High-frequency resolution diamond nitrogen-vacancy center wide-spectrum imaging technology
Authors: Shen Yuan-Yuan , Wang Bo , Ke Dong-Qian , Zheng Dou-Dou , Li Zhong-Hao , Wen Huan-Fei , Guo Hao , Li Xin , Tang Jun , Ma Zong-Min , Li Yan-Jun , Igor Vladimirovich Yaminsky , Liu Jun ,   State Key Laboratory of Dynamic Testing Technology, North University of China, Taiyuan 030051, China,   School of Semiconductor and Physics, North University of China, Taiyuan 030051, China,   Shanxi Key Laboratory of Quantum Sensing and Precision Measurement, North University of China, Taiyuan 030051, China,   Department of Electronic Engineering, Taiyuan Institute of Technology, Taiyuan 030008, China,   Department of Applied Physics, Graduate School of Engineering, Osaka University, Osaka 5650871, Japan,   Advanced Technology Center, Moscow State University, Moscow 119311, Russia
Published: January 2024

High-resolution wide-spectrum measurement techniques have important applications in fields such as astronomy, wireless communication, and medical imaging. Nitrogen-vacancy (NV) center in diamond is well known for its high stability, high sensitivity, real-time monitoring, single-point detection, and suitability for long-term measurement, and has an outstanding choice for spectrum analyzers. Currently, spectrum analyzers based on NV centers as detectors can perform real-time spectrum analysis in the range of several tens of gigahertz, but their frequency resolution is limited to a MHz level. In this study, we construct a quantum diamond microwave spectrum imaging system by combining continuous wave-mixing techniques. According to the spin-related properties of the NV center in diamond, we implement optical pumping by 532 nm green laser light illuminating the diamond NV center. A spherical magnet is used to produce a magnetic field gradient along the direction of the diamond crystal. By adjusting the size and direction of the magnetic field gradient, spatial encoding of the resonance frequency of the NV center is achieved. The magnetic field gradient induces the Zeeman effect on the diamond surface at different positions, generating corresponding ODMR signals. Through accurate programming, we coordinate the frequency scanning step size of the microwave source with the camera exposure and image storage time, and synchronize them circularly according to the order of image acquisition. Ultimately, after algorithmic processing, we successfully obtain comprehensive spectrum data in a range from 900 MHz to 6.0 GHz. Within the measurable spectrum range, the system employs continuous wave-mixing, simultaneously applying resonant microwaves and slightly detuning auxiliary microwaves to effectively excite the NV center. This method triggers off microwave interference effects, disrupting the balance between laser-induced polarization and microwave-induced spontaneous relaxation. Specifically, microwave interference causes the phase and amplitude of the fluorescence signal to change, leading to the generation of alternating current fluorescence signals. This further enhances the response of the NV magnetometer to weak microwave signals. The method enables the system to achieve a frequency resolution of 1 Hz in the measurable spectrum range, and it can separately measure the frequency resolution of multiple frequency points with a frequency step size of 1 MHz. The research results indicate that the wide-spectrum measurement based on NV centers can achieve sub-hertz frequency resolution, providing robust technical support for future spectrum analysis and applications.