25
3-25-3
20
0.0177
Test data
0.810949
0.942861
0.770819
−4.811529
−1.148135
−1.06377
Entire data
0.714298
0.956582
0.7584142
26
3-26-3
8
0.0197
Test data
0.760178
0.912027
0.8164788
−4.569494
−3.024534
−0.95131
Entire data
0.774651
0.835861
0.7968075
27
3-27-3
6
0.0485
Test data
0.586688
0.954093
0.5396927
−0.729404
−3.985483
2.890374
Entire data
0.503455
0.889756
0.5307252
28
3-28-3
16
0.00141
Test data
0.88813
0.707645
0.9106447
−5.604047
−0.933052
−1.90122
Entire data
0.894371
0.802735
0.9359015
29
3-29-3
6
0.000397
Test data
0.507564
0.709963
0.45177
−5.865029
−1.351596
−2.10801
Entire data
0.7348
0.84627
0.7248776
30
3-30-3
6
0.0241
Test data
0.839443
0.792214
0.8946843
−7.977714
−0.504186
−4.21865
Entire data
0.752873
0.612031
0.7235352
31
3-31-3
7
0.0121
Test data
0.619047
−0.24167
0.5628295
2.3735194
−4.250233
5.776631
Entire data
0.685724
0.237457
0.6503848
32
3-32-3
12
0.00525
Test data
0.676626
0.547831
0.6692496
0.4171497
1.1120063
3.866985
Entire data
0.712427
0.738399
0.7062675
33
3-33-3
12
0.00777
Test data
0.903874
0.918511
0.9345398
−4.670028
−3.996412
−1.05047
Entire data
0.861108
0.822352
0.8848927
34
3-34-3
19
0.0281
Test data
0.365745
0.480003
0.421164
−8.402186
−3.453508
−4.62887
Entire data
0.622373
0.562207
0.5819972
35
3-35-3
6
0.00566
Test data
−0.70867
0.903043
−0.591856
−3.106763
0.4439772
0.795056
Entire data
0.097941
0.859707
0.1652056
36
3-38-3
6
0.0131
Test data
−0.59412
0.135391
−0.479609
−10.66344
4.3551262
−6.47462
Entire data
−0.35247
0.263477
−0.36004
37
3-1-1-3
28
0.0179
Test data
0.884277
0.910968
0.8426251
−4.867553
−0.956848
−1.04493
Entire data
0.667791
0.667375
0.6602249
38
3-2-2-3
18
0.0171
Test data
0.878881
0.893853
0.874913
−5.63957
−1.887107
−1.94438
Entire data
0.893016
0.899124
0.8916044
39
3-3-3-3
11
0.00861
Test data
0.85698
0.924045
0.8330365
−4.762418
−0.929011
−1.09533
Entire data
0.850919
0.889318
0.8531049
40
3-4-4-3
6
0.000236
Test data
0.936266
0.969176
0.9508616
−1.857168
−0.245293
−0.66882
Entire data
0.952932
0.978929
0.9696032Then the data were trained and tested as shown in the flow diagram of Figure5 and the percentage of error is calculated using the following formulae: (1)Percentageoferror%=ActualValue-PredictedValueActualValue∗100.Figure 5
Flow Diagram for training and testing of ANN model.Table6 shows the experimental and predicted results with the predicted error percentage. Similarly predictions were done and graphs were plotted as shown in Figures 6–8.Table 6
Experimental and ANN results of training and testing data.
S. number
Experimental results
ANN results
Predicted error
H
UTS
YS
H
UTS
YS
H
UTS
YS
Training set
1
72
252
149
74.17924
255.3464
150.7671
−3.02672
−1.32792
−1.18595
2
76
266
147
78.15725
255.9242
142.0319
−2.83849
3.787894
3.379629
3
65
236
136
70.89582
238.4725
135.2735
−9.07049
−1.04765
0.534189
4
71
249
146
71.6759
247.9369
147.3548
−0.95197
0.426944
−0.92793
5
78
269
152
81.66384
271.4753
153.9232
−4.69723
−0.92017
−1.26526
6
72
239
135
71.65555
240.363
139.2488
0.478404
−0.57029
−3.14725
7
75
248
141
75.12859
247.1022
141.6824
−0.17145
0.362011
−0.48396
8
87
289
167
85.63843
285.8119
164.3899
1.565027
1.103139
1.562942
9
79
258
142
78.52493
257.8554
143.3112
0.601349
0.056062
−0.92335
10
88
293
167
88.26898
291.553
167.574
−0.30566
0.493862
−0.34373
11
81
274
158
82.02498
274.0065
155.8774
−1.26541
−0.00239
1.343432
12
87
291
161
89.01555
286.0511
163.069
−2.31672
1.70066
−1.28508
13
79
258
149
78.54525
258.7912
148.6646
0.575627
−0.30668
0.225122
14
92
299
174
92.93316
300.7147
172.4506
−1.0143
−0.57348
0.89045
15
95
305
176
94.58353
304.0236
174.8126
0.438389
0.320127
0.674637
16
91
285
166
90.14581
286.8076
166.1176
0.938668
−0.63424
−0.07087
17
92
299
171
94.87449
304.6269
175.3976
−3.12444
−1.8819
−2.57167
18
83
284
162
84.7705
283.1482
163.473
−2.13314
0.299932
−0.90924
Testing set
19
66
237
135
72.33027
240.346
135.6869
−9.59132
−1.41181
−0.50878
20
62
232
131
60.56261
237.9408
135.5271
2.318365
−2.56069
−3.45579
21
84
285
158
92.38562
296.7993
170.5431
−9.98288
−4.14011
−7.93869
22
89
284
166
89.62359
286.8772
166.2851
−0.70067
−1.01309
−0.17177
23
78
265
156
77.80651
272.6354
158.4703
0.248062
−2.88128
−1.58353
24
94
298
171
93.83024
300.7667
172.6961
0.180592
−0.92844
−0.99188
25
87
286
162
83.94891
282.625
163.0893
3.507002
1.180066
−0.67239
26
94
301
167
91.36167
291.7642
168.4075
2.806739
3.068358
−0.84281
27
87
287
169
84.6408
284.7666
164.5869
2.71172
0.778174
2.611294
Correlation coefficient (R): for hardness R = 0.95, for UTS R=0.95, and for YS R=0.96.Figure 6
Actual versus ANN predicted results for hardness.Figure 7
Actual versus ANN predicted results for UTS.Figure 8
Actual versus ANN predicted results for YS.


## 2.5.1. Designing, Training, and Testing of Neural Network

In ANN model, the three input parameters, namely, squeeze pressure, die preheating temperature, and melt temperature which has a major influence on mechanical properties of casting, and the output parameters were constrained to hardness, ultimate tensile strength, and yield strength. The data for training and testing have been taken from experiments conducted as per DOE. From the data of 27 experiments, 18 experiments (two-third) were selected for training and 9 experiments (one-third) were selected for testing. Both input dataset and output dataset were fed into neural network toolbox. Before training and testing the network, the input and output dataset were normalized to avoid suppressing. Three neurons corresponding to three inputs were fixed in input layer, three neurons corresponding to three outputs were fixed in output layer, and one/two neurons were fixed in hidden layer. After designing the network, selected training data of both input data and output data (18 dataset) was fed into the 3-1-3 ANN architecture initially. Then, the test input data (9-input data only) was fed into the same trained architecture and the performance was checked in terms of correlation coefficient and percentage of prediction error. Similarly the performance of other various architectures was checked in the same manner as shown in Table5 [37–41].Table 5
ANN architecture.
S. number
Architecture
Number of epochs
Performance: MSE
Correlation
Mean error
Test/entire data
H (BHN)
UTS (MPa)
YS   (MPa)
H   (BHN)
UTS (MPa)
YS (MPa)
1
3-1-3
19
0.0153
Test data
0.327603
−0.52923
0.2819692
6.4070304
0.6680727
9.931497
Entire data
−0.02037
0.017747
0.0346113
2
3-2-3
76
0.0168
Test data
0.94322
0.954007
0.9677214
−5.152297
−1.085981
−1.38332
Entire data
0.809566
0.809297
0.7972548
3
3-3-3
18
0.0125
Test data
0.780081
0.907185
0.7789159
−4.302875
1.2958169
−0.59547
Entire data
0.848023
0.857453
0.8640303
4
3-4-3
6
0.0118
Test data
0.934155
0.907692
0.9122967
−4.275792
−1.165425
−0.62814
Entire data
0.943153
0.908484
0.9054783
5
3-5-3
12
0.0158
Test data
0.839814
0.690353
0.7600678
−110.4625
5.5196954
−10.6531
Entire data
0.791315
0.807815
0.8151711
6
3-6-3
12
0.0143
Test data
0.390528
0.347113
0.345408
−8.036783
−3.622216
−4.14339
Entire data
0.604023
0.614535
0.6054474
7
3-7-3
8
0.016
Test data
0.953263
−0.01524
0.9097742
−4.071106
−3.822994
−0.46965
Entire data
0.87159
0.385303
0.8262986
8
3-8-3
14
0.0157
Test data
0.788937
0.913911
0.8342317
−6.298363
−4.394251
−2.46758
Entire data
0.754908
0.858456
0.8069087
9
3-9-3
14
0.0133
Test data
0.805992
0.760128
0.7849734
−2.171933
−0.727916
1.404604
Entire data
0.836876
0.575532
0.8616371
10
3-10-3
14
0.011
Test data
0.632409
0.420896
0.560555
−2.060248
2.5579382
1.594802
Entire data
0.649051
0.699587
0.6760219
11
3-11-3
12
0.0177
Test data
0.659561
0.584633
0.6891394
−4.41507
0.9423024
−0.76729
Entire data
0.742866
0.717644
0.6901495
12
3-12-3
6
0.0427
Test data
0.93661
0.955082
0.966098
−5.407939
−1.006904
−1.70824
Entire data
0.863574
0.903328
0.9145165
13
3-13-3
8
0.0189
Test data
0.861302
0.68761
0.8270757
−3.423997
0.1655911
0.209299
Entire data
0.80392
0.731365
0.8195485
14
3-14-3
10
0.0179
Test data
0.734746
0.479647
0.7634393
−3.981211
2.7269592
−0.32946
Entire data
0.599238
0.605336
0.5712369
15
3-15-3
13
0.00411
Test data
0.676342
0.953195
0.5946501
−5.790492
−1.623646
−2.05908
Entire data
0.747591
0.742622
0.6952719
16
3-16-3
10
0.0114
Test data
0.689947
0.867599
0.673677
−6.676086
−7.674145
−2.79686
Entire data
0.523877
0.417702
0.5356747
17
3-17-3
9
0.0209
Test data
0.156265
0.651166
0.1065115
−7.384365
5.5971769
−3.46927
Entire data
0.323953
0.505014
0.3186462
18
3-18-3
11
0.0984
Test data
0.403611
0.215978
0.249155
−5.303702
−2.487303
−1.50279
Entire data
0.698538
0.517436
0.7220452
19
3-19-3
8
0.0115
Test data
0.279565
0.964118
0.1682354
−3.403389
−1.713562
0.372705
Entire data
0.636981
0.907228
0.6774376
20
3-20-3
9
0.0101
Test data
0.80951
0.440466
0.7587061
−5.093201
0.2234417
−1.44388
Entire data
0.820222
0.680731
0.8224538
21
3-21-3
19
0.0153
Test data
0.82207
0.735911
0.7792016
−3.23522
−5.201905
0.376968
Entire data
0.779545
0.562689
0.7843417
22
3-22-3
19
0.0033
Test data
0.801136
0.921609
0.8114929
−7.751205
−2.592206
−3.94691
Entire data
0.826023
0.896124
0.8486225
23
3-23-3
19
0.0033
Test data
0.902197
0.669849
0.9400662
−6.302445
0.0397876
−2.65069
Entire data
0.815188
0.748771
0.8190763
24
3-24-3
7
0.0141
Test data
0.896778
0.918436
0.9329285
−4.152075
1.861485
−0.58482
Entire data
0.838781
0.752487
0.8235012
25
3-25-3
20
0.0177
Test data
0.810949
0.942861
0.770819
−4.811529
−1.148135
−1.06377
Entire data
0.714298
0.956582
0.7584142
26
3-26-3
8
0.0197
Test data
0.760178
0.912027
0.8164788
−4.569494
−3.024534
−0.95131
Entire data
0.774651
0.835861
0.7968075
27
3-27-3
6
0.0485
Test data
0.586688
0.954093
0.5396927
−0.729404
−3.985483
2.890374
Entire data
0.503455
0.889756
0.5307252
28
3-28-3
16
0.00141
Test data
0.88813
0.707645
0.9106447
−5.604047
−0.933052
−1.90122
Entire data
0.894371
0.802735
0.9359015
29
3-29-3
6
0.000397
Test data
0.507564
0.709963
0.45177
−5.865029
−1.351596
−2.10801
Entire data
0.7348
0.84627
0.7248776
30
3-30-3
6
0.0241
Test data
0.839443
0.792214
0.8946843
−7.977714
−0.504186
−4.21865
Entire data
0.752873
0.612031
0.7235352
31
3-31-3
7
0.0121
Test data
0.619047
−0.24167
0.5628295
2.3735194
−4.250233
5.776631
Entire data
0.685724
0.237457
0.6503848
32
3-32-3
12
0.00525
Test data
0.676626
0.547831
0.6692496
0.4171497
1.1120063
3.866985
Entire data
0.712427
0.738399
0.7062675
33
3-33-3
12
0.00777
Test data
0.903874
0.918511
0.9345398
−4.670028
−3.996412
−1.05047
Entire data
0.861108
0.822352
0.8848927
34
3-34-3
19
0.0281
Test data
0.365745
0.480003
0.421164
−8.402186
−3.453508
−4.62887
Entire data
0.622373
0.562207
0.5819972
35
3-35-3
6
0.00566
Test data
−0.70867
0.903043
−0.591856
−3.106763
0.4439772
0.795056
Entire data
0.097941
0.859707
0.1652056
36
3-38-3
6
0.0131
Test data
−0.59412
0.135391
−0.479609
−10.66344
4.3551262
−6.47462
Entire data
−0.35247
0.263477
−0.36004
37
3-1-1-3
28
0.0179
Test data
0.884277
0.910968
0.8426251
−4.867553
−0.956848
−1.04493
Entire data
0.667791
0.667375
0.6602249
38
3-2-2-3
18
0.0171
Test data
0.878881
0.893853
0.874913
−5.63957
−1.887107
−1.94438
Entire data
0.893016
0.899124
0.8916044
39
3-3-3-3
11
0.00861
Test data
0.85698
0.924045
0.8330365
−4.762418
−0.929011
−1.09533
Entire data
0.850919
0.889318
0.8531049
40
3-4-4-3
6
0.000236
Test data
0.936266
0.969176
0.9508616
−1.857168
−0.245293
−0.66882
Entire data
0.952932
0.978929
0.9696032Then the data were trained and tested as shown in the flow diagram of Figure5 and the percentage of error is calculated using the following formulae: (1)Percentageoferror%=ActualValue-PredictedValueActualValue∗100.Figure 5
Flow Diagram for training and testing of ANN model.Table6 shows the experimental and predicted results with the predicted error percentage. Similarly predictions were done and graphs were plotted as shown in Figures 6–8.Table 6
Experimental and ANN results of training and testing data.
S. number
Experimental results
ANN results
Predicted error
H
UTS
YS
H
UTS
YS
H
UTS
YS
Training set
1
72
252
149
74.17924
255.3464
150.7671
−3.02672
−1.32792
−1.18595
2
76
266
147
78.15725
255.9242
142.0319
−2.83849
3.787894
3.379629
3
65
236
136
70.89582
238.4725
135.2735
−9.07049
−1.04765
0.534189
4
71
249
146
71.6759
247.9369
147.3548
−0.95197
0.426944
−0.92793
5
78
269
152
81.66384
271.4753
153.9232
−4.69723
−0.92017
−1.26526
6
72
239
135
71.65555
240.363
139.2488
0.478404
−0.57029
−3.14725
7
75
248
141
75.12859
247.1022
141.6824
−0.17145
0.362011
−0.48396
8
87
289
167
85.63843
285.8119
164.3899
1.565027
1.103139
1.562942
9
79
258
142
78.52493
257.8554
143.3112
0.601349
0.056062
−0.92335
10
88
293
167
88.26898
291.553
167.574
−0.30566
0.493862
−0.34373
11
81
274
158
82.02498
274.0065
155.8774
−1.26541
−0.00239
1.343432
12
87
291
161
89.01555
286.0511
163.069
−2.31672
1.70066
−1.28508
13
79
258
149
78.54525
258.7912
148.6646
0.575627
−0.30668
0.225122
14
92
299
174
92.93316
300.7147
172.4506
−1.0143
−0.57348
0.89045
15
95
305
176
94.58353
304.0236
174.8126
0.438389
0.320127
0.674637
16
91
285
166
90.14581
286.8076
166.1176
0.938668
−0.63424
−0.07087
17
92
299
171
94.87449
304.6269
175.3976
−3.12444
−1.8819
−2.57167
18
83
284
162
84.7705
283.1482
163.473
−2.13314
0.299932
−0.90924
Testing set
19
66
237
135
72.33027
240.346
135.6869
−9.59132
−1.41181
−0.50878
20
62
232
131
60.56261
237.9408
135.5271
2.318365
−2.56069
−3.45579
21
84
285
158
92.38562
296.7993
170.5431
−9.98288
−4.14011
−7.93869
22
89
284
166
89.62359
286.8772
166.2851
−0.70067
−1.01309
−0.17177
23
78
265
156
77.80651
272.6354
158.4703
0.248062
−2.88128
−1.58353
24
94
298
171
93.83024
300.7667
172.6961
0.180592
−0.92844
−0.99188
25
87
286
162
83.94891
282.625
163.0893
3.507002
1.180066
−0.67239
26
94
301
167
91.36167
291.7642
168.4075
2.806739
3.068358
−0.84281
27
87
287
169
84.6408
284.7666
164.5869
2.71172
0.778174
2.611294
Correlation coefficient (R): for hardness R = 0.95, for UTS R=0.95, and for YS R=0.96.Figure 6
Actual versus ANN predicted results for hardness.Figure 7
Actual versus ANN predicted results for UTS.Figure 8
Actual versus ANN predicted results for YS.


## 3. Results and Discussions

The main objective of the present work is to study, predict, and analyze the mechanical properties (hardness, ultimate tensile strength, and yield strength) of squeeze casting process parameters of A413 aluminium alloy castings using BP neural network and statistical analysis.


### 3.1. Performance Measurement of Neural Network for Experimental Data

In order to determine the optimal architecture, 40 different networks with different numbers of layers and neurons in the hidden layer have been designed and tested for castings. The performance capabilities of each network are examined based on the correlation coefficient between the network predictions and the experimental values using the test and the entire dataset. It is concluded that the selection of optimum architecture depends on maximum error %, minimum error %, mean error %, and the correlation coefficient. From Tables5 and 6, it is identified that the networks with two hidden layers and four neurons in each layer (3-4-4-3) produced the best performance for each of the output parameters. It was observed that the correlation coefficient was above 0.95 for architecture (3-4-4-3) which has high level of accuracy for prediction. It is also observed that the mean correlation coefficient for the architecture (3-4-4-3) is 0.96615 which is better than the previous architectures. Hence, further, the average percentage error (0.92376) was also less than ±3% which means the ANN predicted results were very much closer to the experimental (actual) results shown in Figures 6–8. It reveals that the prediction of ANN model was found to be in good agreement with experimental data.Therefore, the selected 3-4-4-3 ANN architecture model can be used for predicting the mechanical properties of A413 Al alloy castings processed within the input parameters of squeeze pressure, die preheating temperature, and melt temperature. The process variables that lead to the cast component with the desired properties can be interpolated with the help of the optimal model. This is well suited for aluminum metal casting industries where the real-time experimental runs can be reduced to a greater extent which leads to time and cost saving [38].


### 3.2. Influence of Process Variables on Mechanical Properties

The influential parameters were squeeze pressure, die preheating temperature, melt temperature, pressure holding time, and die material. Among them the first three parameters were taken as variables and other two parameters were taken as fixed ones. The effect of each variable parameter is discussed as follows. The results obtained showed scientific influence of each parameter on the response.


#### 3.2.1. Effect of Squeeze Pressure on Mechanical Properties

The scientific theory for obtaining better results at the maximum squeeze pressure is as follows. During the solidification of casting process, an air gap is formed between the metal and mould interface which is found to have a major influence on the mechanical properties of casting [11]. The air gap reduces the value of heat transfer coefficient in the interface, resulting in prolonged solidification time that leads to formation of microporosity in the castings. In squeeze casting process, the applied squeeze pressure reduces the air gap and decreases the solidification time [27–29].It also reveals that the maximum squeeze pressure increases the metal mold contact which accelerates the solidification process leading to formation of fine dendritic structure of the castings as compared to lower pressure levels. Fine dendritic structure results in high hardness, UTS, and yield strength [11–14, 27–29].Figures9–14 show the effect of squeeze pressure under different levels such as 70, 105, and 140 MPa. By varying the die preheating temperature as 150°C, 225°C, and 300°C and melt temperature 650°C, 725°C, and 800°C, it is observed that the maximum results were obtained for the maximum squeeze pressure of 140 MPa. Coarse and fine dendritic structure is formed when the sample solidified under 70 MPa and 105 MPa. When the applied squeeze pressure increased to 140 MPa, ideal fine dendritic structure is obtained for this volume and shape of the castings. Further increase of applied pressure has no significant effect on the dendritic structure [11–13].Figure 9
Main effect plots for hardness.Figure 10
Main effect plots for UTS.Figure 11
Main effect plots for YS.Figure 12
Contour plot for hardness versus die preheating temp and pressure.Figure 13
Contour plot for UTS versus die preheating temperature and pressure.Figure 14
Contour plot for YS versus die preheating temperature and pressure.


#### 3.2.2. Effect of Die Preheating Temperature

The scientific theory for obtaining better results at a preheating temperature is as follows. Initially before the pouring of molten metal, the die preheating helps to evaporate the entrapped air/gases in the die cavity. After pouring, the preheating of the die affects the rate of heat transfer as it increases the solidification time. The die preheating temperature range depends upon the material, volume, and the shape of the casting which may result in defect-free sound casting in a quality acceptable range.To investigate the effect of varying die preheating temperature, squeeze pressure and melt temperature were fixed since the die preheating temperature is an important parameter which affects the heat transfer rates and consequently the cooling properties of the castings in this process. With higher the die preheating temperature results in delay of solidification time which in turn leads to formation of coarse dendritic structure and reduces the die life, causing hot spots and shrinkage pores. Whereas lower the die pre heating temperature leads to thermal failures in the dies, cold laps on the surface of the castings and air entrapped in the casting resulting in defective casting [10–13].Figures9–14 show the effect of different die preheating temperature (150°C, 225°C, and 300°C), squeeze pressure (70, 105, and 140 MPa), and the melt temperature (650°C, 725°C, and 800°C). By maintaining different levels of squeeze pressure and melt temperature, it is observed that the better results were obtained for a die preheating temperature of 225°C for this volume and shape of the castings.


#### 3.2.3. Effect of Melt Temperature

The scientific theory for obtaining better results at a melt temperature is as follows. Higher the melt temperature leads to formation of coarse dendritic structure due to delay in solidification time whereas lower the melt temperature leads to premature solidification in the castings. However, it must offer sufficient heat to avert premature solidification of the metals before the applied pressure. A suitable pouring temperature is dependent on several factors, such as the liquidus temperature, freezing range of the metal, and die complexity. Pouring temperature between 700 and 750°C plays an important role to change the grain structure evolution tendency with the applied pressure. When the pouring temperature is lower than the critical value, the applied pressure can obviously refine grains. On the contrary, when the pouring temperature is higher than the critical value, the applied pressure leads to the grain structure coarsening slightly [12].Figures9–14 show the effect of different melt temperatures (650°C, 725°C, and 800°C), die preheating temperatures (150°C, 225°C, and 300°C), and squeeze pressure (70, 105, and 140 MPa). By maintaining different levels of die preheating temperature and squeeze pressure, it is observed that the better results were obtained for a melt temperature of 725°C for this volume and shape of castings [27–29].


### 3.3. Statistical Analysis

In order to determine the significance of each parameter that has involved in the process, an Analysis of Variance (ANOVA) was performed based on values of response (hardness, UTS, and yield strength), as shown in Tables7–9. The determination coefficient (R2) value indicates the goodness of fits of the model [33–35]. In this case, the value of the mean determination coefficient (R2=93.096%) and the value of the mean adjusted determination coefficient (adjusted R2=91.023%) are high, which indicates a high significance of the model. It is evident that the squeeze pressure has a strong influence on mechanical properties contribution of about (70–78)% followed by die preheating temperature (15%–18%) and melt temperature. The results show that all three parameters including squeeze pressure, die preheating temperature, and melt temperature are effective in mechanical properties because their P values are lower than 0.005. The main effects plot from Figures 9–11 reveals the effect of each process parameter on the mechanical properties of the castings. The mechanical properties increase drastically to the midlevel and then increase gradually due to applied squeeze pressure. This is because the dendritic structures are coarse and fine due to increase in applied pressure from 70 MPa to 105 MPa and further increase in pressure up to 140 MPa causes a negligible increase in mechanical properties due to ideal fine dendritic structure.Table 7
Analysis of variance for hardness using adjusted SS for tests.
Source
DF
Seq SS
Adj SS
Adj MS
F
P
Pressure
2
1792.89
1792.89
896.44
182.12
0.000
Die preheating temperature
2
354.67
354.67
177.33
36.03
0.000
Melt temperature
2
50.67
50.67
25.33
5.15
0.016
Error
20
98.44
98.44
4.92
Total
26
2296.67
S = 2.21861, R-Sq. = 95.71%, and R-Sq.(adj.) = 94.43%.Table 8
Analysis of variance for UTS using adjusted SS for tests.
Source
DF
Seq. SS
Adj. SS
Adj. MS
F
P
Pressure
2
8978.7
8978.7
4489.3
87.02
0.000
Die preheating temperature
2
2393.6
2393.6
1196.8
23.20
0.000
Melt temperature
2
362.0
362.0
181.0
3.51
0.049
Error
20
1031.8
1031.8
51.6
Total
26
12766.0
S = 7.18254,  R-Sq. = 91.92%, and R-Sq.(adj.) = 89.49%.Table 9
Analysis of variance for YS, using adjusted SS for tests.
Source
DF
Seq SS
Adj SS
Adj MS
F
P
Pressure
2
2926.89
2926.89
1463.44
85.58
0.000
Die preheating temperature
2
693.56
693.56
346.78
20.28
0.000
Melt temperature
2
136.22
136.22
68.11
3.98
0.035
Error
20
342.00
342.00
17.10
Total
26
4098.67
S = 4.13521, and R-Sq. = 91.66%, and R-Sq.(adj.) = 89.15%.In case of die preheating temperature and melt temperature it increases gradually to the midlevel and then decreases drastically to the higher level. This is because the lower die temperature (150°C) and melt temperature (650°C) cause casting defects and premature solidification resulting in lower mechanical properties whereas higher die preheating temperature (300°C) and melt temperature (800°C) cause solidification delay resulting in coarse dendritic structure which leads to loss in mechanical properties of the castings. The graphical model developed using the contour plot determines the effect of independent variables (squeeze pressure and die preheating temperature) on the dependent variables (hardness, UTS, and yield strength) as shown in Figures12–14. The dark green region in the contour plot indicates that higher mechanical properties are obtained due to the increase in squeeze pressure and optimal level of die preheating temperature. The blue region in the contour plot indicates the lower mechanical properties [27–29].


### 3.4. Effect of Process Parameters on Microstructure

Figures15(a)–15(c) show the microstructures of the A413 alloy solidified under different squeeze pressures, which accelerate the formation of dendritic structure of the castings and it was studied through metallurgical microscope. Quantitative metallographic analysis shows that microporosity and other defects are eliminated significantly with the increase in applied squeeze pressure. The microstructure of the cast samples consists of white regions of (α-Al) alpha aluminium dendritic structure in the black regions of (α-Al + Si) eutectic matrix.Figure 15
Microstructure at squeeze casting process: (a) 70 MPa, (b) 105 MPa, and (c) 140 MPa of squeeze pressure (die preheated temperature and melt temperature are 225°C and 725°C which are fixed) at 100x magnification.
(a)
(b)
(c)The dendritic branches act as the load carrying member in the matrix. By the refinement of dendritic branches there is a significant improvement in the mechanical properties of the castings. The cast sample of A413 aluminum alloy at squeeze pressure 140 MPa with die preheating temperature of 225°C and melt temperature of 725°C reveals an ideal fine dendritic structure and shows superior mechanical properties than others. The coarse and fine dendritic structure was formed in the cases of 70 and 105 MPa squeeze pressure with the die preheated temperature and melt temperature of 225°C and 725°C, respectively.


## 3.1. Performance Measurement of Neural Network for Experimental Data

In order to determine the optimal architecture, 40 different networks with different numbers of layers and neurons in the hidden layer have been designed and tested for castings. The performance capabilities of each network are examined based on the correlation coefficient between the network predictions and the experimental values using the test and the entire dataset. It is concluded that the selection of optimum architecture depends on maximum error %, minimum error %, mean error %, and the correlation coefficient. From Tables5 and 6, it is identified that the networks with two hidden layers and four neurons in each layer (3-4-4-3) produced the best performance for each of the output parameters. It was observed that the correlation coefficient was above 0.95 for architecture (3-4-4-3) which has high level of accuracy for prediction. It is also observed that the mean correlation coefficient for the architecture (3-4-4-3) is 0.96615 which is better than the previous architectures. Hence, further, the average percentage error (0.92376) was also less than ±3% which means the ANN predicted results were very much closer to the experimental (actual) results shown in Figures 6–8. It reveals that the prediction of ANN model was found to be in good agreement with experimental data.Therefore, the selected 3-4-4-3 ANN architecture model can be used for predicting the mechanical properties of A413 Al alloy castings processed within the input parameters of squeeze pressure, die preheating temperature, and melt temperature. The process variables that lead to the cast component with the desired properties can be interpolated with the help of the optimal model. This is well suited for aluminum metal casting industries where the real-time experimental runs can be reduced to a greater extent which leads to time and cost saving [38].


## 3.2. Influence of Process Variables on Mechanical Properties

The influential parameters were squeeze pressure, die preheating temperature, melt temperature, pressure holding time, and die material. Among them the first three parameters were taken as variables and other two parameters were taken as fixed ones. The effect of each variable parameter is discussed as follows. The results obtained showed scientific influence of each parameter on the response.


### 3.2.1. Effect of Squeeze Pressure on Mechanical Properties

The scientific theory for obtaining better results at the maximum squeeze pressure is as follows. During the solidification of casting process, an air gap is formed between the metal and mould interface which is found to have a major influence on the mechanical properties of casting [11]. The air gap reduces the value of heat transfer coefficient in the interface, resulting in prolonged solidification time that leads to formation of microporosity in the castings. In squeeze casting process, the applied squeeze pressure reduces the air gap and decreases the solidification time [27–29].It also reveals that the maximum squeeze pressure increases the metal mold contact which accelerates the solidification process leading to formation of fine dendritic structure of the castings as compared to lower pressure levels. Fine dendritic structure results in high hardness, UTS, and yield strength [11–14, 27–29].Figures9–14 show the effect of squeeze pressure under different levels such as 70, 105, and 140 MPa. By varying the die preheating temperature as 150°C, 225°C, and 300°C and melt temperature 650°C, 725°C, and 800°C, it is observed that the maximum results were obtained for the maximum squeeze pressure of 140 MPa. Coarse and fine dendritic structure is formed when the sample solidified under 70 MPa and 105 MPa. When the applied squeeze pressure increased to 140 MPa, ideal fine dendritic structure is obtained for this volume and shape of the castings. Further increase of applied pressure has no significant effect on the dendritic structure [11–13].Figure 9
Main effect plots for hardness.Figure 10
Main effect plots for UTS.Figure 11
Main effect plots for YS.Figure 12
Contour plot for hardness versus die preheating temp and pressure.Figure 13
Contour plot for UTS versus die preheating temperature and pressure.Figure 14
Contour plot for YS versus die preheating temperature and pressure.


### 3.2.2. Effect of Die Preheating Temperature

The scientific theory for obtaining better results at a preheating temperature is as follows. Initially before the pouring of molten metal, the die preheating helps to evaporate the entrapped air/gases in the die cavity. After pouring, the preheating of the die affects the rate of heat transfer as it increases the solidification time. The die preheating temperature range depends upon the material, volume, and the shape of the casting which may result in defect-free sound casting in a quality acceptable range.To investigate the effect of varying die preheating temperature, squeeze pressure and melt temperature were fixed since the die preheating temperature is an important parameter which affects the heat transfer rates and consequently the cooling properties of the castings in this process. With higher the die preheating temperature results in delay of solidification time which in turn leads to formation of coarse dendritic structure and reduces the die life, causing hot spots and shrinkage pores. Whereas lower the die pre heating temperature leads to thermal failures in the dies, cold laps on the surface of the castings and air entrapped in the casting resulting in defective casting [10–13].Figures9–14 show the effect of different die preheating temperature (150°C, 225°C, and 300°C), squeeze pressure (70, 105, and 140 MPa), and the melt temperature (650°C, 725°C, and 800°C). By maintaining different levels of squeeze pressure and melt temperature, it is observed that the better results were obtained for a die preheating temperature of 225°C for this volume and shape of the castings.


### 3.2.3. Effect of Melt Temperature

The scientific theory for obtaining better results at a melt temperature is as follows. Higher the melt temperature leads to formation of coarse dendritic structure due to delay in solidification time whereas lower the melt temperature leads to premature solidification in the castings. However, it must offer sufficient heat to avert premature solidification of the metals before the applied pressure. A suitable pouring temperature is dependent on several factors, such as the liquidus temperature, freezing range of the metal, and die complexity. Pouring temperature between 700 and 750°C plays an important role to change the grain structure evolution tendency with the applied pressure. When the pouring temperature is lower than the critical value, the applied pressure can obviously refine grains. On the contrary, when the pouring temperature is higher than the critical value, the applied pressure leads to the grain structure coarsening slightly [12].Figures9–14 show the effect of different melt temperatures (650°C, 725°C, and 800°C), die preheating temperatures (150°C, 225°C, and 300°C), and squeeze pressure (70, 105, and 140 MPa). By maintaining different levels of die preheating temperature and squeeze pressure, it is observed that the better results were obtained for a melt temperature of 725°C for this volume and shape of castings [27–29].


## 3.2.1. Effect of Squeeze Pressure on Mechanical Properties

The scientific theory for obtaining better results at the maximum squeeze pressure is as follows. During the solidification of casting process, an air gap is formed between the metal and mould interface which is found to have a major influence on the mechanical properties of casting [11]. The air gap reduces the value of heat transfer coefficient in the interface, resulting in prolonged solidification time that leads to formation of microporosity in the castings. In squeeze casting process, the applied squeeze pressure reduces the air gap and decreases the solidification time [27–29].It also reveals that the maximum squeeze pressure increases the metal mold contact which accelerates the solidification process leading to formation of fine dendritic structure of the castings as compared to lower pressure levels. Fine dendritic structure results in high hardness, UTS, and yield strength [11–14, 27–29].Figures9–14 show the effect of squeeze pressure under different levels such as 70, 105, and 140 MPa. By varying the die preheating temperature as 150°C, 225°C, and 300°C and melt temperature 650°C, 725°C, and 800°C, it is observed that the maximum results were obtained for the maximum squeeze pressure of 140 MPa. Coarse and fine dendritic structure is formed when the sample solidified under 70 MPa and 105 MPa. When the applied squeeze pressure increased to 140 MPa, ideal fine dendritic structure is obtained for this volume and shape of the castings. Further increase of applied pressure has no significant effect on the dendritic structure [11–13].Figure 9
Main effect plots for hardness.Figure 10
Main effect plots for UTS.Figure 11
Main effect plots for YS.Figure 12
Contour plot for hardness versus die preheating temp and pressure.Figure 13
Contour plot for UTS versus die preheating temperature and pressure.Figure 14
Contour plot for YS versus die preheating temperature and pressure.


## 3.2.2. Effect of Die Preheating Temperature

The scientific theory for obtaining better results at a preheating temperature is as follows. Initially before the pouring of molten metal, the die preheating helps to evaporate the entrapped air/gases in the die cavity. After pouring, the preheating of the die affects the rate of heat transfer as it increases the solidification time. The die preheating temperature range depends upon the material, volume, and the shape of the casting which may result in defect-free sound casting in a quality acceptable range.To investigate the effect of varying die preheating temperature, squeeze pressure and melt temperature were fixed since the die preheating temperature is an important parameter which affects the heat transfer rates and consequently the cooling properties of the castings in this process. With higher the die preheating temperature results in delay of solidification time which in turn leads to formation of coarse dendritic structure and reduces the die life, causing hot spots and shrinkage pores. Whereas lower the die pre heating temperature leads to thermal failures in the dies, cold laps on the surface of the castings and air entrapped in the casting resulting in defective casting [10–13].Figures9–14 show the effect of different die preheating temperature (150°C, 225°C, and 300°C), squeeze pressure (70, 105, and 140 MPa), and the melt temperature (650°C, 725°C, and 800°C). By maintaining different levels of squeeze pressure and melt temperature, it is observed that the better results were obtained for a die preheating temperature of 225°C for this volume and shape of the castings.


## 3.2.3. Effect of Melt Temperature

The scientific theory for obtaining better results at a melt temperature is as follows. Higher the melt temperature leads to formation of coarse dendritic structure due to delay in solidification time whereas lower the melt temperature leads to premature solidification in the castings. However, it must offer sufficient heat to avert premature solidification of the metals before the applied pressure. A suitable pouring temperature is dependent on several factors, such as the liquidus temperature, freezing range of the metal, and die complexity. Pouring temperature between 700 and 750°C plays an important role to change the grain structure evolution tendency with the applied pressure. When the pouring temperature is lower than the critical value, the applied pressure can obviously refine grains. On the contrary, when the pouring temperature is higher than the critical value, the applied pressure leads to the grain structure coarsening slightly [12].Figures9–14 show the effect of different melt temperatures (650°C, 725°C, and 800°C), die preheating temperatures (150°C, 225°C, and 300°C), and squeeze pressure (70, 105, and 140 MPa). By maintaining different levels of die preheating temperature and squeeze pressure, it is observed that the better results were obtained for a melt temperature of 725°C for this volume and shape of castings [27–29].


## 3.3. Statistical Analysis

In order to determine the significance of each parameter that has involved in the process, an Analysis of Variance (ANOVA) was performed based on values of response (hardness, UTS, and yield strength), as shown in Tables7–9. The determination coefficient (R2) value indicates the goodness of fits of the model [33–35]. In this case, the value of the mean determination coefficient (R2=93.096%) and the value of the mean adjusted determination coefficient (adjusted R2=91.023%) are high, which indicates a high significance of the model. It is evident that the squeeze pressure has a strong influence on mechanical properties contribution of about (70–78)% followed by die preheating temperature (15%–18%) and melt temperature. The results show that all three parameters including squeeze pressure, die preheating temperature, and melt temperature are effective in mechanical properties because their P values are lower than 0.005. The main effects plot from Figures 9–11 reveals the effect of each process parameter on the mechanical properties of the castings. The mechanical properties increase drastically to the midlevel and then increase gradually due to applied squeeze pressure. This is because the dendritic structures are coarse and fine due to increase in applied pressure from 70 MPa to 105 MPa and further increase in pressure up to 140 MPa causes a negligible increase in mechanical properties due to ideal fine dendritic structure.Table 7
Analysis of variance for hardness using adjusted SS for tests.
Source
DF
Seq SS
Adj SS
Adj MS
F
P
Pressure
2
1792.89
1792.89
896.44
182.12
0.000
Die preheating temperature
2
354.67
354.67
177.33
36.03
0.000
Melt temperature
2
50.67
50.67
25.33
5.15
0.016
Error
20
98.44
98.44
4.92
Total
26
2296.67
S = 2.21861, R-Sq. = 95.71%, and R-Sq.(adj.) = 94.43%.Table 8
Analysis of variance for UTS using adjusted SS for tests.
Source
DF
Seq. SS
Adj. SS
Adj. MS
F
P
Pressure
2
8978.7
8978.7
4489.3
87.02
0.000
Die preheating temperature
2
2393.6
2393.6
1196.8
23.20
0.000
Melt temperature
2
362.0
362.0
181.0
3.51
0.049
Error
20
1031.8
1031.8
51.6
Total
26
12766.0
S = 7.18254,  R-Sq. = 91.92%, and R-Sq.(adj.) = 89.49%.Table 9
Analysis of variance for YS, using adjusted SS for tests.
Source
DF
Seq SS
Adj SS
Adj MS
F
P
Pressure
2
2926.89
2926.89
1463.44
85.58
0.000
Die preheating temperature
2
693.56
693.56
346.78
20.28
0.000
Melt temperature
2
136.22
136.22
68.11
3.98
0.035
Error
20
342.00
342.00
17.10
Total
26
4098.67
S = 4.13521, and R-Sq. = 91.66%, and R-Sq.(adj.) = 89.15%.In case of die preheating temperature and melt temperature it increases gradually to the midlevel and then decreases drastically to the higher level. This is because the lower die temperature (150°C) and melt temperature (650°C) cause casting defects and premature solidification resulting in lower mechanical properties whereas higher die preheating temperature (300°C) and melt temperature (800°C) cause solidification delay resulting in coarse dendritic structure which leads to loss in mechanical properties of the castings. The graphical model developed using the contour plot determines the effect of independent variables (squeeze pressure and die preheating temperature) on the dependent variables (hardness, UTS, and yield strength) as shown in Figures12–14. The dark green region in the contour plot indicates that higher mechanical properties are obtained due to the increase in squeeze pressure and optimal level of die preheating temperature. The blue region in the contour plot indicates the lower mechanical properties [27–29].


## 3.4. Effect of Process Parameters on Microstructure

Figures15(a)–15(c) show the microstructures of the A413 alloy solidified under different squeeze pressures, which accelerate the formation of dendritic structure of the castings and it was studied through metallurgical microscope. Quantitative metallographic analysis shows that microporosity and other defects are eliminated significantly with the increase in applied squeeze pressure. The microstructure of the cast samples consists of white regions of (α-Al) alpha aluminium dendritic structure in the black regions of (α-Al + Si) eutectic matrix.Figure 15
Microstructure at squeeze casting process: (a) 70 MPa, (b) 105 MPa, and (c) 140 MPa of squeeze pressure (die preheated temperature and melt temperature are 225°C and 725°C which are fixed) at 100x magnification.
(a)
(b)
(c)The dendritic branches act as the load carrying member in the matrix. By the refinement of dendritic branches there is a significant improvement in the mechanical properties of the castings. The cast sample of A413 aluminum alloy at squeeze pressure 140 MPa with die preheating temperature of 225°C and melt temperature of 725°C reveals an ideal fine dendritic structure and shows superior mechanical properties than others. The coarse and fine dendritic structure was formed in the cases of 70 and 105 MPa squeeze pressure with the die preheated temperature and melt temperature of 225°C and 725°C, respectively.


## 4. Conclusion

A413 aluminum alloy castings with different levels of squeeze pressure, die preheating temperature, and melt temperature were successfully fabricated by squeeze casting route. The influential variables and responses were systematically investigated as per full factorial design. Moreover the use of ANN to predict and ensure the experimental dataset and statistical tool to optimize the process variables were explored in this study. 40 different backpropagation neural network architectures are trained and tested based upon the correlation coefficient and mean error percentage, using the experimental data until an optimum architecture is identified. The following conclusions are evident from this experimental work.(i)
Based on the number architectures that are used to train the ANN model using BP algorithm, the architecture (3-4-4-3) was in good agreement to that of the experimental values with the mean correlation coefficient of 0.96615 and mean error percentage of 0.92376.(ii)
The developed model can provide beneficial data that can be predicted from the wide range of experimental database. Therefore time consuming experiments can be reduced and hence considerable savings in terms of cost and time could be obtained by using developed neural network model which serves as a boon for metal casting industry.(iii)
The results from the statistical tool reveal that optimal level of process variables for obtaining maximum mechanical behaviour (hardness, UTS, and yield strength) are as folllows:squeeze pressure: 140 MPa,die preheating temperature: 225°C,melt temperature: 725°C.(iv)
From the ANOVA analysis, the most significant parameters were identified as squeeze pressure and die preheating temperature with percentage contribution of (70–78)% and (15–18)%, respectively, withR-Sq. value of 93.09%.



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*Source: 714762-2015-08-05.xml*