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## P. 3



# NUREG/CR-015 0 

# Vol . 3 0RNL/NUREG/TM-190/V 3 Dist . Categor y

NRC-RH

Contrac t No . W-7405-eng-2 6 Healt han

dSafet y

Researc hDivisio n

ESTIMATE S OF INTERNALDOS E EQUIVALEN T T O2 2 TARGE T ORGAN S FO RRADIONUCLIDE S OCCURRINGI N ROUTIN E RELEASE S FROM NUCLEA RFUEL-CYCL E FACILITIES , VOL . Il l D . E . Dunning , Jr . G . G . Killoug h S . R . Bernar d J . C . Pleasant * P . J . Wals h *Eas t Tennesse e Stat e Universit y

Manuscrip t Completed : Jul y 198 1 Dat e Published : Octobe r 198 1

NOTIC E Thi s documen t contain s informatio no f a preliminar y nature . I t i s subjec t t o revisio no r correctio nan dtherefor e doe s no t represen t a fina l report .

Prepare dfo r th e U.S . Nuclea r Regulator y Commissio n Divisio no f Health , Sitingan dWast e Managemen t Unde r Interagenc y

Agreemen t DO E 40-550-7 5 NR CFI N No . B041 0 Prepare db

y th e OA KRIDG E NATIONALLABORATORY Oa kRidge , Tennesse e 3783 0 operate db

y UNION CARBID E CORPORATION fo r th e DEPARTMEN T OF ENERGY

## P. 4



# CONTENT S Pag e LIS T OF TABLE S , . . . . i v HIGHLIGHT S v 1 . INTRODUCTION

1 2 . REVISION S OF PREVIOU S REPORT S . 5 3 . COMPUTATIONALMETHOD S 6 4 . METABOLI CMODEL S 8 REFERENCE S 1 2 Appendi xA . Tabulation s o f Committe dDos e Equivalen t t o2 2

Targe t Organ s o f aReferenc e Adul t fro m Uni t In halatio nandIngestionExposure s 1 5 Appendi xB . Tabulation s o f Effectiv e Dos e Equivalen t t oa

Referenc e Adul t fro

m Uni t Inhalationan

dIn gestio nExposure s 6 9



# m

# J_JL
_



# LIS T OF TABLE S Tabl e Pag e 1 . Radionuclide s fo r whic hdos e estimate s ar e tabulate d.. . 2 2 . Fractiona l uptak e b y sourc e tissue s 9 3 . Retentionparameter s fo r sourc e tissue s 1 0 B-l . Organ-specifi c ris kfactor s an dproportiona l weight s .. . 7 2

i v

## P. 6



# HIGHLIGHT S
Thi s repor t i s th e thir do f athree-volume tabulatio no f interna l radiatio ndos e conversio nfactor s fo r manfo r radionuclide s o f interes t inenvironmenta l assessment s o f nuclea r fue l cycles . Thi s volume pro vide s a nupdate dsummary

o f estimate s o f committe ddos e equivalen t fo r 14 2 radionuclide s considere dinth e previou s tworeports . Intake s b

y inhalatio nandingestio nar e considered . Th e Inter nationa l Commissiono nRadiologica l Protectio n(ICRP ) Tas kGroupLung Mode l ha s beenusedt osimulat e th e depositio nan dretentio no f par ticulat e matte r inthe respiratory tract . Result s correspondin gt o activit y media naerodynami c diameter s (AMAD ) o f 0.3 , 1.0 , an d5. 0 y m ar e given . Th e gastrointestina l (GI ) trac t ha s beenrepresente db y afour segmen t catenar y

mode l wit hexponentia l transfe r o f radioactivit y fro m on e segmen t t oth e next . Retentio no f radionuclide s insystemi c organ s i s characterize db

y linea r combination s o f decayin gexponentia l func tions . Fifty-yea r dos e commitmen t pe r microcuri e intak e o f eac hparen t nuclid e i s give nfo r 2 2 targe t organ s includingcontribution s fro m specifie dsourc e organ s plu s the systemi c activit y residinginth e res t o f th e body ; cros s irradiatio ndu e t openetratingradiation s ha s been incorporate dint othes e estimates . A separat e tabulatio no f effectiv e dos e equivalen t fo r al l 14 2 radionuclide s i s provide dalso ; thi s quan tity , a s define db

y ICRP Publicatio n26 , provide s a nindicatio no f th e overal l healtf

hris kresultingfro

m aradionuclid e exposure .

## P. 7



# 1 . INTRODUCTION
Thi s volume present s tabulation s o f dos e conversio nfactor s fo r 2 2 targe t organ s o f ma ndu e t oth e inhalatio no r ingestiono f any o f 14 2 radionuclide s liste di nTabl e 1 . Nuclea r deca y dat a ar e take nfro m Koche r (1977) . Th e presen t tabulatio nprovide s a revise dsummary o f 50 - yea r dos e commitment s publishe dintw opreviou s volume s (Killoughe t al. , 1978a ; Dunnin ge t al. , 1979) . Error s i nth e previou s publications , whic har e correcte dhere , ar e indicate dinSects . 2 an d4 . Ou r objectiv e ha s beent oassembl e dat a an dmodel s tha t ar e believe d t obe representativ e o f th e stat e o f th e ar t i nth e estimatio no f inter na l dos e fro

m ingeste do r inhale dradionuclides , andt oappl y thi s informatio nt oa unifie dcalculatio no f dos e conversio nfactor s fo r thos e radionuclide s whic har e o f concer nt oth e Nuclea r Regulator y Commissio n(NRC ) i nit s regulator y activities . Thi s systemati c approach , embodie dinth e INREM I I compute r cod e (Killoughe t al. , 1978b) , i s no t entirel y

fre e o f difficulties , whic hoccu r a s conceptua l inconsistencies , a s discusse di nth e previou s volumes , o r a s th e requiremen t o f specia l treatmen t fo r certai nradionuclides . For calculation s involvingdecay chain s whic hinclud e a gaseou s isotope , fo r example , th e genera l method ology ha s bee nmodifie dsomewha t t ointerfac e a mode l fo r th e dynamic s o f a ga s i nth e respirator y ai r space s wit hth e Internationa l Commissio n o f Radiologica l Protectio n(ICRP ) Tas kGrou pLungModel . Informatio ninthi s repor t i s organize dinth e followin gmanner . Know nerror s i nth e precedin gvolume s o f thi s repor t serie s ar e docu mente dinChapt . 2 . Chapte r 3 present s a very brie f summary

o f th e model s an

dcalculationa l method s usedb y the INREM

I I code . Mor e ex tensiv e description s may be foundinth e previou s report s inthi s serie s an dinKilloughe t al . (1978b) . Th e metaboli c model s an dparameter s utilize di nthes e calculation s ar e summarize dinChapt . 4 . Appendi xA

give s summary

tabulation s o f committe ddos e equivalen t (rem/uCi ) fo r eac ho f 2 2 tarqe t organ s o f a referenc e adult . Fou r set s o f table s ar e presented : thre e fo r inhalatio nan don e fo r ingestion . Th e inhalatio ntable s correspondt oparticl e activit y media naerodynami c diameter s (AMAD ) o f 0.3 , 1.0 , an d5. 0 ym . Th e respirator y clearanc e clas s o f th e paren t nuclid e (D , W , o r Y , wher e applicable ) i s show nin th e colum

nlabele d"SOL, " an dthe G I trac t absorptio nfractio n"Fl " i s listed . Th e ingestio ntabl e show s onl y th e G I absorptio nfractio no f th e paren t nuclide , inadditio nt oth e dos e conversio nfactors . Inha lationandingestio ncase s ar e presente dfo r eac hchemica l for m o f a radionuclid e considere dappropriate . Appendi xBprovide s estimate s o f th e effectiv e dos e equivalen t resultin gfro

m a 1 yC i intake , correspondin gt oeac hinhalatio nan d ingestio ncas e considere dinAppendi xA . Th e effectiv e dos e equivalen t (ICRP , 1977 ) provide s a measur e o f th e overal l carcinogeni c an dgeneti c ris kresultin gfro

m a radionuclid e exposure . I t i s suggeste dher e a s

1

### P. 8



## Tabl e 1 . Radionuclides fo rwhich dos e estimates are tabulate d

Nuclid e *M- 3 C-l * NA- 2 2 P— 3 2 MN- 5 4 FE-5 5 FE-S 9 CO-5 7 

## co-s e CO-O 0 2N-6 S Rd-U b 

### SR-H- ; SR-9 0 3R- 9 1 »-9 0 Y-« » V-91 M ZR- 9 5 2R-S 7 NB-5 3 NO-SS M N8-9 7 N8-S7* * 40-9 9 

## rc-s s TC-99 M RU-10 3 RU-IO S 4U-10 6 *H-1C3 M RH-IO S RM-1OE M rtH-IOt 58-12 7 re-12 7 TE-127 V TE-12* . TE-129 M Tm-121 TE-131 M TE-13 2 1 -12 9 1-1 3 1 : -1.3 2 : - 13 3 1-13 4 1-13 S CS-13 4 CS-13 5 CS-13 6 CS-13 7 3A-137 M •JA-1-. 0 |_A-1<| 0 CE-l« t CE-14 3 CE-14 4 PR-14 3 PR-14 4 •*»R-1«« M NO-14 7 f»M-l4 7 SM-I4 7 

## Radioactiv e half-lif e (days) i.5\e*2 2.09E* t 9 .50E+< ! 1 .436+ I 3 . 12 E + 2 m .H<_E *m 4 . **6E *1 2.71E+ 2 7.08E* 1 1 .92E* 3 _>.44t*_ ! I .97E* l S.06E+ 1 1.04E+ 4 3.9o£- l 2.676* 0 b.U._£* l 3.45E- 2 6.4UE * 1 7.04£- i J.32E* l 3.0lt* 0 5.01E- 2 6.'.»E-* I _>.7SC* 0 7.77E+ 7 2.SIE- 1 J.J4E* I l.dSE- l 3siste*i J.JDE- 2 1 .47E* 0 'J.21E- 4 3.4&C- 4 3.336* 0 3.-J0E- 1 1 .39E+ 2 4.S3E- 2 3.3oS* l 1 . ?4E- 2 1 S?.S\-*m J.£6E* 0 a-73E* « tt.d«c"*0 9 . iibc- 2 «.o7E- l 3.o*_S*:- 2 ....'SC- l 7.536* 2 H .40E** d t.3lE* l i aioc* y I .77E- 3 t.286* 1 t.odE+ O 3.2S.E * I I.j«e* o 2.-34 6 •2 

### i .3te* i 1.20E- 2 'j.OOE- J 

## i .ne* i •(.5/ie* 2 3.91E1 3 

## Daughter

nuclid e

t-*» 0 

## »-<! *
>-« _ KB-*;! , NB--J7 M Ne-4 £ Ne-<; 7 TC-99 M TC-S 9 RH-1C J RH-IC S RH-IC 6
RM-IC J Tfc-12 7 JE-12 7 1-12 9 TE-12 * I-I3 t •1-13 1 1-13 2 Xfc-13 1 XE-13 J XC-13 '

EA-137 M CA-14 0
PR-14 3 PH-14 *
PH-14 4 PM-1 4 ? SK-1 4 7 

## Branchin g

fractio n

1 . 0C.a1 . 0 C99 3 0.9* 6 1 . 0 1 . 0 0.66 8 1 . 0 .997 5 0.7 2 1 . 0
1 . 0 0 . (-><• & 0.97 6 1 . 0 0.6 4 1 . 0 0.77 6 1 . 0 O.OlOS o C.97 1 0.63 4

0.44 6 1 . 0
1 . 0 0.9(4 8
0.999 4 1 . 0 1 . 0 

## Daughter

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TC-9 9

RH-10S M

TE-127 M

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XE-133 M XE-135 M

RR-144 M 

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Physica ldatafro

mD . C . Kocher,NuclearDecay Data forF.adionucHdee Occurringin Routine Releaaea from NuclearFuel Cycle FaciUties, ORNL/NUREG/TM-102 , 1977 .

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# perhap s abette r singl e measur e o f radiatio nhazardthantota l bod y o r critica l orga ndos e equivalent s inmany applications . Al l calculation s inthi s repor t fo r alpha-emittin gradionuclide s utiliz e aqualit y

facto r o f Q a

# = 2 0 andamodifyin gfacto r N a

# = 1 fo r al l organ s a s recommende db y th e ICRP (1977) . Inpreviou s volume s o f thi s series , additiona l calculation s wer e performe dusingaqualit y facto r o f Q a

# = 10 , inconjunctio nwit hamodifyin gfacto r o f N „ = 5 for bon e (excep t N a

# = 1 fo r bon e fo r isotope s o f radium ) andN a

# = 1 fo r al l othe r organs . Th e presen t approac ht oth e dosimetry o f bone , a s formulate db y ICRP (1977 , 1979) , i s t oconside r th e activ e redmarrow an dth e en dostea l cell s adjacen t t obon e surface s a s the relevan t targe t tissue s a t risk . Dos e estimate s fo r "bone " a s atarge t orga nhave beeninclude d inthi s tabulatio nonl y t ofacilitat e transitio nbetwee nthe ol dan dnew approaches . Th e reade r shoul dnot e tha t the bon e dos e value s tabulate d her e ar e basedonN a 

# ' = 1 , an

dtha t thi s assumptio ni s inconsisten t wit h the earlie r approac ht obon e dosimetry whic hwa s basedo

nacompariso n wit hradium . I t is , however , consisten t wit hthe recen t ICRP guidanc e onmodifyin gfactors , althoughth e relevanc e o f tha t guidanc e wit h respec t t obon e i s questionabl e sinc e ICRP nolonge r consider s bon e t o be atissu e a t risk .

## P.1 1



# 2 . REVISION S O F PREVIOU S REPORT S Inth e precedin gvolume o f thi s serie s (Dunninge t al. , 1979 ) a modifyin gfacto r o f N a

# = 5 wa s inadvertentl y retaine dwit hth e qualit y facto r o f Q a

# = 2 0 incomputin gestimate s o f committe ddos e equivalen t t o the tota l bod

y fro m alph aradiatio ninbone . Thus , al l estimate s o f tota l body

dos e fro

m alpha-emitter s tabulate dintha t repor t ar e sys tematicall y

incorrect . Intha t same report , anerro r inth e calculatio no f th e dos e equiva len t rat e fro

m bon e t o redmarrow , S a 

# (Re dMarrow *• Bone) , fo r alpha emission s inbon e volume produce destimate s o f dos e t o re dmarrow whic h wer e low

b y a facto r o f 2.5 . Thi s erro r wa s introduce dwhe nth e S-facto r fo r tota l bon e t o redmarrow , S a 

# (Re dMarrow -< - Bone) , wa s mistakenl y interprette da s th e valu e fo r trabecula r bon e t o redmarrow , S a 

# (Re d Marrow •* • Trabecula r Bone) , fo r alpha-emittin gradionuclide s assume d t obe uniforml y

distribute di nminera l bon e ( 210 

# Po , 226 

# R a , 232 

# U , 233 

# U , 2 

# 3-U , 23 

# 5U , 236 U f an d

# 238u) . 

# Correction s andrevision s inmetaboli c parameter s have yielde d differen t estimate s o f dos e equivalen t fo r 90 

# Y , 226 

# R a , 228 

# R a , andradio isotope s o f thoriu

m anduranium . Thes e change s ar e describe dinSect . 4 .

# ______ _



# 3 . COMPUTATIONAL METHOD S

INREM I I consider s th e intak e o f a radionuclid e b y ingestio no r inhalation . I

nth e latte r cas e a particulat e for m i s assumed , wit hthe exceptio no f isotope s o f nobl e gases , 3 

# H , andlk 

# C. Dynami c model s ar e applie dt oth e estimatio no f microcurie-da y residenc e o f th e radio nuclid e (an

do f radioactiv e daughter s tha t ar e forme dinth e body ) in th e respirator y

an dG I tract s an

dinothe r organ s whic hma y tendt o concentrat e th e material . Thes e activit y integral s fo r th e sourc e organ s ar e multiplie db y dosimetri c "S-factors " (rem/yCi-day ; Dunning , Pleasant , an

dKillough , 1980 ; Snyde r e t al. , 1974 ) t oprovid e estimate s o f dos e equivalen t t oeac ho f a standar dlis t o f 2 2 targe t organs . Th e term s "source " and"target " refe r t oth e irradiatio no f organ s b y emission s fro m radionuclid e activit y i nothe r organs . Th e dynami c model s includ e th e lungmode l fo r inhale dparticulate s propose db

y a tas kgroupo f th e ICRP (Morro w e t al. , 1966) . Thi s model , wit hparameter s fro m ICR P Publicatio n1 9 (1972b) , i s employe dt oestimat e depositio nan

dretentio ninth e majo r region s o f th e respirator y trac t andt ocalculat e translocatio no f th e inspire dmateria l int oth e blood an dothe r organs . Th e G I trac t i s represente db y a catenar y

mode l o f fou r segment s (Bernard , 1968 ) wit hmea ntransi t times suggeste db y Eve (1966) . Th e mode l permit s absorptio no f activit y int oth e bloodfro m any combinatio n o f th e segments , bu t we generall y assume tha t al l absorptio ni s fro m th e smal l intestine . Retentio no f activit y inorgan s othe r thanth e respirator y an dG I tract s i s modele db y linea r combination s o f u pt ofiv e exponentia l functions . Suc hretentio nfunction s ar e ofte nderive da s approximation s t oothe r functiona l form s [e.g. , th e powe r function s develope db y th e ICRP (1972a ) fo r th e alkalin e eart helements] . Th e reade r i s referre d t oth e precedingvolume s o f thi s serie s fo r a mor e thoroughdiscussio n o f th e genera l methodolog y an dmathematica l model s employed . I nany specifi c application , relativel y few o f th e 2 2 targe t organ s considere dher e ar e likel y t obe o f interest , bu t comparison s may be facilitate db

y thi s mor e complet e listingwhich , moreover , i s consis tentl y provide dfo r al l radionuclide s considered . I t als oseem s likel y tha t some o f th e additiona l informatio nwil l prov e usefu l inth e esti matio no f radiation-induce dhealt heffect s t opopulation s b y mean s o f organ-specifi c ris kfactor s (e.g. , ICR P Publicatio n26 ; ICRP , 1977) . Th e use r shoul dbe carefu l t oselec t appropriat e dos e value s fro m th e tabulations . Fo r example , endostea l cell s an dredmarrow

hav e bee n identifie da s radiosensitiv e tissu e inbon e an dthos e dose s shoul dbe use dinmany

application s rathe r thandese s tabulate dfo r bone . Also , insome situation s i t may be desirabl e t oinclud e th e activit y i nres pirator y

lymp hwit htha t inth e lungfo r computin gdos e t oth e lung

## P.1 3



# (ICRP , 1979) ; however , inthi s repor t the dos e commitmen t t orespiratory lymp h(mas s = 1 5 g ) an

dlung s (mas s = 100 0 g ) ar e tabulate dseparately . I nsome case s considerabl e uncertaint y exist s wit hregardt obot h th e chemica l for

m o f th e inhale dmateria l an dit s aeroso l properties . Moreover , th e fractiona l absorptio nan dretentio no f aradionuclid e fro m ingeste dmateria l migh t be subjec t t oconsiderabl e variabilit y (Dunning an dSchwarz , 1981 ; RyanandDunning , 1981) . Accordingly , th e reade r i s reminde dtha t th e appropriatenes s o f th e dos e estimate s presente dher e may be ope nt oquestio ninsuchsituations . I nmany situation s (e.g. , inoptimizatio ntechnique s o r fo r com parison s wit hothe r radiationinsults) , i t may be desirabl e t oobtai na singl e valu e t oestimat e the ris kincurre dfro m aradiatio nexposure ; th e effectiv e dos e equivalen t (ICRP , 1977 ) may be usefu l inthi s con text . Th e reade r i s referre dt oAppendi xBfo r adiscussio no f thi s quantity , a s wel l a s tabulation s o f the estimate dvalue s fo r eac ho f the 14 2 radionuclide s considere dinthi s report .

## P.1 4



# METABOLI CMODEL S Metaboli c model s an

dparameter s usedfo rcalculation s inthi s repor t ar esummarize dinTable s 2 an d3 . Fo reac helement , Tabl e2 list s th efractiono f activit y enterin gth ebloodwhic hi s assume dt obe transferre dt ovariou s sourc eorgan s inthebody ; tha t radioactivit y whic hi s no t explicitl y

deposite dinaparticula rsourc eorga no rlos t t oearl y excretio ni s uniforml y

distribute dinacomplementary compart men t denote da s "OTHER. " Foreachelemen t o f concer nTabl e3 present s theassume dcoefficient s an dbiologica l half-lives fo reac hexponentia l ter m inorgan-specifi c retentionequation s o f thefor m M. 3



# wher e \

r


# . - radioactivedecay

constan t fo rnuclid ei

(day - 1 

# ) , 1st •Im 

# A.. , = biologica l remova l rat econstan t fo rnuclid ei %3 

# incompartmen t k

o f orga nj

(da y ) , C. ., = dimensionles s fractiona l coefficien t fo rth ek-th 3 

# exponentia l term , M.= numbe ro f exponentia l terms fo rorganj , t / 

# <•?••/._. ) = 

# thefractiono f aninitiall y deposite dquantit y

o f t J 

# ^ ° ' nuclid ei

tha t remain s inorga nj afte rt days . I neac hcase , reference s ar eprovide dt oindicat eth eorigi no f th e metaboli c dat alisted . Th eparameters show

ni nTabl e3 fo rnobl egase s ar eusedher et o represen t onl y

th eretentiono f ga s produce din situ invariou s organ s o f thebody . Translocatio no f nobl egase s t osystemi c organ s fro m the respiratory

andG I tract s i s neglecte d(i.e. , f-\ = 0) . Ga s i s assume d t oente rtheG I trac t onl y throughingestiono rinhalationo f aprogenito r nuclide ; absorptio no f thega s int obloodfro m theG I trac t i s takent o bezer ointhes ecalculations . Wenot etha t themetaboli c model s i nTable s 2 and3 ar eno t equiva len t t othos eusedinth etw opreviou s volume s o f thi s serie s fo rcertai n radionuclides . Th einpu t dat ausedfo r 90 

# Ydos eestimate s inKillough e t al . (1978a ) wer eincorrect , an dhavebeencorrected . Mor ereasonabl e assumption s concerningthedistributio no f radioactivedaughter s o f 226 

# R aand228 

# R ainbon e(surfac eo rvolumedistribution ) haveyielde dTabl e 2 . Fractiona l uptak e b y sourc e tissue s 

## P.1 5

Elemen t Bon e Live r Kidney s Splee nTeste s Thyroi d Othe r Excretion Sodiu m Phosphorou s Manganes e Iro n Cobal t Zinc Rubidiu m Strontiu m Yttriu m Zirconiu m Niobiu m Molybdenu

m Technetiu

m Rhodiu m Rutheniu m Antimony Telluriu m Iodin e Cesiu m Bariu m Lanthanu m Ceriu m Proseodymiu

m Neodymiu m Promethiu

m Samariu m Thalliu m Lead Bismut h Poloniu m Astatin e Franciu m Radiu m Thoriu m Uraniu m Actiniu m Protactiniu

m Neptuniu

m Plutoniu m Americiu m Curiu m Californiu

m 

### 0. 3

0. 3 0.3 5

• 

### 0. 2
1.0 * 

### 0. 5 0.4 5 0.35 7 0.1 5

0.0 2

1.0 * 

### 0. 4

0. 4



## \.<f

0.17 2 0.7 0 0.2 2 

# \ 

# I f \

_0.4 5 

# 1 0.2 5

0.0 8 0.0 7

0.1 5

0.5 7 0.0 8

0.05 5



### 0. 4

0. 5

1.0 = 

### 0. 1

0.0 4

0.4 5 8.55E- 3

0.0 6 0.0 1

0.03 4

0.0 5

0.02 5

0.0 4 1.0 s 

### 0. 4 0. 1

0.1 2

0.0 1 0.01 3

5.0E- 3 1.23E- 3

0.3 3

0.0 1

0.0003 5 

### 0. 7 0.5 5 

### 0. 4 0.90 7 0.4 3 

### 0. 8 1. 0 i.e * 

### 0. 1 0.5 5 0.52 8 0 2 2 0.8 9 

### 1. 0 1. 0 1. 0 0.4 2 0.6 7 

### 1. 0 1.0 " 

### 0. 1

0.0 5

0.9 6 1.0 ° 

### 0. 6 0. 7 0.9 9 

### 1. 0 0.91 3 0.1 6 0.1 2 0.1 5



### 0. 5

0.2 5

0.4 7

0.0 5

0.02 5

0.1 0 0.5 4 Killoughe t al . 1978 -

ICRP 197 9 ICRP 197 9 Killoughe t al . 1978 1 USNR C197 5 Killoughe t al . 197 8 USNRC197 5 ICRP 1972a : ' USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 USNRC197 5 ICRP 1972a * USNRC197 5

USNRC197 5

Li e e t al . 196 0 Bernard197 7 Rus s e t al . 197 5 ICRP 197 9 Hamilto ne t al . 195 3 ICRP . 1979 ^ ICRP 1972 a ICRP 197 9 ICRP 197 9

0.0 5 0.0 4 ICRP 1972b , USNRC197 5

a 0nl y key reference s ar e citedhere . Mor e detaile ddescription s o f metaboli c dat a an dreference s for eac helemen t ma y be foun

di nthe previou s tw ovolume s o f thi s repor t series . "Metaboli c mode l i s derive da s exponentia l fi t t oICRP Publication2 0 retentionmode l for alkalin e earths . Retentionequation s ar e no t normalize dt ounit y

a t tim e 0 . ^Mamillary

mode l wit hnon-normalize dretentio nequations ; fl • 1 . Franciu m i s assume dt ofollow cesiu nmetaboli c behavior . 'Fractiona l uptak e fo r ovarie s 1 s 0.00011 .

## P.1 6

*#3l f 1 . Retentio noaraneter s fo r sourc e tissue s Elemen t Sodiu m Phosonorou s
Manganes e

Iro n Coba1 t Zin c
Krypto n RuDidiu m Strontium
iterium Zirconiu m
Niooiu m Molybdenu m Tecnnet.u m Rutheniu m Phodiu m Antimon y Tellurium

Iodin e

xeno n Cesiu m Barlu n
Lanthanu m Ceriu m J Praseodymiu m

1 Neodymiu m

1 Promethiu m Samariu m

. Tria l 1 iu m Lea d

Bismut n
Poloniu m Astatin e
Rado n
Franciu m Radium
Thorium
Uraniu m
Actiniu m Protactiniu m Neptuniu m Plutoniu m Americiu m Curiu m Californiu m Souree/Orga n

Tota l Bod y
• Bon e Othe r Bon e Live* - Othe r Tota l Bod y Tot* : Bod y Bon e Otne r

Tota l Boc y Bon e Otne r Tota l Bod y Bon e Othe r Tota l Bod y Tota l Bod y Tota l Bod y Tota l Bod y Tota l Bod y Tota l Bod y Bon e Live* " Sidney s Othe r Tnyroi d Othe r

Tota l Body Bon e Otne r

Tota l Bod y

Bon e L i ve r Kidney s Otne r Kidney s Othe r Thyroi d Othe r Bon e Othe r

Bon e Otne r Bon e Othe r Bon e Othe r

' Bon e i Liver , Kidney s Gonad * Othe r c i

1* 0 1. 0 0.2 7

'-.-- • t 4 0. 5

.. 0 0. 6 1. 0 O. i 1.5E- ) 1. 0 -U.S2 5 0.989 ' 1. 0 1. 0 0. 9 0. 5 0.1 5 0.7 « 0.1 5 0.6 7 0.3 5 1. 0 1. 0 1. 0 0.7 6 0.0 5 0.99 7 2.96E- 3 0.1 3 -0.55 5 0.98 4

1. 0

1. 0 -0.32 3 •C.10 4 -5.09E- 2 -3.23E- 2 -0.0 2 0.3 5 0.0 1 -1.9 4 0.29 3 0. 7 0.87 2 0.1 3 0.8 8 0.8 9 1. 0 1. 0 0. 9 0.99 6

1. 0 1. 0 1. 0 1. 0 

# V

15

2 4 0 4 4 200 0 6 40 0 2 0 I.34E- 2 I 1.1 9 3.3 3 800 0 800 0 7 6 1 1. 5 0.34 7 3 1 800 3 10. 2 2 3 9. 2 11. 3 0.24 3 5.2E- *

.*•' • 0.9 6 1.2 4

500 0

4 

# • 1 1 

# ; 0. 1 C l 0. 5 0. 2 0. 2 2.65E- 4 2.65E- 4 1. 4 5.6 8 0.6 3 800 0 70 0 2 0 6

3.6SE 4 1.46E 4



# - 3.65E 4 

# ~

C.-s

O. i O. i 

# o. :

C. 7 2.89E- 3 0. 9 0.4_ 4 

## o.o n

0. 1 0. 5 0.8 5 

## 6. 2 0. 4 0.3 3 0.1 5

0.2 4 0.9 5 •0.048 7 5.39E- 3 0.8 7 0. 5 C.CI 6

-6.24E- 2 8.9JE- 2 4.90E- 2 -6.24E- 3 1.0 2 0.1 5 0.9 9 2.9 4 0.70 7 0. 3 9.14E- 2 0.8 7 1.36E- 2 7.09E- 2

0. 1 0.00 4 < 2

19

4 0 4 0

6 0

40O 6.84E- 2 9 5 3._ 3 97 1

800 0 20 0 5 0 3. 7 9. 9 20 0 10 0

17. 7 117 11. 3 3.42E- 3 135 1.2 4 43 3

10 10 1 0 1 0 5.7 8 5.7 8 50 3 0 3 0



# - 3.UE 135 24 0 28. 9

500 0 150 0 C 3

0. 2

2.0JE- 2

-0.061 3

0.0 4 0.2 5

0.051 4 3.9*1- 2

0.03 ' 0.000 1

0.21 1 8.34E- 3 1.0TE- 3 0.21 1

•_.05E- 2

5.73E- 2 3.34E- 2 l 3

80 0

3.51E- 2

5.7 8

2 2 5 8

117 V.75E- 2

43 3 385 0

32 0 3: 0 22 0 32 g

2.88E- 2

149 0 16 0 C 4

9.22E- 2

0.062 3

0. 2

9.23E- 2

0.02 5

0.17 4 4.25E- 3 4.89E- 4 1.74E- 2

9.08E- 3

2.03E- 3 7.43E- 3 <4

C.32 2

97 1

173 0

0.16 1

385 0

20C 0 200 0 200 0 200 0

0.14 6

161 0 77 6 C S

0.74 4

0.0 8

0.91 4

0.17 7 4.05E- 3 4.22E- 4 1.77E- 2

6.79E- 3

4.60E- 2 7.94E- 4 l 5

3.7 8

666 0

1.8 7

300 0 800 0 800 0 800 0

0.96 3

838 0 404 0 References 0

Klllouo he t al . 1978 a ICRP 197 9

I CR f 197 9

Killougi . e t al . 1978 a USNRC 197 5 Killoug he t al . 1978 a

Bernar dS Snyde r 197 5 USNR C197 5 ICR P 1972a *

USNR C197 5 USNR C197 5

USNR C197 5 USNR C197 5 USNR C197 5 USNR C197 5 USNR C197 5 USNR C197 5 USNR C197 5

USNR C197 5

Bernar d1 Snyde r 197 5 USNR C197 5 ICR P 1972a *

USNR C197 5

li e e t al . 196 0 Bernar d197 7

Rus s e t al . 197 5

ICR P 197 9 Hamilto ne t al . 195 3

ICR P 195 9 Bernar d
_Snyde r 197 5 ICR P 1979 ' ICR P 1972 a

ICR P 197 9

ICR P 197 9

ICR P 1972b , USNR C197 1

^Onl y key reference s ar e cite dhere . Mor e detaile ddescription s o f metaboli c dat a an dreference s fo r eac no f the element s may be foun

dinth e previou s tw

o volume s o f thi s repor t series . ^Exponentia l fit s t o ICRP (1972a ) retentio nequations . Equation s ar e no t normalize dt o unit y a t time 0 Inal l cases . Whe nth e elemen t occur s a s a daughte r I n* deca y even t inth e oody , tr. e appropriat e retentio nequatio nmus t b e normalize danduse di nconjunctio nMit ha n/"j .
"Francmm

i s assume dt o follow cesiu m retentio nbehavior . 

# 1 0

## P.1 7



# estimate s o f dos e t oendostea l surface s an dredmarrow

muc hlowe r than thos e give npreviousl y (Dunninge t al. , 1979) . I nthe revise destimates , eac hdaughte r i s assume dt obe distribute duniforml y throughou t the bon e volume base do

nth e distributio no f the radiu m parent ; thi s i s tantamoun t t oassumin gtha t th e bul ko f th e daughters ' contributio nt odos e i s fro m tha t fractio no f th e daughte r activit y produce din

situ inth e bone . I

n th e previou s estimates , eac hdaughte r wa s accorde dit s independen t depositio ncharacteristics , a s i f i t hadbeendeposite dinth e bon e directl y

fro m blood ; thi s approac hwoul dsignificantl y overestimat e th e dos e contributio nfro m daughter s produce di nthe bon e fro

m radioactiv e decay . Finally , th e metaboli c model s fo r thoriu m an duraniu

m isotope s hav e bee nrevise dbase do ndat a inICR P Publicatio n3 0 (ICRP , 1979) .



# 1 1

## P.1 8



# RSFERBKf S
Bernard , S . R. , 1968 , " A Mode l fo r Estimation1 

# , o f Mea nActivit y Presen t inSegment s o f th e Gastrointestinal . Trac t a t Any Time Pos t Ingestion, " Health. PhysicsDivision Anmrnl 'Psogpess. Report

for Period Ending 'July Sl, 1965, ORNL-4316 , pp . 283-2S7 . Bernard , S . R. , 1977 , "Dosimetri c Oat a msLMetaboli c Mode l fo r Lead, " HealthPhys. 32_ , 44 . Bernard , S . R . andW . S . Snyder , 19-75 * "Metaboli c Model s fo r Estimatio no f Interna l Radiatio nExposur e Received ! b y Huma nSubject s fro

m the Inhalatio

n o f Nobl e Gases, " kealtliPhysiosDivision Annual Progress Report, Period

Ending June 20, 1975; 0RN1L-5046 . Dunning , D . E. , Jr , S . R . Bernard , P . J . Walsh , G . G . Killough , and J . C . Pleasant , 1979 , Estimatesof Internal

Dose Equivalent

to 22 Target

Organsfor

RadionuclidesOccurring in Rouvine Releases fromNuclear

Fuel Cycle Facilities,. Vol. II, 0RNL/NUREG/TM-190/V2 . Dunning , D . E. , Jr . an dG . Schwarz , 1981 , "Variabilit y o f Huma nThyroi d Characteristic s andEstimate s o f Dos e fro m Ingested131 

# I , " Health Phys. 40 , 661 . Dunning , D . E. , Jr. , J . C . Pleasant , andG . G . Killough , 1980 , SFACTOR: •A Computer

Code for

Calculating Dose Equivalent to aTarget

Organ per Microcurie-DayResidence of aRadionuclide in aSource Organ

- SupplementaryReport, 0RNL/NUREG/TM-85/S1 . Eve , I . S. , 1966 , " A Review o f th e Physiology

o f th e Gastrointestina l Trac t inRelatio nt o Radiatio nDose s fro m Radioactiv e Materials, " HealthPhys. 1_2 , 131 . Hamilton , J . G. , C . W . Asling , W . M . Garrison , an dK . G . Scott , 1953 , "The Accumulation , Metabolism , andBiologica l Effect s o f Astatin e inRat s andMonkeys, " Univ . o f Californi a Publication s inPharma cology , Univ . o f Californi a Press , Berkele y an dLo s Angeles . Internationa l Commissio no nRadiologica l Protectio n(ICRP) , 1959 , Report of Committee 2 on Permissible Dose for Internal

Radiation, Publicatio n2 , Pergamo nPress , Oxford . Internationa l Commissio nonRadiologica l Protectio n(ICRP) , 1972a , Alkaline EarthMetabolismir. Adult Man, Publicatio

n 20 , Pergamo

n Press , Oxford . Internationa l Commissio nonRadiologica l Protectio n(ICRP) , 1972b , The Metabolismof

Compoundsof

Plutoniumand

Other Actinides, Publicatio n19 , Pergamo nPress , Oxford .



# 1 2

## P.1 9



# Internationa l CommissiononRadiologica l Protection(ICRP) , 1977 , Annalsof

the ICRP1_

, 1 , Publication26 , PergamonPress , Oxford . Internationa l CommissiononRadiologica l Protection(ICRP) , 1979 , 

# Limitsfor

Intakesof

RadionuclidesbyWorkers, Publicatio n30 , PergamonPress , Oxford . Killough , G . G. , D . E . Dunning , Jr. , S . R . Bernard , an d J . C . Pleasant , 

# 1978a , Estimatesof

Internal Dose Equivalent

to 22 Target

Organs for RadionuclidesOccurring inRoutine ReleasesfromNuclearFuelCycle Facilities, Vol. I, ORNL/NUREG/TM-190 . Killough , G . G. , D . E . Dunning , Jr. , an d J . C . Pleasant , 1978b , 

# INREM II: A Computer

Implementationof

Recent Modelsfor

Estimating the Dose Equivalent

to Organsof

ManfromanInhaled

or Ingested Radionuclide, NUREG/CR-0114 , 0RNL/NUREG/TM-84 . 

# Kocher , D . C , 1977 , Nuclear DecayDatafor

RadionuclidesOccurring in Routine ReleasesfromNuclear Fuel Cycle Facilities, ORNL/NUREG/TM-102 . Lie , R. , R . G . Thomas , an d H . K . Scott , 1960 , "Th e Distributionan

dEx
cretiono f Thallium-20 4 inthe Rat , withSuggested MPC s an d a Bioassa

y Procedure, " HealthPhys. 2_, 334 . ^Morrow , P . W. , D . V . Bates , B . R . Fish , T . F . Hatch , an d T . T . Mercer , 1966 , "Depositionan d RetentionModel s fo r Interna l Dosimetr yo f the Huma

nRespirator

yTract, " HealthPhys. 1_2 , 173 . Russ , G . A. , R . E . Bigler , R . S . Tilbury , H . Q . Woodard , an d J . S . Laughlin , 1975 , "Metaboli c Studie s wit hRadiobismut hI . Retention and"Distributiono f 206 

# B i inthe Norma l Rat, " Radiat. Res. 63 , 443 . Ryan , M . T . an

dD . E . Dunning , Jr. , 1981 , A Comparisonof SOYear

and 

# 70Year Internal Dose ConversionFactors, 0RNL/TM-7415 . Snyder , W . S. , M . R . Ford , G . G . Warner , an d S . B . Watson , 1974 , 

# A Tabulationof

Dose Equivalent

per Microcurie-Dayfor

Source and Target Organsof

anAdult

for VariousRadionuclides, Part 1, ORNL-5000 . U . S . Nuclea r Regulator yCommission(USNRC) , 1975 , Reactor Safety 

# Study— AnAssessment

of Accident

RisksinU.S. Commercial Nuclear Power Plants, WASH-140 0 (NUREG-75/014) .



# 1 3

## P.2 0



# APPENDI XA Tabulation s o f Committe dDos e Equivalen t t o2 2 Targe t Organ s o f aReferenc e Adul t fro m Uni t Inhalatio nan

dIngestionExposure s



# 1 5

### NUCLID E H - 3 

### C-1 4 NA-2 2 is —22
•4N-S 4
FE-S S
FE-5 9
CO-5 7
CO-S 9
CO-6 0
2N-6 5

RB-8 6 SR-8 9
SR-9 0
SP-9 1
Y-9 0 Y-9I M Y-9 1 ZP-9 5
ZP-9 7 S O L



# • * 0 0 

### w 0 

### w



# - V M V 

### w Y 

## • Y W Y 0 W V 0 0 Y 0 Y O Y W 

### w

m W Y W Y F l 

### 0.9 S 0.9 S 0.9 5 0.8 0 0.8 0 I.OOE-O I I.OOE-O I I.OOE-O I l.OOE-O I I.OOE-O I I.OOE-O I S.00E-0 2 5.00E-0 2 S.00E-0 2 5.00E-0 2 5.00E-0 2 5.00E-0 2 O.S O O.S O O.S O 0.9 S 0.2 0 

## i.ooe-0 2 0.2 0 1.006-0 2 0.2 0 I.OOE-0 2 1.006-0 4 I.00E-O 4 I.OOE-0 * 2.00E-0 3 2.00E-0 3 2.00E-0 3 2.00E-0 3 AMA D

» • • 

# •* * 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 

### LUNG S

1 .25E-0 4 6.18E-0 6 I.15E-0 2 1.29E-0 2 0.1 6 4.97E-0 3 4.146-0 2 5.47E-0 3 4.34E-0 2 9.536-0 2 0.1 4 2.S4E-0 2 0.1 1 4.99E-0 2 0.1 0 0.2 2 j 2 . 2 

### 1.24E-0 2 3.76E-0 2 0.1 3 1.296-0 2 I.11E-0 2 0.5 4 I.70E-0 2 I S . 

### 7.08E-0 3 1.I8E-0 2 5.82E-02 * 2.70E-0 4 0.3 4 0.1 2 0.2 2 2.65E-0 2 2.74E-0 2 PE S LY M

2.406-0 4 1.326-0 5 S.21E-0 2 0.1 5 0.3 4 5.696-0 3 3.80E-0 2 2.7IE-0 2 0.S 9 0.2 2 0.2 7 9.73E-0 2 0.5 8 0 . 1 t 0.1 9 0.7 0 2 1 . 

### 1 .3*56-0 2 6.30E-0 2 0.2 7 0.1 5 0 . 1 3 1 . 3 

### 0.2 5 4.75 E 0 2 4.926-0 2 I.74E-0 2 7.07E-0 2 8.046-0 4 1 . 3 

### 0.3 9 0.5 9 2.77B-0 2 2.77E-0 2 S

1 . 7 . S . 1 . 9 . 3 . 6 . 9 . 1 . 6 . 7 . 

### 1 . 3 . 4 . 8 . 2 . 0 . 1 . 1 . 1 . 4 . 

### 1 . 8 . 1 . 4 . 2 . S . 9 . 7 . 

### 1 . S . 9 . 1 . 

### 1 . TOTA L INHALATIO N DOSE S

ALPH A0 *

2 0 (PEM/HICPOCUPIE I
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## i.asE-o s 4.36E-0 4 5.27E-0 4 2.62E-0 3 2.07E-0 4 8.77E-0 3 2.02E-0 6 7.23E-0 8 1 .836-0 * 3.5IE-0 0 1 .136-0 3 1.936-0 3 8.96E-0 S I.52E-0 3 2.76E-0 5 8.556-0 * I.06E-0 5 I.S3E-0 3 4.36E-0 S 8.42E-0 5 5.S5E-0 5 t.336-0 5 2.89E-0 5 8.70E-0 S 3.086-0 2 I.1SE-0 5 4.6IE-0 3 I.31E-0 2 S I WAL L

1 4 3 1 1 6 6 

## a 6 i 2 7 1 1 3 3 1 3 1 2 1 1 3 1 3 3 1 2 6 3 3 1 4 1 .68E-0 3 .58E-0 7 .10E-0 5 .42E-0 4 .24E-0 3

. » 76-0 6 .786-0 6

. 6 3E-0 6 •38E-0 5

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. 1 16-0 3 .246-0 6 .096-0 3 .55E-0 S .50E-0 3 .726-0 5 .016-0 5 .99E-0 6 02E-O S .306-0 2 .44E-0 6 .686-0 3

. 4 0E-0 2 U L I WAL L

2 3 2 2 S 9 1 5 4 3 6 3 T 5 I 4 7 1 4 1 1 3 1 2 4 3 1 2 7 3 3 8 4 . 1 . .976-0 3 .66E-0 7 .39E-0 5 .27E-0 4 .66E-0 3 .086-0 6 .086-0 5 .I0E-0 5 .96E-0 * .68E-0 3 .56E-0 4

•73E-0 2

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S 7 5 1 1 6 7 1 1 8 7 0 1 1 3 B 1 2 4 3 2 5 5 7 4 3 1 1 4 2 3 . 2 4 . 1 . .166-0 3 .926-0 8 .I7E-0 6 .916-0 4 .35E-0 2 .74E-0 6 .236-0 6 .536-0 4

. 4 9E-0 3 .436-0 3 2 86-0 * . 1 1 .14E-0 7 .156-0 6 ,236-0 3 .78E-I 0 .836-0 2 .38E-0 2 .38E-0 4 ,0*6-0 2 .956-0 6

. 1 16-0 3 .46E-0 7

•28E-0 3 02F-0 5 22E-0 S 22E-0 S .76E-0 5 I4E-0 6 836-0 5 49E-0 2 56E-0 S 98E-0 3 49E-0 2 TBOO Y

3.036-0 3 4 . I4E-0 7 2.I6E-0 5 7.53E-0 4 S.8IE-0 4 C.48E-0 6 I.OOE-O S 1.736-0 4 1.416-0 3 3.096-0 3 9.S3E-0 5 0.1 0 9.40E-0 7 8.216-0 8 I.27E-0 4 3.23E-0 T 1.136-0 3 3.64E-0 3 5 . I2E-0 S 4.616-0 3 1.716-0 5 C . 7IE-0 4 1.086-O S 1.99E-0 3 1.936-0 3

« . 016-0 4 7.46E-0 3 2.I6E-0 4 i 3.326-0 5 I.54E-0 4 4.32E-0 2 4 . 176-0 3 5.70E-0 3 3.106-0 2 ADPE N

4.I7E-0 3 3.43E-0 7 I.17E-0 S 5.89E-0 4 I.88E-0 4 I.29E-0 S 1 .34E-0 5 2.3*6-0 4 2.016-0 4 3.046-0 3 S.42E-0 5 I.47E-0 2 1.176-0 8 1.876-0 8 3.33E-0 S 2.566-0 8 6.83E-0 4 2.48E-0 3 3.40E-0 S 3.606-0 3 6.I2E-0 6 8.546-0 4 5.04E-0 6 2.47E-0 3 3.616-0 4 I.I6E-0 4 6.25E-0 S 1.196-0 * 3.16E-0 S I.16E-0 4 e.l7E-0 2 7.08E-0 3 8.0IE-0 3 4.75E-0 2 B L WAL L

4 1 8 1 7 4 2 I 1 3 1 3 2 5 1 8 2 1 1 1 2 3 . 1 . 9 . 2 3 . 1 . 3 . 6 . 3 . 4 . 3 . 6 . 3 . .646-0 4 .826-0 8 .46E-0 7

•73E-0 4 .77E-0 S .47E-0 6 .08E-0 6 .17E-0 4 .00E-0 4 696-0 * 12E-0 5 .92E-0 3 00E-0 9 •73E-0 9 59E-0 5 73E-I 0 73E-0 * 22E-0 3 77E-0 S 73E-0 3 91E-0 6 91E-0 4 4 3E-0 6 23E-0 4 07E-0 4 10E-0 5 2IE-0 S 71E-0 S 25E-0 6 I2E-0 5 836-0 2 546-0 3 27E-0 3 I2E-0 2 KIDNEY S

I.92E-0 3 1.54E-0 7 S.65E-0 6 7 . 4 8E-0 3 3.026-0 * 9.436-0 6 6.52E-0 6 3.386-0 4 2.9IE-0 4 I.44E-0 3 3.00E-0 5 I.03E-0 2 4.47E-0 9 9.316- 0 9 2.06E-0 5 1.11E-0 8 4.5SE-0 4 9.J7SE-0 3 4.82E-0 5 1.I7E- 0 2 9 . 886-0 6 7.S56-0 4 5.006-0 6 2.69E- 0 3 4.22E-0 4 1.4SE- 0 4 4.90E-0 5 8.44E-0 S I.84E-0 5 7.87E-0 5 6.42E-0 2 7.08E-0 3 8.ISE-0 3 4.86E- 0 2 LIVE R

4 3 1 1 5 1 1 4 3 3 5 1 2 1 3 2 6 1 1 2 4 6 4 2 . 4 . 1 . 7 1 . 3 . 1 . 6 . 7 . 

## a . 4 . .13E-0 3 .39E-0 7 .166-0 5 .266-0 2 .306-0 4 .626-0 5 .406-0 5 .64E-0 4 .98E-0 4 .00E-0 3 .56E-0 5 .46E--0 2 ,486-0 8 .966-0 8 .49E-0 5 53E-0 8

•43E-0 4 SOE-0 3 .496-0 5 I9E-0 3 04E-0 6 73E-0 4 2 0 6-0 6 30E-0 3 4IE-0 4 97E-0 4 90E-0 5 19E-0 4 26E-0 5 27E-0 4 63E-0 2 0 8 E-0 3 5 7 E-0 3 96E-0 2

## r o

o NUCLIO C

NB-9 5 NB-97 M NB-9 7 MO-9 9
TC-99 M
TC-9 9

PU-10 3 RU-10 5 RU- I 0 6 RH-I03 M RH-I05 M PH-10 5 RH-10 6 SB-12 7 TE-I27 M TE-12 7 TE-129 M TE-12 9 T6-I3I M TE-I3 I TE-13 2 1-12 9 1-13 1 1-13 2 1-13 3 1-13 4 1-13 5 CS-13 4 CS-13 S CS-13 6 CS-13 7 S C L

Y Y Y D Y O W D W V V V Y Y Y V W 

## w w w w w w w D D O 0 D D 0 0 D 0 F l

1.00E - I.O0E - - 0 2

- 0 2 1.00E-0 2 0.9 5 5.006 - 

## o.a o 0.8 0 0.8 0 0.8 0 4.006 - 4.006 - 4.00E - 4.00E - 4.006 - - 0 2

- 0 2 - 0 2 - 0 2 - 0 2 - 0 2 4.00E-0 2 4 . OOE * 5 . 006 - 0.2 3 0.2 5 0.2 5 0.2 5 0.2 5 0.2 5 0.2 5 0.9 5 0.9 5 0.9 5 0.9 5 0.9 5 0.9 5 0.9 S 0.9 S 0.9 5 0.9 5 - 0 2

- 0 2 AMA D

0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 OVARIE S

1.32E-0 3 4.42E-0 8 2.276-0 6 3.I4E-0 4 2.33E-0 4 6.6IE-0 6 4.06E-0 6 2.3*6-0 4 2.0IF-0 4 9.556-0 4 3.74E-0 5 7.77E-0 3 6.79E-0 9 1 .87E-0 8 5.20E-0 5 I.75E-0 9 7.5IE-0 4 2.44E-0 3 3.386-0 5 3.44F-0 3 5.28E-0 C 3.67E-0 4 2.48E-0 6 1 .696-0 3 3.55E-0 4 3.80E-0 5 I.56E-0 5 6.IIE-0 S 9.3IE-0 6 4.64E-0 S 6.116-0 2 7.086-0 3 7.61E-0 3 4.73E-0 2 PANCREA S

4 3 1 5 2 1 1 2 2 3 t 1 I 2 3 2 7 2 3 3



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5 . 1 . 1 . 9 . 8 . 2 . 2 . 1 . 

## z: i . i . i . 

### i . i . 3 . j . 5 . 1 . 1 . 3 . 2 . 1 . 5 . 2 . 4 . 9 . 1 . 7 . 5 . 7 . 6 . 4 . TOTA L INHALATIO N DOSE S

ALPH A0 - ° 2 0 (HEM/MICROCURIE ) IN E R MA R YMA P 83E-0 3 2.366-0 3 1.9IE-0 3 

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### 1.016-0 3 1.44E-0 7 5.03E-0 6 I.03E-0 3 1.26F-0 4 9.566-0 6 8 . 3 36-0 6 3.03E-0 4 2.60E-0 4 1.356-0 3 2.476-0 5 I.136-0 2 I.5IE-0 8 1.136-0 3 1.9'iE-O S I.066-0 8 3.97E-0 4 2.77F-0 3 1 .97E-0 5 ?. . 70E-0 3 3.75E-0 6 4.7IE-0 4 3.0SE-0 6 I.50E-0 3 S.326-0 4 2.ISE-0 4 4.22E-O S 1.026-0 4 I.86E-0 5 8.316-0 5 S.586-0 2 8.166-0 3 6.73E-0 3 5.03E-0 2 .836-0 3

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•97E-0 4

. 7SE-0 4 .216-0 5 •24E-0 5 .3*6-0 * .016-0 4 .716-0 3 .286-0 5

. 38E-0 2 .886-0 8 

## .aiE-o a .296-0 5

• 27E-0 8

• S7E-0 4

•53E-0 3 •4IE-0 5 .61E-0 3 .126-0 6 .88E-0 4 .856-0 6 •4SE-0 3

. 796-0 4 .666-0 5 .S3E-0 5

. 1 16-0 4 .016-0 5 .I4E-0 4 .216-0 2 .086-0 3 .996-0 3 .786-0 2 .0*6-0 *

.84E-0 9 .206-0 7 .74E-0 4 .0*6-0 5 .07E-0 6

•53E-0 6

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• 87E-0 3 .206-0 2 THYMU S

6.68E-0 3 5.43E-0 7 I.806-0 5 3.99E-0 4 2.72E-0 4 I.99E-0 S 2 . 1 IE-O S 2.34E-0 4 2.0IE-0 4 4.48E-0 3 8.0IE-0 5 I .666-0 2 I.616-0 8 2.7IE-0 8 4.5IE-0 5 4.05E-0 8 9.61E-0 4 2,-ME-0 3 3.46E-0 S 3.886-0 3 6.846-0 6 I.516-0 3 8.456-0 6 4.34E-0 3 9.24E-0 4 7.12E-0 4 I .086-0 4 2.316-0 4 5.S2E-0 5 2.40E-0 4 7.33E-0 2 7.08E-0 3 6.38E-0 3 5.36E-0 2 THYPOI O

.266-0 3 •82E-0 7 .026-0 6

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6.27E-0 4 3.1*6-0 8 1.656-0 6 3.486-0 4 1.146-0 4 9. 4 7E-0 6 4.43E-0 6 2.34E-0 4 2.01E-0 4 5.276-0 4 2.0 9 6-0 5 4.91E-0 3 «.9*6-0 9 8.44E-0 9 2.336-0 5 1.2 0 6-0 9 4.6IE-0 4 2.4SE-0 3 3.39E-0 3 3.346-0 3 S.466-0 6 I . 1 06-0 3 3.I0E-0 6 2.666-0 3 4.S2E-0 4 3.78E-O S 1.586-0 5 7.02E-0 5 I.2SE-0 5 6.19E-0 S 9.S5E-0 2 7.086-0 3 8.46E-0 3 C.20E-0 2TOTA L INHALATIO N DOSE S ALPH AQ » 2 0 (REM/MICROCURIE t



## r o

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BA-I37 M BA- I 4 0 L A- l 4 0 CE-14 1

CE-14 3

CE-14 4

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3R-I44 M

PR-14 4

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SM-14 7 SO L

D 0 W Y W 0 Y W 0 Y W 0 Y W D Y W D Y W D Y W 0 Y



# - O Y W D F l

I.OOE-O I I.OOE-O I 1.006-0 4 1 . 006-0 4 I.OOE-0 4 1.006-0 * 1.006-0 4 I.OOE-0 4 1.006-0 4 1.OOE-0 4 I.OOE-0 4 1.006-0 * 1.006-0 * I.006-0 4 1.006-0 4 I.OOE-0 4 I.OOE-0 4 1.006-0 * 1.006-0 * 1.006-0 4 I.OOE-0 4 1.OOE-0 4 t.OOE-0 4 I.006-0 4 I.OOE-0 4 t.OOE-0 4 1.006-0 * t.OOE-0 4 I.OOE-0 4 I.OOE-0 4 AMA D

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7.00E-0 6 1.636-0 2 2.8IE-0 2 0.1 1 7.15E-0 2 3.98E-0 3 2.3SE-0 2 2.I8E-0 2 6.29E-0 3 S. O 1 . 2 2.80E-0 2 8.60E-0 2 7.11E-0 2 5.8*6-0 3 2.736-0 4 2.586-0 4 2.21E-0 4 6.34E-0 4 6.096-0 4 S.386-0 * 6.66E-0 2 5.436-0 2 5.S0E-0 3 0.5 0 6.216-0 2 1.20E-0 3 2.27 E 0 2 2 3 . 0.3 8 RE S LV M

7.16E-0 6 0.1 8 3.12E-0 2 0.2 1 0.2 1 3.8SE-0 2 2.7IE-0 2 3.01E-0 2 S.7SE-0 2 3 9 . 6 . 1 0.3 0 0.1 2 0.1 5 6.70E-0 2 2.73E-0 * 2.58E-0 4 3.03E-0 4 6.34E-0 4 6.09E-0 4 6.77E-0 4 0.1 4 0.1 0 5.70E-0 2 7 . 5 0.3 5 I.42E-0 2 I.63 E 0 4 1.26 6 0 2 S . O S WAL L S I WAL L U L

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•S7E-0 8 .226-0 3 •IOE-0 3 .806-0 3 .99E- 0 3 •ISE-0 3 .03E-0 3 .306-0 3 .06E-0 3 .316-0 2 .656-0 2 .IIE-0 3 .226-0 3 .94E-0 3 .146-0 4 •3IE-0 7 .156-0 7 .096-0 6 .9IE-0 7 .436-0 7

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2.36E-0 8 7.60E-0 3 1.336-0 2 I.09E-0 2 1.136-0 2 I.75E-0 3 I.05E-0 2 9.03E-0 3 2.04E-O 3 9.856-0 2 0.1 1 1.30E-0 2 1.78E-0 2 1.70E-0 2 2.6IE-0 3 I.99E-0 8 1.66E-0 8 7.14E-0 8 3.0IE-0 8 3.24E-0 8 I.22E-0 7 1.526-0 2 I.43E-0 2 2.39E-0 3 S.28E-0 3 5.33E-0 3 S.60E-0 4 2.18E-0 2 1.98E-0 2 2.216-0 3 T

3 2 1 1 1 3 4 4 

## e 7 6 0 1 1 2 3 4 3 9 . 9 9 1 1 . 2 . 8 . 7 2 . BOD Y •O2E-0 T •3SE-0 3 .IOE-0 3

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3.84E-0 7 2.68E-0 3 8.4IE-0 4 4.73E-0 4 5.25E-0 4 1.516-0 3 I.02E-0 4 1.226-0 4 2.44E-0 4 2.176-0 3 6.29E-0 3 2.75E-0 2 I.07E-0 6 2.96E-0 5 2.48E-0 4 6.106-0 8 9.84E-0 8 1.S5E-0 7 9.28E-0 8 I.47E-0 7 2.46E-0 7 2.99E-0 4 3.67E-0 4 9.9IE-0 4 I.87E-0 4 7.00E-0 4 2.97E-0 3 0.9 5 1 . 6 6 . 5 B L WAL L

2.50E-0 8 I.69E-0 3 3.96E-0 4 4.93E-0 5 8.99E-0 5 3.086-0 4 4.896-0 5 4.69E-0 5 5.986-0 5 3.67E-0 4 2.49E-0 3 1 .136-0 2 S.41E-0 7 1.49E-0 S 1.256-0 4 3.46E-0 9 2.24E-0 8 5.28E-0 8 7.I3E-0 9 3.76E-0 8 9.54E-0 8 6.68E-0 5 8.626-0 5 2.I4E-0 4 9.336-0 5 3.50E-0 4 1.49E-0 3 0.4 8 0.8 0 3 . 3 KIDNEY S

I.77E-0 7 I.63E- 0 3 I.30E- 0 3 2.70E-0 4 2.88E-0 3 1.946- 0 2 7.I2E- 0 5 4.226-0 4 3.09E-0 3 3.04E-0 2 0.2 5 1 . 2 5.846-0 5 1.626-0 3 1.366-0 2 7.946-0 8 I . 4 5E-0 6 3.56E-0 6 I.3OE-0 7 2 . 3 76-0 6 6.4SE-0 6 2.496-0 4 I.68E-0 3 1.236-0 2 1.036- 0 2 3.846-0 2 0.1 6 5 2 . 8 8 . 3.58 6 0 2 LIVE R

3.80E-0 7 1.656-0 3 2.07E-0 3 8.3 9 6-0 * 9.79E-0 3 6.656-0 2 1.5 8 6-0 4 I.37E-0 3 1.066-0 2 0.1 0 0.8 6 4 . 0 2.02E-0 4 5.57E-0 3 4.60E-0 2 2.67E-0 7 4.9 8 6-0 6 1.22E-0 5 3.92E-0 7 8.056-0 6 2.20E-O S 7.3IE-0 4 S.66E-0 3 4.22E-0 2 3.S4E-0 2 0.1 3 0.5 6 1.81 6 0 2 3.03 E 0 2 1.24 6 0 3TOTA L INHALATIO N DOSE S ALPH AO a 2 0 (REM/MICROCURIE I



## r o r o NUCLIO E

SA-13T M 3A- 1 4 0 LA- I 4 0 CE-I4 I

CE- I 4 3

CE-14 4

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O D W Y W D Y W D V 

### w 0 Y W 0 Y tt D Y W 0 Y W D V 

### w D V 

### w 0 F l

I.OOE-O I I.OOE-O I I.OOE-0 4 I.OOE-0 4 I.OOE-0 4 t.OOE-0 4 1.006-0 4 I.OOE-0 4 I.OOE-0 4 1.006-0 * 1.006-0 4 1.OOE-0 4 I.OOE-0 4 1 . 00E-0 4 1.OOE-0 4 1.006-0 4 1.OOF-0 4 I.OOE-0 4 I.OOE-0 4 1.OOE-0 4 1.006-0 4 I.OOE-0 4 I.OOE-0 4 I.OOE-0 4 I.OOE-0 4 I.OOE-0 4 1.006-0 4 I.OOE-0 4 1 . 006-0 4 I.OOE-0 4 AMA D

0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 OVARIE S

4.I2E-0 B 2.67E-0 3 I.09E-0 3 1.556-0 4 2.316-0 4 5.826-0 4 t.82E-0 4 1.636-0 4 1.286-0 4 7.64E-0 4 4.96E-0 3 2.236-0 2 I.07E-0 6 2.96E-0 5 2.486-0 4 6.95E-0 9 4.20E-0 8 9.956-0 8 1.34E-0 8 6.42E-0 8 1 .63E-0 7 2.30E-0 * 2.S7E-0 4 3.866-0 4 I.87E-0 4 7.00E-0 4 2.97E-0 3 0.9 5 1 . 6 6 . S PANCREA S

4 2 1 4 5 1 1 1 2 2 6 2 1 2 2 

### a 1 1 1 1 2 3 3 8 1 7 2 . 0 •42E-0 7 .80E- 0 3 .036-0 3 .79F-0 4 .I2E-0 4 .36E-0 3 .24E-0 4 .37E-0 4

•2IE-0 4 .36E- 0 3

•Of-6-0 3 .616-0 2 .076-0 6 .966-0 5 .486-0 4 ,116-0 8 .146- 0 7 .816-0 7 .266-0 7 •75E-0 7 .84E-0 7 .406-0 * .9IE-0 4 .87E-0 4 •87E-0 * .OOE-0 4 97E-0 3 9 5 

# .( . 6 . 5 BON E R MA R

1.60E-0 7 2.0SE-0 TI 6.36E-0 3 3.99E-0 3 2 7.04E-0 4 7.65E-0 4 4 3.896-0 4 4.I4E-0 4 3 2.72E-0 3 9.33E-0 4 • I.77E-0 2 4.64E-0 3 I 7.26E-0 5 I.056-0 4 6 3.b8E-0 4 2.05E-0 4 8 2.776-0 3 9.68E-0 4 I 2.80E-0 2 I . 1 76-0 2 I 0.2 3 8.876-0 2 5 1 . 0 0.4 1 2 S.38E-0 5 I .656-0 5 1 I.49E-0 3 4.5SE-0 4 Z I.25E-0 2 3.82E-0 3 2 9.696-0 8 7.91E-0 8 5 1.346-0 6 5.836-0 7 9 3.246-0 6 1.356-0 6 I I.23E-0 7 9.44E-0 8 5 2.ISE-0 6 9.21E-0 7 I S.84E-0 6 2.43E-0 6 2 2.98E-0 4 2.84E-0 4 2 I.S9E-0 3 6.02E-0 4 2 I.1IE-0 2 3.IOE-0 3 8 9.94E-0 3 I.056-0 3 I 3.73E-0 2 3.94E-0 3 7 0.1 6 1.686-0 2 2 2.59 E 0 2 0.9 9 O 4.35 E 0 2 1. 7 I.77 E 0 3 6. 8 I MA R .72E-0 7 .616-0 3 .906-0 4 .I2E-0 4 .04F-0 4 .386-0 3 .876-0 5 •33E-0 5 •86E-0 4 •66E-0 3 .82E-0 3 •5TE-0 2 .076-0 6 •96E-0 S .48E-0 4 .47E-0 8 •I2E-0 8 .466-0 7 

### •see-0 8 .07E-0 7

•0IE-O 7 .05E-0 4 •72E-0 4 .4IE-0 4 .87E-0 4 •006-0 4 .976-0 3 . 9 5 

### i. e 6 . 5 ENDOS T

I.62E-0 7 5.826-0 3 6.S2E-0 4 3.65E-0 4 2.146-0 3 1.366-0 2 7.02E-0 5 3.226-0 4 2.23E-0 3 1.906-0 2 0.1 5 0.7 0 4.34E-0 S I.20E-0 3 1.016-0 2 8.086-0 8 9.I0E-0 7 2.186-0 6 9.91E-0 8 1 .456-0 6 3.9IF-0 6 2.646-0 4 1 .246-0 3 8.56E-0 3 6.S5E-0 3 2.466-0 2 0.1 0 3 1 . 5 2 . 2.13 6 0 2 SPLEE N

3.58E-0 7 2.S4E-0 3 7.9IE-0 4 4.316-0 4 3 . 09E-0 4 7 . 156-0 4 I.04E-0 4 1.116-0 4 I.42E-0 4 2.136-0 3 1.336-0 3 2.296-0 2 I.07E-0 6 2.96E-0 5 2.48E-0 4 7.8UE-0 8 l . l IE-0 7 1.66F-0 7 1 . 13E-0 7 1.S9E-0 7 2.536-0 7 2.056-0 4 2.98E-0 4 4.72E-0 4 I.87E-0 4 7 . OOE-0 4 2 . 9 76-0 3 0.9 5 1 . 6 6 . 5 TESTE S

1.636-0 8 2.12E-0 3 1.39E-0 4 1.34E-0 S 7.S6E-0 S 4.S6E-0 4 1 .39E-0 5 2.0SE-0 S 7.866-0 5 5.84E-0 4 4.TOE-0 3 2.IEE-0 2 1.076-0 6 2.96E-0 S 2.48E-0 4 2.44E-0 9 3.73E-0 8 9.096-0 8 4.29E-0 9 5.3IE-0 8 I.48E-0 7 2.I36-0 S 5.386-0 5 2.B7E-0 4 I.87E-0 4 7.OOE-0 4 2.97E-0 3 0.9 5 1 . 6 6 . 5 THYMU S

6.00E-0 7 3.33E-0 3 I.35E-0 3 7.70E-O 4 5.95E-0 4 6.07E-0 4 I.S2E-0 4 1 .586-0 4 1.S2E-0 4 3.48E-0 3 5.S2E-0 3 2.246-0 2 1.076-0 6 2.966-0 5 2.406-0 4 I.33E-0 7 1.63E-0 7 2.03E-0 7 2.07E-0 7 2.516-0 7 3.23E-0 7 4.70E-0 4 4.5IE-0 4 4.48E-0 4 1.87E-0 4 7.OOE-0 4 2.97E-0 3 0.9 5 1 . 6 6 . 5 THYROI D

2.06E-0 / 2.23E-0 3 3 . 59E-0 4 I.55E-0 4 I.72E- 0 4 5.016-0 4 3.876-0 5 4.7IE-0 5 9.64E-0 5 1 . 2 2E- 0 3 4.83E-0 3 2.166-0 2 I.07E-0 6 2.96E-0 3 2 . 4 86- 0 4 2.83F-0 8 t . 186-0 8 1.1IE-0 7 5.87E-0 8 I.07E- 0 7 I.93E-0 7 I.20E-O 4 I.4IE-0 4 3.336-0 4 I.87E-0 4 7.OOE-0 4 2.97E-0 3 0.9 5 1 . 6 6 . 5 UTERU S

4.186-0 8 3.06E-0 3 b.836-0 4 7.37E-0 S 1.486-0 * S.73E-0 4 7.4BE-0 S 7 . 3 4 E-0 5 I.05E-0 4 6.98E-0 4 4.87E-0 3 2.22E-0 2 I.07E-0 6 2.96E-O S 2.48E-0 4 6.686-0 9 4.176-0 8 9.856-0 8 1.306-0 8 C.36E-0 8 I.62E-0 7 9.406-0 5 1.296-0 4 3.59E-0 4 I.87E-0 4 T.OOE-0 4 2.97E-0 3 0.9 3 1 . 6 6 . 5

### TOTA L INHALATIO N DOSE S ALPH A Oa 2 0 (REM/MICROCURIE )



# r o L O NUCLID E

TL-20 7 TL-20 8 TL-20 9 PB-20 9 *»B-2I 0 PB-21 1 *»B-2I 2 PB-21 4 81-21 0 -M-2I I 91-21 2 BI-21 3 81-21 4 PO-21 0

PO-2 M

PO-21 2

<»0-21 3
P0-2I 4

"0- 2 I S
PO-21 6
PO-21 8

AT-21 7 RN-21 9 RN-22 0 PN-22 2 FR-22 1 SO L

W 

## w w w w w w w



# - w w w w w D 

## w D 

## w 0 

## w D 

## w D W D W D W D D 

# * • • 0 F l 0.9 S 0.9 5 0.9 5 8.006-0 2 8.006-0 2 8.00E-0 2 8.00E-0 2 8.00E-0 2 3.006-0 2 5.006-0 2 5.00E-0 2 5.OOE-0 2 5.00E-0 2 I.OOE-O I I.OOE-O I 1.006-0 1 I.OOE-O I I.OOE-0 1 1.006-0 1 l.OOE-O I I.OOE-O I I.OOE-O I I.OOE-O I I.OOE-0 1 I.OOE-O I 1.006-0 1 1.OOE-0 1 I.OOE-O I I.OOE-0 1 0.9 5 0 . 0 0 . 0 0 . 0 0.9 5 AMA D

0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 4 4 4 4 4 4 4 * 4 *0. 3 LUNG S

7.06E-0 5 6.77E-0 S 6.37E-0 5 I.02E-0 3 1 1 . 0.1 4 

# CS) 0.1 2 

### i. a 8.71E-0 3 0.2 7 9.646-0 3 9.086-0 2 7 8 . 1 . 7 4.35E-0 S 4.35E-0 5 2.806-1 1 2.80E-I I 3.6BE-I 0 3.686-1 0 1.316-0 8 1.316-0 6 2.506-0 7 2.S0E-0 7 I.94E-0 S I.94E-0 S 2.44E-0 2 2.37E-0 2 2.S0E-0 6 9.146-0 4 2.166-0 3 2.346-0 3 3.83E-0 2 RE S LY M

7.06E-0 S 6.77E---0 5 6.376-O S 1.036-0 3 1.89 E 0 2 1 .17E-0 3 8.416-0 2 1.396-0 3 B . 2 3.25E-0 S 1.846-0 3 1.586-0 3 7.95E-0 4 3.I0 E 0 2 2 3 . 1.216-1 0 5.536-0 9 4.756-2 4 1.906-2 1 3.63E-1 3 3.63E-1 3 4.39F-I 1 1.736-1 2 9.586-1 0 9.5BE-1 0 3.306-0 7 3.316-0 7 1.60E-0 4 1.176-0 3 1.876-0 8 2.54E-0 6 2.96E-0 S I.22E-0 5 2.77E-0 3 S WAL L S I WAL L UL I WAL L L L I WAL L TBOD Y

2.B5E-0 7 I.32E-0 8 1.136-0 9 I.4IE-I 0 I.03E-0 6 I.9SE-0 6 3.77E-0 7 4.806-0 7 I.02E-0 7 2.I2E-0 6 1.35E-0 6 6.00E-0 7 9.I4E-0 7 3.95E-0 7 I.50E-0 6 3.I6E-0 5 4.09E-0 S 6.52E-0 5 3.25E-0 S I.57E-0 3 1.916-0 3 4.38E-0 3 2.476-0 2 7.I0E-0 2 3. 8 4.586-0 5 I.90E-0 5 7.76E-0 6 8.61E-0 7 2.016-0 3 1.186-0 3 2.I9E-0 3 6.99E-0 3 8.I2E-0 3 3.436-0 2 4.96E-0 5 2.14E-0 5 9.62E-0 6 1.626-0 6 I.76E-0 3 4.70E-0 4 1.09E-0 3 <.076-0 3 1.64E-0 2 3.866-0 2 3.376-0 7 1.716-0 8 4.22E-0 9 1.186-0 9 1.266-0 4 I.08E-0 4 6.336-0 5 4.216-0 5 8.08E-0 6 4.IOE-0 3 S.62E-0 5 2.22E-0 S 1 .6IE-0 S 3.44E-0 6 1.59E-0 4 2.286-0 5 S.76E-0 6 2.67E-0 6 6.39E-0 7 1.376-0 3 I.89E-0 3 4.24E-0 3 2.49E-0 2 7.48E-0 2 1. 8 2.176-0 4 4.87E-0 4 2.86E-0 3 8.58E-0 3 2. 3 1.806-1 1 2.32E-1 2 3.06E-1 2 6.746-1 3 6.23E-0 7 5.49E-I 1 2.33E-I 2 3.07E-I 2 6.75E-I 3 6.236-0 7 I.29E-2 4 9.7BE-3 S S.44E-4 S 8.35E-S 6 4.00E-I 3 1.436-2 3 I.086-3 3 6.036-4 4 9.26E-S S 4.OOE-1 3 1.116-1 4 1 . 4 46-1 4 2.30E-I 4 1.156-1 4 5.276-1 2 1.116-1 4 I.44E-I 4 2.30E-I 4 1.I5E-I 4 5.276-1 2 5.03E-1 6 1.03E-I 5 5.74E-I S I.6SE-1 4 1.89E-I 0 4.64E-I 6 9.336-1 6 S.196-1 5 1.486-1 4 1.896-1 0 3.766-1 1 1 .566-1 1 6.38E-1 2 7.I6E-I 3 3.676-0 9 3.766-1 1 1.56E-I I 6.386-1 2 7.166-1 3 3.67E-0 9 4.6SE-0 9 8.616-0 9 2.7SE-0 8 3.19E-0 8 2.94E-0 7 4.6SE-0 9 8.60E-0 9 2.756-0 8 3.I9E-0 8 2.94E-0 7 6.04E-0 6 2.57E-0 6 1.176-0 6 2. 1 IE-0 7 3.72E-0 * I.02E-0 S 4. 1 16-0 6 I.82E-0 6 2.97E-0 7 3.68E-0 4 6.65E-I 0 2.63E-1 0 1.926-1 0 4.216-1 1 3.596-0 8 2.61E-0 8 1.036-0 8 4.426-0 9 S.516-1 0 1.316-0 3 2.306-0 7 3.69E-0 7 I.I4E-0 6 I.32E-0 6 3.I3E-0 3 I.S5E-0 7 5.24E-0 8 3.08E-0 8 6.86E-0 9 3.396-0 5 2.I2E-0 5 4.30E-0 6 2.57E-0 6 S.74E-0 7 5.826-0 4 AORE N 3.76E - .606 * .426 * . 0 4 6 - . 7 5

•05E -

. 09E - .816 -

•22E - .386 - .316 -

. 02E -

•87E - . 7 8 9

•94E - .256 - .44E -



### • 7SE - .57E - .57E - .74E - .326 - .48E -

• 48E - .266 - .276 - .606 - .656 - .846 - .806 -

•37E - .3SE - .T7E - B L WAL L 0 8 1.776-0 8 0 6 I.3SE-0 7 • 0 7 6.05E-0 8 0 8 3.02E-0 8 0.3 7 •0 5 9.92E-0 6 0 3 5.2IE-0 4 0 5 3.50E-0 5 0 2 6.116-0 3 0 6 6.83E-0 7 

### 0 41.106-0 4 0 5 S.78E-0 6 0 5 3.17E-0 5 0.3 9 1 . 4 I t2.I2E-1 I 1 0 S.40E-1 I 2 3 7.22E-2 4 2 3 1.886-2 3 I 7 2.76E-1 7 I 7 2.76E-I 7 1 3 8.68E-I 4 1 3 1.166-1 3 

### 1 1 1.216-1 1 I I 1.216-1 1 0 9 2.53E-0 9 0 9 2.546-0 9 O S 7.55E-0 6 O S I.28E-0 5 1 0 8.27E-I 1 0 8 7.73E-0 9 0 7 5.S9E-0 8 0 7 1.36E-0 7 0 5 2.816-0 5 KIDNEY S

I.796-0 7 1.00E-0 6 7 . 4 9E- 0 7 I.70E-0 6 

### 4 . 4 I.32E- 03 7 . I9E- 02 5.386-0 3 0.7 1 1.195-0 4 2.53E-0 2 8.57E-0 4 S.86E-0 3 1 4 . S 2 . 7.46E-I 0 I.93E-0 9 2.60E-2 2 6.75E-2 2 5.44E-I 5 5.44E-I S 1.036-1 2 2.07E-I 2 2.23E-0 9 2.236-0 9 4.09E- 0 7 4.09E- 0 7 8.03E-0 4 9 . 3 3E- 0 4 I.01E- 0 8 I.39E-0 6 8.1IE-0 6 1.37E-0 5 I.23E-0 4 LIVE R

3.6 9 E-0 8 2.I6E-0 6 1.146-0 6 S.03E-0 7 3 . 4 3.6*6-0 5 5.76E-0 3 9.29E-0 S 3.56E-0 2 1.3 8 6-0 6 2.326-0 * 3.10E-0 5 7.19E-0 S 2 . 4 8 . 9 I.456-1 0 3.496-1 0 4.46E-2 3 1.166-2 2 1.956-1 5 1.956-1 5 7.876-1 3 9.6SE-I 3 4.346-1 0 4.346-1 0 6.866-0 8 6.87E-0 8 7.23E-0 5 '..026-0 4 3.936-1 0 2.8 3 6-0 7 I.SSE-0 6 I.3SE-0 6 5.79E-0 5

## r o

J* * NUCLID E

TL-20 7 TL-20 8 TL-20 9 ->B-20 9 (-H-2I 0 PB-2 1 1 -••1- 2 1 2 M-21 4 31-21 0 M-2 I I a 1- 2 1 2 9 1-21 3 dl- 2 1 4 *»O-2l 0
-'0-2 1 1
PO- 2 1 2

--U-2I 3

f 0- 2 1 4

••0- 2 I E
P0-2I 6

PO-21 8

4T-2I 7 RN-21 9 1N-22 0 RN-22 2 FR-22 1 SO L

W W 

## • t l 

# « »
w



# -

m w
w
w
w 

# • 0
w 0 H D
w D
w 0



# - 0



# - 0
w D 0 

# * * » 0 F l

0.9 S 0.9 5 0.9 5 8.006-0 2 8.OOE-0 2 8.JOE-0 2 8 . OOE-0 2 8.OOE-0 2 5.006-0 2 5.OOE-0 2 5 . 306-0 2 5.OOE-0 2 5.00E-0 2 t.006-0 1 I.00E-C 1 1 . 30E-0 I I.OOE-C I I.00E-C 1 I.OOE-C I I.OOE-C I I.OOE-C I I.OOE-O I I.OOE-C I 1 .006-0 1 I.OOE-0 1 1 . 506-0 1 I.OOE-O I 

## i . ooe-c i 1 .306 -0 1 0 . J S 0 . ) 0 . 0 0 . 0 O.-J S AMA D

0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 0 . 3 C . 3 C . 3 0 . 3 0 . 3 C . 3 0 . 3 C . 3 0 . 3 0 . 3 0 . 3 C . 3 0 . 3 0 . 3 0 . 3 4 * 4 

# •• * •* * 0 . 3 OVARIE S

3.476-0 8 2.25E-0 7 1 .066-0 7 6.066-0 8 0.7 5 1.976-0 5 1 .IOE-0 3 7.00E-0 5 1 .226-0 2 I .356-0 6 2 . 1 76-0 4 1 . 1 IE-O S 6.33E-0 5 0.7 8 2 . 9 4 . 2 56-1 1 1.086-1 0 1 .4SE-2 3 3.766-2 3 S.52E-I 7 5.53E-I 7 1.746-1 3 2.326-1 3 2.4IE- I 1 2 . 4 16- 1 1 S.296-0 9 S . 3 06-0 9 I .sie-c s 2.SSE-0 5 1.S8E-I 0 1 .546-0 8 1.2IE-0 7 2.72E-0 7 5.606-0 5 PANCR6A S

3.766-0 8 2.166-0 6 1 . I6E-0 6 6 . 046-0 8 0.7 3 2.066-0 5 1 . 146-0 3 7.996-0 5 I.22E-0 2 1 .396-0 6 2.35E-0 4 3 . 45E-O S 6 . J/E-O S 0.7 8 2 . ) 6.00E-I I 1.26E-I 0 I.44E-2. 1 3.75E-2 3 S.S7E-1 7 S.S7E-I 7 1 . 74r-i * 2.326-1 3 2.49E-I 1 2.49E- I 1 5.45E-0 9 5.456-0 9 1.626-0 5 2.67E-0 S 4.3SE-I 0 I.826-0 8 1.516-0 7 3.476-0 7 S.82E-0 5 TOTA L INHALATIO N DOSE S ALPH AO « 2 0 (HEM/MICROCURIE I BON E R MA R VMA R 3.S7E-0 S 3.636-0 8 3.63E-0 S 9.S4E-0 7 I.20E-0 6 1.006-0 6 5.81E-0 7 6.32E-0 7 4.9IE-0 7 3.846-0 6 I.06E-0 6 6.04E-0 8 4 4 . 2. 3 O.T S 3.39E-0 4 2.98E-0 4 2.0IE-0 S 1.70E-0 2 1.506-0 2 1.036-0 3 4.126-0 4 3.38E-0 4 7.34E-0 5 I.23E-0 2 1.266-0 2 1.226-0 2 I.37E-0 6 2.48E-0 6 1.376-0 6 2.22E-0 4 4.02E-0 4 2.24E-0 4 I.74E-0 5 2.6IE-0 S 1.816-0 5 I.33E-0 4 I.ISE-0 4 6.5SE-0 S 0.7 8 0.8 1 0.7 8 2 . 9 3. 0 2. 9 4.87E-I I 8.47E-I I 4.926-1 1 I.156-1 0 2.056-1 0 I.156-1 0 1.4*6-2 3 2.6*6-2 3 I.44E-2 3 3.7SE-2 3 6.8SE-2 J 3.756-2 3 3.516-1 5 9.656-1 6 5.546-1 7 3.516-1 5 9.696-1 6 5.346- I 7 1.036- 1 I S.42E-1 3 1.736-1 3 1.046- I I 6.02E-I 3 2.33E-I 3 8.226-1 0 6.99E-I 0 2.446- 1 I 8.226-1 0 6.99E-I 0 2.44E-1 I I.32E-0 7 1.I3E-0 7 S.04E-0 9 1.316-0 7 I.I3E-0 7 S.0SE-O 9 1.076-0 4 9.46E-0 S 1.556-0 5 I.IOE-0 4 I.07E-0 * 2.S9E-0 5 2.316-1 0 3.52E-I 0 2.4IE-I 0 5.316-0 7 4.52E-0 7 1.636-0 8 2.936-0 6 2.52E-0 6 I.20E-0 7 2.396-0 6 1.686-0 6 3.0IE-0 7 3.626-0 5 I.02E-0 4 S.63E-0 S ENDOS T 4.S0E-0 8 9.60E-0 7 S.6SE-0 7 3.07E-0 6 2 1 . 2.656-0 3 0 . 1 1 I.92E-0 3 S.70E-0 3 1.066-0 3 1 .416-0 3 2.21E-0 S 3.9IE-0 4 0.3 6 1 . 3 2.696-1 0 6.876-t O t.246-2 3 1.626-2 2 2.8IF-I S 2.816 - I S 4.82E-1 2 4.856-1 2 6.436-0 9 6.4.IF-0 9 8.57E-0 7 8.S7E-0 7 S.80E-0 4 6.I0E-0 4 4.55E-1 0 4.15E-0 6 1 .906-0 5 1 .0JF-0 5 4.I0E-0 4 SPLEE N

3.68E-C 8 2.04E-C 6 8.86E-C 7 6.06E-0 8 3 . 5 2.04E-0 S 1.116-0 3 8.42E-C S 0.3 5 I.38E-C 6 2.33E-C 4 2.C6C-C S 7 . 31E -0 3 2 4 . 8 9 . I.29E-0 S 3.32E-C* . 4.466-2 2 I.I6E-2 I 5.386-1 7 5.59E-I 7 a.HE - 1 3 2.596 - 1 2 2.47E-I I 2.48E-I I 5.60E-0 9 S.79E-C * 2 . 2 IE-0 4 S.67E-0 4 3.6SE-I 0 1.776-t e I.486-C 7 3.97E-C 6 5 . 776-0 5 TESTE S

3.466-0 8 8.52E-0 8 4.I4E-0 8 6.086-0 0 0.7 5 1.976-0 5 "B.55E-0 4 6.896-0 5 1.226-0 2 1.3SE-0 6 2.I6E-0 4 8.656-0 6 6.276-0 5 0.7 8 2 . 9 4.ISE-I 1 I.C8E-1 0 I.45E-2 3 3.766-2 3 8.536-1 7 5.536-1 7 1.7*6-1 3 2.32E-I 3 2.416-1 1 2.416-1 1 4.7IE-0 9 4.72E-0 9 I.S0E-0 5 2.S4E-0 5 1 .296-1 0 1.526-0 8 9.60E-0 8 2.66E-0 7 S.53E-0 S THYMU S

3.936-0 8 3.S8E-0 6 1 .936-0 6 6.0*6-0 8 0.7 5 2.I0E-0 5 1 .206-0 3 8.59E-0 S I . 2 2E-0 2 1 .406-0 6 2.446-0 4 4.686-0 5 7.39E-0 5 0.7 8 2 . 9 7.1IE-1 t 1 .376-1 0 1 .446-2 3 3.75E-2 3 S.616-1 7 5.616-1 7 1.746-1 3 2.32E-I 3 2.S2E- I 1 2.526- 1 1 5.69E-0 9 S.70E-0 9 1.69E-0 5 2.73E-0 S 5.816-1 0 1.966-0 8 1.786-0 7 4.00E-0 7 S.94E-0 5 THYROI O

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### TOTA L INHALATIO N DOSE S ALPH A0 a 2 0 (REM/MICROCURIE I



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2 1 1 3 8 4 1 S 0 5 6 2 0 2 

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## a 0 2 2 .49E-0 4 .32E-0 5 .82E-0 2 .086-0 2 .32E-0 2 .65E-0 3 .406-0 2 ,636-0 3 . 1 2 .156-0 2 .026-0 2 .056-0 2 . 1 2 .•8E-0 2 .06E-0 2 . 1 5 1 . 4 S3E-0 2 .276-0 2 .•96-0 2 .0*6-0 2 .706-0 2 . 2 9 026-0 2 J 7 . ,056-0 2 15E-0 2 ,056-0 2 59E-0 * 2 7 .37E-0 2 1 3 .09E-0 2 26E-0 2 TOTA L INHALATIO N DOSE S ALPH AO a 2 0 (REM/MICROCURIE I S WAL L S I WAL L U 1.256-0 * I.30E-0 * 1 7.356-0 6 7.066-0 7 6 8.906-0 3 9.386-0 3 9 1.156-0 3 5.986-0 * 3 2.206-0 3 I . 1 16-0 3 6 3.766-0 3 4.776-0 3 5 2.966-0 3 3.746-0 3 * 1.526-0 5 3.94E-0 3 2 1.706-0 5 4. 1 IE-O S 2 5.S3E-0 3 7.296-0 3 I 4.376-0 3 6.016-0 3 I S.356-0 4 6. 0 16-0 4 I 9.25E-0 * 7.666-0 4 1 2.396-0 3 3.776-0 3 6 2.886-0 3 3.786-0 3 6 1.446-0 2 I .71E-0 2 2 3.97E-0 2 I.T4E-0 2 2 1.47E.-0 2 1.656-0 2 I 1.146-0 2 1.2*6-0 2 I I.I9E-0 2 1.126-0 2 I I.47E-0 3 S.52E-0 4 1 9.35E-0 4 1.866-0 3 I 2 . 1 16-0 3 5.20E-0 3 3 3.586-0 * 8.S6E-0 * 7 I . I 06-0 2 2. 6 7E-0 2 O 1.226-0 3 2.086-0 3 5 1.47E-0 3 2.816-0 3 7 2.556-0 3 6.086-0 3 3 I.87E-0 5 I.07E-0 S 2 I.96E-0 3 4.87E-0 3 2 2.96E-0 3 4.60E-0 3 1 3.086-0 3 4.04E-0 3 I 2.91E-0 3 6.396-0 3 2 3.306-0 3 7.34E-0 3 2 I L I WAL L .37E-0 * .906-0 6 •87E-0 3 .2*6-0 3 .256-0 3 .756-0 3 .966-0 3 .166-0 4 .246-0 4 .28E-0 2 •2IE-0 2 .66F-0 3 •72E-0 3 .136-0 3 .•26-0 3 .*IE-0 2 .666-0 2

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1 .346-0 * I.76E-0 5 1 .51E-0 2 4.196-0 3 3.536-0 3 7.7IE-0 3 4.236-0 3 I.30E-0 3 6.386-0 4 7.98E-0 3 S.OIE-0 3 7.16E-0 4 1.156-0 3 2.23E-0 3 2.64E- 0 3 1.926-0 2 4.3IE-0 2 2.46E-0 2 1 .84E-0 2 1.S2E-0 2 1 .S8E-0 2 2.6IE-0 3 7.37E-0 5 1.836-0 2 1.72E-0 3 6.28E-0 4 1.73E-0 * 7.28E-0 S 1 .28E-0 S 9.45E-0 4 3.S6E-0 3 2.73E- 0 3 4.68E-0 4 3.37E-0 4 B L WAL L

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1 7 1 4 3 6 3 1 6 7 

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ALPH A0 a 2 0 (REM/MICROCURIE I 

### N ERMA

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• 53E-0 3 .•16-0 3 •05E-0 3 •30E-0 3 .406-0 *
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• 08E-0 S .26E-0 2 .826-0 2 .37E-0 2 •79E-0 3 .126-0 3 .136-0 4

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### • 30E-0 4 .896-0 4 •43E-0 3 •64E-0 5

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### 4.656-0 4 3.836-0 4 THYROID

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### TOTA L INHALATIO NDOSE S ALPH A0 a 2 0 

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NB-9 5 NB-97 M NB-9 7 MO-9 9
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## P.7 3



# APPENDI XB
Tabulation s o f Effectiv e Dos e Equivalen t t oaReferenc e Adul t fro m Uni t Inhalatio nan

dIngestionExposure s



# 6 9

## P.7 4



# TH E EFFECTIV E DOS E EQUIVALEN T
Th e effectiv e dos e equivalent , presente dinth e followin g table s fo r inhalatio nan dingestio nexposures , i s a weighte daverag e o f com mitte ddos e equivalent s fo r specifi c organs , wit hth e weight s determine d fro m stochasti c ris kfactor s associate dwit hth e respectiv e organ s a s specifie db

yICR P Publicatio n2 6 (ICRP , 1977) . Th e definitio ni s

H F 

# =]£w,H . r 

# em/yC i (B-l )

wher e H £ 

# = effectiv e dos e equivalent ; j = inde xtha t range s ove r severa l organs , a s specifie di nTabl e B-l ; vi. = weightin g facto r givin g th e pro o 

# portio no f th e stochasti c ris kresultin g fromorga nj unde r unifor m whole-bodyirradiation ; andH . = committe ddos e equivalen t (rem ) t o orga nj resultin g fro mth e intak e o f 1 yC i o f th e radionuclid e unde r consideration
. Th e value s w . assigne db yth e ICR P andth e ris kfactor s J 

# o nwhic hthey

ar e base dar e showni nTabl e B-l . "Remainder, " i ntha t table , refer s t o th e fiv e organs , othe r tha nthos e listed , havin g th e highes t dos e equivalents ; t o eac ho f thes e i s assigne dw . = 0.06 . Fo r computatio no f H E 

# , th e dos e equivalen t t o th e lung include s consider

atio no f radioactivit yresidin g i nth e respirator ylymp hnodes . W e not e her e tha t ICR P Publicatio n3 0 (ICRP , 1979 ) i nit s computatio no f th e annua l limi t o nintak e (ALI ) applie s a 10 % rul e t o Eq . (B-l) , tha t is , th e ter m w-H . i s omitte dfromth e su mi f i t doe s no t excee d10 % o f th e

• J*J 

# maximumw-H. . W e hav e no t applie dthi s rul e incomputin g th e entrie s o f

• J * J 

# thi s tabulation
. Th e effectiv e dos e equivalent , a s define dabove , i s equa l t o tha t dos e equivalent , delivere da t a uniformwhole-bodyrate , tha t corre spond s t o th e sam e expecte dnumbe r (bu t possibl ydissimila r distri

bution ) o f fata l stochasti c healt heffect s a s th e particula r combinatio n o f committe dorga ndos e equivalents , H. , unde r consideration
. Thus , fo r J 

# som e purposes , thi s tabulatio nca nserv e i nplac e o f a mor e extensiv e compilatio no f committe ddos e equivalen t pe r uni t intak e fo r a numbe r o f individua l organs , suc ha s tha t give ni nAppendi xA . 7 1

## P.7 5



# Tabl e B-l . Organ-specifi c ris k factor s andproportiona l weights' 2



# Orga n Ris k (rem) Gonad s Breast s Re dmarro w Lun g Thyroi d Bon e surface s Remainde r Tota l ris k (un i formwhole

bodyirradiation ) 0.2 5 0.1 5 0.1 2 0.1 2 0.0 3 0.0 3 0.3 0 0.0000 4 0.00002 5 0.0000 2 0.0000 2 0.00000 5 0.00000 5 0.0000 5

* . 0.00016 5 Internationa l Commissio no nRadiologica l Protection , Publicatio n26 , 1977 .



# 7 2

## P.7 6



# APPENDI XB REFERENCE S
Internationa l CommissiononRadiologica l Protectio n(ICRP) , 1977 , Annals of the ICRP 1_ , 1 , Publication26 , PergamonPress , Oxford . Internationa l Commissiono nRadiologica l Protection(ICRP) , 1979 , Limitsfor

Intakesof

RadionuclidesbyWorkers, Publicatio n30 , PergamonPress , Oxford .



# 7 3

## EFFECTIV E OCS E CCMMITKEN T FRO M RADIONUCLID E INHALATIO N

(REO/MICCCCUR I £ ) ACTIVIT YMEDIA N AEROOYNAM1 C DIAMETE R NUCL1D E M - 3 

## C-I * NA-2 2 i 

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# NUREG/CR-015 0 

# Vol . 3 0RNL/NUREG/TM-190/V 3 Dist . Category

NRC-RH INTERNALDISTRIBUTION 

# 1 . 2 . 3 . 4 . 5 . 6 . 7-11 . 12-16 . 

# 17 . 18 . 19 . 20 . 21 . 22-23 . 

# 24 . 25 . 26 . J . S . R . D . M . H . D . K . M . C . G . F . S . G . D . R . A . A . R . 0 . J . C r W . E . F . R . E . S . 0 . V . G . C . W . L . Auxie r Bernar d Cheste r Crawfor d ist y Dickso n Dunning , J r Eckerma n Ford Hayne s Hil l Hoffma n Kaye Killough Koche r Legget t Lott s 

# 27 . 28 . 29 . 30 . 31 . 32 . 33 . 34 . 35 . 36 . 37 . 38 . 39-40 . 

# 41 . 42-43 . 

# 44 . 45 . 46 . L . M . McDowel1-Boye r H . R . Meye r C . W . Mille r T . W . Oake s F . R . 0'Donnel l D . C . Parzyc k P . S . Rohwe r M . T . Ryan P . J . Wals h S . B . Watso n J . P . Witherspoo n M . G . Yalcinta s Centra l Researc hLibrar y ORNLY-1 2 Technica l Librar y Laborator y

Record s Departmen t Laborator y

Records , 0RNL-R C RSI C Librar y ORNLPaten t Offic e 

# EXTERNALDISTRIBUTION 47 . J . C . Pleasant , Departmen t o f Mathematics , Eas t Tennesse e Stat e University , Johnso nCity , TN 3760 1 48-49 . Technica l Informatio nCenter , 0R0 , Oa kRidge , TN 3783 0 50 . Offic e o f Assistan t Manager , Energy Researc han

dDevelopment , D0E-0R0 , OakRidge , TN 3783 0 51-215 . Give nDistributio naccordin gt o NRC category R H(NTIS-10 )



# 8 3