The Heroic Legend of Arislan. Superb animation, great plot, handsome characters. Utterly awesome movie. One of my top favorites. The last 30 minutes or so are stunning.
Art is excellent.
My Neighbor Totoro. High-quality kiddie fare. Vampire Hunter D. Wish the art quality were better, but the story's cool. Vampire Princess Miyu. Occasionally needs more plot, but still cool.