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Greenville Pennsylvania, in Mercer County, is 65 miles north of Pittsburgh and has a population of about 6,700. Approximately 15,000 people live within a 15 - mile radius. Greenville is in County. Mercer County Pennsylvania. Return to this State's Index Page Return to the United States Community Page Index Return to the Global Index Top Of This Page Sponsorship opportunities at the local, state and national level.