AQS Site ID State County Latitude Longitude Sulfates Nitrates Crustal OC

010730023 AL Jefferson 33.55306 -86.815 3.7 0.8 1.1 3.0

010732003 AL Jefferson 33.49972 -86.9242 3.4 0.8 1.5 4.0

010890014 AL Madison 34.68767 -86.5864 3.3 1.0 0.6 3.1

011011002 AL Montgomery32.40712 -86.2564 3.3 0.6 0.7 3.5

011130001 AL Russell 32.47678 -84.9991 3.2 0.7 0.6 4.8

040191028 AZ Pima 32.29515 -110.982 1.2 0.6 1.3 1.5

051190007 AR Pulaski 34.75619 -92.2813 2.9 1.0 0.9 3.2

060070002 CA Butte 39.75737 -121.843

060070008 CA Butte 39.76154 -121.842

060190011 CA Fresno 36.78532 -119.774 1.6 4.9 0.8 4.6

060250005 CA Imperial 32.67619 -115.484 1.6 1.6 2.9 4.8

060371103 CA Los Angeles 34.06659 -118.227

060631009 CA Plumas 39.80833 -120.472 0.7 0.5 0.7 11.6

060670006 CA Sacramento38.61378 -121.368 1.1 2.1 0.5 3.7

060670010 CA Sacramento38.55823 -121.493 1.1 2.3 0.6 3.3

060730003 CA San Diego 32.79119 -116.942 2.1 2.8 0.6 3.4

060731002 CA San Diego 33.12771 -117.075 2.2 2.7 0.6 3.7

060850005 CA Santa Clara 37.3485 -121.895 1.2 2.1 0.4 3.3

060990005 CA Stanislaus 37.64158 -120.995 1.5 4.8 0.8 3.8

061072002 CA Tulare 36.33218 -119.291 1.9 6.1 1.0 4.6

061112002 CA Ventura 34.27574 -118.685 1.8 2.5 0.8 2.4

080010006 CO Adams 39.82601 -104.937 1.0 1.4 1.5 2.4

080310025 CO Denver 39.70401 -104.998

080310026 CO Denver 39.77949 -105.005

110010043 DC District of Columbia 38.92185 -77.0132 3.3 1.5 0.5 2.9

120111002 FL Broward 26.08314 -80.2376 2.3 0.6 1.1 1.2

120573002 FL Hillsborough27.96565 -82.2304 2.6 0.6 0.8 2.3

120730012 FL Leon 30.43972 -84.3464 2.7 0.4 0.6 3.8

130210007 GA Bibb 32.77745 -83.6411 3.0 0.5 1.1 4.7

130890002 GA DeKalb 33.68797 -84.2905 3.0 0.6 0.5 3.7

131150003 GA Floyd 34.26054 -85.3233 3.5 0.6 0.7 4.1

132150011 GA Muscogee 32.42905 -84.9316 3.1 0.5 0.6 4.6

081230008 CO Weld 40.20939 -104.824 1.0 1.8 1.6 1.8

090090027 CT New Haven 41.3014 -72.9029 2.3 1.3 0.4 2.6

100010003 DE Kent 39.155 -75.5181 2.9 1.7 0.3 2.1

100032004 DE New Castle 39.73944 -75.5581 3.5 2.5 0.5 2.9

201730010 KS Sedgwick 37.70207 -97.3148 2.2 1.8 1.1 2.2

202090021 KS Wyandotte 39.11722 -94.6356 2.4 1.9 0.9 3.6

210190017 KY Boyd 38.45934 -82.6404 4.0 1.0 0.5 3.4

210430500 KY Carter 38.23887 -82.9881 3.9 0.6 0.3 2.2

2010-2012 3-Year Ave

Speciation Measurements
210670012 KY Fayette 38.06503 -84.4976 4.0 1.6 0.5 2.7

211170007 KY Kenton 39.0725 -84.525

220330009 LA East Baton Rouge 30.46198 -91.1792 3.6 0.9 1.0 3.1

240053001 MD Baltimore 39.31083 -76.4744 3.4 1.8 0.4 3.3

240330030 MD Prince George's 39.05528 -76.8783 3.1 1.1 0.5 2.5

250130008 MA Hampden 42.19438 -72.5551 2.0 0.9 0.2 2.7

260810020 MI Kent 42.98417 -85.6713 2.6 2.5 0.5 2.9

260910007 MI Lenawee 41.99557 -83.9466 3.0 2.6 0.3 2.2

261130001 MI Missaukee 44.31056 -84.8919 1.9 1.0 0.2 1.5

261150005 MI Monroe 41.76389 -83.4719 3.2 2.5 0.4 2.4

261470005 MI St. Clair 42.95334 -82.4562 2.7 1.8 0.3 2.5

261630001 MI Wayne 42.22862 -83.2082 3.0 2.4 0.5 2.5

261630015 MI Wayne 42.30279 -83.1065 3.5 2.5 1.1 2.8

261630033 MI Wayne 42.30667 -83.1488 2.9 2.3 1.4 3.1

270031002 MN Anoka 45.13768 -93.2076

270530963 MN Hennepin 44.95366 -93.2582 1.7 2.4 0.6 2.5

271095008 MN Olmsted 43.99691 -92.4504

280490019 MS Hinds 32.33037 -90.1662

280670002 MS Jones 31.68864 -89.1351 3.3 0.7 0.9 4.0

132450091 GA Richmond 33.43335 -82.0222 3.1 0.7 0.6 4.1

132950002 GA Walker 34.97889 -85.301 3.1 0.7 0.5 4.5

150030010 HI Honolulu 21.32374 -158.089

160010010 ID Ada 43.6007 -116.348 0.7 1.3 0.8 2.8

170310057 IL Cook 41.91286 -87.7227 3.1 3.4 0.9 3.5

170310076 IL Cook 41.7514 -87.7135 2.7 2.7 0.5 2.7

170314201 IL Cook 42.14 -87.7992 2.8 2.8 0.5 2.6

170434002 IL DuPage 41.77107 -88.1525 2.8 2.8 0.5 2.7

171190024 IL Madison 38.70063 -90.1448

180190006 IN Clark 38.27768 -85.7402 4.4 1.7 0.9 3.5

180372001 IN Dubois 38.39144 -86.9292 4.3 2.4 0.5 2.9

180390008 IN Elkhart 41.6569 -85.9684 2.9 2.9 0.4 3.2

180650003 IN Henry 40.00953 -85.5235 3.3 2.7 0.3 2.1

180890022 IN Lake 41.60668 -87.3047 3.3 2.9 1.0 3.0

180892004 IN Lake 41.5855 -87.4745

180970078 IN Marion 39.8111 -86.1145 3.6 2.7 0.5 3.1

181630021 IN Vanderburgh38.01325 -87.5779 4.0 1.9 0.5 3.0

300490004 MT Lewis and Clark 46.85051 -111.987

300930005 MT Silver Bow 46.0024 -112.501

310550019 NE Douglas 41.24749 -95.9731 2.3 2.7 1.2 2.0

320030540 NV Clark 36.14347 -115.079

320310016 NV Washoe 39.52508 -119.808 0.7 0.9 0.8 2.7

340130003 NJ Essex 40.72099 -74.1929 2.7 1.7 0.4 3.3

340273001 NJ Morris 40.78763 -74.6763 2.4 1.1 0.2 1.8

340390004 NJ Union 40.64144 -74.2084 2.9 1.9 0.7 3.1
350010023 NM Bernalillo 35.1343 -106.585 0.9 0.6 1.0 2.3

360010005 NY Albany 42.64225 -73.7546 2.2 1.2 0.5 2.7

360050110 NY Bronx 40.81618 -73.902

360310003 NY Essex 44.39308 -73.8589

360551007 NY Monroe 43.14618 -77.5482 2.4 1.5 0.3 1.9

361010003 NY Steuben 42.09142 -77.2098 2.6 0.9 0.2 1.5

370210034 NC Buncombe 35.6075 -82.5833 3.2 0.6 0.4 2.9

370350004 NC Catawba 35.72889 -81.3656 3.1 1.0 0.4 3.8

370570002 NC Davidson 35.81444 -80.2625 3.1 0.9 0.4 3.8

370670022 NC Forsyth 36.11056 -80.2267 3.1 1.0 0.4 3.2

371190041 NC Mecklenburg 35.2401 -80.7857 3.2 0.9 0.5 3.5

371590021 NC Rowan 35.55187 -80.395 3.1 0.8 0.4 3.5

371830014 NC Wake 35.85611 -78.5742 3.2 0.8 0.5 3.5

380171004 ND Cass 46.93375 -96.8554 1.4 1.7 1.5 1.4

390610040 OH Hamilton 39.12886 -84.504 4.0 2.1 0.5 2.7

390811001 OH Jefferson 40.32207 -80.6063 4.8 1.6 0.5 3.1

390870012 OH Lawrence 38.50811 -82.6593 4.0 1.1 0.8 3.2

390933002 OH Lorain 41.46307 -82.1143 3.1 2.0 0.7 2.8

390950026 OH Lucas 41.62063 -83.6423 3.3 2.5 0.5 2.5

390990014 OH Mahoning 41.09594 -80.6585 3.3 1.9 1.1 2.8

391130032 OH Montgomery39.76066 -84.1877 3.7 2.5 0.5 3.0

391351001 OH Preble 39.83562 -84.7205

391510017 OH Stark 40.78688 -81.3942 3.5 2.4 1.0 3.2

391530023 OH Summit 41.08796 -81.5416 4.4 2.6 0.4 2.8

401091037 OK Oklahoma 35.61413 -97.4751 2.4 1.5 0.9 2.1

401431127 OK Tulsa 36.2049 -95.9765 2.9 1.5 0.9 2.9

410350004 OR Klamath 42.1903 -121.731

410370001 OR Lake 42.18922 -120.354

410392013 OR Lane 43.74435 -122.48

420110011 PA Berks 40.38335 -75.9686 3.2 2.6 0.3 2.6

420210011 PA Cambria 40.30972 -78.915

420270100 PA Centre 40.81139 -77.877 3.1 1.3 0.3 2.2

420290100 PA Chester 39.83446 -75.7682

420430401 PA Dauphin 40.24699 -76.847

420710007 PA Lancaster 40.04667 -76.2833 3.3 2.9 0.3 3.1

420950025 PA Northampton40.62806 -75.3411

421010055 PA Philadelphia39.92252 -75.1868 3.4 2.1 0.5 3.0

421011002 PA Philadelphia40.03598 -75.0024

421255001 PA Washington40.44528 -80.4208

421290008 PA Westmoreland40.30469 -79.5057

421330008 PA York 39.96528 -76.6994 3.4 2.4 0.6 3.0

440070022 RI Providence 41.80778 -71.4151

440071010 RI Providence 41.84157 -71.3608

450190049 SC Charleston 32.79098 -79.9587
450250001 SC Chesterfield34.61537 -80.1988 3.1 0.6 0.4 2.9

450450015 SC Greenville 34.8439 -82.4146 3.2 0.8 0.5 4.0

450790007 SC Richland 34.09396 -80.9623

460990008 SD Minnehaha 43.54792 -96.7008 1.9 2.3 0.6 1.7

470370023 TN Davidson 36.17633 -86.7389 3.5 1.3 0.5 3.2

470654002 TN Hamilton 35.05093 -85.293 3.5 0.8 0.7 4.0

470931020 TN Knox 36.01919 -83.8738 3.5 0.7 0.5 3.4

470990002 TN Lawrence 35.11597 -87.47 3.0 0.7 0.7 2.5

471251009 TN Montgomery36.51471 -87.328 3.5 1.3 0.5 2.9

471451001 TN Roane 35.91676 -84.5036

481130069 TX Dallas 32.81995 -96.8601 2.9 1.2 1.2 2.6

481410044 TX El Paso 31.7657 -106.455 1.3 0.7 2.9 2.6

482030002 TX Harrison 32.66899 -94.1675 2.9 0.5 0.9 4.0

490110004 UT Davis 40.90297 -111.884 0.9 2.2 0.8 1.8

490353006 UT Salt Lake 40.73639 -111.872 1.0 2.6 1.0 2.3

490494001 UT Utah 40.34139 -111.714 0.9 2.5 1.0 2.0

500070012 VT Chittenden 44.48028 -73.2144 1.6 1.0 0.4 2.5

510870014 VA Henrico 37.55652 -77.4003 3.3 0.9 0.4 3.1

530110013 WA Clark 45.64833 -122.587 0.9 0.7 0.3 3.7

530530029 WA Pierce 47.1864 -122.452 1.0 0.7 0.3 3.9

530611007 WA Snohomish 48.05432 -122.172

530770009 WA Yakima 46.59806 -120.499

540391005 WV Kanawha 38.36618 -81.6937 4.0 1.1 0.6 3.5

540511002 WV Marshall 39.91596 -80.7339

540690010 WV Ohio 40.11488 -80.701

550090005 WI Brown 44.507 -87.993

550270001 WI Dodge 43.46611 -88.6211 2.1 2.3 0.4 1.9

550790026 WI Milwaukee 43.061 -87.912 2.4 2.5 0.4 2.4

551198001 WI Taylor 45.20389 -90.6001 1.8 1.6 0.3 1.7

551330027 WI Waukesha 43.02008 -88.2151 2.4 2.5 0.7 2.6

 * These data were derived with the SANDWICH algorithm to represent PM2.5 composition. For simplification purposes, th
EC Sulfates Nitrates Crustal OC EC Sulfates Nitrates Crustal

0.8 4.5 0.1 1.1 6.9 0.8 3.9 0.9 1.2

0.7 4.1 0.1 1.5 5.9 0.8 3.6 0.8 1.8

0.5 4.1 0.3 0.6 5.2 0.5 3.6 1.2 0.7

0.6 3.9 0.0 0.8 5.4 0.6 3.5 0.7 1.0

0.8 3.9 0.1 0.6 6.9 0.8 3.5 0.9 0.7

0.4 1.5 0.0 1.4 1.7 0.5 1.0 0.6 0.9

0.6 3.5 0.3 0.9 6.1 0.6 3.0 1.1 0.9

0.7 1.0 0.6

0.8 2.0 3.0 0.8 7.5 0.8 1.7 4.7 0.7

0.8 2.0 0.2 3.0 8.4 0.9 1.6 1.4 2.0

2.6 4.1 0.9

1.0 0.8 0.1 0.7 8.5 1.1 0.5 0.4 0.8

0.7 1.4 1.0 0.6 5.7 0.7 1.2 2.3 0.6

0.6 1.4 1.2 0.6 4.6 0.6 0.9 2.3 0.6

0.8 2.6 0.4 0.6 6.2 0.8 2.1 3.0 0.5

0.6 2.7 0.3 0.6 5.9 0.6 2.1 3.0 0.6

0.6 1.6 0.6 0.5 6.0 0.6 1.3 2.0 0.4

0.6 1.9 3.4 0.8 5.4 0.6 1.5 4.2 0.9

0.6 2.4 3.6 1.1 6.5 0.6 1.6 4.8 0.9

0.5 2.3 0.3 0.8 5.2 0.5 1.7 2.5 0.5

1.0 1.3 0.8 1.6 2.8 1.0 1.1 1.6 1.3

1.2 1.9 1.0

0.7 4.2 0.6 0.5 4.4 0.7 4.0 1.7 0.5

0.4 3.1 0.0 1.2 2.1 0.4 2.6 0.8 1.0

0.4 3.3 0.0 0.9 2.9 0.5 2.9 0.6 0.8

0.7 3.2 0.0 0.6 4.8 0.7 2.9 0.5 0.8

0.7 3.6 0.1 1.2 7.4 0.8 3.4 0.7 1.3

1.2 3.6 0.1 0.5 6.0 1.3 3.3 0.8 0.6

1.2 4.1 0.1 0.7 6.4 1.2 4.0 0.8 0.9

0.6 3.7 0.1 0.6 6.5 0.6 3.5 0.7 0.9

0.6 1.2 0.8 1.7 2.9 0.6 1.0 2.1 1.6

1.0 2.9 0.4 0.4 4.0 1.0 2.2 1.2 0.4

0.4 3.7 0.9 0.3 3.0 0.4 3.7 2.0 0.4

0.7 4.2 1.4 0.5 3.7 0.8 4.2 3.3 0.5

0.4 2.7 1.2 1.1 3.1 0.4 2.2 1.7 0.9

0.6 2.9 1.2 0.9 4.0 0.6 2.4 2.1 0.9

0.7 4.8 0.5 0.5 4.2 0.7 4.6 1.4 0.5

0.4 4.5 0.3 0.3 3.6 0.4 5.0 0.9 0.3

2010-2012 3-Year Average

SANDWICHed* Speciation Measurements
0.5 5.0 0.8 0.6 3.5 0.6 4.7 2.1 0.5

0.7 4.4 0.0 1.1 4.2 0.7 3.8 1.0 1.2

0.8 4.2 0.9 0.4 4.6 0.8 3.7 1.9 0.5

0.6 3.7 0.5 0.5 3.5 0.6 3.5 1.4 0.6

0.5 2.4 0.4 0.3 4.1 0.6 2.0 0.8 0.3

0.6 3.2 1.8 0.5 3.5 0.6 2.7 2.8 0.6

0.4 3.6 1.8 0.3 3.2 0.4 3.1 2.7 0.4

0.2 2.4 0.7 0.2 2.5 0.2 1.9 0.8 0.2

0.6 4.0 1.7 0.5 3.0 0.6 3.2 2.9 0.4

0.4 3.4 1.0 0.4 3.7 0.5 2.6 1.5 0.4

0.8 3.7 1.6 0.5 3.4 0.8 3.0 2.4 0.5

0.8 4.3 1.6 1.1 2.9 0.9 3.8 2.8 1.1

0.8 3.6 1.5 1.5 3.7 0.8 3.0 2.3 1.3

0.5 2.1 1.8 0.6 3.6 0.5 1.8 2.5 0.6

1.9 3.0 0.5

0.7 4.0 0.1 1.0 5.8 0.7 3.3 0.9 1.3

0.6 3.8 0.1 0.6 6.4 0.6 3.9 0.9 0.7

0.7 3.7 0.1 0.5 5.5 0.7 3.3 1.0 0.6

0.5 1.0 0.7 0.9 3.5 0.6 0.7 1.2 0.9

0.8 3.7 2.4 0.9 4.7 0.9 3.2 4.3 0.8

0.7 3.4 1.8 0.5 4.8 0.8 2.8 3.0 0.5

0.6 3.4 2.1 0.5 4.0 0.6 3.0 3.3 0.5

0.6 3.4 2.1 0.5 4.2 0.6 3.0 3.5 0.6

3.7 2.4 2.6

0.8 5.4 0.9 0.9 4.8 0.8 4.9 2.3 0.8

0.5 5.3 1.4 0.5 4.6 0.6 4.9 3.0 0.4

0.6 3.6 2.1 0.4 4.5 0.6 3.0 3.6 0.4

0.5 4.1 1.7 0.3 3.8 0.5 3.5 3.7 0.3

1.1 4.0 2.3 1.0 4.6 1.1 3.4 3.4 1.0

3.5 3.6 0.7

0.7 4.4 1.8 0.5 4.4 0.7 3.8 3.4 0.5

0.5 4.9 1.1 0.6 4.7 0.6 4.5 2.4 0.6

0.4 2.8 2.2 1.2 3.2 0.4 2.5 3.3 1.2

0.7 0.9 0.4 0.8 3.4 0.7 0.6 1.0 0.8

0.9 3.4 0.6 0.5 3.9 0.9 2.7 1.4 0.4

0.4 3.1 0.3 0.3 3.1 0.4 2.8 1.0 0.3

1.6 3.6 0.8 0.7 4.3 1.6 3.0 1.8 0.8
0.6 1.2 0.1 1.1 3.3 0.6 0.8 0.7 0.7

0.7 2.7 0.7 0.6 3.7 0.7 2.5 1.2 0.5

0.5 2.9 0.9 0.4 3.7 0.6 2.4 1.4 0.4

0.2 3.2 0.4 0.2 3.0 0.3 3.2 0.9 0.2

0.5 3.8 0.1 0.4 4.4 0.6 3.7 0.7 0.5

0.8 3.8 0.3 0.4 5.2 0.8 3.8 1.3 0.5

0.7 3.8 0.2 0.5 5.7 0.7 3.7 1.1 0.5

0.6 3.8 0.3 0.4 3.8 0.6 4.0 1.2 0.5

0.6 3.8 0.2 0.5 5.1 0.6 3.8 1.1 0.5

0.5 3.8 0.2 0.4 5.2 0.5 3.8 1.0 0.5

0.6 3.9 0.2 0.5 4.7 0.6 3.8 0.9 0.5

0.3 1.8 1.3 1.7 2.9 0.3 1.6 1.8 1.6

0.7 4.9 1.3 0.5 4.6 0.7 4.4 2.5 0.4

0.9 5.7 0.8 0.5 3.0 0.9 4.9 1.8 0.5

0.8 4.6 0.5 0.8 4.8 0.9 5.0 1.5 0.7

0.6 3.8 1.3 0.7 3.6 0.6 3.1 2.2 0.6

0.6 4.0 1.8 0.5 3.9 0.6 3.1 2.8 0.6

0.7 4.1 1.3 1.1 3.6 0.8 3.9 2.5 1.2

0.7 4.6 1.6 0.5 4.3 0.8 3.9 3.4 0.5

0.8 4.3 1.6 1.1 4.6 0.8 3.8 3.2 1.3

0.7 5.2 1.7 0.5 3.4 0.7 4.0 2.7 0.4

0.4 2.9 0.8 0.9 4.2 0.4 2.4 1.5 0.7

0.4 3.4 0.8 1.0 5.0 0.5 2.9 1.6 0.9

0.5 0.6 0.5

0.5 0.2 0.8

0.4 0.1 0.3

0.6 4.0 1.4 0.3 4.3 0.7 3.5 2.6 0.3

4.5 1.5 1.1

0.4 3.8 0.6 0.3 3.3 0.4 3.3 1.3 0.3

0.7 4.1 1.5 0.3 4.8 0.7 3.6 3.0 0.3

0.9 4.2 1.0 0.5 4.3 1.0 3.4 2.2 0.5

0.7 4.2 1.4 0.6 4.4 0.8 3.7 2.4 0.6

3.5 0.7 0.6
0.4 3.7 0.1 0.4 4.6 0.4 3.8 0.8 0.4

0.7 3.9 0.2 0.5 5.7 0.7 3.8 1.0 0.6

0.3 2.3 1.7 0.7 3.9 0.3 2.2 2.9 0.6

0.8 4.3 0.6 0.6 4.5 0.8 3.7 1.7 0.6

0.8 4.2 0.1 0.7 5.1 0.8 3.8 1.0 0.7

0.7 4.1 0.1 0.5 5.6 0.8 4.1 0.8 0.5

0.3 3.7 0.1 0.8 3.7 0.3 3.2 0.7 1.0

0.4 4.3 0.6 0.5 4.2 0.4 3.8 1.8 0.5

3.6 0.6 0.5

0.6 3.5 0.3 1.3 4.2 0.7 2.8 1.3 1.1

0.8 1.6 0.1 3.0 4.7 0.8 1.1 0.8 2.4

0.6 3.5 0.0 0.9 5.9 0.6 3.2 0.5 0.8

0.5 1.2 1.8 0.9 3.4 0.5 0.9 2.4 0.7

0.6 1.3 2.2 1.1 3.6 0.7 1.0 3.4 1.2

0.5 1.2 2.0 1.1 3.5 0.5 0.9 2.9 1.1

0.4 2.1 0.6 0.4 3.7 0.4 1.8 1.0 0.3

0.6 4.1 0.2 0.4 4.0 0.6 4.0 1.0 0.4

0.7 1.2 0.1 0.4 4.7 0.7 0.9 0.6 0.3

0.8 1.3 0.1 0.3 5.2 0.8 1.1 0.7 0.3

1.0 0.7 0.3

1.0 4.8 0.4 0.6 5.0 1.0 4.8 1.5 0.6

4.8 1.9 1.1

0.3 2.6 1.6 0.4 4.2 0.3 2.2 2.4 0.3

0.5 3.0 1.7 0.5 4.5 0.6 2.5 2.5 0.5

0.2 2.2 1.2 0.3 3.5 0.3 1.6 1.4 0.3

0.6 2.9 1.8 0.7 5.2 0.6 2.5 2.9 0.7

n. For simplification purposes, the SANDWICH component called "passive" (which is nominally 0.5 ug/m3) was allocated in proportion to 
OC EC Sulfates Nitrates Crustal OC EC Sulfates Nitrates

3.6 1.0 4.9 0.2 1.3 7.0 1.1 4.0 0.8

4.0 0.8 4.3 0.2 1.9 5.5 0.8 3.8 0.8

3.1 0.5 4.5 0.5 0.7 5.1 0.5 3.6 0.9

3.5 0.7 4.2 0.1 1.1 5.0 0.7 3.6 0.5

5.1 0.9 4.3 0.3 0.7 7.1 0.9 3.6 0.5

1.6 0.4 1.3 0.1 1.0 2.0 0.5 1.3 0.6

3.6 0.7 3.7 0.4 0.9 6.3 0.7 3.1 1.1

4.4 0.7 1.0 0.3 0.7 4.5 0.7 1.1 1.8

4.3 0.7 2.1 2.9 0.7 6.8 0.8 1.6 5.5

4.0 0.7 2.0 0.2 2.0 7.9 0.7 1.6 1.6

8.3 1.5 3.3 0.9 0.9 4.9 1.6

9.7 1.0 0.7 0.0 0.9 6.4 1.1 0.7 0.4

3.4 0.7 1.5 1.2 0.6 4.8 0.7 1.2 2.5

3.0 0.6 1.2 1.2 0.7 3.7 0.6 1.2 2.9

3.5 0.8 2.7 0.3 0.5 6.5 0.8 2.3 2.9

4.0 0.7 2.8 0.5 0.7 6.0 0.7 2.1 2.7

3.0 0.6 1.7 0.5 0.4 5.7 0.6 1.3 2.2

3.7 0.7 1.9 2.2 1.0 5.2 0.7 1.7 6.7

4.1 0.6 2.1 2.3 0.9 5.8 0.6 2.1 7.2

2.3 0.5 2.2 0.3 0.5 5.2 0.5 1.9 2.5

2.4 1.0 1.4 0.9 1.4 3.2 1.1 1.1 1.3

2.2 0.9 1.5 1.3 1.1 3.1 0.9 1.1 1.4

3.0 0.6 5.0 0.8 0.6 4.4 0.7 3.3 1.4

1.3 0.4 3.3 0.0 1.1 2.2 0.4 2.4 0.6

2.3 0.4 3.5 0.0 0.9 3.2 0.5 2.8 0.6

3.8 0.7 3.4 0.0 0.8 4.9 0.7 2.9 0.4

4.7 0.8 3.9 0.1 1.3 7.8 0.8 3.2 0.4

3.6 1.3 3.9 0.2 0.6 6.2 1.4 3.3 0.5

4.7 0.9 4.8 0.3 0.9 7.0 1.0 3.7 0.5

5.0 0.7 4.1 0.2 0.9 6.8 0.8 3.4 0.4

1.5 0.5 1.3 1.1 1.7 2.6 0.6 1.0 1.8

2.5 0.8 2.8 0.3 0.5 3.8 0.9 2.6 1.3

2.7 0.5 4.6 1.2 0.4 3.8 0.5 2.6 1.7

3.3 0.8 5.0 2.3 0.6 3.1 0.8 3.2 2.0

2.0 0.4 2.7 1.2 1.0 2.8 0.4 2.3 2.0

3.4 0.6 2.9 1.5 0.9 3.6 0.7 2.5 1.8

3.4 0.7 5.7 0.8 0.5 3.6 0.7 4.2 0.9

2.4 0.4 5.8 0.6 0.3 3.4 0.4 3.7 0.5

Speciation Measuremen

2010 Annual Average

tion Measurements SANDWICHed*
2.9 0.6 5.8 1.3 0.6 3.5 0.6 4.3 1.5

3.2 0.7 4.7 0.0 1.3 4.0 0.7 3.9 0.9

3.2 0.7 4.6 1.1 0.5 4.4 0.8 3.4 1.7

2.5 0.6 4.3 0.7 0.6 3.2 0.7 3.0 1.0

2.3 0.4 2.5 0.3 0.3 4.0 0.5 2.1 1.0

3.0 0.6 3.4 2.1 0.6 3.2 0.7 2.5 2.4

2.5 0.4 3.9 2.0 0.4 2.9 0.5 3.1 2.5

1.6 0.2 2.3 0.5 0.2 2.4 0.2 2.0 1.0

2.5 0.6 4.0 2.2 0.5 2.9 0.6 3.4 2.1

2.6 0.4 3.3 0.9 0.4 3.4 0.5 2.6 1.8

2.6 0.8 3.7 1.7 0.5 3.1 0.9 3.2 2.6

3.3 1.0 4.7 2.0 1.1 2.6 1.0 3.3 2.3

3.3 0.8 3.7 1.6 1.4 3.8 0.9 2.9 2.2

1.9 2.3

2.6 0.5 2.3 2.0 0.7 3.5 0.6 1.8 2.4

2.6 0.5 2.4 2.6 0.6 3.5 0.6

3.2 0.7

4.8 0.8 4.2 0.2 1.4 5.6 0.8 3.6 0.7

4.2 0.7 4.9 0.2 0.7 6.4 0.7 2.9 0.6

4.1 0.7 4.0 0.3 0.6 4.3 0.7 3.5 0.5

1.2 0.3

2.0 0.5 0.9 0.6 1.0 1.9 0.5 0.8 1.6

3.7 0.9 4.0 3.4 0.8 4.9 0.9 3.2 3.0

3.0 0.9 3.5 2.2 0.6 4.6 0.9 2.9 2.7

2.8 0.6 3.6 2.6 0.5 3.2 0.7 2.9 2.7

3.0 0.7 3.7 2.8 0.6 4.0 0.7 3.0 2.8

3.3 0.8 4.4 1.7 2.7 5.3 0.8 3.8 1.8

3.7 0.8 6.0 1.6 0.9 5.1 0.8 4.6 1.5

3.1 0.6 6.0 2.2 0.5 4.2 0.6 4.6 2.3

3.6 0.6 3.8 3.0 0.4 4.6 0.6 3.0 2.5

2.6 0.4 4.4 2.8 0.3 4.2 0.4 3.6 2.2

3.3 1.2 4.1 2.8 1.0 4.5 1.2 3.6 3.0

3.2 0.9 4.3 3.0 0.7 4.2 0.9

3.3 0.7 4.7 2.6 0.5 4.4 0.7 4.0 2.4

3.1 0.5 5.5 1.8 0.6 4.3 0.6 4.4 1.7

0.7 0.3

1.9 0.4 3.0 2.9 1.2 2.8 0.4 2.4 2.4

1.0 0.8

2.6 0.7 0.8 0.5 0.8 3.3 0.8 0.7 0.9

3.4 1.0 3.4 0.4 0.4 3.3 1.0 2.9 1.7

2.0 0.4 3.6 0.3 0.3 2.7 0.4 2.5 0.9

2.9 1.5 3.8 0.7 0.9 3.4 1.6 3.3 1.9
1.9 0.6 1.1 0.1 0.7 2.5 0.6 0.9 0.7

2.8 0.7 3.0 0.7 0.6 3.4 0.7 2.1 1.3

1.5 0.3

2.0 0.4 3.0 0.9 0.4 3.2 0.5 2.4 1.5

1.5 0.3 3.9 0.4 0.2 2.8 0.3 2.6 0.8

2.9 0.6 4.4 0.2 0.5 4.7 0.6 3.5 0.5

4.1 0.9 4.7 0.5 0.5 5.4 0.9 3.1 0.8

4.2 0.7 4.7 0.4 0.5 6.2 0.8 3.1 0.7

3.3 0.6 4.9 0.6 0.5 4.4 0.6 3.0 0.8

3.5 0.7 4.7 0.4 0.6 5.0 0.7 3.2 0.8

3.8 0.6 4.7 0.4 0.5 5.4 0.6 3.0 0.7

3.6 0.6 4.7 0.3 0.6 4.6 0.6 3.3 0.7

1.6 0.3 1.9 1.6 1.7 2.8 0.3 1.5 1.7

3.0 0.7 5.5 1.9 0.5 4.6 0.7 4.3 2.0

3.2 0.9 5.9 1.0 0.5 3.5 0.9 5.4 1.6

3.2 1.0 5.7 0.9 0.8 4.6 1.0 3.8 0.9

2.7 0.6 3.9 1.5 0.7 3.5 0.7 3.4 2.0

2.7 0.6 3.9 2.3 0.6 4.6 0.6 3.5 2.3

3.2 0.8 4.8 2.0 1.3 3.9 0.8 3.4 1.7

3.2 0.8 4.9 2.6 0.5 4.7 0.8 3.8 2.0

3.7 2.4

3.8 0.9 4.7 2.5 1.4 4.4 0.9 3.5 2.1

3.2 0.6 4.9 1.8 0.4 4.8 0.6 4.8 2.6

2.0 0.4 2.9 0.8 0.8 3.9 0.4 2.6 1.9

2.7 0.4 3.5 0.9 0.9 4.9 0.5 3.2 1.7

6.4 0.9 0.6 0.1 0.5 7.8 1.0 0.7 0.8

4.7 0.6 0.6 0.0 0.9 5.1 0.6 0.7 0.4

4.9 0.6 0.7 0.0 0.3 6.2 0.6 0.7 0.2

2.6 0.6 4.4 1.6 0.3 3.4 0.7 3.2 2.1

3.6 0.8 5.5 1.0 1.1 3.9 0.9

2.2 0.4 4.1 0.6 0.3 3.4 0.5 3.2 1.3

3.1 0.7 4.5 1.8 0.3 4.3 0.8 3.2 2.4

3.1 1.1 4.4 1.1 0.6 4.0 1.2 3.9 1.9

3.0 1.3

2.9 0.8 4.6 1.5 0.6 3.9 0.8 3.3 2.0

2.3 0.9

2.7 0.5 4.3 0.1 0.6 3.9 0.5
3.0 0.4 4.6 0.3 0.5 4.7 0.5 3.0 0.5

4.1 0.8 4.7 0.4 0.6 5.9 0.8 3.3 0.6

3.3 0.6

1.6 0.3 2.7 2.6 0.7 3.8 0.3 2.0 2.3

3.4 0.9 4.6 1.1 0.7 4.5 0.9 3.9 1.2

4.1 0.8 4.7 0.2 0.7 5.3 0.9 4.0 0.7

3.6 0.9 4.9 0.1 0.5 6.3 0.9 3.6 0.5

2.5 0.3 3.9 0.2 1.1 3.4 0.4 3.4 0.6

2.8 0.4 4.7 1.1 0.6 3.5 0.4 3.8 1.1

3.8 1.0 4.3 0.1 0.5 6.4 1.0

2.4 0.6 3.4 0.5 1.2 4.4 0.6 3.3 1.3

2.9 0.9 1.4 0.1 2.6 3.6 0.9 1.4 0.7

3.5 0.5 3.8 0.0 0.8 5.2 0.6 3.0 0.5

1.5 0.5 1.2 2.0 0.7 3.1 0.5 1.0 2.5

2.1 0.6 1.3 3.1 1.3 3.5 0.7 1.1 2.7

1.8 0.4 1.1 2.5 1.1 3.1 0.5 1.0 2.9

2.2 0.4 2.3 0.7 0.3 3.5 0.4 1.5 1.0

3.0 0.6 5.1 0.4 0.5 3.5 0.6 3.3 0.8

3.0 0.6 1.2 0.1 0.3 4.0 0.7 1.0 0.7

3.5 0.8 1.3 0.0 0.4 4.9 0.9 1.0 0.8

3.5 0.8 1.3 0.0 0.3 4.9 0.8 1.1 0.8

0.7 1.5

3.8 1.1 5.9 0.9 0.6 4.6 1.1 4.1 1.0

3.1 0.8 5.7 1.4 1.2 3.8 0.8

2.0 0.3 2.7 1.8 0.4 4.1 0.4 2.2 2.2

2.5 0.6 3.1 1.8 0.5 4.5 0.6 2.5 2.7

1.7 0.2 2.1 0.9 0.4 3.8 0.3 2.0 1.9

3.0 0.6 3.1 2.2 0.7 5.5 0.7 2.7 2.6

as allocated in proportion to the concentration value of the five PM2.5 constituents which now sum to the FRM mass.
Crustal OC EC Sulfates Nitrates Crustal OC EC Sulfates

1.0 2.8 0.7 4.9 0.1 1.1 7.1 0.7 3.1

1.3 4.4 0.7 4.5 0.1 1.3 6.6 0.8 2.9

0.5 3.3 0.5 4.5 0.2 0.5 5.7 0.5 2.8

0.5 3.5 0.6 4.3 0.0 0.5 5.4 0.6 2.8

0.4 5.0 0.7 4.3 0.0 0.5 7.2 0.7 2.6

1.5 1.5 0.4 1.7 0.0 1.7 1.7 0.5 1.3

0.7 2.7 0.5 3.8 0.3 0.8 6.3 0.5 2.6

0.6 7.7 1.4 1.3 0.9 0.7 8.4 1.5

0.7 4.9 0.8 2.1 3.7 0.8 7.4 0.8 1.4

2.6 4.6 0.8 2.0 0.2 2.7 7.6 0.8 1.8

0.6 12.4 1.1 0.9 0.0 0.6 9.1 1.1 0.7

0.5 3.8 0.7 1.5 1.5 0.5 6.0 0.7 1.0

0.5 3.5 0.6 1.5 2.0 0.5 5.0 0.6 1.1

0.7 3.6 0.8 2.9 0.4 0.7 5.8 0.8 1.9

0.6 3.6 0.6 2.8 0.4 0.6 5.7 0.6 2.2

0.4 3.6 0.7 1.6 0.8 0.5 6.3 0.7 1.1

0.7 4.7 0.7 2.2 5.8 0.8 6.0 0.7 1.3

1.0 4.8 0.6 2.7 4.9 1.0 6.8 0.6 1.8

0.7 2.4 0.5 2.4 0.3 0.8 5.0 0.6 1.7

1.6 2.5 1.0 1.3 0.8 1.7 2.4 1.1 0.9

1.2 2.1 0.7 1.4 0.7 1.3 2.6 0.8

0.4 2.9 0.6 4.1 0.6 0.4 4.0 0.6 2.7

0.8 1.3 0.4 3.0 0.0 0.9 2.1 0.4 2.1

0.6 2.4 0.4 3.4 0.0 0.6 3.0 0.5 2.3

0.4 3.9 0.7 3.5 0.0 0.5 5.1 0.7 2.2

0.9 4.9 0.7 3.6 0.0 1.0 8.4 0.8 2.6

0.4 3.8 1.3 3.8 0.0 0.4 6.3 1.3 2.6

0.5 3.8 1.4 4.4 0.0 0.5 6.5 1.4 2.8

0.4 4.6 0.6 3.9 0.0 0.5 6.8 0.6 2.4

1.7 1.7 0.6 1.2 0.9 1.8 2.5 0.6 0.9

0.4 2.6 1.0 3.2 0.4 0.4 4.1 1.0 2.1

0.3 1.6 0.3 3.3 0.8 0.3 2.0 0.4 2.5

0.4 2.7 0.7 4.0 1.1 0.4 3.8 0.7 3.0

1.1 2.3 0.4 2.8 1.4 1.2 3.2 0.4 2.2

0.7 3.6 0.6 3.0 1.2 0.8 4.2 0.6 2.3

0.4 3.2 0.6 4.9 0.4 0.4 4.1 0.6 3.3

0.2 1.9 0.3 4.4 0.2 0.3 3.1 0.4 3.0

2011 Annual Average

Speciation Measurements SANDWICHed*
0.5 2.5 0.5 5.3 0.8 0.6 3.3 0.6 3.2

0.7 3.2 0.7 4.7 0.1 0.7 4.2 0.8 3.1

0.4 3.3 0.8 4.2 0.8 0.4 4.1 0.9 3.1

0.4 2.4 0.5 3.6 0.4 0.4 3.6 0.6 2.8

0.2 3.1 0.6 2.5 0.5 0.3 4.2 0.7 1.8

0.4 2.8 0.6 3.2 1.6 0.5 3.6 0.6 2.5

0.3 2.0 0.4 3.8 1.7 0.3 3.2 0.4 2.7

0.2 1.4 0.2 2.5 0.8 0.2 2.5 0.2 1.9

0.4 2.1 0.5 4.3 1.3 0.5 2.7 0.5 3.0

0.3 2.2 0.4 3.3 1.1 0.3 3.4 0.4 2.9

0.5 2.5 0.8 3.9 1.7 0.6 3.1 0.8 2.7

0.9 2.6 0.7 4.1 1.5 0.9 2.7 0.8 3.3

0.9 2.7 0.8 3.6 1.4 1.0 3.2 0.8 2.9

0.4 2.1 0.4 2.3 1.8 0.4 2.8 0.5 1.5

0.6 2.4 0.5 2.2 1.9 0.6 3.3 0.5 1.5

0.5 3.9 0.6 3.8 0.1 0.6 6.6 0.7

0.9 4.1 0.6 4.5 0.0 0.9 6.1 0.7 2.8

0.5 4.1 0.5 3.5 0.0 0.5 6.7 0.5 2.5

0.4 4.5 0.7 4.0 0.0 0.4 5.9 0.7 2.6

0.4 -0.1 0.1 1.8 0.0 0.5 1.1 0.1 1.2

0.7 2.8 0.6 1.0 1.2 0.8 3.3 0.6 0.7

1.0 3.4 0.9 4.0 1.9 1.1 4.6 0.9 2.7

0.5 2.6 0.7 3.6 1.8 0.5 4.3 0.7 2.4

0.4 2.3 0.5 3.5 2.1 0.4 3.8 0.6 2.6

0.5 2.7 0.6 3.7 2.1 0.5 4.0 0.6 2.2

3.3 3.8 0.9 4.5 0.9 3.4 6.1 1.0

0.8 3.3 0.7 5.6 0.6 0.9 4.7 0.8 3.7

0.4 2.8 0.5 5.7 1.4 0.4 4.6 0.6 3.4

0.4 2.9 0.6 3.7 1.6 0.4 4.5 0.6 2.6

0.3 2.0 0.4 4.5 1.1 0.3 3.8 0.4 2.8

0.8 2.9 1.0 4.3 2.3 0.8 4.3 1.1 2.9

0.4 3.0 0.7 4.9 1.6 0.5 4.3 0.7 3.1

0.5 2.8 0.5 5.3 0.9 0.5 4.7 0.5 3.3

0.2 1.0 0.1 0.9 0.1 0.3 1.8 0.1 0.7

0.8 2.0 0.4 2.9 1.8 0.9 3.7 0.4 1.9

1.1 2.9 1.0 1.3 0.1 1.2 4.5 1.1 1.2

0.8 3.0 0.8 0.9 0.5 0.8 3.6 0.8 0.7

0.4 3.8 0.9 3.7 0.6 0.4 4.6 1.0 2.5

0.2 1.7 0.3 3.1 0.1 0.2 3.2 0.4 2.1

0.6 3.3 1.7 4.1 0.7 0.7 5.0 1.8 2.4
1.1 2.7 0.6 1.2 0.2 1.2 3.7 0.7 1.0

0.5 2.9 0.8 2.6 0.8 0.6 3.9 0.8 1.9

0.1 1.1 0.1 1.9 0.1 0.2 2.0 0.1 1.5

0.3 2.1 0.5 3.0 1.0 0.3 4.1 0.5 2.3

0.2 1.3 0.2 3.2 0.4 0.2 2.8 0.2 2.1

0.3 2.7 0.5 4.1 0.1 0.3 4.0 0.5 2.3

0.3 3.6 0.7 3.8 0.1 0.3 4.8 0.8 2.4

0.4 3.3 0.6 3.9 0.1 0.4 4.9 0.6 2.4

0.2 2.5 0.5 3.6 0.3 0.2 3.0 0.5 2.4

0.4 3.5 0.6 3.9 0.2 0.4 5.2 0.6 2.5

0.3 3.2 0.5 3.7 0.1 0.3 4.9 0.5 2.5

0.4 3.6 0.5 4.0 0.2 0.4 4.6 0.6 2.5

1.2 1.3 0.3 1.8 1.3 1.3 2.9 0.3 1.2

0.4 2.5 0.6 5.3 1.2 0.4 4.8 0.6 3.3

0.4 3.0 0.9 6.4 0.8 0.4 2.7 0.9 3.9

0.6 2.9 0.8 4.2 0.4 0.6 4.7 0.8 3.3

0.4 2.7 0.6 4.1 1.3 0.5 3.6 0.6 2.8

0.5 2.3 0.6 4.3 1.6 0.5 3.3 0.6 3.2

0.9 2.4 0.7 4.2 1.1 0.9 3.1 0.7 2.7

0.4 2.7 0.6 4.8 1.1 0.4 4.0 0.7 3.3

0.3 2.1 0.6 4.5 1.6 0.3 3.7 0.7 2.8

0.8 2.8 0.7 4.4 1.2 0.8 4.2 0.7 3.2

0.3 2.9 0.6 5.8 1.6 0.3 3.0 0.6 4.3

0.8 2.3 0.4 3.1 1.0 0.9 4.3 0.4 2.1

0.7 3.0 0.4 3.6 1.0 0.7 5.0 0.5 2.6

0.5 7.5 1.0 0.9 0.3 0.6 8.8 1.0

0.7 7.4 0.9 0.9 0.2 0.8 7.1 0.9

0.2 6.5 0.7 1.0 0.0 0.2 8.0 0.7

0.3 2.2 0.6 4.1 1.0 0.3 3.7 0.6 2.9

0.2 1.9 0.4 3.9 0.6 0.2 2.8 0.4 2.9

3.0

0.3 2.7 0.6 4.0 1.2 0.3 3.7 0.6 3.0

2.6

0.4 3.1 0.9 4.8 0.8 0.4 3.8 0.9 2.8

0.3 2.5 0.6 3.8 0.3 0.3 4.2 0.6 2.4

0.5 2.7 0.6 4.1 1.1 0.6 3.8 0.7 3.2

0.3 2.2 0.5 2.8 0.3 0.3 4.0 0.5 2.1
0.3 2.9 0.4 3.6 0.0 0.3 4.6 0.4 2.3

0.4 3.7 0.6 4.0 0.0 0.4 5.3 0.7 2.5

0.5 3.7 0.6 3.9 0.1 0.5 5.5 0.6 2.4

0.6 1.6 0.3 2.4 1.8 0.6 4.0 0.3 1.5

0.4 3.2 0.7 4.7 0.4 0.5 4.4 0.8 2.8

0.5 4.1 0.8 4.6 0.0 0.5 5.3 0.8 2.8

0.4 3.0 0.6 4.2 0.1 0.5 5.3 0.7 2.8

0.6 2.5 0.3 4.1 0.2 0.6 3.5 0.3 2.6

0.4 3.2 0.4 4.6 0.4 0.4 4.7 0.4 3.0

1.1 2.8 0.7 4.0 0.2 1.1 4.0 0.7 2.6

3.5 2.4 0.7 1.7 0.1 3.6 6.0 0.8 1.4

0.6 5.2 0.7 3.5 0.0 0.6 7.1 0.7 2.7

0.8 1.6 0.5 1.2 2.3 0.9 3.2 0.5 0.9

0.8 2.3 0.7 1.4 2.5 0.9 3.2 0.7 0.9

0.9 2.0 0.5 1.3 2.6 1.0 3.0 0.5 0.9

0.4 2.5 0.4 1.9 0.6 0.5 3.6 0.4 1.6

0.3 3.1 0.6 4.0 0.2 0.3 4.0 0.6 2.5

0.3 4.6 0.8 1.2 0.3 0.3 5.6 0.9 0.9

0.2 4.2 0.8 1.3 0.2 0.3 5.3 0.9 0.9

0.2 4.2 0.8 1.4 0.1 0.2 5.5 0.9

0.5 4.0 0.7 0.9 1.2 0.5 4.8 0.7 0.7

0.5 3.0 0.9 5.0 0.3 0.5 4.7 0.9 3.1

3.6

1.9

0.3 1.8 0.3 2.7 1.5 0.3 4.1 0.3 2.1

0.4 2.4 0.5 3.1 1.9 0.4 4.5 0.6 2.3

0.3 1.7 0.2 2.5 1.5 0.3 3.3 0.3 1.7

0.6 2.5 0.6 3.2 1.9 0.6 5.2 0.6 2.2
Nitrates Crustal OC EC Sulfates Nitrates Crustal OC EC

0.7 0.9 2.5 0.6 3.7 0.1 1.0 6.6 0.7

0.7 1.4 3.5 0.6 3.5 0.1 1.4 5.7 0.7

0.8 0.5 3.0 0.5 3.4 0.1 0.5 4.8 0.5

0.5 0.7 3.6 0.5 3.3 0.0 0.7 5.8 0.6

0.5 0.6 4.3 0.7 3.1 0.0 0.6 6.6 0.7

0.5 1.6 1.5 0.4 1.6 0.0 1.7 1.6 0.5

0.9 1.1 3.3 0.6 3.1 0.2 1.1 5.8 0.7

4.4 0.9 4.7 0.8 1.8 2.3 1.0 8.2 0.8

1.8 4.0 5.9 1.0 2.1 0.2 4.2 9.6 1.0

0.6 0.7 12.8 1.0 1.0 0.2 0.7 9.9 1.1

1.6 0.5 4.0 0.7 1.2 0.4 0.5 6.4 0.7

1.7 0.6 3.3 0.5 1.4 0.5 0.6 5.0 0.6

2.6 0.5 3.2 0.7 2.4 0.3 0.5 6.4 0.8

2.4 0.7 3.4 0.5 2.7 0.1 0.7 6.0 0.6

2.1 0.4 3.3 0.6 1.4 0.5 0.5 6.1 0.6

3.6 0.7 3.1 0.5 1.7 2.2 0.7 5.2 0.5

6.2 1.2 4.8 0.7 2.4 3.6 1.2 7.0 0.7

2.4 1.1 2.3 0.5 2.1 0.2 1.1 5.4 0.5

1.2 1.6 2.4 0.9 1.1 0.7 1.7 2.7 0.9

1.5 0.5 2.8 0.7 3.4 0.4 0.5 4.6 0.8

0.6 1.4 1.1 0.4 2.8 0.0 1.5 2.0 0.4

0.6 1.0 2.2 0.4 2.9 0.0 1.1 2.6 0.5

0.4 0.6 3.6 0.7 2.8 0.0 0.7 4.5 0.8

0.5 1.1 4.5 0.7 3.1 0.0 1.2 6.1 0.7

0.5 0.5 3.8 1.1 3.1 0.0 0.6 5.5 1.2

0.6 0.6 3.9 1.2 3.3 0.0 0.6 5.7 1.2

0.4 0.5 4.1 0.5 2.9 0.0 0.6 6.0 0.6

1.6 1.5 2.2 0.6 1.1 0.5 1.6 3.5 0.7

1.5 0.4 2.7 1.1 2.6 0.5 0.5 4.1 1.2

1.6 0.3 2.1 0.4 3.1 0.8 0.3 3.4 0.4

2.0 0.4 2.7 0.7 3.7 0.9 0.5 4.3 0.7

1.5 1.2 2.3 0.4 2.7 0.9 1.2 3.2 0.5

1.7 1.0 3.8 0.6 2.8 0.8 1.1 4.2 0.7

0.8 0.5 3.5 0.7 3.9 0.2 0.6 4.9 0.7

0.4 0.3 2.4 0.3 3.5 0.0 0.3 4.1 0.3

2012 Annual Average

Speciation Measurements SANDWICHed*
1.3 0.5 2.6 0.5 3.9 0.4 0.6 3.8 0.5

0.8 1.2 2.8 0.6 3.8 0.0 1.2 4.4 0.7

1.9 0.4 3.4 0.8 3.7 0.8 0.4 5.3 0.8

1.0 0.4 2.6 0.6 3.4 0.4 0.4 3.8 0.6

1.0 0.2 2.7 0.5 2.2 0.3 0.2 4.3 0.6

2.3 0.5 2.8 0.6 3.1 1.5 0.5 3.7 0.6

2.5 0.3 2.1 0.4 3.2 1.7 0.3 3.6 0.4

1.1 0.2 1.5 0.2 2.4 0.8 0.2 2.5 0.2

2.5 0.5 2.5 0.6 3.7 1.6 0.5 3.4 0.6

2.2 0.4 2.7 0.5 3.6 1.2 0.4 4.2 0.5

2.3 0.5 2.4 0.7 3.4 1.3 0.6 4.0 0.8

2.3 1.2 2.7 0.8 4.1 1.3 1.3 3.6 0.9

2.5 1.9 3.2 0.9 3.5 1.6 2.0 4.2 0.9

1.9 0.5 2.2 0.4 1.8 1.4 0.5 4.1 0.5

2.2 0.5 2.4 0.5 1.9 1.6 0.6 4.1 0.5

0.6 0.6 3.2 0.5 3.3 0.1 0.7 5.6 0.6

0.6 0.6 4.0 0.6 3.0 0.0 0.6 6.0 0.6

0.6 0.5 4.9 0.7 3.1 0.0 0.5 6.3 0.7

0.3 0.4 -0.1 0.1 1.8 0.0 0.5 1.6 0.1

1.1 0.8 3.6 0.6 0.9 0.4 0.9 5.4 0.6

2.7 0.8 3.2 0.8 3.3 1.8 0.8 4.7 0.8

2.3 0.5 2.5 0.7 3.0 1.3 0.5 5.6 0.7

2.5 0.5 2.6 0.6 3.2 1.6 0.6 4.9 0.6

2.2 0.4 2.5 0.6 2.7 1.4 0.5 4.6 0.6

1.4 1.0 3.4 0.8 4.5 0.5 1.0 4.6 0.8

1.8 0.5 2.8 0.5 4.2 0.7 0.5 4.9 0.5

2.5 0.4 3.0 0.5 3.2 1.8 0.4 4.4 0.6

2.0 0.3 1.7 0.6 3.5 1.3 0.3 3.4 0.7

2.5 1.1 2.9 1.1 3.4 1.7 1.1 4.9 1.2

2.3 0.6 2.9 0.6 3.8 1.4 0.6 4.5 0.6

1.5 0.5 3.1 0.5 4.0 0.6 0.6 5.1 0.5

0.3 0.3 2.0 0.1 0.9 0.2 0.3 3.3 0.1

2.5 1.5 2.0 0.4 2.3 1.9 1.6 3.2 0.4

0.8 1.8 3.0 0.9 1.4 0.0 1.9 4.3 1.0

0.8 0.8 2.5 0.6 0.9 0.2 0.8 3.3 0.7

1.9 0.5 2.7 0.8 3.1 0.8 0.5 3.9 0.8

1.3 0.3 1.9 0.4 2.6 0.5 0.3 3.6 0.4

2.0 0.6 3.0 1.4 3.0 0.8 0.6 4.4 1.5
0.6 1.2 2.3 0.6 1.2 0.1 1.3 3.8 0.6

1.2 0.5 2.5 0.6 2.4 0.5 0.6 3.8 0.6

0.3 0.1 1.0 0.1 1.9 0.1 0.2 2.0 0.2

1.5 0.4 1.7 0.7 2.8 0.8 0.4 3.9 0.7

0.9 0.2 1.6 0.2 2.6 0.3 0.3 3.3 0.3

0.6 0.5 3.2 0.5 2.8 0.0 0.5 4.4 0.6

0.9 0.4 3.8 0.8 2.8 0.1 0.4 5.3 0.8

0.9 0.5 3.9 0.7 2.9 0.1 0.5 6.0 0.8

0.8 0.4 3.8 0.7 2.9 0.1 0.4 4.1 0.7

0.8 0.5 3.5 0.6 3.0 0.0 0.5 5.2 0.6

0.7 0.4 3.4 0.5 3.0 0.0 0.4 5.2 0.5

0.7 0.5 3.4 0.6 3.0 0.1 0.5 4.8 0.6

1.4 1.8 1.3 0.2 1.6 0.9 2.0 2.8 0.3

1.7 0.5 2.6 0.6 4.0 0.8 0.5 4.3 0.7

1.4 0.5 3.2 0.8 4.6 0.7 0.6 2.9 0.9

0.7 1.0 3.6 0.8 3.8 0.1 1.1 5.2 0.8

1.8 0.9 2.9 0.6 3.4 1.1 1.0 3.7 0.6

2.5 0.5 2.5 0.5 3.8 1.6 0.5 3.8 0.6

1.6 1.2 2.8 0.7 3.3 0.9 1.3 3.7 0.7

2.0 0.7 3.0 0.7 4.0 1.2 0.7 4.2 0.7

2.1 0.4 2.0 0.5 3.5 1.2 0.4 3.4 0.6

2.0 1.0 3.1 0.7 3.9 1.2 1.0 5.2 0.8

2.5 0.6 2.4 0.8 4.9 1.5 0.6 2.3 0.8

1.2 1.1 2.1 0.4 2.5 0.5 1.1 4.4 0.4

1.2 1.2 2.9 0.5 3.1 0.5 1.2 5.2 0.5

3.0 0.4 2.9 0.7 3.5 1.7 0.4 5.6 0.7

1.5 0.3 2.3 0.4 3.5 0.7 0.3 3.6 0.5

2.8 0.5 2.8 0.9 3.8 1.5 0.5 5.3 0.9

3.2 0.4 3.5 0.8 3.8 1.7 0.4 6.2 0.8

1.9 0.6 3.0 0.8 3.3 0.4 0.6 5.9 0.8

2.2 0.5 3.0 0.8 3.5 1.0 0.5 5.1 0.9

1.6 0.4 2.4 0.6 2.9 0.6 0.4 4.5 0.7

2.7 0.6 3.3 0.8 3.9 1.5 0.6 5.4 0.8

1.1 0.3 2.5 0.5 2.6 0.4 0.3 4.7 0.5
0.5 0.5 2.8 0.4 2.9 0.1 0.5 4.6 0.4

0.9 0.4 4.0 0.7 3.0 0.1 0.5 5.8 0.8

0.5 0.5 3.6 0.6 2.9 0.0 0.6 4.9 0.7

1.6 0.7 1.8 0.3 1.8 0.8 0.8 3.9 0.3

1.0 0.5 3.0 0.7 3.5 0.2 0.5 4.7 0.7

0.8 0.9 3.8 0.8 3.4 0.0 0.9 4.7 0.8

0.7 0.5 3.7 0.7 3.3 0.1 0.6 5.2 0.7

0.6 0.5 2.5 0.3 3.1 0.0 0.6 4.2 0.3

1.1 0.5 2.9 0.4 3.6 0.2 0.6 4.3 0.4

1.1 1.5 2.6 0.6 3.1 0.2 1.6 4.0 0.7

0.5 2.7 2.4 0.8 1.8 0.0 2.8 4.5 0.8

0.5 1.1 3.4 0.5 3.2 0.0 1.2 5.5 0.5

1.8 0.9 2.3 0.5 1.1 1.2 1.0 3.9 0.5

1.5 1.0 2.6 0.6 1.1 1.0 1.1 4.2 0.7

1.7 1.1 2.4 0.5 1.1 1.0 1.2 4.4 0.5

1.0 0.3 2.6 0.4 2.0 0.4 0.3 4.0 0.5

0.9 0.4 3.2 0.6 3.1 0.1 0.4 4.4 0.6

0.7 0.4 3.5 0.6 1.2 0.1 0.4 4.5 0.7

0.7 0.2 4.0 0.7 1.2 0.0 0.3 5.5 0.8

1.3 0.6 4.8 0.7 0.9 0.6 0.7 6.5 0.7

0.8 0.7 3.7 1.0 3.6 0.2 0.8 5.6 1.0

0.9 1.2 4.0 0.8 4.2 0.3 1.2 5.7 0.8

1.9 0.3 2.1 0.4 2.4 1.3 0.3 4.3 0.4

2.2 0.4 1.9 0.3 2.5 1.5 0.5 4.2 0.3

2.2 0.4 2.4 0.5 2.8 1.4 0.5 4.4 0.5

1.6 0.3 1.7 0.2 2.2 1.3 0.4 3.4 0.2

2.1 0.8 2.4 0.5 2.6 1.4 0.8 4.9 0.5
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

3.5 4.3 4.7 3.3 4.0 4.3 5.0 2.9 2.8

3.5 3.4 4.2 3.2 3.4 4.4 4.7 2.7 2.6

3.9 3.4 4.3 3.0 3.5 4.1 4.2 2.8 2.5

3.2 4.1 3.5 3.1 3.3 4.1 4.4 2.5 2.2

3.5 4.1 3.6 2.7 3.1 4.1 5.0 2.1 2.4

0.7 0.9 1.3 1.0 0.8 1.4 1.8 1.1 0.8

2.6 3.1 3.8 2.6 3.3 3.1 3.7 2.3 2.6

0.5 0.9 0.8 0.7 0.7 1.2 1.4 0.9 0.7

1.7 1.4 2.1 1.4 1.3 1.3 2.1 1.9 1.1

0.9 1.9 2.3 1.3 0.9 1.7 2.4 1.3 1.1

1.2 2.9 4.4 1.7 1.2 2.6

0.5 0.8 0.5 0.4 0.4 0.9 0.8 0.6 0.5

0.9 1.1 1.7 1.0 0.8 1.2 1.8 1.1 0.7

0.8 0.8 1.2 0.8 0.8 1.1 1.8 1.2 0.8

1.2 2.4 3.4 1.5 1.1 2.5 3.9 1.6 1.2

1.0 3.1 3.4 1.1 0.9 2.3 4.0 1.5 1.2

1.3 1.3 1.6 1.0 0.9 1.2 1.7 1.3 0.8

1.6 1.4 1.6 1.3 1.8 1.1 1.9 2.1 1.0

1.4 1.6 2.0 1.5 1.8 1.7 2.5 2.3 1.6

1.0 2.1 2.5 1.1 0.8 2.1 3.6 1.1 0.9

1.4 1.3 0.9 1.0 1.0 1.1 1.3 0.9 0.9

1.3 1.4 0.9 1.1 0.9 1.2 1.3 0.9 1.0

3.2 4.2 5.6 3.1 3.0 3.3 4.6 2.3 2.6

2.9 2.6 2.5 2.5 3.0 3.1 1.7 1.7 2.3

2.8 3.3 2.7 2.7 3.2 3.4 2.7 1.8 2.4

3.4 3.5 2.2 2.4 3.2 3.9 2.9 1.7 2.4

3.4 4.1 3.5 2.5 2.3 4.0 4.4 2.0 2.6

3.4 3.9 3.4 2.5 3.2 4.2 3.8 1.9 2.5

4.4 4.0 4.8 2.9 3.4 4.5 4.6 2.3 2.5

3.7 4.0 3.4 2.8 3.0 4.2 4.6 2.0 2.1

1.3 1.2 0.8 0.7 0.8 1.2 1.1 0.7 0.7

2.1 2.6 2.4 1.7 2.5 2.7 3.4 1.8 2.1

3.4 3.2 5.4 2.6 2.9 3.3 2.1 2.1 2.5

5.9 3.4 4.8 2.6 3.8 3.5 3.7 2.0 3.0

2.5 1.9 2.6 1.7 2.4 3.0 2.2 1.6 1.9

3.3 2.5 2.1 1.6 3.0 2.9 2.5 1.7 2.1

4.9 4.7 4.9 4.1 3.8 4.3 6.0 2.6 3.0

5.0 4.6 6.4 4.0 3.8 4.0 4.9 2.1 2.7

Speciation Measurements

Sulfates
4.5 4.5 5.4 4.2 3.9 4.2 6.7 2.2 2.7

4.1 4.7

3.7 4.7 3.7 3.4 3.9 4.4 4.5 2.7 2.7

3.4 3.5 4.9 3.0 3.3 3.8 4.0 2.4 2.8

3.6 3.0 4.6 2.8 2.7 3.3 3.9 2.1 2.5

1.7 2.1 2.6 1.7 2.3 2.0 2.3 1.5 1.9

2.1 2.5 3.3 2.8 2.5 2.4 3.1 2.0 2.6

2.5 3.3 4.0 2.7 3.0 3.3 4.4 1.7 3.2

1.2 2.0 2.3 1.8 2.1 2.0 2.3 1.7 2.6

2.9 2.8 4.6 2.4 2.9 3.8 5.1 1.9 3.6

1.4 2.9 3.6 2.5 2.3 2.6 3.7 2.0 3.4

2.8 2.8 4.0 2.3 2.7 3.4 4.5 2.2 3.0

2.5 4.5 5.2 3.1 2.8 3.2 5.1 2.0 3.8

2.2 3.4 3.4 2.9 3.0 2.3 4.3 1.9 4.0

2.5 1.6 1.6 1.7 1.9

2.4 1.8 1.6 1.6 2.4 1.6 1.5 1.6 2.0

2.2 1.8 1.8 1.6

3.5 3.2 2.6 3.1 3.7 3.4 2.7 2.4

3.2 3.5 3.5 3.1 3.7 4.5 4.0 2.4 2.7

3.5 4.8 4.4 3.0 2.5 3.9 3.7 1.6 2.5

3.5 3.3 4.2 2.3 3.6 3.5 4.3 2.4 2.1

1.7 1.4 0.8 0.7 1.5

0.8 0.6 0.6 0.8 0.8 0.8 0.8 0.8 0.5

3.3 2.9 3.7 3.1 3.3 3.4 3.7 2.5 3.5

2.3 3.3 3.3 2.5 3.1 2.7 3.8 2.2 2.0

2.2 3.5 3.3 2.9 3.4 2.3 3.5 2.2 2.4

2.5 3.8 2.9 2.9 3.2 3.2 3.7 2.0 2.7

3.7 3.5 4.3 3.4 4.3 4.1 5.1 1.5 2.4

4.2 4.9 5.8 4.5 4.1 4.6 7.7 2.1 3.2

5.0 5.2 5.3 4.2 4.7 4.1 7.1 2.6 2.9

2.1 2.9 3.7 3.3 3.0 3.0 4.2 1.9 3.2

3.4 2.8 3.9 4.0 3.4 3.3 5.7 2.1 2.6

3.1 3.5 3.6 3.4 4.4 3.0 4.7 2.1 3.2

2.9 4.0 3.9 3.0 3.1 3.2 4.5

3.7 3.2 4.7 3.5 3.4 3.7 6.6 2.4 3.0

4.4 4.3 5.5 3.7 4.2 4.6 6.3 2.5 2.7

0.9 0.6 0.6 0.5 0.6

0.7

3.4 2.1 2.6 2.0 1.9 3.2 2.9 1.6 2.2

0.8 0.5 1.2 1.5 0.8 0.7

0.4 0.8 0.7 0.4 0.4 0.8 0.9 0.6 0.4

2.2 2.7 3.8 2.1 2.8 3.1 3.8 2.1 2.4

2.5 2.9 3.7 2.1 2.0 2.3 3.8 1.9 2.1

2.7 3.3 3.9 2.1 3.0 3.4 4.1 2.6 2.6
0.8 1.0 0.9 0.7 0.5 1.1 1.2 0.8 0.6

1.9 2.5 3.8 1.6 2.2 1.8 2.9 1.7 1.8

3.2 3.4

1.6 1.5 2.0 1.0 1.5

1.9 2.4 3.2 1.9 2.2 2.6 3.1 1.8 2.4

2.3 3.7 4.5 2.2 2.5 2.3 4.0 1.8 2.1

4.1 3.8 4.6 2.2 2.5 4.2 5.4 2.1 1.9

3.8 3.9 4.9 2.6 2.7 4.0 3.9 1.8 2.4

3.7 4.0 4.5 2.8 3.0 3.7 3.8 2.0 2.4

4.1 4.5 4.3 3.2 2.1 4.0 3.4 2.4 2.3

3.6 4.0 4.7 3.0 2.8 3.9 4.3 1.9 2.5

3.8 4.4 4.4 2.7 2.9 3.8 3.5 1.8 2.6

3.5 4.6 4.4 2.7 2.7 3.6 4.8 2.2 2.2

2.2 1.3 1.3 1.5 1.7 1.7 1.4 1.1 1.5

4.0 4.2 5.9 3.5 4.0 4.1 6.8 2.4 2.9

4.2 5.7 5.3 4.6 5.1 5.4 7.2 4.1 4.4

5.3 4.9 5.3 4.5 4.7 2.0 5.4 2.9 2.8

2.8 3.4 4.2 2.1 3.2 3.1 4.9 2.4 3.3

2.9 2.8 4.0 2.7 3.0 3.6 5.7 1.7 4.2

3.7 4.5 4.5 2.9 3.1 2.9 5.4 2.4 3.0

4.1 3.3 5.0 3.4 3.4 4.0 5.9 2.1 2.9

3.6 3.5 5.1 2.4 2.8

3.4 3.8 5.1 2.9 3.4 4.1 4.1 2.5 3.4

3.4 3.5 5.7 3.4 4.0 5.3 6.3 3.6 6.0

2.4 2.3 2.7 2.3 2.9 3.5 2.3 1.6 1.9

3.2 3.1 3.3 2.1 4.4 3.2 2.6 2.4 2.1

0.3 0.6 0.6 0.4 0.4 1.0 0.8 0.6 0.3

0.4 0.6 0.5 0.4 0.5 1.3 0.7 0.5 0.5

0.2 0.5 0.6 0.4 0.4 1.0 0.9 0.5 0.3

3.2 3.3 4.9 2.7 2.8 3.6 4.5 2.0 2.8

4.3 5.0 5.3 3.4

3.1 3.8 3.8 2.6 1.9 3.7 5.3 1.8 3.3

3.6

3.5 3.5 4.9 2.4 3.2 3.5 4.5 1.7 3.3

3.1

3.3 3.5 4.4 2.5 2.9 5.7 4.6 2.2 2.8

2.3 3.5 4.3 2.0 2.4

3.5 3.7 4.7 2.9 2.8 3.8 4.7 1.9 3.3

1.7 2.4 3.4

2.1 1.7 2.4 2.3 2.5 1.8 2.2

3.3 3.9 3.6 3.2
3.6 4.3 4.6 2.8 2.5 3.9 3.9 1.8 2.6

3.9 4.0 4.7 2.6 2.6 3.9 4.8 1.8 2.5

2.8 4.1 4.5 2.0 2.3

3.1 1.6 1.9 2.1 2.0 2.0 2.4 1.6 1.5

4.1 3.9 3.8 3.0 4.1 3.4 5.0 2.8 2.2

4.2 3.5 4.4 2.9 4.9 3.9 4.6 2.5 2.4

5.1 4.1 4.9 2.4 2.7 4.9 4.8 2.0 2.8

3.2 3.1 3.8 2.8 3.5 3.4 4.0 2.5 2.4

3.8 3.7 4.4 3.1 3.7 3.6 5.1 2.5 2.0

4.8 3.5 2.9 3.0 3.5 4.1 6.0

2.0 3.3 3.4 2.5 3.6 3.8 3.4 2.4 2.3

0.9 1.3 1.4 0.9 0.9 1.6 1.7 1.3 1.0

2.4 3.7 3.9 2.8 2.7 3.6 3.4 2.2 2.5

1.2 0.9 0.9 0.8 0.9 0.9 1.0 1.0 0.9

1.5 0.8 1.0 0.9 1.3 0.9 1.1 1.0 0.7

1.1 0.8 0.9 0.7 0.8 1.1 1.2 0.7 0.8

1.7 1.5 2.6 1.3 1.7 1.2 1.4 1.6 1.8

3.8 4.4 5.0 2.9 2.9 3.7 4.2 2.4 2.4

0.8 0.9 1.4 0.6 0.7 0.8 1.2 1.1 0.8

0.9 1.0 1.5 0.8 0.8 0.9 1.6 0.9 0.6

0.6 1.2 1.7 0.6 0.7 1.2 1.7 0.8 0.6

0.7 0.8 0.6 0.5 0.9 0.9 0.6

5.9 4.2 5.8 3.5 3.6 4.4 5.9 2.4 2.9

5.9 2.6 3.4

4.3 4.7 5.9 4.2 3.6 4.8 8.8

2.0 2.3

2.1 2.2 2.5 1.9 2.0 2.3 2.4 1.9 2.3

2.3 2.6 2.8 2.2 2.2 2.5 3.3 2.2 2.9

1.5 1.6 1.7 1.9 1.9 2.3 1.6 2.2 2.4

2.0 2.7 2.6 2.7 2.2 3.0 3.4 2.0 2.9
2012 2012 2012 2010 2010 2010 2010 2011 2011

2 3 4 1 2 3 4 1 2

3.5 3.5 2.7 1.6 0.6 0.5 1.0 1.3 0.5

3.7 3.0 2.5 1.3 0.5 0.4 1.0 1.3 0.5

3.3 3.2 2.1 2.2 0.5 0.4 1.6 1.4 0.5

3.4 2.7 2.7 1.3 0.4 0.3 0.8 0.9 0.4

3.3 2.3 2.5 2.0 0.4 0.4 0.9 0.9 0.4

1.4 1.9 0.9 1.1 0.3 0.2 0.8 1.0 0.3

3.2 2.5 2.3 2.1 0.5 0.4 1.5 2.2 0.5

1.6 1.0 0.4 0.4 2.0 1.9 0.7

0.8 1.3 0.7

1.6 1.8 1.2 7.6 1.6 1.4 8.2 5.8 1.3

1.8 2.6 1.5 1.8 1.2 0.8 1.6 2.4 0.8

4.0 4.8 3.7 4.1 4.9 2.8

1.1 1.1 0.3 0.7 0.3 0.2 0.5 0.5 0.3

1.2 1.3 0.6 4.2 0.8 0.8 3.3 3.7 0.8

1.4 1.4 0.9 3.8 0.7 0.8 3.8 3.0 0.8

2.4 3.1 0.9 2.9 3.2 3.1 2.9 2.0 2.2

2.7 2.9 1.9 3.2 3.7 2.7 2.2 1.7 2.1

1.4 1.6 0.7 2.8 1.2 1.7 2.5 2.6 1.0

1.4 1.6 1.3 5.8 1.5 1.6 7.9 9.4 0.9

2.4 2.2 1.1 5.6 2.2 2.7 8.7 6.9 2.4

2.1 2.6 1.3 2.4 2.8 2.4 2.3 1.7 2.5

1.0 0.9 0.7 3.3 1.4 0.4 1.4 2.0 0.8

1.3 1.2 3.7 1.4 0.4 2.1 1.8 1.0

0.6

2.6 3.2 2.4 2.4 1.2 0.6 2.4 2.5 0.8

2.6 1.9 1.6 1.2 0.7 0.5 0.7 0.8 0.6

2.6 2.0 2.0 0.8 0.6 0.4 0.7 0.8 0.5

2.3 2.1 2.0 0.7 0.4 0.3 0.6 0.6 0.3

3.1 2.3 2.2 1.3 0.5 0.3 0.4 0.5 0.4

2.9 3.0 1.9 1.4 0.5 0.3 1.0 0.8 0.3

3.5 3.0 2.2 1.4 0.5 0.3 1.1 0.6 0.4

3.0 2.3 2.2 1.4 0.4 0.3 0.6 0.5 0.4

1.2 1.2 0.6 3.9 1.6 0.6 2.4 2.6 1.1

2.0 2.2 2.1 1.4 1.5 0.6 1.2 1.8 1.2

2.2 2.9 2.5 3.8 1.4 0.7 2.2 2.7 1.3

2.9 3.3 2.7 7.5 1.7 0.8 3.2 4.2 1.2

2.9 2.0 1.9 4.0 0.5 0.4 1.9 4.4 0.8

2.8 2.4 2.0 6.3 0.8 0.5 0.9 4.7 0.9

3.6 4.1 2.4 2.7 0.5 0.4 1.9 1.7 0.6

3.0 3.9 2.2 2.1 0.3 0.2 1.1 0.9 0.3

Speciation Measurements

Nitrates
3.6 4.1 2.2 3.7 1.0 0.7 2.9 2.7 0.9

4.9 0.8

3.8 3.2 2.7 1.3 0.8 0.5 1.3 1.4 0.8

3.1 3.7 2.7 2.9 1.3 0.7 2.7 3.1 1.0

2.6 3.7 2.3 2.1 1.2 0.4 1.7 2.1 0.6

1.6 2.0 1.8 0.9 0.6 0.4 1.2 1.8 0.6

2.5 2.7 2.2 4.3 0.9 0.9 5.1 4.6 1.8

2.4 2.8 2.3 4.7 0.9 1.2 4.0 4.7 1.8

1.8 1.9 1.3 0.5 0.3 0.2 2.1 2.0 0.3

2.2 3.9 2.4 5.7 0.9 1.2 3.6 3.8 1.1

2.6 3.3 2.4 1.2 1.0 0.7 3.2 3.1 1.2

2.6 3.1 2.3 4.6 1.1 0.9 3.1 4.8 1.9

3.0 3.8 2.6 4.2 1.3 1.1 4.6 3.9 1.7

3.1 2.0 2.4 3.4 1.1 0.9 3.7 4.2 1.4

1.4 1.2 1.5 4.9 1.1

1.3 1.2 1.7 5.7 1.1 0.5 2.7 5.4 1.2

8.0 1.1 0.6 2.4

3.6 0.4 0.4 1.0 1.2 0.4

3.5 2.7 2.3 1.9 0.5 0.4 0.9 1.1 0.5

2.9 2.5 2.2 1.9 0.7 0.4 0.7 1.0 0.5

3.3 2.8 2.3 1.7 0.4 0.3 1.5 0.7 0.5

1.2 0.9 1.3 0.4 0.3

0.8 0.8 0.7 2.3 0.5 0.4 1.7 2.7 0.5

2.4 3.1 1.8 9.3 1.6 1.1 5.3 5.9 3.1

2.1 3.0 2.5 5.8 1.5 0.8 3.8 5.0 2.2

2.3 3.5 2.4 6.5 0.9 0.8 4.9 6.3 1.5

2.1 2.6 1.6 6.6 1.7 0.7 5.0 5.7 2.1

2.4 0.2 4.6 0.9 0.7 3.5 4.5 1.1

3.7 5.0 2.9 4.8 0.8 0.7 3.0 2.7 0.9

3.4 4.6 2.7 6.3 1.4 0.7 3.7 4.9 1.1

2.3 2.8 2.1 5.6 1.2 1.0 6.5 4.2 2.1

2.9 3.1 2.6 7.2 1.6 1.1 5.0 4.2 1.8

2.7 2.9 2.7 6.3 1.0 0.8 5.4 5.8 2.1

7.1 1.5 0.9 5.1 5.2 2.1

3.3 3.0 3.0 7.2 1.1 0.9 4.3 4.8 1.6

3.4 4.3 2.7 4.6 1.0 0.6 3.3 3.6 0.9

0.7 0.7 0.6 0.5 0.2

0.4 1.6

2.0 1.8 1.7 8.2 1.3 0.7 3.0 4.9 1.4

1.4 1.8 0.7 1.0 1.4 0.3

1.0 1.0 0.4 2.0 0.4 0.2 1.2 1.7 0.3

2.7 2.5 2.3 1.8 1.4 0.6 1.9 2.3 1.9

1.9 2.3 1.9 1.4 1.1 0.4 1.4 0.8 1.0

2.7 1.8 2.6 2.7 1.6 0.8 1.9 2.5 1.8
1.2 1.3 0.6 1.2 0.3 0.2 0.8 1.0 0.4

1.9 2.1 1.9 2.1 0.7 0.4 1.6 2.8 0.6

2.6 1.9

1.5 1.6 1.2 0.6 0.3

2.0 2.6 2.1 2.7 0.7 0.3 1.8 2.9 0.8

1.9 2.6 1.9 1.4 0.5 0.2 1.4 1.4 0.6

2.8 2.5 2.1 1.0 0.5 0.4 1.0 0.7 0.4

2.6 2.5 2.0 1.7 0.9 0.7 2.0 1.5 0.6

2.7 2.5 2.0 1.8 0.5 0.5 1.5 1.3 0.6

2.3 2.9 2.0 1.6 0.7 0.5 2.1 2.0 0.4

2.9 2.7 1.9 1.5 0.6 0.5 1.6 1.6 0.4

2.7 2.6 2.0 1.5 0.6 0.4 1.4 1.2 0.6

2.5 3.0 2.1 1.4 0.7 0.4 1.1 1.4 0.5

1.3 0.9 1.3 4.5 0.7 0.3 1.9 3.8 1.0

3.3 4.2 2.8 5.6 1.0 0.8 2.5 4.2 1.3

3.2 4.6 3.5 3.1 0.7 0.4 2.8 3.3 0.9

3.5 4.5 2.3 3.2 0.5 0.4 2.1 2.3 0.2

2.5 3.3 2.2 5.2 0.9 0.8 2.1 3.8 1.2

2.9 3.3 2.3 5.5 0.8 0.9 4.0 4.7 1.5

2.6 3.2 2.0 5.2 0.8 0.7 3.4 3.2 1.2

3.5 3.8 2.8 7.6 1.2 0.9 3.8 2.7 2.3

2.7 3.0 2.6 4.8 1.7

3.3 3.5 2.7 6.9 1.3 1.0 3.7 3.8 1.6

3.7 4.2 3.1 5.2 1.6 0.8 3.2 4.9 1.3

2.8 2.0 1.7 3.0 0.7 0.4 1.9 3.8 0.8

3.3 2.8 2.1 3.4 0.7 0.5 2.0 3.9 0.7

0.7 0.7 1.0 0.3 0.3 0.7 1.4 0.4

0.8 0.7 0.3 0.2 0.1 0.4 0.7 0.2

0.7 0.8 0.2 0.1 0.0 0.2 0.2 0.2

3.0 3.0 2.6 3.8 2.2 1.2 3.1 3.0 2.0

3.0 0.7 0.4 2.1

2.6 3.1 2.7 2.2 0.9 0.4 1.6 1.6 1.8

2.3

2.8 3.2 2.5

3.2 3.0 2.6 4.7 2.6 1.8 3.0 3.5 2.1

2.6 2.5 2.3

3.2 2.8 2.5 3.8 1.8 1.0 2.1 3.1 1.6

2.3 2.7 2.1 1.7 1.0

4.2 2.7

2.2

3.4 3.4 2.6 3.9 1.8 1.1 2.9 2.9 1.8

1.2 0.8 0.5

1.8 2.4 2.1 0.5 1.0 1.6 0.7

1.1 0.5 0.4 0.8
2.7 1.9 2.1 1.5 0.4 0.4 1.0 1.0 0.4

2.4 2.9 2.2 0.8 0.5 0.4 2.2 1.0 0.4

3.0 2.4 1.9 1.4 0.4

1.5 1.5 1.4 6.8 0.9 0.6 3.3 3.9 2.5

3.3 3.7 2.0 3.9 0.6 0.4 1.9 1.8 0.7

3.5 3.0 2.3 1.5 0.5 0.5 1.3 0.9 0.6

3.4 2.5 2.3 1.1 0.4 0.4 1.1 0.8 0.4

2.7 3.1 2.1 1.1 0.4 0.3 1.2 1.4 0.4

3.4 4.1 2.3 4.0 0.6 0.5 1.9 1.9 0.5

0.8 0.4 0.2 1.1 0.6 0.3

3.5 2.7 1.9 2.3 0.6 0.7 1.5 2.0 0.7

1.5 1.9 1.2 1.6 0.4 0.3 0.8 0.9 0.4

3.5 2.6 2.1 0.6 0.4 0.4 0.6 0.9 0.5

0.9 1.1 0.7 5.7 0.8 0.3 2.6 4.8 0.6

0.9 1.1 0.7 8.8 0.7 0.3 3.9 5.6 0.6

1.0 1.1 0.6 7.5 1.1 0.4 2.8 7.1 0.6

1.4 1.9 1.4 2.1 0.5 0.3 1.3 1.9 0.5

2.5 2.9 2.3 1.5 0.6 0.4 1.3 1.6 0.5

0.9 1.4 0.6 0.8 0.5 0.5 0.7 1.1 0.3

1.0 1.7 0.4 0.9 0.6 0.5 0.8 1.2 0.4

0.7 0.6 0.9 0.8 0.9 0.7

0.8 0.8 0.7 1.6 2.6 2.2 0.2

3.9 3.1 2.3 3.1 0.6 0.5 1.6 1.6 0.8

3.7 4.8 2.7

4.3 0.6 0.4 2.2 2.2 0.8

2.2 1.8 1.3

2.0 2.1 1.8 4.7 1.0 0.8 3.1 4.1 1.9

2.1 2.6 1.5 3.9 1.4 0.9 3.9 4.2 2.4

1.7 1.2 1.6 1.4 0.5 0.5 3.3 3.1 1.5

1.7 2.5 1.5 4.3 1.2 0.9 5.3 3.8 2.8
2011 2011 2012 2012 2012 2012 2010 2010 2010

3 4 1 2 3 4 1 2 3

0.4 0.8 1.0 0.5 0.4 1.0 0.7 1.4 1.7

0.3 0.9 0.9 0.4 0.4 0.9 0.9 1.9 2.5

0.3 1.2 1.2 0.6 0.4 1.1 0.3 1.1 1.0

0.2 0.5 0.6 0.4 0.3 0.7 0.4 1.5 1.6

0.3 0.6 0.8 0.4 0.3 0.7 0.3 0.6 1.3

0.3 0.9 0.7 0.4 0.4 0.6 0.5 1.2 0.8

0.4 1.3 1.3 0.5 0.4 1.3 0.4 1.0 1.5

0.5 4.2 1.1 0.7 0.5 0.5 1.1

0.5 0.6 1.8

1.6 13.2 9.5 1.3 1.6 5.3 0.4 0.5 1.3

0.8 2.5 2.2 1.2 1.0 2.8 1.6 2.1 2.2

1.2 0.8 0.7

0.2 0.6 0.7 0.5 0.3 0.9 0.7 0.9 1.2

0.9 4.4 2.7 0.8 0.9 1.8 0.3 0.8 0.9

0.9 6.9 2.5 1.0 1.0 2.5 0.4 0.7 0.8

3.4 3.9 2.3 2.7 2.5 3.0 0.6 0.5 0.5

3.1 3.7 2.0 2.8 2.4 2.5 0.7 0.6 0.7

1.5 3.8 3.2 1.5 1.9 1.7 0.4 0.4 0.4

1.4 15.3 5.5 1.6 1.3 5.9 0.5 0.7 1.4

2.7 16.9 13.6 3.0 2.7 5.6 0.5 0.7 1.7

3.7 2.0 1.9 2.4 2.5 2.9 0.4 0.6 0.6

0.4 2.1 2.7 0.6 0.4 1.4 1.2 1.1 1.5

0.5 2.2 3.9 0.9 0.5 1.0 1.0 1.2

1.5

0.7 1.7 2.1 0.9 0.7 2.4 0.5 0.8 0.5

0.5 0.5 0.7 0.5 0.6 0.5 0.4 1.5 1.7

0.4 0.5 0.7 0.6 0.5 0.6 0.3 1.3 1.4

0.2 0.3 0.5 0.3 0.2 0.4 0.2 1.0 1.5

0.3 0.4 0.8 0.5 0.4 0.6 0.7 1.9 2.2

0.2 0.6 0.8 0.4 0.4 0.6 0.3 1.1 0.7

0.3 0.5 0.9 0.4 0.3 0.7 0.4 1.5 1.0

0.2 0.4 0.5 0.4 0.2 0.7 0.6 1.3 1.1

0.9 2.8 2.0 0.9 1.0 2.5 1.1 1.1 2.2

1.0 1.1 2.6 0.9 0.7 2.1 0.3 0.6 0.4

1.4 1.3 3.0 0.8 0.5 2.1 0.2 0.6 0.5

0.8 1.8 3.4 1.2 0.8 2.8 0.5 0.7 0.5

0.4 2.4 2.1 0.9 0.4 2.7 0.5 1.0 1.3

0.4 1.2 2.4 1.0 0.6 2.9 0.7 1.0 0.8

0.3 1.0 1.1 0.5 0.5 1.1 0.4 0.5 0.7

0.1 0.6 0.4 0.3 0.2 0.6 0.2 0.4 0.3

Speciation Measurements

Nitrates
0.7 1.8 1.7 0.7 0.7 1.9 0.3 0.6 0.6

0.3 0.5

0.5 1.1 1.0 0.6 0.6 1.0 0.5 1.3 2.1

0.8 1.9 2.6 1.1 0.7 3.1 0.4 0.7 0.5

0.4 1.0 1.6 0.6 0.4 1.6 0.4 0.8 0.8

0.3 1.3 1.7 0.6 0.5 1.4 0.2 0.4 0.2

0.8 2.4 3.1 1.3 0.7 4.2 0.3 0.8 0.4

1.0 2.4 3.9 1.2 0.8 4.0 0.3 0.7 0.3

0.2 1.6 2.4 0.5 0.3 1.3 0.1 0.4 0.1

0.9 2.6 4.0 1.3 1.0 3.6 0.3 0.7 0.4

0.8 1.9 3.5 1.5 0.6 3.0 0.2 0.5 0.4

1.1 2.6 3.3 1.3 1.0 3.7 0.4 0.7 0.5

1.2 2.4 4.0 1.3 0.9 2.9 0.6 1.6 1.1

1.1 2.3 4.1 1.4 0.6 3.8 0.8 1.3 1.1

0.5 2.6 3.1 0.7 0.4 3.3

0.6 2.5 3.4 1.0 0.4 3.8 0.4 0.8 0.5

0.4 0.6 0.4

0.3 1.0 0.8 0.4 0.8 2.2

0.3 0.8 0.8 0.4 0.4 0.9 0.4 1.1 2.1

0.4 0.5 1.0 0.5 0.3 0.7 0.3 1.0 1.1

0.3 0.7 0.9 0.4 0.3 0.7 0.5 1.0 0.5

0.2 0.2 0.3 0.3 0.2 0.3

0.3 2.8 1.5 0.4 0.7 1.6 0.3 0.7 1.9

1.0 2.0 4.3 1.3 1.1 4.3 0.5 1.1 0.7

1.0 2.5 2.6 1.4 1.0 4.4 0.4 0.7 0.5

0.7 2.5 3.5 1.5 0.7 4.3 0.2 0.6 0.5

0.9 2.6 3.4 1.1 0.9 3.4 0.3 0.6 0.3

0.7 0.8 2.1 0.6 0.1 1.4 2.4 2.7

0.7 1.7 1.7 0.8 0.9 2.3 0.4 0.9 0.9

0.7 2.4 2.3 1.0 1.0 2.9 0.3 0.5 0.5

1.0 2.7 4.2 1.1 0.9 3.8 0.2 0.5 0.3

0.8 2.2 3.0 0.9 0.8 3.4 0.2 0.4 0.3

0.9 3.2 3.9 1.1 0.9 4.1 0.7 1.3 1.0

1.0 0.5 1.0 0.6

0.7 2.5 3.0 1.2 0.9 3.9 0.3 0.6 0.5

0.6 1.8 2.0 0.8 0.7 2.5 0.4 0.7 0.6

0.1 0.3 0.5 0.2 0.2 0.5

1.1 0.4

0.6 2.6 4.8 1.0 0.6 3.4 0.9 1.8 1.0

0.3 1.2 1.0 0.4 0.5 1.0

0.2 1.5 1.2 0.4 0.4 1.1 1.0 0.8 0.8

0.8 1.9 2.7 1.2 0.7 3.2 0.3 0.4 0.4

0.4 1.2 2.1 0.7 0.4 2.2 0.2 0.4 0.2

1.1 2.4 2.8 1.2 0.7 3.2 0.6 1.1 1.1
0.2 1.2 0.8 0.4 0.3 0.9 0.5 1.2 0.5

0.4 1.3 1.9 0.6 0.4 1.8 0.4 0.8 0.6

0.6 0.9

0.1 0.3 0.5 0.2 0.1 0.5

0.4 1.8 2.2 0.7 0.4 2.6 0.3 0.6 0.4

0.3 1.1 1.3 0.4 0.2 1.6 0.2 0.4 0.2

0.3 0.5 0.8 0.6 0.5 0.7 0.2 0.9 0.6

0.4 0.8 1.5 0.6 0.5 1.1 0.2 0.8 0.6

0.4 0.6 1.4 0.7 0.4 1.1 0.3 0.6 0.7

0.3 0.6 1.3 0.4 0.4 1.2 0.2 0.8 0.8

0.3 0.8 1.1 0.5 0.4 1.0 0.4 0.7 0.8

0.3 0.6 1.2 0.4 0.4 1.0 0.2 0.8 0.7

0.3 0.7 1.0 0.5 0.4 1.0 0.3 0.9 0.6

0.4 1.6 2.5 0.8 0.3 2.2 0.4 1.8 1.6

0.7 1.9 2.2 0.9 0.7 2.8 0.3 0.5 0.5

0.5 1.9 2.7 0.6 0.6 1.8 0.4 0.4 0.6

0.3 0.9 1.0 0.6 0.4 0.8 0.7 0.9 0.6

0.6 2.2 3.2 0.9 0.6 2.5 0.4 1.3 0.4

0.7 2.4 5.4 1.2 0.9 2.5 0.3 0.7 0.5

0.7 1.8 2.8 0.8 0.6 2.0 1.2 1.5 0.8

0.8 2.3 2.3 1.0 0.9 3.7 0.4 0.6 0.4

0.8 2.3 2.8 1.5 0.7 3.2

0.9 2.1 3.2 1.1 0.8 2.8 0.6 2.1 1.4

1.0 3.1 5.6 1.1 0.7 2.6 0.3 0.7 0.5

0.3 2.6 1.7 0.6 0.5 2.0 0.4 0.7 1.3

0.3 1.8 1.9 0.6 0.6 1.9 0.6 1.0 1.3

0.2 1.2 1.0 0.3 0.3 0.6 0.6 0.4

0.1 0.4 0.5 0.2 0.3 0.6 0.7 1.3

0.2 0.2 0.2 0.2 0.2 0.3 0.4 0.3

1.4 2.2 5.0 1.9 1.2 3.9 0.2 0.5 0.3

0.7 1.4 1.1

0.6 1.2 2.4 0.8 0.4 2.3 0.2 0.4 0.2

3.7

4.5 1.7 1.0 4.0

1.9 2.1 4.8 2.0 1.5 4.4 0.2 0.5 0.3

2.7 1.4 0.7 2.9

1.0 2.1 3.3 1.4 0.7 3.5 0.3 0.9 0.6

0.7 1.7 2.6 0.7 0.7 2.5

0.3 1.4

1.0

1.0 2.1 4.4 1.5 1.2 3.6 0.5 0.7 0.6

0.2 0.9 0.4

0.5 0.9 1.8 0.5 0.4 1.8 0.1

0.3 0.6 1.0
0.2 0.4 1.0 0.4 0.3 0.6 0.2 0.6 0.8

0.3 0.7 1.8 0.4 0.4 1.0 0.2 1.0 0.8

0.3 0.5 0.8 0.4 0.3 0.7

0.7 2.2 2.1 1.0 0.5 2.8 0.2 0.7 0.6

0.4 1.9 1.4 0.6 0.6 1.5 0.3 0.7 1.0

0.4 0.8 1.1 0.6 0.5 1.1 0.3 1.2 0.9

0.3 0.6 1.1 0.5 0.4 0.9 0.3 0.5 0.6

0.2 0.6 0.9 0.3 0.3 0.9 0.4 1.2 1.8

0.4 1.5 1.1 0.7 0.6 1.8 0.3 0.6 0.9

0.2 0.3 0.8 0.6

0.6 2.0 1.6 0.6 0.7 1.5 0.5 1.1 2.2

0.3 1.1 0.8 0.4 0.4 0.6 1.4 3.1 1.5

0.3 0.5 0.6 0.3 0.4 0.6 0.3 0.7 1.9

0.3 4.3 3.8 0.6 0.5 2.2 0.4 0.9 0.9

0.3 4.4 3.3 0.5 0.4 1.9 1.7 1.4 1.1

0.4 3.6 4.1 0.8 0.6 1.4 0.6 0.9 2.0

0.2 1.3 1.8 0.5 0.4 1.4 0.3 0.6 0.3

0.3 1.0 1.2 0.6 0.4 1.3 0.3 0.7 0.6

0.3 1.3 0.8 0.5 0.7 0.7 0.3 0.3 0.4

0.5 1.0 0.8 0.6 0.7 0.6 0.6 0.3 0.2

0.6 0.9 0.9 0.4 0.3 0.2

0.3 3.4 2.2 0.4 0.5 2.1 0.7

0.4 1.2 1.2 0.6 0.4 1.0 0.5 0.7 0.7

0.3 1.1 1.4 0.6 0.4 1.3

0.6 1.2 1.2 1.0

3.1 3.7 0.8 0.6 2.3

0.6 2.2 3.4 1.1 0.6 3.6 0.1 0.4 0.6

0.7 3.3 4.4 1.1 0.8 2.7 0.3 0.6 0.5

0.4 2.4 3.4 0.4 0.2 2.6 0.3 0.6 0.2

0.8 3.0 4.4 0.7 0.7 2.6 0.4 0.9 0.7
2010 2011 2011 2011 2011 2012 2012 2012 2012

4 1 2 3 4 1 2 3 4

1.2 1.4 1.0 0.9 0.9 0.8 0.8 1.2 0.8

1.9 1.4 1.8 0.9 1.0 1.7 0.9 1.7 1.0

0.4 0.3 0.8 0.5 0.4 0.3 0.6 0.7 0.3

0.6 0.3 0.7 0.7 0.4 0.7 0.6 1.0 0.5

0.5 0.3 0.7 0.5 0.3 0.4 0.6 0.9 0.4

0.9 1.5 2.0 1.6 1.0 1.6 1.9 1.0 1.7

0.7 0.4 0.9 1.0 0.6 0.7 0.9 2.0 0.7

0.4 0.3 0.5 1.2 0.5 0.4 1.3

0.6 1.3 0.6

0.5 0.4 0.5 1.3 0.8 0.6 0.8 1.3 1.0

2.0 2.5 2.3 2.6 2.8 2.9 3.2 3.3 6.7

0.9 0.9 1.1

0.3 0.5 0.5 0.8 0.5 0.5 1.1 0.7 0.3

0.4 0.3 0.4 0.7 0.5 0.3 0.6 0.6 0.4

0.6 0.4 0.5 0.6 0.6 0.4 0.7 0.7 0.6

0.5 0.5 0.6 0.5 1.0 0.6 0.6 0.4 0.5

0.5 0.5 0.5 0.6 0.7 0.7 0.8 0.6 0.5

0.5 0.5 0.3 0.4 0.7 0.5 0.5 0.4 0.5

1.0 0.4 0.5 1.1 0.9 0.5 0.9 1.0 0.3

0.6 0.4 0.7 1.9 0.9 1.0 1.2 1.8 0.8

0.4 0.4 0.7 0.7 1.2 1.6 1.7 0.7 0.4

1.2 1.1 2.1 1.7 1.5 1.2 2.0 0.9 2.2

0.9 0.9 1.5 1.5 0.8 0.9 1.3 1.1

1.0

0.3 0.2 0.4 0.3 0.5 0.4 0.5 0.6 0.4

0.5 0.5 0.8 1.6 0.3 0.4 1.5 3.6 0.3

0.3 0.3 0.6 1.0 0.3 0.5 1.0 2.1 0.5

0.4 0.3 0.6 0.6 0.3 0.4 0.4 1.4 0.3

0.4 0.7 1.7 0.9 0.4 0.8 1.4 1.4 0.8

0.4 0.2 0.5 0.5 0.3 0.4 0.5 0.8 0.4

0.7 0.4 0.7 0.6 0.3 0.5 0.7 0.6 0.5

0.4 0.3 0.7 0.5 0.3 0.3 0.6 0.9 0.4

1.8 1.0 1.7 1.9 2.0 0.6 2.6 1.5 1.2

0.4 0.4 0.4 0.4 0.4 0.4 0.5 0.4 0.4

0.2 0.2 0.4 0.3 0.2 0.2 0.5 0.3 0.2

0.5 0.4 0.4 0.3 0.4 0.4 0.5 0.4 0.5

0.9 0.7 1.3 1.8 0.7 0.6 1.3 1.3 1.4

1.1 0.4 0.7 1.0 0.8 0.7 1.1 1.4 0.9

0.4 0.3 0.4 0.4 0.4 0.3 0.7 0.6 0.5

0.3 0.2 0.3 0.2 0.2 0.2 0.3 0.5 0.2

Speciation Measurements

Crustal
0.6 0.4 0.5 0.7 0.7 0.5 0.6 0.7 0.4

1.0 0.4 0.7 1.0 0.6 0.5 0.9 2.5 0.8

0.3 0.3 0.4 0.4 0.4 0.4 0.5 0.5 0.3

0.4 0.3 0.4 0.4 0.5 0.3 0.5 0.4 0.4

0.2 0.3 0.3 0.2 0.2 0.2 0.3 0.2 0.2

0.8 0.3 0.3 0.6 0.4 0.4 0.6 0.7 0.3

0.3 0.2 0.3 0.3 0.2 0.2 0.5 0.3 0.3

0.1 0.1 0.2 0.2 0.2 0.2 0.3 0.3 0.1

0.3 0.2 0.4 0.8 0.4 0.4 0.7 0.5 0.4

0.3 0.2 0.4 0.3 0.3 0.3 0.5 0.4 0.3

0.4 0.4 0.7 0.6 0.4 0.4 0.8 0.5 0.5

1.1 0.8 1.1 1.0 0.7 1.3 1.9 0.9 0.8

2.1 0.9 0.8 1.1 1.0 1.5 2.4 2.3 1.6

0.2 0.3 0.4 0.4 0.3 0.6 0.6 0.4

1.0 0.5 0.7 0.5 0.5 0.3 0.6 0.8 0.5

0.7

0.6 0.3 0.7 0.8 0.3 0.3 0.5

1.7 1.0 1.3 0.8 0.4 0.3 0.6 1.3 0.3

0.6 0.2 0.6 0.7 0.3 0.4 0.6 1.1 0.3

0.4 0.3 0.5 0.4 0.3 0.4 0.6 0.6 0.4

0.4 0.4 0.4 0.3 0.8 0.6 0.1 0.2

0.8 0.5 0.6 1.5 0.4 0.3 0.7 1.5 0.7

0.8 0.4 1.2 1.7 0.8 0.5 1.1 1.0 0.6

0.5 0.3 0.6 0.5 0.4 0.2 0.7 0.8 0.4

0.5 0.2 0.4 0.4 0.4 0.3 0.6 0.9 0.3

1.1 0.4 0.6 0.7 0.3 0.3 0.6 0.5 0.4

3.9 2.8 3.8 1.9 4.8 2.1 3.6 0.0

1.2 0.6 0.9 0.8 1.0 1.0 1.1 1.2 0.7

0.5 0.3 0.6 0.4 0.3 0.3 0.6 0.8 0.3

0.5 0.3 0.4 0.4 0.4 0.3 0.5 0.4 0.3

0.3 0.3 0.5 0.3 0.2 0.2 0.5 0.3 0.3

0.9 1.0 0.8 0.8 0.6 0.9 1.5 1.0 1.0

0.6 0.5 1.2 0.7

0.5 0.3 0.6 0.5 0.4 0.4 0.6 0.9 0.4

0.6 0.4 0.8 0.5 0.3 0.3 0.6 0.8 0.4

0.2 0.2 0.4 0.1 0.2 0.4 0.5 0.1

0.6

0.9 0.4 0.7 1.1 1.1 1.2 1.6 2.3 0.7

0.9 0.9 0.9 1.3 1.3 1.7 2.2 1.6 1.6

0.5 1.0 0.5 0.7 0.9 0.7 1.2 0.6 0.6

0.4 0.3 0.4 0.5 0.5 0.4 0.6 0.6 0.4

0.2 0.1 0.2 0.3 0.2 0.2 0.3 0.3 0.2

0.6 0.4 0.6 0.7 0.7 0.5 0.7 0.6 0.6
0.5 0.8 1.8 1.0 0.7 0.9 1.9 0.9 1.0

0.4 0.5 0.6 0.3 0.7 0.4 0.6 0.6 0.4

0.1 0.2 0.2 0.1 0.1 0.2 0.2 0.1

0.2 0.3 0.3 0.3 0.3 0.3 0.5 0.4 0.3

0.1 0.1 0.2 0.2 0.2 0.2 0.3 0.3 0.2

0.2 0.2 0.5 0.4 0.2 0.3 0.6 0.7 0.2

0.3 0.2 0.5 0.3 0.2 0.3 0.5 0.6 0.3

0.4 0.3 0.5 0.4 0.3 0.3 0.5 0.6 0.5

0.3 0.2 0.4 0.2 0.2 0.2 0.4 0.7 0.3

0.3 0.3 0.5 0.4 0.3 0.3 0.4 0.7 0.3

0.3 0.2 0.5 0.3 0.2 0.2 0.4 0.6 0.2

0.3 0.3 0.5 0.5 0.3 0.3 0.5 0.7 0.3

2.6 0.3 0.6 2.2 1.7 0.7 2.1 3.6 1.0

0.4 0.3 0.5 0.4 0.3 0.4 0.7 0.4 0.6

0.5 0.3 0.4 0.4 0.3 0.5 0.7 0.6 0.3

0.8 0.5 0.2 0.8 0.9 1.3 1.2 0.8 0.8

0.5 0.2 0.4 0.4 0.7 0.8 0.9 0.9 1.0

0.7 0.3 0.4 0.5 0.7 0.4 0.6 0.6 0.3

1.3 0.8 0.8 0.9 0.9 0.6 1.7 1.4 1.1

0.5 0.2 0.5 0.4 0.4 0.4 0.7 0.8 0.7

0.2 0.4 0.2 0.2 0.2 0.3 0.7 0.3

1.2 0.6 0.8 0.9 0.9 1.2 1.0 1.1 0.6

0.2 0.2 0.5 0.3 0.3 0.5 1.0 0.5 0.3

0.6 0.6 1.0 1.3 0.4 0.6 1.1 1.8 0.7

0.6 0.5 0.8 1.0 0.5 0.7 0.8 2.1 1.1

0.3 0.6 0.3 0.7 0.4 0.5 0.5 1.3

0.8 0.7 0.6 1.1 0.4 0.6 0.9 1.5

0.1 0.2 0.2 0.3 0.1 0.1 0.3 0.5

0.2 0.2 0.3 0.2 0.3 0.3 0.4 0.4 0.3

1.3

0.2 0.1 0.3 0.2 0.2 0.3 0.3 0.3 0.3

0.2

0.4 0.5 0.5 0.4

0.2 0.2 0.3 0.3 0.3 0.4 0.4 0.4 0.4

0.4 0.5 0.9 0.5

0.4 0.3 0.4 0.4 0.4 0.3 0.6 0.5 0.4

0.2 0.4 0.3 0.4 0.3 0.5 0.4 0.3

0.5 0.4

0.4

0.4 0.4 0.5 0.7 0.5 0.5 0.8 0.6 0.5

0.2 0.2 0.2 0.3 0.2 0.3 0.5 0.3 0.2

0.4
0.2 0.1 0.5 0.5 0.2 0.2 0.5 1.0 0.2

0.3 0.3 0.7 0.4 0.2 0.2 0.5 0.8 0.3

0.3 0.7 0.6 0.3 0.3 0.5 0.8 0.4

1.1 0.2 0.4 1.0 0.6 0.5 1.0 1.0 0.5

0.5 0.3 0.6 0.5 0.4 0.4 0.6 0.7 0.4

0.4 0.4 0.6 0.5 0.4 0.5 1.2 1.1 0.8

0.4 0.2 0.8 0.4 0.4 0.4 0.6 0.8 0.4

0.7 0.4 0.9 0.6 0.4 0.5 0.7 0.7 0.3

0.3 0.2 0.5 0.5 0.3 0.4 0.6 0.8 0.4

0.2 0.2 0.4 0.4

0.6 0.6 1.1 2.1 0.6 0.9 1.0 3.0 1.0

3.7 3.2 6.2 2.5 2.1 2.5 2.8 2.5 2.8

0.3 0.3 1.0 0.9 0.3 0.6 0.8 2.3 0.7

0.5 0.5 0.9 1.0 0.7 0.8 1.3 1.1 0.6

0.6 0.8 0.9 0.8 0.7 0.9 1.2 1.0 0.8

0.8 0.7 1.2 1.0 0.8 1.0 1.7 1.1 0.6

0.1 0.2 0.7 0.5 0.2 0.4 0.4 0.3 0.2

0.3 0.2 0.4 0.3 0.3 0.3 0.4 0.6 0.3

0.2 0.4 0.1 0.3 0.3 0.2 0.3 0.7 0.3

0.3 0.3 0.2 0.3 0.2 0.2 0.3 0.4 0.1

0.3 0.3 0.2 0.2 0.3 0.3

0.5 0.5 0.2 0.7 0.4 0.4 0.6 1.1 0.4

0.5 0.3 0.6 0.4 0.5 0.6 0.7 0.8 0.8

0.6 1.3 1.9 0.9 1.0 0.9

1.0 0.7 0.8 0.9

0.2 0.2 0.4 0.4 0.2

0.3 0.2 0.2 0.3 0.5 0.5 0.5 0.6 0.2

0.5 0.2 0.4 0.4 0.4 0.4 0.5 0.5 0.3

0.3 0.2 0.3 0.2 0.3 0.3 0.5 0.4 0.2

0.7 0.5 0.6 0.9 0.5 0.7 1.0 0.9 0.5
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

3.4 5.2 2.9 3.1 2.6 3.0 2.9 2.9 2.0

3.4 3.8 3.7 5.1 3.7 5.3 5.5 3.3 3.3

3.0 2.9 3.0 3.6 2.8 4.1 3.6 2.6 3.2

3.5 3.1 2.8 4.5 2.9 4.1 3.7 3.0 3.5

5.7 5.5 3.0 6.4 5.4 7.3 4.2 3.2 5.5

2.1 1.2 0.9 2.1 2.1 0.9 1.0 2.0 2.0

2.7 3.7 3.5 4.6 2.9 2.8 2.5 2.5 1.6

5.4 1.6 3.2 7.5 11.2 1.8 2.9 15.1 7.8

5.5 2.0 3.5 6.4 5.1 1.8 3.3 9.3 7.0

3.1 3.4 4.3 5.2 4.9 3.1 3.4 7.1 6.5

9.9 7.1 8.3 7.8 10.0 8.2

15.8 5.8 3.2 14.2 16.3 5.6 2.8 24.9 27.2

4.9 1.1 2.0 5.3 4.4 1.2 2.2 7.5 6.5

3.7 1.1 2.8 4.4 3.0 1.5 2.6 7.0 4.0

4.5 1.8 2.4 5.1 3.7 1.9 2.6 6.3 3.2

5.1 2.5 3.0 5.6 3.3 1.8 3.1 6.1 3.3

3.5 1.8 2.6 4.2 4.0 2.0 2.3 6.1 4.5

3.8 1.5 4.1 5.3 5.0 1.8 2.5 9.6 3.8

4.1 3.0 4.7 4.7 4.3 2.4 4.5 7.9 7.0

1.9 2.0 3.3 2.2 1.7 2.1 3.5 2.4 1.5

3.2 1.7 2.1 2.7 2.2 1.6 2.7 3.3 2.8

3.2 1.8 1.7 2.3 1.8 1.8 2.3 2.4 2.6

3.1 2.8 3.6 2.7 2.0 3.0 3.3 3.1 2.3

2.3 0.8 0.5 1.5 1.6 2.0 0.7 0.8 1.3

2.3 2.2 1.9 2.9 2.9 2.8 1.8 2.1 3.0

3.5 3.4 2.4 6.1 5.0 3.6 3.8 3.3 5.0

4.9 5.3 3.8 5.0 5.5 5.5 5.6 3.1 4.8

2.7 4.1 3.2 4.5 3.9 4.4 3.3 3.5 4.0

3.6 5.0 3.9 6.2 3.6 4.7 3.7 3.1 3.8

5.3 6.4 3.6 4.7 4.1 6.1 4.5 3.6 5.0

1.4 1.1 1.7 1.9 1.5 1.2 2.0 2.3 1.6

2.3 2.6 2.4 2.7 2.4 2.2 2.8 3.0 2.4

2.2 2.5 3.5 2.5 1.6 2.2 1.1 1.6 2.1

3.5 2.9 3.8 3.0 2.4 2.7 3.0 2.6 2.7

1.5 1.8 2.7 2.1 2.3 2.8 2.0 2.3 1.8

3.5 3.0 3.1 4.0 3.3 3.9 2.9 4.4 4.0

3.3 3.2 3.3 3.9 2.7 3.1 3.5 3.3 3.5

2.0 2.3 2.8 2.6 1.5 2.3 2.4 1.4 2.0

Speciation Measurements

Organic Carbon
2.6 1.9 3.4 3.7 1.9 2.6 3.6 1.8 2.5

3.0 2.1

2.7 3.2 2.8 4.1 3.3 3.1 3.0 3.5 2.2

3.3 2.8 3.3 3.4 3.2 2.9 3.1 3.8 3.4

2.2 2.9 2.6 2.3 1.8 2.6 2.8 2.3 2.1

1.7 2.7 2.4 2.6 3.1 2.0 4.3 2.8 3.3

2.5 2.7 3.3 3.7 2.6 2.5 2.9 3.0 2.3

2.0 2.7 2.7 2.7 2.2 1.9 2.2 1.8 1.8

1.0 2.0 2.1 1.4 0.9 1.8 2.0 1.0 1.6

2.2 2.4 2.6 3.0 1.9 1.8 2.8 1.9 2.0

1.3 2.9 3.2 3.0 2.0 2.3 2.6 1.8 2.5

2.3 2.0 3.2 2.7 2.5 2.4 2.6 2.3 1.9

2.4 3.5 3.7 3.5 2.5 2.2 3.4 2.2 2.6

2.2 3.5 3.8 3.6 2.7 2.3 3.4 2.6 3.0

1.9 2.2 2.2 2.2 1.7

2.7 2.2 3.0 2.6 2.5 2.2 2.5 2.5 2.0

2.7 2.4 2.6 2.7

3.6 3.1 3.5 3.1 5.3 3.7 3.4 2.1

4.6 3.5 3.9 7.0 3.4 4.4 4.8 3.7 2.9

4.4 4.6 3.1 4.8 2.6 4.4 6.3 3.1 5.4

4.3 2.7 2.8 6.6 4.1 4.4 3.9 5.4 5.8

0.0 -0.1 -0.1 -0.2 -0.1

2.0 1.1 2.4 2.6 2.7 1.1 3.3 4.1 1.9

3.6 2.9 3.9 4.4 2.9 3.5 3.6 3.6 3.3

3.1 2.6 3.2 3.1 2.2 2.8 2.9 2.4 2.2

2.6 1.9 3.0 3.4 2.4 1.9 2.4 2.4 1.9

2.4 2.8 3.5 3.3 2.5 3.0 3.2 1.9 2.2

2.5 2.6 3.8 4.5 3.8 3.8 3.9 3.8 2.2

3.5 2.8 3.5 5.0 2.7 3.4 3.8 3.3 3.0

3.3 2.4 3.3 3.3 3.1 3.1 3.0 2.2 2.6

2.6 2.5 4.7 4.4 2.7 2.6 3.2 3.1 2.9

2.1 2.1 2.5 3.8 2.0 2.3 2.2 1.3 1.5

3.2 2.5 3.8 3.6 3.2 3.1 3.2 1.9 2.5

3.1 2.6 3.7 3.4 2.6 2.7 3.2

2.7 3.1 3.5 3.8 2.9 3.2 3.4 2.6 2.6

2.6 2.8 3.5 3.5 2.9 3.2 3.2 2.1 3.0

0.3 0.5 2.5 0.8 0.3

9.6

1.7 2.2 2.2 1.4 1.6 2.5 2.1 2.0 2.0

3.0 3.8 1.3 1.7 4.9 4.3

3.4 1.2 2.3 3.4 3.3 1.3 2.9 4.6 2.8

2.4 4.1 4.1 3.0 2.8 3.0 5.1 4.2 2.3

1.9 2.2 2.2 1.6 0.8 1.7 2.3 1.8 1.8

2.7 3.1 3.0 2.9 2.8 3.2 3.5 3.8 2.9
2.6 1.1 1.2 2.6 2.6 3.9 1.6 2.8 2.1

2.1 2.9 2.8 3.5 3.5 2.2 3.4 2.5 2.3

2.7 3.5

0.6 0.9 2.6 0.4 0.4

1.5 2.1 2.4 1.9 2.0 2.3 2.4 1.9 1.6

1.1 1.8 1.9 1.3 1.0 1.2 1.8 1.3 1.1

2.4 2.8 3.0 3.2 2.4 3.2 2.8 2.4 3.0

4.0 3.5 3.5 5.4 3.5 4.1 3.5 3.4 4.7

4.1 3.4 3.4 6.2 3.2 3.4 3.3 3.3 3.9

2.3 3.2 3.7 3.9 2.1 2.6 2.4 3.0 3.8

2.9 3.7 3.3 4.3 2.9 4.1 3.2 3.9 3.7

3.0 3.7 3.3 5.1 2.7 3.1 3.4 3.6 3.1

2.5 4.1 3.8 3.8 3.1 3.6 4.3 3.2 3.4

1.2 1.8 2.1 1.5 0.8 0.9 1.8 1.7 0.9

2.8 2.3 3.5 3.2 2.2 2.5 2.7 2.4 2.3

2.5 2.9 3.3 4.2 2.3 2.9 3.1 3.5 3.5

3.5 3.0 3.1 3.3 2.0 3.3 3.1 3.0 4.4

2.1 2.7 3.2 2.8 2.2 2.3 3.6 2.8 2.7

2.3 2.5 2.8 3.1 2.1 2.0 3.2 2.1 2.7

2.7 2.9 3.4 3.8 2.0 2.0 3.2 2.5 2.5

3.0 2.6 3.5 3.8 2.0 3.0 2.9 2.7 2.5

2.2 2.3 2.1 1.8 1.8

3.8 3.4 4.0 4.0 2.4 2.8 3.0 2.9 3.1

2.6 3.5 3.3 3.5 2.3 3.5 3.4 2.3 2.5

1.2 1.7 3.1 2.1 2.1 2.6 2.2 2.2 1.6

2.9 2.9 2.5 2.4 3.1 3.9 2.6 2.5 2.5

10.2 2.2 0.9 12.3 10.1 4.4 2.5 13.1 11.2

5.9 1.7 2.4 8.5 13.8 2.6 2.7 10.5 12.5

9.2 1.5 1.5 7.3 10.0 2.5 2.4 11.0 12.7

2.3 2.9 2.7 2.4 1.8 2.1 2.6 2.1 3.3

3.3 3.1 3.2 4.9

2.0 2.5 2.1 2.3 1.2 2.1 2.3 2.2 2.6

2.9

2.9 3.4 3.0 3.0 2.3 2.6 2.9 2.8 3.5

1.9

2.6 3.8 3.1 2.7 2.2 3.7 3.7 2.7 2.7

1.4 3.0 2.9 2.7 2.1

2.8 3.2 2.8 3.0 2.1 2.7 3.5 2.4 3.2

1.8 2.3 2.7

1.4 2.5 2.2 1.7 2.5 2.3 2.7

3.1 2.3 1.7 3.6
3.1 3.2 3.2 2.7 2.1 3.5 3.6 2.2 3.0

2.9 4.2 3.8 5.8 3.2 4.7 4.1 3.0 4.8

3.8 3.7 4.0 3.3 3.9

1.3 1.6 1.9 1.8 1.0 1.2 2.0 2.0 1.2

3.6 2.8 3.0 4.3 2.8 2.9 3.5 3.4 3.1

3.4 4.0 3.7 5.2 4.0 5.2 3.9 3.5 3.9

4.0 3.2 3.5 3.9 2.2 4.2 3.0 2.5 3.3

2.0 2.8 2.5 2.8 1.9 3.2 2.8 2.0 2.4

2.2 2.4 3.3 3.2 2.2 3.4 4.1 3.0 2.7

2.4 4.3 3.9 4.7 2.2 4.4 6.0

2.3 1.9 2.4 2.8 2.7 3.4 2.4 2.7 2.3

3.8 1.5 1.6 4.7 3.1 2.9 1.7 2.1 2.3

3.0 3.5 3.6 3.8 10.3 3.2 3.8 3.3 2.7

1.7 0.8 1.7 1.7 1.6 0.7 1.8 2.5 1.7

2.8 1.0 1.8 2.7 2.4 1.2 2.2 3.2 2.2

2.6 0.9 1.9 1.6 2.2 1.4 1.8 2.5 1.9

1.7 2.5 2.7 2.0 2.1 1.8 3.8 2.5 2.6

2.6 3.0 3.5 3.0 2.4 3.2 3.0 3.6 3.1

3.6 1.3 1.9 5.3 7.5 1.0 1.6 8.2 4.9

4.7 1.5 1.8 6.3 7.5 0.9 1.8 6.4 6.1

4.8 1.6 2.3 5.4 6.3 1.6 2.1 6.7 4.5

3.9 6.6 6.7 0.8 2.6 6.1 5.5

3.5 3.3 4.1 4.4 2.6 3.2 3.2 3.0 3.7

1.7 3.5 5.0

3.1 2.6 3.0 3.9 2.6 2.4 3.3

1.8 1.6

1.9 1.8 2.3 1.8 1.5 1.8 2.0 1.9 2.0

2.2 2.4 3.0 2.5 2.1 2.3 2.6 2.5 2.4

1.2 1.8 2.3 1.6 1.3 1.7 1.9 1.8 1.7

2.3 2.7 3.4 3.8 1.8 2.7 2.9 2.5 2.6
2012 2012 2012 2010 2010 2010 2010 2011 2011

2 3 4 1 2 3 4 1 2

2.3 2.0 3.6 1.1 1.3 0.7 1.0 0.6 0.7

4.0 3.4 3.4 0.7 0.7 0.7 1.1 0.7 0.8

3.2 2.8 2.8 0.5 0.4 0.5 0.6 0.5 0.5

3.3 2.6 4.8 1.0 0.4 0.4 0.9 0.7 0.5

3.4 2.9 5.2 1.0 0.7 0.4 1.3 0.9 0.6

0.9 1.1 1.9 0.6 0.3 0.3 0.6 0.6 0.2

3.6 3.2 4.5 0.6 0.6 0.6 0.8 0.5 0.4

2.7 0.6 0.2 0.5 1.3 1.3 0.7

2.4 4.1 4.5

2.3 3.2 6.2 1.0 0.3 0.5 1.2 0.8 0.3

5.1 3.2 8.8 0.6 0.6 0.8 0.8 0.9 0.4

1.9 1.1 1.4 1.8 1.6 1.0

7.0 3.4 13.6 1.6 0.7 0.4 1.4 1.5 0.5

1.6 2.7 5.2 1.0 0.2 0.4 1.1 0.8 0.2

1.9 3.6 3.9 0.7 0.3 0.5 0.9 0.5 0.3

1.9 2.2 5.6 0.9 0.4 0.5 1.2 0.8 0.4

2.4 2.9 4.9 0.9 0.4 0.5 1.0 0.6 0.3

2.2 2.4 3.9 0.6 0.2 0.4 1.0 0.8 0.3

2.3 3.2 3.3 0.7 0.3 0.6 1.2 0.7 0.3

3.8 4.0 4.2 0.6 0.3 0.6 0.8 0.6 0.3

2.1 3.4 2.2 0.5 0.3 0.6 0.6 0.4 0.4

1.4 3.0 2.2 1.4 0.6 0.8 1.3 1.0 0.5

2.1 3.1 1.1 0.6 0.6 1.0 0.8 0.5

2.2

2.2 3.1 3.4 0.7 0.5 0.6 0.7 0.5 0.5

1.1 0.7 1.1 0.6 0.3 0.3 0.5 0.5 0.4

2.2 1.3 2.2 0.5 0.3 0.3 0.7 0.5 0.4

2.6 2.8 4.1 0.8 0.5 0.3 1.2 0.9 0.5

4.4 3.7 4.9 0.9 0.7 0.5 1.0 0.8 0.7

3.5 3.2 4.4 1.1 1.4 1.4 1.5 1.1 1.3

4.2 3.1 4.4 0.7 0.9 0.6 1.6 1.3 1.6

3.9 3.0 4.8 0.9 0.7 0.5 0.8 0.6 0.7

2.4 3.1 1.9 0.5 0.3 0.5 0.8 0.5 0.3

2.3 2.7 3.3 0.8 0.9 0.7 1.0 0.8 0.8

1.6 2.2 2.4 0.5 0.4 0.5 0.5 0.3 0.3

2.5 2.9 2.9 0.9 0.6 0.7 1.0 0.6 0.6

2.9 2.3 2.1 0.4 0.3 0.4 0.4 0.4 0.4

3.7 3.6 3.8 0.6 0.5 0.7 0.7 0.5 0.5

3.7 3.2 3.7 0.7 0.7 0.7 0.8 0.5 0.6

2.8 2.6 2.0 0.4 0.3 0.5 0.5 0.3 0.4

Speciation Measurements

Elemental Carbon
2.8 2.8 2.4 0.5 0.4 0.5 0.8 0.4 0.5

0.7 0.7

2.8 2.5 3.8 0.7 0.7 0.6 0.9 0.7 0.7

2.7 2.9 4.7 0.7 0.6 0.6 1.0 0.9 0.6

2.5 3.0 3.0 0.6 0.6 0.7 0.7 0.4 0.5

2.4 2.6 2.4 0.3 0.5 0.4 0.6 0.8 0.4

2.7 3.2 3.2 0.5 0.6 0.7 0.8 0.5 0.5

2.1 2.4 2.1 0.4 0.4 0.5 0.5 0.4 0.3

1.1 2.1 1.0 0.1 0.2 0.2 0.2 0.1 0.2

2.1 2.9 2.8 0.5 0.4 0.8 0.7 0.4 0.4

2.7 2.9 2.5 0.2 0.5 0.5 0.6 0.4 0.4

2.3 3.0 2.5 0.8 0.7 1.0 0.8 0.6 0.7

2.6 3.1 2.3 0.6 1.1 1.1 1.1 0.6 0.6

2.9 3.7 3.1 0.5 0.7 1.0 1.1 0.6 0.7

2.1 2.5 2.4 0.3 0.4

2.2 3.0 2.6 0.5 0.4 0.5 0.6 0.5 0.4

0.5 0.4 0.5 0.6

3.7 0.5 0.5 0.7 0.6 0.7

3.5 2.9 3.6 0.8 0.6 0.6 1.2 0.6 0.5

3.2 2.9 4.6 0.7 0.6 0.4 1.0 0.5 0.5

4.4 3.4 6.0 0.7 0.5 0.5 0.9 0.5 0.7

-0.1 0.0 -0.2 0.1 0.1

1.4 8.3 2.7 0.5 0.3 0.4 0.6 0.6 0.3

2.5 4.3 2.8 0.8 0.7 0.9 1.0 0.6 0.9

2.4 3.0 2.4 1.0 0.7 0.9 0.8 0.6 0.8

2.7 3.5 2.6 0.5 0.5 0.8 0.8 0.4 0.4

1.9 3.2 2.6 0.5 0.6 0.7 0.8 0.5 0.6

1.7 4.8 0.6 0.6 1.0 1.0 0.8 0.9

3.4 3.6 3.6 0.6 0.7 0.8 1.1 0.6 0.7

2.8 3.2 2.7 0.6 0.4 0.6 0.7 0.5 0.5

2.5 3.5 3.1 0.5 0.4 0.7 0.8 0.4 0.5

1.6 2.1 1.7 0.4 0.3 0.4 0.6 0.3 0.4

2.8 3.6 2.6 1.0 1.2 1.4 1.0 1.1 0.8

0.7 0.9 1.0 0.9 0.6 0.7

3.1 3.1 2.9 0.6 0.6 0.8 0.9 0.6 0.7

3.0 3.3 2.9 0.5 0.5 0.6 0.6 0.5 0.5

0.9 6.0 0.6 0.1 0.1

6.8 1.4

1.6 2.7 1.8 0.4 0.4 0.4 0.4 0.3 0.4

1.4 2.0 4.4 1.0 1.2 0.3

1.5 2.9 2.7 1.0 0.3 0.5 1.0 0.9 0.3

2.7 3.0 3.0 0.8 1.1 1.1 1.0 0.9 0.8

1.6 2.3 1.9 0.4 0.4 0.4 0.4 0.2 0.3

2.8 2.8 3.5 1.2 1.7 1.7 1.5 1.2 1.6
1.6 2.0 3.2 0.7 0.3 0.4 0.8 0.8 0.5

2.4 2.7 2.7 0.5 0.6 0.6 0.9 0.8 0.5

2.1 1.4

1.4 1.3 0.6 0.1 0.1

1.4 1.9 1.9 0.3 0.5 0.5 0.5 0.4 0.4

1.6 2.1 1.8 0.2 0.3 0.3 0.3 0.2 0.2

3.7 2.3 3.7 0.6 0.5 0.6 0.6 0.4 0.5

3.2 2.9 4.4 0.8 0.6 0.7 1.3 0.7 0.8

3.2 3.0 5.6 0.8 0.5 0.6 1.1 0.5 0.6

3.5 3.3 4.6 0.5 0.5 0.6 0.8 0.4 0.5

3.1 2.9 4.2 0.6 0.6 0.5 0.8 0.5 0.6

3.4 3.0 4.1 0.6 0.4 0.4 0.8 0.4 0.5

3.1 3.2 3.9 0.5 0.6 0.5 0.8 0.5 0.5

1.1 2.1 1.2 0.3 0.3 0.3 0.3 0.2 0.2

2.7 2.7 2.7 0.5 0.6 0.8 0.8 0.4 0.6

3.2 3.3 3.0 0.8 0.7 0.9 1.0 0.6 0.9

3.6 3.2 3.0 1.1 0.9 0.9 1.0 0.5 1.0

3.0 3.4 2.5 0.4 0.5 0.7 0.8 0.4 0.5

2.4 3.0 2.0 0.5 0.5 0.6 0.7 0.4 0.5

3.0 3.5 2.3 0.6 0.8 0.9 0.9 0.5 0.6

3.2 3.4 3.0 0.6 0.8 0.9 1.0 0.5 0.7

1.9 2.3 2.0 0.5 0.7

3.3 3.3 2.8 0.7 0.9 1.0 0.9 0.5 0.7

2.5 2.6 1.8 0.4 0.6 0.6 0.7 0.4 0.6

2.5 2.3 1.9 0.3 0.3 0.4 0.5 0.4 0.3

3.4 2.9 2.9 0.5 0.4 0.3 0.5 0.5 0.5

2.6 6.7 1.4 0.3 0.2 1.8 1.3 0.6

1.5 5.6 0.7 0.3 0.4 1.0 1.6 0.4

2.5 3.8 1.1 0.2 0.2 0.7 1.0 0.3

2.1 3.0 3.4 0.5 0.7 0.7 0.7 0.4 0.5

0.8 0.7 0.6 1.2

1.9 2.1 2.4 0.4 0.4 0.5 0.5 0.3 0.4

2.7

2.5 2.8 3.2

2.8 3.3 4.2 0.6 0.7 0.7 0.8 0.4 0.5

2.3 3.3 4.4

3.2 3.0 3.3 1.1 1.3 1.2 0.9 0.7 0.8

2.0 2.8 2.9 0.4 0.6

2.5 1.7

3.2

3.0 3.3 3.7 0.7 0.8 0.8 0.8 0.5 0.5

0.5 0.4 0.5

1.8 2.6 3.0 0.3 0.6 0.5 0.3

0.6 0.4 0.3 0.6
2.7 3.0 2.4 0.5 0.4 0.4 0.4 0.3 0.5

3.7 3.1 4.5 0.7 0.7 0.6 1.2 0.6 0.6

3.3 3.4 3.8 0.7 0.5

2.1 2.4 1.5 0.3 0.3 0.3 0.4 0.2 0.3

2.8 3.0 3.2 0.7 0.8 0.7 1.2 0.5 0.7

3.9 2.9 4.7 0.7 0.8 0.7 1.1 0.7 0.8

3.6 3.2 4.7 0.8 0.8 0.9 1.0 0.5 0.7

2.4 2.7 2.5 0.4 0.3 0.3 0.4 0.3 0.3

2.6 3.5 2.7 0.4 0.4 0.4 0.5 0.3 0.4

1.2 1.2 0.8 0.9 0.6 0.7

3.0 2.4 2.8 0.6 0.5 0.5 0.8 0.7 0.6

2.2 2.1 3.0 1.2 0.5 0.6 1.2 1.0 0.5

4.2 2.8 4.0 0.5 0.7 0.4 0.6 1.1 0.4

1.1 4.8 1.8 0.6 0.3 0.3 0.6 0.5 0.2

1.5 4.1 2.6 0.9 0.4 0.4 0.9 0.7 0.4

1.3 4.6 1.8 0.6 0.3 0.3 0.5 0.6 0.3

2.2 3.2 2.5 0.3 0.3 0.4 0.4 0.4 0.3

2.7 3.2 3.8 0.6 0.5 0.6 0.7 0.5 0.6

1.6 3.6 4.0 0.7 0.3 0.4 1.0 1.3 0.2

1.7 3.3 5.0 1.0 0.3 0.4 1.5 1.4 0.2

1.1 0.4 0.5 1.1 1.3 0.3

1.2 6.8 5.6 0.8 1.3 1.1 0.2

3.9 3.4 4.0 0.9 0.9 1.1 1.4 0.7 0.9

3.4 2.9 4.6

0.7 0.6 0.7 1.1 0.5 0.6

2.2 3.0 1.7

1.7 2.3 1.7 0.3 0.3 0.3 0.4 0.3 0.3

2.3 3.3 1.6 0.5 0.5 0.7 0.6 0.4 0.4

1.4 2.6 1.1 0.2 0.2 0.2 0.3 0.2 0.2

2.2 3.4 1.5 0.6 0.6 0.7 0.8 0.5 0.6
2011 2011 2012 2012 2012 2012 2010 2010 2010

3 4 1 2 3 4 1 2 3

0.8 0.7 0.6 0.5 0.4 0.9 4.4 5.3 5.6

0.7 0.7 0.8 0.6 0.5 0.7 4.4 4.0 4.9

0.5 0.5 0.5 0.5 0.3 0.5 4.8 4.2 5.2

0.5 0.6 0.6 0.5 0.3 0.7 4.1 4.8 4.1

0.5 0.8 1.1 0.5 0.4 0.8 4.4 5.0 4.4

0.2 0.6 0.6 0.2 0.3 0.6 1.0 1.3 1.7

0.4 0.5 0.4 0.6 0.5 1.1 3.2 3.7 4.4

1.0 2.8 2.4 1.0 0.7 1.3 1.1

0.6 1.3 1.5

0.5 1.6 1.2 0.3 0.5 1.1 2.0 1.9 2.9

0.7 1.2 1.1 0.7 0.5 1.7 1.1 2.4 2.8

1.4 3.8 5.6

0.3 2.1 2.0 0.6 0.2 1.4 0.6 1.1 0.8

0.4 1.2 1.2 0.3 0.3 0.9 1.2 1.4 2.2

0.4 1.1 0.7 0.3 0.4 0.7 1.0 1.1 1.6

0.5 1.4 0.9 0.4 0.4 1.3 1.6 3.0 4.4

0.4 1.0 0.7 0.4 0.5 0.6 1.3 4.0 4.5

0.4 1.3 0.8 0.3 0.4 0.8 1.6 1.7 2.1

0.4 1.5 0.6 0.3 0.4 0.6 1.9 2.0 2.1

0.5 1.0 1.0 0.4 0.6 0.7 1.7 2.1 2.7

0.7 0.7 0.4 0.3 0.5 0.6 1.3 2.8 3.2

1.1 1.5 1.3 0.5 0.8 1.0 1.6 1.7 1.2

0.8 0.9 1.0 0.6 0.7 1.6 1.9 1.2

1.0

0.6 0.9 0.6 0.7 0.6 0.9 3.9 5.2 7.0

0.3 0.3 0.4 0.4 0.3 0.4 3.7 3.2 3.3

0.3 0.5 0.6 0.3 0.2 0.5 3.7 3.8 3.2

0.5 0.7 1.1 0.5 0.4 0.9 4.2 4.0 2.8

0.6 0.8 0.8 0.6 0.4 1.0 4.2 4.6 4.0

1.1 1.5 1.3 0.9 0.9 1.4 4.4 4.4 4.0

1.5 1.1 1.3 1.3 1.0 1.1 5.4 4.7 5.5

0.5 0.6 0.8 0.5 0.3 0.7 4.6 4.5 3.9

0.5 0.9 0.7 0.4 0.5 0.9 1.5 1.6 1.1

1.0 1.3 1.2 1.0 1.1 1.2 2.6 3.2 3.0

0.3 0.4 0.4 0.2 0.4 0.4 4.1 4.1 6.8

0.7 0.8 0.8 0.5 0.6 0.9 6.3 4.4 6.2

0.3 0.5 0.4 0.4 0.4 0.5 3.0 2.5 3.0

0.5 0.6 0.8 0.5 0.6 0.7 3.9 3.2 2.5

0.7 0.6 0.7 0.6 0.6 0.7 6.0 5.7 5.9

0.4 0.3 0.3 0.3 0.3 0.3 6.0 5.4 7.0

Speciation Measurements

Elemental Carbon
0.7 0.5 0.6 0.5 0.5 0.5 5.5 5.9 6.9

4.9 6.0

0.7 0.8 0.7 0.5 0.5 0.7 4.9 5.5 4.3

0.7 1.1 1.0 0.5 0.7 1.0 4.1 4.5 6.3

0.6 0.7 0.5 0.5 0.6 0.7 4.6 3.6 5.6

0.8 0.6 0.7 0.5 0.4 0.5 2.2 2.7 3.1

0.6 0.6 0.5 0.5 0.6 0.7 2.5 3.4 4.4

0.4 0.4 0.4 0.3 0.4 0.4 2.9 4.2 5.1

0.2 0.2 0.3 0.2 0.2 0.2 1.7 2.6 2.7

0.7 0.6 0.6 0.5 0.7 0.5 3.3 3.7 6.0

0.5 0.3 0.5 0.5 0.5 0.5 1.7 3.7 4.6

1.0 0.8 0.5 0.7 0.9 0.7 3.2 3.7 5.1

1.1 0.7 0.8 0.9 0.9 0.7 2.9 5.8 6.5

0.9 0.9 0.9 0.8 0.9 0.8 2.6 4.3 4.3

0.5 0.5 0.4 0.4 0.4 0.5

0.6 0.5 0.4 0.4 0.5 0.6 2.8 2.4 2.0

2.7 2.4 2.4

0.6 0.7 0.5 0.5 4.0 3.7

0.7 0.7 0.6 0.5 0.4 0.7 4.2 4.3 4.2

0.5 0.6 0.8 0.4 0.3 0.9 4.4 6.0 5.3

0.7 0.8 0.8 0.7 0.5 0.8 4.0 4.1 4.9

0.1 0.1 0.1 0.1 0.1 0.1

0.6 0.9 0.5 0.3 0.9 0.6 1.0 0.9 0.9

0.9 1.1 0.8 0.7 1.0 0.7 3.6 3.8 4.7

0.8 0.7 0.6 0.7 0.8 0.6 2.7 4.2 4.2

0.6 0.7 0.5 0.5 0.7 0.6 2.3 4.6 4.1

0.7 0.5 0.5 0.4 0.6 0.6 2.9 4.9 3.6

0.8 1.1 0.8 0.6 0.9 4.3 4.2 5.2

0.9 0.8 0.8 0.7 0.7 0.8 5.1 6.1 7.1

0.6 0.5 0.5 0.4 0.5 0.5 5.9 6.7 6.6

0.7 0.6 0.6 0.5 0.6 0.5 2.5 3.8 4.7

0.5 0.4 0.6 0.7 0.6 0.6 4.0 3.7 5.1

1.3 0.9 1.0 1.4 1.2 0.8 3.7 4.5 4.4

0.9 3.3 5.2 5.0

0.8 0.6 0.6 0.6 0.7 0.6 4.3 4.2 6.0

0.6 0.5 0.6 0.5 0.5 0.5 5.1 5.6 6.7

0.1 0.1 0.1 0.1 0.3 0.1

1.4 0.8

0.5 0.4 0.5 0.3 0.5 0.4 3.9 2.7 3.1

0.6 1.8 1.3 0.4 0.5 1.4

0.5 1.3 0.9 0.3 0.5 0.8 0.6 1.1 1.0

1.0 0.9 0.7 0.6 0.7 1.0 2.7 3.5 4.9

0.4 0.4 0.4 0.3 0.4 0.5 3.2 3.8 4.6

2.3 2.0 1.3 1.2 1.4 1.8 3.3 4.3 5.0
0.3 0.8 0.7 0.3 0.3 1.0 1.0 1.3 1.2

0.9 0.8 0.6 0.5 0.6 0.7 2.3 3.2 4.5

3.9 4.4

0.2 0.1 0.1 0.2 0.2 0.1

0.6 0.6 0.5 0.6 0.8 0.9 2.3 3.1 4.1

0.3 0.2 0.2 0.2 0.3 0.3 3.0 4.5 5.2

0.5 0.5 0.6 0.5 0.4 0.7 5.0 4.5 5.4

0.7 0.9 1.1 0.5 0.5 0.9 4.7 4.8 6.1

0.6 0.6 0.8 0.5 0.5 1.0 4.7 5.0 5.6

0.4 0.6 0.8 0.5 0.5 0.9 4.9 5.6 5.3

0.6 0.8 0.7 0.4 0.4 0.7 4.5 4.8 5.8

0.5 0.7 0.5 0.4 0.4 0.7 4.9 5.2 5.3

0.6 0.6 0.7 0.4 0.4 0.8 4.6 5.8 5.2

0.3 0.3 0.2 0.2 0.2 0.2 2.6 1.7 1.6

0.8 0.7 0.6 0.7 0.7 0.7 4.7 5.4 7.5

1.0 1.1 0.9 0.8 0.8 0.8 5.0 7.0 6.6

0.8 0.9 1.0 0.8 0.7 0.6 5.8 5.7 6.0

0.8 0.7 0.6 0.6 0.7 0.5 3.2 4.4 5.3

0.8 0.6 0.6 0.5 0.6 0.4 3.4 3.7 5.1

0.9 0.8 0.7 0.7 0.8 0.6 4.3 5.7 5.7

0.7 0.7 0.7 0.8 0.7 0.6 4.8 4.4 6.3

0.8 0.6 0.6 0.5 0.6 0.5

0.7 0.8 0.8 0.7 0.8 0.6 4.1 4.9 6.5

0.8 0.6 0.6 0.8 1.0 0.6 3.7 4.5 7.3

0.3 0.5 0.4 0.4 0.3 0.4 3.0 2.9 3.1

0.4 0.5 0.5 0.4 0.3 0.6 4.0 3.8 3.9

0.2 1.6 1.7 0.4 0.6 0.4 0.8 0.8

0.4 1.1 1.4 0.2 0.7 0.5 0.8 0.6

0.2 1.1 1.2 0.3 0.5 0.3 0.9 1.0

0.7 0.7 0.8 0.4 0.7 0.8 3.9 4.3 6.4

5.2 6.1 6.3

0.4 0.5 0.5 0.3 0.4 0.6 3.9 4.7 4.8

0.6

1.0 0.6 0.9 1.0

0.7 0.7 0.8 0.5 0.7 1.0 4.1 4.5 6.3

0.7 0.6 0.8 1.0

1.0 1.0 0.8 0.7 0.8 1.0 4.1 4.6 5.6

0.6 0.8 0.5 0.4 0.6 0.9

0.5 0.4

0.9

0.8 0.8 0.8 0.7 0.8 1.0 4.2 4.8 5.9

2.2 3.0 4.4

0.5 0.6 0.6 0.3 0.4 0.6 2.4

4.3 4.6 4.2
0.4 0.4 0.5 0.4 0.3 0.4 4.5 4.9 5.3

0.6 0.6 1.1 0.5 0.4 0.9 4.9 4.8 5.8

0.5 0.7 0.8 0.5 0.5 0.8

0.4 0.4 0.3 0.3 0.3 0.3 3.6 2.1 2.5

0.8 0.9 0.7 0.7 0.6 0.7 4.9 5.0 4.6

0.8 0.8 0.9 0.7 0.6 1.0 5.3 4.4 5.3

0.8 0.6 0.7 0.7 0.5 0.9 6.2 4.8 5.6

0.3 0.3 0.4 0.3 0.2 0.3 4.0 3.8 4.4

0.5 0.5 0.4 0.4 0.4 0.4 4.6 4.8 5.5

0.8 6.1 4.4 3.4

0.6 0.9 0.6 0.6 0.5 0.8 2.5 3.9 4.0

0.5 0.8 0.9 0.5 0.5 1.2 1.1 1.7 1.8

0.5 0.6 0.5 0.5 0.5 0.5 3.0 4.3 4.5

0.4 0.7 0.6 0.3 0.5 0.6 1.5 1.2 1.2

0.6 1.0 0.7 0.4 0.6 0.8 1.9 1.1 1.3

0.3 0.8 0.6 0.3 0.5 0.5 1.4 1.2 1.1

0.4 0.5 0.5 0.3 0.5 0.5 2.1 2.0 3.3

0.6 0.8 0.6 0.4 0.5 0.7 4.9 5.6 6.1

0.3 1.4 0.9 0.3 0.5 0.7 1.0 1.2 1.7

0.4 1.3 1.1 0.3 0.5 0.9 1.2 1.4 1.8

0.5 1.3 1.0 0.8 1.5 2.1

0.4 1.1 1.0 0.2 0.6 1.0 0.9

0.9 1.0 1.0 0.9 0.8 1.1 7.1 5.3 7.1

0.4 0.8 1.0 0.6 0.6 0.8

1.0 5.0 5.7 6.9

0.3 0.3 0.3 0.4 0.4

0.3 0.4 0.4 0.3 0.3 0.3 2.5 2.9 3.1

0.6 0.7 0.6 0.4 0.6 0.4 2.7 3.4 3.6

0.2 0.3 0.3 0.2 0.2 0.2 2.0 2.1 2.1

0.8 0.6 0.6 0.5 0.6 0.4 2.4 3.6 3.2
2010 2011 2011 2011 2011 2012 2012 2012 2012

4 1 2 3 4 1 2 3 4

4.2 5.1 5.2 5.8 3.6 3.4 4.0 4.0 3.3

3.9 4.2 5.1 5.3 3.4 3.1 4.4 3.5 3.0

3.8 4.5 5.0 4.9 3.5 3.1 3.9 4.0 2.7

3.9 4.3 4.8 4.8 3.1 2.7 4.0 3.2 3.3

3.3 4.0 5.1 5.6 2.5 2.9 3.8 2.8 2.9

1.3 1.0 1.9 2.3 1.5 1.1 1.8 2.4 1.2

3.3 4.1 3.7 4.3 2.9 3.1 3.7 3.0 2.8

0.9 0.9 1.6 1.7 1.0 0.9 2.1

1.0 1.7 0.9

1.8 1.6 1.7 2.7 2.4 1.4 2.1 2.3 1.5

1.7 1.2 2.2 2.8 1.6 1.4 2.2 3.1 1.8

2.2 1.4 3.3

0.5 0.5 1.1 1.1 0.7 0.6 1.3 1.5 0.4

1.2 1.0 1.5 2.2 1.3 0.9 1.5 1.7 0.8

1.1 1.0 1.4 2.1 1.6 1.0 1.7 1.7 1.1

1.9 1.4 3.1 4.9 2.0 1.5 3.0 3.8 1.1

1.4 1.2 3.0 5.1 1.8 1.6 3.4 3.6 2.1

1.3 1.1 1.4 2.1 1.6 1.0 1.7 2.0 1.0

1.6 2.1 1.5 2.4 2.7 1.3 1.9 2.2 1.6

1.9 2.2 2.3 3.3 3.0 2.0 3.1 2.9 1.4

1.5 1.1 2.6 4.6 1.4 1.2 2.6 3.2 1.6

1.3 1.2 1.3 1.6 1.1 1.1 1.3 1.2 0.9

1.5 1.1 1.5 1.6 1.1 1.3 1.7 1.5

0.7

3.8 3.7 4.1 5.5 2.9 3.3 3.3 3.9 3.0

3.0 3.7 3.6 2.4 2.4 3.0 3.4 2.7 2.1

3.3 4.1 4.0 3.4 2.3 3.0 3.3 2.7 2.5

2.7 3.8 4.5 3.4 2.2 3.0 3.1 2.8 2.5

2.9 2.7 4.5 4.9 2.5 3.2 3.7 2.9 2.6

3.0 4.1 4.7 4.2 2.2 3.1 3.3 3.6 2.3

3.6 4.4 5.2 5.2 2.7 2.9 4.0 3.4 2.7

3.3 3.5 4.7 5.1 2.4 2.7 3.6 2.8 2.7

0.9 1.0 1.6 1.5 0.9 0.7 1.5 1.5 0.8

2.2 3.1 3.4 4.1 2.3 2.6 2.6 2.7 2.7

3.3 3.5 4.2 2.8 2.8 3.0 2.8 3.5 3.1

3.0 4.5 4.5 4.4 2.6 3.7 3.7 4.1 3.3

2.2 2.9 3.8 2.6 2.0 2.3 3.6 2.4 2.3

2.0 3.6 3.5 3.0 2.1 2.6 3.4 2.9 2.5

5.1 4.8 5.2 6.7 3.1 3.7 4.3 4.7 2.9

4.7 4.6 4.8 5.6 2.5 3.2 3.5 4.5 2.7

Sulfates

SANDWICHed*
5.2 4.9 5.3 8.1 2.8 3.4 4.4 5.2 2.8

4.3 5.0 5.2 5.3 3.2 3.2 4.5 3.9 3.4

3.7 4.1 4.8 4.9 3.0 3.5 3.8 4.4 3.2

3.4 3.4 4.0 4.3 2.5 3.2 3.1 4.4 2.7

2.1 2.8 2.6 2.6 1.9 2.4 1.9 2.4 2.2

3.4 3.0 3.1 4.0 2.5 3.1 3.2 3.4 2.6

3.2 3.5 4.2 5.5 2.1 3.7 3.0 3.5 2.6

2.3 2.5 2.6 2.7 2.1 3.0 2.4 2.4 1.7

3.0 3.5 4.9 6.3 2.4 4.3 2.9 4.7 2.9

3.0 2.7 3.4 4.6 2.5 4.1 3.3 4.0 3.0

2.8 3.1 4.3 5.6 2.7 3.7 3.4 3.8 2.8

3.7 3.3 4.0 6.4 2.5 4.7 3.7 4.7 3.2

3.5 3.5 3.0 5.4 2.4 4.7 3.8 2.4 2.9

2.9 2.1 2.1 2.1 2.2 1.8 1.6 1.8

2.0 2.8 2.1 1.9 2.0 2.3 1.7 1.5 2.0

2.0

3.3 3.9 4.3 3.9 3.2 3.0 4.2

4.0 4.7 5.5 4.7 2.9 3.1 4.1 3.1 2.9

3.7 3.4 4.5 4.4 1.9 3.0 3.4 2.9 2.6

2.9 4.6 4.0 4.7 2.9 2.5 3.8 3.3 2.8

2.4 2.1 1.3 1.2 2.2 1.9 1.4 1.8

1.1 1.0 1.2 1.0 1.0 0.6 1.1 1.1 0.9

3.7 3.8 4.3 4.6 3.2 4.0 3.0 3.9 2.1

3.1 3.7 3.4 4.7 2.7 2.4 2.7 3.7 3.1

3.4 3.9 2.9 4.3 2.8 2.8 3.0 4.2 2.8

3.5 3.7 4.0 4.7 2.5 3.2 2.7 3.2 1.8

4.0 5.3 4.9 6.0 1.7 2.8 2.9 0.3

5.5 5.2 5.6 9.0 2.5 4.0 4.6 6.0 3.5

5.0 5.7 5.2 8.8 3.1 3.5 4.3 5.9 3.3

4.0 3.5 3.9 5.2 2.3 3.7 3.0 3.6 2.6

4.8 4.1 4.4 6.8 2.6 3.2 3.8 3.8 3.0

3.9 5.2 3.9 5.6 2.5 3.7 3.3 3.6 3.2

3.6 3.7 4.0 5.6

4.2 4.0 4.7 7.9 2.9 3.5 4.2 3.8 3.6

4.5 5.2 5.8 7.3 3.0 3.3 4.2 5.2 3.2

1.2 0.9 0.8 0.7 0.8 1.0 0.9 0.8

0.6

2.4 2.2 4.1 3.4 1.9 2.6 2.5 2.3 2.0

1.0 0.6 1.6 1.9 1.1 0.9 1.7 2.3 0.9

0.6 0.5 1.1 1.2 0.8 0.5 1.3 1.3 0.5

2.6 3.4 3.9 4.7 2.7 3.1 3.4 3.1 2.8

2.8 2.6 3.0 4.3 2.4 2.7 2.4 2.8 2.4

2.7 3.6 4.3 5.1 3.3 3.3 3.4 2.2 3.1
0.9 0.7 1.5 1.6 1.0 0.8 1.6 1.6 0.8

2.0 2.6 2.3 3.4 2.1 2.2 2.3 2.5 2.4

2.1 1.9 2.3 1.4 2.0 2.0 2.1 1.7

2.4 2.6 3.3 3.8 2.3 2.9 2.5 3.2 2.6

2.8 3.2 2.9 4.7 2.3 2.7 2.2 3.2 2.4

2.8 3.1 5.0 5.9 2.6 2.4 3.4 3.0 2.4

3.2 3.6 4.8 4.5 2.3 2.9 3.1 3.0 2.4

3.4 3.9 4.6 4.4 2.6 3.0 3.2 2.9 2.5

4.0 2.7 4.7 4.0 3.0 3.0 2.7 3.4 2.5

3.6 3.6 4.7 4.9 2.3 3.0 3.4 3.3 2.3

3.4 3.8 4.7 4.0 2.2 3.3 3.2 3.0 2.4

3.3 3.5 4.3 5.6 2.6 2.8 3.0 3.5 2.6

1.8 2.0 2.1 1.8 1.4 1.8 1.7 1.1 1.6

4.3 4.9 5.1 8.1 2.9 3.6 4.1 5.1 3.4

5.0 5.4 6.8 8.5 5.0 5.2 3.8 5.5 4.0

5.3 4.9 2.2 6.2 3.5 3.3 4.1 5.0 2.7

2.6 3.8 4.0 5.6 2.9 3.9 3.0 4.0 2.7

3.2 3.5 4.6 7.0 2.0 4.4 3.6 4.2 2.8

3.5 3.5 3.7 6.5 3.0 3.7 3.2 3.8 2.4

4.1 4.2 5.0 7.4 2.6 3.6 4.4 4.8 3.4

4.3 4.5 6.3 3.0 3.4 3.6 3.7 3.2

3.4 4.1 5.2 5.1 3.1 4.0 4.2 4.3 3.2

4.2 4.3 6.8 7.9 4.2 6.4 4.7 5.0 3.6

2.8 3.5 4.3 2.8 2.0 2.4 3.2 2.4 2.1

2.5 4.9 3.8 3.0 2.9 2.6 3.9 3.2 2.6

0.5 0.6 1.4 1.1 0.7 0.5 0.9 0.9

0.5 0.6 1.6 0.9 0.6 0.6 1.1 0.9

0.6 0.5 1.4 1.3 0.7 0.5 1.1 1.1

3.3 3.4 4.5 5.9 2.4 3.3 3.9 3.8 3.2

4.3

3.2 2.4 4.9 5.9 2.3 3.9 3.4 3.5 3.2

2.8

4.3 3.7 4.0 3.1

2.9 3.7 4.5 5.9 2.0 3.8 4.2 3.9 3.1

3.9 3.4 3.1 2.8

3.2 3.6 6.9 5.8 2.9 3.5 4.1 3.5 3.2

3.1 4.5 5.1 2.5 3.0 2.8 3.3 2.6

4.7 3.3

2.6

3.5 3.4 4.8 5.9 2.3 3.9 4.3 4.5 3.1

2.1 3.0 2.9 3.0 2.3 2.8 2.3 2.8 2.6

4.0
3.5 3.2 4.5 4.4 2.3 3.2 3.3 2.4 2.5

3.3 3.5 4.7 5.4 2.3 3.3 2.7 3.4 2.7

3.6 4.5 5.0 2.4 2.8 3.5 3.0 2.3

2.6 2.3 2.4 3.0 1.9 1.9 1.9 1.8 1.7

3.7 5.3 4.3 5.7 3.6 2.8 4.0 4.6 2.4

3.7 5.5 4.7 5.3 3.1 3.1 4.1 3.6 2.8

2.9 3.5 5.6 5.2 2.5 3.6 3.9 3.0 2.9

3.4 4.5 4.1 4.5 3.1 3.0 3.3 3.6 2.6

3.9 4.8 4.4 6.0 3.0 2.6 4.1 4.9 2.9

3.5 4.3 4.7 6.4

3.2 4.7 4.5 4.0 2.9 2.9 4.1 3.2 2.4

1.2 1.1 2.0 2.2 1.6 1.3 1.8 2.4 1.5

3.3 3.2 4.0 4.0 2.6 3.0 4.1 3.2 2.5

0.9 1.1 1.3 1.3 1.3 1.1 1.2 1.4 0.9

1.1 1.6 1.3 1.4 1.3 0.9 1.2 1.4 0.9

0.8 1.1 1.4 1.7 1.0 1.0 1.3 1.4 0.8

1.7 2.1 1.6 1.7 2.1 2.2 1.8 2.4 1.8

3.7 3.9 4.5 4.8 3.0 2.9 3.0 3.4 2.9

0.8 0.9 1.1 1.5 1.3 1.0 1.3 1.7 0.8

1.0 1.0 1.3 2.0 1.1 0.8 1.3 2.0 0.6

0.8 0.8 1.5 2.1 1.0 0.8

1.0 0.8 0.8 1.2 1.1 0.8 1.1 1.0 0.9

4.2 4.6 5.3 7.0 2.8 3.6 4.6 3.6 2.8

6.7 3.0 4.0 4.4 5.3 3.1

5.2 4.5 5.8 9.8

2.4 2.6 2.9 2.3 1.6

2.2 2.4 3.0 3.0 2.3 2.8 2.6 2.6 2.1

2.6 2.6 3.1 4.0 2.7 3.4 2.7 3.2 1.8

2.2 2.3 2.8 2.0 2.6 2.8 2.2 1.7 2.0

3.1 2.6 3.7 4.2 2.4 3.3 2.1 3.1 1.8
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

0.7 0.0 0.0 0.1 0.4 0.0 0.0 0.0 0.1

0.7 0.0 0.0 0.1 0.4 0.0 0.0 0.0 0.1

1.5 0.0 0.0 0.6 0.7 0.0 0.0 0.2 0.3

0.3 0.0 0.0 0.1 0.0 0.0 0.0 0.0 0.0

1.1 0.0 0.0 0.2 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.3 0.0 0.0 0.0 0.1 0.0

1.3 0.0 0.0 0.5 0.8 0.0 0.0 0.3 0.4

0.0 0.0 0.0 1.2 0.9 0.0 0.0 2.8 0.1

5.6 0.0 0.0 6.1 4.0 0.0 0.0 10.9 7.3

0.4 0.0 0.0 0.4 0.1 0.0 0.0 0.6 0.4

1.0 1.4 0.4 1.0 2.0 0.3

0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1

2.8 0.0 0.0 1.9 2.6 0.0 0.0 3.2 1.2

2.4 0.0 0.0 2.4 1.9 0.0 0.0 6.2 1.0

0.6 0.2 0.1 0.4 0.1 0.0 0.0 1.6 0.5

1.1 0.6 0.0 0.1 0.0 0.0 0.0 1.6 0.0

1.3 0.0 0.0 0.7 1.3 0.0 0.0 1.9 1.7

4.1 0.0 0.0 4.7 9.7 0.0 0.0 13.5 4.2

3.2 0.0 0.0 6.0 5.1 0.0 0.0 14.5 11.4

0.6 0.1 0.0 0.4 0.2 0.3 0.5 0.2 0.3

2.8 0.5 0.0 0.5 1.4 0.0 0.0 1.6 2.3

3.4 0.4 0.0 1.4 1.0 0.0 0.0 1.9 3.8

1.6 0.2 0.0 1.4 1.7 0.0 0.0 0.5 0.6

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.6 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.2

0.7 0.0 0.0 0.3 0.0 0.0 0.0 0.2 0.1

0.8 0.0 0.0 0.3 0.0 0.0 0.0 0.0 0.0

0.6 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

2.8 0.6 0.0 1.2 1.7 0.0 0.0 1.8 0.9

0.8 0.0 0.0 0.6 1.3 0.1 0.0 0.3 1.1

3.3 0.1 0.0 1.5 2.0 0.2 0.5 0.4 1.9

6.2 0.3 0.0 2.5 3.7 0.1 0.0 0.6 2.4

3.6 0.0 0.0 1.2 4.1 0.0 0.0 1.6 1.5

6.1 0.0 0.0 0.1 4.3 0.0 0.0 0.4 1.4

2.2 0.0 0.0 1.1 1.2 0.0 0.0 0.3 0.3

1.8 0.0 0.0 0.5 0.5 0.0 0.0 0.1 0.0

Nitrates

SANDWICHed*
3.3 0.0 0.0 1.9 2.1 0.0 0.0 0.9 0.7

4.6 0.0

0.0 0.0 0.0 0.0 0.3 0.0 0.0 0.1 0.0

2.3 0.2 0.0 1.9 2.3 0.1 0.0 0.6 1.3

1.4 0.2 0.0 1.0 1.4 0.0 0.0 0.2 0.7

0.4 0.0 0.0 0.8 1.4 0.0 0.0 0.6 0.7

4.1 0.0 0.0 4.4 4.5 0.6 0.0 1.3 2.4

4.5 0.0 0.0 3.7 4.6 0.7 0.0 1.4 3.2

0.1 0.0 0.0 1.9 1.9 0.0 0.0 1.2 2.1

5.6 0.0 0.0 3.1 3.7 0.3 0.0 1.2 3.0

0.9 0.0 0.0 2.6 3.0 0.4 0.0 1.0 2.6

4.5 0.0 0.0 2.5 4.9 0.6 0.0 1.4 2.4

4.0 0.0 0.0 4.1 4.0 0.8 0.0 1.4 3.1

3.2 0.0 0.0 3.1 4.3 0.4 0.0 1.1 3.3

5.0 0.3 0.0 2.0 2.7

5.8 0.0 0.0 2.1 5.6 0.2 0.0 1.8 3.1

8.7 0.0 0.0 1.6

0.0 0.0 0.1 0.3 0.0 0.0 0.1 0.0

0.9 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.9 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1

0.9 0.0 0.0 0.4 0.1 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.0

1.6 0.0 0.0 1.0 2.5 0.0 0.0 2.4 1.0

9.4 0.0 0.0 4.3 6.0 1.4 0.0 0.4 3.2

5.7 0.2 0.0 2.9 4.9 0.8 0.0 1.5 1.7

6.3 0.0 0.0 4.2 6.6 0.1 0.0 1.5 2.7

6.9 0.0 0.0 4.2 5.7 0.7 0.0 1.9 2.8

4.2 0.0 0.0 2.4 3.8 0.0 0.0 0.0 1.0

4.4 0.0 0.0 1.8 1.8 0.0 0.0 0.8 0.6

5.6 0.0 0.0 3.1 4.1 0.0 0.0 1.5 1.1

5.7 0.0 0.0 6.1 4.0 0.5 0.0 1.7 3.6

7.2 0.0 0.0 4.0 3.3 0.0 0.0 1.3 1.9

6.5 0.0 0.0 4.8 5.8 0.7 0.0 2.7 3.1

7.4 0.0 0.0 4.4 5.0 0.7 0.0

7.0 0.0 0.0 3.4 4.2 0.3 0.0 1.7 2.2

4.3 0.0 0.0 2.7 2.7 0.0 0.0 1.0 0.9

0.4 0.0 0.0 0.2 0.4

1.1

8.9 0.0 0.0 2.7 5.1 0.0 0.0 1.9 4.5

0.1 0.3 0.0 0.0 0.1 0.0

1.3 0.0 0.0 0.5 1.0 0.0 0.0 0.8 0.3

0.9 0.0 0.0 0.8 1.6 0.4 0.0 0.5 1.4

0.7 0.0 0.0 0.6 0.2 0.0 0.0 0.3 0.9

2.0 0.0 0.0 0.8 1.7 0.3 0.0 0.8 1.4
0.5 0.0 0.0 0.1 0.3 0.0 0.0 0.7 0.0

1.6 0.0 0.0 1.1 2.7 0.0 0.0 0.6 1.1

1.9 0.1

0.4 0.0 0.0 0.0 0.1

2.4 0.0 0.0 1.0 2.8 0.0 0.0 1.1 1.4

0.7 0.0 0.0 0.8 1.0 0.0 0.0 0.6 0.6

0.4 0.0 0.0 0.4 0.1 0.0 0.0 0.1 0.1

0.9 0.0 0.0 1.3 0.5 0.0 0.0 0.0 0.3

0.9 0.0 0.0 0.9 0.4 0.0 0.0 0.0 0.3

0.9 0.0 0.0 1.4 1.3 0.0 0.0 0.0 0.2

0.7 0.0 0.0 0.9 0.8 0.0 0.0 0.0 0.1

0.8 0.0 0.0 0.6 0.4 0.0 0.0 0.0 0.1

0.6 0.0 0.0 0.4 0.6 0.0 0.0 0.0 0.2

4.8 0.0 0.0 1.5 4.1 0.2 0.0 0.9 1.7

5.6 0.0 0.0 1.9 3.6 0.3 0.0 1.0 1.3

2.3 0.0 0.0 1.7 2.1 0.0 0.0 1.1 1.8

2.2 0.0 0.0 1.4 1.4 0.0 0.0 0.2 0.3

5.0 0.0 0.0 1.2 3.9 0.2 0.0 1.1 2.5

5.4 0.0 0.0 3.6 4.7 0.3 0.0 1.4 4.3

5.0 0.0 0.0 2.9 3.1 0.3 0.0 1.1 2.2

7.7 0.0 0.0 2.8 2.1 1.0 0.0 1.4 1.5

4.6 0.4 0.0 1.5 2.3

7.0 0.0 0.0 3.2 3.5 0.3 0.0 1.1 2.3

4.6 0.3 0.0 2.4 4.7 0.0 0.0 1.7 4.4

1.9 0.0 0.0 1.2 2.6 0.0 0.0 1.5 0.5

2.3 0.0 0.0 1.4 3.0 0.0 0.0 1.0 1.0

0.2 0.0 0.0 0.1 0.7 0.0 0.0 0.5 0.2

0.0 0.0 0.0 0.0 0.5 0.0 0.0 0.1 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

3.3 0.5 0.0 2.5 2.5 0.6 0.0 1.1 3.8

2.6 0.0 0.0 1.4

1.6 0.0 0.0 0.9 1.2 0.5 0.0 0.5 1.0

3.2

4.1 0.6 0.0 2.4 3.0 0.7 0.0 1.0 3.6

0.0

3.1 0.4 0.0 0.8 2.3 0.2 0.0 0.7 2.0

0.7 0.0 0.0 0.4 1.2

3.3 0.4 0.0 2.2 2.4 0.9 0.0 1.2 3.6

0.8 0.0 0.0

0.0 0.4 1.2 0.0 0.0 0.1 0.6

0.2 0.0 0.0 0.1
0.7 0.0 0.0 0.4 0.2 0.0 0.0 0.0 0.2

0.1 0.0 0.0 1.5 0.1 0.0 0.0 0.0 0.4

0.6 0.0 0.0 0.0 0.0

7.4 0.0 0.0 2.9 4.3 1.4 0.0 1.6 0.9

3.5 0.0 0.0 0.8 1.0 0.0 0.0 0.8 0.3

0.6 0.0 0.0 0.2 0.0 0.0 0.0 0.0 0.1

0.2 0.0 0.0 0.3 0.2 0.0 0.0 0.0 0.3

0.4 0.0 0.0 0.3 0.7 0.0 0.0 0.0 0.0

3.7 0.0 0.0 0.9 1.2 0.0 0.0 0.5 0.2

0.1 0.0 0.0 0.4 0.2 0.0 0.0

1.3 0.0 0.0 0.5 0.4 0.0 0.0 0.6 0.4

0.5 0.0 0.0 0.0 0.0 0.0 0.0 0.3 0.1

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

5.6 0.0 0.0 2.2 5.0 0.0 0.0 4.2 3.5

8.9 0.0 0.0 3.6 5.8 0.0 0.0 4.2 2.8

7.5 0.0 0.0 2.6 7.5 0.0 0.0 3.0 3.6

1.9 0.0 0.0 0.9 1.7 0.0 0.0 0.6 1.1

0.9 0.0 0.0 0.6 0.8 0.0 0.0 0.1 0.4

0.2 0.0 0.0 0.1 0.6 0.0 0.0 0.5 0.1

0.0 0.0 0.0 0.0 0.6 0.0 0.0 0.3 0.1

0.0 0.0 0.0 0.1 0.3 0.0 0.0 0.3 0.4

0.6 2.1 1.7 0.0 0.0 3.1 1.4

2.6 0.0 0.0 0.9 0.9 0.0 0.0 0.3 0.4

0.0 0.4 0.6

4.1 0.0 0.0 1.4 1.7 0.1 0.0

2.4 3.2

4.5 0.0 0.0 2.6 4.1 0.4 0.0 1.3 2.8

3.7 0.2 0.0 3.2 4.1 1.4 0.0 2.3 3.4

0.6 0.0 0.0 3.0 3.2 0.6 0.0 2.0 3.2

4.4 0.0 0.0 4.4 3.7 1.8 0.0 2.1 3.6
2012 2012 2012 2010 2010 2010 2010 2011 2011

2 3 4 1 2 3 4 1 2

0.0 0.0 0.2 0.7 1.5 1.7 1.2 1.4 1.1

0.0 0.0 0.2 1.0 2.0 2.5 1.9 1.5 1.9

0.0 0.0 0.2 0.4 1.1 1.1 0.4 0.3 0.9

0.0 0.0 0.0 0.5 1.6 1.7 0.6 0.3 0.7

0.0 0.0 0.0 0.3 0.7 1.4 0.5 0.3 0.7

0.0 0.0 0.0 0.6 1.4 0.9 1.0 1.6 2.2

0.0 0.0 0.4 0.5 1.0 1.6 0.7 0.4 0.9

0.0 0.5 0.5 1.2 0.4 0.3 0.5

0.0 0.0 0.9

0.0 0.0 1.9 0.5 0.6 1.3 0.5 0.4 0.6

0.0 0.0 0.3 1.6 2.2 2.2 2.1 2.6 2.4

1.2 0.9 0.8 0.9 1.0 1.2

0.0 0.0 0.6 0.7 1.0 1.4 0.3 0.5 0.5

0.0 0.0 0.4 0.3 0.9 0.9 0.4 0.4 0.4

0.0 0.0 0.8 0.4 0.8 0.9 0.6 0.4 0.5

0.2 0.0 0.6 0.6 0.5 0.5 0.5 0.6 0.7

0.2 0.0 0.0 0.7 0.7 0.7 0.6 0.5 0.5

0.0 0.1 0.1 0.4 0.4 0.4 0.5 0.5 0.3

0.0 0.0 4.4 0.6 0.8 1.4 1.1 0.4 0.5

0.0 0.0 3.0 0.5 0.8 1.8 0.7 0.5 0.8

0.0 0.1 0.6 0.5 0.6 0.6 0.4 0.4 0.7

0.0 0.0 0.7 1.2 1.2 1.7 1.3 1.2 2.3

0.3 0.0 1.0 1.1 1.3 1.0 1.0 1.6

0.8

0.0 0.0 1.1 0.5 0.8 0.6 0.3 0.2 0.4

0.0 0.0 0.0 0.4 1.6 1.9 0.5 0.5 0.8

0.0 0.0 0.0 0.3 1.3 1.5 0.3 0.4 0.6

0.0 0.0 0.0 0.3 1.0 1.6 0.4 0.4 0.7

0.0 0.0 0.0 0.7 2.0 2.2 0.4 0.8 1.8

0.0 0.0 0.0 0.3 1.1 0.7 0.4 0.2 0.5

0.0 0.0 0.1 0.4 1.6 1.0 0.8 0.4 0.7

0.0 0.0 0.0 0.7 1.3 1.1 0.4 0.3 0.7

0.0 0.0 1.2 1.2 1.2 2.3 2.0 1.1 1.8

0.0 0.0 1.1 0.3 0.6 0.4 0.5 0.4 0.5

0.0 0.0 1.1 0.2 0.7 0.6 0.2 0.2 0.5

0.0 0.0 1.3 0.5 0.7 0.6 0.5 0.4 0.4

0.0 0.0 2.2 0.5 1.1 1.4 1.0 0.7 1.3

0.0 0.0 1.8 0.7 1.0 0.8 1.1 0.4 0.8

0.0 0.0 0.3 0.4 0.5 0.7 0.5 0.4 0.5

0.0 0.0 0.1 0.3 0.4 0.3 0.3 0.2 0.3

Crustal

SANDWICHed*
0.0 0.0 1.0 0.3 0.6 0.7 0.6 0.4 0.5

0.4 0.6

0.0 0.0 0.0 0.5 1.4 2.3 1.0 0.4 0.8

0.0 0.0 2.0 0.4 0.7 0.5 0.4 0.3 0.5

0.0 0.0 0.8 0.4 0.8 0.8 0.5 0.3 0.4

0.0 0.0 0.6 0.2 0.4 0.3 0.3 0.3 0.3

0.1 0.0 3.5 0.3 0.9 0.4 0.8 0.4 0.4

0.0 0.0 3.4 0.4 0.7 0.3 0.3 0.2 0.4

0.0 0.0 1.0 0.1 0.5 0.1 0.2 0.1 0.2

0.0 0.0 3.2 0.4 0.7 0.4 0.3 0.2 0.4

0.1 0.0 2.1 0.3 0.6 0.4 0.4 0.2 0.4

0.1 0.0 2.9 0.4 0.7 0.5 0.4 0.4 0.7

0.0 0.0 2.1 0.7 1.6 1.1 1.1 0.8 1.1

0.1 0.0 3.1 0.9 1.4 1.2 2.2 0.9 0.9

0.0 0.0 2.7 0.2 0.3

0.1 0.0 3.3 0.4 0.8 0.5 1.0 0.5 0.7

0.4 0.7 0.5 0.7

0.0 0.8 2.3 0.6 0.3 0.7

0.0 0.0 0.2 0.4 1.2 2.2 1.8 1.1 1.4

0.0 0.0 0.0 0.3 1.0 1.1 0.6 0.3 0.6

0.0 0.0 0.1 0.5 1.1 0.5 0.4 0.3 0.5

0.0 0.0 0.0 0.4 0.5

0.0 0.0 0.6 0.4 0.8 2.1 0.9 0.5 0.6

0.1 0.0 4.0 0.5 1.1 0.7 0.9 0.4 1.2

0.1 0.0 3.6 0.4 0.8 0.6 0.5 0.3 0.6

0.1 0.0 3.6 0.2 0.6 0.6 0.5 0.2 0.5

0.0 0.0 2.8 0.4 0.6 0.3 1.2 0.4 0.6

0.0 0.0 1.4 2.5 2.8 4.0 2.9 3.9

0.0 0.0 1.2 0.4 0.9 1.0 1.2 0.6 1.0

0.0 0.0 1.9 0.3 0.6 0.5 0.5 0.3 0.6

0.0 0.0 3.5 0.3 0.5 0.3 0.5 0.3 0.4

0.0 0.0 3.1 0.2 0.5 0.3 0.4 0.3 0.5

0.1 0.0 3.6 0.7 1.4 1.0 0.9 1.0 0.9

0.5 1.1 0.6 0.6 0.5 1.2

0.1 0.0 3.2 0.4 0.7 0.5 0.5 0.3 0.6

0.0 0.0 1.4 0.4 0.7 0.6 0.6 0.4 0.8

0.0 0.0 0.4 0.2 0.2

0.7 0.4

0.0 0.0 2.9 0.9 2.0 1.1 0.9 0.4 0.8

0.0 0.0 0.1 1.0 0.9 1.0

0.0 0.0 0.3 1.0 0.9 0.9 0.6 1.1 0.6

0.1 0.0 1.9 0.3 0.4 0.5 0.4 0.3 0.4

0.0 0.0 1.2 0.2 0.5 0.2 0.2 0.2 0.2

0.0 0.0 1.9 0.6 1.1 1.1 0.6 0.4 0.7
0.0 0.0 0.2 0.5 1.3 0.5 0.6 0.9 1.9

0.0 0.0 1.0 0.4 0.8 0.6 0.5 0.5 0.6

0.6 0.9

0.0 0.0 0.1 0.1 0.3

0.0 0.0 1.9 0.3 0.6 0.4 0.3 0.3 0.3

0.0 0.0 0.8 0.2 0.5 0.2 0.2 0.1 0.2

0.0 0.0 0.1 0.2 1.0 0.6 0.2 0.2 0.5

0.0 0.0 0.1 0.3 0.9 0.6 0.3 0.2 0.5

0.0 0.0 0.2 0.3 0.7 0.7 0.4 0.3 0.5

0.0 0.0 0.2 0.2 0.8 0.8 0.3 0.2 0.4

0.0 0.0 0.0 0.4 0.7 0.8 0.3 0.3 0.5

0.0 0.0 0.0 0.2 0.8 0.7 0.3 0.2 0.5

0.0 0.0 0.0 0.3 0.9 0.6 0.3 0.3 0.5

0.0 0.0 1.8 0.4 1.9 1.8 2.7 0.3 0.7

0.0 0.0 1.8 0.3 0.6 0.5 0.4 0.3 0.5

0.0 0.0 1.0 0.4 0.5 0.6 0.5 0.3 0.4

0.0 0.0 0.1 0.7 0.9 0.7 0.9 0.5 0.2

0.0 0.0 2.0 0.4 1.3 0.5 0.5 0.3 0.5

0.1 0.0 2.1 0.3 0.8 0.6 0.7 0.3 0.5

0.0 0.0 1.3 1.2 1.6 0.8 1.4 0.8 0.9

0.0 0.0 3.2 0.4 0.6 0.4 0.6 0.2 0.6

0.0 0.0 2.4 0.2 0.4

0.0 0.0 2.3 0.6 2.2 1.5 1.3 0.6 0.9

0.0 0.0 1.7 0.3 0.7 0.5 0.3 0.2 0.5

0.0 0.0 1.4 0.4 0.7 1.4 0.6 0.6 1.0

0.0 0.0 1.1 0.6 1.0 1.4 0.7 0.5 0.8

0.0 0.0 0.6 0.6 0.4 0.3 0.6 0.4

0.0 0.0 0.7 0.8 1.4 0.8 0.7 0.7

0.0 0.0 0.3 0.4 0.3 0.2 0.2 0.2

0.5 0.0 2.4 0.2 0.5 0.3 0.3 0.2 0.3

0.7 1.4 1.1 1.3

0.0 0.0 1.8 0.2 0.4 0.2 0.2 0.1 0.3

2.3

0.0 0.0 2.8

0.0 0.0 3.0 0.2 0.5 0.3 0.2 0.2 0.4

0.2 0.0 1.6

0.1 0.0 1.9 0.3 0.9 0.6 0.4 0.3 0.5

0.0 0.0 1.2 0.3 0.4

0.0 0.8

0.3

0.0 0.0 2.5 0.5 0.7 0.7 0.4 0.4 0.6

0.3 0.9 0.4

0.0 0.0 1.0 0.1 0.2 0.3 0.3

0.3 0.6 1.1 0.4
0.0 0.0 0.0 0.2 0.6 0.9 0.2 0.1 0.5

0.0 0.0 0.0 0.2 1.1 0.8 0.3 0.4 0.7

0.0 0.0 0.0 0.3 0.7

0.0 0.0 2.1 0.2 0.8 0.6 1.1 0.2 0.5

0.0 0.0 0.5 0.3 0.7 1.1 0.5 0.3 0.6

0.0 0.0 0.0 0.4 1.2 0.9 0.4 0.5 0.6

0.0 0.0 0.2 0.3 0.6 0.6 0.4 0.2 0.8

0.0 0.0 0.0 0.4 1.3 1.9 0.8 0.4 1.0

0.0 0.0 0.8 0.3 0.6 1.0 0.3 0.2 0.6

0.3 0.8 0.6 0.2 0.2 0.4

0.0 0.0 0.3 0.5 1.2 2.3 0.7 0.6 1.1

0.0 0.0 0.0 1.5 3.4 1.6 3.8 3.3 6.3

0.0 0.0 0.1 0.3 0.7 2.0 0.4 0.3 1.0

0.0 0.0 1.3 0.5 1.0 1.0 0.5 0.6 1.0

0.0 0.0 1.1 1.8 1.5 1.2 0.6 0.8 1.1

0.0 0.0 0.4 0.6 1.0 2.1 0.8 0.7 1.4

0.0 0.0 0.6 0.3 0.6 0.3 0.2 0.3 0.8

0.0 0.0 0.1 0.3 0.7 0.6 0.3 0.2 0.4

0.0 0.0 0.1 0.3 0.4 0.4 0.2 0.4 0.2

0.0 0.0 0.0 0.6 0.3 0.2 0.3 0.3 0.2

0.4 0.3 0.3 0.3 0.3 0.2

0.0 0.0 1.1 0.7 0.5 0.5 0.3

0.0 0.0 0.2 0.6 0.7 0.7 0.5 0.3 0.6

0.0 0.0 0.7

1.2 1.3 1.1 1.1 0.7 0.8

0.0 0.0 1.8

0.1 0.0 3.0 0.1 0.4 0.6 0.3 0.2 0.2

0.1 0.0 2.1 0.3 0.7 0.5 0.5 0.2 0.4

0.0 0.0 2.2 0.3 0.6 0.2 0.3 0.2 0.3

0.0 0.0 2.1 0.4 0.9 0.7 0.8 0.5 0.6
2011 2011 2012 2012 2012 2012 2010 2010 2010

3 4 1 2 3 4 1 2 3

0.9 0.9 0.9 0.9 1.3 0.8 3.5 8.2 8.3

1.0 1.1 1.8 1.0 1.8 1.1 3.7 6.2 6.3

0.5 0.4 0.4 0.7 0.8 0.4 3.5 5.3 6.1

0.7 0.5 0.7 0.6 1.0 0.5 3.9 5.8 4.5

0.5 0.3 0.4 0.6 0.9 0.4 6.5 8.5 5.2

1.7 1.1 1.8 2.2 1.1 1.8 2.7 1.5 1.6

1.0 0.6 0.7 1.0 2.1 0.7 4.3 6.4 7.3

1.3 0.5 0.4 1.4 5.7 1.6 3.0

0.7 1.4 0.7

1.3 0.8 0.6 0.9 1.4 1.0 9.1 3.1 5.3

2.7 2.9 3.0 3.3 3.4 6.9 6.8 7.7 9.6

4.6 4.6 5.0

0.9 0.5 0.5 1.1 0.8 0.3 10.4 2.9 1.4

0.7 0.5 0.4 0.7 0.6 0.4 6.2 2.3 3.7

0.6 0.7 0.5 0.8 0.8 0.6 4.6 1.1 4.0

0.5 1.0 0.6 0.6 0.5 0.5 7.3 5.7 5.2

0.6 0.7 0.8 0.9 0.6 0.5 6.6 5.4 4.7

0.4 0.7 0.5 0.5 0.4 0.5 5.4 5.1 5.4

1.2 0.9 0.5 0.9 1.0 0.3 4.8 2.2 6.7

2.0 0.9 1.0 1.2 1.9 0.8 5.7 4.1 5.7

0.7 1.2 1.7 1.7 0.7 0.4 4.4 5.9 6.3

1.8 1.6 1.3 2.2 1.0 2.4 3.5 3.0 3.4

1.6 0.9 0.9 1.3 1.2 3.1 3.0 3.4

1.1

0.4 0.5 0.4 0.5 0.6 0.4 5.2 3.6 5.0

1.8 0.3 0.4 1.6 3.8 0.3 3.0 2.2 1.2

1.1 0.3 0.5 1.0 2.3 0.5 3.4 3.2 2.1

0.6 0.3 0.4 0.4 1.4 0.3 4.5 4.9 2.6

0.9 0.4 0.8 1.5 1.5 0.9 6.0 9.7 8.2

0.5 0.3 0.5 0.5 0.8 0.4 3.6 7.4 7.4

0.6 0.4 0.5 0.7 0.7 0.5 4.2 7.5 8.2

0.5 0.3 0.3 0.6 0.9 0.4 5.6 9.7 5.8

2.1 2.1 0.7 2.7 1.6 1.3 1.8 2.2 3.1

0.4 0.5 0.4 0.5 0.5 0.4 3.1 3.8 4.2

0.3 0.2 0.2 0.5 0.4 0.2 2.1 3.9 5.8

0.3 0.4 0.4 0.5 0.5 0.5 1.8 3.1 4.7

1.9 0.7 0.7 1.4 1.4 1.5 2.5 2.5 3.4

1.0 0.8 0.7 1.2 1.5 1.0 3.0 3.6 3.6

0.4 0.4 0.3 0.7 0.7 0.5 2.8 3.4 4.4

0.2 0.3 0.2 0.4 0.6 0.2 1.3 3.6 6.0

Crustal

SANDWICHed*
0.7 0.7 0.6 0.6 0.7 0.4 3.0 2.6 4.3

2.2 2.2

1.0 0.6 0.6 0.9 2.6 0.9 3.0 4.2 3.5

0.4 0.4 0.4 0.5 0.5 0.3 3.1 4.4 5.9

0.4 0.5 0.3 0.5 0.4 0.4 1.6 3.7 4.8

0.2 0.2 0.2 0.3 0.2 0.2 2.9 4.6 4.4

0.7 0.4 0.4 0.6 0.7 0.4 2.7 3.0 4.1

0.3 0.2 0.2 0.5 0.3 0.3 1.6 3.6 3.6

0.2 0.2 0.2 0.4 0.3 0.1 1.5 3.2 3.6

0.8 0.4 0.4 0.7 0.6 0.4 1.2 2.9 4.3

0.3 0.3 0.3 0.6 0.4 0.3 1.8 4.0 4.4

0.6 0.5 0.4 0.8 0.6 0.5 2.4 2.4 4.5

1.0 0.8 1.3 2.0 1.0 0.8 2.1 2.6 3.4

1.1 1.1 1.6 2.5 2.4 1.6 1.9 3.7 5.7

0.5 0.5 0.3 0.6 0.6 0.4

0.6 0.5 0.3 0.7 0.8 0.5 3.0 3.4 4.3

2.4 3.2 4.3

0.8 0.3 0.3 0.5 6.7 5.4

0.8 0.5 0.3 0.6 1.4 0.4 4.8 5.6 5.6

0.7 0.3 0.4 0.6 1.1 0.3 5.7 7.3 6.3

0.5 0.4 0.4 0.6 0.6 0.4 2.6 3.8 5.9

0.5 0.4 0.9 0.7 0.2 0.2

1.6 0.5 0.4 0.8 1.6 0.8 2.8 0.9 1.5

1.8 0.8 0.5 1.1 1.0 0.6 3.4 4.5 5.7

0.6 0.5 0.2 0.7 0.9 0.4 4.0 4.6 5.5

0.4 0.4 0.3 0.7 0.9 0.4 1.6 2.4 5.0

0.7 0.4 0.3 0.6 0.5 0.4 2.8 3.8 5.4

2.0 5.0 2.2 3.7 0.0 4.1 5.8 5.5

0.8 1.1 1.1 1.2 1.2 0.7 4.1 4.1 5.7

0.5 0.3 0.3 0.7 0.8 0.3 3.7 3.4 5.0

0.4 0.4 0.4 0.6 0.4 0.3 3.6 3.6 6.1

0.3 0.3 0.2 0.5 0.3 0.3 3.3 3.7 4.1

0.9 0.6 1.0 1.6 1.0 1.0 4.0 3.5 5.5

0.7 3.1 3.4 5.1

0.5 0.4 0.4 0.7 0.9 0.4 3.1 4.4 5.0

0.6 0.3 0.3 0.6 0.9 0.4 2.6 4.6 5.7

0.5 0.1 0.3 0.4 0.5 0.1

0.6 10.3

1.1 1.2 1.3 1.7 2.5 0.7 2.1 2.5 4.0

1.4 1.4 1.8 2.3 1.7 1.6

0.7 0.9 0.7 1.3 0.7 0.6 4.7 1.7 2.6

0.5 0.5 0.4 0.6 0.7 0.4 2.1 3.4 5.0

0.3 0.2 0.2 0.4 0.3 0.2 1.5 3.2 3.7

0.8 0.7 0.6 0.8 0.6 0.6 3.2 3.3 3.8
1.1 0.7 1.0 2.0 1.0 1.1 2.8 2.3 2.0

0.4 0.8 0.5 0.6 0.7 0.5 2.7 3.9 3.3

2.2 3.9

0.2 0.1 0.1 0.3 0.2 0.1

0.4 0.4 0.3 0.5 0.5 0.3 2.0 3.1 4.4

0.2 0.2 0.2 0.3 0.3 0.2 1.8 3.3 4.1

0.4 0.2 0.3 0.7 0.7 0.3 3.1 5.0 6.4

0.3 0.3 0.3 0.5 0.7 0.3 5.0 4.7 5.8

0.4 0.3 0.3 0.5 0.7 0.5 5.4 5.4 6.3

0.2 0.2 0.2 0.4 0.7 0.3 2.6 4.6 5.4

0.4 0.3 0.3 0.5 0.8 0.4 2.8 5.4 6.1

0.3 0.2 0.3 0.4 0.6 0.2 4.4 5.5 5.8

0.5 0.3 0.4 0.5 0.7 0.4 2.6 5.7 6.0

2.4 1.8 0.7 2.3 3.8 1.0 2.4 3.6 2.9

0.5 0.4 0.4 0.7 0.4 0.6 3.9 3.5 6.2

0.4 0.3 0.5 0.8 0.6 0.4 2.1 2.9 4.6

0.8 1.0 1.4 1.2 0.8 0.8 4.6 3.8 6.1

0.4 0.7 0.8 1.0 1.0 1.1 2.7 2.6 4.5

0.5 0.8 0.4 0.6 0.6 0.3 4.5 4.0 5.6

1.0 0.9 0.7 1.8 1.5 1.1 2.7 3.5 5.2

0.5 0.4 0.5 0.7 0.9 0.8 3.1 3.7 6.2

0.3 0.3 0.2 0.3 0.7 0.3

0.9 0.9 1.2 1.1 1.1 0.6 2.7 3.9 5.4

0.3 0.3 0.5 1.0 0.5 0.3 4.4 5.0 4.9

1.4 0.4 0.7 1.2 1.9 0.8 3.4 3.1 5.4

1.1 0.5 0.7 0.9 2.2 1.2 4.9 5.3 5.1

0.8 0.5 0.5 0.5 1.3 12.7 2.7 1.9

1.3 0.4 0.6 1.1 1.6 6.3 2.2 3.6

0.3 0.1 0.1 0.4 0.5 10.9 2.3 2.7

0.3 0.3 0.3 0.4 0.4 0.3 2.9 3.9 4.0

2.9 3.7 4.0

0.2 0.2 0.3 0.4 0.3 0.3 2.7 3.8 4.3

0.3

0.4 0.5 0.5 0.4

0.3 0.3 0.4 0.5 0.4 0.4 3.8 4.4 4.8

0.4 0.5 0.9 0.5

0.4 0.4 0.4 0.6 0.5 0.4 3.1 4.7 3.9

0.3 0.4 0.3 0.5 0.4 0.4

0.5 0.4

0.5

0.7 0.6 0.6 0.8 0.6 0.5 3.0 4.7 4.2

3.1 4.1 5.6

0.3 0.3 0.3 0.5 0.3 0.2 4.6

3.9 3.9 2.9
0.5 0.2 0.3 0.6 1.1 0.2 3.7 5.5 5.6

0.4 0.2 0.2 0.5 0.8 0.3 3.9 6.1 6.5

0.6 0.3 0.4 0.6 0.9 0.4

1.1 0.6 0.5 1.0 1.0 0.5 4.2 3.4 3.9

0.6 0.4 0.4 0.6 0.8 0.4 3.8 3.7 5.3

0.5 0.4 0.5 1.2 1.2 0.9 3.7 5.2 5.8

0.4 0.4 0.4 0.6 0.8 0.4 5.1 6.3 7.3

0.6 0.4 0.6 0.7 0.7 0.3 3.6 3.4 3.6

0.6 0.3 0.4 0.6 0.8 0.4 1.6 3.7 4.8

0.4 4.8 6.5 8.9

2.2 0.6 1.0 1.0 3.2 1.0 5.4 3.8 4.5

2.6 2.2 2.7 3.0 2.6 3.0 4.1 1.7 2.4

0.9 0.3 0.7 0.9 2.4 0.8 3.5 5.8 6.3

1.1 0.7 0.9 1.4 1.2 0.6 2.8 1.8 4.5

0.9 0.7 0.9 1.4 1.1 0.9 4.9 1.6 2.8

1.1 0.8 1.1 1.8 1.2 0.7 3.9 2.3 4.0

0.6 0.3 0.4 0.5 0.3 0.2 3.1 3.7 4.3

0.4 0.3 0.3 0.5 0.6 0.3 1.9 3.5 5.3

0.4 0.3 0.2 0.4 0.7 0.3 4.4 1.8 3.1

0.3 0.3 0.2 0.3 0.4 0.1 6.3 2.2 3.4

0.2 0.3 0.3 5.8 2.4 4.6

0.8 0.4 0.4 0.7 1.2 0.5 4.4

0.4 0.5 0.7 0.7 0.9 0.8 3.0 4.7 6.3

0.6 1.4 1.9 1.0 1.0 0.9

0.9 1.9 4.4 5.4

0.2 0.2 0.4 0.4 0.2

0.3 0.5 0.5 0.5 0.6 0.2 4.1 3.7 4.2

0.5 0.4 0.4 0.6 0.5 0.3 4.1 3.8 4.8

0.3 0.4 0.3 0.5 0.4 0.2 2.6 3.5 4.3

0.9 0.5 0.8 1.1 0.9 0.5 4.6 4.6 5.4
2010 2011 2011 2011 2011 2012 2012 2012 2012

4 1 2 3 4 1 2 3 4

8.0 5.4 8.2 8.1 6.7 5.3 7.4 6.8 6.7

5.8 4.3 8.9 8.5 4.7 4.9 6.4 6.4 5.1

5.4 4.2 7.2 7.4 4.1 4.2 5.3 5.5 4.4

6.0 4.0 6.3 7.5 3.8 5.3 5.7 4.8 7.4

8.0 6.4 10.7 7.1 4.5 7.3 5.6 5.5 7.9

2.1 2.6 1.1 1.1 2.0 2.1 0.7 1.3 2.2

7.1 5.3 7.1 6.9 5.8 5.5 5.3 6.0 6.5

7.5 11.5 2.1 2.5 17.3 8.2 1.8

1.3 3.1 4.5

9.9 7.0 3.6 5.1 13.9 11.2 3.8 5.8 11.9

7.5 7.8 6.2 6.6 9.9 11.7 10.3 6.2 10.1

5.2 6.2 4.3

10.8 12.2 4.4 1.8 18.1 19.6 5.0 2.6 12.2

7.2 5.7 3.5 4.2 10.3 8.9 3.5 5.3 8.1

5.0 3.8 3.1 4.3 8.6 5.1 3.8 5.6 5.7

7.7 5.8 4.7 5.2 7.5 5.9 5.7 6.1 8.1

7.1 5.2 4.2 5.4 8.1 4.9 5.8 5.5 7.7

6.8 5.8 5.2 4.8 9.2 6.9 6.2 5.4 6.0

7.1 4.6 3.1 4.2 12.1 6.0 3.9 4.7 6.1

7.8 7.4 3.8 5.6 10.5 9.9 6.1 5.3 6.7

4.1 3.8 5.6 6.6 3.8 2.9 6.0 6.8 5.7

3.2 1.9 1.5 3.1 2.9 2.5 2.2 4.6 1.5

2.8 2.1 2.5 3.1 2.6 1.7 4.6 4.3

2.3

3.8 2.6 4.6 5.0 3.9 3.3 4.2 5.4 5.7

2.5 3.1 3.1 0.6 1.6 2.3 1.9 1.6 2.4

3.9 3.6 3.8 2.1 2.5 3.7 2.6 1.0 3.1

7.4 6.0 5.1 5.5 4.0 5.5 3.2 3.7 5.4

7.4 8.4 10.3 9.7 5.3 6.5 6.3 5.1 6.3

6.4 5.2 8.1 7.1 4.8 4.6 5.1 5.5 6.6

8.1 5.1 8.7 7.4 4.7 4.8 5.9 5.5 6.7

6.0 5.6 8.9 7.8 4.7 6.4 6.1 5.5 6.1

3.1 1.7 2.4 3.0 3.0 2.1 3.5 5.1 3.3

3.9 3.5 3.8 4.8 4.2 4.6 3.1 3.8 4.9

3.4 2.4 3.0 0.6 1.9 4.0 3.0 3.6 2.9

2.6 1.6 4.4 5.2 3.9 4.6 3.9 4.6 4.2

2.9 3.4 3.8 2.4 3.4 3.0 3.7 3.2 2.7

4.3 3.1 5.2 4.2 4.2 4.1 4.3 4.4 4.2

3.8 2.2 3.7 6.6 3.8 3.9 5.9 5.1 4.9

2.9 1.4 3.8 5.1 2.1 2.8 4.8 5.3 3.4

Organic Carbon

SANDWICHed*
4.2 2.2 3.7 5.2 2.0 3.0 4.2 4.6 3.6

5.4 2.8 4.8 4.6 4.6 4.4 4.3 4.2 4.9

4.1 3.1 4.1 4.3 5.0 3.9 5.1 5.8 6.5

2.6 1.5 4.6 5.1 3.1 2.3 3.8 5.2 3.9

3.9 4.1 3.1 6.2 3.5 3.4 3.9 5.6 4.2

3.1 3.0 3.5 3.9 4.1 3.3 3.4 4.2 4.1

2.8 2.5 3.0 3.7 3.7 3.0 3.4 4.3 3.7

1.3 1.1 3.2 3.9 1.9 2.5 2.1 3.5 2.0

3.1 1.7 2.3 3.8 3.0 2.9 2.9 4.3 3.5

3.4 2.5 3.5 4.5 3.2 4.1 4.3 4.3 4.1

3.0 1.9 3.2 4.0 3.3 2.9 3.6 5.3 4.4

2.3 2.2 1.8 3.8 2.9 3.7 2.4 4.7 3.5

3.9 2.8 2.5 3.6 3.8 4.0 3.1 6.3 3.4

2.0 2.9 3.2 3.2 2.6 3.3 5.6 5.0

3.1 2.9 3.0 3.9 3.5 2.6 3.5 5.4 4.9

4.0

4.9 4.5 9.2 7.0 5.7 3.7 6.6

6.4 3.8 6.5 8.2 5.7 4.9 6.9 5.4 5.4

6.2 4.0 7.6 10.7 4.3 7.2 5.3 5.4 6.4

4.9 3.1 6.5 8.0 6.2 6.2 6.6 5.7 6.8

1.6 1.5 0.5 1.0 1.4 1.8 1.3 1.7

2.4 2.7 1.1 4.0 5.5 3.4 2.0 12.0 4.2

5.9 3.5 6.2 5.1 3.6 4.0 4.1 6.0 4.9

4.4 2.9 5.3 4.7 4.1 5.6 4.8 6.3 5.7

4.1 2.1 3.8 5.6 3.8 4.6 3.8 6.5 4.7

4.1 3.3 4.5 4.8 3.5 4.2 2.9 6.5 4.9

5.8 5.2 6.9 7.4 5.1 4.2 5.4 14.1

6.3 3.4 4.8 6.3 4.3 3.8 4.6 5.5 4.6

4.7 4.3 4.9 5.6 3.4 4.3 4.7 5.5 5.2

5.0 3.6 4.3 5.3 4.9 4.6 3.4 5.3 4.0

5.8 3.0 4.5 5.2 2.6 2.8 3.5 4.7 2.6

5.1 3.9 4.8 4.9 3.7 4.4 4.8 5.7 4.6

5.1 3.2 4.1 5.1

5.2 3.0 4.6 5.4 4.1 3.7 4.6 5.0 4.7

4.2 3.7 5.6 6.1 3.4 4.5 4.6 6.6 4.7

0.6 1.2 3.7 1.5 0.8 2.1 8.7 1.7

8.2

2.5 2.5 5.1 4.4 2.7 2.7 2.6 3.9 3.7

4.6 5.5 3.2 3.0 6.4 6.3 3.1 3.1 4.9

4.3 3.9 1.6 3.2 5.6 3.9 1.8 3.8 3.7

2.7 3.2 4.8 5.6 4.6 2.9 4.0 4.1 4.5

2.3 1.4 3.7 4.9 2.7 2.7 4.0 4.4 3.3

3.3 3.6 5.3 5.6 5.5 4.4 3.9 4.2 5.2
3.0 2.9 7.3 1.5 3.0 2.7 3.4 4.1 4.9

3.9 4.2 2.4 6.3 2.8 3.2 3.8 4.3 4.1

1.1 1.8 4.1 1.1 1.4 2.9 2.6 1.1

3.2 3.1 4.8 4.9 3.5 3.3 3.8 5.1 3.6

2.0 1.5 2.8 5.2 1.9 1.7 3.6 4.2 3.6

4.3 2.8 4.7 5.2 3.3 4.3 5.0 3.3 5.2

6.0 3.6 5.2 5.7 4.6 6.1 4.5 4.5 6.3

7.5 3.6 5.4 6.5 4.2 5.8 5.1 4.9 8.0

5.1 1.5 3.1 4.1 3.3 2.9 4.4 4.4 4.6

5.6 3.4 6.2 6.1 5.1 4.8 4.9 4.9 6.1

6.0 3.6 5.1 6.0 4.9 4.4 4.9 5.0 6.5

4.1 3.1 5.0 6.3 4.0 4.5 4.4 5.2 5.0

2.4 1.4 2.4 3.1 4.9 2.3 1.4 3.8 3.8

5.0 3.2 5.1 6.5 4.3 3.6 4.1 5.6 3.9

4.5 1.2 2.8 4.8 1.9 1.9 3.7 4.0 2.0

3.9 1.9 7.5 5.8 3.6 6.3 5.5 5.1 3.9

4.2 3.0 2.8 5.1 3.8 3.4 4.1 4.2 2.9

4.3 2.5 2.8 4.8 3.0 3.8 3.7 4.9 3.0

4.0 1.5 2.8 4.6 3.6 2.8 3.8 4.7 3.6

5.9 2.8 4.6 5.1 3.7 3.4 4.8 5.0 3.7

2.9 3.7 4.9 3.2 2.4 3.2 4.1 3.8

5.7 3.1 4.6 4.1 4.9 5.6 4.5 6.1 4.8

4.8 2.0 3.9 4.0 2.2 0.8 3.1 3.7 1.6

3.5 4.4 5.3 3.8 3.8 3.2 4.9 5.0 4.4

4.1 3.9 7.0 4.8 4.2 4.4 5.7 5.8 4.8

13.7 11.3 4.8 3.4 15.8 13.1 3.1 8.8

8.2 12.7 1.6 2.3 11.6 12.1 1.6 6.7

8.9 11.3 3.8 3.7 13.1 11.4 2.3 5.2

2.9 2.6 4.2 4.3 3.7 7.4 4.9 5.2 5.0

4.8

2.9 1.6 2.8 3.1 3.6 4.0 3.0 3.7 3.8

4.6

6.5 4.6 5.2 4.8

4.3 2.8 4.2 3.5 4.4 8.7 4.6 5.6 6.2

5.4 6.4 5.1 6.7

4.2 3.2 2.9 5.8 3.1 3.7 5.7 5.4 5.4

2.3 4.7 5.3 4.3 3.2 4.0 5.3 5.5

4.6 2.3

4.9

3.5 2.7 4.1 5.0 3.5 6.7 4.2 5.0 5.5

4.6 3.6 3.7 5.3 3.4 4.5 3.7 5.2 5.4

4.9
4.1 3.3 6.0 6.1 3.1 4.2 3.9 5.7 4.4

7.0 3.4 6.7 7.0 4.2 6.3 5.3 4.8 6.5

4.6 5.3 7.4 4.6 5.3 4.9 4.7 4.6

3.6 2.9 3.8 4.3 4.9 3.0 4.1 4.2 4.2

5.3 3.1 4.3 6.2 3.8 4.3 4.7 4.9 5.1

6.5 4.7 6.5 6.0 4.1 4.6 5.0 3.8 5.6

6.4 3.5 8.1 5.9 3.7 4.2 5.9 5.3 5.6

2.9 2.0 4.7 5.1 2.4 3.3 4.2 5.1 4.1

4.1 2.8 5.1 6.9 3.8 3.7 3.7 5.5 4.5

5.2 3.1 6.8 8.5

3.8 3.1 5.7 3.5 3.8 3.6 5.0 3.8 3.7

6.0 5.8 10.6 4.2 3.2 3.6 5.9 4.3 4.4

5.4 12.7 5.6 5.8 4.4 4.2 7.1 4.8 5.7

3.4 3.7 1.3 3.4 4.2 2.8 1.9 7.7 3.2

4.7 3.7 1.5 3.0 4.8 3.2 3.0 6.4 4.0

2.2 2.9 2.7 2.9 3.6 3.0 3.8 7.4 3.3

3.2 3.4 2.6 4.9 3.3 3.9 3.9 4.2 3.9

3.1 2.3 4.4 4.7 4.4 3.7 3.6 5.0 5.4

6.6 8.1 2.2 2.6 9.2 5.0 2.2 4.8 5.9

7.9 8.7 1.6 2.7 8.2 6.9 3.1 5.0 6.9

7.0 7.7 2.5 3.5 8.3 5.2

7.5 7.2 0.8 3.0 8.2 7.0 1.5 8.9 8.8

4.5 3.2 5.1 6.5 4.1 4.5 5.9 6.6 5.3

3.7 4.3 5.2 5.5 5.9 6.1

3.4 1.7 3.6 6.9

4.2 4.3 4.0 4.9 3.9

4.6 4.0 4.3 4.1 3.8 4.2 3.5 4.9 4.4

5.2 3.7 4.9 4.6 4.7 4.7 3.9 5.6 3.6

4.8 2.3 3.8 3.5 3.6 3.0 2.9 4.8 3.1

7.2 4.5 5.1 5.5 5.6 5.7 3.6 5.8 4.3
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

1.1 1.3 0.8 1.0 0.7 0.7 0.8 0.8 0.6

0.8 0.8 0.7 1.1 0.7 0.8 0.8 0.8 0.8

0.6 0.5 0.5 0.7 0.5 0.5 0.6 0.6 0.5

1.0 0.4 0.4 1.0 0.7 0.5 0.6 0.7 0.7

1.1 0.8 0.4 1.4 1.0 0.6 0.5 0.8 1.2

0.7 0.3 0.3 0.6 0.7 0.2 0.2 0.7 0.7

0.7 0.7 0.6 0.8 0.5 0.4 0.4 0.6 0.4

0.6 0.3 0.6 1.3 1.3 0.7 1.1 2.9 2.5

1.0 0.3 0.5 1.2 0.9 0.3 0.6 1.6 1.2

0.7 0.6 0.8 0.9 1.0 0.4 0.7 1.2 1.1

2.0 1.2 1.4 1.9 1.7 1.0

1.7 0.8 0.4 1.5 1.5 0.6 0.3 2.1 2.0

1.0 0.2 0.4 1.1 0.9 0.3 0.4 1.3 1.2

0.7 0.3 0.5 0.9 0.6 0.3 0.4 1.2 0.8

0.9 0.4 0.6 1.3 0.9 0.4 0.5 1.5 0.9

0.9 0.4 0.5 1.0 0.6 0.3 0.5 1.1 0.8

0.6 0.3 0.4 1.0 0.8 0.3 0.4 1.4 0.8

0.7 0.4 0.6 1.2 0.7 0.3 0.4 1.5 0.6

0.6 0.3 0.6 0.8 0.6 0.3 0.5 1.1 1.0

0.5 0.4 0.6 0.7 0.5 0.4 0.7 0.7 0.4

1.4 0.7 0.8 1.4 1.1 0.5 1.2 1.6 1.3

1.2 0.7 0.7 1.1 0.8 0.5 0.8 1.0 1.0

0.7 0.6 0.6 0.7 0.5 0.5 0.6 0.9 0.7

0.7 0.3 0.3 0.5 0.5 0.4 0.4 0.3 0.5

0.5 0.4 0.3 0.7 0.6 0.5 0.4 0.5 0.7

0.8 0.5 0.4 1.2 0.9 0.6 0.5 0.8 1.2

1.0 0.7 0.5 1.0 0.9 0.7 0.7 0.8 0.9

1.1 1.5 1.4 1.6 1.1 1.4 1.2 1.6 1.3

0.7 0.9 0.6 1.6 1.4 1.6 1.6 1.2 1.4

1.0 0.7 0.5 0.8 0.6 0.7 0.5 0.6 0.8

0.5 0.4 0.5 0.8 0.6 0.4 0.6 0.9 0.7

0.8 0.9 0.8 1.1 0.9 0.9 1.1 1.3 1.3

0.5 0.4 0.5 0.6 0.4 0.3 0.3 0.4 0.5

0.9 0.6 0.8 1.1 0.7 0.6 0.7 0.9 0.8

0.4 0.3 0.4 0.5 0.4 0.4 0.3 0.5 0.5

0.6 0.5 0.7 0.8 0.5 0.6 0.6 0.6 0.8

0.7 0.7 0.7 0.8 0.5 0.7 0.7 0.7 0.8

0.4 0.4 0.5 0.5 0.3 0.4 0.4 0.3 0.4

Elemental Carbon

SANDWICHed*
0.6 0.5 0.5 0.8 0.5 0.5 0.7 0.5 0.6

0.7 0.8

0.8 0.7 0.6 0.9 0.8 0.7 0.8 0.9 0.7

0.7 0.7 0.7 1.0 0.9 0.6 0.7 1.1 1.0

0.6 0.6 0.7 0.7 0.5 0.5 0.6 0.7 0.6

0.4 0.5 0.5 0.6 0.8 0.4 0.8 0.6 0.8

0.6 0.6 0.7 0.9 0.5 0.5 0.6 0.7 0.5

0.4 0.4 0.5 0.6 0.4 0.4 0.5 0.4 0.4

0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.3

0.5 0.5 0.8 0.8 0.4 0.4 0.8 0.6 0.6

0.2 0.5 0.5 0.6 0.4 0.4 0.5 0.4 0.5

0.9 0.7 1.0 0.9 0.7 0.7 1.0 0.8 0.6

0.6 1.1 1.2 1.2 0.6 0.6 1.1 0.8 0.9

0.5 0.8 1.0 1.1 0.6 0.7 1.0 0.9 0.9

0.3 0.4 0.5 0.5 0.4

0.5 0.5 0.6 0.6 0.5 0.4 0.6 0.6 0.4

0.5 0.5 0.6 0.6

0.6 0.5 0.7 0.6 0.7 0.6 0.8 0.5

0.9 0.6 0.6 1.2 0.7 0.6 0.7 0.8 0.6

0.8 0.6 0.4 1.1 0.5 0.5 0.6 0.6 0.8

0.8 0.5 0.6 1.0 0.6 0.7 0.7 0.9 0.9

0.2 0.1 0.1 0.1 0.1

0.5 0.3 0.5 0.7 0.7 0.3 0.6 0.9 0.6

0.8 0.7 1.0 1.1 0.6 0.9 1.0 1.2 0.8

1.0 0.8 0.9 0.9 0.6 0.8 0.8 0.7 0.6

0.5 0.5 0.8 0.9 0.5 0.5 0.7 0.7 0.5

0.6 0.7 0.8 0.9 0.6 0.6 0.8 0.5 0.6

0.6 0.7 1.1 1.1 0.9 1.0 0.9 1.2 0.8

0.7 0.7 0.9 1.1 0.6 0.7 0.9 0.9 0.9

0.7 0.5 0.6 0.7 0.5 0.6 0.6 0.5 0.5

0.5 0.5 0.7 0.8 0.5 0.6 0.7 0.6 0.6

0.4 0.3 0.4 0.6 0.4 0.4 0.5 0.4 0.6

1.1 1.2 1.5 1.1 1.1 0.9 1.4 0.9 1.0

0.7 0.9 1.0 1.0 0.6 0.7 1.0

0.6 0.6 0.8 0.9 0.6 0.7 0.8 0.6 0.6

0.5 0.5 0.6 0.7 0.5 0.5 0.6 0.5 0.6

0.1 0.1 0.1 0.1 0.1

1.4

0.4 0.5 0.4 0.4 0.3 0.5 0.6 0.4 0.5

1.1 1.3 0.3 0.7 1.9 1.4

1.0 0.4 0.6 1.1 1.0 0.4 0.6 1.4 0.9

0.8 1.2 1.1 1.1 1.0 0.9 1.0 1.0 0.7

0.4 0.4 0.4 0.4 0.2 0.4 0.4 0.5 0.4

1.3 1.8 1.8 1.5 1.2 1.6 2.3 2.1 1.4
0.8 0.3 0.5 0.9 0.9 0.5 0.4 0.9 0.7

0.5 0.7 0.7 0.9 0.9 0.6 1.0 0.8 0.7

2.2 1.5

0.1 0.1 0.2 0.1 0.1

0.3 0.5 0.5 0.5 0.4 0.5 0.6 0.6 0.5

0.2 0.3 0.3 0.3 0.2 0.2 0.3 0.3 0.2

0.7 0.5 0.6 0.7 0.4 0.5 0.5 0.6 0.6

0.8 0.7 0.7 1.4 0.7 0.8 0.7 0.9 1.2

0.8 0.5 0.7 1.1 0.6 0.6 0.6 0.7 0.9

0.5 0.6 0.6 0.9 0.5 0.5 0.4 0.7 0.9

0.7 0.6 0.6 0.9 0.6 0.6 0.6 0.8 0.7

0.6 0.5 0.5 0.8 0.4 0.5 0.5 0.7 0.6

0.5 0.7 0.6 0.8 0.6 0.5 0.6 0.7 0.7

0.3 0.3 0.3 0.4 0.2 0.3 0.4 0.3 0.3

0.6 0.6 0.8 0.9 0.5 0.6 0.8 0.7 0.6

0.9 0.8 1.0 1.1 0.6 0.9 1.1 1.1 1.0

1.1 1.0 0.9 1.1 0.5 1.1 0.8 0.9 1.0

0.4 0.5 0.8 0.9 0.4 0.5 0.8 0.8 0.6

0.5 0.5 0.7 0.8 0.5 0.5 0.9 0.6 0.7

0.6 0.9 0.9 0.9 0.5 0.7 0.9 0.9 0.8

0.6 0.8 0.9 1.0 0.5 0.7 0.7 0.8 0.7

0.5 0.7 0.8 0.6 0.6

0.7 1.0 1.0 1.0 0.5 0.7 0.8 0.8 0.8

0.4 0.7 0.7 0.8 0.4 0.7 0.9 0.6 0.6

0.3 0.4 0.4 0.5 0.4 0.4 0.4 0.5 0.4

0.5 0.5 0.4 0.5 0.5 0.5 0.4 0.5 0.5

1.5 0.4 0.2 1.8 1.4 0.6 0.3 1.7 1.7

0.8 0.4 0.4 1.0 1.7 0.5 0.5 1.2 1.5

1.1 0.3 0.2 0.8 1.1 0.3 0.3 1.1 1.3

0.5 0.7 0.8 0.7 0.4 0.5 0.7 0.7 0.8

0.9 0.7 0.6 1.3

0.4 0.5 0.5 0.5 0.3 0.4 0.4 0.5 0.5

1.1

0.7 0.8 0.8 0.8 0.5 0.5 0.7 0.7 0.8

0.7

1.2 1.4 1.3 1.0 0.7 0.8 1.0 1.0 0.8

0.5 0.6 0.7 0.8 0.6

0.7 0.9 0.8 0.8 0.5 0.6 0.8 0.8 0.8

0.5 0.5 0.5

0.3 0.6 0.6 0.4 0.5 0.6 0.6

0.6 0.4 0.3 0.6
0.6 0.4 0.4 0.5 0.4 0.5 0.4 0.5 0.5

0.7 0.7 0.6 1.2 0.7 0.6 0.6 0.7 1.2

0.7 0.5 0.6 0.7 0.8

0.3 0.3 0.3 0.4 0.2 0.3 0.4 0.4 0.3

0.8 0.9 0.8 1.2 0.5 0.7 0.9 0.9 0.8

0.8 0.8 0.7 1.1 0.7 0.8 0.8 0.8 0.9

0.9 0.9 0.9 1.1 0.5 0.7 0.8 0.7 0.7

0.4 0.4 0.3 0.4 0.4 0.4 0.4 0.3 0.4

0.4 0.4 0.4 0.5 0.3 0.4 0.5 0.5 0.5

1.2 1.2 0.8 0.9 0.6 0.7 0.8

0.6 0.5 0.6 0.8 0.7 0.6 0.6 0.9 0.7

1.3 0.5 0.7 1.2 1.1 0.6 0.5 0.9 1.0

0.5 0.7 0.4 0.6 1.1 0.5 0.5 0.7 0.5

0.6 0.3 0.4 0.7 0.5 0.3 0.5 0.8 0.6

0.9 0.4 0.5 1.0 0.7 0.4 0.6 1.0 0.8

0.7 0.3 0.4 0.5 0.6 0.3 0.4 0.8 0.7

0.3 0.4 0.4 0.4 0.4 0.3 0.5 0.5 0.5

0.7 0.5 0.6 0.7 0.5 0.6 0.6 0.8 0.7

0.8 0.4 0.4 1.1 1.4 0.3 0.4 1.5 1.0

1.1 0.4 0.4 1.6 1.4 0.3 0.4 1.4 1.2

1.1 0.4 0.5 1.1 1.3 0.4 0.5 1.4 1.1

0.8 1.4 1.2 0.2 0.4 1.2 1.0

0.9 0.9 1.1 1.5 0.8 0.9 1.0 1.1 1.1

0.5 0.9 1.0

0.7 0.6 0.8 1.2 0.5 0.6 1.0

0.4 0.4

0.4 0.3 0.4 0.4 0.3 0.3 0.4 0.4 0.4

0.5 0.5 0.7 0.7 0.5 0.4 0.6 0.8 0.6

0.2 0.2 0.2 0.3 0.2 0.3 0.2 0.3 0.3

0.6 0.6 0.7 0.8 0.5 0.6 0.8 0.6 0.6
2012 2012 2012

2 3 4

0.6 0.5 1.0

0.6 0.5 0.7

0.5 0.4 0.6

0.5 0.3 0.8

0.5 0.4 0.9

0.2 0.3 0.6

0.7 0.5 1.1

1.0

0.7 1.4 1.6

0.4 0.5 1.2

0.7 0.5 1.8

0.7 0.2 1.4

0.3 0.3 1.0

0.4 0.4 0.7

0.4 0.4 1.3

0.4 0.5 0.6

0.3 0.4 0.8

0.3 0.4 0.6

0.4 0.6 0.7

0.4 0.5 0.6

0.6 0.8 1.1

0.6 0.7

1.1

0.7 0.7 1.0

0.4 0.3 0.4

0.4 0.3 0.6

0.5 0.4 1.0

0.6 0.5 1.1

0.9 1.0 1.4

1.3 1.0 1.1

0.5 0.3 0.7

0.4 0.5 1.0

1.1 1.2 1.3

0.3 0.4 0.5

0.6 0.7 0.9

0.5 0.4 0.6

0.6 0.6 0.7

0.7 0.6 0.8

0.4 0.3 0.3
0.5 0.5 0.5

0.6 0.5 0.8

0.6 0.7 1.0

0.5 0.6 0.7

0.5 0.4 0.5

0.5 0.7 0.7

0.3 0.4 0.4

0.2 0.2 0.2

0.5 0.7 0.5

0.5 0.5 0.5

0.8 0.9 0.7

1.0 0.9 0.7

0.8 1.0 0.8

0.5 0.4 0.5

0.5 0.5 0.6

0.6

0.5 0.4 0.7

0.4 0.4 0.9

0.7 0.5 0.8

0.1 0.1 0.1

0.3 1.0 0.6

0.7 1.0 0.7

0.7 0.8 0.7

0.5 0.7 0.6

0.5 0.7 0.6

0.6 1.0

0.7 0.7 0.9

0.4 0.5 0.5

0.5 0.6 0.5

0.8 0.7 0.7

1.5 1.2 0.9

0.6 0.7 0.6

0.5 0.5 0.5

0.1 0.3 0.1

1.4

0.3 0.5 0.4

0.4 0.5 1.5

0.3 0.5 0.9

0.7 0.8 1.0

0.3 0.4 0.5

1.2 1.5 1.9
0.3 0.4 1.1

0.5 0.6 0.7

0.2 0.2 0.1

0.7 0.9 0.9

0.2 0.3 0.3

0.5 0.4 0.7

0.6 0.6 1.0

0.6 0.6 1.0

0.6 0.5 1.0

0.5 0.5 0.8

0.4 0.4 0.7

0.5 0.5 0.8

0.2 0.3 0.2

0.7 0.7 0.7

0.8 0.8 0.8

0.8 0.7 0.7

0.6 0.7 0.6

0.5 0.7 0.4

0.7 0.8 0.6

0.8 0.8 0.7

0.5 0.6 0.5

0.8 0.9 0.7

0.9 1.1 0.6

0.4 0.3 0.4

0.5 0.3 0.6

0.4 0.6

0.3 0.7

0.4 0.5

0.5 0.8 0.8

0.3 0.4 0.6

0.6

0.7 0.9 1.1

0.5 0.8 1.1

0.6 0.9 1.0

0.7 0.8 1.1

0.5 0.6 0.9

0.5 0.4

0.9

0.7 0.8 1.0

0.3 0.4 0.6
0.4 0.4 0.4

0.5 0.5 0.9

0.5 0.5 0.9

0.3 0.3 0.3

0.7 0.6 0.7

0.7 0.7 1.0

0.7 0.6 0.9

0.3 0.2 0.4

0.4 0.4 0.4

0.6 0.5 0.8

0.5 0.5 1.2

0.5 0.5 0.6

0.4 0.6 0.6

0.4 0.6 0.9

0.3 0.5 0.6

0.4 0.5 0.5

0.5 0.5 0.8

0.3 0.5 0.8

0.4 0.5 0.9

0.3 0.7 1.0

1.0 0.8 1.1

0.7 0.6 0.9

0.4 0.5 0.4

0.3 0.3 0.3

0.5 0.6 0.4

0.2 0.2 0.2

0.6 0.6 0.4