National Bureau of Staadards

Library, K.W. Bldg

JUIM ? P 1964

NBS MONOGRAPH 34—Volume 2

Tables of Chemical Kinetics

Homogeneous Reactions

(Supplementary Tables)

U.S. DEPARTMENT OF COMMERCE

NATIONAL BUREAU OF STANDARDS
Tables of Chemical Kinetics

Homogeneous Reactions

(Supplementary Tables)

These tables are issued in the form of punched loose sheets, temporarily assembled

under a paper cover. This cover can be removed at the discretion of the subscriber

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loose-leaf binder.

Each table is designated by a six-digit number, the first two of which refer to the

type of reaction, the third to the phase of the homogeneous reaction, gaseous (1), liquid

(2), or solid (3). The indication of the phase is repeated at the upper right-hand

corner of the first sheet of each table. The second three-digit group of the table number

refers to the types of substances involved. Within each table, reactions are numbered.

In tables including more than one page, the table number is repeated at the head of

each page, and the pages are numbered. Each table starts on a new sheet.

Earlier tables in this series were published as Circulars of the National Bureau of

Standards. The present tables on this subject will appear in the NBS Monograph

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Monograph 34

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. 35

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*

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For sale by the Superintendent of Documents, U.S. Government Printing Office Washington, D.C., 20402 - Price $2.00
UNITED STATES DEPARTMENT OF COMMERCE • Luther H. Hodges, Secretary

NATIONAL BUREAU OF STANDARDS • A. V. Astin, Director

Tables of Chemical Kinetics

Homogeneous Reactions

(Supplementary Tables)

National Bureau of Standards

A. V. Astin, Director

National Research Council, Division of Chemistry

Committee on Kinetics of Chemical Reactions

M. L. Kilpatrick, Chairman

J. Bigeleisen H. Taube

R. Noyes M. Wallenstein

C. Satterfield

Project Office: Hepburn Hall, St. Lawrence University, Canton, New York

C. H. Stauffer, Project Director

A. R. Amell D. M. Kern

E. Buncel H. G. Kuivila H. B. Feldman P. E. Merritt H. S. Johnston H. Taube

National Bureau of Standards Monograph 34 —Vol. 2

To Accompany National Bureau of Standards C510, Supplements 1 and 2,

and Monograph 34—Vol. 1

Issued July 1, 1964
Library of Congress Catalog Card Number : 52-60566

II
Preface

These tables have been prepared and organized as a supplement to the tables of chemical

kinetics in National Bureau of Standards Circular 510, Supplement 1 to National Bureau of Standards Circular 510, and National Bureau of Standards Monograph 34. Code abbreviations for literature references, definitions of symbols and quantities used in the tables are given

in the introduction of NBS Circular 510. A brief description of the method used in compiling

these tables and the limitation of coverage are given in the preface to Supplement 1 of the

NBS Circular 510. A description of the numbering system used in classifying reactions for the tables and an index are given in Supplement 2 of the NBS Circular 510.

The present volume contains information pertaining to substitution, exchange, and ehmination reaction types and extends the material on these reaction types found in NBS Monograph 34, Volume I. The date on each page gives the year and month to which the literature

had been surveyed. Significant omissions or errors should be reported to the Director of the

Project: Dr. Charles H. Stauffer, Head, Department of Chemistry, St. Lawrence University,

Canton, New York.

The Director of the Project and his associates gratefully acknowledge the financial assist- ance provided by the Office of Ordnance Research, Department of the Army, Office of Naval

Research, Atomic Energy Commission, National Science Foundation, and the National Bureau

of Standards to make the compilation of these data possible. The Director of the Project

gratefully acknowledges the able assistance of his associates and collaborators in the review

and analysis of the material in the chemical literature. He also acknowledges the assistance

of the staff of the National Academy of Sciences and of the members of the Committee on Chemical Kinetics of the National Academy of Sciences, Division of Chemistry.

C. H. Stauffer
Contents

(Supplementary Tables)

Page Preface iii

Subject index iv

Tables 1
Homogeneous Reaction Kinetics

SUBJECT INDEX

EXCHANGE-SUBSTITUTION

300 ISOTOPIC EXCHANGE lllie 01 laDI6 1 a D 1 e 302 IsDtpic exchang ,,. .,, (number of paqes)

2 (liquid) ^ km; number

I so topic exchange carbon-Isotope exchange (5) 302.440

It II halogen on ivth group hallde (1) 302.474

II II halogen Isotope exchange between ivth group and

Vth group atoms (2) 302.475

n II exchange of oxygen on vth group element (3) 302.560

n 11 halogen exchange between vth group halldes (1) 302.575

II II Vth group elements between oxidation states (2) 302. 590

ti 11 Og exchange with HgO and HgO^ (1) 302.600

11 II

, hydrogen, exchange with water (1) 302.601

n II VI th group cyanide complex with CN~ (1) 302.640

11 II VI th group NHg complex with NHg (1) 302.650

n II exchange Involving VI th group element as central atom m both reactants (9) 302.660

II VI th group central element complexed with

exchanging VII th group Ions (1) 302.670

II Vlth group element between oxidation states (1) 302. 690

n Vlth group element Involving complexed valence

states (2) 302.696

n II cyanide Ion with VII th group cyanide complex (1) 302.740

11 II PYch^inffp of nyvfTPD flttached tn VTTth ffTmin el pmpnt (2) 302.760

II II Vllth group element between oxidation states (3) 302.790

II II N-bonded complex exchanging on Vlllth group element (2) 302.850

n n

; Vlllth group Ion exchange with N-bonded complex (6) 302.858

II II

; 0-bonded complex exchanging on villth group element 12;

II n

; halogen Ion exchange on villth group complex

II 11

; Vlllth group element between oxidation states 0\J (C • O C7 U

310 HYDROGEN SUBSTITUTION

312 Hydrogen substitution (liquid)

Hydro gen substitution; hydrogen substitution by oxygen (alkoxy)

(phenoxy) on boron hydrides (5) 312.301

N II ; hydrogen replacing ivth group element on aromatic C

n II ; H on aliphatic C with group I metal (1) 312.411

11 n

; hydrogen replacing halogen on aliphatic c (1) 312.417

n II ; H on aromatic C replaced by C. Aromatic

alkylatlon (26) 312.442

II II ; H on nitrogen replaced by NC^ (2) 312.552

EXCHANGE OF SUBSTITUENTS

332 Exchange of substituents (liquid)

Exchange Of substituents; Ilnd group metal on aliphatic C exchange (1) 332.221

II n " ; Ilnd group metal on aromatlc-C replaced

by N (1) 332.252

II II II ; iind group metal on aliphatic C replaced

by acid radical (3) 332.261

1

2S

1-3

National Bureau of Standards - National Research Council December, I96O
Homogeneous Reaction Kinetics

SUBJECT INDEX ( continued)

Title of Tab I e 330 EXCHANGE OF SUBSTITUENTS (continued) (number of pages)

332 Exchange of substituents (liquid)

Exchange of substituents; vth group element on aliphatic C replaced by c

" "" ; N02{N0g) replaced by N on aliphatic or

aromatic C

" "" ; ROSO^ on aliphatic c replaced by R'S

" " " ; SO " on aromatic C replaced by halogen

3

" " "

; halogen for halogen on aromatic carbon

" " " ; halogen exchange for halogen on ivth

group element

(1)

(1)

(2)

(2)

(5)

(2)

T ab I e number

332.541

332.551

332.661

332.672

332.772

332.774

380 COORDINATIVE EXCHANGE

382 Coordinative exchange (liquid)

exchange; HgO replaced by N compound In Group I complex (1) 382. 105 HgO or solvent replacing N compound on Group i complex (solvent not always shown on equation) (2) 382. 150 HgO replacing halogen on Group i complex (1) 382. 170

" ' HgO replacing N compound In Group ll complex (1) 382.250

" ' H^O (oh ) exchange with halogen on Group V

c omp lex (2) 382. 570

n

* C compound replacing H^o In Group VI complex (0 382.604

n

• N-compound replacing H^o on Group VI complex (2) 382.605

" ' HgO (HgO"*^ replacing C-compound on Vlth group complex (1) 382.640

HgO (HgO^ (0H~) replacing N-compound on Vlth group complex (4) 382.650

II halogen replaced by h^o (HgO"*") (0H~) on Vlth group complex (H^o not always shown In complex) (3) 382.670

II HgO or 0H~ replacing carboxylate In VIII th group complex (2) 382.800

II N-compound replacing H^o In villth group complex

(HgO not always shown In formula of complex) (5) 382.805

II S compound replacing H^o In Vlllth group complex

(H^O not always shown) (2) 382.806

II halogen replacing H^o In Vlllth group complex (2) 382.807

n Ho replacing (CN~) (SCN") (CO ") on Vlllth group complex (2) 382.840

II N or p-compound replacing a c-compound In VIII th group complex (1) 382.845

II H20(0H ) replacing N compound In Vlllth complex

(H^O not always shown In formula of complex) (11) 382.850

II N or P-compound replacing n or p-compound In Vlllth group complex (5) 382.855

II » S-compound replacing N-compound In villth group complex (1) 382.856

National Bureau of Standards - National Research Council December, I960
Homogeneous Reaction Kinetics

SUBJECT INDEX (continued)

Title of Tab I

e

380 COORDINATIVE EXCHANGE (continued) (number of pages)

382 Coordinative exchange (liquid)

Coordlnatlve exchange; H^o replacing S-compound In Vlllth group complex (1) 382.860

N-compound replacing S-compound In Vlllth

group complex (l) 382.865

HgO, 0H~ or 0R~ replacing halogen In villth

group complex (H^O not always shown In complex) (22) 382.870

N-compound replacing halogen In Vlllth group complex (6) 382.875

ROH, RCOO~, CO ~ or S compound replacing

3 halogen In Vlllth group complex (2) 382.876

Halogen replacing halogen In Vlllth group complex (l) 382.877

4oo ELIMINATION

400 PROTON ELIMINATION

CO U02 Proton elimination (liquid) • c

Proton elimination; proton elimination from OH-hond (Carboxyllc acids

a"C3

and phenols, Ionization and recombination) (3) 402.461 a

420 BOND-UNSATURATION ELIMINATION

1422 Bond-unsaturation elimination (liquid) Co

05 Bond-unsaturation elimination; Hg(ll) from ethylenic addition O

compound (5) 422.421

430 RING-CLOSURE ELIMINATION

U32 Ring-closure elimination (liquid)

Ring-closure elimination; elimination of hydrogen hallde from halohydrins with ring closure (8) 432.471

H " ; elimination of hydrogen hallde, or hallde

ion to form N-containlng ring (11) 432.475

National Bureau of Standards - National Research Council Decerrber, I96O

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