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The museum resulted from the purchase by the city of the Buenos Aires home of Enrique Larreta, perhaps the most prominent Argentine exponent of Hispanic modernism in literature, and Ambassador to France from 1910 to 1919. Larreta made numerous visits to Ávila, Spain, during his tenure, and he amassed a large collection of medieval art, armor, tapestries, Spanish Renaissance art, Spanish baroque art and decor, manuscripts, wood carvings, and French furniture, among other collections.