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Sebilangan lagu lain dikarang untuk filem oleh Sherman Brothers dan sama ada ditolak atau dipotong oleh kerana waktu. Richard Sherman, dalam pembebasan DVD 2004, menandakan bahawa lebih daripada 30 lagu telah dikarangkan di pelbagai tahap perkembangan filem. Tiada rakaman lakonan pada mana-mana lagu ini telah dibebaskan ke orang ramai, hanya demo atau persembahan kemudiannya dilakukan oleh pengarang lagu — dengan pengecualian reprise atas bumbung "Chim-Chim-Cheree" dan "smoke staircase yodel" disebut di bawah.

"The Chimpanzoo", was originally to follow "I Love to Laugh" during the Uncle Albert "ceiling tea party" sequence, but it was dropped from the soundtrack just before Julie Andrews and company were to record it. The fast-paced number was not unveiled to the public until Richard Sherman, aided by recently uncovered storyboards, performed it on the 2004 DVD edition. The re-creation suggests it was to have been another sequence combining animation and live action.

"Practically Perfect" was intended to introduce Mary but instead the melody of the piece was used for "Sister Suffragette" (used to introduce Winifred (Mrs. Banks)). A different song with the same name was written for the stage musical.

"The Eyes of Love", a romantic ballad, was intended for Bert and Mary, but according to Richard Sherman, Julie Andrews suggested privately to Disney that this song was not suitable. In response, "A Spoonful of Sugar" was written.

"Mary Poppins Melody" was to be performed when Mary introduces herself to the children. Elements of the song later became part of "Stay Awake". The melody was the basis for a couple of other songs that were ultimately cut from the film.

"A Name's a Name". Heard on a recording taken of a meeting between the Sherman Brothers and P.L. Travers, this song was originally intended for the nursery scene that later became "A Spoonful of Sugar." The melody was reused for "Mary Poppins Melody".

"You Think, You Blink" was a short piece that Bert was to sing just before entering the chalk painting (and starting the "Jolly Holiday" sequence). In the film, Dick Van Dyke simply recites the lyric instead of singing it.

"West Wind" was a short ballad to be sung by Mary. The song was later retitled "Mon Amour Perdu" and used in the later Disney film, Big Red.

"The Right Side" was to be sung by Mary to Michael Banks after he gets out of bed cranky.  It was recycled for the Disney Channel television series, Welcome to Pooh Corner as Winnie the Pooh's personal theme song.

"Measure Up" was to accompany the scene in which Mary takes the tape measure to Jane and Michael.

"Admiral Boom" was to be the theme song for the cannon-firing neighbor of the Banks Residence, but it was cut by Walt Disney as being unnecessary. The melody of the song remains in the film, and the bombastic theme is heard whenever Boom appears onscreen. One line from this song ("The whole world takes its time from Greenwich, but Greenwich, they say, takes its time from Admiral Boom!") is spoken by Bert early in the film.

"Sticks, Paper and Strings" was an early version of "Let's Go Fly a Kite."

"Lead the Righteous Life", an intentionally poorly-written hymn, was to have been sung by Katie Nanna (Elsa Lanchester) along with Jane and Michael prior to Mary Poppins' arrival. The melody was later reused for a similar song in The Happiest Millionaire

"The Pearly Song" was not deleted per se but was instead incorporated into "Supercalifragilisticexpialidocious".

The Compass Sequence, a precursor to "Jolly Holiday", was to be a multiple-song sequence. A number of possible musical components have been identified: