There are whole books written on the subject, and I could go on and on about it myself. But I won't. Organization contributes to Ease of Use. Uniformity and Precision affect Appearance, etc. With the exception of Completeness and Relevance, each quality is roughly as important as any other.
Content is king.
Without complete content, no site is worth the effort. The more complete the content, the better. Not only does a site need content, it needs content appropriate to the site itself. The content needs to meet people's expectations. Additionally, the site's content should by current.