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In 2006, Betty formed a pop duo called WigWam, with Alex James, bassist from Blur. They released a one-off single also entitled "WigWam".

In August 2007, she released a new single titled "Take Off". The song, which was playlisted on Radio 1's dance-oriented shows, was a joint project with the London-based dance act Jack Rokka and, as such, is much more dance-oriented than her previous work. She went on to perform the collaboration in a live set at Manchester Pride in 2007, along with some of her other songs. The video sees Betty Boo's trademark look resurrected and even features the 'Boosters' - Betty Boo's backing dancers, who always appear with identical hair and outfits to Betty - and the Betty Boo spiral. Betty appeared on ITV's Loose Women on 16 October 2007 to promote the single, and has also appeared as an interviewee on BBC Three's "The Most Annoying Pop Songs..." show, passing comment on several songs that made the top 100 list.