Optimization of the GSFC TROPOZ DIAL retrieval using synthetic lidar returns and ozonesondes – Part 1: Algorithm validation
Authors: Sullivan J. T. , McGee T. J. , Leblanc T. , Sumnicht G. K. , Twigg L. W. 
Published: April 2015

Abstract. The main purpose of the NASA Goddard Space Flight Center TROPospheric OZone DIfferential Absorption Lidar (GSFC TROPOZ DIAL) is to measure the vertical distribution of tropospheric ozone for science investigations. Because of the important health and climate impacts of tropospheric ozone, it is imperative to quantify background photochemical and aloft ozone concentrations, especially during air quality episodes. To better characterize tropospheric ozone, the Tropospheric Ozone Lidar Network (TOLNet) has recently been developed, which currently consists of five different ozone DIAL instruments, including the TROPOZ. This paper addresses the necessary procedures to validate the TROPOZ retrieval algorithm and develops a primary standard for retrieval consistency and optimization within TOLNet. This paper is focused on ensuring the TROPOZ and future TOLNet algorithms are properly quantifying ozone concentrations and the following paper will focus on defining a systematic uncertainty analysis standard for all TOLNet instruments. Although this paper is used to optimize the TROPOZ retrieval, the methodology presented may be extended and applied to most other DIAL instruments, even if the atmospheric product of interest is not tropospheric ozone (e.g. temperature or water vapor). The analysis begins by computing synthetic lidar returns from actual TROPOZ lidar return signals in combination with a known ozone profile. From these synthetic signals, it is possible to explicitly determine retrieval algorithm biases from the known profile, thereby identifying any areas that may need refinement for a new operational version of the TROPOZ retrieval algorithm. A new vertical resolution scheme is presented, which was upgraded from a constant vertical resolution to a variable vertical resolution, in order to yield a statistical uncertainty of <10%. The optimized vertical resolution scheme retains the ability to resolve fluctuations in the known ozone profile and now allows near field signals to be more appropriately smoothed. With these revisions, the optimized TROPOZ retrieval algorithm (TROPOZopt) has been effective in retrieving nearly 200 m lower to the surface. Also, as compared to the previous version of the retrieval, the TROPOZopt has reduced the mean profile bias by 3.5% and large reductions in bias (near 15 %) were apparent above 4.5 km. Finally, to ensure the TROPOZopt retrieval algorithm is robust enough to handle actual lidar return signals, a comparison is shown between four nearby ozonesonde measurements. The ozonesondes agree well with the retrieval and are mostly within the TROPOZopt retrieval uncertainty bars (which implies that this exercise was quite successful). A final mean percent difference plot is shown between the TROPOZopt and ozonesondes, which indicates that the new operational retrieval is mostly within 10% of the ozonesonde measurement and no systematic biases are present. The authors believe that this analysis has significantly added to the confidence in the TROPOZ instrument and provides a standard for current and future TOLNet algorithms.