NATL INST. OF STAND & TECH NIST

PUBLICATIONS

AlllDb 13fibM^

1Mb mII

Selected Values of Chemical

Thermodynamic Properties

Part 2.

Tables for the Elements TwentyThree Through Thirty-Two in the

Standard Order of Arrangement

D. D. WAGMAN, W. H. EVANS, I. HALOW, V. B. PARKER,

S. M. BAILEY AND, R. H. SCHUMM

270-2

- U51S3

o

*z

A*"

.»' »F C,

\ *

*£AU Of

•A o

U.S. DEPARTMENT OF COMMERCE

National Bureau of Standards
THE NATIONAL BUREAU OF STANDARDS

The National Bureau of Standards is a principal focal point in the Federal Government for assur- ing maximum application of the physical and engineering sciences to the advancement of technology

in industry and commerce. Its responsibilities include development and maintenance of the national

standards of measurement, and the provisions of means for making measurements consistent with

those standards; determination of physical constants and properties of materials; development of methods for testing materials, mechanisms, and structures, and making such tests as may be necessary, particularly for government agencies; cooperation in the establishment of standard practices

for incorporation in codes and specifications; advisory service to government agencies on scientific and technical problems; invention and development of devices to serve special needs of the Govern- ment; assistance to industry, business, and consumers in the development and acceptance of commercial standards and simplified trade practice recommendations; administration of programs in cooperation with United States business groups and standards organizations for the development

of international standards of practice; and maintenance of a clearinghouse for the collection and

dissemination of scientific, technical, and engineering information. The scope of the Bureau's

activities is suggested in the following listing of its three Institutes and their organizational units. Institute for Basic Standards. Applied Mathematics. Electricity. Metrology. Mechanics. Heat. Atomic Physics. Physical Chemistry. Laboratory Astrophysics.* Radiation Physics. Radio Standards

Laboratory:* Radio Standards Physics; Radio Standards Engineering. Office of Standard Reference

Data. Institute for Materials Research. Analytical Chemistry. Polymers. Metallurgy. Inorganic Materials. Reactor Radiations. Cryogenics.* Materials Evaluation Laboratory. Office of Standard Refer- ence Materials. Institute for Applied Technology. Building Research. Information Technology. Performance

Test Development. Electronic Instrumentation. Textile and Apparel Technology Center. Technical

Analysis. Office of Weights and Measures. Office of Engineering Standards. Office of Invention and

Innovation. Office of Technical Resources. Clearinghouse for Federal Scientific and Technical

Information.**

•Located at Boulder, Colorado, 80301. ** Located at 5285 Port Royal Road, Springfield, Virginia, 22171.
UNITED STATES DEPARTMENT OF COMMERCE • John T. Connor, Secretary

NATIONAL BUREAU OF STANDARDS • A. V. Astin, Director

NBS TECHNICAL NOTE 270-2

ISSUED MAY 6, 1966

Selected Values of Chemical Thermodynamic Properties

Part 2. Tables for the Elements Twenty-Three Through Thirty-Two

• in the Standard Order of Arrangement

D. D. Wagman, W. H. Evans, I. Halow, V. B. Parker,

S. M. Bailey and, R. H. Schumm

National Bureau of Standards / Institute for Basic Standards / Washington, D.C.

NBS Technical Notes are designed to supplement the Bureau's regular publications program. They provide a means for making available scientific data that are of transient or limited interest. Technical Notes may be

listed or referred to in the open literature.

For sale by the Superintendent of Documents, Government Printing Office

Washington, D.C, 20402 - Price 40 cents

PREFACE

Technical Note 270-2 is the second of a series of publications

containing material prepared as a revision of the tables of Series I

of National Bureau of Standards Circular 500, Selected Values of

Chemical Thermodynamic Properties. This Note contains revised

Tables 24 to 32, covering the elements silicon, germanium, tin,

lead, boron, aluminum, gallium, indium, and thallium, and compounds of these elements following the Standard Order of Arrangement.

Tables for the first twenty-three elements and their compounds,

and a discussion of the symbols, conventions, units of energy, and

conversion factors used in this series are given in National Bureau

of Standards Technical Note 270-1.

Donald D. Wagman, Chief,

Thermochemistry Section,

in
CONTENTS

Preface iii

Table 24 Silicon 1 Table 25 Germanium 7

Table 26 Tin 11

Table 27 Lead 17

Table 28 Boron 26

Table 29 Aluminum 37

Table 30 Gallium 48

Table 31 Indium 53

Table 32 Thallium 57

Cumulative Index 63

IV
Si-SiOc

24

COW

w

to

COa

H

PiW

P<o

u

z

>>P

O

w

sH

<!UI—

S

w

Xu

o

COW

<

>

P

uH

U

W

w

CO

o

atO.

id U

4)

T)C

n)a

o

hCw

S

o

s s

00

4-1

53

IDu

c

a)

(0

,£>3

CO

S.5?

o >

0)

CO

o

0) P

C

nl

3

o

00

st

o

in Ost

O

00

CO

00

CM av

oo c^j

in

u-v cm vo

i-i vo m

o

o oin

oo

CM

o °^

r-l 00 VO s o\ <f 00 c

VO Ol CM OV CM St st en

CO on vO en m vO

in \o 00 st CM CA

r-» r~- 00 T-l t-i >-l VO cn .-1 t-l CM St

f-t CM en o- m vO

~.n en t-l o O

CO 00 r-. m in m CM st m

n Ov r-- st CO ^ CM vo st

t-l s*

CM

COo

St

CM

VO

COo

St CO mCO 3

o o

St o

St vO

u ojjoOtiOoOoOciOCXloOCiOoCoOoOciO MM

n) 43 N o

J-l u

U <n

01 iH 3 M

cr o

, + +

+ CM CO + +

co w co en c/i co co

+ + 4 i A

ob ch r-i i-i i-i c CM CO o O 1-1 i-( i-l -W t-l 1-1 1-1 1-t •H

CO CO CO CO CO CO CO CO CO
SiO,

24

U

vo -d- ^ o OV

r_t VO VO CM CO 00 •tf in ° P. o O£ O o O Ov r~- o

vD r—1

r-l t—i r-l rH ovrH SI

o>

r-l

p-v o 00 <* <t 00 2 r_, <t CM ao r-l OV CO

*-) co

rt

O ,_J 00m CM 9 VO vO CO rv vo ov CO o 1-1 r-l -* vO CO CM vl- -* r~- si- rv m vO

U

°3? in co o> r-* oo o o

CM ov to rH vo vO CO I vO o ui rv CM vO

ao tt r-l CN CM CO CM CN

>- Ov OCM om H PC fH o

ao

a o

n! (M CM CO U <f CI vo <f r-l

O vO r-. vO r-i in 00 00

4_l 3

vt en co o i—1

00 00 <r <t oo <! ov in

O

rtO

O r-l CO vO in r-l i—i

r-l cm vo r~. i m

o> CM CM CM CM CO CO <f «± >*

m rH I "o I 1 1 i 1 1 1 • i i 1 c £

n) *»

0-. o

13o

CM OV

00

<r cm CM CM r-l OV r-l r~. o o vO CM

O i-~

n

X r-»

m r-~ <t vO 00 Ov CM 00 <t CM vt I—1

r~- ov oo r-i oo

h <J r-l r-i r— r-l 00 r-l CM CM oo oo

mm oo ov co -t

CWc

CM CM 1 CM CM CM CO CO -cf <r vo rH O

CO

m

idE zoo

oo

<4-l 3 ^ «o

coo r-l

M

r-l

O oo f—l CM

rH

M 1 h CO

*—i

fd

O OV 00 00 r-i

m CM CN Ov vO <! oo >

<t r* ov r-l o in 00 vo -4t

m -* CM "3 x £ .5?

a\ r-i r-l CM o r-l CO vt 00 r-l 00 00

at o r-l CM CO r-i r-l r-l r-l I—1 CM o O uV Ov <M CM CM 00 vO r-l N CD st (V. VO c £

CM CO VO Ov r~. Ov eo CO CO I"- -3- vD

W

10 X

r-l r-l r-l r-l

V

id

O c

1-1 O 60 cr oo 00 00cr

i-l 00U cr

u cr cr cr o o 60 60 6 i rt r-i id 0) rt ra to id

r-l 1-4 r-l r-4

C

rt II II II II > E B e

0. ^

nj 01 0) cu 01 X 4-1 4-1 4-1 4J c id id id id C 4-1 4-1 4-1 4-1 W uc

rt

2*

Iny

co p

CD

4J

a

4J

01

4J

00

4J

(0

n

aa CO rO3

0)

4-1 i

•o

01 01 01

a >%

NN

N

H c

rt •o 1H 1-1 1-1 i-l

•r4

a c a

C

r4 o o o o

ti 4-1 1-4 1-1 i-i 1-1 1 1 EJ •^ c c c c

rH

£) 2 pi 3 p

r-N CM >—'

^^

fc vO <t i r*iv CM vC PCo m r>

0> PI

O EC ^ o o

VO oo o O o •H CM CM

CS <r 3 S3 1-1 i-l v^ CO 1-1 1-1 CN O PC PC CM CO CO CO 1-1 — co co Pn fe

i-l 1-1 i-i 1-1 i-l c\ <1 CO CS CM VO i-l iH

CO CO CO CO CO PC PC PC PC PC PC CO CO
SiCl3 H

24

W2w

co

COaH

05W

ftO

ft

JHQO%

o5WH

<5Ui—( SwXu

ftowwD

<5>QWHUww

en

>-

ofcW

•r-1 oC

Rj

0-cW 3

n)

tou3 •~\ CQ co

i—

-*

«) CM Co CO •|H

cd iZ H o

SP

©CM

SB

H-i 3

0)UC

a)m

,£) CO

U«3 X M CO o >

ft ^

rd COo

CO

0) oC

cdo

ft o

VO

i-l CO CM

0000

VO oo

vo

LOCO

oo r-» <r <r

CO

ir>

r-i -ii

CO in

00 CO OO

vO r~- vo

IT) LO

m o

c^

CO

vi- CO CM CO vo 00 CT> CM

r-~ o 00

O

O 1-1 o O • CM o vO <f

-* u-i 00 «tf

0000

00 vo

vO

CT 60 60 D*

cd co 60

M i-l 00

11 II B B ^ *

cu cu u 4J

to to o

CMOvO I vo

CM pn CO Pk VO CO fa 1-1 fn PS PC en

1-1 1-4 1-1 CM

CO CO 00 PC

i-i r-i pa

CM ^1- o O

C

I-l i—

1-4 CO CM i-l

CJ>

O o PG PCO

•H 1-1 1-1 1-1 1-1 1-1 00 00 CO oo oo oo
SiBr

24 2

>«QO

a5WIH<Ul-H wuou

£><>pwHuww

to

U

to

(4CW

JO

Xi6

T3c

(4a

n)cw 3

rt4)

In3 •-n CQ <ti—

sjrt CM c

01

•r*

*-» XI

n)

(ti 2 H e ex

CO

•nP

433

CO 3 4= £ .5? U 4) £u

CO

0) DCO

fa o

CO CO OV o CO

CM o

00

in

CM

CTi CTN

O

00 CT\ i-< -I i-l CM O 0> 00

<t

O -I in o ^

CMo B

CO

cc COm o

60 60 00

CM ^i ^t en

Ij 1j co oa pa

u

oa pa Ij co cm oaM

en cm pa 1-1 l-H i-l -<f co

as 35 ECOOO

M PC CO

1-( 1-1 1-1 •H 1-1 1-1 i-l i-l -rl CO CO CO CO CO CO co co CO

CM

coH
Si 3 C

24

Ww

CO

toWi—

H

CiWo2

5hQOWsH

<!UwUO

toW<>PwHUWW

to

u

(n CO o CX

SPI00 S1

OO

>t-l

CO

u«3 J3 g .5? ^

COuo

to

<u D

T3C

rt

«J£o

CMst

a\m

vO VO CO

st

vo

st

o>

VO vO

oo

asstO

st

in

m to

VO VO VO

oo

I-- O

in st

r-4 !"•

CM CM CM

st

CT\ VO CO

<no

vO

mvO

<t oo

CM COVO O

vo o

-vi- vo

St

co

VO

COco

vo

COco

VD

CO

CO

vO

CO

CO

oooCT\ CO

CO

00

st

00o

st

00o

<t

CM co CM co St CM

I-- 00 co st

m C^ o\ o 00 o> o vO O I—

r-4 1—

CM CM• o CM 00 o CM VO st m vo 00 C\ ON

60 60 60 60 00 60

•x 4-1 o O o

01 CO CM CM c

4-1 —I

w BC PC

<fl « • «

4-1 c TJ

m

m o

in o (1)

m CTN o

60

O

N in rm • Hi •H 1-C T3 X ,Q fi .-i

4-1 01 3 o C

is

m .C

u t4 t4

vo

/-N VO

sc CO [K o [XI •H

**• J^ CO

1-1 CM CM <t CO • /-n 55 SC st st

CO St In

ccl co o 60

T-i CO x> X 3 (11 o JC

co

CJ c_> CM C

CO CO CO CO
SiH3 (CH3)-Si(OC2H5) 3 Cl

24

st st o 00 00 ctn CM o

,_,

r-. CO o i-l r^ CO St o

u-i ° a

£ m r^ CM 00 oo st St r^ vo o i-t i-i CM CM st CO r^ m

CTn

i-Ii

r-l 00 m ON on r-. 00 CT> in 3

• U

CM

i-l

CO

st m

i-i o

CTN

CM

vo" m

VOCO

00 m

VO

CM

aj

oo

CO vO VO i

r^ VO oo o CM VO

1-1 i-l U

'pP in

vo I-l co «* av o vO I-l a> CM CO r^ r-l

' X

CM in CM CO m -I m

co CO CO <f m vO VO O

>- o\ I-l r-4 sr

in

CO a o st

<o

IN) co i-H CO U a CM

vw ON m 00 CTN

S3 St CO en r^- 00 00

n) in CM CM CM CM in

4) 1 1 i-i -I i X

o

i i

-ac £

(TJ ^> ON >a

o u

i-l 00 00

00 co m m CM

in

•£ X cm' CO r^. -d- 00 ON CM VO St St m a\ ov r-l St

00

st

ON

CM M -Q 1 vO m m vO CTn O CM CO CTN co i-i CO ON CW

c

1 i 1 r-l CO CM CO r-l i-i St st 1

55ool-l

OO

U-I I O ctn m

vO

00 O

St

i- ,J CM 00 r-. M 1 .-i r-l In

vt-»

CO i 1

flj O CM I-l i-i i-l CM CM <! VO o- 00 vO CM oo in St CM VD

CO

CM

r—oo

CTn -I

U"> O vO CM CM ON VO O <r r~- co OO CM r-4 !-H CO > 5

£ .5?

1- 0> £ In ^

st st m 1^ r- CTN CM 00 CO CT\ CM 1

CO 00 CTV O

oru

VO VO 00 O O st

CM

00

CMVO

CO -I

CM

CM

CM

CMSt

CO

oo

CO

CM

r-l CO

CO

CM

VO

00 cW

to

St m m vO vo r-~ co r-l <t CM m vO o VO vO CM o i-l i-l i-H r-i 1-1 CM r-l 1-1 CM 1-1

J3 1) O" O* a- O" cr cr O" V cr bd cr

i-i

r-4 6

X)

ro CO

00 00 00 00 00 00 ri-H 60 •H •H -H •r-l •H •H •H 00 o CJ •H

i-i

c

id>•a.

rt

01

01c

01c A c 01 C

<0

(0

r-4 c o 01 fS 01 X i-l .rf w 01 •rH e 01 01 03 c o CO 09Ou

o

,_4

(J Pu

01 CD c c r-l 01 03 r-4 O

c

flj

01 01 a r-4 01 CO <0 •H c r-l i-l U

h C c <0 t4 a 1-1 I-l CO 0} •H CO o

01 01 aj i-l CO (0 1-1 •H

r?

r-l CO •H r-l 03 U c r-4 01 r-l 01 •H i-H 1-4 CO CO •H

rS" "O rC o

4-1 «

1-1 u

J-I

3

CO <0 >> c •H c CO >. •H r-l r? o co rH o

4) I-l 4J 09 CO <o r-4 J3 CO >s x\ &

o >^ r-l

T-l 01 I-l r-4 !-H >n 4J i-H jC o 4-1 4S A >N CO CO u 1-1 >, •H A 01 >-. 4J 4-S 01 O 4-1 U x:

X) r-4 03 co A CO u 6 XI 01 4J g J 01 01 4-1 c

>n i-l t-l u i-l 01 <o 4J <0 01 a] 4-1 <0 5 01 A r*> >> 01 >v e id 01 u E u 01 h CO 4J i-l C 6 A •H 4J 1-1 4-1 •H u •H 4-> X 5

id 3

01 •H i-l i-i 4-1 L4 01 u 01 u 01 r4 01 01 M

e a > •a 01 4-> 4-1 u 4J 4J 4-1 4J 4-> XI 4-1

*—

\

£

u o CO /—

V

CO I-l VO

v_^ CM CO CO ^r» St

CM /TMvCO X

CJ

r-l u

CO

•"Nm

St ^"N CM •-V co /-\ St *^N -* m ^—

V

1-1 g

o

CM CO g

s

CO n /-s ^ m •-v ^P y»\ PS in CO

55CM

•H

01 3

6 s s

PSCM U

CO g

•—

v

CO g

CM o

in

PSCM g

o

CO g

CM o

PSCM O

CO

>«-vCO

55

COCO

PSCM

CO CO CO CM CO >• N-^ O N— 8

•

o \~* o g

"st "st co w PS PS * PS S3 ^-* PS v-^ PS >-• PS s^- fa fa

•H •H •H •H •H •H 1-1 •r4 H •H •H •H 1-1 ^^ •H •H g •H H CO CO CO CO CO CO co CO CO CO CO CO CO *—

CO CO **~* CO
Ge-GeH,

25

coW

w

co

coa

H

BSW

CUO

Pi

2

5h. QO

a

wH

<Ui—i w

asu

h

O

COH

<:p

wH

U

ww

co

u

co

"So a

(0

d

Ca

co

3

0)

CQ

.—

IT) co

'i-l 2

J3

H

9

ioo OCM

3

CO

O

w

M

1- 41 ^

4)

(4 CO

4) D

c

o

o

CO

LA m oo cm oo cn <r>

00

1-H

u-i

oo

o

00

o

St

st

ON

o1—1 CM

m <t

cr* rv

S|- rH

m m 00 m CM o\ VO o CT> CM CM 00 m CO CM

St CO CO vi- I—

l-( MD St <t vo 1—1 r-l i—

CM st

oo

CM.

en cm oo en

00 60 00 00 OO 00 00 00 00

^1 ,0

41

. + + + +

+ cm en st ""> CM cn St o

(U 4) 4> 4) 4) 4> 4) <u 01 a) o o o o o o O O o o

n)C

o

60

a)

cm cn + O O St St

cm cn PC EC

4) 4) 41 4) O O o o
Ge 9 H2 6 25

u

>u

4>cw

(0 XI

X>6

Ca

nt X.c u

c

n)

U

£ .5?

U. 01 =£

fa. ^

O

mC

C

cfl

o

o

00 00 CO

lA 00 vO

O

<n go 9i «

00

-ct 00 O 00 o

St

to ot 00 00

00 o

X li en a

4) c O W

fa fa %

CN St en 4) i-i r-t fa fa X o o U

41 41 4) CN « 01 o o O S3 o O

r-l CO O i-l en o

41 41
GeTe.

25

coW2w

co

coaw

cuoU2QOwHUswuo

tou<>QWHUWw

CO

Q

r^ -d- r~~ ON in

m CM ON

m • P.

oo CO <f- oo r^ o om

vO

O oo <r co -J co oo oo oo

a> CM i—

CM i—*

>n

i-H

bl

X)

*13 "^ NO NO ON

m • rt i—

1-1 NO NO 00 -* NO

&o

U o ON on

in

NO CM

CO

NO

NO CMOt—t NO i—

NO

in

'pP in nO NO r^

m in CO VO CM CO 00 NO CM 1 co r^ On r-i o i-i CM co

>-

00ON

Lfl

CM in CM NO CO CM CM CM

oo

(X o

nJ (VI U

in CM o . O in <t i—i ,

4-> 9

in on NO

O i—

-*m r- o

n) CM r^ r~ CM 1 CO CM -I -I

4) I I i 1 I 1 I X

XI 6

rt ^j

>.

d CM in -J

ex

u CO

O i-i r^ CM ON NO NO in co o oo

M ^ vO in CO r—

r—

r—l co CO in NO CM

m CN CM M3 CM <)

w

m i—i i oo r-~ CM '-, CO I-l CO i-H CM <f CM CM 1 •* -* S

rt

M CO

H-l 3 o oo

i—i NO CO

CM

O

CM co

in

CM

CM o 3

in vO i-l CM CM <1-

h

>•

rt i—1 4-J £.2>

1- CU > h ^

ON 00o

NO

CM

co

CM OSON

00o

00

I—* oo

m ON ON bfh

CM CM

CM

CM

m

in

CO

NO

CMo m

CM

NO NO

in

1-4

i-4 o

1^-

1^

CW

(0

in CO ON in CM 00

O o CO in o CM

-i CM CO i—

co in CM 1—1 1—1 i-i CM CO

-Q

u ^ rt tr M 60 i-i 00 60

y 60 CJ 60 rr 60 o 60 o CJ 60 CJ 60 60 CO

i—

rt

C

rt^a

rt

4->

d cW OC

rt

CD £>CO

O

01

O

CM X P co

X) <) c

i-i

rt r-l

rt Sc u

CON^ fn mCM

^i

cu CM <f

m co CN 3

rt H

U

U

U CO CM <f S3 CM CD CU (U

CO,

m

m PC

M 1-1 I-I c/> CZ> CO

HH CU o $ a $

ai cu o

cu O 8 o 8 8

cu O
Ge 3 N4 -Ge 2 SiC

25

2

Q

O

sw

H

<

wo

o

w

<;>

p

wH

U

w

w

coM

C

•r-i -C

ID

c

(!)

(0

u

t« 0> 5;

0)

U

CO

<u n

C

G

cm cm eg cm

O

in O

O rCM 3

oo

m m cm m

60 00 60 00 00 60 00 00 00 60

-* CM T-l 1-1 CJ T-l 3 + CM o o o •H CO CO T-l en en Pn O c_> c_> cm en v-' CO cm en co c

4) 01 01 oi 01 01 01 0) 01 0) 01 0) <u o o o o o o o o O o o o O

10
Sn-SnFn 26

O

coM

cm

>

cW

C

Ri

cW

3

nJV

h

1

*"-\ CQ

I-l

"rt CM c

CD

• W*-> ,0

nl

fl) 2 H

o d,

©CM

J3

u

CD

in vo

in in in

o .co in cm

in

COOoo

i oco

co i-i -d- co

vO CO

CT* vO

CO 1

COCO

oo in in co

60 00 00

Id

<u

T)a

01 >>

4-1 «

T-l h

cfl 43 60 &

3

£

•\ M 1-1 1-1 m

fc

id

II II ii £ 6

T3 a

B

•v •s (U cu

CU 0) 4-) 4-1 0)

4-1 4J rt rt u

rt rt 4-1 4-1 ca 4J 4-1 •H •I* 4-1 0) co a.

i-i CO

• • u y • T3 T3 CU cu T3

4-1 4-1 n M 4-1 CO CO P. p. CO

CO vj

CO CO

CM <f St O B X

C C C

CO CO CO

o

o

C C C

CO CO CO

EC K

O O +

11
SnO(OH)F

26

U

in in in

vO

° a

o CT» en

en

CM

CJN i-l 6/

4) -I

>n o

3 ,_^ 00 <)•

•") •

CO

U

(J ciCM

CM

vO M3 00

MD

CM CDen

1

iTI CM in

in

en

CO tt

>- ON OCM

oin m

.^H X i—i u

Cfj 00 a cr- m CM U M

in <t vO CO CM en CT% r*- o

4-* 3

oo o\ —l CM m en -* en in

itf co en r» O o O CM CTv in

4> f—

i

•—I 1—

1

r-i i-4 i r-4 X

i 1 1 t 1 i

c ji

rt>a N4- <r r^ CO co CM <f CM r^- m r^ mo *cr md ej\ <t %

.* o> r- ON 00 o vD CM CM CM Ol » CO O H 00 u en r»- r^ 1^- CM i—

t

CM r—i in en en en en en O i i l CM r-l C 1 i 1 | i i i i i i 1 W

c

£ »oH o M3

(—1 ZM s o CM H t—

(

i-4 In I w.

cd >

M

i—< 4-» vD CO vO r^ er> CM oo o vO D X CO <r on CM <r o o m \D E .5? MS H in MS o in <f J ^

4) >-. t> co ~J- 0> in in o i-H f—

ON c £

00 in 00 CM CM M3 en r^- 00

(0

f—

1

1-1 1-1 CM CM CM en ^H 1—1

Cv

n) cr cr a cr cr u cr

cr

t>0 cr cr cr CJ a

T3 W

a a <9 cd a '""

to a) ea

C

crj i-i -J

>- li II 0- E E

rd ,G c • •s r-l CD 01 C 1-1 o 4-1 4-1 W 1) '^ cjX

X CD ed o fX 4-1 4-1 c t-i i-H c •-< 0) CO r-l rt L. cr a) u

II at II c

II • II CO c

o TJ m in

,a E c E

•W E 4J 4-1 T _ P^ E

3

ft CO CO SC CM CM u * a> •o at ... .« in cm cj o

s: cj o o

cm O O O

V

•c U • 4-1 i—

i

<u 4-1 ,—

t

i-l 4J c <d o a) CJ N cd cj O o O CJ CJ O cj r^ in

Cfj aJ 4J 4-1 P= t-t 4-1 X K 4J a CO CD c 0] O (OS K CO

n! 10 cr cr cr 3= X en vO

•H • a) •H • « a CJ CJ O CJ 3 •o *o a 1 •a T3 E u c 4J c c 4J c c 4-1 gg 3 CO -H 3 co -1 •h CO •^ p

CM

v—

fc o O

vO CM CM

CM fe

•-s. X

CM 1 W

A) re • 1 CM r-l i-l o + CM CM en -*

* VC o o

J3 i—i t—

i

I—

I

X X

(1) o CJ CJ o o CJ CJ o o

c c c c c c c = c

00 co co CO CO CO CO CO CO

12
26

V

aoM

c

•ft X,

go

(3 W

a

o

(0e s

o H

o P- O

I00 ©CM

P3

4)U

C

co +j

to

U

«

co i—< *-» 6.2?

*i co

r.. >*

CO

I-l u

(0 p

c

CO

n)

£

o

CO

stu~l St CO CTt CJN

CMCO

ooo

CM

CO CO

CO CM 00 OO vO CM CM O co ^o m co

ON 00 VO 00 m in co o m O CO o CM CO i-<

i i Oi-l

cri

1 oI-l i cy>

i

St- CO

1^- VD

i-l CM St 00

00 00

u-> CO

CO StCr- CO CD CO

ON vO on o <T. Sf O m r^ 0^ Sf vO o\ 00 Sf

CM m st- CO CN aj i-i o o\ 1^.

u-l CM CO CO CO

13* o •H

i-l CO 00 60 u

um

CO.

CM

I-l M

C

co St

!-i U

CO 00

ti en m ffi <Ti 6

S3 cm w m CM C7. O st- « O UJ O <u CM 8 o*8 O O r-~ O 4J Uo 8

CO 4J o co O W CO 01 CO K O co O tu u S

"O c u

1-1 oCM K

00

CO

1-1

i-l pq CO

!-i st m CO PQ U tc i-l i-l CM m o u O M

a c e a c

CO CO CO CO CO

13
Snl2 26

OQcomc

re XIc

•-03

rei)

In3

PQ1co

re 2 u

rda

rt U

re XC

(1) >aoucUc

f. 5 a>

>-. cWXX6C>XcW

's? moc

n!

ca J33

CO

0/u

U

00

rsl

U

©3 X. £ .5?

1-

V£

4/

reo

to

<D Dvc

cd

R)o

^3oo

c^

oo

CO

f-l -1

00 inm <t

<t 0^ a\ -•t- rH CM CM t-t

00

t-l 00 COo

oo iri oo oo

II II B e „

9) «T

4J 4J

a)a

MM CO c a C

go CO CO

CM

O + '-n «-' CO cm «d- c*

CM -J- CJ CM • • •

-<t o C ^ CM CSI CM

cm o co <u CO >* i-l i-l r-

« a ^ a

** lz

OOO

a ft

a

CO CO CO CO co

g ^ CO CO CO

14
Sn(CHo)

26 4

U

c

oM

cX00rt

r^

1—

ON

iri 6 Or 6

covO

CTv

i-l

0/m

XI 3>-> CO

O

V CO

CMO

CM

ico M

> OCNI ein H EC <—

U

CO

(X o

rt rv] u vw OA

rt 5

i—

o

<u I—

PC

1

JS

n)

I—* >- riO

CO av CM CM -( CO i-l co m CO m i-i m m 2 ^ h» F-l CM l~- O <f t—i in on co O p^ <r i-i cm in CM <) h <c] CO CM i—

co co m vO 00 O in co <r i-l CM i i-i i 1—1 i—

i-l i—1 CM 1 1 I-l i-l CM i—i R 1 i i i i 1 i i i

rt n

0©

4-1 5 o

h

*H—

rt ON vo av m O i-i CO <J\ O i-l CM <f oo VD CO o >• "3 ,£ 6 .5?

co in vO 00 O vO 00 CM vO OS m r~ as r^ o CO

ctf m -* m m VD vO l~- in m m vo r~- <t r^- oo oo O Jh <1> m vO CM <f OV CO i-l Ov VO CO r~~ m i-i o <f 00 c ° £

ON r~ i-l i-< CM vO CO CO O CM m cm i-i m vo i^ w

CM co CO CO CO CO <f CO <f <f <r m CO i—i 1—1 i—i

£> a

CO

w a* cr

£> o o- O O o o o o o o o o o •H 00 i-i oo •H 60 6

XI

rt i-l i—i 1—1

C

ni>

P.

cd

4-J c

cW

in

(LI U

a

rt

to

u

03DD

T3C

rt

rt

£

1-4

II6

oT

4-1 rt 4Jw

•a

4-> 0]

CO

vO

1-1 co co co

CO

ECCM CM vo

CM

ro

CO g

PQR g g g

CO CO

co P3 fE CO CO in ECCM CO <t ^ !J CM CO n m ca rC S3 E2 g g i—i S~\ /—

•-\

a>

• a CM

CM

CM CM CM § CM CO m on

~cf COfd CO

pa COcs •~* 3 u CO J-l <T S-l SJ >J CM CM CM CM ,M 1-1 CJ u o

PQ <r PQ pq pq pq R R R

I-l H I-l H I-l CJ *^ v^^ >^-^

fi R g ^ a C R R R R fi R H co g CO S~' CO CO CO co co co co co CO CO co co

15
Sn(C2 H5

) 2 H2-Sn(CH 3 )3l

26

O in a p. o

vo U £ Crv t-i orV

T) 3

•

en

U

idu

1

in

ao W

s OCM

e

iTI

.,_ 33 f^ u

id CO a aid l\J o ow

rt 3

8I

"o C £

a! _

>a

o

idu

•-t o o a> ov vO .-I -J- CM vT CM

CM ~-( vo r» CM CM O ^ .-I O in cm t-i u <] i—

(

T-I 1 r~ CM t-l CM CM 00 <f CO CO

1 1 1 I 1 1 1 1 1 cW

c

l-l

oom

9

oO

h

V*H>

idr DC o in

in o>

r-. co oen

vO ~J O

vO O

or CI 00 oo ov in vo r~ r~. u 00 • • • • • • • V U 0) • CM vO -J- r~ CT> co O

c 5

00 Ov CM CO CM r-l vt VT> W

v. £5

<~i CM CM ro CM CM CM X 1) cr cr cr cr cr cr a*

£1

id •rl 00 T-l 00 •H f-l oo f-i O fl -H

i—

l

i—i i—i *-* a

XI

(/)

c

id>a

id £ c

IDc

C a) W o

u

c

id

•r-t a

i-o

104) P

a

.co

t-i ID ,0 a

>»o X CM c

i-H <t

id 33 rH

VO O

id o O

3 c c

£

•H •rt

^-s u m VO CM 33 CM v^

fc PS CM * r-l VJ vO CM C_> ^ <r vO O « H

CM •"N CO CM •-v •—

\

CM CO CO m •-N 33 m m ^"N y—s /—

*

a> 33 CI o x 33 co co co

CM w 33 CM O 33 33 33 3

id H

O o U O v—

o o o N—' N—

CM v—' N_• \-^ c c c c e £3 C3 CJ CO 00 oo co CO CO CO 00

16
Pb-Pb(OH) 2 27

WW

tnaH

PiWo

Pi&po

cri WEH<Uswxuow«>QWHUWw

UcoMcc3

n)v

CQ

i-H

ojCOz

a. uvE

T>C

a.ocWcoo>U

0)CW

(0 X>X•iH oC

rt>.a.

X.CW o |X

°p?ICO

0J|

J33

^-i *j 3 X! g .5? £

tuo

coVDc

rto d

"0 ou-1

CO

00 <r

m CO i-l CO -tf o

sj <* vO

m «* U"| 00

o> CO

1-4 CN

l~-

m

m

co I CO

vO oo

CO

oo o o

00 60 60 £

Ti

II

U

B

CQ

m

4-1 C) CO o 4-1 m CO

en •H • T) •a 3 4-1 3 m

u

CO

.-1 co -t + + + + + » CM o o ffl

L CN1 CO vt U0 o o o eg CO o .£) XI X X XI XI X X X X x>

H4 P-l Pi p-l p-l P-l Ph Ph PU p-l P4

CS|

w o o X ^w' a X

PM

17
H

2 PbG

2 27

in o a

NO o £ ON

1-13

•->

oj

13 -* 1-4 in in

co

O

O VO NO ON m m i-i

i-4

NO

CM st CMco

On

CM

I

in

co tt

>- ON COM

ein u

00 a oaj N u

00 1-4 ON 00 1CO

00 <o <f 00 CO 1-1 m 1-4 NO co m ON CM NO

rt SI m r^ CM CO O st r^ ON CM ON m 00 1-4 i-4 NO NO

ON co i-l CM CO r~ st CO st 00 r-- NO r^ O 1 1 01 i-i CM CM vtf- .-1 r-4 1-1 1 1 1 I-l X

o

i 1 1 1 1 1 1 1 o

c £

rt! ^7 > a ON a

o tt o oo m r^ st 1-1 On co r-~ ON

j_ 3 00 St On 00 ON m m d 00 r~ St m On m m CM 00 00 r>. r-~ c

CM CM -3- 1—

i

i-i CM 1 1 1 1 W

c

• 1 1 1 1 1

£ O

OO

14-1 a d 5 O

h

v—

,

(4 >

«—< 4-» CM ON On On 00 r^ o- CO NO ON CM i-l CM

0/ 3 X i-l on no r^ 00 00 00 St ON st O St ON

t. £ .5? CM m i-~ i-i 1-1 1-1 -4 NO O m O NO O

4)c

b HI 00 On NO ON u-> CO CM 00 CO ON O St" !5 m oo on r^ CM st 00 St r-. r-l St ON r^ W CM no oo co CM CM CM CM CM CO CO CM co

01

1-1

,0 1) X cr

rt cr cr cr cr cr cr O cr cr CJ cr O cr cr rr 1-1 cr cr 3 in

tO CO 03 CO 00 to to to to ID to to 1-1 CO to

C

n) -I 1-1 1-4 1-1 a

II II 1-1 II II

rt e E II B B X

cW

c

oi «r E

01 V

OJ

4-1 4-1 r. u 4-1 4J a to Oi to 03 u

c a 4-1 4J 4-1 4J 4J

00 1-1 i-l 1-4 i-l 1-1 1-4 CO 1-1 to 00 1-1 i-i 00

rt i- 4J

+-> y II II II II II II . II 00 s II II B GO 10 a x> •O XI XI 41 4J e e e b B B 4-1 B . 4-1 6 S 4-1 3 to 03 x> 00 00 W s •t •* * * - ^ 4J s -, 0

c

Ml 11 Hi Oi 01 01 41 »** 01 00 •*s ai 01 Ml

4J 4-1 4-1 4-1 4-1 4-1 • 4-1 • 4J 4-1 » o a; CO CO CO CO 10 a CO Ml to to O

rt o 4-1 4-14J4-I 4-1 4-1 4-1 •O 4-1 st 4-1 O

n)

oo 00 to 00 to to 00 to 00 01 CO 00 .-1 to 00

00 00 N 00 O 00 "p 1-4 • t 1-1 • 1-1 1-1 • O 1-1 o T3 "O "O ^ XI O a XI c a 0 XI XJ £ d 4-1 4-1 4-1 4-1 4J 4-1 a 4J a 4J a 4J a

•^ 3 CO 60 00 00 00 co 3 00 •H 3 00 i-i to 3

CM

r-~ CM h + + + N Nt •* CM

1 st -3" oo ^-*\ CO •~^ •-N y~\ + ro

0> CM •—

V

— X — co O

3

O SB o o o + CM ' co st O i-i XI O N—' N—' N./ + CM <J- 1-1 1-4 f-l 1-1 1-1 O

rt P4 ^-^ co -3" no fa fa fa u O O O v—

H CM x XXX X X X X X X X X X

w P4 Ph P4 P4 P4 P* P-. PL, E-i p-1 CM C44 PL4
PbBrF

27

W2waH

atW

a,o

Phu2QOWHUswKU

Inoww<>QWHUWw

u

in

i—i ° p. • o £ i-H in

VO

cn o> I-l 13

>v <-h -I VO ON in

1-1 <d » • 3 CO u cn 00 l—1 O •-> U

CM cn «* oo

8P1

iTl

ooM

>. OCM in H EC i—i O

id CO* a o

ni CvJ o cn in U oo i-I r^ CM VO in m O On o>

© cn

«j ^

•*

m vo CM CM in r^ CM r^ r-lm 00

id i-i

O i-i cn vO in

m oo I i-t I © 0) t-i m i-i 1 1 i i i 1 I-H I *o i 1 I 1 ac j:

ex)

"ido

>-Prs oo •tf oo vO in •* cn cn cn s X 3

CT\ en r-. VO oo

© CM r-~ i-i

*H ^J cn in CM vO in <t CM r-~ cn c

r-i i-i CM r-l 1 t I i-l i-H CM

W i I 1 1 1 1 1

idEu

oo

M

O iw3 o

•-^ In,+-l

n) >-

i—t 4-> in in -J- o © i-l O-N oo r~ r~- <f r^ r~ vO r-- 3 X co r-~ vO m i-H >* cn o 1-4 CT> O CT\ oo r^ cn £

.<? CM «* vO VO r-~ VO o o on

OO r-l cn inO

01

u o> i-l <f i-- cn i-l i-l F^ r^. VO in cn

© cn vo VO

C > O CM «* in

O VO 00 VO «* cn >J3 cn i-i cn

©

W

(0

in r^ Ov CM

Oi-i CM CM cn <r cn **

m oo

©I-H cn

43 i> 43

id

O o O o CJ cr o tr tr tr tr

O tr CJ CJ CJ o c

-0

W

<da « aa <a c

id i-i >. i-i ii a.

id

ii 6 £ G e

4)

C 4J = w uoc

id

ID

4-1

P4o

10

a;

i-i

II e

41

•l-J a)

4-1 SO

10

4-1 09

"O

4J

l-H

II E

i-ineT-i

ii S 3

CO J-l CO ^ V CO .« 01 01 01 T3 4-J 4J 4J 4J C a • ^ o a S) «

id

u •a o 4-1 4-1 4-1

L

id co 01N

co

CO

co CO CO

C

*-* « •H •H • i 3 CM T3 Pi 13 a T3 •o IS. £

i-l i-l c 4J 4-> 4-1

7- CJ CO •H 3 CO CO CO •-s u 43 en CN CM Ph CM CM i N-/ En CM l-l i-l • CM CM U U

r~. t-l CJ o CM *~\U P3 pa 2

CM

u 43 43 *~\ + cn PO 43 43

43 P-l Ph Pm pa 1 cn o . 43 Ph Ph 2

a> Ph• • • o o i-l + CM cn o u Ph • Ph c o o I-l Vw> cj u U ^ u pa • O 6 U 3 o rO 43 o 43 Ph PS PQ pq pq N^ o 43 £

pa

id 43 PU Ph 43 PM 43 XI J3 43 43 43 43 PM 43 v. H

Ph CM en Ph cn Pm Ph PM Ph Ph Ph Ph CM cn Pm

H19
Pbl

27 Z

><QO2

a.w

3SE-

<;u2w

asu

u.oww>QWHUWw

u

CO 1

o\ oo sO

r—

<* SO

O

•ao oE

oo

r-l

rH St

CM

CM

rH

in

01

cu sO T3

OS OS r-l rH •

"<3 1^ r> 00 00 in St so St

m

>s co

U rH in «* t-l in Os in r-l St

r-l <f

m r~ CM CO St so 00 CM 3

l-J

U

=Pi

in

sO

sO

in

Qs

oo

X • >• o\ o St •*

otsi in

.PH EG

—

u

CO

a o

rt

r\i o Os sO

U IH oo in St co in Os

O vO CO r-.

O CM CO

*j s o rH o co

r* o st co St so St w-l St"

rt CM -* CO St vO 00 CM Os St Os St CM 1 1 1 1 i 1 1 1 rH CM CM CO 1 as

"o 1 1 1 1 c E

rt t > rt -* P^ a " 

u OS 00 st vO o rH 00 rH 00 SO p~

© St oo SO 1

.*

— ^

rH sO oo

O o- o OS rH so 00

OO St oo St

S* CM rH o CM so I-H sO 00 so Os oo co oo CM c 1 1 rH <r 1 rH CM rH CM in cm CM co CO 1 Wc i 1 1 1 1 i i t 1 1

rt OO

X r-< CM

Q MM

a 00 oo

hjJ P-J

© • h

f—

r-. i-5 «* rH 1 CM1 ***

rt >

6f

rH 4-» <r o> co 00

m 00 <r CM CM SO St 00 rH o o 3 .c Os Os O o Os oo m in m r-l <-< so r^ 3

co CM in £ .5? o OS Os oo Os OS CM CM CM CO CO r^ CO sO oo rH

0)

U

V st o r~ «t SO 00 Os r- CO OS r*- • Os sO OS CM SO c £

CO sO 00 1-4 in r~ CO 00

O rH sO OS OS CM St r- 00

W

(0

co st in r- in SO CM CM CO co CO co co St

in r- Os CM

X 0/ X rt cr o c O" cr tr o CJ

u

u

a o* CJ CJ

O CI CJ

O 5

-a

03

a « « aa at ca r-l > r-< II 0- H

ii E

43C

C

B

4) 4J

W 01oc

rt

CO

a.uo

COCD c

t-inE

at

4-1 «

4Jn

4Ja

4-1

i-i

iiE

r-4

IIE 3 •o a

10 4J

41 eg • n 4) 4)

X 4-1 • 4-1 4-1 C M o S3 aj

rt 4-1 *o o 4J 4J

C

(«

a 4)M oo

CO CO c

•— •rl •H • 1 3 o c o "O •D K £

4-1 o c 4J 4-1 PC2

I) •H 3 a

O o r^ t-< CM o «* PC CM o O 1 s—

U. in [X, o -O J3

r^ CM • St -O Ph Ph 2

CM *-N

M Ph CM CO 1 CO CO sO sO so 2 V CM o CO St o o o o St St St c + CM CO St r-l CM o o CM CM CM CO O O O 41 3 H M M 1-1 v_^ l-l CO CO CO CO CO CO CO CO CO CO CO L a pQ X) -Q -Q JO -O X) X> ri -O jO -O J3 XI XI £i -O v. H

Ph Ph P-i PM Ph P-i Ph ft Ph Ph Ph Ph Ph Ph Ph Ph Pm ~

20
PbCl

2

* NH3 27

10Ww

to

toa

H

u

&

o

PiPu

P

o

I

W

DCH

<U

wu

o

towD

>

p

wH

U

ww

to

U

coM

C

njC

5)

3

idu

t-i

co

rt 2

n) H

op.

SP

ocm

O

c

rt

<n X>3

10

ed

E.5P

o >

0)

id to

uy

vP

C

nj

3

o

o

00

in o> oo n

o

00

I

oo 0\ CM I-l I-l o o

O a\ o o O o o

.-i

1

i I-l

1

i-l

1

i-l

1

r-M

1

.-H

1

enm

I

o

a

oo oo o

vT CF\ 00 en

t-i r^ r^ CN| • « • o <t 00 I-l m en CTn cr\ en <n en CM

o

o

o CM en CO o\ oo

CM CM en

CO CM en «* 00 en en en <t

os

oX•uu

o

— cm W W o

o

o

oCM O

tti oo

o -s o o

mo

<u CO-O

Ph

<! o0J 0) 00 H

XI .n

Ph Ph

o

<u H

XI

Ph

sT

en §

XI

Ph s

Ph

o 5*

XI ]^, <=n >£> Ph » • •

• CM CM CM LU CM •—

v

•-n •-\ J^

y~\ en en cn • en o p o c 55 5=5 55 5=5 <-H ^^ ^^ v^ \—

u X X X rQ ,n

Ph Ph Ph F4 P4

21
PbCl2 - 3/2 NH 3 27 2QOwIH<U1—1 wu

InO

toWP

<!>QWHOWw

co o Pu O £

On

i-l 6J ^ T3

i-H3 , o CM

>-) e a) • • U

vO r~

C/3 on <t U i

in

cm

00X

>- a. OCM

m ."^ X —

id CO a o^

n! (VI On U um o- CM

4_« 9r-l ON

IT) o On

41 CM i-M I *0 1 1 c E

<i

'--*

>•a o u

SO to

O CO

mCM CO 00 CO o in 00

O CO cm o o O 00

X -* i-M CM oo oo r~ CO in NO NO CO -* r~ On r-l r~ •* sf CM

h <] (Nl co

m * -tf CfN i-l CO CO COm no oom o I-l CO NO

1-1 I-l i-l CM CM i-l r-l i-l CM i i I-M CM CO r- CM

C 1 1 i i 1 1 1 1 1 1 1 I 1 1 . WcE Q

0O tf

W 9 o h

IT) CM r~

m -m <r ON ON

O NO CO -J- OnO CM -tf co

O CO > 3 X -* m <r <f CO CO NO O r- m i—1 CM NO m <t NO NO i-M or £ .5? NO .-m <r co M3 o O i-l no CM moo -M CM r-» 00 CO

CI i- &> CO CM co <!• ON <r i-M CO

O CO ON 00 "0 no r^ CM o r~ c 5 O i-( co i-i O 00 O i-l NO O vO r^ On <f ON NO 1

CO

WD

CO CO co -tf vO CO -tf •>» «tf uo <!•<! O- >n

m ON

1—

oCM

co

,0

V

-O

It

O

O CJ o o o o o O o o o o o o O

O

-a

co c

rt>>ad

x: c cW 0)uc

nj

10 J33

CO

a.uu

01<u C

-oc

rt

a)

CO

CO

1-1 CO oCM XNO• NO § co -3- co CO CO S co

co J* CO

CM CM § CO J2 CO § § "°. § § co

CM CO

g

co co

j§ S §

co CM t-i co • P5 cm co

m co

—-v PC *5 z z -* <! CM

4) CM

H

K

N in oo

CM CM CM CM i-l CM CM CM CM CM • • • CM CM <r 3 i-l i-M I-l I-l U u u u u M CM CM CM CM CM I-l M o o o CJ O XI m PP « M pq M M M 1-1 M X X co XI x X XI Cm Xi X Xi X XI x xi x X X Cm Cm X

Pm CM Cm Pm CM Cm Pm Cm Cm CM Pm Pm Cm Pm Pm CO CO Cm

22
PbO PbC03 27

Wi—

W

oo

ooWHWo

Piui—

<!PoWH

<!UI-H wuowwp<>QWHUWW

U

m o-\ r—

CM 00 CM

m

vO o ex U o

i-i VO

o"

CM

mCM

ov

1-1 Of

>> X>

1-13

•n e

GO

cdu o

oo oo

CO

1-1 00

Cfi -It oo «+ <n oo

0O iH "*

O csP in

oo

K

>- ocvl in

*j to .—

o

CO CO a o

cd cm O CM CO in

m 00 CM

•*-> 3

r- en r» o-v cr.

m CO O r- oo <f r-s Ov

a> CM <t CM 1-4 <-i 1-1 a 1 I i 1 i 1

T3 6

n! ^

a. o

cdu <fr vO o o 0> VD 1-1 ^ CO i-l in

m 5 X CM VO <3" CM \0 i-4 CM 00 r~- r~- oo Ov

^H ^i

O 00 00 OO 1-^ 1-4 "0 CM r~- vo o i-l cWc

CO1 Oi-M1

CM1i-41 cr> i-i i i 1

1-41 i r-l CM1 CM1 2 ow

oo

14-1

M 3 o h

M-l cd >•u i—t -M 00 oo r-~ oo

O av oo r~- i-m in

O vt avO OV 3 X <3- oo i-» t-4 r-- vo 00 vO OO i-i VO -* CT. -I 00 £ .5? 00 1-4 O "O 1-4 i-l vo 00 vD 00 -* vO i-i CM 00

<u ^ <u •* iH

m i-H l~- oo <fO CO -*

m 1-1 r~- in o c £ h ^ m 00 "0 i-l oo o ov i-4 CO U0 oo O vO C7> ON W

CO

OO 00 "0 00 CM OO r^

O 00 o 00 i-l CM CM <t

1-4 CM rH CM i-4 CM

XI 0! X>

rt o o" cr o o o o o o O

uyO o rr o a

XI

m

to aj CD

C

cd>.d

cd Xj c aw uue

ni

to X>oo

-t-> &o

10<D D

-aC

ni

CtJ g

i-l

II

<u u

CD

4-1 03

T3 o

CM oCM

S3 oCMS3 ^^ IS S3 CM CM

r~-

Jh CM i-l i-l 1 i-l • • i

En oo 1 vO 00 CO oo OO

CM p-{ CM CM CM oo 00

M I-lM I-l 00

p^ /-*\ ^N •^v

M I-l 00 in XI Xi

~d- r» r~- -* PM Pm < < CO co 8

CDOO o 0O .* <f XI *<) CM CM Pm o o CM CM CM CM CM CM CO o PM 3 o PM PM \—

PM PM 1-1 I-H

M 1-1

H I-l 8

CM

<d GO N_' *-• oo S3 S3 XI Xl XI £> XI Xi CJ 6 H xi XI Xl Xi X> xi PM PM PM PM Pm PM Xi XI XI

PM PM PM PM PM PM oo OO oo CO 00 co PM PM PM

23
Pb(CH 3

) 4 27

U in • o- "o

vO o £

ON

I-l OJ >1

1-4 T) 3

>-> ioo

o

"<3O MO co'

8P

i

in

IN)

oo X

>- ©CM in

CO

a. o

nj IM

r~ i-i U IW r» m -<f -I -* -* V43

rt 3 d CO* m r^ CM* 143 r^ en r- r^ cr. 00 oo CM u i .-i <-> t 1-4 I-l CM I i ' 1 ' ' T3C E

nj pH > O

«i oo »> vO vO CN a u •<r -* vD •-( o 00 co r^ r^ m r-. h 5t ^ co cm oo CM vO o co O CM r-l CM co ^ cm co -1 i-l CM »-l o CO CO CO <r CM c

CM CM CM CN CM CN -* I-l W

c

1 1 1 i 1

ooi o

In

«J >

«-H •*-» o in o\ oo VO in o 143 m o

ox 3 x co r-~ co o CM co 00 CM o\ CM E .5? co en >* CM CM CM CM CO CM M3

0) - _ r-. in CO CM r^ ^ m OS m co c 5 MO i-i CM in o mo CNI Pi -* CM W

ID

CM CO on CM CM CN co co in r^. x 0/ X D- cr cr

rt i-l 60 i-i i4 00 cr (J cr cr cr o cr cr cr CJ CJ CJ 3 09

f—

M »—

i

CO CO CO CD CO CO CO

C

rt r-4 •-I

0-

I-H I-l II i-4 I-l II

II II B II II E X

CW HIo

c

rt

ID X

3

co

o.

LaO

00

a; O

B

«T

4J

IS u

to

•o"

B

«T u

<a u

go

4J

CO

4-1 CO

•o

4-1 CD

E

«T u

CO

4-1CO

•o

6

01

4-1 CO

4-1 BO

XI

oT

4-1 03

4-1 09 o4-1 CO CO 4-1 4-1 4J U

CO to to CD O X! , s CN C • K « u ._ mm o 33

(fl OJ

4-1 4J •a

ai o

00

Ill 4-4 01 o

00 O rt a ID N 0} CO N to O

3 i E

1-1 •H 4-1 i-l •H o- o O

c •a 01 C •a CM CM E o o O S CJ o c c W W "4-1 U-l i-l 3 <D 1-1 3 1-1 CO oo u o

N-' + CM CM co X

fc ~* y*-\ O Ph

' •—

\

si- + CM CO CO CO o CN CM

.<* CM •—

s

X

g

X X •

*»-\ B m 6 g

o O Pm CM

0) en K u o o • •-v K BC CM CM tM CM CM CN CM z 3 o CJ o o o o o o i—l o

rt V—

sw' v~^ v-^ CJ N-^ E- X X X XI X X XI X X X

Ph Ph Ph Ph PM Ph pi Ph Ph Ph

24
Pbl2 . Snl2 . 8H2 27

CM oo • r—< O i-» U m o & ^-J cm" . vO U CM CO Q

ON

.-h as

<u

a i-H3

T3

u-i CM VO

00c

»"3 o

CO

i-<

r-. CM !c

CDCO t—

O ( w e3° in W r\l 2w 1oo OCM iTl

00 COW CM r- VO O o <-l • * <r OO -*

rt +j 3

U"l CM VO OO CO cr.

w

.-I CO CO CO

CM

ON

CM o X O 1 1

JS o >• o

rt <-t CO

00 CT\ 00 CM CM o\

1—1

0.

u

v • • 2 3 X VO CO i-4 IT> CM -* o h <j CO r~- r^. CM CM VO CO

4-> CM CM CO CO 1 vO z W I 1 1 1 1 Q3 1 1w

oo « 3 o HJ VH

n) CM -ci- <f sf 00 o > 3 45 r-- in r-~ vO CT> CM

H-1

bo CM CO CM •* * vO s h • » k • u U CJ m CO CO vO CO r-~ w c > vO CM oo O CO r^ DC H

CM CO CM

m 00 CT.

U 01 a. a, o

43

436

to

O

Cto CO

O

u§ u ° 1 o u

CO CO ca CO W

nj I-I <>

II S

.-h

II

a 4j

C <u e w fi o 4J •\ UW

(0 a

w 0>oc

id

en

M

.5* i-h

II

en u

00

•a

01

J-l CD

4-1 m

W

CO cm

CO

VM

43CO

DC

R)

ai 4J

CD 44

4J

(0

oi 44

— CO >

ca 6

44

CO

T3

CO >-> CO 01 3

CO

U IS

N • O 1-1 •H

ni 3 •a •H ID

a

U £

44 43

C o o u to u a •H CM 2 •-s |H m «

00

(4 CM CM CM M

CM

l-l

GO• H

•^v -*

C c D

i-H 43

a) H

+co s

CO

CO o OT-l co

CO

CM

COCM

ffl N^ CO CN

H l-l 2

43 43 43 43 43 43

Ph Ph FM Ph Ph Ph

25
B- 28

n ^ m \o r^ o 00 00 OS <t 00 r-- 1—

VO oo os CO Os CM VO o vO Os OS

a. • • • in o 6

CM CM -* r-~ vO oI—

cnmm vO

vOOS

i-l OJ

<u

X

>-.

v + "»^ O vO in en CM sf en o m in 3>-> o

to

O

u i—

i-i

VO

vO

en

CM00

st

vO

00St

00m

OS

001

OSmOS

CM

vO

oo

oo

vOvO o

-ISt

8P i/S rvj o

os

CM

in

.—

en

f—

r-* m

sfOsO

cnO

m

in

in o

SO

OS

en

CM

CM

vOCM

St

m

vOo

oo tf

OO i—

CM CM CM CM CM en CM > os o

CO

au o O »—i CM

m o

en vO

in

00 vO OSCM

*-" U-l

O st

m f-t en CM o m CM 00 CM o 3

CM 00 i rd .-I r- so ^-i oo 00 OS CM o .—

i .—i—

CM CM i-4 SO i—

u i i l l I

"o

•ac 6

rt ^ St CM OS

O

O St r~- VO > rd Os m CO OS o 00 a- in oo vO r~- CM 00 vO St a u O O

CO CM

CCo m

00 vO 00OS vO i—

st00

ooO 3

OS

OS o O

St

CM

i- ^J i—

CO OS r^ r^ vO i-i i 1—

i—

en CM CM i-4 c

1-1 r^ 1 i i 1 1 Wc

t—

•£ 00 St <t en vO Os t-t cn

rt oo *; CM vr> vt vO OJ CM OS o r-- >* r^ ogpa i oO o CO

en CM <to

OS ovO

O OS

in OSo

CMO

i—

O vOo O

i—

on OS r^

in

.—i r-l1 cni CMl I-I

*H

id -a- oo 00 CM 00 o Os >

co- in

I—1 CM o Os o O Os OS St

"3 £ T-t CM 1—

O CM CM en .-l en g .2? oo vO 00 00 vO VO CM 00 00

tv

u <u o T-l so CM en OS in I-I cn

Cw

(0 ° £

f-l CM CM <t

m vO

mi—

r-l i—

X£

HI

U

OrU

rd o o 00 00 00 60 00H 00 00 00 O* 00 o O OO o" 00 00

a

T3

w

B as IB

C

rt>a

rt X c cW

00CM oc

10 XI3 o

COVCXc

rd

(TJ £

ell

i-H

11e

41mu

0)

•a

(A

IIB

<D

<d

01

•o

to 1 + - 1 CM C" p^ 3 t I - CM CV O o O en

<t) + T - CM o o o CM CS st 5C as H

pa pa pa pa pa pa pa pa pa pa pa pa pa pa pa

26
HB(OH) 2 28 co4-» 60a

•f-i Aisn) o CM CO on <t ON °a "o

vo I—1i—1 O ON o o E

CO vO CO CM CM o

i—i

CO CM

m -d 1-1

m

vo X)

on

i—i o

<t -cl- <f

coo

CMON o

CM <f

in

CO

i-i oCO vO in CT\ <t

m CM <f ON CM r^ 3

CM in CO -d- vo <f co i-H in

>-|

O

°p?1

in

CM in

CO

I-l co

-4

CMvo

vo

CM CO

VO CO

r~ on

-d- mm

coM CM r- CO vo in CM

>- ON OCM U1

•r4 tS i—* O 00* a o

CM i-l co vo

n-l 3

CO o o

CO o

i-4

oo

i-4

ON VO in i-i

0>

CM

in

CM r-4 -dm CM CM CM -d -cl- -d- m h~ r-^ CO vo CM

i—l i-i i—l r-4 I 1

XI

nj ,6

,—

i—1 o in -d- i^ CO CM > rt. m in O oo CM in in r^ -d vo oo m i—i CO m CO

Qu 2 ^ r-l co vO

m o t~- "^ -d- CO CM

O r-~. CM on CO vf

M

1-4 i-H i-4 1-4 CM i—1 CM 1-4 o\ 00 CO co 1 i—l 1—1 1-4 1-4

C 1 1 1 1 W

vO vo Ov

4j o

ON CM o as vo oo £ o

oo

4-1 3

CMCMVO

CO

-d- vo O CO CO

Ih

B

1-4 .-1 CM 1 r-4 CO

1-4 fe pa

rt CT\ 00 r^ r^ r- hi vO 00 CO r^ > 'B £

CM ON co vo CM in i—l

r^ -d- CO or -d- vO CM CM -d- •d- CM i—i co CO ^ E .2? co VO CO I-l 1-1 on CM co oo co h <U <f 1-^ CO CO m -d CM CO ov in ^ i-H CM in VO vo r^ CM <f CM -d-

(0

i-l

X> 4) ,Q vT DV

rt cr 60 60 o t4 60 •H 60 i-4 60

O 60 o yu 60 60 60 CO

nj i—1

i-l i—1

i-l c

nJ II

>> CM a X

rg

CD

4-1 td

W

01ua

rt

to X>

uD

i-i

4-1 to

T3

4J

to o

1-1 to CJ CM u ^3

T3

u .-) t4 e

to PC c o

J-l

m •H .e

Rl in oi o

1—1o uo

a! c i-i o ^c 3

13 rO c 4-1

4-1 e 3 o (J E

to •H

O e o

*^x »H CM

v—

CO fc CM

-d- CM

<D

O i—l

O i-4 PC PC 1 vO i-l o> 1-4 i—l

PC CM o o 3 -d pc PC PC PC PC o o pa v—^

n) PC CM -d- um vo 1-4 pa CM pa

pa pa pa pa pa pa pa PC PC PC

27
H3 B03 28

U

in o

"o -<r p. u £

ON

m

NO

br ON

.-1

O

cn

H3

co

u

CM

t—

oo

00

m

-tf

•->

U

CM en CM 1

in

co tt

>- ON OCM 9in u

fd 00

a. o u

fNJ

O NO in

NO

m NO 00 r- oo i-i 3

.—i—m CM NO f—

o

0-»

cn en r-~

m f—

~tf

m <J CM CM CM CM in NO NO

X

"o T3C £

rO "^ in ao

in ON

m en CM i-l t-l

O

O to > (4 in vo CM en to cn en co en en CM

o- ,, , u

hi s .* .-i r-~ NO NO vO NO NO NO nO no i—

ON <f

g no co

m

mm

mm inmm CM 00 <t CM CM CM CM CM CM CM CM CM CM CO CM m c i i i 1 i 1 1 1 1 1 I l Wc

CM

rt oo tt

f—

CO £ 2o

4-1 i o 00

M C£

m

O CM U< CQ 1

**-»

fl) f—

in ON r*- r-l CO 00 r-. >h

CO

O ON r-~m CO r-~

m 3 X co -* to 00 m m <» m E .? 00 00 oo NO -* •tf CM CM

1* 0) 1—

00 -*O co t-i NO r-~

C £ NO r~ ON ON 00 cn in in W

ao

»-l i-i i—

r-l

ja 0/ £:

rt

O 00 cr cr cr cr cr 60 00 cr cr 6 </} « to to to CO CO to C i-i

rt

II ^a E

(TJ •* £ c

cv

4-1 c a U U

(Jc

4-> a.

4-3

T-l .-! I-I r-l r-l o

CO

4-1 CO o o o o o o o

IIB IB

IIB

IIe B

J3

V CM CM CM CM CM CM CM 3 .« x x X X X X X «\ i -\ ^ ** W V

CD 01 cu <u 0) o o o o o o o 4-1 4-1 4-> 4-1 4-1 T2 NO o o o o o o n) CO CO id CO C -rJ t—

cm

mO o o 4-» 4-1 4J 4J 4J

rd co

•\ •* *sm to 1 TM 10 CO

tt) "9

-I

m o CN

1-1 i—

T3 TJ ° M -o -o c c 4J 4-1 4J 4-J £ 3 •H CQ 01 CM m to 0) h

CO CO

N—' CM

O

00 In

O pa CM 1 CM X f

cn

•St CO /—

1 r^

4) co /s CO to /—

CM r^ o >—

O X O o X o O <t

.£> PQ o oa pa

O pa <* pa

rt en

N—

CM CM pa EC pa CM

H

x CQ

X

X

w

v-'

X

X

28
BC1

28

W2wwi wW>—i H

PiWoo2QO

OSwIH

<!UwXoowu

S3

«!>QWHUWw

u

i^~ vO o in

_ 1—I o O o>

P. o £

r^ CM oo

p--

T-l—i

in

vo X) on

1-4 CJ\ oo

1—1

l»» ro oo

!-H] o

CO

rtu r-~

O in tom o O 3 <t vo CM <t I*. <f in

>->

U

°o? in oo £

oo

CM r^ 00 i-i i "*"" O r-~ o r-4 oo w CM CM <t CM

>> ocm oin

•rH

X f—

o

oo' i (X o o

rt U o3

tM

oomt-- CTv m

mo

r-4 00 ooCM

(4

0)

coi CM CM inCO

en

00

CMCOCO

co s "o 1 C

a!>-

j:

rt CM

m o- <f -* CM

m r^ ON o m CO1

0-u

a

u

o\ i—i

VD o VO -*

m 00m ov o m CO vo CO in <1 CO CM f» o\ 00 r^ <f o- vO r^ vf VO VO 00 r~- m 1 CM CN CM co co r-4 in CO CM CM CO CO <) r-^

C 1 1 1 i 1 i l 1 1 1 i wc

CM

"Xj

M

co 00 00 oo

4-1 ON o •* o 5 o er. CM

I—1

co inCO

Pd i CN CO

h o

pa 1

rt <J- CM vO vO 00 <f vO i-l CM in vO

m o CM

>.

»-H *-» ON VO <) in 00 vO CM <C

m CM COm vO CM <r

&p

D

X

O

O o i—i o CM r-l CM r-l CM r-4 <f CO CO VO

u £ .5? 00 00 00 VO 00 <f 00 00 00 00 00 <t <!- * CM

(h <U OS r-. VO r-~

m r-» I~~ COm CM <) 1-4 CTi co VO ^ CM vO 00 ON -* co 00 VD vo 00 00 o r-4 r~- <!

W

03

r-4 1-H i—l 1-4

-O 4) -O 4-1 60 00

Ww 60 60 60

w 60 60 a* cr 60 60 cr 60

a

w « rt rt rt

an

C

rt>-a • «v

.-c

CM

O o bT

CO o m

SB

1—1

CM

u p. CJ I-H » !-< r-i i-i c

II 00

rt

u <D IIm II II ii

u

CO

C CN X 8 + E 6 B 3 P c ^ s g

•s •s •s

w 0) 0) 0) a) <D 01 X< o XI U 4-1 4-1 4-1 4-1 CM o 0) CfJ r-» « w ei c PS u 4-1 4-1 VO 4-1 4-1 4-1 rt o

4-1 CO CO «*

CO CO CO

rt

m

C • i-l 'a T) TJ o 13 X) c G 4J 4J C 4J 4-1 4-1 £

1-1 •H CO CO T-t CO 10 0) ^N M

«* I 00

CM

b 1 CM

CM s P- CM X o

CO CN

X 1 X CM CO

<D ^N /-^ CM o X PH Ph o 1—1 1 vt PH <f X Ph N-* o co co •tf Xi en -tf Ph t* O PH o a CM C" O O Ph i—l m P-i Ph Ph CM o pa pa N-^ o Ph Ph CO CO co C_> H pa pa pa CO pa *^ X pa pa pa pa pa pa pa pa

29
BC1,

28 ' Ww

inWwo

0,(J

<cz

>-QO

erf WX

t-<Uwuoww

E>J>QW

i-> UWJw

u3

flj VU3

•-*. «

00

rt CM Co 1) +» J3

(ti rt £ H I

0\ ©cm uc

in3

CO

'J

00C3 X E

.2>

U 1) £ncO

co o

in o O Hm o

oo

St CM VO I—) CnJ 00 St

en

O co o m o m o 00

vO ov

m o <* vo t-i CM CO

CI r>. o CTi co CM r-. r^ in

CM vo o> r-« CM st o o C

to 00 St i—

m 00 o CTV LO

00 00 00

O •_l CM

CM

U

O

•- o z m u

m

3= vo

CM oz

vO

CO st o .-i ^^ CM o i-i i-i 33 33 CM p^

1-1 o o co co 1* CM c o o o O O t-l i-l >-i M o pa pa CO co O U pa pa

cq ^^

v

— pa pa pa pa pa pa

30
NH,

28

B3 H7 U o on ON ON oo CM 00 t—1

-d- p. "o sf OO CO r-» ON !-) r^ o . o s

ro 4t

m in vo h- <f r-- o t—i

t-l I—1

i—i

t—l

m

in

0J

41 vo 13

on CM vO VO o CO ITl -* r-i CO

"rt <f o t-1 ON «tf vO

m r-. VO o

>N

,—1

00

u oo tf •sf VO en I—1

CO o ON 00 3

VD r~ r^ r~ oo in

m CO vo

•->

U

°n? ID

-cl- vo r-. ON -dm 00 vO r^

cm in 00 r- o CM oo CM r— CM *"" o en <t- vO o o VO O r^ oo « co co CO CO <f CM o CM vo

>- OCM LTI

•rH

W <—< O

(tj CO

D- o

n) CM vO CM r- u o

U-l ON o VO oo , . 3

<r ON * vO

c\i vO

m *

a; i 1—1 X "o

rt ^n o <f in

>- o o rm oo r^

a.

u

p3 X. p» i-i ON vO r-» vo 4 o -d- vO

u <J t—1

00 CM co

m t-i 66 vO

m -ct i •jf 1 i—i 1 cwco g

00

4-1 3 o 00 i-H o1-1 o -cl- ^ pi t-l CO vO in o 1 i—i h PQ

"o

rt 00 <* CM 00 r- <f <r > 3 5 £ .5?

vo h» vO CM <f

m On

O st CO r-- r^ ON

or T-l CM CM 00 CM l-s CO in i—i

vO r-i

O t-i

rH (~~ vO vO

O u-| 00 On r-~ oo 00 00 p»

m

4)CW

03

m a; £

00 on t-l VO t-l CM •* in i"-

m <f 00 VO

CM 00 VO

O ON <t l-~ 00 t-l f> CM in

m i—1

t-i t-l CM CO tH r-i

£> ai £>

«t 60 00 60 60 60 60 60 60

O 60 o O 60 o o 60

a

w

C

Hi>.a

a! c 1-1 C c w

01uc .& o

41

u

OS 13

IS

10 t-l

uo

4) a) & P co U

(3rt

60

a)

a

4-1

U R) td 4J H t-i

rt d> c

4-1 ^5 o

oa

•HU

4-1 0) ^v h

VO vO

PSCM 00 h

CM

U CM co

to

PQCM

W

co

4) CM CM PQ

M PQ /—\

PQ 3

Pn

u CM CO CM CO CO

U PQ T-l T-l CO CM 00 00 «* co

rt PQ fn

U

u l-l 00 00 CM CM fe 53 ji*

H PQ PQ PQ PQ PQ pa pq PQ PQ 00 PQ

N

— ^

31
B 3 N3 H6 28

U

3

IT) 4)h

1 «~N CQ

r~

"rt

00

CM co ill

• fH +» XI

(ti 0) z H

5

OO

VH

J33

03

3 J= E

.5°

id

P

cSm

E

o

sr

CO

00

o

CMVO

3

c 3

00 o 00 vO CM Ov CM r^ vO vO St o m CO CM 1-^ CO CO 00 CJv vO o o vO

00 00 r~- St vO 00 in >-l

St CO .-1 CM in 1—1 o f—

1

oo 00 St o o-\ o (-- u-i

o&

o

u

o xo

o

O CM

CM X X <t

r#« 00 c CO CO o b

o O in pa

pa pa pa <t St St c g

3= !z 5

3

u

X o CO

CM pa r-1 pa CO O CM X CO pa Pu co pa i-i • co X co o CO c Pi i-H (U Pb o X u u

X pa CM P-. P-, p-l pa en

32
(CH3 ) 2 0. BF3 28

coWw

co

coaH

PiW

OhO

PL, uQO

b5wH

<!uSwXuO

coW>pwHUWW

to

U

CM

m

m 1-1 i—i ON o vO i—i vO CM o 00

p. • • O £

CM i—ir» <f 1—1

in

1—1 CM in i—l CM •* in

0/ voav X)

i-i »—i

cd

oo

i—i

CM ^o

m <f 00 ^ •

i-l on o vo r—m

O -* OV r~- |-~ r~- CM VO CM 3 m r^ 00 o in m I~~. VO CJV m CTv

•")

U

1—1 i—i 1

(Nl co

co CO

oo

CMO o

ONo

vo

CO

m

00M i-i CO CO CO <f i—i >- o\ I—1

i-i

T

in o

rd 00

a. o

cd IM o u VH3

r~- r-~.

vOooCM

CM

OOCOCM

CM

CMCO

CMCO o

00 o

r-^

00

OJ

i-i i CM i—i i—l r^ i^ i—i o\ i 1 i—i i—l i-i i-i CM I

X)c ^£_ Ov oi 00

>. o

nl CM r-~

m r^- in vO

m i-~.m CM

O 00 -J ov

m

a o o ffi X r~- <f o\ <f

m vo l-~ VO <f 00 CO

m

O o O 00 00 ^ <3 i-H co CM CO CO Vf CO CM -d- CO CM i—i m •tf CO CO CM I i i i 1 l i—i i-i CM CM CM CM 1 co co c i 1 1 1 1 i i W

VO

ni oo

M

00co

m

mo £ o o i—l vo CO CM in

Ih Pi oo i-i CM <r CM o i-H 1 1 1 h

co

n) CM CM CM * in o> 5

oo CM r-~ >- 3 2

cnm VO r-~-m r~-

m OV

m

or CO io i-l ov -cj- 00 i-l Ov

O r~

m 6 .2? VO CM Cv o> CO 00 CTV Ov -* oo u <0 co in in r-^ i-i CO CO m i—l CO ^ co in m CT\ <f r~- o <t O i—i W

DO

»H i-i i—l i—i

,Q OJ ,D

-*-1 w cr ow

w cr

cd 60

O 1-1 60 i-i CO 60 T4 60 1-1 60 i-i 60 60 t4 60 3 CO

T-l .-1 i-l 1-1 i—i i-t

C

rt>^a

cd ,c c cw oc

cd

4-> in

uu c

COc C

cd

01a

OJ

(3

01 CO cd

u

u id cd 43 <u u u o o i-i U 3 p o o Xi ja o O

to VO CM x> 42

U

>•, £> x< XJc

i-l o >, >1

X t^ >v

SB 55

XX o o XX

r—

m o o 45 4= o o

n)

O

X .e £ 4-1 4J Xi X.

cd l vo

M 4-1 11) 9J 4-1 4-1

C

O 9J si E e OJ 0) 3 e e •H i-i i-l 1-1 c 1-1 •H P p Sj M

1-1 XI XI 4-1 4-1 4-1 4J vO

s-*. P3 00 CM CO v^ pa Pn oo CM CO CM pa CM

co

COm

co

COco

m

pa

OCM 6CM

<u CO

w

O o W CM *^N s-^ 3

EC CM

O o o t> CO CO

UO o U CO o o X BB

cd CM ** v—

s^

W

w v-^ ^*-^

uO

H pa pa pa pa pa pa pa pa ^^ 1
(C2 H5 ) 2 O.BF3 28

QO

aiWXHJ<UwohowU<>QWHUWw

CO

U

oo o

P.

m

u £ o

CO

U1

nO

as On XI

r-J o "rt t O NO r^ no

m_ 3 CO u m 00 m no -* f^ CM CM

•-)

U

m r-. r-~ on <! r- in oo e3° in

CM

oo

K

m

>.

O-v OCM in

H

X ^-* o

rd 00 a o

rt rg in U IM

S3

oo

m

i-i

no in

.-1

m

oo oo

NO o O <f

ON <f

m

—1 -I CM r-l »—

O) ' ' X O

-o E

IT) ^7 00 NO > o

«i co 00 CM CM

m r-i CM NO o i~- NO oo

m CM

O CO ON r-l

a

u o

•p ^ J- co VO 00 r-~ on 00 in no o o o o CM -tf o r^ o-

%4 ^ m j' 00 r^

m <f noO ON CM r-1 <t CO CO CO CM nom

co co CM i-H 1 1 1 1 1 1 1 i c 1 ' 1 i 1 i c

n! oo

M

mCM £ § o -I

>- Pi ^J -I O i h P3

rt ON ON NO 10 CM

O CM co oo > "3 2

ON CM 00 oo r~- ON en CM NO

Of CM co r~ vO oo NO CM ON -tf u £ .5? ON en r^ to CO On o oo ON c

i- i/

M 00 nO in NO in £<f CN £* <r O CM ON en r-~ s* r-

-« i—i

r-l t—ii-i —I

/^

u

,a

•— cr cr D* D* cr cr cr

n] i-l 00 «r4 00 r-l 60 •H t-I 60 •H 60 •H 60 o O 60 CJ 60 6

T3

to

r-H r-< i—( 1-1

—i

»—* i—l

C

rt>a

rt T]

C (11 <u c C c W

0)uc

4-1 rto

rto •"-1 x Xi

*-'

(T) s- o o y u u (A CO o o

XI (D 1—1 3 c xu X

>N o o

rt

Jx

<i

4-1 4-1 0) a) E e e

t-i •h

•o •o

*~s ^ co CO cn o\ fe CM i—i

r-i co PS CO CO N^ pa T—1

i—l o o w pa ca PC 00 u O pa CM pa CO pa z

CM o pa •—* **"N • CO PC CM CM in i—i m 00 CM o 2= pa

y-^ r~> PC o PC CM /^ CM CO CO

0) in o CM o CM /-^

m PC •—

/-^ 3 PC ci f_> o U CO PC fe CO CO

CM PC o en o PC CM CO

x PC

rt c_> C_> 35 o O PC o O H Vw' v"~' pa O pa v N"^ CQ •--• ^

34
BF3 . P(CH 3 ) 3 28

Uco

*-»0X1 c

XIo

COW2w

coWMHwo

a,u2

:*Qo

PiwHUwuo

COw

<!>QWHUww

CO

ct)

rd X)C

rtj 3v3

ffl i-H

rtj CO o

ctj Ua

CD X

XIc

rd>-(XOuCWco

rdgMOh

Mi

4)Cw

en

.Q6

X)c

cd

>*. ai—i

td W

,0

rd H i

ON OCM

OS3

CO

U

r\J

00

rdU o

033 ,G £ .5? u o

=5

<u

a)

<P

X)c

rdO

CM

CO

CO

on

00

00

CO

CN <f

in 00 -* 1^ ON ON o ^o CN m

uo

00

00

oo

a)UO

XI

0)e

CO

i-lOc m

PSo nX n o

Fn *^ « m

ffl oo S3

la *^*\

O

CO CO CN

•"N

W « n o u

S3 o o U ^^ ^^ ECO

35
(CH 3

) 3 As- B(CH3 ) 3 -PbO 2B2 3 28

U

c H

60 H

c 3

>-> X.

U)n)

t—t £

UiW

2

w

i

>-

en m W

a

H U

BJ *j W id O

OS -ac

Du n!>.a

o

u

cW

co

E §

o g

3

n)

0)

Fh ^«\ 3 i-i CQ

i-i

i-H co

«) CM e V

*-* ,£>

cS

IT) £ H

u

c

<«

3

U

£

u

4) c

C

rd

O

en vo in

00 60 00 o o

E E

_a a_

>, :*

^-^ cd <d cn t—

«-< 33 00 60 cn

pa co

CO <in <cn o

c

en cn CM

pa paCM cn cn CM u • B X i-i •H T-( o o o u r/l CO w .o x v-^ —

pa pa pa Pm p-,

36
A1-(A10) 2 29

COW

W

CO

LOWi—

i

H

PiW

&

O

p5(XU

P

O

eiW

H

<JU

w

K

U

Ow

W

<;>

Q

W

H

U

W

w

to

U

Q

co

+>boC

•r-* ,13

IDa

h M

6

C

rt>•ft

cW

3

n)V

Mi s-\

ffl

,_, ON

nl cm C

<t> •»H

4-1 £:

n) a 2 H

CO

O

ox

ci i—

i

+-> 3 X.

I- <u O £

ni CO

u

enID P

c

n)

O

oI—

I

CM

in vo oo coO

oo

ro

O

00 O

eno ONo

<t r-^ VO o i-i St <f VO 1-^ t--

r-~ m o\ m CM r^ <-t «.+ o r~- CM VO co

t-i O

OV CM CM Cv in 00

t-l t—I Ov VO 00 l"» o F-l <f m

o ov CO <f 00

CO o o CM .-1 VO 00 00 vO vO Ov ON on OV CJN CO CM oo ON in m * ITl VO oo

00 60 00 60 6060606060606060 60 W

, + +

f- CM CO

i-l t-l .-I «U <; <l

+ + + + m vo r^ + + O

00 Ov

t-1 t-l ,-1 t—

I

< < < <

CM O t-l i-l < <

O ci-i i-i <c <

o

37
A12 3 29

U

o~ r^ CM ON CM CO in

A '—

oo CO CM <f

O NO ON

a • • o E

oo r-

in <r I-- r^ r^

H CO CM <f r-<

nNO

c/

f-l T3

l*- in NO t-i oo NO 00

i-l3 o

CO 15u CM

i—

CO

oo

m

CO

00

oo

co

i-i

00m

I-)

a

CM .—1 CO <f CM in i-i

°p°1

U0

<N1 -3- t-i NOCM

oo

oo tt

CO o r-l i-^

>N ON e CM CM CM CM org iTi

.,_. SB i-H u

00

a a*

ri fM O U-i CM CO r-- in

CM ON CM oo NO

0) 3

oo i-~ vO o nO in in

O r-~ CM

O r-- on co -tf <f m NO r-< NO ON -*

en <r> -d- -*

m r-i CO 1 r-l CO I

"o i i 1 1 i 1 1 1 13C E

n! ^,

>«

_ n! NO

a l+J

u in o in •—* ON CM P~

m

r-l 1 X

O oo i-i

m

O CM 00 CMO i—

1—1 in NO r-l NO ON o on on ON ON r^ l-~ f—

f-l NO 1—

O in NO NO in c

<t co co CO CO -* <f NO NO 1 co CO 1 CM CO

Wc i > 1 1 l 1 1 i i 1 i £ oo

ON 00 CM

njE S

OO

14-1 S3

m

CM

NO

r-l

O

00

u on NO NO

m

V CO 1 CO

h

J i i

"o

cfl CM

m CMm «tf ON vO o ON r^ >

•—' *-* i—

vo r~- on in oo co I—

ON vO

OJ 3 .x: vD r- o 00

O ooO 1—1 r~. r^

rH E .5? On on o ON

O ONO o ON on c

I*

V i—1 ON NO i-- o CO 00

mm CO 5 o •-I m CM CM <f r^ ON <!• 00

U

ga

1—

•-I

—t

X)

D

a P.

.Q 4rJ

u

u

rt t_)

O

O

O o (J tj o 00O cr o a- 60 cr o* o

(/>

to e a) « tO c

rt>a

n) X

C cW <uuc

a)

(0

a.

r-O

[04) P

t-i

IIe

i-4

II

r-4

II

1-1

II

w

p 41 <D 41 «r

-cc

"2 4-1 4-1 4-1 4-1 c a) <u <u cO CO a) <d s

4J

u 4-1 4-1 4-1 4-1 4-1 4-1 rt 1-4 o •H T4 0) 0] to to d o e a. to 1-1 o ,e <0 .O HI • 3E V a) X> {n o -o •d •a

«\ o •H i-l a) 4J 4-1 4-1 4J

ci co > .o •o 00 fi 0) t» to to *~\ i- eg o

on fc< o CM

CNI CM

5C CO +

•*

V CO CO CO CM

x PC + + 3 o O O CO EC o o CM cv CO

CM CM CM PS PC

O N^X ^^ pt. rZ4 rb |xi n) i—

i-l

—

1-1 1-4 r-( r-4 1-1 i-l 1-4 1-1 r-4

H < < < < < < < < < <: < < 1

38
A1C13 29

W

2

w

toWI—

(

H

W

ftO

oi&

UI—

i

<

Qo

wH

<!u

w

ow

w

p>

P

wH

U

w

w

to

U

u

rdft O

cu s

C

rt>.a

o

VhcW

fi

3

rtV

u

3 •—

s

CQ CO

,_, O

rt CM C

CD -^ rd

rti rd 2 H

°p?

CO

CD " XI

"(3u

U

«

rd ' u

rd

g .?

>h cd ° ^

XIc

rd

o

CO

vO

o

CM co co

r-» ro vO m cm

OO VO vO vO O

in in in co

CM CM CM CM <f <r

CM CM

•4

covO

Ov <r CO 00 in m m

i—

1

CO cy> in -* r^ o

r-» m r^ CTi en CO <t

CT\ a> av av <f CO CO o r^ r-i CO CM r^ en

<f vo VD <t vO as CO

w cr ET w

<fl nj cd nt H

II i-i e

II

CD 6

4-) CO

4-> OJ CO

rr a* cr tr cr cr cr

a) «J a CO a) CO CO

XI en o

cu c N #« HI H T)

rJ 01 o

N m •i-i

i <r c o

oo

o

00+

fa

PCo

ooo

CM CM CM CM CM CM CM

fi |H PC PC PC PC PC

(11 4-1 cd O

o

o o

o

o

o

oo

o

o

o o

o

o o

o

o

o

oo

CO 1—1 en m or-l o

co o

m

o

o

fa

) VO fa vo fa fa r-l 1-1 fa CM O <1 U

r-l r-l r-l CO i—

l

< <d <C PC <

39
A1C13

29

u ° P, "o U £

in

vO

ON a

i—

E>

>-)

o

CO

"rtu in r~- -I

U

1

in

oo tt ^

on OCM

3= in u

00 a o^

ft (VJ u vh o r~

rt 3 i ON

a> s CM DC "o

i 1

-ac £

rt ^

, > <i r~ 3

00 r-~ m ov CM VO 00 en r» m CO vO O CM

a. U-l u m o m o ON m l"N 00 .-1 en 00 CO in CO O m ro in

M s ^ vO m m en CM 1-4 O ON vO vO m en CM i-i o O in en oo

^J

>S- -3- <t -* -* <t -3- en -3 «tf -* <f -3- -* -* St VD •<»• o

c

CM CM CM CM CM CM CM CM CM CM CM CM CM CM CM CM i-i vO m

W

c

i 1

o

rt£

u

2

OO

<4-l X

s

| o

h 3< m O

>

h

JS * CM i-i 3 £ CO 00 £ .5? <t vO a I* 0) f-4 vO c £ <t vO W

01

CM CM

-O A) -O

rt cr cr or cr or O* o* cr cr o- O" cr C D* O* cr o 60 3 W

o « « <o Cd « a <B a) « (0 <a « a a a)

C -I n

ll >a

O o O O O O o o O o o o o o o o

CM IN CM CM CM CM CM CM CM CM CM CM CM CM CM CN CM

rt PC X PC PS PC X X pa EC EC EC EC PC PC EC PC X X c O o o O o o o o O O O o o o o o ^ c

CO en en en en en en en O o o o o o o o <u CM CM CM CM CM CM CM CM vO \o vO VO vO vO vO VO 4-1 u u '^ CO u

c a + + + + + + + + + + + + + + + + 4-1 (A

rt h r-4 i-i i—

i—

i—* i-l i—

1—

i—

1—1 —I i-l i-l i-l i-( 1—1

*-» CJ o c_> cj r_> o CJ O o u o c_> o o CJ o

go CO PC a: = X X PS 3d X EC EC EC EC EC 3= PC PC o

X> 0; u

3 c m <0 10 oo CM

.-i CM -* In. I-l in in ON ON m o ON ON Sf oo en d -d- t-^. -tf oo en o r^ <r O o 1-1 i—l CM en en <t <t c

rt o o I—

CM o- m in vO i-l o- 00 vO o- 00 CM vO 1-4 o o CM <f oo CM <r vO 00 o in o i-l CM r^ en oo

ti .-1 i—

i—i i-i 1-1 CM en en <t <t CO c C

y—v £

T-l t4 <* u N_^

0*V o O

CM fc CM

ECvO

vO

0) en en i-H

T-t i—

CJ 3 cj o CM

rt I-l i-i .-1 H < < <

40
AH3 29

coWw

10

COWHH

<*W&O

Pi

PhuQOwH

<JUw

&4Owwp<>puHOww

in

UcoMC

rt £C

co3

id«M3

PQ<—

rtco

r-l

n)

U

oja

a) U

rt

4>

T>C

tiaocWcoo

>-

Ml

0)CW3

X)c

_aHx-4-> CW

rt H

0)uc

rt

to

CO

rt3 X

r.. !>

01

COuwPcao om co o

00

co

mm a-> in

CM CM CM

l~~ ©

CO

m in O 00 ON o

oo Is- VO ^o o vO

I-l CM o o> f~. r~ m <t

.-i 00

O

<f 00 ^D n CO I-~ co m O

in t-H -JT

rt

0)c

r-H a) ID 3

II o C

ai o H o

CM

EC c

4-1

*s CM 0) »#i 01

4-1

W

m

u

xi

C

ffl o 00 PQ

M •*

U

•U o £ m

h

m VO i OT o P3 co P3 m w «v w CM K CM vO \ CO X o u CJ CJ u

<d <! <c <d

41
29

u

00 o o

ON o oo CN

a. • o £

r- CNNO

r^ r--.

m

NO

0/

1-1

on T) i—

o> CN

>n

B "id

O CN <r r-l oo

i-H3

>-> CO o in r--- on CN <r m in en i—

i—1-1

U

5PI

in

no cn in

CN

00 tt

r-i on

>. on o CN o

ocsi ir o

id 00 a O^

<d r\) 00

m CM

O 00 ON 00 NO

t« 3

in

en

O

>*

NONO 3

00

NO

4) h> t^ i—

X "o ' 1 i—

0c £

id .5 > id Ovl 00 en o

"4-4 o in o en cn in t—

CJN NO -tf ^ r-l o 3 ^ en 00 en cn cn vO cjn CN CN en CN o en m 00 NO

in CN %J r^ CN

O o nO CN i—

m 00 ^i- o en r~ t^

C

r-l r-

oo o-n ON CN i—

CN CN i—

r-l I—I r-i i 1 1 CN | 1 1 1 i wc 1

"- o Eu g

0©

lw

a 00

M 5 O 00 ot-.

hJ<:

<d -d- in o co oo On ON en 8

<t NO CN >

atu

CT>mm r-~ on en i—

cn 00 -cl- en en 00 3 £ 00 -cr in <f en CN r— O CN 00 in <t vO 00 £ .5? tn o i—

r-i CN -cr en <T <f r~ 00 00 r~ ON o k, a; in ON o CN O nO in r-~ r- O m o nO o c 5

,—i in in ~J in nO NO ON nOO r-- cjn cn <f

W

ID

00 "' cn <r nO •—i 1-1 1-1 en <r CN -cr

X l -=

id BO 00 o o cr cr CJ o o o o u CJ o o o

•S) a) CO c

rd>a

<fl X c cU uC

R)

03 -C

u

co C

re

id£

IIB

<u

i-l CO u

CO

•o

i-l CO oCN o

CN

X. oo ^s t. nO .-i NO CN N—

Ui en en en

O CN CO CO CO ON /-> #—n ,^* CO O CN CN CN CN

<t

OO

-cr O

Jf CO PS

X ECCN en cn

<u vO en CO CO CO cn en en cn cu <u H CO N-^ r-l r-l r-l i-i cn CO H 3 CN CO CN CS1 CN CN o O U 03 r-l CN CN z

id i-l r-l r-l T-H i—

!—

r-l r—

t—

r-H i—

r-H T—l r-l

H < < <! < <: < < < <d < <C < < <

42
AlBr 3 - 6NH3

29

coWW

CO

cowMH

eiw

cuo

pi(XuPo

c^w

acH

<!uwuo

COw&>QWHUWw

CO

U

m

(X • • E

CO O- in ON vO

ON

6f I—l

T-l XI

t-l

U

(4 1—<

00

CM

co

1—i

1—1

—1 6P?1 m

C\]

00M

>• ocs en

.,-< to r—1 u

00

a

O

O VW

rvl

r--

d 3

vO

on VO

CM

QJ 1—1 m

DC

"o 1 a e

rt

r_, CM

>, n! CO CO vO

&-

O ON CM ON VO 00

O CM •* VO <f CO VO r^ CM

4->c s ,*

vO 1—1

1—1 r^ CM vO CO ON CO <f

m VO r~- CM VO CO ^j r^ l~s 00 ON i—l m 00 CO VO CO <!• 1—1 i~» m t—l

<f

CM CM vO 00 CM CM CM CO CO CO * in 1—1 CM CO CO 1 1 2

00

U-l ^ M ^J S t 3<

rt CM CM CO i—l 1—1 CO VO CM 00 r^-

O T-l CO VO CM

>.

1—1 4-> VO 00 * i—l CM CM co <r <f in on ON

O T-l CM

6jt u 3 nC ON 00 CO r^ CO CO ON CM in T-l VO CO

O VO ON B.21 ^ cu

ON 1—1 CO 00 <f <f in

m

O r^ h«. 00 00 00

(U CM i-H

m

O VO <f 00 in CM ON I-l CO r-» T-l 00 c £ r-l CM r^ m 00 00 T—1

CO in 00 r~- 00 i—1

in VO

w CM CO CO 1—1 i—l T-l CM CM CM CM co CM CO CO CO

J3 cv X rt

W CJ

a CJ CJ CJ

O CJ CJ CJ CJ CJ 6 CO

cd

C

rt>>a c OCM PC

a)c

i-l

in

COm • H <jcd !h

II *-* CO O +

CO

g

XI cu r-l 3 m, C_) CO <u EC T> cfl vO C 4-1 rt CO 1—1

ni vo

CO CO 3 4-1 c g

CO T4

OCM CM

1—1

VO

T-l CO ON

CM VO ON CO co CO CO

O CO CO CO

h CO CO CO

CO «*

j§

g jg

g

<f

0-

CO §

>—

Z Z CO in VO r-- Iz; 1—1 IS CO in VO

CO CO CO

u

O CO CO co co CO co CO CO CO co CO CO s z z I—l F-l T-l T-l T-l I—1

I—l T-l

uuu

u 3 *«> CJ O O O CQ PQ pq m

rd i—l r-J 1—1 T-l I-l T-4 1—1 I—1

T—1

I—l T-l 1—1 •-I 1-1 1—1 H < <: < < < < < <S <c «J! < < < < <

43
AlBr 3

* 7NH3 29

CN

P.

I-I

• o £ in

inno

0/

111 ON

i-i -o

>N

i-l3

->

c

CO

I"*u

f- CN

i-l o

in <f

1 o

1

lil

IN)

co X

>- on OCM in

>r4 IS **

CO* a

n) <VJ o o CN

It 3

r-~ i-i 00 ON

<f -J- I "o

1 1

C £

rt ^

> o a <T «* CM CM a. V t~~ in CM o on ON o\ NO ON o 00 CN CM NO 00 O

1

X

<t co p^ on in r- CM in <t o o CN CO i—

1—

I-l CM VJ no o 0\ f—

O 00 i—CO r^ in 00 NO ON ON ON ON o\ C

CO <r ~tf fH CM CM CO CO CO <f in m m m in m in w

c

I

oo

lw

55 o £ M

s

a) CO o o CO m oo <t o CM NO ON CO >

~-t *J CM -d- r- m VD r-~ 00 ON O CN NO CO 3 X CM CO CO CM CO <f r~- o 1^ ON o ^1- £ .5? ON ON "I

r^ f~ CO oo ON ON o CO i—

I) t- 01 1/1 ON m -a- 00 CN ON NO o ON oo l"» c ° £ CO 1—1 o CM in ON o CM VO CN <f CO W

a

ff\ <r in vt -* -* m in in NO l-~ CN

J2 Cu ,a

rt CJ u o CJ U CJ u u U CJ CJ CJ O

- cr cr cr V

6

•a

c/>

ecl cd CO a CO

c

nl>a

rt X c

CH

4)o

c

(0

a

>-. u

(0 P

I-l

IIe O o o o

3 CN CM CN CM W 01 X X X X

•p "0 cd o o o o

c •u o o o o

rt U) in o in o

rt I—

i-i CM

»—

-a 3 4J C

£

CO i-l

ON

CM

en CO ZON

CO

i-4 CO

CO

CO

CO

in

CO CO xZ

CO

ON

CO

CO

1—1

CO oCN

CM O

ca

N—S

0! co en CO I-l —I ij 1j 1-1 CO CO CO CO CO CO CO CO < .£> « pa pa M t-l i-i I-I i—

M M I-I -*

tfl T-l i-i i-i i~l I-I i—

I-I i-i i-l I—

I-I x H < < < < < < < < < < <: 5Z

44
A1(CH3 ) 3 29

(Aww

to

COWHWoo<z

><po

pjw

ac

E-i

<!ul-H W

DuUo

tOw<>QWHUww

en

U

r~- •-I ON o rH ro en CM in ON i-l a. • • • • o 6 n m CM o r^ r~- VO oo CM oo CM co

voON

CK

a) 73

i-H i-i CO

r-l ^ vO CMO1-^ ON

vo

CM

mo

>. rd • • • • • iH CO u vO <f i-l ON I-l o 3 VO vO CM CO CM m

i-i

O

r-l i—l CO 6P?I

in

00

CM

m00

vO

CO r-l co M m i-i ON i—l

>- ov

a co r-~ CO 00 OCM in m

»H

X 1—* U

00

(X o

rd O o

4-1

M i—l CM ro r~- ON ON ^

rt 3 o m CM CO VO CM 00 CM 00 VO <t l <u i-l tH CO 00 1 I oB

r-l CM CO

rd ^

>- cd - f-l

O <}• vO

n, CM <r

m CM r^ CO 00 <t- ON o o 00 ON vo r-~

<\^ CM CM CM

O 00 ON ON <t VO ON CO r-^ ON CM r~- on ON ON CM o in co r~- CO CO CM <r CO i-l

CW

IT>

m

m <f <f r-^ 1 <r i—i I—l <f i i I ' i i i—1 1 CM CM1 i ' 1 <t-

*J

w o m i—i vO

rd

g eo <f 00 r^ r-~

g

»*-i £ ffi

O i-i ^t CM oo ON

M s

i-i vO CM -tf CM o «* CO i-l i 1 h 3 1 i v*n <

rt <f o I-I CO ON CM CM -* i-i CO <f r-^ >

or

1-H -4-> r» 1-1 o m CM 00 VO 00 co

m ON vO 3 rC CM o I-I m m CO O 1-1 o 00 m 00 £ .9 CO en <f ON ON CO r-. I-l ON ON ON O

0) V. 4) PI vO

O r^ i—i r~. o ON I—l r-~ CO CM

C ^ in 00 CM

m CM vO o r~- o r- ~tf r^

W

0)

<f r^ ON i-H i—i CO CM

i-i I-l i—i

XI i> X

4J

Rj o* O" o* o o O o o o o 60 CJ

O i-l 60 3

T3

W 01

a a)

i—i

C

rd>>a

Bi X-*-» c W 1)oC

rd

(0 Xi3

fto

<P o

CM oCM oc\

OCM

O

CM

CU

i-l •H

ct) C

n)U

O w) to X X pa X X CM 4J VO ON <U * o O o • ,

4-1 oo

B o o o CO CO 1-1 i-i S

rd

m o inO o a i-l

m

•^ •t s o co CO •H ooC

CM CO CO CM -dm i-l /-v

O 9 X U <f g

(3 CM oo CO a) o E o

i-i I-l

OO Xi P-i cc) ••^ • CM CM *—

On CM CM i—l i-l

m v^-* *~N ^s < < i—i ON k «* <f CO CO co CO <: CM

CO oCO

OCM oCM

X

P-i

X

Ph CO

C^

HI .-I I—l ,—^-v <t CO CO ffi CM CO

X I—1 < < -* <r o !-» Vi § 01 O o o X «tf «* X Pj P-, u « N^-' <! CM <f vy

rd ffi

g i-< I-l I—l r-l VO i-i i—1

T-l !-<

H s z n^- N—/

<: < <c <!X < <: < <:

45
A12 (CH 3 ) 6 29

toW

fa

IT;

coWH

Pi

fa

fao

a;fau

<3z>ao

ai

faIH<UwIu

fao

cou

<:>pwHUww o £

cnen

ejv

OVO

Ov

en

ov

CMvO

CO

VO

00

00

CM Ov

CM CM CM

mm

m r^

in

0/

4) VO T3 Ov

i-l CO en CJV

F-H -3- CM

O CJVm vo i-i 00

>v

i-l3 o m CM

O CM co 00 r-~

O

CM

.—

CM CM CM <)• v* <f VD

U

3?1

in

INI VO

00Ocn00

CMVO

1—

oo

M

>< ov

O «tf cn <f OCM tO

tt4 3= ~^

oo

a o^

CO U

no

•v* CO 00 in vO

m en

4-> 9

CM

O r-^ cn 00 CM i-H

<fl I CM CM CM ON

O 1—

i) VO VO vo Ov 00 Ov 00 X £ 1 1 1 1 1 1 .—1 1 vc !! rt , > cd Ov a •y o i-H en 1—

ov o- vO vO i-H cn 1 m CM in <f O in vo CM Ov m Ov en <f CM vO

Ih

m inm .* i-< r^

mm VO r^ 1-^ rO en CM en c

-3- 1 CM 1—VO vO VO ov OV Ov CM 1—1 1 1 1 1 1 1 1 1 1 t r-K 1 Wc 1 1

rO£

1h 2

OO *

CO

OvO

CMVO i| ^ o I—

m

CMm

COm

vo vO1 vO

fa 3

VfcH < d <r

m 00 <t 3

in CM

m >

6/M

.—» *-» en vO

O CM vO 1-1 cn vO Ov cn 3 j: p~ *-* CM in CM 3

vO

m 00 cn £ .5? —i "* CM <* CO 1-1 en m vO

0) i«

v ^t s

-3- CM in CM 00 vO 00 00 co c ° £ <J- en Ov CM VO m CM Ov e'- <!- W

DO

I-l CM 1—

"^ en 1—C 1 <f i-l CN en

CM

Q

V

cr

r*"

rO 60O 1-1 oo

O

Ou CJ

OO

OO

b CO

1-1 c

rt>a

rt x c cW uoc

corn

4-1 aawC

Ma

4-1 0)

a) 3 M CD CO 4-1 O 4-1

m

4-> •H CD 4J -c e i-l c 4-1 1-1 c 3 CO <u CO i-l 0) 0) a c

1-1 3 4J

1-1 E

1-1

C

1-1 4JiH

O

a £ en a) c 1—

i-H .—i i-l CN % 3 •—

-0 CO 1—

O 1—

i-l 33

1-1 en

G ^

1-1 CO CO 3 O

Ot-l £ a 33 cn

1-1 en

l-i CO CO

O

X CMXB 1-1

u

—

v^

O PC 33 CN < i-l i-< 1-1 CM CM M

a.

CM

fa VD en <! <: < p^ cn

1-1

I-l £1 P- en CM GO z S3 in O O Pm en

3:

O CM en en

O CM CM • • m O ^-^ y~^ ,—

1-1 •H -H CO cn

N-' en en en cn do C/l 00H

M CM 3 CM 3: 3: 33 33 CM CM vO 1-1 1-1 «

R) .-1

O r_>

O 1—

1—

1-1 < < 1—

H <C < < < CM CN <

46
A1(BH4 ) 3 29

toM2w

to

tow

&<ou

<<Qow

ECH

<JOi—

wXuo

COw&

<!>PwHUww

CO

u o in

p. • U s

in

t-l

bfV

X) o rt tH VD

a c/3

u O-v

O

>-)

U

vo ctn

SP1

in

ooM

4-) 0C4 in o

00

ft o d (Nl V VD 3 co co

4> | S

(5 e i

nj ^

>. rt * ft M, u vD <^ 3 ^ CO CO CO u "^ ^O I c 1 £ 1

OO

M 5 o

.f

Fo

ALUM

u nj ITI t—

>

bfu

.-H 4-J CO o 3 X! I-l I—

6 .J? r^ m

0) fc 4) vO r-1

C5 15 lO p^

10

r-l

XI Oj X> nj

O t-1 60 6 10

I—

C

rt>

ft

n)

4-1C cW 0)UC

nj

in

co

fto

in4) P

-oc

a) 9£

t5

i-i

h

CM CO

-sf

0) CM PS

T-l CO

,£> PQ

rt i-l 1—1 H < <d

47
Ga

30

c/> W2u

c/1

toW»—

H

PiW

0,o

a:

(Xo

<;z

><QO2

bJuIHJUI—

wu

Inoww

-3>QWHUUJW

co

oo vO vO o o _ •—

o vD o o a vD vo r^ CM r^- o £ CM in or vO V

i-l T3

r-- oo i-l a\

>v r~ end ON

CM coo

vO

MD 3 00 tf i m CM «* O

g, in

INI

t-i to r- co vO CM r~ 1 co m i-l o ^

oo

Cfi OCM in

r-l i-i CM CM

IrH

X ~^ o

IT) oo a o^

ccl ro * u IM

r-

o vO o co ON l O r^ I—

00

O oo CM vO o <r

rO

m CM CI vO «tf <r <r en vO 1 1 r-l CM i I-l I 1 c £

rt) **-* a

CO o -or CM

>• o CI CM o m vO 00 00 r^ r^ «* a u

•5 ^ O r-t vO o o O i-i <t v£> 00 1-4 CO CM

r - >- ^ >43 o 00 o> m r-~ o vO 00 CM M3 m CM

CM vO co 1 00 I-I 1 1 CM 1 C H CM I Wc

rt §

oo o

CM

CI

00

CI £ M 1 O © M3 -a-" r^

m

mm 1co r%

u iJ vD o r^ 00 vO o \0

m CM

i-J CM vD CI 00 r~*

U s

1-1 CM

w- £ .2?

o> 00 ON 00 oo r*^- r^ > CM t

I-l I-I CI CO CM CN CM

Ofur- r^ r^ <t ~* r-- r^ r1h 4)

ctn CTv

m rm r^ o vO CM MO CI 00 i-i m OO r>» 00 O

[0

i-l i—i-i r-4 i-l

X 11

T

X rt

O i-l OO OO oo cr oo cr oo 00 00 cr CJ oo o 00 00 cr cr

co <0 CO CO <o

T3

m

C

rt>a

ft) £ C cW 0)uc

'-S(X r-i i-l t-i i-i -I

rt) o

II II II II II

D

J2

(0CD e E S e B 3 Cc

01

4-1

CD*

4-1CO •u

CO o

•H

"I

01

4-1 CO

4-1 CO

4-1 •u

u 4-J 4-1 a> eg CO o CO CO it X,u 3 u T3 73 XI •o £ u (J 4-1 4-1 4-1 00 CO CO CO. CO CO *~v h 1-1 O O fc en +

CM 1 1 y-s CM CI co PS CM + + + CI o o x. o o + CM CO St CN o O CM CM X o N—

co

CO ID

n CO CO CO CO CO CO CO CO CO co

O

H o o o O

OO o o O

O e> C3a

X

_

48
Gal

30

coW

COWi—i HW

a,o

bj&u2QOW

a:

<5Ui—

SwUo

COW<PwHUWw

CO

U

in o o vo °a 'o as m r^ r~- o E

r^ oo oo 00

in

bi

cy

v£) ON

d

-i

,—

c

CO -* st in o s]-'

CM* O CO 00

p

CN u-1 CO CN

m 00 vO st

i-i

U t 1 I CM as l~>. i—

ooM

>-4 CM co st

£*

OS 0<N in

CN CM CM CM

•M

w <—

o

rd 00 ! (X a^

n) cm U 14-1 oo r^ i-4 oo st St r~

m o m j

53 CM oo oo i-l CN OS in oo r-l M3 i-i st r^- as I-I OO n CM O CM 00 OO , i-l r-4 -i i-l 1-1 CM i r-4 | 1 i-4 j ffi 1 1 i 1 1 i 1 i T3 £ d ^ 1 >• o

cd * m CN 0O 00 i— -I <t o <t ^4 cn st CM as <3 o O 00 v£> oo oo o^ m r^ O 00 i-i CM 1^. 00 « | en VD CN O r~- oo i-4 CM o i^~ co r-l as co m

C

CN 1 r-4 CM CM CM 1 i-4 i-l -I CM 1 1 iH i-l i Wc i 1 ' I i ' ' 1 1 1 i1ji

a) 2 OO

M 6 1

14-1 o . . st

u 3 ^J o as o r~ o a vO r-4 r-l j h g 1 1 ' 1 HH

cd > .—1 -*->

m St CN oo r^ in CO a\ oo ON r^ ~£> st

br CO 00 s* I-l i-l i-i r- r~~

m CN st

m CM

h

r^- r~ l~» r^ r~- r~ i-4 o -I VO st 00 VO

4) 1-

V co o>

O oo r~ VO

m o CM OS a\ as vO

-5 o i-i CN oo o CM o i^-

m St o 00 as

w

to

i-l -4 I-I I-l i-l i-i i-i oo 1-4 co 00 i-i

,13 0) XI

id tr rr o oo cr a* o cr

m CJ 60 XT 00 &0 o cr cr 00 6 co

co CO CO CO CO CO co co

C

cd>-IX

rd ,C

a

aw

0)oc

p.

•iH i-i r-4 i-4

H r-4

a

u

10

u

co

II II II II II

CO E E E s ^ ^ ^ ^

"0c

tu cu <u cu <u

4-1

up 4J 4J

CD CO CO CO CO

id 4J 4-1 4-1 4-1 4J

<d

co CO CO CO CO

T3 T3 T3 T3 T3

4-1 4J 4J P 4-1 •"V

CO CO CO CO CO CMO fc

CO + CN , on

CN

CD /-~S oo •"N 00 1 2 w o w + + CO 1-1 CO st o CO o CN CN oo !-t 1-1 o U u U

rd ^-^

a fc4 fe 1*4 1*4

Uu CO

m pq

m

M

H

CO CN CO co co CO CO co co o CO CO CO CO O w O a a O o o O \s o C3 CJ5 CO

49
Gal.

30'

w

to

W

o

u

2

Q

O

W

X

H

<!ul-H wu

h

ow

w

>

Qw

H

u

w

w

>- M

3

n)V

u

i y-N «

COo

(A co co U

4-> J3

fd id 2 H

a5

o

id

C 00 C o

C u '£ u

c .t?

id u

4J o

O i» J3 <U 3 P

v

cn

o

<t

CO

O

I/O o\ CO

-T u-l CT> o o^ CM

oo m r~ o CO co H CM CM CO en -3-

CM CO CO on 00 O r-l r-l o r~ O CO O

u"> <! VO VO <X< moO O r-~ cm

o

CO CO CO co xj CO CO co co p^ as g ^1- CO g

§ ^

X

a St

CO uo vO r~ 1-1 g m vO r-. Ov r-l CO CO CO co CO CO CO CO CO CO C

I-l I-l I—

r-l 7-\ u u U l-i M I-l u o o U o M « PQ m w pq o o o o o o o o o o o

50
GaCl3 * CH3CI

30

W2wwW1—

HWo

ftu2QOwH

«!U1-4 swuowW>PwHUww

UP o

K)a

n) O

rtvX

-ac

nJocWao

rtO |J

>-

oreH 3

4>b •~N d >*

PQ

O , CO

n)CO

u

•i-) *-» ,£> d td Z H oc

ttj

CO o£

1) " 3 rC £.5? o >O

toa> Pco

-3- en

00 o

IT)I m

CO

O

<*

""> cn cr\ <*i >-i n m vo o r~- 10 to w*l VD vo

if

CO CO CO i-Hu

a

p-i P-I vf n c

r-t 1-1 Pa oB s O O O O CD O O

51
2GaCl3 - CH 3 Cl-Ga(CH3 ) 3 - (CH3 ) 2 S

30

10WW

toWH

PiW

CUo

Ohu2

<;zQO

cdWIH<Ot—t wXuoww>QWHUWu

CO

p. "o u E

in

uV

i-l •o

rH o

to

•-)

U 1 1

in i

=0 tt j >- on OCM IT,

.,_ PC i-H u

00

a

O

nJ tSJ U UH

rt 3 uX "o 1 c £ J" n) « l >-a

COm CT\ o st CMm oo ON i-H 2 ^ r^ vD <f o i-i St 1— on O r-»

m

h <j r^ 00 o\ o o r~

O ON

m St CO

CM CM •-h CM CM CM I-l I-l i 1 1 C 1 1 i 1 1 1 1 1 Wc

to ~ OO

w £ 5M

UH

aO

-j

h el ' 1 Vh -" -

nJ vO CO oo o CO kO i-l 00 st o\ > "3 X st r~ p~ \0 o CM on co NO in

atuv© ao in i-H CM CO CO 00

m on

<u Ih Qj CM St <t St

O st St CO oo MD c 5 O !-H m CO m CM O i-l CO r~~ st o- CM CM CM CO <r r~ CO i—

1

r* 2 cr Q 5

co

u o o OO cj o o •H 60 6

t-l

rt>a

"rt x c cW

4>uca

en XIco oa

«D Cc

rt

ro£ 8 O oCM

•ooCM •^

!-) .-1 CM f*s -P i- i-H u u CM •"% in u

m

O

m 5 8

•^ in * u « ^-^ h

CO SC co * CM pq co ^-^ o 8

CM CO sCM CJ jf? • co u S

C_> N—

CO • • N»^ ^-^ CM CM •-N

at en CO

M CO 3

i-i u

i-H o i-ico

t-lCO1-tCOi-lCOi-iCO

pq

I-l _P

S= 8

to to

uu c_> CJ

m

wa v—

o a ra tO to to to o CO to

H CM CMaO o e> C5 CMO o

52
In-InCl,

31

coWW

CO

COaHwoo2

><PO

eJwH

i—i w

DCUhOwW&>PwHUww

CO

uQ

Cn 00 oo r^ op. "o CO OA r-*. O

in

O £ O <f r~. CM r^-

i—)

bi

41

CM 3

T3 3 i l CM i-4 o e id oo in in on VO

CO

U o co

i—i

r-l «3

CO1

vO

in CM

ON —lCM1 O

°pP in 00 in 00

IN] r^ 00

O <f r~ ON i m •* m —I O 1-4

ao « -4 r-i CM CM CM CM

>. 0<M ITI

.,-1 EC i—4 u

id 00

cu o

<d fvl U a\ in ON

<M oo ON i—l <f i—1

in <f 00 in

4_> 33 • • • • > • • n) o on CM CM CO r*- oo in •* m

<D <* 1 i—l CM oo on o- r-~ CM

ffi

O£ 1 1 i—ii I 1-41 13

id ^j

>- (do * m vO 00 vO o- r^ 1-4 s

i-i

O ^ in i-l o in CM in in MO in <f <f

<3 o 00 CO on r^ in * 1-1 CM i-l i—i o\ 00 oo -00 <f oo ao OS

4->

m o\ CM r^ CM CO on ON CM in i-4 oo <* <f •* r-l CM OO c 1-1 vO CM 1 m CM 1 i r-l 1 i -4 1 Wa

i-( CM 1 1 1

id£ S o m

<N

oo CMco CM 1

CM

eo

1-4 3 o o 00 c-4 M3 CO 00 r-l CM CM 00 00 a

HI

m ct> CM r*. CM as a. in i-4 <r o 1-1 VD CM m 1 h i-4 CM >

id ON 00 00 r^ in 00 CO ON 3 s 6 -21 CM tf 1-4 CO CM CN CO 1-4 r» f^

oil oo vO oo vD 00 00 oo 00 CM i-4 d 1- n> <f ON o r^ in 1-4 00 CO o 1-4 c ^

1-4 CM CO r-- i-i CO <J- CO in CM

Wm

i—i CM —I CM 1-4 1-4 1-4 1-4 1-4 CM " X> CD Xi

CO

u 60 OO o* 00 O* 60 tr 60 60 60u 60 60 rr cr 60

O 50U 60

•rH id cd cd cd cd c

id>.a.

id A

C

dW

0)oc

<d

CO

P.uo

ca

IU PC

<d

rd£

r-i

ll 6

•\ cu

4-1 <d

j-> in

•cj

i-i

ii B

<U

4-1

ctf 4-1 to

-I

ll 6

cu

4-1 cd 4J

CO a

1-4

II e

cu

4-1 cd

4-1 CO

r4

IIB

•\ cu 4J

cd 4J

CO

T3

4J 4-1 4-1 '4-1 4J 1-4

*•—s ^ in to CO CO CO 1-4 1-4

r-1

fo + +

CO CM CM

0) co EC EC CO + * + O EC O O i-4 1-4 3

id H + «M «* CM o CM EC

O \»x v—^ Pn

u

u c a Pi c c c a a a a a c c a a M M M H H I-I M M M H M 1-4 1-4 M M

53
In 2 Cl 3 31

W

O Q

3

n)V

U *^\ 3 CM

ffl 7-t i—

CO

n)Co 0)

• i-4 *-» •Q

rt

flj £ H

OCM

C

cfl *-» in XI3W

U

*

3 .c E .S?

>-, 4) £

u

nl W

O

T3C

O

o

oo

O co

o

i-4 vO co oo

\0 On VO in co i-i O <f

CO

CO

U"l CM

r-< O

o

00

CO -* <r CM vO O CM CO 00 o CO r-l O 00

u-> oo r~ 00 r~ \D 00

c_> X

l-l CO n ^l U co

CM m PQ H M

c c C c c M M l-l l-l M

co co w c/>

co ^^ + d* -j- co OCO <N

54
InP

31

toW

2

w

a

H

osw

fto

os

ftu

QO

wH

u

s

wU

ftow

w

D

<>

P

W

U

w

w

U

u

ria

IT) u

rdD

c

n)>.

0-o

CW

co

rdE

InO

ft

>•of

01cW

CO XI6

XlC

rda

cW

3

rd

4)

Vh3 •-^ W en

^~'

i-H .-1 rd CO C

cu

•*-» XI

rd rd 2 H

00

CJ\ sr

S3

of

1) XI

I—

I

rdu

O

X

ox

s x: g .5?

r° ^

rd W

(2XIc

rd

36

I-. o

ft

oo

CO 0-1 CM

as in o\ in 0~ in o^ vo cm

cm cm cm co in

r^ © O CM rH <f

CO CM CM

CO C7* CO

CM 00 CO m CM VD

cm co in O

CM CM CM CO CO

ON o

CO o vO r-- in o> o CO •* «*

©

O

CO

CO CO CO CO CO CO X CO CO CO w CO CO

CO K K PS z PJ W S 3 CO co CO CO K w

W z fs 23 25 in s S3 3 in PS PS w pu 3 z

3 CM CO m r^ i-i CO in r^ -I S S3 13 13 co r-l co CM in r^ C^ i-< CM

cu CO CO CO CO CO CO co CO CO co

cu H r-H «-l 1-1 l-H I-l t-i u H U U co CO CO CO CO co

-1 CM '^, O C) D CI CO O pq pa w m M H H H M M Hj c e C d a e c c CI c ti c C e a a C c C c H l-l M H M M H M i-i H H H M 1-1 H M H I-I M w

55
InAs-In(CNS) 3 31

toW2w

to

10WI—i HwO

0*UZQO2wXH<Uw

DCu

u<o

towD>PwHUww

to

uQ

CM C-J

—

St 00

p, * o E

0/

4J

H I—

m TJ

NO ^.

as •—i

H vO

—I •

CO

<du 00 o"

>> CM

i-i3

>-]

U 1

in

<N1

00

X

>. on OCM in u

a) CO a C*

rt

IN) 1 u CO i-l CO «* ft St

*-» S3 CM NO CM 00 St NO ON

rd i-l 1 a\ vo I-l ft CI

a> 1 t-l CO 1 I "o 1 ' I c £ i: n) ^j > o 2 o co co I-l ON I

.* <* r^ cm in 1-H in ON

t-t ^ I-l i co r- NO st r^ \ c 1 r-l i-i i , Wc 1 I E

I-! S3

oo9 O

En

Mo

V*H

M

O n) >M

CM o o r- in i-i CM St NO

"9 i; <t r- CM <* vO <t r-l

OO 00 NO e .s?

r~~ in co oo oo <t 00 oo On On

O

O Ih

V on vO co CM

O in 00 ON CMO ON c £* CO CO m O On Jo

r^ r-l r- CO CO

U i—

cm CO CM CM <t nO i-l CM CM

XI I) X (D tl cj 50 00 er cr o U

u tr o- cr CO

eg

a co <d si

XIc i-H nj^

II

a e

a) », ~ * c

0)

4-1 c a w

COocm

0) XI3

to

auy

gg Q

IIM E E

4-J CO

i-l i-H

II II -o

4-) e e co

<u a> 01 III "O o 4-1 4-1 (J 41 tl c a ca a) ea N

(d 4J 4-1 CO CO 4J 4J «H

CO CO c

td o i—

. t-< 3 O "D CO CO •o "O 1 £

4-1 4-1 CM CM CO 4-1 4-1

C

*TM\ CO CO y^ *-^ CM CO CO 3

<f

M CO CO •-N 1 ^ ^ CO

i-l

h + CM CJ o ^n +

CO o o

CM CM o

CM

CM CO + ^\ yN. CM CO CO

u CM CM CM CO CO • z z z

f-H CO ,o X)

O C_> r-f I-l cou o o

.D t

09 CO c s-< o CO HI CO •—' n_-

R)

C c M

C c C

C c c c H M M M N-' M M I-l 1-1 M M M

56
Tl-TIOH

32

W

W

WI—

(

H

PSH

&

O

u

QO

a:wH

<:oi—

i

wu

ow

u

<>

a

u

H

O

ww

U

coM

C

cd

T3V

C

Rj 10

3

n)0> «

"(3co

• iH 2

idc.

It O

itVX

C

cda

o

cW

c

Q

>

Of' M

CW

6

C

n)>. n

cW

c r-* id f-

-*-» o

CD.

1/3 J3 <V 3 D

XIc

rt

J3

rt H

ex

4) "

=1 J3 C M

Cti

cd

O

CO oCO

cost o

co o

CO

1-1 r-t

!

CM ! St <o st

CM O r^ CO CM m o oo o IT) O r^ t-i m st CO * CO i i m CO

i i 00 st

1

s±

CO CM

CO <f 3

CO CMSt

1^ St St <t <t

in in in ' in in st

in

COstSt

oo st

CO

CO cr cr o* cr tr rr

CO CO CO a) CO CO

01 CJ u •U

CO CO •u u

CO CO 00 W . • TJ a

C U 4J

o o o WWW CM CM CM CM CM CM CN —U PC i-l- P- o o o o o o iri o in O O O co m r~~ o m o

+ + CM co

CO st + o o o rn st CM CM CM o

H H H H

57
TIOH

32

v.W2w

IT) waw

Oho

a;a,u2zQOWXH

«.Ur-H wu

InOwW

E>J>QWHUww

t/J

uacMc5 m r- CM rH ^ o

CM CM

in

0/ SO XI

Os —-^ CM o>

—I

"to <f r- OS

mm CO

>s </) o 1

so' •tf VO CO rH OS I-~

1-1 CM CM CO CM -tf «* t-l 3 1 >-> u i

in

00o

CO o

COo

GO

M

>. at

O «* co OCM kTt >H W -* u

00

a. o

co (V) CO oo o i-H r-H O o CO <d- oo m CM CO in CM i-H OS r- SO r~

4-> 3 m SO CO oo i-H ^ <f 3

OS OS CTs en

O ffl -* •tf i m CM r^ r^ CO co CM r^

(1 i i F-l i i 1 1 1 i i X "o '

•ac u - 

^£

rt ^J >

Q.

nJ os CM as r~

O o vO SO vO CM in co r~~ cm vo i-H

O o CO . c s ^ CO r- co oo 00 -*' 00 ^O 00 rH i-H CO m 1 £. c < in r^ nj- r^. i i r^ in

i-H <t 1-H CO 1 1 1 1 <J- r--i || ; °

to 5 oo

X

rHOS 3 >l-l O M

S3

© OS ! o

>J <!• | d I | v*-. H | n! 00 CM <r 00 O o O >M

.—I -4-* -* CM 00 -* CO so ON 3 X 00 OS vO r~ CM r~ CM £ .5? CO CO CO CO 00 CM r^

aj t. 01 oo in CO co Os

m o c £

CO in CM -tf CO r- I-H

W

CO

CM CM CM CM CM CM co

X 4> .c

to cr cr cr cr o O 30 D" cr crO cr cj oo cr cr cr cr cr CJ

a

-a

•4-1 en

CO CO a) CO <0 <0 CO CO CO CO CO CO aj c

cd i—

1—rH > II II II a

rd e e E X C

•s •s „ C

01 •u

Vu

01

4-> to uu P.

CO 4J

CO 4J

CO 4J c I-H CO t-i i-i r-H CO I-H CO I-H I-H l-H

ft)

uU II II II II II

a II II II <n DO a X» T3 X CD s 4J £ e E 4J S 4-1 E E E 3 n

00 CO co

C/j

0) .«. 01 01 CU • M o O 01 mm cu OJ 01

X 4J 4-> 4J 4J

p CM CM 4-1 • 4-1 4J 4J c CO o CO <0 03 CJ W as CO o CO <0 CO

rt 4J o 4J 4J 4J

O 4-1 o 4J 4J 4-1 CO CO CO CO CO CO o o CO CO CO CO CO

ifl CO CO o o CO "3 1H . . • •H 00 00 •H • T3 T> •o 13 T3 T3 T3 T3 T3 •d •a £

4J c 4J AJ 4-1

G c c 4-1 c 4-1

V 4-1 •-n CO 3 CO CO CO 3 •H •H CO 3 CO CO CO CM (h s_^ CMCO h + CM CO

o> + ^"N *~s + + 1 rH CM w m CM CM CM CM co

.o S3 tfi o o fr. i-H I-H i-H rH rH

toOO \^y Nr^ fe 5S

O o OO

O

H

•-I r-l i-H r-l i-l i-< r-t r-l rH rH T-l H H EH H H EH H EH EH H H

58
TIBr,

32

Wsw

inWHwo

D<O2QO

odwXH

<:ui—

wxuoww>pwHUww

U

O PL o U £

Of

cu ON TJ

1—

^ in oo oo i

CO

ON ^ ro * . . . I-l 00 U in CM 00 oo' 00 ON co co" o st" CO ON o 3>-> O i CO LO vO CM st st i-i CM oo i-i St oo 11 SP1

UN

fSJ

oo

w

>- on ocm un • rH K —

1 u

cd 00 1 a o U

tM oo o on o i

y-i 00 vO oo

m i-l o m ON LTl st oo CM r^ CM j

53 CM U0 o 00 ON o CM CO CO i-H 00 CO CO St" St vO o

I-l 1 1 St CO CO 1-1 CM U0 CM I/O 00 1 1 1 1 1 1 HI 1

•ac £

In) ^

>- •

cd r^ CM j a o o ON O st 1-1 st St st O r^ CM o r-l 00 r^ CM r^ CM ON * st CM st ON st ON CM I-l ON 1^ o ON ^3 CO ON O ON m o i oo t^ 00 CO CM St CM st 1 CM CO CM U"> U0 st LO CO ON c i 1 1 CO r-l 1 1 i 1 1 1 1 1 l 1 CO 1 H 1 1 i o

nj S OO

w £ 5M 9 o i| Yl h S3

Eh ' * VO O o CM O O o ^£> o

>. 3Z o CM o 1-4 ON oo r~- oo VO br ON oo St CM r^ oo ON in o M £ . 6.

r^ i-i VO 00 CM i-i o -I o

1j CO CM no ON 1

st" st st VO sr" & 00 st r^ 00 00 vO st i-l CM

W

01

co CO st CM CM co st

m in

,Q <U

•l-H to er O* a" o o*

M cr D* o oo cr cr o* cr tr

W er- O* o cr

a

XI

W

CO CD as IS CO £0 CO (0 CO CO CO CO as CO CO c

nj r-4 p-l i-i 1-1 >>a

II 1! II 11

to

g 6 e g

A ^ ^ ^ ^ C

CU 01 cu cu

0) 4J 4-1 4-1 4J

w 4-> CO aj CO CO i u (X U 4-1 4-1 4-1 < Ho

i-H CO I-l i-l CO i-l CO 1-1 i-i i-l i-i CO i-i

II . II II II II 11 II II

B II co

co XI TD X) X)

-Q <D

g 4-1g

g 4-1 6 4J e 6 g

g 4-1g 3 P

CO CO CO CO tn ^

cu cu cu cu cu cu CU CU cu : X1 c

4-1 4-1 4-1 • 4-1 4-> 4J 4-1 4-1 4J i a) CJ CO CO o as CJ CO CO CO CO CJ CO

co 4-J o 4-J 4-> o 4-> o 4-1 4J 4-1 4-1 4J

CO CO CO CO CO CO CO CO CO CO CO co CO

co co CO CO CO 3 • •H • •r4 , •H , . •H

13 X) XI XI XI T3 X) XI X) XI xi XI xi £

4-1

C 4-1 4-)

C 4-1

a 4-1 4-1 4-1 4-1 c 4-> en

CO 3 CO CO 3 CO 3 CO CO CO CO 3 tn ! >~^ CM h o o CO CM W

<t

CM

cu 1 CM CO + + 1 f i i—

CO CO sj i-l

OM CM CM CO CO st

J3 i-i I-l r-l CJ i-l

u

UUu

uu ^j

(TJ

u o O CM

O

M PQ

m pqm pq pq

H t-i 1-1 i-l i-l i-l I-l i-i i-i i-t i-i 1-4 r-l H SH H H H H H H EH H H H

5S
TlBr03 32

W

w

CV) w

w

o.o

IXut—i «

Q

O

w

X

H

<;u

Wu

o

w

ID

>

Q

W

H

U

Ww

u

c

n)

ind

3 X.

° S

01

<0 p

X

c

n)

O

oo \D <r O \D \o

00 r» CM en <r r-H H

i-~ oo r~~ oo o CO O i-i CH CM !-< oo •tf oo 00 t-l ON t-l o o --r in t-( r^ f—

<

<f o o

<f r^- co <f <f co U~l

cr cr cr XT o cr cr o rr a

a <a <u <0 aj <D <o

II II 0

u e R

01.- <D <u

• 4J 4J a CO ca o 4J 4-1 ca CO CO

en •H

•o n XJ s 4-> 4J - CO co

CO tH O o

U M n «

O O CM CM X

u 1-1 CM

PQ o >-l CSI CM CQ U pq o

J i si- CO (J <f O

•tf o m co o CO

-1 l-l M CM CO CM

Ir< t-l tr<

60
T1(CH3 C02 ) 32

[fl W

coaH

PSwo

PH&o

>HQOw

DCH<Uwuow>pWHUWw

10

00 6 ° P. o

'o

rco" CM

Q in

01 as T)

rH

r-H i-i «tf

O

m rH

60 >v e ft)

•iH

1-1 co

u i-h VO

m 00 in «3- r^

p >*

m CO CO vO vO CO

.C

•"1

m

O

°p?1

in

rsl

00 tto

ITl

u

ft) CO

CU o

ft) O

rg

14-1 CO <r in in

i-h -tf «tf CO •* CO 00 vO CT\ CTv

4-1

ft) 3

sf" vo in o vo •* vf I-l CM vO*

i-i CM i-l r^ CO CO CO CM iH -* i rH CM 1 i 1 rH

DC o 1 1 1 a 6

a) ^

>* A) . o CO CO

a. o •* 00 CO CM CT> VO

O CO

m COm rH 00 o s ^ •

*H CM >tf rH CM

m 00 00 00 CMmm CO r~- r^ vom rH I-H m CM m m -cr -* O co a\ 00 vo CM CM rH c

CM 1 1-1 1 i 1 1 i-l i-i i i rH 1 rH rH

W 1 1 l i 1 1 1 o

•rH

ft) B

g

00

HH « MJ 3 o oh 3H

ft) in «tf vO VO

O i-i o> r~- I-H i-i i-i in COm o

>- rH •*-> o\ CM r» •* o o <f

Om iH 1-4 vO ON om 3 X! co co CTv i-l <f ON r~~ o i-i CM r~ vO «* o rH £ .S?

-d- vo vO vO CO CO CO «tf o> CO CO CO r^ <t oo> IH V i-i CO rH CTv vO vO VO i-i o rH in CM 00 m CO £ o CO in oo CO «* vO CM OV vO CO 00 vo CO vO W

01

CO

m in r- in CM CM CM CM CO CO CO •* CM CM

V

•rH rt o* o y

y

y

yy cr cr D* cryyyyyyy cr

4-> CO

CO «j aj CO to CO c

ft) i-i >-

II

a

rt 6

4-> c * W

01

ai 4J

CD

01

ua

nj

a, 4J -0 ^

rH 01 i-l i-i

ft) C

n) CO

01

CO

y II • II II co D oCM wo e

T3U

0) e a

CO at 4J "" 01 4J oT

4J

VtH "-* <o

y CO CO

ft)

ft) £ oCO

•u

CO o01

4-1 01 4J

01 3 CM

PS . 0] . V •o T3 *o T3

(h

a 4JC

u •U 3

•H 01 3 0} 01 CQ CM to CO ^*%

i—1

co CO CO S CO CM

•*V <f CO + § CO

g

CO 8 01 •* o o CM + CO CO j5 CO CO ^p

4->

ft) 2 3 oCO

0) COai at CO CO

ai CO

CO o CoCO

r-4 CO • r-l U

CO 8 s S ft) w CM CM v^ CM 3 s s ^ O CJ pq H CM o Vw* H rH s s £

i-l i-i 1-1 1-1 I-l i-l s s

rH rH rH rH

HHH E-i

H

HH

HHHH

61
Tl(CH 3 CO^)-TlCNS

32

o P. O 6 m •o

vO ^~. C* t—

r*. in CM

i-l • n) co u O C* Mf 00

t-lD

in CO VO in o U

i

iTl

00 K

>-

oin

OO a a~ U

rM

en rH rH CM O O CM -J CO

rt 5

vO ooo

C*

.—

oo

i-H 11 i I-l X "o c 6

n! ^

>-. ort 00 m a> a u oo m o v£> 00 m m

o 34 X

u ^ -tf vO vO r~- vO CTi vO

i-h m m CM rH 1-H c

i-< i W

c oo tt i O

v« H

rt rH CM CM 00 >

r-l i-l 1

i-l 3 X co 3

oo in E .5?

-tf CO -*

4> U 0> c* 00 vO CM c ° £

-* o Sf vO W CM CO CM CM

.a lb x> m

cr

cr -h cr cr O O O" cr 6 w

<0 ,-1 (0 a 09 <o

c

n) rH > II a

rt E X

cW o

c

p. 01

01 4J

eg

4-1 c 1-1 i-i 4J rH 0)

rt b <0

*-* u II II e II en a •H •o X V e 6 e s 4J 3 P

r-l CO

l/> •V * D •V 01 01 m 01 TS u •u 4J . C a CO 09 (0 o

rt u 4J 2

4-1 o

to 00 o 0] CO

n) r-l CO %

r-l , •H

TJ T3 2

a •o

4J 4-1 4J C

CO CO j-i CO 3

N-^ CM k •—

CO CM 8 m

1

<u co X •"\

I-H S ef S o CO

XI o s *z

co- ^ o v^' o o

rn i-H 1-4 1-1 1-1 r-l H H EH H EH

62
Announcement of New Technical Notes on

Selected Values of Chemical Thermodynamic Properties

Superintendent of Documents

Government Printing Office

Washington, D. C. 20402

Dear Sir:

Please add my name to the announcement list of new

publications to be issued in the series: NBS Technical

Note 270 - Selected Values of Chemical Thermodynamic

Properties.

Name

Company

Address

City State Zip Code

(Notification key 341)

CUMULATIVE INDEX

Chemical

Symbol Element

Al Aluminum

Ar Argon

As Arsenic

At Astatine

B Boron

Bi Bismuth

Br Bromine

C Carbon

CI Chlorine

F Fluorine

Ga Gallium

Ge Germanium

H Hydrogen

He Helium

I Iodine

In Indium

Kr Krypton

O Oxygen

N Nitrogen

Ne Neon

P Phosphorus

Pb Lead

Po Polonium

Rn Radon

S Sulfur

Sb Antimony

Se Selenium

Si Silicon

Sn Tin

Te Tellurium

Tl Thallium

Xe Xenon

Table Part and Page

Number Number

29 2 - 37

5 1 - 17

20 1 - 93

13 1 - 42

28 2 - 26

22 1 - 101

11 1 - 31

23 1 - 104

10 1 - 24

9 1 - 21

30 2 - 48

25 2 - 7

2 1 - 12

3 1 - 15

12 1 - 36

31 2 - 53

6 1 - 18

1 1 - 11

18 1 - 61

4 1 - 16

19 1 - 83

27 2 - 17

17 1 - 60

8 1 - 20

14 1 - 43

21 1 - 97

15 1 - 56

24 2 - 1 26 2 - 11

16 1 - 58

32 2 - 57

7 1 - 19
U.S. DEPARTMENT OF COMMERCE

WASHINGTON, D.C. 20230

POSTAGE AND FEES PAID

U.S. DEPARTMENT OF COMMERCE

OFFICIAL BUSINESS