A method of producing a member for electrophotography comprising an electro-conductive support, an elastic layer, and a surface layer, the method comprising: a step of hydrolyzing and condensing a hydrolyzable silane compound represented by the following general formula and a chelate titanium compound represented by the following general formula to obtain a surface-layer coating liquid; a first step of forming, on a surface of the elastic layer, a coat of a surface-layer coating liquid containing the hydrolyzed condensate of the hydrolyzable silane compound represented by the following general formula and the chelate titanium compound represented by the following general formula; and a second step of crosslinking the hydrolyzed condensate in the coat through cleavage of an epoxy group in the hydrolyzed condensate to form the surface layer: [Chem. 1] General formula R 1 -Si (OR 2) (OR 3) (OR 4) in the general formula, R 1 represents a hydrocarbon group represented by any one of the following general formulae to, and R 2 to R 4 each independently represent a hydrocarbon group; in the general formula, R 5 and R 6 each independently represent a linear or branched alkyl group having 1 or more and 20 or less carbon atoms, and R 7 to R 10 each independently represent a hydrogen atom, an alkyl group having 1 or more and 3 or less carbon atoms, or an alkoxy group having 1 or more and 3 or less carbon atoms; in the general formulae to: R 11 to R 13, R 16 to R 18, R 23, R 24, R 29, and R 30 each independently represent a hydrogen atom, an alkyl group having 1 or more and 4 or less carbon atoms, a hydroxyl group, a carboxyl group, or an amino group; R 14, R 15, R 19 to R 22, R 27, R 28, and R 33 to R 36 each independently represent a hydrogen atom or an alkyl group having 1 or more and 4 or less carbon atoms; R 25, R 26, R 31, and R 32 each independently represent a hydrogen atom, an alkoxyl group having 1 or more and 4 or less carbon atoms, or an alkyl group having 1 or more and 4 or less carbon atoms; and n, m, l, q, s, and t each independently represent an integer of 1 or more and 8 or less, p and r each independently represent an integer of 4 or more and 12 or less, and "*" represents a bonding position with a silicon atom in the general formula. a step of hydrolyzing and condensing a hydrolyzable silane compound represented by the following general formula and a chelate titanium compound represented by the following general formula to obtain a surface-layer coating liquid; a first step of forming, on a surface of the elastic layer, a coat of a surface-layer coating liquid containing the hydrolyzed condensate of the hydrolyzable silane compound represented by the following general formula and the chelate titanium compound represented by the following general formula; and a second step of crosslinking the hydrolyzed condensate in the coat through cleavage of an epoxy group in the hydrolyzed condensate to form the surface layer: [Chem. 1] General formula R 1 -Si (OR 2) (OR 3) (OR 4) in the general formula, R 1 represents a hydrocarbon group represented by any one of the following general formulae to, and R 2 to R 4 each independently represent a hydrocarbon group; in the general formula, R 5 and R 6 each independently represent a linear or branched alkyl group having 1 or more and 20 or less carbon atoms, and R 7 to R 10 each independently represent a hydrogen atom, an alkyl group having 1 or more and 3 or less carbon atoms, or an alkoxy group having 1 or more and 3 or less carbon atoms; R 11 to R 13, R 16 to R 18, R 23, R 24, R 29, and R 30 each independently represent a hydrogen atom, an alkyl group having 1 or more and 4 or less carbon atoms, a hydroxyl group, a carboxyl group, or an amino group; R 14, R 15, R 19 to R 22, R 27, R 28, and R 33 to R 36 each independently represent a hydrogen atom or an alkyl group having 1 or more and 4 or less carbon atoms; R 25, R 26, R 31, and R 32 each independently represent a hydrogen atom, an alkoxyl group having 1 or more and 4 or less carbon atoms, or an alkyl group having 1 or more and 4 or less carbon atoms; and n, m, l, q, s, and t each independently represent an integer of 1 or more and 8 or less, p and r each independently represent an integer of 4 or more and 12 or less, and "*" represents a bonding position with a silicon atom in the general formula.