First of all, the entire grounds themselves are beautiful. Walking down the stairway into the villas is about as picturesque as we could've imagined. At check-in, Elias gave us a great overview of Santorini on a map, highlighting some of the activities and places we may want to visit. We took him up on several - whether it was the ATV rental to go visit the south of the island (great beaches) to dinner recommendations - and he did not lead us astray. Although the rooms do not face the sunset/caldera, it is just a short walk (2min) up to the main caldera path that will take you from Firostefani to Fira or Imerovigli, with tons of great restaurants and shops in between all of them.
As someone that didn't want to deal with as many tourists in Fira or Oia, this was the most perfect place to stay. Firostefani has all the amenities you need, and is only a 10 min walk to Fira on the main road, or ~20 minutes on the scenic caldera path. Although still a somewhat busy area, we were always refreshed coming back to our little oasis at the Villas to get away from shoulder to shoulder crowds. 10/10 would highly recommend.