MAGNETIC PARTICLES, SUBSTRATE COMPRISING SUCH PARTICLES, SECURITY DOCUMENT AND METHOD FOR DETECTING SUCH PARTICLES

Abstract: The present invention relates to a method and an apparatus for detecting the presence of particles in a substrate the base material of which has electromagnetic properties substantially differing from the corresponding electromagnetic properties of the particles. The invention also relates to the particles and to the substrate comprising such particles which allow to recognise easily a document as being a genuine security document in order to prevent the document from being copied or in order to contribute to its authentication.

Description: MAGNETIC PARTICLES, SUBSTRATE COMPRISING SUCH PARTICLES, SECURITY DOCUMENT AND METHOD FOR DETECTING SUCH PARTICLES Field of the invention. The present invention relates to a method and an apparatus for detecting the presence of particles in a substrate the base material of which has electromagnetic properties substantially differing from the corresponding electromagnetic properties of the particles. The invention also relates to the particles and to the substrate comprising such particles which allow to recognise easily a document as being a genuine security document in order to prevent the document from being copied or in order to contribute to its authentication. The invention is intended primarily to be used in the identification or authentication of all type of security documents having a paper or synthetic base material such as bank notes, cheques, passports, credit-cards, tickets, lottery- tickets and bonds which comprise the above particles, but it is also applicable to other applications in which objects need to be recognised. Background of the invention. The prior art has already dealt in an extensive way with the identification of security documents. Some prior art solutions go in the direction of recognition of possible characteristic patterns printed at the surface of some security documents. In order to prevent genuine security documents from being falsely copied by means of high-resolution colour photocopying apparatus, the prior art has also proposed to add to the fibrous structure of the base material of the substrate or to the surface of the document one or more security elements allowing the identification and/or making difficult the manufacturing of the document. US-A-4 1 14 032 (priority date 1973) and US-A-4 218 674 (filing date 1975) disclose a similar system where the security documents have fibres which are coated with a magnetic or magnetizable material embedded therein. The mere presence of the magnetic fibres inside the security documents is tested or, as an improved feature, the distribution of the magnetic fibres in the security document is measured so that every single security document can be given a unique mark. Up to 500 million different possible combinations may be obtained. EP-A-0 625 766, EP-A-0 632 398 and EP-A-0 656 607 (all filing date in 1993) disclose a system where the fibres consist of magnetic powder as core of a polymer sheath. Magnetic detection is done by DC current used to excite a coil. Because of magnetic prehistory or disturbing of magnetic fields or deformations of the security documents, however, the repetitivity of such a magnetic scanning system is not ensured and accurate discrimination between genuine security documents and counterfeit documents is not always guaranteed. So detection is not always distinctive. Moreover, if characters on the security document have been printed by means of a magnetic ink which is detectable by means of a sorting apparatus, there may be interference between the magnetic fibres and the magnetic ink of the characters. Other embodiments disclosed in the prior art are based on the detection of particular electromagnetic properties of the security elements. FR 2 425 937 discloses a method of dispersing metallic fibres, more particularly stainless steel fibres, inside the fibrous structure of paper in order to allow the identification by means of microwaves. US-A-4 820 912 (priority date 1985) discloses an alternative system where the security documents comprise randomly distributed electrically conductive fibres. By scanning the documents by means of microwaves the unique distribution of the fibres inside the security document can be obtained. Up to 64 320 different possible combinations of the mark characterising this distribution can be obtained. Application of this microwave technique to reproduction apparatus such as photocopying apparatus in order to prevent security documents from being copied, such as disclosed in WO-A- 95/24000 (priority date 1994) fails to distinguish security documents from printed circuit boards (PCB's) or from greeting cards having decorative metal foils on its surface. On the other hand, the system does not discover the presence of the fibres if a metal plate is put above a genuine security document. Particular cover lids of photocopying apparatus or metallic parts in the neighbourhood of the photocopying apparatus, may disturb the system. As a consequence, these systems are not completely reliable. The prior art has also provided a number of optical authentication systems. Some of them have been disclosed already in US-A-3 313 941 (filing date 1963) and in US-A-3 449 585 (filing date 1966). All optical systems, however, suffer from the major drawback that wear or damage or dirt on the surface of genuine security documents can cause the security documents as being no longer recognised as authentic. Summary of the invention. It is an object of the present invention to avoid the drawbacks of the prior art. It is another object of the present invention to provide for a robust recognition system that allows to distinguish genuine security documents from other objects or documents. It is also an object of the present invention to provide for a system which prevents genuine security documents from being copied. it is still an object of the present invention to provide for a system that does not interfere with conventional magnetic character readers. It is a further object of the present invention to provide for a substrate such as a security document, more particularly a banknote, including security elements, easily detectable in an anti-photocopy system. According to a first aspect of the present invention, there is provided a method for detecting the presence of magnetic elongated particles in a substrate the base material of which has magnetic properties substantially differing from the corresponding magnetic properties of the elongated particles said particles having a magnetic saturation field H s greater than 100 A/m, preferably greater than 200 A/m and most preferably greater than 300 A/m. Preferably the base material is made of a non-magnetic material. Preferably the elongated particles have such a long and thin form that their demagnetisation factor N is smaller than 1/250, preferably smaller than 1/1000 and their cross-sectional diameter is smaller than 30 micrometer.. The magnetic saturation field H 3 is preferably smaller than 1000 A/m. The terms "magnetic saturation field H s " are herein defined as the magnetic field at the onset of the saturation flux density B s . The terms "cross-sectional diameter" herein refer to the maximum cross-sectional dimension. The method comprises the following steps : (a) emitting an electromagnetic source signal of one or more particular base frequencies to the substrate so that any present magnetic elongated particles go into a non-linear part of their B-H curve for at least part of a cycle of the source signal ; (b) detecting an electromagnetic detection signal emanating from the substrate ; (c) testing the detection signal for the presence of particular higher harmonics of the base frequencies or of any linear combination of the base frequencies as well as the harmonics, where the particular higher harmonics are indicative of the presence of the magnetic elongated particles. Using the non-linearity of the magnetisation properties of the labelling material, i.e. the change in magnetic flux density B with applied magnetic field H as an effective parameter for detection is a technique which is known as such in electronic article surveillance (EAS) or anti-theft systems. The signals which can be obtained from this approach are very distinctive and the electronics and signal processing can be straight forward. EAS systems have been disclosed in an extensive way in the patent literature. Some examples are FR 763 681 (filing date 1933), US-A-3 631 442 (filing date 1967), US 3 990 065 (filing date 1975) and EP-A-0 153 286 (priority date 1984). A number of substantial differences between EAS systems and the present invention are, however, apparent. In EAS systems anti-theft labels are used to trigger alarms at the exit areas of shops if the products have not been offered at the pay-desk. The exit area of a shop is much larger than the volume required for detection of magnetic elongated particles in security documents. A typical exit gate has a width of about 1 m, while in the present invention distances of only a few cm, e.g. of only 0.5 to 5 cm, between the magnetic field and the magnetic elongated particles are sufficient to perform the detection. This basic difference leads to a number of properties which are different for application of the present invention : 1) The magnetic material of EAS labels is rather bulky, since it must be present in a sufficient volume to trigger off the alarm in the relatively large exit area ; a typical cross-sectional dimension is about 1 mm and the length can be several cm long. In contrast herewith, the magnetic elongated particles according to the present invention have a much smaller volume. Their demagnetisation factor N is smaller than 1/250, preferably smaller than 1/1000 and their cross-sectional diameter is smaller than 30 micrometer, preferably smaller than 15 micrometer and most preferably ranging from 1 to 10 micrometer. The maximum value for the demagnetisation factor N is chosen so that the magnetic elongated particles can be detected by means of an apparatus with acceptable coil dimensions and power dissipation so that they can be installed on e.g. a photocopier or a bank note counting machine. Preferably the demagnetisation factor N is greater than 1/100000 in order to avoid setting off EAS alarms. 2) The magnetic material of EAS labels can be classified as very soft magnetic material, i.e. material having a very small coercive force H c and a relatively high dynamic permeability μ d , since small magnetic fields H covering the exit area of a shop must be able to saturate the EAS labels. In contrast herewith, the magnetic elongated particles according to the present invention, although still being classified as soft magnetic materials, have such a shape and/or composition and/or structure that they are effectively magnetically hard enough to stay below the saturation point of their B-H loop in the fields used in the shop systems so that they do not generate high enough signals to activate the shop alarms. In comparison with EAS labels, the magnetic elongated particles according to the present invention have preferably a lower magnetic dynamic permeability μ d and therefore require a substantially higher magnetic field to reach saturation. The magnetic saturation field H 9 of magnetic elongated particles according to the present invention is greater than 100 A/m, preferably greater than 200 A/m and most preferably greater than 300 A/m. This lower value is chosen not to trigger off EAS alarms. Preferably the magnetic saturation field H s is smaller than 1000 A/m so that it can be achieved by means of a detector apparatus with acceptable coil dimensions and power dissipation that it can be built in a photocopier or a bank note counting machine or an automatic vending machine. The inventors have experienced so far that anything over 1000 A/m will be difficult to achieve with an air cored coil. It is possible, however, to obtain a magnetic saturation field greater than 1000 A m when making use of a ferrite cored coil or when making use of ferromagnetic powders in the core. The magnetic saturation flux density preferably ranges from 0.1 to 1 Tesla, and the dynamic permeability μ d (for definition see below) ranges from 100 to 10000. Within the context of the present invention, all these magnetic properties have been determined by use of an alternating current magnetometer at frequencies from 10 kHz to 100 kHz. 3) Due to the bulky material of EAS labels, the frequencies applied are limited in order to reduce eddy current losses. In contradistinction herewith, much higher frequencies (higher than 1 kHz) can be applied in the present invention, since the magnetic elongated particles have a much lesser volume. The corresponding harmonics have also a much higher frequency (higher than 10 kHz) and typical harmonics have an order of ten or higher. 4) In EAS systems the problem of covering the large volume of the exit area of a shop and the problem of orientation-sensitive EAS labels has led to a number of embodiments where two or more base frequencies are used or to the use of an additional rotating magnetic field in order to create a global spatial magnetic field which is insensitive to the orientation of the EAS. Due to the much more limited sizes of the volumes required for the present detection method, such complications are not necessary for the present invention. A source signal of a single base frequency has proved to be sufficient. In an embodiment of the present invention, the method comprises the additional step of : (d) generating a signal which prevents from taking a true copy in case said particular harmonics are present. According to a second aspect of the present invention, there is provided a detection apparatus for detecting the presence of magnetic elongated particles in a substrate the base material of which has magnetic properties substantially differing from the corresponding magnetic properties of the elongated particles, said particles having a magnetic saturation field H s is greater than 100 A/m, preferably greater than 200 A/m and most preferably greater than 300 A/m. Preferably the base material is made of a non-magnetic material. Preferably the elongated particles have such a long and thin form that their demagnetisation factor N is smaller than 1/250 and their cross-sectional diameter is smaller than 30 micrometer. The apparatus comprises : (a) an oscillator for emitting an source signal of one or more base frequencies to the substrate ; (b) a detector for detecting an detection signal emanating from the substrate ; (c) a signal processor for examining the detection signal for the presence of any particular higher harmonics of the base frequencies or of any linear combination of the base frequencies, where the particular higher harmonics are indicative of the presence of the magnetic elongated particles. According to a particular embodiment of the apparatus, both the source signal and detection signal are electrical signals and the apparatus further comprises a drive coil for converting the source signal into a magnetic drive field, and a detection coil for converting a detection magnetic field into the detection signal. The coils are so arranged to null out the magnetic drive field in the detection coil in order to avoid saturating the amplifier and to minimise any cross-coupling which can occur with conducting materials. According to a preferable embodiment of the apparatus the drive coil is arranged around a ferrite core. The ferrite core has a U-shape and a drive coil is arranged around each leg of the U-shaped ferrite core. A detection coil is also arranged around each leg of the U-shaped ferrite core. Each detection coil is preferably divided into two parts, with one part at both sides of the drive coil. These two parts of a detection coil are wired in anti-phase in order to null out the drive signal. Next to a drive coil and a detection coil, a third coil may be present around the ferrite core in order to detect the presence of any ferrous metals. The apparatus according to the second aspect of the present invention can be used in automatic vending machines, bank note counting machines and reproduction apparatus. With respect to the use in reproduction apparatus, in order to detect the presence of any security documents in the whole scanning region, the following embodiments can be used : 1) the use of more than one drive coil and more than one detection coil ; 2) drive coils and detection coils forming a daisy chain ; 3) the use of only one drive coil and one detection coil, both having an elongated form ; 4) the use of one drive coil and more than one detection coil. According to the third aspect of the present invention, there is provided an elongated magnetic particle for being incorporated in a base material of a substrate where the base material has magnetic properties differing substantially from the corresponding magnetic properties of the particle. Preferably the base material is made of a non-magnetic material. The particle has such a long and thin form that its demagnetisation factor N is smaller than 1/250, preferably smaller than 1/1000. The cross-sectional diameter of the particle is smaller than 30 micrometer, preferably smaller than 15 micrometer, preferably ranging from 1 to 10 micrometer and its magnetic saturation field H s is greater than 100 A/m, preferably greater than 200 A/m, and most preferably greater than 300 A/m. The magnetic field strength inside the material is given by H in = H app - N x M where M is the magnetisation of the material, H app is the applied magnetic field and N is the demagnetisation factor. With uniform magnetisation this reduction in the internal field strength can be considered as a reduction in the apparent permeability from its true value of μ r , which is the so-called bulk magnetic permeability or magnetic permeability of the material, to the magnetic apparent or effective permeability μ r \ where 1/μ r = 1/μ r ' - N, or μ r ' = μ r / (1 + Nμ r ) The effect of the reduction in permeability therefore causes the B-H loop to shear into a shape which has a higher saturation field and lower remanence. In case of a sphere, the demagnetisation factor N = 1/3. Whereas for long, thin ellipsoids (approximating to cylinders represented by the elongated particles such as fibres) N is given by : N = [In (2p) - 1] / p 2 where p is the length to diameter ratio. For a fibre of 8 micrometer diameter and 3 mm length, N is equal to 1/25000. Based on these equations if, as an example, we take a material with a bulk permeability μ r of 100000 then a sphere of identical material would appear to have an magnetic apparent permeability μ r ' approximately 7000 times smaller than a fibre with the dimensions shown above. This will then have a direct effect on the magnitude of the field required to saturate the material in each case. Thus spheres, or powders of approximately spherical form would not be suitable for the application described herein. Preferably, the magnetic saturation flux density B 3 of the magnetic elongated particle ranges from 0.1 to 1 Tesla, preferably from 0.1 to 0.5 Tesla. The apparent or effective magnetic permeability μ r ' is measured at d.c. The magnetic dynamic permeability μ d . parameter is an indicator of the sensitivity of the particle in practical situations taking account of bulk permeabilities, shape factors, the a.c. frequency of the drive fields and the field limits which are typical in EAS gates and which would be practical in our proposed new invention system. The magnetic dynamic permeability μ d is therefore herein defined as the ratio of the saturation flux density B s to the magnetic saturation field H s multiplied by μ 0 ., measured at an a.c. frequency. If the materials do not saturate at the fields used in the magnetometer then the magnetic dynamic permeability μ d is defined as the ratio of the flux density B to μ G H at the maximum field used in the experiment (e.g. about 1000 A/m). The magnetic dynamic permeability μ d is clearly related to the apparent magnetic permeability μ r ' and both parameters would have the same or close to the same value at d.c. in a low loss material in which sheer due to demagnetisation dominates the shape of the measured B-H- loop. The magnetic dynamic permeability μ d of the magnetic elongated particle preferably ranges from 100 to 10000. The terms "magnetic elongated particle" refer to an elongated particle itself made of a magnetic material and possibly of a magnetic material and a non- magnetic material. In particular the magnetic material can be coated or encapsulated with a non-magnetic material or the elongated particle can be made of a non-magnetic material being coated with a magnetic material or incorporating a magnetic material. The thickness of the coating may range from 1 to 5 micrometer. The magnetic material can be made starting from an alloy comprising components chosen among Fe, Cr, Co, Cu, Ni, Mo, Mn, Nb, B, V, C, Si and P, more particularly among Ni, Fe, Mo, Mn, C, and Si. Soft magnetic materials have been disclosed for example in EP-A-0 295 028 and in US-A-4 298 862. A suitable alloy composition responds to the general formula : Ni a Fe b Cr c Co d Cu β MO f Mn g P h NbiB j k SiiC m , where a to m represent integers. More particular alloy compositions have 52 to 85 % of nickel (Ni) and varying amounts of other components. An example of a good working alloy composition is : 80.00 % Ni, 4.20 % Mo, 0.50 % Mn, 0.35 % Si; 0.02 % C, the balance being Fe. Other typical compositions are : Some of these compositions are commercialised under names as μ-metal, Permafi, Permalloy, Supermalloy, Vitrovac and Metglas. As non-magnetic and non-metallic material glass, carbon or synthetic material such as polymers especially polypropylene and polyethylene can be mentioned. According to a preferable embodiment of this third aspect of the present invention, the elongated particle is a fibre which can be a metallic fibre or a non- metallic fibre coated with a magnetic substance. The fibres can be uniformly dispersed and distributed all over the substrate and therefore not easily missed by the detection system. The fibres can preferably uniformly and individually dispersed all over the substrate in order to prevent them the formation of agglomerates of fibres. Additionally, since the fibres are dispersed inside the substrate, they are not easily removable by the counterfeiters who would like to remove them before making a photocopy and reinstate them inside the substrate after photocopy thereof. The fibres are preferably hard drawn or work hardened metal fibres, e.g. manufactured according to the technique of bundled-drawing which is well known as such. This manufacturing technique has the advantage of yielding a much higher production rate than hot melt production techniques. Hard drawing makes the magnetic fibres also 'harder * from a magnetic point of view, i.e. less soft-magnetic so that a higher magnetic saturation field H s is required. This is particularly useful in the present invention since it helps to distinguish from EAS tags and prevents from setting the alarms in EAS gates. The inventors have also found that the magnetic dynamic permeability μ d of the hard drawn fibres can be doubled by annealing. This still keeps the saturation field H, sufficiently high, but makes the fibres more sensitive. The magnetic elongated particles may also be amorphous metal fibres. According to a fourth aspect of the present invention, there is provided a substrate comprising a base material and elongated particles inside the base material. The magnetic properties of the elongated particles differ from the corresponding magnetic properties of the base material said particles having a magnetic saturation field ranges from 100 A/m, preferably from 200 A/m and most preferably from 300A/m. Preferably the base material is made of a nonmagnetic material. Preferably the elongated particles have such a long and thin form that their demagnetisation factor N is smaller than 1/250 and their cross- sectional diameter is smaller than 30 micrometer. Preferably the base material is a non-magnetic material such as plastic or a fibrous structure like paper. Preferably the elongated particles have a magnetic saturation flux density ranging from 0.1 to 1 Tesla, preferably from 0.1 to 0.5 Tesla and a magnetic dynamic permeability μ d ranging from 100 to 10000. Summarizing, the combination of shape, composition and structure of the magnetic elongated particles is such that - the magnetic field required to achieve saturation of the flux density in the particle is sufficiently greater than that produced in EAS systems and sufficiently lower than that required to saturate hard ferromagnetic material such as iron, steel or plate, and - the magnetic remanent flux density is sufficiently lower than those of magnetic ink used in the magnetic coding system as defined in the international standard for magnetic ink character recognition ISO 1004. These properties are fulfilled when the combination of shape, composition or structure of the magnetic elongated particles is such that the elongated particles have : i) a saturation field ranging from 100 to 1000 A/m ; ii) a saturation flux density ranging from 0.1 to 1 Tesla ; iii) a magnetic dynamic permeability μ d ranging from 100 to 10000. The magnetic elongated particles, especially the fibres, have a mean cross- sectional diameter ranging from 1 to 30 micrometer (μm), preferably from 5 to 15 micrometer, and a length ranging from 1 to 20 mm, preferably ranging from 2 to 10 mm. Most preferably the elongated particles are hard drawn or work hardened metal fibres, but can also be amorphous metal fibres. The magnetic elongated particles can be made of an alloy comprising components chosen among Ni, Fe, Cr, Co, Cu, Mo, Mn, P, Nb, B, V, Si, and more particularly Fe, Ni, Mo, Mn, Cu. The base material of the substrate can be made of paper or of a synthetic material, especially a plastic such as polypropylene or polyethylene. The magnetic elongated particles can also be made of magnetic and nonmagnetic material. Preferably the substrate according to the fourth aspect of the present invention, has a quantity of magnetic elongated particles, especially fibres, ranging from 0.1 to 5 per cent, preferably from 0.2 to 2 per cent, most preferably from 0.5 to 1.5 per cent by weight relative to the weight of the substrate. If the substrate is a paper sheet, its thickness commonly varies from 20 to 300 micrometer. Bank notes usually have a thickness varying between 80 and 120 micrometer. The elongated particles may be uniformly or randomly dispersed in the whole substrate and/or may be present only in selected parts of the substrate. The fibres may be distributed within a substrate in selected parts thereof according to methods known in the art and especially in methods disclosed in WO 96/14469 (PCT/FR95/01405). Preferably the fibres are includes in parts of bank notes corresponding to printed areas so that the fibres are less visible. More particular, the fibres are included outside any watermark area. Most preferably, the fibres are outside the areas which are printed with magnetic ink so as to avoid any possible electromagnetic interference. In one preferred embodiment the fibres are present within the substrate in areas having the form of tapes of a width of at least 20 mm. Preferably, the elongated particles, especially the fibres have a colour near to the colour of the base material. This can be realised by the deposit of a covering or a coating providing to the fibres the wished colour. Methods of depositing such a coating have been disclosed in French patent application FR 95 02868 and in international application PCT/FR/96 00390. The present invention also provides a security article such as a security document, more particularly a bank note, adapted to be authenticated, said security article comprising particles and a substrate according to the invention. Therefore the present invention provides a security article, such as a bank note, adapted to be authenticated, said security article incorporating magnetic particulate material which requires a field strength of at least 100 A/M (and preferably of at least 300 A/M) before it will saturate, thereby to prevent such articles triggering electronic article surveillance systems. Short description of the drawings. The present invention will now be illustrated in more detail with reference to the accompanying drawings wherein - FIGURE 1 compares the B-H curve of a magnetic elongated particle according to the invention with B-H curves of other objects ; - FIGURE 2 schematically illustrates a configuration of a detection apparatus according to the present invention ; - FIGURE 3 shows how a drive coil and a detection coil of an invention apparatus can be arranged ; - FIGURE 4, FIGURE 5, FIGURE 6 and FIGURE 7 all illustrate embodiments of drive coil(s) and detection coil(s) for use in a reproduction apparatus ; - FIGURE 8 illustrates a preferable embodiment of drive and detection coils arranged around a ferrite core. Detailed description of an embodiment. Reference number 10 in FIGURE 1 refers to a B-H curve of an EAS label which can be designated as "very soft magnetic". It is characterised by a very low saturation field H s and a rather high level of magnetic dynamic permeability. Reference number 12 refers to a B-H curve of a magnetic elongated particle which is to be embedded in a substrate according to the present invention. Although being also a soft magnetic material, it is not that "very soft" as is an EAS label. The saturation field H' s is higher than the corresponding values of an EAS label. Reference number 14 refers to the B-H curve of a mild steel plate clearly showing a saturation field that is much larger than H, and H' s It will be clear from FIGURE 1 that the low magnetic fields applied in EAS systems to saturate the EAS labels do not saturate the magnetic elongated particles according to the present invention and do not trigger the alarm systems in shops. It will also be clear from FIGURE 1 that magnetic fields applied in the present invention to saturate the magnetic elongated particles are still in the relatively linear part of a B-H curve of a mild steel plate and will not create the same series of higher harmonics. This difference can be used in order to discriminate between the two types of materials and even to detect the marker tag in the presence of large Ferro-magnetic objects. The following table shows an experimental comparison of actual markers and examples of common magnetic objects measured in a magnetometer at between 20 Hz to 20 kHz. Table. Type of material + geometric saturation saturation dynamic dimensions flux field H s permeability density B s (A/m) μ d [Bs/tøoHs)] (Tesla) EAS label 0.35 30 (200 Hz) 10000 32 mm x 0.8 mm x 25 μm 80 (11 kHz) paper clip > 1000 60 mild steel plate » 1000 30 12 mm x 9 mm x 1 mm hard drawn magnetic metal fibre 0.55 500-600 730 3 mm length x 8 μm diameter (11 kHz) μ o = 4πx10 "7 N/A 2 The EAS label in the table has a volume and mass which is about 3000 times that of the metal fibre of the table. The above figures represent the relative differences between the materials. It should be appreciated, however, that in practical cases for EAS tags and the invention system, the actual magnetisation of the scanning or interrogating field needs to be taken into account at the orientation of the material in the field, the bulk of material present and the frequencies used. The magnetic metal fibre had an a.c. remanence of 0.3 Tesla in the measurement. In practice the d.c. remanence would be lower than this so that no significant electromagnetic noise signals are generated which interfere with other magnetic code systems. In particular, the fibres did not give any significant signal with a standard magnetic character reader reading characters made for magnetic inks. In other words, using the measurement method and definition of maximum residual signal levels as defined in the International Standard for magnetic ink character recognition, ISO 1004, the effect of remanent flux density is acceptable. Experimental results show that it is possible to detect a good signal amplitude at high harmonics from the fibre mentioned in the above table and that at high frequencies there is very low interference from harmonics from the drive electronics. With the small cross sectional area of the fibres the eddy current losses are small up to quite high frequencies and the output signals are increased by the fact that the detected voltage is proportional to the rate of change of flux density. With bulk ferromagnetic materials the eddy current losses are much higher at high frequencies and so they don't generate very high harmonics. Using a base frequency to sweep the fibres (which are characterised in the table above) around their B-H loop at 20 kHz, and a peak field greater than 600 A/m it was found that at frequencies between 100 kHz and 1 MHz there was a stream of harmonics from the fibres and very much smaller signals from other common electrically conducting objects. In practice the base frequency and the detection frequency or frequencies can be selected to maximise the signal from the particular fibre marker and minimise signals from other common objects and signals generated from the apparatus in which the system is installed. Tests carried out by the inventors have proved that the invention system provides a good discrimination between a security document with magnetic elongated particles and paper, books, hands, printed circuit boards, metallic foil greeting cards, non metallic bindings of documents, spiral metal bindings of documents, paper clips, metal plates and photocopier lid materials. A security document lying under a non-magnetic metal plate could be easily identified (this in great contrast with a microwave system where the metal plate conceals the magetic fibres for the microwaves) A suitable drive and detection circuit is shown in FIGURE 2. A resonant drive power oscillator 16 is used to minimise harmonic generation and the oscillator 16 is driven by a frequency which is divided down from the selected harmonic. As an example, the inventors have found that, amongst other harmonics, the 19th harmonic of 20 kHz, at 380 kHz may be a good choice as it gives good signals from fibres with very small signals from common Ferro-magnetic materials such as mild steel. The oscillator 16 generates an electrical source signal which is fed to a drive coil 18 which transforms the electrical source signal into a magnetic drive signal. A detection coil 20 suitably arranged with respect to the drive coil 18, detects any field emanating from magnetic elongated particles and transforms this into an electrical detection signal. A high pass filter 22 is used to reduce the fundamental frequency, as this can be coupled between the coils by conducting metals and overload the amplifiers. A phase sensitive detector 24 is used to provide good signal-to-noise ratio. Oscillator 26 operates at the frequency of the selected harmonic, and frequency divider 28 divides the frequency in order to obtain the base frequency. Other high harmonics are also suitable and it is an advantage to combine several to derive the final detection signal. FIGURE 3 illustrates how the drive coil 18 may be advantageously arranged with respect to the detection coil 20. The direction of the magnetic field generated by the drive coil is shown in hatched lines, except for that part of the magnetic field that goes through the detection coil 20, which is shown by means of arrows 30 and 32. Drive coil 18 and detection coil 20 partially overlap and are so arranged that the part of the magnetic flux density which goes in one direction (arrow 30) through detection coil 20 is almost equal to the part of the flux density which goes in the other direction (arrow 32) in order to null-out the drive field in the detection coil whilst providing a region above the overlapping coils in which the magnetic field is effective in coupling into the magnetic elongated particles. An equivalent nulling effect could also be provided electronically by a negative feedback of the fundamental frequency. FIGURE 4, FIGURE 5, FIGURE 6 and FIGURE 7 all show embodiments of arrangement of drive coil and detection coil to be used in reproduction apparatus such as high-resolution colour photocopying apparatus. The arrangement is such that a bank note with a width of only 7 cm can be detected on a scanning area of 21 cm x 29.7 cm (if it comprises magnetic elongated particles). According to FIGURE 4, four pairs of a drive coil 18 with a detection coil 20 are arranged on a suitable carrier 34 at regular distances along the width of the scanning area so that the presence of any genuine bank note will be detected irrespective of its position on the scanning area. In the embodiment of FIGURE 5 a plurality of drive coils 18 and a plurality of detection coils 20 form a daisy chain wherein a drive coil 18 is alternated with a detection coil 20 and vice versa. In the embodiment of FIGURE 6 the drive coil 18 takes the form of an elongated eight with the height of the eight equal to the width of the scanning area. The detection coil takes the form of an elongated ellipse with the length of the longitudinal axis equal to the width of the scanning area. Drive coil 18 and detection coil 20 are arranged one above the other so that here also the part of the magnetic flux density which goes in one direction through detection coil 20 is almost equal to the part of the flux density which goes in the other direction in order to null-out the drive field in the detection coil. FIGURE 6 shows for didactical reasons a drive coil 18 and a detection coil 20 at a distance apart from each other, but they are to be arranged next to one another. FIGURE 7 shows schematically an embodiment with only one drive coil 18 and four detection coils 20 so arranged that the drive magnetic field balances out in detection coils 20. Description of a preferable embodiment. Referring to FIGURE 8, drive coils 18 and detector coils 20' and 20" are arranged around a ferrite core 36. For use in a reproduction apparatus, the ferrite core 36 is positioned at a few mm from a glass platen 38. A security document 40 comprising elongated magnetic particles 41 is positioned on the glass platen. The ferrite core 36 is used to ensure a higher magnetic field at the level of the security document 40 for a given drive current. The ferrite core 36 must not saturate in order to avoid from creating additional non-linearities and harmonics. The ferrite core 36 is preferably U-shaped. This means it has two legs 42 connected by a "bridge" 43. The bridge 43 ensures that the flux flow is kept away from any neighbouring metal of the reproduction apparatus. A drive coil 18 is wired somewhere in the middle of each leg 42. The detector coil is divided into two parts 20' and 20". One part 20' is wired at the side of the glass platen 38 around the leg 42, the other part 20" is wired at the down side around the leg 42. Both parts 20' and 20" are wired in anti-phase, as designated by reference number 44, in order to null out the received drive signal and other sources of interference such as the presence of a lamp in the reproduction apparatus. The wiring in anti-phase, however, does not null out the signals received from any alongated magnetic particles 41 since one part 20', the top coil part, of the detection coil is positioned much nearer to the magnetic particles than the other part 20", the bottom coil part. Next to the drive coil and the detection coil, a third coil may be wired around the ferrite core in order to detect the presence of any ferrous metal on the glass platen 38. As is known in the art, the presence of any ferrous metal may disturb the magnetic flux pattern so that a ferrous metal could be used to hide the presence of any security documents with elongated magnetic particles. For reason of simplification this third coil is not shown in FIGURE 8.

Claims: CLAIMS 1. A magnetic elongated particle for being incorporated in a base material of a substrate with magnetic properties differing substantially from the corresponding magnetic properties of said particle, said particle having a magnetic saturation field greater than 100 A/m, preferably greater than 300 A/m. 2. A magnetic elongated particle according to claim 1 wherein said particle has such a long and thin form that its demagnetisation factor N is smaller than 1/250, preferably smaller than 1/1000 and a diameter being smaller than 30 micrometer. 3. A magnetic particle according to claim 1 to 2 wherein said particle has a magnetic saturation flux higher than 0.1 Tesla, preferably ranging from 0.1 to 1 Tesla. 4. A magnetic particle according to claims 1 to 3 wherein said particle has a magnetic dynamic permeability μ d ranging from 10 to 10000, preferably from 100 to 10000. 5. A magnetic particle according to anyone of claims 1 to 4 wherein the combination of shape, composition and structure of the magnetic particle is such that they have : i) a saturation field ranging from 100 to 1000 A/m ; ii) a saturation flux density higher than 0.1 Tesla, preferably ranging from 0.1 to 1 Tesla ; iii) a magnetic dynamic permeability μ d ranging from 10 to 10000, preferably from 100 to 10000. 6. A magnetic particle according to anyone of claims 1 to 5 wherein said magnetic particle is made of a magnetic material and a non magnetic material. 7. A magnetic particle according claim 6 wherein said magnetic particle is made of a non-magnetic material coated or encapsulated with a magnetic material. 8. A magnetic particle according to anyone of claims 1 to 7 wherein said magnetic particle has a mean cross-sectional diameter ranging from 1 to 30 micrometer and a length ranging from 1 to 20 mm. 9. A magnetic particle according to anyone of claims 1 to 8 wherein said particle has a D.C. magnetic remanence smaller than 0.3 Tesla. 10. A magnetic particle according to anyone of claims 1 to 9 wherein said particle is a metal fibre. 1 1. A magnetic particle according to claim 10 wherein said particle is a hard drawn or work hardened metal fibre . 12. A magnetic particle according to claim 11 wherein said metal fibres have been annealed. 13. A magnetic particle according to claim 10 wherein said particle is an amorphous metal fibre. 14. A magnetic particle according to anyone of claims 1 to 13 wherein said magnetic article is made of an alloy comprising components chosen among Ni, Fe, Cr, Co, Cu, Mo, Mn, Nb, Si, V, B, C and P. 15. A magnetic particle according to claim 14 wherein the said alloy comprises components chosen among Ni, Fe, Mo, Mn, Si and C. 16. A substrate comprising a base material and elongated particles inside said base material, the magnetic properties of said particles differing from the corresponding magnetic properties of said base material, the particles having a magnetic saturation greater than from 100 A m preferably greater than 300 A/m according to anyone of claims 1 to 15. 17. A substrate according to claim 16 wherein said base material is made of paper or plastic. 18. A substrate according to anyone of claims 16 to 17 wherein the quantity of magnetic elongated particles in said substrate ranges from 0.1 to 5 % by weight relative to the weight of said substrate. 19. A security article comprising a substrate as claimed in claims 16 to 18. 20. A security document comprising a substrate as claimed in claims 16 to 18. 21-. A security document as claimed in claim 20 wherein the document is a bank note. 22. A. security document according to claims 20 to 21 comprising said magnetic elongated particles uniformly dispersed inside said substrate, said substrate comprising a paper or plastic sheet. 23. A security document as claimed in claims 20 to 22 wherein the said elongated particles are dispersed in selected parts of the substrate. 24. A security document as claimed in claims 20 to 23 wherein the magnetic elongated particles are made of metallic fibres, the quantity of magnetic fibres in said substrate ranging from 0,2 to 2 %, the substrate being a paper sheet. 25. A method for detecting the presence of magnetic elongated particles in a substrate or a security document according to anyone of claims 16 to 24, said method comprising following steps : (a) emitting an electromagnetic source signal of one or more particular base frequencies to said substrate so that any present magnetic elongated particles go into a non-linear part of their B-H curve for at least part of a cycle of the source signal ; (b) detecting an electromagnetic detection signal emanating from said substrate ; (c) testing the detection signal for the presence of particular higher harmonics of said base frequencies or of any linear combination of said base frequencies and of said harmonics, said particular higher harmonics being indicative of the presence of said magnetic particles. 26. A method according to claim 25 wherein said source signal has only one base frequency. 27. A method according to claim 26 wherein said base frequency is higher than 1 kHz. 28. A method according to anyone of claims 25 to 27 wherein said particular higher harmonics have a frequency higher than 10 kHz. 29. A method according to claim 28 wherein said particular higher harmonics are of the order of ten or higher. 30. A method according to claim 25 or 26 wherein sait particular higher harmonics is of the order of 19 and has a frequency of 380 kHz. 31. .A method according to anyone of claims 25 to 26 wherein, in addition to said electromagnetic source signal, microwaves are emitted to said substrate to detect the presence of any present magnetic elongated particles. 32. A method according to anyone of the preceding claims wherein said method comprises the following additional step : d) generating a signal which prevents from taking a true copy in case said particular harmonics are present.

Inventors: BURRELL JONATHAN, DOUBLET PIERRE, FISHER JOHN, ROBERTSON PAUL ANDREW, BURRELL, JONATHAN, DOUBLET, PIERRE, FISHER, JOHN, ROBERTSON, PAUL, ANDREW
Applicants: ARJO WIGGINS SA, BEKAERT SA NV, ARJO WIGGINS S.A., N.V. BEKAERT S.A.
Application year: 1997
Main classification: G07D7
IPC codes: B42D15, B42D107, G06K7, G07D7, G07F7, H01F1