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Mortensen made his film debut in a small role in Peter Weir's 1985 thriller "Witness" starring Harrison Ford and continued to appear in several notable films, including "The Indian Runner" (1991), "Carlito's Way" (1993), "Crimson Tide" (1995), "Daylight" (1996), "The Portrait of a Lady" (1996), "G.I. Jane" (1997), "Psycho" (1998), "A Perfect Murder" (1998), "A Walk on the Moon" (1999), and "28 Days" (2000).