# Intense ү-Ray Bursts following the Interaction of Laser Pulse with Steep Density Gradients

Authors: S. Chintalwad; S. Krishnamurthy; S. Morris; B. Ramakrishna
Journal: Laser and Particle Beams
 (2022)

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## Abstract

We investigate the production of intense ү-rays following the interaction of ultraintense laser pulse with a hybrid combination of under-dense plasma associated with a thin foil of fully ionized Al or Cu or Au at the rear side. Relativistic electrons are accelerated following the interaction of high intensity laser pulses with an under-dense plasma. These electrons are then stopped by the thin foils attached to the rear side of the under-dense plasma. This results in the production of intense-ray bursts. So, the enhancement of photon generation is due to the under-dense plasma electrons interacting with different over-dense plasma. Using open-source PIC code EPOCH, we study the effect of different electron densities in the under-plasma on photon emission. Photon emission enhancement is observed by increasing the targetZ in the hybrid structure. Hybrid structure can enhance photon emission; it can increase the photon energy and yield and improve photon beam divergence. Simulations were also performed to find the optimal under-dense plasma density for ү-ray production.


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## Body

## 1. Introduction

Recent developments in laser intensities of the order of 1022 to 1023 Wcm−2 are possible due to the production of femto-second pulses by the introduction of the Chirped Pulse Amplification (CPA) technique [1]. The increase in laser intensity [2] has advanced the fields related to science and technology. In particular, the laser-plasma interaction has been the frontier of research with regard to accelerator physics [3], radiography [4], radiation therapy [5], and laboratory astrophysics [6]. Relativistic electrons are accelerated to MeV energies with the currently available intense laser systems. The nonlinear processes [7] associated with these relativistic electrons lead to radiation ranging from X-rays to ү-rays. High-energy X-rays are employed for very high-resolution imaging such as Thomson scattering and high-energy sources. The bright ү-ray sources are also useful in nuclear physics related to waste management and in the production of ү-ү colliders. [8], which are of fundamental importance to the science community. Besides using proton bunches generated from the ion acceleration in the inertial confinement fusion (ICF) application [9–11], the bremsstrahlung radiation generated from laser wake field acceleration (LWFA) could also be used in ICF [12, 13]. Edward et al. [14] used laser-accelerated electrons in solid targets and under-dense plasma (gas-jet) to produce a highly collimated, high-flux beam. Radiography of complex and dense materials using ү-sources was demonstrated by Glinec et al. in 2005 [15]. However, such sources could not be employed in practical applications due to poor control of beam parameters such as divergence and energy controlling the beam quality must be improved. Such a compact ү-ray source can be used in industrial applications such as detector calibration and testing.PET (positron emission tomography) is a radioisotope-based imaging technology used in cancer diagnosis [16]. Proton beams from conventional accelerators, such as LINAC, are generally used to produce radio isotopes. However, radioisotopes can also be produced by photo-nuclear processes arising from ү-ray irradiation. LWFA is a promising path for ү-ray-based radioisotope production which has emerged from current technology. This method uses compact tabletop lasers over high-end particle accelerators which are inexpensive and accessible. Radioisotope activation with the ү-rays produced by the bremsstrahlung of LWFA electrons have been demonstrated by various experiments [17–19]. For practical applications, it is crucial to achieve the desired beam features such as the source size, divergence, and electron-photon conversion efficiency. Using conventional accelerators in the low-energy range, analysis of bremsstrahlung sources for target material and thickness was performed by Marzini et al. [20], and LWFA-based bremsstrahlung sources are a key advancement for laser plasma-based particle sources which can be used for various applications. On the other hand, the Direct Laser Acceleration (DLA) mechanism accelerates electrons by laser electromagnetic waves in the ion channel or the plasma bubble through betatron resonance. In (DLA), the electrons in the ion channel or the plasma bubble are imparted with much higher energy than in vacuum [21]. The (DLA) regime is also very attractive due to a wide variety of potential practical applications such as the production of the MeV range of ultrarelativistic electrons that can serve as compact X-ray radiation sources [22]. Apart from this, the (DLA) regime is also useful in novel sources of other energetic particles such as ions [23], neutrons [24], and positrons [25].Recent studies have shown that the ү-rays produced by laser-driven bremsstrahlung [26–28] and Compton scattering or Thomson scattering [29–32] which are based on laser-wake field accelerators [33–36] can produce highly collimated and quasimonochromatic ү-rays. Bremsstrahlung is produced when a charged particle is stopped by the strong electric fields inside the atomic nuclei. When a laser interacts with a plasma, the emitted photon energy is determined by the laser’s intensity, as well as target parameters such as thickness, atomic number, and the cross section of electron interaction with an atomic nucleus. The interaction of a high-intensity laser pulse with a target is divided into two steps: first, the laser-plasma interaction produces MeV electrons [37–39], and then, in a high Z solid target, the process of the production of bremsstrahlung when a high intensity laser pulse interacts with matter is basically due to the production of MeV electrons by laser and subsequent quenching of these electrons in the strong field of the atomic nuclei. The interaction cross section to produce bremsstrahlung radiation is increased with increase in Z of the target [40]. The processes involving the atomic nucleus, such as bremsstrahlung e−+Z⟶e−+γ+Z, play an important role in the production of plasmas with a high charge state or/and large atomic number Z. The interaction of a high-energy electron bunch with a high-Z target such as copper or gold is where bremsstrahlung radiation would be most important. With the help of high laser intensities, the bremsstrahlung may produce comparable amounts of ү-ray radiation. Laser Wake-Field Acceleration (LWFA) [41] or (DLA) mechanisms can accelerate electrons in under-dense plasma. In a double-layer interaction setup [42, 43], firstly, a high-intense laser pulse interacts with the under-dense plasma and accelerates hot electrons in the under-dense region by LWFA or DLA [44, 45], and then these accelerated electrons are stopped by the nuclear potential of the foil target placed at the rear side of the under-dense region. Higher electron energy leads to more efficient ү-ray emission as the bremsstrahlung cross section increases with electron energy [46, 47]. In plasma, the bremsstrahlung emission is strongly dependent on the interaction cross section between the incoming electron and the nuclear potential of the target. Furthermore, the cross section depends on the Z of the target. The cross section (σb) is proportional to αre2Z2 where α=e2/ℏc=1/137 is the fine structure constant and re=e2/mc2 is the classical electron radius, respectively. The interaction cross section increases with increasing the Z of the target. For the Al (Z = 13) target, interaction cross section has σb≈169αre2, for Cu target (Z = 29), it is around σb≈841αre2, and for the Au target (Z = 79), cross section will be σb≈6241αre2 [48, 49].In this paper, we investigate the photon emission by the bremsstrahlung mechanism; we use the open-source particle-in-cell (PIC) code EPOCH [50] for this study. The bremsstrahlung mechanism is studied using the Monte Carlo (MC) algorithm, which is already included in the EPOCH code [46]. We study the relative strength of the bremsstrahlung radiation for various densities of the under-dense plasma. When an ultra-intense laser with an intensity I=4×1021Wcm−2 is used to irradiate the under-dense plasma with the density of 0.02nc to 2nc, by attaching fully ionized targets such as Al or Au or Cu to the rear side of the under-dense plasma, the effect of the rear side target electron density on the emission of ү-rays is discussed in detail.


## 2. Simulation Set-Up

The simulations were performed with the 2D PIC code EPOCH. The simulation box covers (0μm to 50 μm) along the x-direction and (−10 μm to 10 μm) along the y-direction with 5000 × 2000 cells with a cell size of 10 nm along the x-direction and y-direction. The under-dense hydrogen plasma with an electron density of (0.02nc to 2nc) is placed at 1 μm to 41 μm with 40 μm thickness. Electrons and ions have 32 macroparticles per cell. A P-polarized laser pulse of wavelength 0.8 μm with a focal spot radius of 1 μm is used. The peak intensity is 4×1021Wcm−2 with a pulse duration of FWHM 30 fs. The laser pulse has a Gaussian spatial and temporal profile. The laser pulse enters the simulation box from x = 0 μm left boundary at the start of the simulation (t = 0), Al, or Cu, or Au with a thickness of 1 μm attached to the rear side of the under-dense plasma has been considered as a fully ionized plasma with the electron density ne = 455nc for Al, ne = 2238nc for Cu, and ne = 4234.4nc for Au where nc is electron critical density nc=ε0meω02/4πe2 with laser frequency ω0=2πc/λ0 where ε0, me, e,andλ are permittivity of free space, the mass of an electron, electron charge, and laser wavelength, respectively. The critical density corresponding to the laser wavelength λ  = 0.8 μm is nc=1.71×1021cm−3. Only photons with energies greater than 50 keV are considered in all simulations. For computational convenience and in order to look into only the high-energy photons, we have considered only those photons with energy above 50 keV. The interaction set-up for double layer simulation is shown in Figure 1.Figure 1
Simulation interaction set-up.


## 3. Results and Discussions

To study the photon emission in this double layer interaction setup, firstly, the interaction of a laser pulse with a 40μm thick under-dense hydrogen plasma containing electrons and protons with a density of 0.2nc is considered. The interaction of ultraintense laser pulses with various under-dense plasma densities is then compared. The simulation results showing the electron density in under-dense plasma and corresponding electric field are presented in Figures 2(a) and 2(b). When an ultraintense laser pulse interacts with under-dense plasma, the laser pulse propagates through the plasma with minimal energy loss. As shown in Figure 2(a), the bubble regime is not formed sufficiently for the LWFA of the electron acceleration scheme. Figure 2(b) shows the corresponding transverse electric field in the under-dense plasma. When the laser pulse penetrates the plasma, the ponderomotive force causes electrons to be expelled sideways. Ions form a positively charged sheath behind the laser pulse because they are not expelled as quickly as electrons. The electrons are then pulled back towards the laser axis by the electrostatic field created.Figure 2
(a) Electron density distribution in under-dense plasma for 0.2nc (b) corresponding transverse electric field, (c) electron energy, and (d) photon energy spectrum for 0.2nc.
(a)(b)(c)(d)The electron and photon energy spectra are shown in Figures2(c) and 2(d). In the electron energy spectrum, the purple line indicates the electron energy in the under-dense plasma when the laser pulse approaches the end of the under-dense plasma, and the electron energy is higher in under-dense plasma than after interacting with the rear foil. The electron energy in the under-dense target is 189 MeV. The corresponding electron energy values for Al, Cu, and Au are 85 Mev, 75 MeV, and 80 MeV, respectively. Only when these high-energy electrons from the under-dense plasma interact with the rear foil attached to the under-dense target can photon emission be enhanced. Figure 2(d) shows the photon energy for all three foils; the obtained maximum photon energy values for Al, Cu, and Au are 61.3 MeV, 116 MeV, and 149.6 MeV, respectively. The highest photon energy is found in the case of the Au target. As increasing the Z of the target, the bremsstrahlung emission increases due to the increase in the interaction cross section between the electron and the ion. The photon number from the bremsstrahlung mechanism is shown in Figure 3.Figure 3
Photon number (above) and angular distribution of photons (below) for 0.2nc.The comparison of photon numbers generated from Al, Cu, or Au indicate that the number generated by Al is smaller than that generated by Cu and Au. The emitted photon number is found to be around 4 × 109, 4.2 × 1012, and 4.5 × 1013 for Al, Cu, and Au, respectively. The results indicate a maximum bremsstrahlung photon energy and the photon numbers for higher Z (Au). The simulation time is restricted to 300 fs, but the photon emission is expected to happen at a longer time scale. In addition, the angular distribution of photons is depicted in Figure 3. In Al target, the focused photon number along the θ = 0° is higher compared to Cu and Au. In case of Cu and Au, the emitted photons are mostly perpendicular to the laser direction, at about θ = ±90°. This transverse emission has also been observed by Morris, S. et al. [46]. But in the case of the Au target, the emitted photons along the transverse directions are one order of magnitude higher than the Cu target. The photon emission direction is longitudinal for Al, and in the case of Cu or Au, the photons are emitted along the transverse direction.We have performed additional simulations to understand the role of a higher under-dense plasma density and its corresponding effect on the emission of photons. We performed simulations by setting the density of the first layer ranging from 0.02nc to 2nc keeping all simulation parameters similar except for the under-dense plasma density. Figures 4(a) and 4(b) show the electron density and electric field for the ne = 2nc. Due to the self-focusing effect, the laser pulse gains a smaller transverse profile and a higher peak intensity; the electrons in the under-dense plasma are highly focused compared to the ne = 0.2nc. The laser pulse loses its significant energy within the under-dense region for higher plasma density and less amount of the high energy electron bunch gets reflected by the foil leading to reduced photon emission. The corresponding electron and photon energy spectra are shown in Figures 4(c) and 4(d). In the electron energy spectrum, the electron energy in the under-dense plasma is taken just before interacting with the foil in both the cases 0.2nc and 2nc. The electron energy in the under-dense target is 135 MeV, and electron energy for Al, Cu, and Au is 58 MeV, 65 MeV, and 68 MeV, respectively. The photon energy is higher in the Au case than in the Al and Cu cases. The corresponding photon energy for Al, Cu, and Au is 29.1 MeV, 55.3 MeV, and 81.3 MeV, respectively.Figure 4
(a) Electron density distribution in under-dense plasma for 2nc (b) corresponding transverse electric field, (c) electron energy, and (d) photon energy spectrum for 2nc.
(a)(b)(c)(d)In addition, we also looked into the photon number and distribution of the photons in different targets in Figure5. The emitted photon number is found to be around 1.4 × 108, 4 × 1012, and 4.3 × 1013 for Al, Cu, and Au, respectively. The generated photon number by the Al target is smaller than the Cu and Au targets. The maximum photon energy and the corresponding photons emitted are relatively higher for Au. In addition, we also depict the angular distribution of photons. In the Al target, the focused photons are relatively high compared to Cu and Au. But in the case of the Au target, the photons are comparatively higher than the Cu target. For a given laser pulse, the photon yield and energy can be affected by the parameters of under-dense plasma density. We performed a series of PIC simulations by varying the under-dense plasma density to obtain the optimal density for the highest photon yield and corresponding energy. Here, we changed the density of the under-dense plasma, but the length of the under-dense plasma is fixed to 40 μm. The results shown in Figure 6 are the photon energy dependence on different densities in all three targets. The photon number and energy decrease with increasing under-dense plasma density. The optimal density is found to be ne = 0.2nc. At this density, the number and energy of the photons are high compared to other densities. If the length and density of an under-dense plasma are too small, the resulting electron energy and number are limited. When under-dense plasma is too long and too dense, filamentation may occur, and thus, the laser absorption efficiency will be reduced in hydrogen layers with a higher density. Both are disadvantageous to the generation of high-energy photons.Figure 5
Photon number (above) and angular distribution of photons (below) for 2nc.Figure 6
The photon energy dependency on different densities in under-dense plasma.


## 4. Conclusion

A hybrid double-layer setup has been studied via 2D EPOCH simulations for the gamma ray production following the interaction of high intensity (I = 4 × 1021 Wcm−2) short-pulse laser. The results confirm photon energy enhancement for Au (high Z) target with the interaction of MeV electrons driven by the laser pulse interacting with the under-dense plasma in the hybrid structure. MeV electrons are accelerated in the under-dense region through well-known laser-plasma mechanisms such as LWFA and DLA. In conclusion, our simulations suggest an improved photon beam divergence and conversion efficiency of laser energy to photons if a high Z layer is present in the hybrid target. This study will be of fundamental importance for various applications in high-intensity laser-plasma interactions.



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