AQS Site ID State County Latitude Longitude Sulfates Nitrates Crustal OC

010799000 AL Lawrence 34.34343 -87.3388 3.2 0.6 0.6 2.2

020130002 AK Aleutians East55.32467 -160.508 0.8 0.1 0.1 0.2

020680003 AK Denali 63.72534 -148.966 0.4 0.1 0.2 0.4

021220009 AK Kenai Peninsula 59.98267 -152.661

021700011 AK Matanuska-Susitna 62.31475 -150.318 0.4 0.1 0.1 0.4

022909000 AK Yukon-Koyukuk 66.93093 -151.492 0.5 0.1 0.1 0.5

040018001 AZ Apache 34.05848 -109.441 0.8 0.1 0.7 0.7

040038001 AZ Cochise 32.11707 -109.468 1.0 0.2 1.0 0.6

040039000 AZ Cochise 31.34918 -109.54 1.2 0.3 4.3 1.3

040058100 AZ Coconino 36.07781 -112.13 0.8 0.2 1.1 0.7

040058102 AZ Coconino 35.97312 -111.985 0.7 0.2 0.7 0.6

040058103 AZ Coconino 35.14064 -111.97 0.7 0.2 2.9 1.1

040070010 AZ Gila 33.6547 -111.107 1.1 0.3 1.3 0.8

040078100 AZ Gila 34.09087 -110.943 0.9 0.2 1.0 1.0

040159000 AZ Mohave 36.0193 -114.069 0.8 0.2 1.1 0.5

040170119 AZ Navajo 34.8225 -109.892 0.8 0.2 1.0 0.7

040190005 AZ Pima 31.95 -112.801 1.3 0.3 1.5 0.4

040190021 AZ Pima 32.17454 -110.737 1.1 0.3 1.5 0.7

040199000 AZ Pima 32.24871 -111.218 1.2 0.4 2.5 0.7

040218001 AZ Pinal 33.29347 -111.286 1.2 0.4 1.6 0.7

051019000 AR Newton 35.82589 -93.2032 2.6 0.9 0.9 1.9

051130003 AR Polk 34.45441 -94.1433 2.7 0.7 1.0 1.8

060179000 CA El Dorado 38.976 -120.104 0.5 0.2 0.4 0.9

060199000 CA Fresno 37.22064 -119.156 0.7 0.3 0.6 0.8

060270101 CA Inyo 36.50861 -116.848 0.9 0.2 1.2 0.6

060299001 CA Kern 34.82194 -118.887 1.1 0.6 0.9 1.3

060379000 CA Los Angeles 34.37892 -117.692 0.8 0.5 1.0 0.8

060379034 CA Los Angeles 34.81306 -118.884

060410002 CA Marin 38.12306 -122.908 1.1 0.7 0.2 0.5

060430003 CA Mariposa 37.71326 -119.705 0.7 0.3 0.6 1.0

060519000 CA Mono 38.08802 -119.178 0.5 0.1 0.5 0.5

060659000 CA Riverside 33.46364 -116.971 1.5 1.0 0.6 1.1

060690003 CA San Benito 36.48522 -121.157 0.9 0.6 0.4 0.9

060719002 CA San Bernardino 34.07139 -116.391 1.0 0.6 0.8 0.7

060719010 CA San Bernardino 34.19393 -116.914 0.9 1.2 0.6 0.9

060839000 CA Santa Barbara34.73389 -120.008 1.0 0.6 0.7 0.8

060893003 CA Shasta 40.53681 -121.574 0.5 0.1 0.4 1.1

060930005 CA Siskiyou 41.71194 -121.509 0.5 0.1 0.4 1.1

061059000 CA Trinity 40.78625 -122.806 0.5 0.2 0.3 1.1

061071001 CA Tulare 36.49889 -118.824 1.3 1.2 0.8 1.9

2010-2012 3-Year Ave

Speciation Measurements
080039000 CO Alamosa 37.72492 -105.519 0.6 0.2 1.2 0.8

080450015 CO Garfield 40.085 -107.312

080579000 CO Jackson 40.5383 -106.677 0.5 0.1 0.5 0.6

080679000 CO La Plata 37.3038 -107.484 0.6 0.2 1.6 0.8

080699001 CO Larimer 40.27828 -105.546 0.6 0.2 0.6 0.7

080839000 CO Montezuma37.19841 -108.491 0.7 0.2 1.2 0.5

080979000 CO Pitkin 39.15359 -106.822 0.5 0.1 0.7 0.4

110010042 DC District of Columbia 38.88083 -77.0325 3.0 1.2 0.7 1.9

120179000 FL Citrus 28.74868 -82.5548 2.5 0.4 0.8 1.9

120860030 FL Miami-Dade25.38833 -80.6833 2.1 0.4 1.0 1.0

121290001 FL Wakulla 30.0925 -84.1611 2.7 0.4 0.7 1.9

130499000 GA Charlton 30.74072 -82.1282 2.8 0.4 0.7 2.4

132139000 GA Murray 34.78532 -84.6264 3.0 0.5 0.6 2.0

081039000 CO Rio Blanco 39.9153 -107.635

081119000 CO San Juan 37.65941 -107.801 0.6 0.1 0.9 0.6

090050005 CT Litchfield 41.82134 -73.2973 1.9 0.6 0.3 1.2

200170001 KS Chase 38.43414 -96.5605 2.2 1.5 0.9 1.6

201950001 KS Trego 38.77008 -99.7634 1.5 1.0 1.2 1.0

210619000 KY Edmonson 37.13187 -86.1479 3.4 1.1 0.5 1.9

212219000 KY Trigg 36.78428 -87.8501

220719000 LA Orleans 30.10863 -89.7617 3.3 0.6 1.0 1.7

221279000 LA Winn 32.05758 -92.4352

230031020 ME Aroostook 46.69634 -68.0326 1.1 0.2 0.4 1.3

230050103 ME Cumberland44.10736 -70.7286 1.3 0.2 0.2 1.2

230059002 ME Cumberland43.83246 -70.0638 1.5 0.3 0.2 1.6

230090103 ME Hancock 44.37705 -68.2609 1.3 0.2 0.2 0.9

230199000 ME Penobscot 44.94798 -68.6479 1.4 0.3 0.3 1.6

230291004 ME Washington45.12584 -67.2654 1.2 0.2 0.2 0.9

240239000 MD Garrett 39.7059 -79.0121 3.4 0.6 0.4 1.4

250010002 MA Barnstable 41.9758 -70.0236 1.8 0.5 0.2 1.1

250070001 MA Dukes 41.33047 -70.7852 2.0 0.6 0.3 1.2

250154002 MA Hampshire 42.29849 -72.3341 1.8 0.5 0.3 1.4

260839000 MI Keweenaw 47.9167 -89.1501 1.2 0.5 0.2 1.0

261539000 MI Schoolcraft 46.2889 -85.9503 1.5 0.6 0.2 1.1

270759000 MN Lake 47.9466 -91.4957 1.0 0.5 0.3 1.2

271339000 MN Rock 43.71579 -96.1916 1.7 2.0 0.9 1.2

271379000 MN St. Louis 48.4126 -92.8288 1.1 0.5 0.3 1.0

271699000 MN Winona 43.9373 -91.4053 1.8 1.9 0.5 1.4

290390001 MO Cedar 37.69 -94.035 2.5 1.5 1.1 1.8

292070001 MO Stoddard 36.97 -90.14 2.8 1.1 1.3 2.3

150019002 HI Hawaii 19.43118 -155.259

150099000 HI Maui 20.80879 -156.284

150099001 HI Maui 20.7585 -156.248 0.8 0.1 0.2 0.0

160230101 ID Butte 43.46056 -113.562 0.5 0.4 0.6 1.2
160370002 ID Custer 44.17038 -114.928 0.4 0.1 0.5 1.9

170191001 IL Champaign 40.05224 -88.3725 2.9 2.2 0.5 1.6

181759000 IN Washington38.53465 -86.2604

191370002 IA Montgomery40.96911 -95.045 2.1 2.1 0.8 1.4

191770006 IA Van Buren 40.69508 -92.0063 2.3 2.1 0.6 1.5

200139000 KS Brown 39.97912 -95.5685

292130003 MO Taney 36.61388 -92.9223 2.6 1.0 0.8 1.9

300279000 MT Fergus 47.58223 -108.72 0.7 0.3 0.6 0.8

300299001 MT Flathead 48.51039 -113.998 0.5 0.2 0.5 1.6

300479000 MT Lake 47.77328 -114.27 0.4 0.1 0.4 1.1

300499000 MT Lewis and Clark46.8261 -111.712 0.4 0.1 0.4 1.0

300779000 MT Powell 47.12209 -113.155 0.4 0.1 0.8 1.5

300819000 MT Ravalli 45.85969 -114.001 0.4 0.1 0.4 2.5

300859000 MT Roosevelt 48.30795 -105.103 1.3 0.8 0.7 1.0

300870762 MT Rosebud 45.64833 -106.557 0.7 0.3 0.6 1.1

300899000 MT Sanders 47.95477 -115.672 0.4 0.1 0.4 1.0

300919000 MT Sheridan 48.48705 -104.476 1.2 0.7 0.8 0.9

310699000 NE Garden 41.76268 -102.434 1.0 0.7 0.7 0.8

311719000 NE Thomas 41.88879 -100.339 1.3 0.9 0.8 0.9

320339000 NV White Pine 39.00515 -114.217 0.5 0.1 0.6 0.6

330074002 NH Coos 44.30817 -71.2177 1.3 0.1 0.2 1.1

330115001 NH Hillsborough42.86175 -71.8784 1.5 0.3 0.2 1.0

330150018 NH Rockingham42.86254 -71.3802

340019000 NJ Atlantic 39.46502 -74.4488 2.8 1.0 0.4 1.6

350039000 NM Catron 33.2205 -108.236 0.8 0.1 0.9 0.9

350059000 NM Chaves 33.45991 -104.405 1.6 0.6 1.8 0.9

350279000 NM Lincoln 33.46881 -105.535 1.2 0.2 1.3 0.8

350281002 NM Los Alamos 35.80417 -106.298 0.8 0.2 0.8 0.9

350399000 NM Rio Arriba 36.01394 -106.845 0.6 0.2 0.9 0.7

350539000 NM Socorro 33.86959 -106.853 0.9 0.2 1.2 1.0

350559000 NM Taos 36.58544 -105.453 0.6 0.1 0.7 0.5

361019000 NY Steuben 42.0912 -77.2096

370110002 NC Avery 35.97222 -81.9331 2.6 0.2 0.4 1.8

370870035 NC Haywood 35.37917 -82.7925 2.3 0.3 0.5 1.4

380070002 ND Billings 46.8943 -103.379 1.1 0.6 0.7 0.9

380130004 ND Burke 48.64193 -102.402 1.3 0.9 0.9 0.9

391219000 OH Noble 39.94283 -81.3376 3.7 1.0 0.5 1.5

400019009 OK Adair 35.75074 -94.6697

400319000 OK Comanche 34.7324 -98.7134 2.2 1.0 1.1 1.5

400450890 OK Ellis 36.08551 -99.9354 1.7 0.9 1.2 1.2

400719010 OK Kay 36.95622 -97.0314

410050010 OR Clackamas 45.28862 -121.785 0.4 0.2 0.4 0.8

410330010 OR Josephine 42.10428 -123.681 0.5 0.1 0.2 1.1

410358001 OR Klamath 42.91 -122.14 0.4 0.1 0.4 0.7
410610010 OR Union 45.22475 -118.514 0.5 0.2 0.5 1.1

410630002 OR Wallowa 45.07986 -116.845 0.5 0.3 0.5 1.3

420019000 PA Adams 39.92322 -77.3076

420859000 PA Mercer 41.42691 -80.1451

450190046 SC Charleston 32.94102 -79.6572 2.9 0.5 0.6 2.0

460330132 SD Custer 43.5578 -103.484 0.8 0.4 0.6 1.0

460710001 SD Jackson 43.74561 -101.941 1.0 0.4 0.6 0.8

470090101 TN Blount 35.63149 -83.9435 3.0 0.4 0.5 1.7

481099000 TX Culberson 31.83315 -104.81 1.3 0.3 1.9 0.8

490170101 UT Garfield 37.61838 -112.174 0.6 0.2 0.6 0.6

490379000 UT San Juan 38.45868 -109.822 0.7 0.2 0.8 0.5

490530130 UT Washington 37.1983 -113.151 0.7 0.2 0.8 0.6

490559000 UT Wayne 38.30218 -111.293 0.6 0.2 0.7 0.6

500038001 VT Bennington 43.14818 -73.1263

500070007 VT Chittenden 44.52839 -72.8688 1.5 0.4 0.2 1.2

511139000 VA Madison 38.52294 -78.4345 2.8 0.6 0.4 1.3

511639000 VA Rockbridge 37.62666 -79.5123 3.1 0.6 0.5 2.3

530090013 WA Clallam 48.29786 -124.625

530090014 WA Clallam 48.37182 -124.595

530090020 WA Clallam 48.37163 -124.596 0.7 0.2 0.1 0.7

530370004 WA Kittitas 47.39981 -121.427 0.5 0.2 0.2 0.9

530390010 WA Klickitat 45.74982 -121.401

530390011 WA Klickitat 45.66422 -121.002 0.8 0.6 0.8 1.4

530410007 WA Lewis 46.62435 -121.387 0.4 0.1 0.2 0.7

530470012 WA Okanogan 48.38753 -119.929 0.4 0.1 0.2 0.9

530530014 WA Pierce 46.78472 -121.738 0.6 0.1 0.2 0.9

530730022 WA Whatcom 48.73142 -121.066 0.5 0.1 0.1 0.7

540939000 WV Tucker 39.10534 -79.4259 3.2 0.5 0.4 1.5

560050123 WY Campbell 44.6522 -105.29 0.8 0.3 1.0 1.0

560199000 WY Johnson 44.33344 -106.957 0.5 0.1 0.5 0.7

560299002 WY Park 44.74472 -109.382 0.5 0.1 0.6 0.8

560359000 WY Sublette 42.97483 -109.759 0.5 0.1 0.6 0.8

560359001 WY Sublette 42.84648 -109.64 0.5 0.1 0.6 0.7

560399000 WY Teton 44.56522 -110.401 0.5 0.2 0.4 1.0

780209000 VI St. John 18.33695 -64.7956 1.5 0.3 2.6 0.2

* These data were derived with the SANDWICH algorithm to represent PM2.5 composition. For simplification purposes, the 
EC Sulfates Nitrates Crustal OC EC Sulfates Nitrates Crustal

0.3 4.2 0.1 0.7 3.0 0.4 3.3 0.8 1.0

0.1 1.3 0.0 0.1 1.2 0.1 0.7 0.1 0.1

0.0 0.7 0.1 0.2 0.4 0.1 0.4 0.1 0.2

0.0 0.7 0.0 0.2 0.4 0.1 0.4 0.1 0.2

0.0 0.8 0.0 0.1 0.7 0.1 0.5 0.1 0.1

0.1 1.2 0.0 0.8 0.8 0.1 0.7 0.1 0.5

0.1 1.5 0.0 1.2 0.7 0.1 0.9 0.2 0.8

0.3 1.6 0.0 4.6 1.8 0.3 1.1 0.3 4.8

0.1 1.1 0.0 1.3 0.9 0.1 0.8 0.2 1.2

0.1 1.0 0.0 0.9 0.7 0.1 0.6 0.2 0.6

0.2 1.0 0.0 3.2 1.2 0.2 0.7 0.2 2.5

0.1 1.5 0.0 1.5 1.0 0.1 1.0 0.2 1.1

0.2 1.3 0.0 1.1 1.2 0.2 0.8 0.2 0.7

0.1 1.2 0.0 1.3 0.7 0.1 0.8 0.2 1.0

0.2 1.2 0.0 1.2 0.9 0.2 0.8 0.2 1.0

0.1 1.8 0.0 1.7 0.7 0.1 1.1 0.3 1.2

0.1 1.6 0.0 1.7 0.9 0.2 1.0 0.4 1.3

0.2 1.7 0.0 2.8 1.0 0.2 1.0 0.4 2.0

0.1 1.7 0.0 1.8 0.9 0.1 1.1 0.4 1.1

0.2 3.4 0.3 1.0 2.6 0.3 2.7 1.0 1.2

0.2 3.6 0.2 1.0 2.4 0.2 2.7 0.8 1.3

0.1 0.8 0.0 0.5 1.1 0.1 0.5 0.2 0.5

0.1 1.0 0.0 0.8 1.2 0.1 0.7 0.3 0.8

0.1 1.3 0.0 1.4 0.8 0.1 0.8 0.2 1.0

0.1 1.5 0.0 1.0 2.1 0.2 1.0 0.6 0.9

0.2 1.1 0.0 1.1 1.2 0.2 0.6 0.5 0.9

0.1 1.5 0.2 0.2 2.7 0.1 1.2 0.8 0.2

0.1 1.1 0.0 0.7 1.5 0.1 0.6 0.2 0.6

0.1 0.8 0.0 0.7 0.6 0.1 0.5 0.1 0.6

0.2 2.0 0.0 0.6 2.0 0.2 1.5 1.0 0.6

0.1 1.3 0.0 0.4 1.8 0.2 0.9 0.6 0.4

0.1 1.4 0.0 1.0 1.1 0.1 0.9 0.8 0.8

0.1 1.3 0.0 0.7 1.5 0.2 0.9 1.4 0.7

0.1 1.4 0.0 0.8 1.5 0.1 1.0 0.6 0.8

0.1 0.7 0.0 0.5 1.4 0.1 0.4 0.1 0.6

0.1 0.7 0.0 0.5 1.5 0.1 0.4 0.1 0.4

0.1 0.7 0.0 0.4 1.6 0.1 0.4 0.2 0.4

0.2 1.8 0.4 0.9 3.1 0.2 1.3 1.0 0.8

2010-2012 3-Year Average

SANDWICHed* Speciation Measurements
0.1 0.9 0.0 1.4 0.8 0.1 0.5 0.2 1.3

0.1 0.8 0.0 0.6 0.8 0.1 0.5 0.1 0.6

0.1 0.9 0.0 1.8 0.9 0.1 0.6 0.2 2.0

0.1 0.9 0.0 0.8 0.9 0.1 0.6 0.3 0.6

0.1 1.0 0.0 1.4 0.6 0.1 0.6 0.2 1.4

0.1 0.7 0.0 0.9 0.6 0.1 0.4 0.1 0.8

0.8 4.0 0.5 0.7 2.9 0.9 3.5 1.3 0.9

0.3 3.4 0.0 0.9 2.5 0.4 2.7 0.4 1.1

0.1 2.9 0.0 1.1 1.8 0.2 2.3 0.4 1.1

0.2 3.7 0.0 0.8 2.7 0.3 3.1 0.4 1.0

0.3 3.8 0.0 0.7 3.1 0.3 3.2 0.4 1.0

0.2 4.0 0.0 0.6 2.6 0.3 3.4 0.6 0.8

0.1 0.8 0.0 1.1 0.6 0.1 0.5 0.1 1.1

0.2 2.6 0.1 0.3 1.7 0.2 1.9 0.5 0.4

0.2 2.9 1.0 1.0 2.1 0.3 2.2 1.6 0.9

0.1 2.0 0.5 1.3 1.4 0.1 1.5 1.1 1.0

0.3 4.5 0.5 0.6 2.4 0.3 3.9 1.3 0.8

4.0 1.5 0.9

0.3 4.5 0.0 1.1 2.3 0.4 3.5 0.7 1.3

2.8 0.4 1.2

0.2 1.6 0.1 0.4 1.9 0.2 1.1 0.2 0.5

0.2 1.9 0.0 0.2 1.7 0.2 1.3 0.2 0.3

0.3 2.1 0.1 0.2 2.4 0.3 1.5 0.2 0.3

0.1 1.8 0.0 0.2 1.5 0.1 1.2 0.2 0.3

0.3 1.9 0.1 0.3 2.2 0.3 1.3 0.2 0.4

0.1 1.7 0.0 0.2 1.3 0.1 1.1 0.2 0.2

0.3 4.5 0.3 0.5 1.5 0.3 3.7 0.7 0.6

0.2 2.5 0.0 0.2 2.2 0.2 1.8 0.4 0.3

0.2 2.8 0.1 0.3 2.5 0.2 2.0 0.6 0.4

0.2 2.4 0.1 0.3 1.7 0.3 1.8 0.4 0.4

0.1 1.7 0.3 0.3 1.4 0.1 1.2 0.5 0.3

0.1 2.0 0.4 0.3 1.3 0.2 1.4 0.7 0.3

0.1 1.4 0.3 0.3 1.5 0.1 1.0 0.4 0.4

0.2 2.2 1.4 1.0 2.0 0.2 1.8 2.3 1.0

0.1 1.5 0.4 0.3 1.4 0.1 1.1 0.5 0.4

0.2 2.4 1.5 0.5 1.8 0.2 1.8 2.0 0.6

0.3 3.3 1.0 1.2 2.4 0.3 2.6 1.7 1.0

0.4 3.7 0.6 1.4 3.1 0.4 3.2 1.2 1.8

3.3 0.1 0.3

1.3 0.2 0.2

0.0 1.2 0.0 0.3 0.1 0.0 0.8 0.1 0.3

0.1 0.7 0.2 0.7 1.6 0.1 0.4 0.4 0.7
0.2 0.7 0.0 0.6 2.3 0.2 0.4 0.1 0.6

0.3 3.7 1.5 0.6 2.5 0.4 3.0 2.8 0.7

4.4 2.0 0.8

0.3 2.7 1.7 0.9 2.3 0.3 2.1 2.4 0.8

0.3 3.0 1.6 0.7 2.3 0.3 2.2 2.5 0.7

2.2 2.3 1.0

0.3 3.4 0.6 0.8 2.4 0.3 2.7 1.1 0.9

0.1 1.0 0.3 0.7 1.0 0.1 0.8 0.4 0.5

0.2 0.8 0.1 0.6 2.1 0.3 0.5 0.2 0.6

0.1 0.7 0.0 0.5 1.5 0.1 0.4 0.1 0.5

0.1 0.7 0.0 0.5 1.2 0.1 0.4 0.2 0.6

0.1 0.7 0.0 1.0 1.9 0.1 0.4 0.1 0.8

0.2 0.7 0.0 0.5 3.4 0.2 0.4 0.1 0.5

0.1 1.6 0.6 0.8 1.0 0.1 1.5 0.9 0.9

0.1 1.0 0.1 0.7 1.6 0.1 0.7 0.3 0.6

0.1 0.7 0.0 0.5 1.4 0.1 0.5 0.1 0.5

0.1 1.5 0.5 0.9 1.0 0.1 1.4 0.8 0.7

0.1 1.4 0.4 0.8 1.2 0.1 1.1 0.8 0.7

0.1 1.8 0.6 0.9 1.3 0.1 1.4 1.0 0.6

0.1 0.8 0.0 0.8 0.7 0.1 0.5 0.1 0.7

0.1 1.9 0.0 0.2 1.5 0.1 1.2 0.1 0.2

0.2 2.1 0.1 0.3 1.4 0.2 1.5 0.2 0.3

0.3 3.7 0.3 0.4 2.4 0.3 3.0 1.1 0.6

0.1 1.2 0.0 1.1 1.1 0.1 0.8 0.1 0.7

0.1 2.2 0.2 1.9 1.5 0.1 1.5 0.6 1.4

0.1 1.7 0.0 1.4 1.1 0.1 1.1 0.1 1.1

0.1 1.1 0.0 0.9 1.1 0.2 0.7 0.2 0.7

0.1 1.0 0.0 1.1 0.8 0.1 0.6 0.2 0.8

0.2 1.3 0.0 1.4 1.3 0.2 0.8 0.2 0.9

0.1 0.9 0.0 0.8 0.7 0.1 0.5 0.1 0.6

0.3 3.5 0.0 0.5 2.6 0.3 3.1 0.3 0.7

0.2 3.1 0.0 0.5 1.8 0.2 2.5 0.3 0.7

0.1 1.5 0.4 0.8 1.0 0.2 1.3 0.8 0.8

0.2 1.7 0.6 1.0 1.2 0.2 1.7 1.1 0.8

0.3 4.9 0.6 0.5 1.8 0.4 4.0 1.2 0.7

0.2 3.0 0.4 1.2 2.1 0.2 2.3 1.0 1.1

0.2 2.3 0.5 1.3 1.6 0.2 1.7 1.0 1.0

0.1 0.7 0.0 0.5 1.3 0.1 0.4 0.1 0.3

0.1 0.8 0.0 0.2 1.8 0.1 0.5 0.1 0.2

0.1 0.6 0.0 0.5 0.9 0.1 0.3 0.1 0.5
0.1 0.8 0.1 0.6 1.6 0.1 0.5 0.3 0.5

0.1 0.8 0.1 0.6 1.7 0.1 0.5 0.3 0.5

3.6 1.3 0.6

3.2 1.1 0.6

0.3 3.9 0.0 0.6 3.0 0.3 3.3 0.5 0.8

0.1 1.1 0.2 0.7 1.1 0.1 0.8 0.5 0.6

0.1 1.4 0.2 0.7 1.0 0.1 1.2 0.5 0.6

0.3 4.0 0.0 0.5 2.5 0.3 3.4 0.4 0.7

0.1 1.7 0.0 2.1 1.2 0.1 1.1 0.2 1.4

0.1 0.9 0.0 0.8 0.6 0.1 0.6 0.3 0.6

0.1 1.0 0.1 0.9 0.6 0.1 0.7 0.3 0.8

0.1 1.1 0.0 1.0 0.7 0.1 0.6 0.2 0.8

0.1 0.9 0.0 0.8 0.7 0.1 0.6 0.3 0.6

1.7 0.3 0.3

0.2 2.2 0.2 0.2 1.6 0.2 1.6 0.3 0.3

0.2 3.8 0.1 0.4 1.9 0.2 3.2 0.7 0.6

0.5 4.1 0.2 0.5 3.0 0.5 3.5 0.7 0.7

1.1 0.3 0.3

0.1 1.0 0.0 0.2 1.1 0.1 0.7 0.3 0.2

0.1 0.8 0.0 0.2 1.3 0.2 0.5 0.3 0.3

0.9 0.6 0.3

0.2 1.0 0.3 0.9 2.0 0.2 0.8 0.9 1.0

0.1 0.6 0.0 0.3 1.0 0.1 0.4 0.1 0.3

0.1 0.6 0.0 0.3 1.2 0.1 0.4 0.1 0.3

0.1 0.9 0.0 0.2 1.5 0.2 0.5 0.1 0.2

0.1 0.9 0.0 0.2 1.0 0.1 0.5 0.1 0.2

0.2 4.3 0.1 0.5 1.7 0.2 3.5 0.5 0.7

0.1 1.1 0.2 1.2 1.2 0.2 0.9 0.4 1.1

0.1 0.8 0.0 0.6 1.0 0.1 0.5 0.1 0.5

0.1 0.8 0.0 0.7 1.1 0.1 0.4 0.2 0.6

0.1 0.8 0.0 0.7 1.0 0.1 0.5 0.1 0.7

0.1 0.7 0.0 0.7 0.9 0.1 0.4 0.1 0.7

0.1 0.7 0.0 0.6 1.4 0.1 0.4 0.1 0.5

0.1 2.0 0.0 2.7 2.0 0.1 1.7 0.3 3.3

n. For simplification purposes, the SANDWICH component called "passive" (which is nominally 0.5 ug/m3) was allocated in proportion to 
OC EC Sulfates Nitrates Crustal OC EC Sulfates Nitrates

2.2 0.3 4.4 0.2 1.0 2.5 0.4 3.6 0.6

0.2 0.1 1.1 0.0 0.1 0.8 0.1 1.0 0.1

0.4 0.0 0.6 0.0 0.3 0.5 0.1 0.5 0.1

0.5 0.1

0.4 0.0 0.7 0.0 0.3 0.5 0.1 0.5 0.1

0.9 0.1 0.7 0.1 0.2 1.3 0.1 0.5 0.1

0.6 0.1 1.1 0.0 0.7 0.5 0.1 0.8 0.1

0.4 0.1 1.4 0.0 1.0 0.4 0.1 1.0 0.2

1.2 0.3 1.5 0.0 5.1 1.0 0.3 1.2 0.4

0.6 0.1 1.1 0.0 1.4 0.6 0.1 0.8 0.2

0.6 0.1 1.0 0.0 0.8 0.7 0.1 0.7 0.2

1.0 0.2 1.0 0.0 2.7 0.8 0.2 0.8 0.2

0.8 0.1 1.4 0.0 1.2 0.8 0.1 1.1 0.3

0.9 0.1 1.2 0.0 0.9 1.0 0.2 0.9 0.2

0.5 0.1 1.2 0.0 1.2 0.5 0.1 0.8 0.2

0.6 0.2 1.1 0.0 1.2 0.9 0.2 0.8 0.2

0.4 0.1 1.6 0.0 1.4 0.5 0.1 1.4 0.4

0.6 0.1 1.5 0.0 1.5 0.6 0.2 1.1 0.4

0.6 0.1 1.5 0.0 2.2 0.6 0.2 1.3 0.4

0.6 0.1 1.5 0.0 1.3 0.5 0.2 1.2 0.4

1.8 0.2 3.5 0.4 1.2 2.1 0.2 2.7 1.0

1.8 0.2 3.6 0.3 1.4 2.0 0.2 2.8 0.8

0.7 0.1 0.7 0.0 0.6 0.8 0.1 0.6 0.1

0.9 0.1 1.0 0.0 1.0 1.2 0.1 0.7 0.3

0.6 0.1 1.2 0.0 1.2 0.6 0.1 0.9 0.2

1.5 0.2 1.4 0.0 1.0 2.2 0.2 1.2 0.6

0.6 0.2 1.0 0.0 1.1 0.6 0.2 0.8 0.5

0.4 0.1 1.7 0.3 0.3 2.5 0.1 1.1 0.7

0.8 0.1 0.9 0.0 0.7 1.1 0.1 0.8 0.3

0.5 0.1 0.7 0.0 0.8 0.5 0.1 0.5 0.1

1.1 0.2 2.0 0.0 0.7 1.9 0.3 1.5 0.9

0.9 0.1 1.3 0.0 0.5 1.7 0.2 1.0 0.6

0.8 0.1 1.3 0.0 0.9 1.1 0.2 0.9 0.5

0.9 0.2 1.2 0.0 0.7 1.6 0.2 0.9 1.1

0.9 0.1 1.4 0.0 0.9 1.5 0.1 1.1 0.6

0.9 0.1 0.7 0.0 0.7 0.9 0.1 0.5 0.1

0.7 0.1 0.7 0.0 0.6 0.8 0.1 0.5 0.1

0.7 0.1 0.7 0.0 0.5 0.9 0.1 0.5 0.1

1.9 0.2 1.7 0.2 0.9 2.9 0.2 1.5 1.4

Speciation Measuremen

2010 Annual Average

tion Measurements SANDWICHed*
0.6 0.1 0.8 0.0 1.5 0.5 0.1 0.6 0.2

0.5 0.0 0.8 0.0 0.7 0.4 0.1 0.5 0.1

0.6 0.1 0.9 0.0 2.2 0.3 0.1 0.6 0.2

0.6 0.1 0.9 0.0 0.8 0.6 0.1 0.6 0.2

0.5 0.1 0.9 0.0 1.7 0.4 0.1 0.7 0.2

0.3 0.1 0.7 0.0 1.0 0.3 0.1 0.5 0.1

1.9 0.9 4.5 0.6 0.9 2.4 1.0 3.1 1.1

1.9 0.3 3.6 0.0 1.2 2.1 0.4 2.7 0.4

0.9 0.2 3.1 0.0 1.2 1.2 0.2 2.1 0.4

2.0 0.3 4.2 0.0 1.0 2.5 0.3 2.8 0.3

2.1 0.3 4.3 0.0 1.0 2.4 0.3 2.8 0.3

2.0 0.3 4.5 0.1 0.9 2.2 0.3 3.1 0.4

0.5 0.1 0.8 0.0 1.3 0.4 0.1 0.6 0.1

1.3 0.2 2.6 0.1 0.5 1.5 0.2 2.1 0.6

1.5 0.2 2.9 1.2 0.9 1.6 0.2 2.3 1.7

1.0 0.1 2.1 0.7 1.1 1.1 0.1 1.5 1.0

2.0 0.3 5.1 0.8 0.8 1.9 0.4 3.5 1.0

2.2 0.3 5.1 1.0 0.9 2.8 0.4

1.8 0.4 4.7 0.1 1.4 2.1 0.4 3.6 0.5

2.2 0.3 3.8 0.0 1.3 2.8 0.3

1.4 0.2 1.5 0.1 0.6 1.8 0.2 1.3 0.2

1.1 0.2 1.8 0.0 0.3 1.5 0.2 1.5 0.2

1.5 0.3 2.0 0.0 0.4 1.9 0.3 1.6 0.3

1.0 0.1 1.8 0.0 0.3 1.3 0.1 1.4 0.3

1.5 0.3 1.8 0.0 0.4 1.9 0.3 1.5 0.3

1.0 0.1 1.6 0.0 0.3 1.1 0.1 1.3 0.2

1.5 0.3 4.9 0.4 0.7 1.2 0.3 3.5 0.6

1.1 0.1 2.5 0.0 0.4 1.9 0.2 1.9 0.4

1.2 0.2 2.8 0.1 0.4 2.3 0.2 2.3 0.6

1.4 0.2 2.6 0.1 0.4 1.7 0.3 1.9 0.5

1.0 0.1 1.7 0.4 0.4 1.2 0.1 1.3 0.5

1.1 0.1 2.0 0.5 0.4 1.3 0.2 1.6 0.6

1.0 0.1 1.5 0.2 0.4 1.2 0.1 1.1 0.5

1.1 0.2 2.3 2.0 1.1 1.5 0.2 1.7 1.8

1.1 0.1 1.5 0.3 0.5 1.4 0.1 1.1 0.5

1.4 0.2 2.3 1.7 0.7 1.7 0.3 2.0 2.1

1.7 0.3 3.4 1.3 1.1 1.8 0.3 2.7 1.6

2.6 0.4 4.1 0.8 1.9 3.1 0.4 3.0 1.2

0.0 0.0 4.4 0.0 0.4 0.3 0.0

0.3 0.0 1.8 0.0 0.3 0.5 0.1 1.2 0.2

0.0 0.0 1.2 0.0 0.4 0.1 0.0 0.7 0.1

0.5 0.1 0.7 0.1 0.9 0.5 0.1 0.5 0.5
1.3 0.1 0.6 0.0 0.7 0.9 0.2 0.4 0.1

1.6 0.3 3.8 2.2 0.7 2.1 0.4 3.2 2.2

1.9 0.4 5.7 1.2 0.8 2.5 0.4

1.3 0.3 2.7 2.1 0.9 1.9 0.3 2.2 2.1

1.4 0.2 2.8 2.2 0.8 2.0 0.3 2.6 2.1

1.7 0.3 2.8 1.8 1.1 1.9 0.3

1.9 0.3 3.5 0.7 1.0 2.0 0.3 2.8 1.2

0.7 0.1 1.1 0.4 0.6 0.8 0.1 0.8 0.2

1.4 0.2 0.7 0.1 0.7 1.7 0.3 0.6 0.2

0.9 0.1 0.7 0.0 0.6 1.1 0.1 0.5 0.1

0.6 0.1 0.7 0.0 0.7 0.6 0.1 0.4 0.1

1.1 0.1 0.6 0.0 1.0 1.3 0.1 0.5 0.1

0.7 0.1 0.6 0.0 0.6 0.8 0.1 0.5 0.1

1.1 0.1 1.9 0.8 1.0 1.0 0.1 1.2 0.7

0.6 0.1 1.1 0.2 0.7 0.6 0.1 0.7 0.2

0.9 0.1 0.7 0.0 0.6 1.1 0.1 0.5 0.1

0.9 0.1 1.7 0.7 0.7 0.9 0.1 1.1 0.6

0.7 0.1 1.6 0.6 0.8 0.9 0.1 1.0 0.7

0.8 0.1 1.9 0.8 0.7 0.9 0.1 1.4 0.9

0.8 0.1 0.8 0.0 0.9 0.7 0.1 0.5 0.1

0.9 0.1 1.8 0.0 0.2 1.1 0.1 1.6 0.2

1.1 0.2 2.2 0.0 0.4 1.3 0.2 1.6 0.3

1.9 0.4

1.6 0.3 4.0 0.5 0.6 1.9 0.3 3.0 1.0

0.6 0.1 1.2 0.0 0.9 0.6 0.1 0.8 0.1

0.8 0.1 2.0 0.2 1.5 0.9 0.1 1.7 0.6

0.7 0.1 1.5 0.0 1.3 0.5 0.1 1.5 0.2

0.7 0.1 1.0 0.0 0.8 0.6 0.1 0.8 0.2

0.5 0.1 0.9 0.0 1.0 0.4 0.1 0.6 0.2

0.7 0.1 1.2 0.0 1.0 0.5 0.1 0.9 0.3

0.4 0.1 0.8 0.0 0.8 0.4 0.1 0.6 0.2

1.9 0.3 4.1 0.0 0.7 2.3 0.3 2.6 0.2

1.6 0.2 3.5 0.0 0.8 1.8 0.2 2.4 0.3

0.9 0.1 1.7 0.7 0.9 0.8 0.2 1.1 0.5

1.1 0.2 2.1 0.8 0.9 1.1 0.2 1.2 0.8

1.6 0.4 5.2 1.0 0.7 1.7 0.4 4.1 0.9

2.9 1.3

1.4 0.2 3.1 0.4 1.2 1.7 0.2 2.3 1.1

1.0 0.2 2.3 0.6 1.1 1.1 0.2 1.8 1.0

0.4 0.1 0.7 0.0 0.4 0.7 0.1 0.5 0.2

1.1 0.1 0.8 0.0 0.2 1.8 0.1 0.6 0.1

0.6 0.1 0.5 0.0 0.7 0.6 0.1 0.4 0.1
0.8 0.1 0.8 0.1 0.6 1.0 0.1 0.5 0.2

1.0 0.1 0.8 0.1 0.6 1.2 0.1 0.6 0.4

1.8 0.3 4.7 0.7 0.6 2.0 0.4

2.1 0.4 4.2 0.7 0.6 2.4 0.5

2.0 0.3 4.4 0.0 0.8 2.7 0.3 3.1 0.4

1.2 0.1 1.1 0.3 0.7 1.1 0.1 0.9 0.3

0.8 0.1 1.6 0.2 0.8 0.7 0.1 1.0 0.4

1.8 0.3 4.5 0.1 0.8 2.3 0.3 3.2 0.3

0.6 0.1 1.6 0.0 1.6 0.5 0.1 1.2 0.3

0.6 0.1 0.9 0.1 0.7 0.5 0.1 0.6 0.2

0.5 0.1 1.0 0.2 0.9 0.4 0.1 0.7 0.2

0.6 0.1 1.0 0.0 1.0 0.6 0.1 0.7 0.2

0.5 0.1 0.9 0.1 0.8 0.4 0.1 0.6 0.2

0.9 0.1 2.4 0.0 0.4 1.1 0.2 1.6 0.4

1.3 0.2 2.3 0.2 0.3 1.5 0.2 1.7 0.4

1.3 0.2 4.3 0.2 0.6 1.6 0.2 2.9 0.6

2.3 0.5 4.6 0.2 0.7 2.6 0.5 3.2 0.6

0.7 0.2

1.1 0.2 1.6 0.0 0.4 2.6 0.2

0.6 0.1 1.1 0.0 0.3 1.0 0.1 0.7 0.2

0.7 0.1 0.8 0.0 0.3 0.9 0.2 0.6 0.2

1.2 0.2 1.3 0.1 0.4 1.6 0.2 0.9 0.6

1.2 0.2 1.1 0.5 1.1 1.4 0.3 0.7 0.5

0.4 0.0 0.7 0.0 0.4 0.6 0.1 0.4 0.1

0.8 0.1 0.6 0.0 0.4 1.0 0.1 0.4 0.1

0.7 0.1 0.9 0.0 0.3 1.1 0.2 0.6 0.1

0.7 0.1 0.8 0.0 0.3 1.0 0.1 0.6 0.1

1.6 0.2 4.7 0.2 0.7 1.5 0.2 3.4 0.5

0.7 0.1 1.2 0.2 1.3 0.6 0.1 0.8 0.3

0.5 0.0 0.7 0.0 0.6 0.6 0.1 0.6 0.1

0.4 0.0 0.7 0.0 0.8 0.5 0.1 0.5 0.1

0.5 0.1 0.8 0.0 0.8 0.4 0.1 0.5 0.1

0.5 0.1 0.7 0.0 0.9 0.4 0.1 0.5 0.1

0.5 0.1 0.7 0.0 0.7 0.6 0.1 0.5 0.2

0.2 0.2 2.2 0.0 3.5 1.2 0.2 1.4 0.3

as allocated in proportion to the concentration value of the five PM2.5 constituents which now sum to the IMPROVE sampler's mass mea
Crustal OC EC Sulfates Nitrates Crustal OC EC Sulfates

0.4 2.6 0.4 4.8 0.1 0.4 3.5 0.4 2.5

0.1 0.2 0.1 1.5 0.0 0.1 1.4 0.1 0.7

0.1 0.3 0.0 0.9 0.0 0.2 0.3 0.1 0.4

0.1 0.2 0.0 0.9 0.0 0.1 0.6 0.0 0.4

0.1 0.3 0.0 0.9 0.0 0.1 0.4 0.1 0.3

0.1 0.4 0.0 0.9 0.0 0.1 0.5 0.1 0.5

0.7 0.6 0.1 1.2 0.0 0.9 0.8 0.1 0.8

1.2 0.8 0.1 1.4 0.0 1.3 1.0 0.1 1.1

3.8 1.4 0.3 1.6 0.0 4.0 2.4 0.3 1.3

0.9 0.8 0.1 1.2 0.0 1.1 1.1 0.1 0.8

0.6 0.7 0.1 1.1 0.0 0.8 0.9 0.1 0.7

2.3 1.0 0.2 1.1 0.0 2.6 1.3 0.2 0.8

1.4 0.7 0.1 1.5 0.0 1.6 1.0 0.1 1.1

0.9 1.1 0.2 1.3 0.0 1.0 1.4 0.2 0.9

1.1 0.6 0.1 1.2 0.0 1.3 0.8 0.1 0.9

0.9 0.7 0.2 1.2 0.0 1.0 0.9 0.2 0.9

1.8 0.5 0.1 1.9 0.0 2.0 0.9 0.1 1.4

1.5 0.7 0.1 1.6 0.0 1.7 1.2 0.2 1.1

2.3 0.7 0.2 1.8 0.0 2.5 1.3 0.2 1.3

1.9 0.7 0.1 1.7 0.0 2.1 1.2 0.1 1.3

0.7 2.0 0.3 3.6 0.3 0.7 3.1 0.3 2.3

0.5 2.0 0.2 3.8 0.2 0.6 2.8 0.3 2.6

0.3 0.9 0.1 0.9 0.0 0.4 1.3 0.1 0.6

0.4 0.9 0.1 1.0 0.0 0.5 1.3 0.1 0.8

1.0 0.5 0.1 1.3 0.0 1.1 0.8 0.1 0.9

0.7 1.4 0.2 1.7 0.1 0.8 2.1 0.2 1.0

1.0 0.7 0.2 1.1 0.0 1.2 1.1 0.2 0.9

0.9

0.1 0.5 0.1 1.5 0.2 0.2 2.8 0.1 0.9

0.4 1.2 0.1 1.1 0.0 0.5 1.8 0.1 0.8

0.4 0.5 0.1 0.8 0.0 0.5 0.7 0.1 0.5

0.5 1.1 0.2 2.0 0.0 0.6 2.2 0.2 1.4

0.3 1.0 0.1 1.5 0.0 0.4 2.0 0.2 0.9

0.7 0.7 0.1 1.4 0.0 0.8 1.0 0.1 1.1

0.5 0.9 0.1 1.3 0.1 0.6 1.6 0.2 1.0

0.6 0.8 0.1 1.5 0.0 0.7 1.6 0.1 1.0

0.3 0.8 0.1 0.8 0.0 0.4 1.1 0.1 0.5

0.3 0.8 0.1 0.8 0.0 0.3 1.2 0.1 0.5

0.2 1.2 0.1 0.8 0.0 0.3 1.7 0.1 0.5

0.7 2.0 0.2 2.0 0.6 0.7 3.2 0.3 1.3

2011 Annual Average

Speciation Measurements SANDWICHed*
1.1 0.9 0.1 0.9 0.0 1.3 1.1 0.1 0.6

0.4 0.4 0.0 0.8 0.0 0.5 0.5 0.1 0.5

1.1 0.6 0.1 0.9 0.1 1.3 0.8 0.1 0.6

0.5 0.6 0.1 0.9 0.0 0.7 0.7 0.1 0.6

0.9 0.5 0.1 1.0 0.0 1.1 0.6 0.1 0.7

0.6 0.3 0.1 0.8 0.0 0.8 0.5 0.1 0.5

0.6 2.1 0.9 4.1 0.4 0.6 3.2 0.9 2.6

0.5 2.0 0.3 3.6 0.0 0.5 2.8 0.4 2.2

0.6 1.2 0.2 2.9 0.0 0.7 2.4 0.2 2.0

0.4 2.2 0.3 3.8 0.0 0.5 3.3 0.3 2.3

0.5 3.1 0.3 3.8 0.0 0.5 4.2 0.4 2.4

0.3 2.3 0.3 4.1 0.0 0.4 3.1 0.3 2.4

0.6

0.6 0.5 0.1 0.9 0.0 0.8 0.5 0.1 0.6

0.2 1.3 0.2 2.9 0.1 0.2 1.8 0.2 1.7

0.7 1.8 0.3 3.0 1.2 0.8 2.5 0.3 2.0

0.8 1.1 0.1 2.0 0.5 0.9 1.6 0.2 1.4

0.3 2.1 0.3 4.6 0.5 0.4 2.7 0.3 2.9

0.6 1.7 0.3 4.9 0.0 0.6 2.6 0.4 2.8

0.3 1.3 0.2 1.8 0.1 0.3 1.9 0.2 1.1

0.1 1.3 0.2 2.2 0.0 0.1 1.8 0.2 1.2

0.1 1.8 0.3 2.3 0.1 0.2 2.7 0.3 1.3

0.1 1.0 0.1 2.0 0.0 0.1 1.6 0.1 1.1

0.2 1.7 0.3 2.1 0.1 0.2 2.3 0.3 1.3

0.1 1.0 0.1 1.9 0.1 0.1 1.5 0.1 1.1

0.3 1.5 0.3 4.7 0.2 0.3 1.8 0.3 2.9

0.2 1.2 0.2 2.6 0.1 0.2 2.4 0.2 1.6

0.2 1.3 0.2 3.1 0.1 0.2 2.8 0.2 1.7

0.2 1.5 0.3 2.6 0.2 0.2 1.9 0.3 1.5

0.2 1.2 0.1 1.8 0.3 0.2 1.7 0.1 1.1

0.2 1.1 0.1 2.1 0.5 0.2 1.3 0.2 1.4

0.2 1.5 0.1 1.5 0.3 0.2 2.0 0.1 1.0

0.7 1.1 0.2 2.3 1.2 0.7 2.1 0.2 1.5

0.2 1.0 0.1 1.5 0.4 0.3 1.4 0.1 1.0

0.3 1.4 0.2 2.6 1.7 0.4 1.9 0.3 1.6

0.8 2.0 0.3 3.6 1.1 0.9 2.7 0.3 2.3

0.9 2.4 0.4 3.8 0.6 1.0 3.3 0.4 2.3

0.2 0.3 0.0 1.8 0.0 0.2 0.8 0.1

0.2 0.0 0.0 1.2 0.0 0.2 0.1 0.0 0.9

0.4 0.8 0.1 0.8 0.3 0.5 0.9 0.1 0.5
0.3 1.1 0.1 0.7 0.0 0.4 1.3 0.1 0.4

0.4 1.7 0.3 4.2 1.4 0.4 2.7 0.4 2.4

0.6 1.5 0.3 2.9 1.5 0.7 2.5 0.3 2.0

0.4 1.6 0.3 3.3 1.6 0.5 2.7 0.3 2.1

0.5 2.0 0.3 3.6 0.8 0.6 2.5 0.3 2.2

0.4 0.7 0.1 1.1 0.2 0.5 0.9 0.1 0.6

0.4 1.5 0.2 0.9 0.1 0.4 2.1 0.3 0.5

0.3 1.0 0.1 0.8 0.0 0.3 1.3 0.1 0.4

0.3 0.6 0.1 0.7 0.0 0.4 0.8 0.1 0.4

0.4 1.1 0.1 0.8 0.0 0.4 1.5 0.1 0.4

0.3 1.4 0.1 0.7 0.0 0.3 1.9 0.1 0.4

0.5 0.9 0.1 1.6 0.5 0.6 1.0 0.1 1.0

0.4 0.9 0.1 1.1 0.1 0.5 1.2 0.1 0.7

0.3 0.9 0.1 0.8 0.0 0.4 1.2 0.1 0.4

0.6 0.8 0.1 1.4 0.4 0.7 0.9 0.1 1.1

0.5 0.8 0.1 1.4 0.3 0.6 1.3 0.1 0.8

0.5 0.9 0.1 1.9 0.6 0.6 1.3 0.1 1.1

0.4 0.5 0.1 0.9 0.0 0.6 0.5 0.1 0.5

0.1 1.3 0.1 2.2 0.0 0.1 1.9 0.2 1.1

0.2 1.1 0.2 2.2 0.1 0.2 1.5 0.2 1.3

0.2 2.0 0.3 2.5 0.1 0.2 2.9 0.4 1.5

0.3 1.8 0.3 4.0 0.3 0.3 2.9 0.3 2.3

0.9 1.0 0.1 1.2 0.0 1.0 1.3 0.1 0.9

2.2 1.1 0.1 2.3 0.2 2.3 2.0 0.1 1.6

1.4 0.9 0.1 2.1 0.0 1.6 1.5 0.1 1.1

0.8 1.3 0.2 1.1 0.0 0.9 1.6 0.2 0.8

0.9 1.0 0.1 1.0 0.0 1.1 1.3 0.1 0.7

1.3 0.9 0.1 1.3 0.1 1.4 1.2 0.2 1.0

0.6 0.6 0.1 1.0 0.0 0.8 0.8 0.1 0.6

0.3 1.8 0.3 3.6 0.0 0.3 2.8 0.3 2.1

0.4 1.5 0.2 3.3 0.0 0.4 2.0 0.2 1.9

0.6 0.8 0.1 1.5 0.3 0.7 1.1 0.2 0.9

0.6 0.9 0.2 1.6 0.5 0.7 1.2 0.2 1.1

0.3 1.6 0.3 5.4 0.5 0.4 1.9 0.3 3.1

0.6 2.7 0.4 3.8 0.6 0.7 3.8 0.4 2.5

1.0 1.7 0.2 3.1 0.5 1.1 2.6 0.2 2.0

1.2 1.4 0.2 2.4 0.4 1.3 2.1 0.2 1.6

0.2 0.9 0.1 0.7 0.0 0.2 1.4 0.1 0.5

0.1 1.2 0.1 0.9 0.0 0.2 1.9 0.1 0.5

0.2 0.7 0.1 0.7 0.0 0.3 0.9 0.1 0.4
0.4 1.2 0.1 0.8 0.1 0.5 1.7 0.1 0.5

0.4 1.0 0.1 0.9 0.2 0.4 1.3 0.1 0.5

0.4 2.3 0.3 4.2 0.0 0.4 3.7 0.3 2.4

0.4 0.8 0.1 1.3 0.2 0.5 0.9 0.1 0.7

0.5 0.8 0.1 1.4 0.2 0.5 1.0 0.1 0.9

0.3 1.8 0.3 4.3 0.0 0.3 2.9 0.3 2.4

2.5 0.9 0.1 1.7 0.0 2.7 1.9 0.1 1.4

0.5 0.6 0.1 1.0 0.1 0.6 0.7 0.1 0.6

0.6 0.4 0.1 1.1 0.1 0.7 0.5 0.1 0.7

0.7 0.6 0.1 1.1 0.0 0.9 0.6 0.1 0.7

0.6 0.5 0.1 1.0 0.0 0.7 0.6 0.1 0.6

0.1 0.9 0.1 2.3 0.1 0.2 1.3 0.2

0.1 1.3 0.2 2.3 0.3 0.2 1.8 0.2 1.4

0.2 1.3 0.2 3.9 0.1 0.3 2.2 0.2 2.4

0.3 2.4 0.5 4.2 0.2 0.3 3.2 0.5 2.5

0.1 0.4 0.0 1.1 0.0 0.1 1.0 0.1 0.6

0.1 0.6 0.1 1.2 0.0 0.1 1.1 0.1 0.6

0.1 0.7 0.1 0.9 0.0 0.1 1.0 0.2 0.5

0.2 1.3 0.2 1.3 0.1 0.2 2.0 0.2

0.8 1.2 0.2 1.0 0.2 0.9 1.7 0.2 0.7

0.1 0.4 0.0 0.6 0.0 0.1 0.6 0.1 0.4

0.2 0.6 0.1 0.7 0.0 0.2 0.8 0.1 0.4

0.1 0.9 0.1 1.0 0.0 0.2 1.5 0.2 0.5

0.1 0.6 0.1 1.0 0.0 0.1 0.8 0.1 0.5

0.3 1.5 0.2 4.5 0.1 0.3 2.0 0.2 2.6

0.7 0.8 0.1 1.1 0.2 0.8 1.0 0.1 0.7

0.4 0.6 0.1 0.9 0.0 0.6 0.8 0.1 0.5

0.4 0.7 0.1 0.8 0.0 0.5 0.8 0.1 0.5

0.4 0.5 0.1 0.8 0.0 0.5 0.6 0.1 0.5

0.4 0.5 0.1 0.8 0.0 0.5 0.6 0.1 0.5

0.3 0.9 0.1 0.8 0.1 0.4 1.2 0.1 0.5

1.7 0.2 0.0 1.9 0.0 1.8 2.3 0.1 1.5

MPROVE sampler's mass measurement.
Nitrates Crustal OC EC Sulfates Nitrates Crustal OC EC

0.5 0.6 1.9 0.3 3.4 0.0 0.6 2.9 0.3

0.1 0.1 0.2 0.1 1.1 0.0 0.1 1.2 0.1

0.1 0.2 0.4 0.0 0.7 0.1 0.2 0.3 0.1

0.1 0.1 0.2 0.0 0.7 0.0 0.1 0.6 0.0

0.1 0.1 0.3 0.0 0.6 0.0 0.2 0.4 0.1

0.1 0.1 0.3 0.0 0.8 0.0 0.1 0.4 0.1

0.2 0.8 0.9 0.1 1.2 0.0 1.0 1.1 0.1

0.3 1.1 0.5 0.1 1.6 0.0 1.3 0.6 0.1

0.3 4.5 1.3 0.2 1.7 0.0 4.8 2.0 0.3

0.2 1.3 0.8 0.1 1.2 0.0 1.4 1.2 0.1

0.2 0.9 0.5 0.1 1.0 0.0 1.1 0.7 0.1

0.3 4.0 1.2 0.2 1.0 0.0 4.3 1.4 0.2

0.3 1.5 0.8 0.1 1.6 0.0 1.7 1.2 0.1

0.2 1.2 1.0 0.2 1.3 0.0 1.4 1.2 0.2

0.2 1.2 0.5 0.1 1.3 0.0 1.4 0.7 0.1

0.2 1.2 0.7 0.2 1.2 0.0 1.4 1.0 0.2

0.3 1.5 0.5 0.1 1.9 0.0 1.6 0.7 0.1

0.3 1.6 0.7 0.1 1.6 0.0 1.8 1.0 0.1

0.5 3.4 0.8 0.2 1.8 0.0 3.6 1.2 0.2

0.3 1.9 0.7 0.1 1.8 0.0 2.1 1.1 0.1

0.6 1.0 1.7 0.2 3.2 0.0 1.0 2.6 0.3

0.6 1.1 1.5 0.2 3.5 0.1 1.1 2.4 0.2

0.2 0.5 0.9 0.1 0.9 0.0 0.5 1.2 0.1

0.4 0.7 0.7 0.1 1.1 0.0 0.9 1.1 0.1

0.2 1.6 0.6 0.1 1.3 0.0 1.8 0.9 0.1

0.6 1.1 1.1 0.1 1.4 0.1 1.2 1.9 0.2

0.5 1.0 1.0 0.2 1.2 0.0 1.2 1.8 0.2

0.7 0.6 0.7 0.1 1.3 0.0 0.8 1.0 0.1

0.6 0.2 0.4 0.1 1.3 0.2 0.2 2.9 0.1

0.3 0.7 1.0 0.1 1.2 0.0 0.8 1.6 0.1

0.1 0.6 0.5 0.1 0.8 0.0 0.8 0.7 0.1

1.0 0.6 1.0 0.2 2.0 0.0 0.7 2.0 0.2

0.6 0.4 0.9 0.1 1.2 0.0 0.4 1.9 0.1

0.6 1.0 0.7 0.1 1.5 0.0 1.2 1.1 0.1

1.0 0.7 0.9 0.1 1.4 0.0 0.8 1.4 0.2

0.6 0.6 0.7 0.1 1.4 0.0 0.7 1.4 0.1

0.2 0.5 1.5 0.2 0.7 0.0 0.5 2.0 0.2

0.2 0.5 1.8 0.2 0.7 0.0 0.6 2.5 0.2

0.2 0.4 1.5 0.1 0.8 0.0 0.5 2.2 0.1

1.3 1.0 1.8 0.2 1.7 0.4 1.1 3.0 0.2

2012 Annual Average

Speciation Measurements SANDWICHed*
0.2 1.2 0.9 0.1 0.9 0.0 1.4 1.0 0.1

0.2 0.5 1.0 0.1 0.8 0.0 0.7 1.5 0.1

0.2 1.7 1.1 0.1 0.9 0.0 1.9 1.4 0.1

0.2 0.7 1.0 0.1 0.8 0.0 0.9 1.4 0.1

0.2 1.2 0.6 0.1 1.0 0.0 1.4 0.9 0.1

0.1 0.7 0.6 0.1 0.7 0.0 0.9 0.9 0.1

1.2 0.5 1.8 0.8 3.4 0.4 0.6 3.0 0.8

0.4 0.7 1.8 0.3 3.0 0.0 0.8 2.7 0.3

0.4 1.4 0.9 0.1 2.8 0.0 1.5 1.9 0.1

0.3 0.7 1.5 0.2 3.1 0.0 0.8 2.3 0.2

0.4 0.6 1.9 0.2 3.2 0.0 0.7 2.7 0.3

0.4 0.6 1.8 0.2 3.3 0.0 0.6 2.4 0.2

0.1 0.8 0.9 0.1 0.8 0.0 0.9 1.3 0.1

0.1 0.9 0.8 0.1 0.9 0.0 1.0 1.0 0.1

0.6 0.2 1.2 0.2 2.3 0.1 0.2 1.7 0.2

1.2 1.1 1.5 0.2 2.7 0.6 1.2 2.1 0.2

0.9 1.7 1.1 0.1 1.9 0.4 1.9 1.6 0.2

0.8 0.5 1.7 0.3 3.9 0.2 0.6 2.5 0.3

0.5 1.2 1.4 0.3 3.8 0.0 1.3 2.2 0.3

0.3 0.3 1.3 0.2 1.5 0.1 0.3 1.9 0.2

0.3 0.2 1.3 0.2 1.8 0.0 0.2 1.9 0.2

0.4 0.1 1.6 0.3 1.8 0.1 0.2 2.6 0.3

0.3 0.1 0.9 0.1 1.7 0.0 0.2 1.6 0.1

0.3 0.2 1.5 0.3 1.8 0.0 0.3 2.3 0.3

0.2 0.1 0.9 0.1 1.6 0.0 0.2 1.3 0.1

0.6 0.4 1.3 0.3 3.9 0.2 0.4 1.6 0.3

0.5 0.2 1.0 0.2 2.2 0.0 0.2 2.3 0.2

0.6 0.2 1.0 0.1 2.3 0.1 0.2 2.4 0.2

0.6 0.2 1.3 0.2 2.2 0.1 0.2 1.7 0.3

0.5 0.2 0.9 0.1 1.5 0.3 0.2 1.3 0.1

0.5 0.2 0.9 0.1 1.9 0.3 0.2 1.2 0.2

0.5 0.3 1.0 0.1 1.3 0.3 0.3 1.4 0.1

1.9 1.1 1.2 0.2 2.0 1.0 1.2 2.3 0.2

0.6 0.3 1.0 0.1 1.3 0.5 0.3 1.3 0.1

1.7 0.5 1.3 0.2 2.2 1.3 0.6 1.8 0.2

1.2 1.6 1.8 0.3 3.0 0.5 1.7 2.6 0.3

0.8 1.3 2.0 0.3 3.0 0.2 1.3 3.0 0.4

0.1 0.2 0.0 0.0 1.4 0.0 0.3 0.1 0.0

0.3 0.7 2.3 0.2 0.7 0.1 0.8 3.5 0.2
0.1 0.5 3.4 0.3 0.6 0.0 0.6 4.7 0.3

1.7 0.5 1.5 0.3 3.2 0.9 0.6 2.6 0.3

2.0 1.0 1.5 0.3 2.5 1.4 1.1 2.5 0.3

1.7 0.7 1.4 0.3 2.8 1.1 0.8 2.3 0.3

0.7 0.8 1.8 0.3 3.0 0.2 0.9 2.5 0.3

0.2 0.8 1.0 0.1 0.9 0.1 1.0 1.4 0.1

0.2 0.5 1.8 0.2 0.7 0.1 0.6 2.6 0.3

0.1 0.5 1.4 0.1 0.6 0.0 0.5 2.2 0.1

0.1 0.4 1.7 0.1 0.6 0.0 0.5 2.3 0.1

0.1 1.3 2.2 0.2 0.6 0.0 1.4 3.0 0.2

0.2 0.4 5.4 0.4 0.6 0.0 0.4 7.5 0.5

0.7 0.7 0.9 0.1 1.4 0.5 0.8 1.0 0.1

0.3 0.7 1.9 0.2 1.0 0.1 0.8 3.0 0.2

0.1 0.4 1.3 0.1 0.6 0.0 0.5 1.9 0.1

0.7 1.1 1.0 0.1 1.4 0.5 1.2 1.3 0.2

0.4 0.9 0.9 0.1 1.2 0.1 1.0 1.5 0.1

0.7 1.4 1.0 0.1 1.6 0.4 1.5 1.6 0.1

0.1 0.7 0.6 0.1 0.8 0.0 0.9 0.9 0.1

0.2 0.1 1.0 0.1 1.6 0.0 0.2 1.5 0.1

0.4 0.2 0.9 0.2 1.8 0.1 0.2 1.4 0.2

0.5 0.2 1.8 0.3 2.0 0.2 0.3 2.6 0.4

0.9 0.3 1.4 0.3 3.2 0.2 0.3 2.2 0.3

0.1 1.2 1.0 0.1 1.2 0.0 1.3 1.3 0.1

0.6 1.7 0.9 0.1 2.2 0.1 1.9 1.6 0.1

0.2 1.3 0.8 0.1 1.5 0.0 1.4 1.4 0.1

0.2 0.9 0.8 0.1 1.2 0.0 1.1 1.1 0.1

0.2 1.0 0.6 0.1 1.0 0.0 1.2 0.8 0.1

0.3 1.5 1.5 0.2 1.3 0.0 1.7 2.2 0.2

0.2 0.7 0.6 0.1 0.9 0.0 0.9 0.8 0.1

0.2 0.4 1.7 0.3 2.9 0.0 0.4 2.7 0.3

0.3 0.4 1.1 0.1 2.7 0.0 0.4 1.7 0.2

0.5 0.8 0.9 0.1 1.2 0.3 0.9 1.2 0.2

0.8 1.2 0.8 0.2 1.5 0.5 1.4 1.2 0.2

0.8 0.4 1.4 0.3 4.1 0.4 0.5 2.0 0.3

0.9 1.1 2.1 0.3 3.3 0.3 1.2 3.1 0.3

0.9 1.4 1.2 0.2 2.7 0.3 1.5 2.0 0.2

0.8 1.3 1.2 0.2 2.2 0.3 1.5 1.7 0.2

0.2 0.7 1.0 0.1 0.7 0.0 0.8 1.8 0.1

0.1 0.2 1.0 0.1 0.7 0.0 0.2 1.8 0.1

0.1 0.5 0.9 0.1 0.7 0.0 0.6 1.1 0.1
0.2 0.6 1.3 0.1 0.7 0.0 0.7 2.0 0.1

0.2 0.7 1.7 0.1 0.7 0.0 0.8 2.7 0.2

0.5 0.5 1.8 0.3 3.2 0.0 0.6 2.7 0.3

0.3 0.8 0.9 0.1 1.0 0.1 0.9 1.3 0.1

0.3 0.8 0.9 0.1 1.2 0.1 0.9 1.2 0.1

0.3 0.5 1.5 0.2 3.3 0.0 0.5 2.3 0.2

0.3 1.9 0.9 0.1 2.0 0.0 2.1 1.2 0.1

0.2 0.8 0.6 0.1 0.9 0.0 0.9 0.8 0.1

0.2 0.9 0.7 0.1 1.0 0.0 1.1 0.9 0.1

0.2 0.9 0.6 0.1 1.1 0.0 1.1 0.8 0.1

0.2 0.8 0.7 0.1 0.9 0.0 1.0 1.1 0.1

0.4 0.2 1.0 0.2 1.9 0.1 0.2 1.6 0.2

0.6 0.3 1.1 0.2 3.3 0.0 0.3 1.9 0.2

0.5 0.4 2.3 0.5 3.4 0.1 0.4 3.2 0.5

0.2 0.1 0.4 0.0 0.9 0.0 0.1 1.0 0.1

0.2 0.1 0.7 0.1 0.9 0.0 0.1 1.1 0.1

0.2 0.2 1.4 0.2 0.7 0.0 0.2 2.1 0.2

0.5 0.6 1.6 0.2 1.0 0.2 0.7 2.9 0.3

0.1 0.2 1.3 0.1 0.6 0.0 0.3 1.9 0.1

0.1 0.3 1.3 0.1 0.6 0.0 0.3 1.9 0.1

0.1 0.2 1.1 0.1 0.8 0.0 0.2 1.9 0.2

0.1 0.1 0.8 0.1 0.8 0.0 0.2 1.3 0.1

0.4 0.4 1.2 0.2 3.6 0.1 0.4 1.6 0.2

0.3 1.3 1.4 0.2 1.0 0.2 1.4 1.9 0.2

0.1 0.6 1.2 0.1 0.7 0.0 0.7 1.7 0.1

0.2 0.7 1.4 0.1 0.8 0.0 0.8 2.1 0.1

0.2 0.6 1.3 0.1 0.7 0.0 0.7 1.9 0.1

0.1 0.6 1.2 0.1 0.7 0.0 0.7 1.7 0.1

0.2 0.5 1.7 0.1 0.7 0.0 0.6 2.5 0.2

0.4 2.8 0.1 0.0 2.0 0.0 3.0 2.5 0.0
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

3.0 3.4 4.0 2.8 3.8 4.0 4.4 2.4 1.9

0.5 0.7 0.8 0.8 1.4 1.1 0.7 0.7 0.8

0.4 0.4 0.3 0.4 0.7 0.8 0.3 0.3 0.6

0.6 0.8 0.4 0.3 0.4

0.3 0.5 0.3 0.4 0.6 0.7 0.3 0.3 0.4

0.6 0.5 0.3 0.4 0.8 0.8 0.2 0.4 0.6

0.5 0.9 0.9 0.7 0.4 1.0 1.1 0.6 0.5

0.7 1.0 1.2 0.8 0.5 1.1 1.5 0.9 0.6

0.8 1.2 1.4 0.9 0.7 1.4 1.6 1.0 0.8

0.7 0.8 1.0 0.5 0.5 1.0 1.0 0.7 0.5

0.5 0.7 0.9 0.4 0.5 0.9 1.0 0.6 0.4

0.5 0.7 1.0 0.5 0.5 0.9 1.1 0.6 0.5

0.7 1.0 1.5 0.8 0.6 1.2 1.5 0.9 0.7

0.6 0.8 1.2 0.7 0.4 1.1 1.2 0.7 0.6

0.6 0.8 1.2 0.5 0.4 1.1 1.2 0.7 0.5

0.6 0.8 1.0 0.7 0.5 1.0 1.2 0.7 0.6

0.7 1.1 1.7 0.8 0.7 1.5 2.3 1.0 0.7

0.7 1.1 1.4 0.9 0.5 1.4 1.6 1.0 0.6

0.7 1.0 1.5 0.9 0.7 1.4 1.9 1.1 0.8

0.8 1.0 1.6 0.8 0.7 1.3 1.8 1.0 0.8

2.1 3.2 3.2 2.1 2.8 3.1 3.1 1.8 1.9

2.3 3.5 3.1 2.0 2.9 3.2 3.1 1.9 2.0

0.3 0.6 0.6 0.3 0.3 0.8 0.8 0.5 0.3

0.4 0.8 1.0 0.4 0.3 0.9 1.1 0.4 0.3

0.5 1.0 1.1 0.6 0.5 1.2 1.2 0.6 0.5

0.6 1.4 1.6 0.6 0.5 1.8 1.8 0.7 0.4

0.5 0.8 0.9 0.4 0.4 1.0 1.2 0.6 0.4

1.2 0.6 0.4

1.5 1.2 1.3 0.8 0.7 1.3 1.4 1.0 0.7

0.4 0.7 1.0 0.3 0.3 1.0 1.2 0.6 0.4

0.3 0.6 0.6 0.3 0.2 0.7 0.6 0.4 0.3

0.7 1.9 2.4 0.9 0.5 1.9 2.6 0.9 0.6

0.5 1.0 1.2 0.7 0.5 1.1 1.7 0.8 0.5

0.6 1.1 1.3 0.6 0.4 1.0 1.6 0.7 0.5

0.6 1.1 1.2 0.5 0.4 1.1 1.4 0.5 0.4

0.6 1.1 1.5 0.6 0.5 1.1 1.7 0.8 0.5

0.3 0.5 0.6 0.3 0.2 0.7 0.6 0.4 0.2

0.3 0.6 0.4 0.4 0.3 0.6 0.7 0.4 0.2

0.3 0.5 0.6 0.4 0.2 0.6 0.7 0.4 0.2

0.7 1.5 2.1 0.8 0.6 1.8 2.4 1.0 0.6

Speciation Measurements

Sulfates
0.5 0.7 0.6 0.4 0.4 0.8 0.8 0.5 0.4

0.3 0.9 0.6

0.5 0.5 0.5 0.4 0.4 0.6 0.6 0.4 0.4

0.6 0.7 0.7 0.4 0.5 0.8 0.8 0.5 0.4

0.5 0.7 0.7 0.4 0.5 0.7 0.8 0.5 0.4

0.6 0.7 0.8 0.4 0.4 0.8 0.9 0.6 0.5

0.4 0.5 0.5 0.4 0.3 0.6 0.6 0.4 0.3

2.9 3.9 4.1 2.9 2.4 3.6 4.4 2.1 2.3

2.9 3.0 2.4 2.5 3.0 3.2 2.8 1.7 2.0

2.6 2.5 1.8 2.2 2.7 2.8 1.5 1.4 1.8

3.0 3.5 3.3 2.8 3.0 3.6 3.0 1.7 2.0

3.0 3.4 3.2 3.1 2.9 3.3 3.2 1.9 2.4

2.8 3.7 4.8 2.4 2.6 3.9 4.1 1.7 1.9

0.5 0.4

0.4 0.6 0.6 0.4 0.4 0.8 0.7 0.4 0.4

1.5 2.1 2.8 1.2 1.8 2.0 3.0 1.7 1.5

2.2 2.5 2.5 1.8 2.8 2.6 2.3 1.5 1.6

1.5 1.8 1.8 1.0 1.4 1.7 1.8 1.0 1.0

3.9 4.2 4.5 3.1 3.7 3.5 4.8 2.1 2.3

3.6 4.4 4.6 3.3 0.9

3.1 4.4 3.6 3.1 3.3 4.3 4.6 2.3 2.5

2.6 3.4 3.0 2.4

1.0 0.9 1.5 0.9 1.6 0.9 1.3 1.2 1.3

0.9 1.4 2.0 0.8 1.6 1.2 1.9 1.3 1.4

1.0 1.7 2.3 0.8 1.6 1.5 2.1 1.4 1.3

0.8 1.3 2.0 0.7 1.5 1.4 1.6 1.3 1.2

1.0 1.2 2.0 0.9 1.9 1.3 1.5 1.4 1.5

0.8 1.1 1.8 0.7 1.5 1.2 1.4 1.1 1.2

3.1 3.8 5.3 2.8 2.9 3.3 5.9 2.1 2.3

1.3 2.1 2.7 1.2 1.7 2.2 2.3 1.4 1.4

1.6 2.3 3.0 1.3 1.9 2.4 3.5 1.5 1.4

1.4 2.1 2.6 1.2 1.7 1.9 2.5 1.5 1.5

1.6 1.3 1.0 1.0 1.5 1.2 1.2 1.2 1.3

1.5 1.5 1.7 1.2 1.6 1.5 1.8 1.4 1.5

1.5 1.1 0.7 0.9 1.3 1.1 0.9 1.0 1.2

2.6 1.5 1.6 1.5 2.0 1.9 1.8 1.2 1.8

1.8 1.0 0.7 0.9 1.3 1.1 1.1 1.0 1.4

2.0 1.6 1.8 1.6 2.3 1.9 2.3 1.6 1.8

2.8 2.8 2.7 2.1 3.7 2.6 2.8 1.9 1.8

2.8 3.4 3.6 2.9 3.3 3.6 2.9 2.0 1.8

8.0 1.3 0.8 3.0

1.8 1.3 0.6 1.4 2.3 1.2 0.7 0.6 1.7

0.9 0.9 0.4 0.9 1.2 0.8 0.6 0.4 1.0

0.4 0.5 0.4 0.5 0.4 0.7 0.6 0.5 0.3
0.4 0.5 0.4 0.3 0.3 0.7 0.5 0.3 0.3

2.9 3.2 3.4 2.4 3.3 3.1 4.2 2.3 2.3

4.0 5.1 5.6 3.0

2.4 2.0 2.3 1.8 2.5 2.4 2.3 1.7 2.1

2.7 2.2 2.1 1.8 3.1 2.3 3.1 1.9 2.2

2.5 2.2 2.3 1.8 2.6 2.7

2.4 2.9 3.1 2.3 3.2 2.8 3.1 1.9 1.8

1.1 0.7 0.6 0.7 1.2 0.7 0.6 0.5 0.5

0.5 0.5 0.5 0.4 0.6 0.7 0.6 0.5 0.4

0.4 0.6 0.4 0.4 0.4 0.6 0.5 0.4 0.3

0.3 0.5 0.4 0.4 0.2 0.5 0.5 0.4 0.3

0.3 0.5 0.4 0.4 0.5 0.5 0.5 0.4 0.3

0.3 0.5 0.4 0.4 0.4 0.5 0.6 0.3 0.3

3.1 1.0 0.8 1.1 2.1 1.1 0.9 0.7 1.1

1.0 0.7 0.6 0.7 1.0 0.7 0.7 0.5 0.5

0.4 0.5 0.5 0.5 0.3 0.6 0.6 0.4 0.3

2.5 0.9 0.9 1.3 1.4 1.2 1.0 0.7 1.1

1.5 1.0 1.2 0.8 1.2 1.1 1.1 0.7 0.7

1.8 1.3 1.3 1.1 1.7 1.4 1.6 0.8 0.8

0.4 0.6 0.7 0.4 0.3 0.6 0.7 0.4 0.3

1.1 1.2 1.8 0.9 1.5 1.2 2.4 1.1 1.1

1.2 1.8 2.3 0.8 1.3 1.4 2.2 1.4 1.2

1.7 1.8 2.4 1.5 1.6

2.7 3.4 4.1 1.9 2.4 3.5 4.1 1.9 2.1

0.6 0.9 1.2 0.6 0.4 0.9 1.1 0.6 0.5

1.2 1.8 1.7 1.2 1.3 2.0 2.1 1.4 0.9

0.5 1.8 1.1 0.8 1.5 2.3 1.4 0.8 0.7

0.5 0.8 0.8 0.5 0.5 1.0 1.0 0.6 0.5

0.5 0.7 0.8 0.4 0.4 0.8 0.9 0.4 0.4

0.5 1.0 1.0 0.7 0.5 1.2 1.2 0.7 0.7

0.4 0.7 0.6 0.3 0.4 0.8 0.8 0.4 0.4

2.0 3.2

2.9 3.3 4.2 2.0 1.9 3.2 4.1 1.3 1.7

1.6 3.3 3.8 1.4 1.4 3.3 3.7 1.2 1.3

2.0 1.1 0.9 1.1 1.3 1.2 1.0 0.7 0.8

2.8 1.2 1.1 1.8 1.4 1.0 1.4 0.9 1.4

3.5 4.1 5.4 3.1 3.7 3.8 6.5 2.4 2.9

3.4 3.2 2.4 3.3 3.3 3.0 2.1 2.1

1.9 2.9 2.6 1.7 2.6 2.8 2.5 1.5 1.7

1.6 2.2 1.9 1.2 1.7 2.0 2.1 1.2 1.1

2.2 3.1

0.3 0.5 0.6 0.3 0.3 0.5 0.7 0.4 0.3

0.2 0.8 0.7 0.3 0.2 0.8 0.9 0.4 0.2

0.1 0.4 0.4 0.4 0.2 0.5 0.6 0.4 0.2
0.5 0.6 0.6 0.5 0.4 0.6 0.7 0.4 0.3

0.5 0.5 0.5 0.5 0.5 0.7 0.7 0.5 0.4

2.8 3.8 5.2 2.5

2.7 3.3 4.7 2.1

3.1 3.9 3.3 2.9 2.9 3.7 3.9 2.0 2.5

1.1 0.8 0.7 0.7 1.0 0.9 0.9 0.6 0.6

1.9 0.9 1.0 1.0 1.3 1.1 1.1 0.7 0.7

2.8 3.7 4.7 2.4 2.6 3.6 4.7 1.9 2.1

0.7 1.2 1.5 0.9 0.8 1.3 2.0 0.8 0.7

0.6 0.6 0.7 0.5 0.4 0.8 0.8 0.5 0.4

0.9 0.7 0.7 0.5 0.5 0.8 0.8 0.6 0.5

0.6 0.6 0.9 0.4 0.4 0.9 1.0 0.6 0.4

0.6 0.6 0.7 0.4 0.4 0.8 0.8 0.6 0.4

1.2 1.7 3.1 0.8 1.1 1.5 2.5 1.3 1.2

1.3 1.7 2.4 0.9 1.6 1.3 2.3 1.5 1.3

2.3 3.6 4.8 2.2 2.0 3.0 4.9 1.6 1.8

3.0 3.8 4.4 2.8 2.7 3.2 4.9 2.0 2.2

0.4 0.4 0.9 1.0 0.5 0.4

0.7 1.2 1.4 1.2

0.4 0.8 1.1 0.5 0.4 0.9 1.2 0.5 0.3

0.4 0.6 0.9 0.4 0.3 0.6 0.9 0.4 0.3

0.8 0.8 1.3 0.7 0.5 0.9 1.3 1.0

0.8 0.7 0.9 1.0 0.4 0.7 1.0 0.8 0.6

0.3 0.4 0.5 0.3 0.3 0.4 0.5 0.3 0.3

0.3 0.5 0.4 0.3 0.3 0.6 0.5 0.3 0.3

0.3 0.7 0.9 0.3 0.3 0.7 1.1 0.4 0.2

0.3 0.6 0.8 0.4 0.3 0.7 1.0 0.3 0.2

2.6 3.7 5.3 2.5 2.4 3.2 6.2 1.7 2.0

1.1 0.9 0.7 0.7 1.1 0.7 0.7 0.6 0.6

0.4 0.6 0.5 0.4 0.5 0.7 0.6 0.5 0.3

0.5 0.5 0.4 0.3 0.4 0.6 0.5 0.5 0.4

0.5 0.6 0.5 0.4 0.4 0.7 0.6 0.4 0.3

0.4 0.5 0.4 0.4 0.4 0.7 0.5 0.4 0.3

0.5 0.5 0.4 0.4 0.4 0.6 0.5 0.4 0.3

2.0 2.2 1.5 1.0 0.9 2.0 1.5 1.2 1.0
2012 2012 2012 2010 2010 2010 2010 2011 2011

2 3 4 1 2 3 4 1 2

3.1 2.8 2.2 1.4 0.3 0.2 1.1 1.1 0.3

0.9 0.5 0.7 0.1 0.1 0.1 0.1 0.2 0.1

0.4 0.3 0.3 0.2 0.0 0.0 0.0 0.1 0.0

0.6 0.3 0.3 0.1 0.1

0.4 0.2 0.3 0.1 0.1 0.1 0.0 0.1 0.1

0.8 0.2 0.3 0.2 0.1 0.1 0.1 0.1 0.0

1.0 1.2 0.5 0.1 0.2 0.1 0.1 0.2 0.2

1.2 1.7 0.8 0.2 0.2 0.1 0.1 0.2 0.2

1.3 1.8 1.1 0.5 0.3 0.2 0.3 0.4 0.3

1.2 1.1 0.5 0.2 0.2 0.2 0.1 0.2 0.2

0.9 1.0 0.4 0.2 0.2 0.1 0.2 0.2 0.2

1.1 1.0 0.5 0.3 0.3 0.2 0.2 0.3 0.3

1.3 1.7 0.8 0.2 0.3 0.2 0.2 0.3 0.3

1.0 1.4 0.7 0.2 0.3 0.2 0.1 0.2 0.3

1.2 1.4 0.6 0.2 0.3 0.3 0.1 0.2 0.3

1.1 1.2 0.6 0.3 0.2 0.2 0.1 0.4 0.3

1.5 2.2 1.0 0.3 0.4 0.3 0.2 0.4 0.3

1.3 1.7 0.9 0.5 0.3 0.2 0.4 0.4 0.4

1.4 2.0 1.0 0.5 0.3 0.3 0.4 0.6 0.3

1.3 2.0 1.1 0.5 0.3 0.2 0.3 0.6 0.3

3.1 2.5 2.0 1.9 0.5 0.3 1.4 2.2 0.5

3.7 2.6 2.1 1.5 0.4 0.4 1.0 1.5 0.5

0.9 0.9 0.3 0.2 0.2 0.1 0.1 0.1 0.2

1.1 1.2 0.4 0.2 0.5 0.4 0.1 0.1 0.4

1.1 1.6 0.5 0.1 0.3 0.3 0.2 0.2 0.2

1.5 1.5 0.6 0.4 0.8 0.5 0.5 0.5 1.0

1.1 1.5 0.6 0.7 0.7 0.3 0.3 0.5 0.6

1.3 1.5 0.4

1.2 1.1 0.6 1.7 0.3 0.3 0.9 1.2 0.3

1.1 1.3 0.4 0.2 0.3 0.2 0.2 0.2 0.3

0.8 0.8 0.3 0.1 0.2 0.1 0.1 0.1 0.1

2.1 2.2 0.8 1.0 1.5 0.9 0.7 0.6 1.3

1.1 1.3 0.5 0.5 0.7 0.5 0.6 0.4 0.8

1.2 2.1 0.5 1.0 1.1 0.5 0.7 0.6 0.6

1.3 1.7 0.4 1.2 2.3 1.1 0.9 0.8 1.7

1.4 1.5 0.6 0.6 1.0 0.5 0.4 0.4 0.8

0.7 0.7 0.3 0.1 0.2 0.1 0.1 0.1 0.2

0.7 0.6 0.3 0.1 0.1 0.1 0.1 0.2 0.1

0.8 0.7 0.4 0.2 0.1 0.1 0.2 0.1 0.1

1.9 1.9 0.8 0.9 0.7 0.5 2.0 1.5 0.8

Speciation Measurements

Nitrates
0.8 0.8 0.4 0.3 0.2 0.1 0.1 0.2 0.2

0.1 0.2

0.7 0.7 0.4 0.2 0.2 0.1 0.1 0.1 0.2

0.9 0.7 0.5 0.3 0.2 0.1 0.2 0.4 0.2

0.8 0.7 0.4 0.4 0.4 0.2 0.2 0.3 0.2

0.9 0.8 0.5 0.3 0.2 0.1 0.1 0.2 0.2

0.7 0.6 0.3 0.1 0.2 0.1 0.1 0.1 0.2

2.3 3.4 2.4 2.1 0.8 0.5 1.7 2.1 0.6

2.5 2.0 2.2 0.4 0.5 0.3 0.3 0.5 0.4

2.7 1.8 1.8 0.5 0.4 0.3 0.4 0.5 0.4

2.6 2.3 2.2 0.5 0.4 0.3 0.4 0.5 0.3

2.5 2.2 2.5 0.4 0.4 0.3 0.4 0.4 0.4

3.1 2.8 1.8 0.9 0.3 0.2 0.9 0.8 0.3

0.8 0.6 0.4

0.8 0.7 0.4 0.1 0.2 0.1 0.1 0.1 0.2

1.5 1.9 1.7 0.6 0.5 0.3 0.6 0.8 0.5

2.7 2.0 1.8 3.5 0.6 0.2 2.0 4.1 0.9

2.0 1.6 1.2 2.7 0.5 0.2 0.9 1.7 0.6

3.1 3.9 2.3 3.0 0.6 0.2 1.6 2.5 0.5

3.1 0.5 0.3 1.9 0.6

3.6 2.7 2.5 1.4 0.4 0.3 0.7 1.0 0.4

0.6 0.3 0.2 0.3

0.9 0.9 1.0 0.3 0.1 0.1 0.2 0.5 0.1

1.1 1.4 1.1 0.2 0.2 0.1 0.2 0.4 0.1

1.5 1.2 1.3 0.3 0.3 0.2 0.2 0.5 0.3

1.1 1.2 1.1 0.2 0.2 0.2 0.2 0.4 0.2

1.2 1.2 1.3 0.3 0.2 0.1 0.2 0.6 0.2

1.0 1.1 1.1 0.2 0.2 0.1 0.1 0.3 0.1

2.8 4.0 2.3 1.4 0.4 0.2 0.8 1.2 0.4

1.8 1.7 1.5 0.4 0.5 0.3 0.4 0.6 0.4

1.7 1.9 1.7 0.7 0.8 0.5 0.6 0.8 0.5

1.2 1.9 1.5 0.5 0.4 0.2 0.6 0.8 0.3

1.1 0.8 1.1 1.3 0.2 0.1 0.7 0.9 0.1

1.5 1.3 1.2 1.5 0.2 0.1 0.9 1.3 0.1

0.9 0.7 1.0 0.9 0.2 0.1 0.6 0.8 0.1

1.5 1.4 1.3 5.7 0.8 0.5 2.3 3.9 1.1

1.0 0.6 1.0 1.1 0.2 0.1 0.6 1.1 0.1

1.5 1.4 1.8 4.6 0.6 0.3 2.3 4.9 1.0

2.7 2.3 2.4 4.1 0.5 0.2 2.1 3.7 0.6

2.6 2.7 1.9 2.7 0.4 0.2 1.5 3.1 0.5

0.1 0.1 0.1 0.1

1.2 0.1 0.2 0.2 0.2 0.2 0.3

0.7 0.9 0.9 0.1 0.1 0.1 0.1 0.1 0.1

0.6 0.7 0.4 0.7 0.2 0.1 0.5 0.7 0.2
0.6 0.6 0.3 0.1 0.1 0.1 0.1 0.1 0.1

2.7 2.6 2.1 6.3 1.2 0.5 3.1 4.5 1.3

4.8 1.0 0.6 1.7

2.0 1.9 1.9 5.7 0.7 0.4 2.7 4.5 1.2

2.2 2.2 1.9 6.4 0.7 0.2 2.6 4.9 1.0

5.6 0.7 0.3 2.6 4.1 1.0

2.6 2.5 2.0 2.3 0.4 0.2 1.6 3.1 0.4

0.7 0.7 0.6 1.1 0.1 0.0 0.4 0.6 0.1

0.6 0.5 0.4 0.4 0.1 0.1 0.2 0.2 0.1

0.5 0.5 0.3 0.2 0.1 0.1 0.1 0.2 0.1

0.5 0.5 0.3 0.2 0.2 0.1 0.1 0.1 0.2

0.5 0.5 0.3 0.1 0.1 0.0 0.2 0.1 0.0

0.5 0.6 0.3 0.1 0.1 0.1 0.1 0.1 0.1

1.0 0.8 1.3 2.5 0.2 0.1 0.9 1.8 0.3

0.7 0.8 0.6 0.8 0.1 0.1 0.3 0.4 0.1

0.6 0.4 0.3 0.1 0.1 0.1 0.2 0.1 0.1

1.0 1.0 1.1 1.9 0.2 0.1 1.1 1.3 0.4

1.0 1.0 0.6 2.1 0.4 0.2 0.7 1.3 0.6

1.4 1.4 0.9 2.5 0.5 0.2 1.0 1.6 0.7

0.7 0.8 0.3 0.2 0.2 0.1 0.1 0.1 0.1

0.9 1.2 1.1 0.1 0.1 0.2 0.1 0.3 0.1

1.0 1.6 1.2 0.3 0.2 0.1 0.2 0.5 0.2

1.3 1.6 1.5 0.7 0.3

2.2 3.1 2.0 1.9 0.7 0.4 1.2 1.8 0.8

1.1 1.2 0.6 0.1 0.2 0.1 0.1 0.1 0.2

2.1 2.2 1.2 1.0 0.3 0.3 0.8 0.5 0.4

1.5 1.4 0.7 0.1 0.2 0.1 0.1 0.2 0.3

1.1 1.1 0.6 0.2 0.2 0.1 0.1 0.2 0.3

0.9 0.9 0.5 0.2 0.2 0.1 0.1 0.2 0.2

1.2 1.3 0.7 0.3 0.2 0.1 0.2 0.4 0.2

0.8 0.9 0.4 0.1 0.2 0.1 0.1 0.1 0.2

1.1 0.4

2.7 2.5 1.6 0.4 0.2 0.1 0.3 0.4 0.2

2.5 2.6 1.2 0.3 0.4 0.2 0.2 0.3 0.3

1.1 0.8 0.8 1.9 0.4 0.1 1.0 0.9 0.6

1.3 0.8 0.9 2.2 0.4 0.2 1.4 1.7 0.5

3.1 4.1 2.2 3.0 0.4 0.2 1.4 1.9 0.5

3.2 2.5 2.2 0.3 0.3 1.9 3.0 0.4

2.6 2.1 1.7 2.1 0.5 0.3 1.1 2.1 0.6

2.4 1.8 1.3 2.5 0.4 0.2 0.9 1.9 0.5

2.5 1.2

0.8 0.6 0.3 0.1 0.2 0.2 0.1 0.1 0.2

0.7 0.7 0.3 0.1 0.2 0.2 0.1 0.1 0.2

0.7 0.5 0.3 0.0 0.1 0.1 0.1 0.1 0.1
0.7 0.6 0.3 0.5 0.1 0.1 0.3 0.4 0.1

0.7 0.5 0.3 0.7 0.1 0.1 0.3 1.0 0.1

1.9 1.0 0.4 1.8

2.1 0.5 0.2 1.5

2.5 2.5 2.1 0.6 0.4 0.3 0.5 0.7 0.4

0.8 0.9 0.5 1.2 0.2 0.1 0.4 0.7 0.2

1.2 0.9 0.8 1.1 0.3 0.2 0.4 0.7 0.3

3.1 2.8 1.7 0.7 0.3 0.1 0.6 0.6 0.3

1.7 2.0 1.3 0.3 0.2 0.1 0.3 0.3 0.3

0.9 0.8 0.4 0.5 0.2 0.1 0.2 0.2 0.2

0.9 0.8 0.5 0.8 0.2 0.1 0.1 0.4 0.1

1.0 1.0 0.5 0.3 0.2 0.2 0.1 0.2 0.2

0.8 0.8 0.5 0.7 0.2 0.1 0.1 0.2 0.1

1.1 1.9 0.4 0.3 0.1 0.3 0.5 0.3

1.3 1.6 1.3 0.8 0.2 0.1 0.3 1.1 0.1

2.4 3.9 1.6 1.3 0.5 0.2 0.8 1.0 0.4

2.5 3.2 2.1 1.2 0.4 0.3 0.8 1.3 0.3

0.7 0.9 0.4 0.1 0.2 0.2

0.4 0.3 0.3 0.4

0.8 0.9 0.3 0.2 0.3 0.3 0.2 0.1 0.2

0.6 0.9 0.2 0.3 0.2 0.3 0.2 0.2 0.2

0.7 0.4 0.6 0.8 0.6 0.4

0.5 0.9 0.9 1.5 0.3 0.2 1.5 0.9 0.2

0.5 0.5 0.2 0.3 0.1 0.1 0.1 0.1 0.1

0.5 0.5 0.2 0.2 0.1 0.1 0.2 0.1 0.1

0.6 1.0 0.2 0.1 0.2 0.2 0.1 0.1 0.1

0.6 0.9 0.3 0.1 0.1 0.2 0.1 0.1 0.1

2.8 4.0 1.8 0.9 0.3 0.2 0.6 0.8 0.3

0.8 0.8 0.6 1.1 0.2 0.1 0.2 0.7 0.2

0.6 0.7 0.3 0.1 0.2 0.1 0.0 0.2 0.2

0.6 0.7 0.3 0.2 0.2 0.1 0.1 0.2 0.2

0.6 0.7 0.4 0.2 0.2 0.1 0.1 0.2 0.2

0.6 0.6 0.3 0.1 0.2 0.1 0.1 0.2 0.1

0.6 0.6 0.4 0.2 0.2 0.1 0.1 0.3 0.2

1.9 2.0 1.1 0.3 0.4 0.4 0.2 0.3 0.4
2011 2011 2012 2012 2012 2012 2010 2010 2010

3 4 1 2 3 4 1 2 3

0.2 0.8 0.5 0.3 0.2 0.7 0.5 1.1 1.7

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.0 0.1 0.2 0.0 0.0 0.1 0.2 0.3 0.1

0.1 0.0 0.1 0.1 0.1 0.0

0.0 0.1 0.1 0.1 0.0 0.0 0.2 0.3 0.1

0.0 0.1 0.1 0.0 0.0 0.0 0.2 0.2 0.0

0.1 0.1 0.2 0.3 0.1 0.1 0.4 1.0 0.4

0.2 0.2 0.2 0.4 0.3 0.1 0.7 1.6 0.6

0.2 0.5 0.3 0.3 0.3 0.3 3.6 5.4 2.4

0.1 0.1 0.1 0.3 0.1 0.1 0.7 2.0 1.6

0.2 0.1 0.2 0.3 0.1 0.1 0.4 1.3 0.6

0.2 0.2 0.3 0.4 0.2 0.2 0.6 3.5 4.4

0.2 0.3 0.3 0.4 0.2 0.2 0.4 2.2 0.9

0.2 0.2 0.3 0.3 0.2 0.1 0.4 1.4 0.6

0.2 0.2 0.2 0.4 0.2 0.1 0.6 1.4 1.6

0.1 0.2 0.2 0.3 0.2 0.1 0.5 2.2 0.9

0.3 0.4 0.3 0.4 0.3 0.2 1.0 1.6 1.2

0.3 0.4 0.3 0.4 0.3 0.2 0.9 2.2 1.0

0.3 0.5 0.5 0.5 0.4 0.4 1.9 2.7 1.5

0.3 0.4 0.3 0.4 0.3 0.3 0.7 1.8 1.1

0.2 1.0 0.9 0.4 0.3 0.8 0.5 1.4 2.2

0.2 1.1 0.8 0.4 0.4 0.9 0.4 1.1 3.0

0.1 0.1 0.2 0.2 0.2 0.1 0.7 0.7 0.5

0.4 0.1 0.2 0.4 0.4 0.4 1.2 0.9 1.0

0.2 0.1 0.2 0.3 0.3 0.1 0.7 1.6 1.4

0.3 0.7 0.8 0.7 0.3 0.7 0.7 0.9 1.8

0.3 0.4 0.5 0.5 0.6 0.6 1.3 1.1 0.9

0.2 0.8 0.8 1.0 0.5 0.5

0.3 1.0 1.2 0.3 0.3 0.4 0.3 0.3 0.1

0.2 0.4 0.4 0.4 0.3 0.3 0.7 0.6 0.9

0.1 0.1 0.2 0.2 0.1 0.1 0.7 0.7 0.9

0.9 0.7 0.8 1.9 0.8 0.7 0.4 0.8 0.8

0.6 0.8 0.6 0.7 0.7 0.4 0.3 0.6 0.6

0.5 0.4 0.8 0.7 0.5 0.4 0.7 1.1 1.0

1.1 0.7 1.1 1.6 0.8 0.7 0.8 0.9 0.7

0.5 0.5 0.4 0.9 0.5 0.4 0.5 1.2 1.1

0.1 0.1 0.1 0.2 0.2 0.2 0.5 0.6 1.0

0.1 0.1 0.1 0.1 0.3 0.1 0.4 0.5 0.6

0.1 0.2 0.1 0.2 0.2 0.3 0.3 0.5 0.6

0.5 2.9 2.4 0.9 0.5 1.3 0.5 0.8 1.7

Speciation Measurements

Nitrates
0.1 0.2 0.3 0.2 0.1 0.1 0.6 2.8 1.1

0.1

0.1 0.1 0.2 0.2 0.2 0.1 0.3 1.3 0.5

0.1 0.2 0.3 0.3 0.1 0.1 0.5 5.1 1.6

0.1 0.1 0.3 0.3 0.2 0.2 0.5 1.3 0.6

0.1 0.1 0.2 0.2 0.1 0.1 0.4 4.1 1.0

0.1 0.1 0.2 0.2 0.1 0.1 0.4 2.0 0.6

0.4 1.4 1.7 0.6 0.3 2.0 0.7 1.3 0.8

0.3 0.5 0.5 0.4 0.4 0.4 0.4 1.7 2.0

0.2 0.4 0.4 0.4 0.4 0.4 0.4 1.8 1.9

0.2 0.3 0.4 0.3 0.3 0.3 0.4 1.1 1.8

0.2 0.3 0.5 0.3 0.3 0.4 0.4 1.1 1.7

0.1 0.4 0.6 0.3 0.2 0.6 0.4 1.4 1.2

0.1 0.2 0.2 0.1 0.1

0.1 0.1 0.1 0.2 0.1 0.1 0.6 3.1 0.5

0.4 0.7 1.1 0.4 0.2 0.9 0.3 0.9 0.4

0.2 1.7 1.5 0.6 0.3 2.1 0.4 1.1 1.3

0.4 1.1 1.2 0.7 0.4 1.4 0.4 1.2 1.3

0.2 1.0 1.1 0.5 0.3 1.3 0.5 1.1 1.0

0.5 1.1 1.4

0.3 0.5 0.6 0.4 0.4 0.6 0.5 1.9 2.4

0.4 1.4 2.5

0.1 0.3 0.5 0.1 0.1 0.3 0.8 0.7 0.4

0.1 0.2 0.4 0.2 0.1 0.4 0.2 0.5 0.3

0.3 0.3 0.5 0.4 0.2 0.6 0.2 0.6 0.4

0.2 0.3 0.4 0.2 0.1 0.3 0.2 0.5 0.3

0.2 0.4 0.5 0.2 0.1 0.4 0.5 0.6 0.4

0.1 0.3 0.3 0.2 0.1 0.2 0.2 0.4 0.2

0.2 0.7 0.8 0.4 0.2 1.1 0.5 0.9 0.8

0.3 0.4 0.8 0.4 0.3 0.5 0.2 0.6 0.4

0.5 0.5 0.8 0.5 0.4 0.7 0.3 0.6 0.5

0.2 0.5 1.0 0.3 0.2 0.7 0.3 0.7 0.4

0.1 0.8 0.9 0.1 0.1 0.7 0.3 0.5 0.3

0.1 0.9 0.9 0.3 0.1 0.8 0.2 0.6 0.3

0.1 0.9 1.1 0.1 0.1 0.9 0.3 0.5 0.2

0.6 1.4 2.8 1.3 0.6 3.0 0.5 1.0 0.8

0.1 0.7 1.2 0.1 0.1 1.0 0.3 0.6 0.3

0.3 2.2 2.8 0.6 0.3 3.1 0.4 0.8 0.5

0.2 2.0 1.4 0.5 0.3 2.4 0.5 1.2 1.6

0.2 1.0 1.2 0.4 0.2 1.2 1.1 2.1 1.6

0.8 0.4 0.1

0.1 0.2 0.2 0.3 0.3 0.5 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.3 0.7 0.1

0.1 0.9 0.4 0.1 0.3 0.4 0.4 0.8 1.1
0.1 0.0 0.1 0.1 0.3 0.1 0.4 0.8 0.8

0.5 2.5 2.5 0.8 0.5 3.2 0.4 0.9 0.8

0.5 1.0 1.0

0.4 2.3 3.4 0.8 0.4 3.3 0.5 0.8 0.9

0.4 2.2 2.5 0.7 0.4 3.1 0.4 0.8 0.7

0.4 1.1 1.2

0.2 1.1 0.8 0.4 0.3 1.2 0.5 1.3 1.4

0.0 0.2 0.3 0.1 0.1 0.3 0.3 0.8 0.7

0.1 0.2 0.2 0.1 0.1 0.2 0.4 0.6 1.1

0.1 0.2 0.1 0.1 0.1 0.1 0.3 0.5 0.9

0.1 0.1 0.1 0.1 0.2 0.1 0.3 0.7 0.9

0.0 0.1 0.1 0.1 0.1 0.1 0.6 1.0 1.5

0.1 0.1 0.1 0.1 0.5 0.2 0.3 0.5 1.0

0.1 0.5 1.2 0.3 0.1 1.1 0.5 1.1 0.9

0.1 0.1 0.3 0.1 0.3 0.4 0.4 0.6 0.8

0.1 0.2 0.1 0.1 0.1 0.1 0.4 0.6 0.7

0.2 0.6 1.3 0.4 0.2 1.1 0.4 0.8 0.8

0.2 0.5 0.8 0.4 0.2 0.4 0.4 0.8 1.1

0.3 1.0 1.0 0.5 0.3 1.0 0.3 0.8 0.7

0.1 0.1 0.2 0.2 0.1 0.1 0.8 1.0 0.9

0.1 0.2 0.3 0.1 0.0 0.2 0.0 0.5 0.2

0.2 0.4 0.6 0.2 0.1 0.5 0.2 0.6 0.3

0.3 0.5 0.8 0.3 0.2 0.7

0.4 0.9 1.3 0.5 0.3 1.2 0.4 0.8 0.8

0.1 0.1 0.1 0.2 0.1 0.1 0.6 1.4 0.5

0.4 1.1 0.8 0.5 0.5 0.7 0.6 2.5 1.2

0.2 0.2 0.2 0.3 0.2 0.1 0.4 2.5 0.8

0.1 0.3 0.3 0.3 0.1 0.2 0.3 1.4 0.5

0.1 0.1 0.2 0.3 0.2 0.1 0.6 1.8 0.6

0.1 0.5 0.3 0.3 0.2 0.3 0.5 1.5 0.7

0.1 0.1 0.2 0.2 0.2 0.1 0.4 1.5 0.4

0.3 0.8

0.1 0.2 0.3 0.2 0.1 0.3 0.4 1.0 0.9

0.2 0.3 0.3 0.5 0.2 0.3 0.3 1.5 0.6

0.2 0.3 0.7 0.3 0.1 0.7 0.4 0.8 1.0

0.3 0.9 1.5 0.6 0.2 0.9 0.4 1.0 1.0

0.2 1.0 1.2 0.4 0.3 1.4 0.5 1.0 0.7

0.3 1.7 1.3 0.4 0.4 1.4 1.2 1.9

0.3 1.4 1.6 0.5 0.4 1.1 0.7 1.1 1.8

0.3 1.3 1.3 0.6 0.3 1.0 0.4 1.3 1.2

0.6 1.9

0.2 0.1 0.1 0.2 0.3 0.1 0.3 0.4 0.3

0.2 0.1 0.1 0.2 0.2 0.1 0.2 0.3 0.3

0.1 0.1 0.1 0.1 0.1 0.1 0.6 0.6 0.7
0.1 0.2 0.2 0.1 0.1 0.1 0.4 0.5 0.8

0.1 0.4 0.2 0.1 0.1 0.2 0.3 0.6 0.7

0.4 0.8 0.7

0.4 0.8 0.6

0.3 0.4 0.6 0.4 0.3 0.5 0.4 0.8 1.5

0.1 0.2 0.4 0.2 0.1 0.3 0.3 0.7 0.9

0.2 0.2 0.4 0.2 0.1 0.6 0.4 0.7 0.8

0.1 0.3 0.5 0.3 0.2 0.5 0.4 1.1 1.0

0.2 0.4 0.3 0.3 0.3 0.2 1.0 2.1 0.8

0.1 0.4 0.3 0.3 0.1 0.1 0.5 0.9 0.7

0.1 0.2 0.2 0.2 0.1 0.2 0.4 1.7 0.7

0.1 0.2 0.2 0.2 0.1 0.1 0.5 1.2 1.1

0.1 0.3 0.2 0.2 0.1 0.2 0.4 1.1 0.8

0.2 0.5 0.9 0.3 0.2 0.2 0.7 0.4

0.1 0.5 0.7 0.2 0.1 0.5 0.2 0.5 0.3

0.3 0.6 0.7 0.5 0.3 0.7 0.4 0.9 0.8

0.2 0.4 0.5 0.3 0.2 1.0 0.4 1.0 0.9

0.1 0.2 0.2 0.2 0.2 0.2

0.3 0.3 0.6

0.2 0.2 0.2 0.3 0.3 0.2 0.3 0.2 0.2

0.2 0.3 0.1 0.2 0.4 0.2 0.3 0.3 0.3

0.4 0.7 0.4 0.3 0.4

0.3 0.8 0.6 0.2 0.3 0.9 0.6 1.5 1.6

0.1 0.1 0.1 0.1 0.2 0.1 0.5 0.4 0.2

0.1 0.2 0.1 0.1 0.1 0.1 0.3 0.4 0.2

0.2 0.1 0.1 0.1 0.2 0.0 0.3 0.3 0.3

0.1 0.1 0.1 0.1 0.1 0.1 0.3 0.3 0.2

0.2 0.5 0.6 0.4 0.2 0.6 0.4 1.0 1.0

0.1 0.2 0.6 0.1 0.2 0.4 0.8 0.8 1.7

0.1 0.1 0.1 0.2 0.2 0.1 0.5 0.7 0.5

0.1 0.2 0.2 0.2 0.2 0.1 0.4 0.8 1.2

0.1 0.1 0.1 0.2 0.2 0.1 0.7 0.9 0.7

0.1 0.1 0.1 0.2 0.1 0.1 0.6 1.0 0.7

0.1 0.4 0.2 0.1 0.2 0.2 0.3 0.7 1.0

0.3 0.2 0.2 0.5 0.4 0.2 1.5 5.6 5.4
2010 2011 2011 2011 2011 2012 2012 2012 2012

4 1 2 3 4 1 2 3 4

0.5 0.3 0.6 0.5 0.2 0.4 0.5 1.0 0.4

0.2 0.2 0.1 0.1 0.1 0.1 0.1 0.0 0.1

0.2 0.2 0.2 0.0 0.0 0.1 0.2 0.2 0.1

0.1 0.1 0.0 0.1 0.0 0.1 0.0 0.1

0.2 0.2 0.2 0.0 0.1 0.1 0.2 0.0 0.3

0.1 0.1 0.2 0.0 0.0 0.1 0.2 0.0 0.1

0.3 0.6 1.4 0.6 0.3 0.7 1.6 0.7 0.4

0.5 1.0 2.1 1.0 0.6 1.1 1.9 0.8 0.7

7.6 5.1 5.0 2.3 2.7 5.3 5.3 2.8 4.7

0.4 0.6 1.6 1.0 0.5 0.8 2.6 1.0 0.7

0.2 0.6 0.9 0.7 0.3 0.8 1.7 0.7 0.4

1.4 1.0 4.2 3.0 1.1 1.9 6.0 5.0 3.0

0.7 1.0 2.0 2.0 0.5 1.3 3.0 1.1 0.7

0.5 0.5 1.8 1.0 0.3 0.8 2.6 0.8 0.7

0.5 0.6 1.7 1.5 0.6 0.8 2.4 1.0 0.7

0.5 0.5 1.8 0.9 0.4 0.9 2.1 0.9 0.8

1.0 1.4 2.6 2.5 0.7 1.5 2.2 1.1 1.0

1.2 1.0 2.5 1.6 1.0 1.4 2.6 1.4 1.2

1.8 2.0 2.7 2.8 1.6 3.8 4.6 2.4 2.6

0.9 1.2 2.4 3.4 0.7 1.8 3.1 1.3 1.2

0.6 0.2 1.3 0.9 0.3 0.5 0.9 1.9 0.6

0.5 0.3 0.7 0.8 0.3 0.6 0.8 2.5 0.4

0.2 0.3 0.4 0.3 0.2 0.2 0.9 0.5 0.3

0.2 0.3 0.5 0.5 0.3 0.3 1.2 1.0 0.4

0.4 1.0 1.2 1.0 0.6 1.4 2.2 2.0 0.9

0.4 0.3 1.0 1.1 0.5 0.4 1.6 1.5 0.7

0.5 1.3 0.8 0.9 1.0 1.0 1.5 1.0 0.6

0.4 0.3 0.5 1.3 0.5 0.3

0.1 0.1 0.2 0.1 0.2 0.2 0.3 0.1 0.2

0.2 0.2 0.5 0.6 0.3 0.3 1.1 1.0 0.3

0.2 0.3 0.5 0.4 0.2 0.3 1.1 0.8 0.3

0.4 0.2 0.9 0.6 0.5 0.5 0.8 0.7 0.4

0.3 0.2 0.3 0.5 0.3 0.2 0.6 0.5 0.3

0.4 0.5 0.8 0.9 0.6 0.8 1.7 1.2 0.5

0.2 0.4 0.7 0.5 0.3 0.5 1.3 0.6 0.3

0.3 0.4 0.8 0.8 0.5 0.3 1.2 0.6 0.3

0.2 0.2 0.3 0.5 0.2 0.2 0.7 0.7 0.3

0.2 0.1 0.3 0.5 0.1 0.2 0.7 0.7 0.5

0.2 0.1 0.2 0.4 0.1 0.1 0.6 0.5 0.3

0.3 0.2 0.7 1.2 0.5 0.4 1.3 1.7 0.6

Speciation Measurements

Crustal
0.7 0.6 2.7 0.7 0.5 0.9 2.3 0.7 0.8

0.2 1.3 0.6

0.2 0.3 0.8 0.3 0.2 0.5 1.0 0.5 0.3

0.7 0.5 2.5 1.0 0.6 0.6 3.1 1.3 1.8

0.2 0.4 0.9 0.5 0.3 0.5 1.6 0.5 0.3

0.3 0.6 1.8 0.8 0.4 0.9 2.6 0.7 0.6

0.3 0.4 1.2 0.5 0.3 0.6 1.7 0.4 0.3

0.6 0.4 0.8 0.5 0.6 0.5 0.6 0.5 0.5

0.5 0.4 0.6 0.9 0.2 0.3 0.6 1.7 0.3

0.3 0.3 0.6 1.4 0.2 0.2 1.4 3.9 0.2

0.5 0.3 0.6 0.7 0.2 0.2 0.5 1.8 0.3

0.6 0.3 0.7 0.8 0.2 0.3 0.5 1.3 0.3

0.4 0.2 0.6 0.3 0.2 0.3 0.5 1.2 0.2

0.3 0.7 1.4 0.6 0.3

0.2 0.5 1.3 0.4 0.4 0.7 2.0 0.4 0.3

0.2 0.1 0.2 0.2 0.2 0.2 0.3 0.2 0.2

0.7 0.4 0.9 1.1 0.4 0.7 1.1 1.8 1.0

1.0 0.4 1.1 1.2 0.5 0.9 1.7 2.4 1.9

0.5 0.2 0.5 0.3 0.2 0.4 0.5 0.9 0.4

0.6 0.3

0.5 0.3 0.7 1.1 0.2 0.3 0.9 3.3 0.5

0.5

0.2 0.3 0.3 0.2 0.2 0.4 0.3 0.3 0.2

0.1 0.1 0.2 0.1 0.1 0.2 0.2 0.1 0.1

0.1 0.1 0.1 0.2 0.1 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1

0.2 0.2 0.2 0.2 0.2 0.4 0.2 0.2 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1

0.4 0.2 0.4 0.3 0.2 0.3 0.4 0.5 0.2

0.2 0.1 0.2 0.1 0.2 0.1 0.3 0.2 0.2

0.2 0.2 0.2 0.2 0.2 0.2 0.3 0.2 0.2

0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.1

0.3 0.1 0.2 0.2 0.2 0.1 0.3 0.3 0.1

0.2 0.1 0.2 0.2 0.2 0.1 0.3 0.2 0.1

0.4 0.1 0.2 0.2 0.2 0.2 0.4 0.3 0.2

1.6 0.2 0.5 0.9 1.2 0.3 1.1 2.0 1.1

0.5 0.1 0.2 0.3 0.3 0.2 0.4 0.3 0.2

0.7 0.2 0.3 0.5 0.4 0.2 0.7 0.9 0.3

0.8 0.3 0.8 1.5 0.6 0.7 1.4 2.8 1.6

2.3 0.3 1.3 1.2 0.9 0.8 1.8 1.5 0.9

0.2

0.1 0.2 0.3 0.1 0.1 0.2 0.6

0.1 0.2 0.3 0.1 0.1 0.4 0.3 0.1 0.1

0.4 0.2 0.5 0.8 0.2 0.6 0.9 0.8 0.4
0.2 0.4 0.4 0.5 0.1 0.3 0.7 0.9 0.2

0.6 0.2 0.5 0.5 0.4 0.3 0.6 0.9 0.4

0.7

1.0 0.2 0.6 0.8 0.8 0.6 1.0 1.6 0.8

0.9 0.3 0.5 0.6 0.4 0.3 0.8 1.4 0.5

1.3 0.3 0.8

0.6 0.2 0.8 0.9 0.3 0.5 0.8 1.5 0.6

0.4 0.2 0.2 0.8 0.3 0.3 1.1 1.7 0.2

0.2 0.1 0.2 1.0 0.1 0.2 0.4 1.3 0.1

0.2 0.2 0.2 0.7 0.1 0.1 0.4 1.1 0.2

0.3 0.1 0.3 0.5 0.1 0.2 0.7 0.7 0.1

0.3 0.1 0.2 1.0 0.1 0.2 0.5 3.6 1.0

0.2 0.2 0.3 0.4 0.1 0.2 0.5 0.6 0.2

1.1 0.3 0.3 0.9 0.5 0.4 0.8 1.3 0.2

0.5 0.5 0.4 0.7 0.2 0.3 0.9 1.3 0.2

0.3 0.2 0.2 0.7 0.2 0.1 0.5 0.8 0.3

0.6 0.2 0.4 1.2 0.7 0.6 1.1 2.2 0.3

0.6 0.3 0.5 0.7 0.6 0.5 0.9 1.2 0.9

0.6 0.2 0.6 0.8 0.6 0.7 1.9 2.0 1.0

0.2 0.3 0.5 0.6 0.2 0.6 1.4 0.6 0.3

0.1 0.1 0.2 0.1 0.1 0.1 0.2 0.1 0.1

0.2 0.1 0.2 0.1 0.1 0.2 0.2 0.1 0.1

0.2 0.2 0.2 0.2 0.2 0.3 0.4 0.2

0.3 0.2 0.4 0.3 0.2 0.2 0.4 0.4 0.2

0.3 0.6 1.7 0.6 0.5 1.2 2.4 0.6 0.5

1.1 1.5 4.6 1.8 0.9 1.3 2.1 1.8 1.6

0.6 1.2 2.9 1.1 0.6 1.4 2.0 0.9 0.7

0.4 0.5 1.7 0.7 0.3 0.7 1.5 0.7 0.6

0.3 0.5 1.8 0.8 0.6 0.9 1.8 0.7 0.7

0.7 0.7 2.6 1.1 0.6 1.3 2.1 1.3 1.3

0.2 0.5 1.2 0.5 0.3 0.5 1.5 0.5 0.4

0.3 0.2 0.5 0.2 0.1 0.2 0.4 0.6 0.2

0.3 0.2 0.6 0.2 0.4 0.3 0.4 0.6 0.2

0.8 0.2 0.3 1.1 0.7 0.4 1.0 1.6 0.4

0.8 0.2 0.4 1.4 0.6 0.7 1.1 2.6 0.6

0.6 0.3 0.5 0.3 0.2 0.3 0.6 0.5 0.3

0.6 0.3 0.8 1.1 0.4 0.5 0.8 2.2 0.9

0.7 0.5 1.6 1.5 0.4 1.1 1.2 2.5 0.7

1.0 0.5 1.9 1.9 0.5 0.6 1.3 2.4 1.1

0.2 0.1 0.1 0.4 0.1 0.1 0.5 0.7 1.3

0.1 0.1 0.2 0.3 0.1 0.1 0.2 0.3 0.1

0.3 0.1 0.2 0.3 0.1 0.2 0.7 0.4 0.6
0.2 0.2 0.2 1.2 0.2 0.2 0.5 1.2 0.5

0.3 0.2 0.3 0.7 0.2 0.3 0.8 1.4 0.4

0.3

0.4

0.5 0.2 0.5 0.8 0.2 0.3 0.5 1.2 0.3

0.4 0.3 0.5 0.7 0.2 0.4 1.1 1.2 0.4

0.7 0.3 0.5 0.6 0.5 0.4 0.9 1.2 0.7

0.4 0.2 0.6 0.3 0.2 0.4 0.5 0.8 0.2

1.7 2.5 4.8 1.7 1.0 2.3 2.1 1.6 1.5

0.3 0.5 0.8 0.5 0.2 0.7 1.4 0.6 0.3

0.3 0.4 1.1 0.5 0.3 0.8 1.8 0.7 0.5

0.4 0.5 1.0 0.9 0.4 0.8 1.8 0.7 0.5

0.2 0.5 0.9 0.5 0.3 0.7 1.5 0.6 0.4

0.1 0.1 0.2 0.1 0.1 0.1 0.2 0.2

0.2 0.1 0.2 0.1 0.1 0.2 0.2 0.1 0.1

0.3 0.2 0.4 0.2 0.2 0.2 0.4 0.5 0.1

0.4 0.2 0.4 0.3 0.2 0.4 0.5 0.5 0.3

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.2

0.1 0.0 0.1 0.1 0.0 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.2 0.1 0.1 0.2 0.3 0.1

0.2 0.1 0.1 0.4 0.1

0.4 0.2 0.8 1.6 0.4 0.1 0.2 1.6 0.6

0.1 0.1 0.1 0.2 0.1 0.1 0.3 0.3 0.1

0.1 0.0 0.2 0.3 0.1 0.1 0.3 0.4 0.1

0.1 0.1 0.1 0.3 0.0 0.0 0.2 0.3 0.1

0.1 0.0 0.1 0.2 0.0 0.1 0.2 0.2 0.1

0.4 0.2 0.5 0.2 0.2 0.3 0.5 0.5 0.2

1.0 0.3 0.5 1.2 0.8 0.6 1.4 2.5 0.6

0.2 0.4 0.6 0.5 0.2 0.6 0.8 0.6 0.2

0.2 0.4 0.5 0.6 0.2 0.3 0.8 1.2 0.3

0.2 0.4 0.6 0.4 0.2 0.4 1.2 0.5 0.3

0.3 0.4 0.6 0.4 0.2 0.4 1.1 0.7 0.3

0.2 0.3 0.4 0.4 0.1 0.4 0.7 0.6 0.2

0.5 0.2 2.4 2.9 1.2 0.6 4.4 5.8 0.5
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

1.5 2.5 2.4 2.3 2.4 3.3 2.5 2.2 1.8

0.1 0.2 0.2 0.1 0.3 0.2 0.2 0.1 0.1

0.3 0.6 0.7 0.2 0.3 0.6 0.2 0.2 0.4

0.1 0.2 0.4 0.1 0.1

0.1 0.5 0.9 0.3 0.2 0.5 0.5 0.2 0.2

0.2 1.1 2.2 0.2 0.1 0.7 0.3 0.3 0.3

0.4 0.6 0.8 0.5 0.6 0.5 0.9 0.4 0.8

0.3 0.4 0.5 0.5 0.3 1.6 0.7 0.3 0.3

1.5 1.0 0.9 1.6 1.5 1.5 1.0 1.4 1.3

0.4 0.6 0.9 0.5 0.3 0.7 1.3 0.9 0.3

0.2 0.3 1.4 0.4 0.2 0.5 1.9 0.2 0.2

0.7 0.7 1.1 1.7 0.6 0.7 1.4 1.4 0.7

0.5 0.8 0.8 0.9 0.5 0.6 1.0 0.6 0.6

0.8 0.7 0.7 1.6 0.6 0.6 2.4 0.8 0.7

0.3 0.6 0.8 0.4 0.2 0.7 0.8 0.5 0.3

0.5 0.4 0.8 0.7 0.4 0.7 0.9 0.5 0.4

0.4 0.4 0.3 0.5 0.5 0.5 0.4 0.5 0.5

0.6 0.6 0.7 0.6 0.7 0.7 0.7 0.7 0.7

0.6 0.6 0.5 0.7 0.7 0.7 0.8 0.7 0.8

0.6 0.6 0.6 0.7 0.6 0.6 0.9 0.6 0.5

1.3 1.8 2.3 1.8 1.9 2.5 2.3 1.4 1.6

1.3 1.9 2.2 1.8 1.8 2.4 2.4 1.5 1.3

0.6 0.5 1.1 0.7 0.3 0.7 1.8 0.8 0.7

0.2 0.7 2.0 0.7 0.3 0.8 1.9 0.5 0.2

0.3 0.6 1.0 0.3 0.2 0.6 0.9 0.3 0.2

0.8 1.4 3.0 0.9 0.7 1.5 2.3 1.0 0.7

0.6 0.7 0.8 0.4 0.6 0.7 1.0 0.5 0.6

0.7 0.6 0.4

0.6 0.2 0.2 0.8 0.8 0.3 0.2 0.9 0.7

0.3 0.7 1.7 0.6 0.3 0.8 2.8 0.9 0.4

0.2 0.3 1.1 0.4 0.1 0.4 1.3 0.2 0.2

0.7 1.2 1.6 1.0 0.6 1.2 1.5 1.0 0.6

0.9 0.8 0.8 1.0 0.8 1.0 0.9 1.3 0.9

0.6 1.0 1.0 0.5 0.4 0.8 1.1 0.5 0.4

0.4 1.1 1.4 0.5 0.4 1.1 1.6 0.5 0.4

0.6 0.9 1.3 0.8 0.4 0.8 1.3 0.8 0.4

0.3 0.5 2.2 0.4 0.2 0.6 1.4 1.1 0.6

0.4 0.5 1.2 0.7 0.4 0.5 1.4 1.0 0.4

0.6 0.4 1.2 0.8 0.4 0.4 1.7 2.2 0.6

0.9 1.8 3.6 1.3 1.0 2.0 3.3 1.6 1.1

Speciation Measurements

Organic Carbon
0.6 0.6 0.7 0.6 0.5 1.6 1.0 0.6 0.5

0.2 0.6 0.7

0.2 0.5 0.7 0.3 0.1 0.4 0.6 0.3 0.2

0.4 0.6 0.8 0.5 0.4 0.7 1.0 0.4 0.3

0.4 0.7 1.0 0.4 0.3 0.7 1.0 0.3 0.3

0.4 0.5 0.7 0.5 0.4 0.5 0.7 0.3 0.3

0.1 0.3 0.6 0.3 0.1 0.5 0.6 0.2 0.1

1.9 2.1 1.8 2.0 1.7 2.4 2.0 2.2 1.8

1.9 1.9 1.4 2.2 2.6 1.7 1.9 1.8 2.1

1.1 0.7 0.8 1.0 1.1 1.7 1.3 0.8 0.8

1.9 1.8 1.7 2.6 3.2 2.0 2.1 1.6 1.7

2.0 2.2 1.9 2.4 3.0 4.1 3.5 1.9 2.6

1.2 2.3 2.5 1.8 2.1 3.4 2.2 1.5 1.6

0.3 0.2

0.3 0.6 0.7 0.5 0.3 0.5 0.8 0.3 0.2

0.9 1.6 1.5 0.9 1.0 1.2 1.9 1.1 1.1

1.0 2.0 1.6 1.2 1.6 2.7 1.7 1.2 1.3

0.6 1.1 1.3 0.8 0.7 1.6 1.5 0.6 0.6

1.5 2.1 2.6 1.9 1.8 2.5 2.5 1.6 1.6

1.6 2.5 2.4 2.4 0.9

1.6 2.0 1.5 2.1 1.8 1.7 1.7 1.7 1.2

1.7 2.3 2.4 2.6

0.9 2.1 1.6 1.0 1.2 1.0 1.8 1.2 1.5

0.7 1.5 1.4 0.9 1.1 1.1 1.9 1.2 1.5

1.2 1.7 1.6 1.3 1.7 1.1 2.4 1.9 1.9

0.5 1.4 1.3 0.6 0.7 0.8 1.4 0.8 0.9

1.1 1.8 1.5 1.5 1.9 1.2 1.6 2.0 2.1

0.6 1.4 1.2 0.7 0.8 0.9 1.4 1.0 0.8

1.3 1.7 1.9 1.3 1.4 1.6 1.7 1.2 1.2

0.8 1.2 1.5 0.8 0.8 1.1 1.7 1.0 1.0

0.9 1.4 1.4 0.9 1.0 1.1 1.7 1.3 1.1

1.1 1.7 1.6 1.1 1.3 1.2 2.1 1.3 1.5

0.6 1.2 1.5 0.5 0.5 1.2 2.2 0.8 0.6

0.7 1.6 1.5 0.8 0.7 1.2 1.6 0.9 0.7

0.7 0.9 1.8 0.7 0.5 1.0 3.1 1.5 0.6

0.9 1.0 1.2 1.2 0.8 1.2 1.3 1.2 1.0

0.8 1.0 1.7 1.0 0.6 0.8 1.5 1.0 0.7

1.5 1.4 1.5 1.3 1.3 1.5 1.8 1.3 1.2

1.7 1.8 1.8 1.7 2.1 2.1 2.0 1.8 1.9

2.1 2.0 2.9 3.3 2.2 2.6 2.3 2.5 2.2

0.2 0.1 -0.1 0.0

0.2 0.3 0.2 0.4 0.3 0.4 0.2 0.3 0.2

0.1 0.1 -0.1 0.0 0.1 0.1 0.0 0.0 0.0

0.3 0.4 1.1 0.5 0.2 0.4 1.9 0.7 0.3
1.1 1.3 1.7 1.0 0.6 0.6 2.4 0.8 0.6

1.4 1.5 1.9 1.5 1.6 1.8 1.9 1.5 1.3

1.7 1.8 2.2 1.8

1.0 1.4 1.6 1.2 1.1 1.8 1.6 1.3 1.3

1.3 1.5 1.5 1.4 1.6 1.8 1.9 1.3 1.3

1.4 1.8 1.8 1.7 1.5 2.2

1.8 1.9 1.9 2.0 2.2 2.4 1.9 1.7 2.2

0.6 0.5 1.2 0.6 0.4 0.5 1.3 0.6 0.3

1.4 0.8 1.8 1.6 0.9 1.0 2.3 1.9 0.8

0.5 0.6 1.3 1.0 0.3 0.6 2.0 1.3 0.3

0.2 0.4 1.2 0.7 0.1 0.4 1.5 0.5 0.1

0.5 0.5 1.5 2.1 0.3 0.5 2.2 1.5 0.4

0.3 0.5 1.3 0.6 0.2 0.4 4.4 0.6 0.2

0.8 0.7 1.9 1.0 0.7 0.9 1.3 0.8 0.5

0.4 0.5 1.0 0.5 0.3 0.5 2.2 0.4 0.2

0.4 0.6 1.4 1.3 0.2 0.5 1.5 1.3 0.3

0.6 0.7 1.7 0.7 0.5 0.7 1.1 0.8 0.4

0.4 0.6 1.3 0.6 0.6 1.1 1.1 0.5 0.3

0.5 0.7 1.3 0.7 0.8 1.1 1.2 0.6 0.4

0.4 0.3 0.5 1.8 0.3 0.5 0.9 0.3 0.3

0.2 1.2 1.6 0.7 0.7 1.1 2.5 0.7 0.7

0.7 1.5 1.5 0.6 0.8 0.9 1.7 0.9 1.0

1.9 1.5 2.5 2.0 2.1

1.3 1.6 1.8 1.5 1.4 2.3 1.8 1.7 1.4

0.3 0.7 0.9 0.4 0.4 2.3 1.0 0.4 0.3

0.6 0.8 0.9 1.0 0.8 1.7 1.1 0.7 0.5

0.5 0.9 0.7 0.5 0.4 1.4 1.2 0.4 0.3

0.5 0.7 0.7 0.7 0.5 2.0 1.9 0.6 0.5

0.3 0.5 0.7 0.5 0.3 1.6 1.8 0.2 0.2

0.6 0.7 0.6 0.8 0.7 1.3 0.8 0.7 0.5

0.2 0.6 0.5 0.3 0.2 1.2 0.9 0.2 0.2

1.0 1.5

1.4 2.1 2.2 1.8 1.5 2.5 1.8 1.4 1.9

0.8 2.0 2.4 1.0 0.9 2.3 1.8 0.9 0.9

0.7 0.7 1.3 0.8 0.5 0.8 1.2 0.6 0.3

0.7 0.9 1.9 0.8 0.6 1.0 1.2 0.8 0.5

1.6 1.5 1.6 1.8 1.7 1.7 1.6 1.3 1.3

1.8 2.0 2.3 3.0 2.8 2.5 2.3 2.2

0.9 1.7 1.8 1.3 1.7 2.2 2.1 0.9 1.0

0.7 1.1 1.3 1.0 1.2 2.3 1.4 0.7 0.7

1.0 2.8

0.2 0.3 0.9 0.5 0.2 0.3 2.5 0.7 0.1

0.9 0.8 1.5 1.3 1.1 0.7 1.0 1.9 1.1

0.3 0.4 1.0 0.5 0.1 0.3 1.4 1.0 0.2
0.5 0.4 1.3 1.1 1.7 0.4 1.6 0.9 0.3

0.6 0.6 1.5 1.3 0.6 0.6 1.7 1.2 0.4

1.4 2.0 2.2 1.6

1.9 2.0 2.5 2.2

2.0 1.7 1.5 2.9 2.5 3.1 2.0 1.5 2.5

0.6 0.5 1.0 2.9 0.5 0.7 1.5 0.4 0.3

0.5 0.7 1.1 0.6 0.5 0.9 1.3 0.6 0.3

1.1 2.2 2.4 1.5 1.4 2.5 2.0 1.3 1.4

0.4 0.7 0.6 0.7 0.5 1.6 0.9 0.5 0.4

0.3 0.5 0.8 0.6 0.2 0.6 1.3 0.3 0.2

0.5 0.4 0.6 0.5 0.3 0.3 0.6 0.4 0.3

0.4 0.4 0.9 0.5 0.4 0.6 0.8 0.5 0.4

0.3 0.3 0.7 0.5 0.3 0.5 0.8 0.4 0.2

0.5 1.3 1.5 0.4 0.5 0.8 1.5 0.7 0.7

1.0 1.6 1.7 0.9 1.2 1.1 2.0 1.1 1.0

0.8 1.6 1.9 0.9 0.9 1.7 1.7 1.0 1.0

2.3 2.1 2.4 2.6 2.2 2.2 2.5 2.6 2.4

0.5 0.3 0.2 0.3 0.8 0.3

1.3 0.6 0.7 1.8

0.5 0.5 0.9 0.7 0.4 0.4 0.9 0.8 0.4

0.4 0.4 1.3 0.7 0.3 0.4 1.3 0.6 0.2

0.9 0.8 1.3 1.9 0.9 0.9 1.5 2.0

1.1 0.6 1.6 1.7 0.9 0.6 1.7 1.6 1.1

0.3 0.3 0.9 0.3 0.1 0.2 0.9 0.3 0.1

0.3 0.4 1.4 0.9 0.1 0.5 1.1 0.6 0.1

0.4 0.5 1.1 0.6 0.6 0.5 1.4 1.0 0.4

0.2 0.4 1.5 0.6 0.1 0.4 1.2 0.5 0.1

1.8 1.5 1.9 1.3 1.7 1.6 1.6 1.2 1.2

0.6 0.5 0.9 0.7 0.6 0.6 1.5 0.7 0.4

0.3 0.3 0.9 0.3 0.2 0.2 1.6 0.3 0.1

0.2 0.3 1.0 0.3 0.2 0.5 1.7 0.4 0.2

0.3 0.3 1.0 0.4 0.2 0.4 1.1 0.3 0.1

0.3 0.3 0.8 0.4 0.3 0.3 1.0 0.3 0.2

0.2 0.3 1.2 0.4 0.2 0.4 2.3 0.6 0.2

0.3 0.2 0.4 0.1 0.2 0.3 0.1 0.1 0.1
2012 2012 2012 2010 2010 2010 2010 2011 2011

2 3 4 1 2 3 4 1 2

2.2 1.9 1.8 0.3 0.3 0.3 0.4 0.4 0.4

0.2 0.2 0.1 0.1 0.1 0.1 0.0 0.1 0.1

0.4 0.4 0.2 0.0 0.0 0.1 0.0 0.0 0.1

0.3 0.4 0.1 0.0 0.0

0.6 0.5 0.1 0.0 0.0 0.1 0.0 0.0 0.0

0.5 0.4 0.1 0.0 0.1 0.1 0.0 0.0 0.1

0.8 1.2 0.7 0.1 0.1 0.1 0.1 0.1 0.1

0.8 0.7 0.3 0.1 0.1 0.1 0.1 0.1 0.2

1.3 1.2 1.4 0.4 0.2 0.2 0.3 0.3 0.2

0.9 1.0 0.9 0.1 0.1 0.1 0.1 0.0 0.1

0.6 0.8 0.4 0.0 0.1 0.2 0.1 0.0 0.1

1.6 1.4 1.2 0.2 0.1 0.2 0.3 0.1 0.1

0.8 1.0 0.9 0.1 0.1 0.1 0.1 0.1 0.1

1.3 1.3 0.8 0.1 0.1 0.1 0.2 0.1 0.1

0.7 0.9 0.4 0.1 0.1 0.1 0.1 0.0 0.1

0.9 1.1 0.5 0.2 0.1 0.2 0.2 0.2 0.1

0.5 0.5 0.4 0.1 0.1 0.1 0.1 0.1 0.1

0.8 0.9 0.5 0.1 0.1 0.1 0.2 0.2 0.1

0.9 0.8 0.7 0.2 0.1 0.1 0.2 0.2 0.1

0.8 0.9 0.6 0.1 0.1 0.1 0.2 0.1 0.1

1.9 1.8 1.6 0.2 0.2 0.2 0.3 0.3 0.3

1.8 1.6 1.4 0.2 0.2 0.2 0.3 0.3 0.3

0.8 1.5 0.6 0.1 0.1 0.1 0.1 0.0 0.1

1.2 1.2 0.5 0.0 0.1 0.2 0.1 0.0 0.1

0.7 1.2 0.3 0.0 0.1 0.1 0.1 0.0 0.1

1.6 1.5 0.6 0.1 0.1 0.3 0.1 0.1 0.2

0.7 2.1 0.6 0.3 0.1 0.1 0.2 0.2 0.1

1.0 1.1 0.4

0.2 0.3 0.5 0.1 0.0 0.0 0.1 0.1 0.0

1.2 1.7 0.7 0.0 0.1 0.2 0.1 0.0 0.1

0.5 1.1 0.1 0.0 0.0 0.1 0.0 0.0 0.0

1.2 1.3 0.8 0.2 0.2 0.3 0.2 0.1 0.2

0.8 1.0 0.9 0.1 0.1 0.2 0.2 0.1 0.1

0.9 1.0 0.4 0.1 0.2 0.2 0.1 0.1 0.1

1.2 1.4 0.4 0.1 0.2 0.2 0.1 0.1 0.2

0.9 1.0 0.4 0.1 0.1 0.2 0.1 0.0 0.1

0.6 4.3 0.5 0.0 0.1 0.3 0.1 0.0 0.1

0.6 5.5 0.7 0.1 0.0 0.1 0.1 0.0 0.1

0.6 3.8 0.8 0.1 0.0 0.1 0.1 0.0 0.0

2.4 2.4 1.2 0.1 0.2 0.4 0.2 0.1 0.2

Speciation Measurements

Elemental Carbon
1.2 1.5 0.6 0.1 0.1 0.1 0.1 0.1 0.1

0.0 0.1

0.7 2.5 0.7 0.0 0.1 0.1 0.0 0.0 0.0

2.0 1.6 0.5 0.1 0.0 0.1 0.1 0.1 0.1

1.2 2.3 0.4 0.1 0.1 0.1 0.1 0.1 0.1

0.7 1.2 0.3 0.1 0.0 0.1 0.1 0.1 0.1

0.5 1.6 0.2 0.0 0.1 0.1 0.1 0.0 0.1

1.3 1.5 2.5 0.9 0.8 0.9 1.1 0.8 1.0

1.8 1.3 2.0 0.4 0.3 0.2 0.5 0.4 0.3

0.8 1.1 0.8 0.2 0.1 0.1 0.2 0.2 0.2

1.4 1.2 1.7 0.4 0.2 0.2 0.4 0.4 0.2

1.7 1.6 1.6 0.4 0.3 0.2 0.4 0.4 0.4

2.7 1.6 1.5 0.2 0.3 0.3 0.3 0.3 0.3

0.8 2.1 0.3

1.1 1.5 0.3 0.1 0.1 0.1 0.1 0.0 0.1

1.1 1.4 1.0 0.2 0.3 0.3 0.2 0.2 0.2

1.8 1.6 1.4 0.2 0.3 0.2 0.2 0.3 0.4

1.4 1.5 0.8 0.1 0.1 0.1 0.1 0.1 0.2

1.9 1.9 1.6 0.3 0.3 0.4 0.3 0.3 0.3

0.3 0.3 0.3 0.4 0.1

1.5 1.0 2.0 0.4 0.3 0.3 0.5 0.4 0.3

0.3 0.3 0.2 0.3

0.9 1.4 1.2 0.2 0.2 0.2 0.2 0.2 0.1

1.1 1.5 1.1 0.1 0.2 0.2 0.1 0.2 0.1

1.4 1.5 1.6 0.2 0.2 0.3 0.2 0.3 0.2

0.6 1.2 0.8 0.1 0.2 0.2 0.1 0.1 0.1

1.0 1.3 1.8 0.2 0.3 0.2 0.3 0.4 0.2

0.7 1.1 0.9 0.1 0.1 0.1 0.1 0.1 0.1

1.3 1.4 1.3 0.3 0.3 0.3 0.3 0.3 0.3

1.1 1.3 0.8 0.1 0.1 0.2 0.1 0.1 0.2

1.1 1.2 0.7 0.2 0.2 0.2 0.2 0.1 0.1

1.1 1.4 1.1 0.2 0.2 0.2 0.2 0.3 0.2

0.9 1.6 0.5 0.1 0.1 0.1 0.1 0.1 0.1

0.9 1.4 0.6 0.1 0.2 0.2 0.1 0.1 0.1

0.8 1.6 0.9 0.1 0.1 0.1 0.1 0.1 0.1

1.1 1.8 1.1 0.2 0.2 0.2 0.3 0.2 0.2

0.8 1.8 0.7 0.1 0.1 0.1 0.1 0.1 0.1

1.1 1.7 1.2 0.3 0.2 0.2 0.3 0.2 0.2

1.8 1.6 1.8 0.3 0.2 0.2 0.3 0.3 0.3

2.0 1.8 2.1 0.4 0.3 0.4 0.4 0.4 0.4

0.0 0.0 0.0 0.0

0.3 0.0 0.0 0.1 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.5 7.6 0.7 0.0 0.0 0.1 0.1 0.0 0.0
0.8 10.3 1.7 0.2 0.1 0.1 0.1 0.0 0.1

1.4 1.8 1.3 0.3 0.3 0.4 0.4 0.3 0.3

0.4 0.3 0.4 0.4

1.4 1.8 1.3 0.2 0.3 0.3 0.2 0.2 0.3

1.5 1.7 1.2 0.3 0.2 0.2 0.3 0.3 0.3

0.3 0.3 0.3 0.3 0.3 0.3

1.7 1.5 1.7 0.3 0.2 0.2 0.3 0.3 0.3

0.7 2.7 0.5 0.1 0.0 0.1 0.1 0.1 0.1

1.1 3.6 1.6 0.3 0.1 0.2 0.3 0.2 0.1

0.8 3.7 0.9 0.1 0.1 0.1 0.1 0.0 0.1

0.6 5.6 0.5 0.0 0.0 0.1 0.1 0.0 0.0

0.7 5.8 2.1 0.1 0.0 0.1 0.2 0.0 0.1

0.7 18.3 2.3 0.0 0.0 0.1 0.1 0.0 0.0

0.9 1.9 0.5 0.1 0.1 0.1 0.1 0.1 0.1

1.2 6.1 0.3 0.1 0.1 0.1 0.1 0.0 0.1

0.7 2.9 1.2 0.1 0.1 0.1 0.1 0.0 0.1

0.8 2.3 0.6 0.1 0.1 0.2 0.1 0.1 0.1

0.8 2.0 0.4 0.1 0.1 0.1 0.1 0.1 0.1

1.0 2.0 0.6 0.1 0.1 0.1 0.1 0.1 0.1

0.4 1.5 0.3 0.1 0.0 0.1 0.1 0.0 0.0

1.0 1.6 0.6 0.1 0.1 0.2 0.1 0.1 0.1

0.9 1.2 0.7 0.1 0.2 0.2 0.1 0.1 0.1

1.4 1.8 1.8 0.4 0.2

1.3 1.7 1.3 0.3 0.3 0.3 0.3 0.3 0.3

2.1 1.1 0.4 0.1 0.1 0.1 0.1 0.1 0.3

1.2 1.1 0.8 0.1 0.1 0.1 0.2 0.1 0.1

1.2 1.2 0.4 0.0 0.1 0.1 0.1 0.0 0.1

0.8 1.3 0.7 0.1 0.1 0.1 0.1 0.1 0.2

0.8 1.0 0.3 0.0 0.1 0.1 0.1 0.0 0.2

3.7 1.2 0.7 0.1 0.1 0.1 0.2 0.2 0.2

0.6 1.2 0.2 0.1 0.1 0.0 0.0 0.1 0.1

0.2 0.3

1.8 1.7 1.5 0.2 0.3 0.3 0.3 0.2 0.3

1.4 1.3 0.7 0.1 0.3 0.3 0.2 0.1 0.2

0.8 1.9 0.5 0.1 0.1 0.2 0.2 0.1 0.1

0.8 1.3 0.5 0.2 0.2 0.3 0.2 0.2 0.2

1.6 1.4 1.3 0.4 0.3 0.3 0.4 0.3 0.3

2.3 1.7 2.2 0.2 0.3 0.4 0.4 0.3

1.6 1.4 1.0 0.2 0.2 0.2 0.2 0.3 0.2

1.5 1.7 0.9 0.1 0.1 0.2 0.2 0.2 0.2

0.2 0.5

0.4 2.6 0.9 0.0 0.0 0.1 0.1 0.0 0.1

0.7 1.1 1.0 0.1 0.1 0.1 0.1 0.1 0.1

0.7 2.2 0.6 0.1 0.1 0.1 0.1 0.1 0.0
0.6 3.4 0.8 0.1 0.0 0.1 0.1 0.1 0.0

0.7 4.3 1.4 0.1 0.1 0.1 0.1 0.1 0.1

0.3 0.3 0.4 0.3

0.4 0.4 0.5 0.5

1.5 1.5 1.8 0.4 0.2 0.2 0.4 0.4 0.3

0.5 2.2 0.5 0.1 0.1 0.1 0.3 0.1 0.1

0.9 2.1 0.5 0.1 0.1 0.1 0.1 0.1 0.1

1.7 1.5 1.3 0.2 0.3 0.3 0.3 0.2 0.3

1.3 1.5 0.6 0.1 0.1 0.1 0.1 0.1 0.1

0.6 1.4 0.2 0.0 0.1 0.1 0.1 0.0 0.1

0.4 1.6 0.3 0.1 0.0 0.1 0.1 0.0 0.0

0.6 1.1 0.4 0.1 0.1 0.1 0.1 0.1 0.1

0.7 1.6 0.3 0.1 0.0 0.1 0.1 0.0 0.1

0.8 1.2 0.1 0.2 0.2 0.1 0.1 0.1

1.0 1.3 0.9 0.2 0.2 0.2 0.2 0.2 0.1

1.3 1.4 0.9 0.2 0.2 0.3 0.2 0.1 0.2

2.0 2.3 2.7 0.5 0.4 0.5 0.5 0.4 0.4

0.2 0.6 0.5 0.1 0.0 0.0

0.2 0.1 0.1 0.3

0.6 1.2 0.6 0.1 0.1 0.1 0.1 0.0 0.1

0.5 3.7 1.2 0.1 0.1 0.2 0.1 0.1 0.1

0.1 0.1 0.2 0.2 0.2 0.2

0.9 2.8 1.8 0.3 0.1 0.2 0.3 0.2 0.1

0.4 3.7 0.8 0.0 0.0 0.1 0.0 0.0 0.0

0.3 3.7 0.8 0.0 0.0 0.1 0.1 0.0 0.1

0.7 2.7 0.7 0.1 0.1 0.2 0.1 0.1 0.1

0.4 2.1 0.5 0.0 0.1 0.1 0.1 0.0 0.1

1.3 1.3 1.0 0.3 0.2 0.2 0.2 0.2 0.2

1.1 3.7 0.4 0.2 0.1 0.1 0.2 0.1 0.1

0.9 3.4 0.3 0.0 0.0 0.1 0.0 0.0 0.0

0.6 4.5 0.3 0.0 0.0 0.1 0.0 0.0 0.0

1.3 3.3 0.4 0.0 0.0 0.1 0.0 0.0 0.0

1.0 3.3 0.4 0.0 0.0 0.1 0.1 0.0 0.0

0.5 5.4 0.5 0.0 0.0 0.1 0.0 0.0 0.0

0.2 0.2 0.1 0.1 0.1 0.4 0.0 0.0 0.1
2011 2011 2012 2012 2012 2012 2010 2010 2010

3 4 1 2 3 4 1 2 3

0.4 0.3 0.3 0.4 0.3 0.3 3.9 4.6 5.3

0.1 0.0 0.1 0.1 0.1 0.0 0.8 1.1 1.3

0.0 0.0 0.1 0.0 0.0 0.0 0.7 0.6 0.5

0.0 0.0 0.0 0.0 0.1 0.0

0.0 0.0 0.0 0.1 0.0 0.0 0.6 0.8 0.5

0.0 0.0 0.0 0.1 0.0 0.0 0.9 0.7 0.4

0.1 0.1 0.1 0.1 0.1 0.1 0.8 1.3 1.4

0.1 0.1 0.1 0.1 0.1 0.1 1.1 1.5 1.8

0.2 0.4 0.3 0.2 0.2 0.3 1.0 1.6 2.0

0.1 0.1 0.1 0.1 0.1 0.1 1.0 1.2 1.5

0.3 0.0 0.0 0.1 0.1 0.1 0.9 1.1 1.2

0.2 0.3 0.2 0.2 0.2 0.3 0.8 1.0 1.3

0.1 0.1 0.1 0.1 0.1 0.2 1.1 1.4 2.1

0.3 0.2 0.1 0.1 0.1 0.2 0.9 1.2 1.7

0.1 0.1 0.1 0.1 0.1 0.1 1.0 1.2 1.7

0.2 0.2 0.1 0.2 0.2 0.2 1.0 1.1 1.4

0.1 0.1 0.1 0.1 0.1 0.1 1.1 1.6 2.3

0.1 0.2 0.1 0.1 0.1 0.1 1.1 1.6 2.0

0.1 0.2 0.2 0.1 0.1 0.2 1.1 1.4 2.1

0.1 0.1 0.1 0.1 0.1 0.1 1.3 1.4 2.3

0.2 0.2 0.3 0.2 0.2 0.2 2.8 4.3 4.3

0.2 0.2 0.2 0.2 0.2 0.2 3.0 4.7 4.1

0.2 0.1 0.1 0.1 0.2 0.1 0.5 1.0 0.9

0.1 0.1 0.1 0.1 0.1 0.1 0.6 1.1 1.4

0.1 0.1 0.0 0.1 0.1 0.0 0.8 1.5 1.6

0.2 0.1 0.1 0.2 0.2 0.1 0.9 1.9 2.1

0.1 0.2 0.3 0.1 0.4 0.1 0.7 1.2 1.3

0.1 0.1 0.1 0.1 0.2 0.1

0.0 0.1 0.1 0.0 0.0 0.1 2.0 1.7 1.8

0.2 0.1 0.1 0.1 0.2 0.1 0.6 1.1 1.3

0.1 0.0 0.0 0.1 0.1 0.0 0.5 0.9 0.9

0.3 0.2 0.1 0.2 0.3 0.2 1.0 2.6 3.3

0.1 0.2 0.1 0.1 0.1 0.1 0.8 1.5 1.7

0.2 0.1 0.1 0.1 0.2 0.1 0.8 1.5 1.8

0.3 0.1 0.1 0.2 0.2 0.1 0.9 1.5 1.8

0.1 0.1 0.1 0.1 0.1 0.1 0.9 1.6 2.0

0.2 0.1 0.0 0.1 0.5 0.1 0.4 0.9 0.8

0.1 0.1 0.0 0.1 0.4 0.1 0.5 0.9 0.7

0.1 0.2 0.1 0.1 0.3 0.1 0.5 0.8 0.9

0.3 0.3 0.2 0.2 0.3 0.2 1.0 2.0 2.8

Speciation Measurements

Elemental Carbon
0.1 0.1 0.1 0.1 0.1 0.1 0.7 0.9 0.9

0.1

0.1 0.0 0.0 0.1 0.2 0.1 0.8 0.8 0.8

0.1 0.1 0.1 0.2 0.1 0.1 0.9 0.9 1.0

0.1 0.0 0.0 0.1 0.2 0.1 0.8 1.0 1.0

0.1 0.1 0.0 0.1 0.1 0.1 0.9 0.9 1.1

0.1 0.0 0.0 0.1 0.2 0.0 0.6 0.7 0.8

0.8 0.9 0.7 0.6 0.6 1.1 3.7 5.1 5.5

0.2 0.4 0.4 0.2 0.2 0.4 3.9 4.0 3.3

0.1 0.2 0.2 0.1 0.1 0.1 3.6 3.4 2.4

0.2 0.2 0.2 0.2 0.1 0.2 4.0 4.6 4.4

0.3 0.3 0.4 0.2 0.2 0.3 4.0 4.6 4.4

0.2 0.2 0.2 0.2 0.2 0.2 3.6 4.9 6.4

0.0 0.0 0.1 0.2 0.0

0.1 0.1 0.0 0.1 0.2 0.1 0.7 0.9 0.9

0.3 0.2 0.2 0.2 0.2 0.2 2.1 2.9 3.8

0.2 0.2 0.2 0.2 0.2 0.2 2.6 3.3 3.4

0.1 0.1 0.1 0.2 0.2 0.1 1.9 2.5 2.5

0.3 0.3 0.3 0.3 0.3 0.3 4.8 5.6 5.9

4.5 5.8 6.1

0.3 0.3 0.3 0.3 0.2 0.4 4.2 5.8 4.7

3.5 4.5 3.9

0.2 0.2 0.3 0.1 0.2 0.2 1.3 1.2 2.1

0.2 0.2 0.2 0.2 0.2 0.2 1.4 1.9 2.7

0.4 0.4 0.3 0.2 0.2 0.3 1.5 2.3 3.1

0.2 0.1 0.1 0.1 0.1 0.1 1.3 1.8 2.8

0.2 0.4 0.4 0.2 0.2 0.3 1.4 1.6 2.7

0.1 0.1 0.1 0.1 0.1 0.1 1.3 1.5 2.5

0.3 0.3 0.3 0.3 0.3 0.3 3.9 5.1 7.0

0.2 0.2 0.2 0.1 0.2 0.1 1.9 2.9 3.7

0.2 0.2 0.1 0.1 0.2 0.1 2.3 3.1 4.0

0.3 0.3 0.3 0.2 0.3 0.2 2.0 2.9 3.5

0.2 0.1 0.1 0.1 0.1 0.1 2.1 1.8 1.4

0.2 0.2 0.1 0.1 0.2 0.1 1.9 2.0 2.4

0.2 0.2 0.1 0.1 0.1 0.1 2.1 1.6 0.9

0.2 0.3 0.3 0.2 0.2 0.2 3.1 2.1 2.2

0.1 0.2 0.1 0.1 0.1 0.1 2.3 1.5 1.0

0.3 0.3 0.2 0.2 0.2 0.2 2.4 2.2 2.5

0.2 0.4 0.3 0.3 0.2 0.3 3.4 3.8 3.6

0.3 0.4 0.4 0.3 0.3 0.4 3.5 4.5 4.8

10.4 1.9 1.2

0.0 0.1 0.0 0.1 2.4 1.9 1.0

0.0 0.0 0.0 0.0 0.0 0.0 1.3 1.3 0.7

0.1 0.1 0.0 0.1 0.6 0.1 0.6 0.8 0.6
0.2 0.1 0.1 0.1 0.8 0.1 0.6 0.8 0.6

0.4 0.4 0.3 0.3 0.3 0.3 3.4 4.3 4.5

4.9 6.7 7.3

0.3 0.3 0.3 0.3 0.3 0.3 2.8 2.7 3.1

0.3 0.3 0.3 0.3 0.2 0.3 3.2 3.0 2.9

3.1 3.0 3.1

0.2 0.3 0.3 0.3 0.2 0.3 2.9 3.9 4.2

0.1 0.1 0.0 0.1 0.2 0.1 1.5 1.1 0.8

0.3 0.3 0.2 0.2 0.4 0.2 0.7 0.8 0.7

0.1 0.1 0.0 0.1 0.3 0.1 0.6 0.9 0.6

0.1 0.1 0.0 0.1 0.4 0.0 0.6 0.8 0.6

0.2 0.2 0.1 0.1 0.4 0.2 0.6 0.7 0.5

0.3 0.1 0.0 0.1 1.5 0.2 0.6 0.8 0.6

0.1 0.1 0.1 0.1 0.2 0.1 3.5 1.5 1.2

0.2 0.1 0.0 0.1 0.5 0.0 1.3 1.1 0.9

0.1 0.1 0.0 0.1 0.2 0.1 0.6 0.8 0.7

0.1 0.1 0.1 0.1 0.2 0.1 2.8 1.2 1.3

0.1 0.1 0.1 0.1 0.2 0.1 1.9 1.5 1.7

0.1 0.1 0.1 0.1 0.2 0.1 2.2 1.9 1.8

0.1 0.1 0.1 0.0 0.1 0.0 0.7 0.9 1.1

0.2 0.1 0.1 0.1 0.2 0.1 1.6 1.7 2.5

0.2 0.2 0.2 0.1 0.2 0.1 1.8 2.5 3.2

0.3 0.4 0.4 0.3 0.3 0.4

0.3 0.3 0.3 0.2 0.3 0.3 3.5 4.6 5.5

0.1 0.1 0.1 0.2 0.1 0.1 0.9 1.3 1.7

0.1 0.2 0.1 0.1 0.1 0.2 1.6 2.5 2.3

0.2 0.1 0.1 0.1 0.1 0.1 0.9 2.4 1.6

0.2 0.1 0.1 0.1 0.1 0.1 0.9 1.2 1.2

0.2 0.0 0.0 0.1 0.1 0.0 0.8 1.1 1.2

0.1 0.2 0.1 0.4 0.1 0.2 0.8 1.4 1.5

0.1 0.0 0.1 0.1 0.1 0.0 0.6 1.0 1.0

2.7 4.3

0.3 0.2 0.3 0.3 0.2 0.3 3.9 4.4 5.6

0.2 0.1 0.1 0.2 0.2 0.1 2.2 4.5 5.1

0.2 0.1 0.1 0.1 0.2 0.1 2.3 1.6 1.3

0.2 0.2 0.2 0.2 0.2 0.2 3.1 1.7 1.5

0.3 0.3 0.3 0.3 0.4 0.3 4.3 5.5 7.1

0.3 0.4 0.4 0.3 0.2 0.4 4.5 4.2

0.2 0.2 0.2 0.2 0.2 0.2 2.5 4.0 3.6

0.2 0.2 0.1 0.2 0.2 0.2 2.0 3.1 2.6

2.7 4.1

0.2 0.1 0.0 0.1 0.2 0.1 0.5 0.8 0.8

0.1 0.2 0.1 0.1 0.1 0.1 0.4 1.2 1.1

0.1 0.1 0.1 0.1 0.2 0.1 0.2 0.6 0.5
0.1 0.1 0.0 0.1 0.3 0.1 0.8 0.9 0.9

0.1 0.2 0.1 0.1 0.3 0.1 0.8 0.8 0.8

3.6 5.0 6.9

3.5 4.4 6.2

0.2 0.3 0.4 0.2 0.2 0.3 4.2 5.1 4.5

0.1 0.1 0.1 0.1 0.2 0.1 1.4 1.2 1.1

0.1 0.1 0.1 0.1 0.2 0.1 2.2 1.4 1.4

0.3 0.2 0.2 0.3 0.2 0.2 3.7 4.9 6.2

0.1 0.1 0.1 0.1 0.1 0.1 1.0 1.6 2.2

0.1 0.1 0.0 0.1 0.1 0.0 0.9 0.9 1.1

0.1 0.1 0.1 0.1 0.2 0.1 1.2 1.0 1.0

0.1 0.1 0.1 0.1 0.1 0.1 0.9 0.9 1.3

0.1 0.1 0.0 0.1 0.2 0.1 1.0 0.9 1.0

0.2 0.1 0.2 0.1 0.2 1.8 2.4 4.2

0.2 0.2 0.2 0.1 0.2 0.2 1.9 2.4 3.3

0.3 0.2 0.2 0.2 0.3 0.2 3.0 4.8 6.3

0.5 0.5 0.5 0.4 0.4 0.5 3.8 5.0 5.9

0.0 0.1 0.0 0.0 0.0 0.1

0.9 1.7 2.0

0.1 0.1 0.1 0.1 0.1 0.1 0.7 1.3 1.6

0.2 0.1 0.1 0.1 0.4 0.2 0.6 0.9 1.2

0.2 0.3 1.1 1.3 1.9

0.2 0.3 0.2 0.1 0.3 0.3 1.0 0.9 1.2

0.1 0.0 0.0 0.0 0.3 0.1 0.5 0.8 0.7

0.1 0.1 0.0 0.0 0.3 0.1 0.5 0.8 0.6

0.2 0.2 0.1 0.1 0.3 0.1 0.5 1.1 1.4

0.1 0.1 0.0 0.0 0.2 0.1 0.5 0.9 1.2

0.2 0.2 0.2 0.2 0.2 0.2 3.4 4.9 7.0

0.2 0.2 0.1 0.1 0.3 0.1 1.5 1.3 1.0

0.1 0.0 0.0 0.1 0.3 0.0 0.5 1.0 0.8

0.1 0.0 0.0 0.1 0.3 0.0 0.7 0.8 0.7

0.1 0.0 0.0 0.1 0.3 0.0 0.8 0.8 0.7

0.1 0.0 0.0 0.1 0.3 0.0 0.7 0.8 0.7

0.2 0.1 0.0 0.1 0.4 0.1 0.8 0.8 0.6

0.0 0.0 0.0 0.0 0.0 0.0 2.6 2.7 2.0
2010 2011 2011 2011 2011 2012 2012 2012 2012

4 1 2 3 4 1 2 3 4

3.8 5.0 5.2 5.8 3.3 2.7 4.2 3.8 2.9

1.3 2.1 1.7 1.1 1.1 1.3 1.4 0.9 1.1

0.6 1.1 1.2 0.6 0.6 0.9 0.7 0.4 0.6

1.0 1.3 0.7 0.5 0.7 0.9 0.6 0.6

0.7 1.0 1.2 0.7 0.6 0.7 0.8 0.4 0.5

0.7 1.1 1.3 0.4 0.7 1.0 1.2 0.5 0.6

1.1 0.7 1.4 1.6 1.0 0.8 1.4 1.8 0.7

1.2 0.8 1.5 2.1 1.3 0.9 1.7 2.5 1.3

1.2 0.9 1.9 2.2 1.4 1.1 1.8 2.5 1.4

0.8 0.8 1.4 1.4 1.0 0.8 1.6 1.5 0.8

0.7 0.7 1.3 1.4 1.0 0.7 1.3 1.4 0.7

0.6 0.7 1.3 1.5 0.9 0.7 1.4 1.4 0.7

1.1 1.0 1.7 2.1 1.4 1.1 1.7 2.3 1.2

1.0 0.7 1.6 1.7 1.1 0.9 1.4 2.0 1.1

0.8 0.7 1.5 1.7 1.0 0.8 1.7 1.9 0.9

1.0 0.7 1.4 1.7 1.1 0.9 1.5 1.7 0.9

1.2 1.0 2.1 3.2 1.4 1.1 2.1 3.0 1.4

1.3 0.7 1.9 2.2 1.5 0.9 1.8 2.3 1.3

1.3 1.0 2.0 2.5 1.6 1.1 1.9 2.7 1.4

1.2 1.1 1.8 2.4 1.5 1.1 1.8 2.7 1.5

2.8 3.6 4.1 4.2 2.4 2.5 4.1 3.4 2.7

2.7 3.8 4.3 4.2 2.6 2.8 5.0 3.4 2.8

0.5 0.5 1.1 1.1 0.7 0.4 1.3 1.3 0.5

0.7 0.5 1.4 1.6 0.7 0.5 1.5 1.8 0.7

0.9 0.7 1.7 1.7 1.0 0.7 1.6 2.2 0.7

0.8 0.7 2.5 2.4 1.0 0.6 2.0 2.0 0.9

0.7 0.6 1.4 1.6 0.9 0.6 1.5 2.0 0.8

1.8 0.9 0.6 1.8 2.1 0.7

1.2 1.0 1.8 2.0 1.4 0.9 1.7 1.6 0.9

0.6 0.5 1.4 1.7 0.8 0.6 1.6 1.8 0.7

0.6 0.5 1.1 0.9 0.7 0.5 1.1 1.2 0.5

1.3 0.7 2.5 3.5 1.4 0.9 2.9 3.0 1.2

1.0 0.8 1.6 2.4 1.2 0.7 1.6 1.9 0.8

0.9 0.7 1.5 2.3 1.1 0.7 1.6 2.9 0.8

0.8 0.6 1.5 2.0 0.8 0.6 1.8 2.4 0.7

1.0 0.8 1.6 2.4 1.3 0.8 1.9 2.1 0.9

0.6 0.5 1.1 0.9 0.6 0.4 1.1 0.9 0.5

0.6 0.5 1.0 1.0 0.6 0.5 1.1 0.8 0.5

0.6 0.5 1.0 1.0 0.5 0.4 1.2 0.9 0.6

1.2 0.9 2.4 3.2 1.4 0.9 2.5 2.5 1.1

Sulfates

SANDWICHed*
0.7 0.6 1.1 1.1 0.8 0.6 1.2 1.1 0.7

0.5 1.2 0.9

0.7 0.6 0.8 0.9 0.8 0.6 1.0 0.9 0.6

0.7 0.7 1.1 1.2 0.8 0.7 1.2 1.0 0.7

0.7 0.8 1.0 1.2 0.8 0.6 1.1 1.0 0.6

0.8 0.7 1.2 1.3 0.9 0.7 1.2 1.2 0.7

0.6 0.5 0.9 0.9 0.6 0.5 1.0 0.8 0.5

3.7 3.1 4.7 5.8 2.8 3.0 3.1 4.5 3.1

3.3 4.1 4.3 3.8 2.4 2.8 3.3 2.7 3.0

3.0 3.7 3.7 2.0 2.0 2.6 3.7 2.4 2.5

3.8 4.0 4.8 4.0 2.4 2.7 3.6 3.1 3.0

4.1 3.9 4.3 4.3 2.6 3.3 3.4 2.9 3.4

3.2 3.5 5.1 5.5 2.4 2.6 4.2 3.8 2.4

0.9 0.6 1.1 0.9 0.7

0.6 0.6 1.1 1.1 0.7 0.6 1.1 1.0 0.6

1.8 2.5 2.8 4.1 2.4 2.2 2.2 2.6 2.4

2.3 3.4 3.4 3.1 1.9 2.1 3.6 2.8 2.3

1.4 1.9 2.4 2.4 1.4 1.4 2.7 2.1 1.6

4.0 4.8 4.7 6.3 2.9 3.1 4.2 5.2 3.1

4.1 1.3

4.2 4.5 5.7 6.1 3.2 3.4 4.8 3.6 3.3

3.2

1.3 2.2 1.4 1.8 1.8 1.8 1.4 1.3 1.5

1.2 2.3 1.8 2.6 2.0 1.9 1.6 1.9 1.6

1.2 2.3 2.1 2.8 2.0 1.9 2.0 1.7 1.8

1.1 2.1 2.0 2.2 1.9 1.8 1.7 1.6 1.6

1.3 2.5 1.9 2.1 2.0 2.0 1.7 1.8 1.8

1.1 2.2 1.8 2.0 1.7 1.7 1.5 1.7 1.6

3.7 3.8 4.4 7.7 2.9 3.1 3.8 5.4 3.2

1.7 2.3 3.1 3.2 2.0 1.9 2.4 2.4 2.2

1.8 2.5 3.2 4.7 2.1 2.0 2.4 2.6 2.4

1.7 2.3 2.7 3.4 2.1 2.1 1.8 2.7 2.1

1.4 2.0 1.8 1.6 1.7 1.8 1.6 1.1 1.5

1.6 2.1 2.1 2.4 1.9 2.0 2.1 1.9 1.7

1.3 1.8 1.6 1.2 1.4 1.6 1.4 1.0 1.4

1.9 2.4 2.6 2.5 1.6 2.3 2.1 1.8 1.7

1.3 1.7 1.6 1.6 1.4 1.8 1.4 0.8 1.3

2.0 2.7 2.6 3.1 2.1 2.3 2.2 2.0 2.2

2.7 4.6 3.6 3.7 2.4 2.4 3.6 3.1 3.0

3.7 4.2 4.8 3.9 2.6 2.4 3.5 3.6 2.6

3.9

2.1 3.1 1.8 1.1 1.1 2.4 1.8

1.4 1.8 1.3 0.9 0.8 1.5 1.0 1.4 1.5

0.7 0.6 1.1 0.8 0.7 0.5 1.0 0.9 0.5
0.6 0.5 1.0 0.7 0.6 0.5 0.9 0.8 0.4

3.0 4.0 4.2 5.5 2.9 3.0 3.6 3.4 2.7

3.9

2.2 3.0 3.2 3.2 2.2 2.6 2.7 2.6 2.3

2.3 3.7 3.1 4.1 2.4 2.7 3.0 3.0 2.4

2.3 3.2 3.7

3.0 4.0 3.8 4.2 2.4 2.4 3.6 3.4 2.7

1.0 1.7 1.1 0.9 0.8 0.8 1.1 0.9 0.9

0.6 0.9 1.0 0.8 0.7 0.6 0.9 0.7 0.6

0.7 0.8 1.0 0.8 0.6 0.5 0.8 0.6 0.5

0.7 0.5 0.9 0.7 0.6 0.5 0.9 0.7 0.5

0.6 1.0 0.9 0.7 0.5 0.6 0.8 0.6 0.4

0.6 0.7 0.9 0.8 0.6 0.5 0.8 0.8 0.4

1.4 2.6 1.6 1.3 1.0 1.4 1.4 1.1 1.6

1.0 1.5 1.0 1.0 0.8 0.8 1.0 1.1 1.0

0.7 0.7 0.9 0.8 0.6 0.6 0.9 0.6 0.5

1.6 1.7 1.7 1.4 1.0 1.3 1.5 1.3 1.4

1.1 1.5 1.5 1.6 1.0 1.0 1.5 1.3 0.8

1.4 2.1 2.0 2.2 1.2 1.2 2.0 1.9 1.2

0.6 0.6 0.9 1.1 0.8 0.6 1.1 1.1 0.5

1.3 2.3 1.7 3.2 1.7 1.7 1.4 1.7 1.6

1.3 1.9 2.0 3.1 2.0 1.7 1.5 2.3 1.7

2.2 2.6 3.2 2.1 2.2 1.8 2.2 2.0

2.6 3.2 4.7 5.5 2.6 2.8 3.0 4.2 2.8

0.9 0.7 1.3 1.6 1.0 0.8 1.5 1.8 1.0

1.7 1.7 2.7 2.9 1.9 1.3 2.9 2.9 1.7

1.3 2.2 3.0 2.0 1.3 1.1 2.1 2.0 1.1

0.8 0.8 1.3 1.4 0.9 0.8 1.6 1.6 0.9

0.7 0.6 1.1 1.3 0.7 0.7 1.2 1.3 0.8

1.0 0.8 1.6 1.7 1.0 1.0 1.6 1.8 1.0

0.6 0.6 1.2 1.2 0.8 0.6 1.2 1.3 0.6

2.8 2.7 4.3 5.4 1.9 2.3 3.6 3.4 2.3

2.1 2.0 4.4 4.9 1.8 2.0 3.4 3.5 1.8

1.4 1.7 1.7 1.4 1.0 1.1 1.5 1.2 1.1

2.2 1.7 1.5 2.0 1.2 1.8 1.9 1.0 1.2

4.0 4.7 5.1 8.5 3.3 3.8 4.2 5.5 3.0

3.1 4.1 4.4 4.0 2.8 2.8 4.2 3.3 2.9

2.4 3.4 3.7 3.3 2.0 2.3 3.5 2.8 2.4

1.6 2.3 2.7 2.9 1.6 1.6 3.3 2.4 1.7

0.6 0.6 0.9 0.9 0.6 0.5 1.1 0.9 0.4

0.5 0.3 1.3 1.3 0.6 0.3 1.1 1.1 0.4

0.6 0.4 0.9 0.8 0.7 0.5 1.1 0.7 0.4
0.7 0.5 1.0 1.0 0.7 0.6 1.1 0.8 0.4

0.8 0.7 1.1 1.0 0.8 0.6 1.1 0.7 0.4

3.2

2.7

3.9 3.8 4.9 5.2 2.7 3.3 3.4 3.4 2.9

0.9 1.4 1.3 1.3 1.0 0.9 1.2 1.2 0.8

1.4 1.8 1.5 1.5 1.0 1.0 1.7 1.2 1.1

3.3 3.5 4.8 6.3 2.6 2.9 4.1 3.8 2.3

1.3 1.2 1.8 2.7 1.2 1.0 2.3 2.7 1.9

0.8 0.6 1.1 1.2 0.9 0.6 1.3 1.2 0.7

0.8 0.8 1.2 1.2 1.1 0.7 1.3 1.2 0.7

0.7 0.7 1.3 1.5 1.0 0.7 1.4 1.4 0.8

0.7 0.7 1.1 1.2 1.0 0.6 1.2 1.1 0.7

1.3 1.7 2.1 3.4 2.0 1.8 1.6 2.6

1.4 2.2 1.8 3.2 2.1 1.9 1.9 2.2 1.8

3.0 2.7 4.0 6.5 2.3 2.6 3.3 5.2 2.3

3.7 3.5 4.3 6.4 2.7 2.9 3.4 4.3 2.8

0.6 0.7 1.4 1.5 0.8 0.7 1.1 1.3 0.6

1.6

0.7 0.7 1.4 1.7 0.7 0.6 1.2 1.3 0.5

0.6 0.6 1.1 1.3 0.7 0.5 1.0 1.2 0.4

1.0 0.8 1.4 1.9 1.4

1.1 0.6 1.1 1.4 1.0 0.8 0.7 1.2 1.1

0.6 0.6 0.7 0.8 0.6 0.5 0.8 0.7 0.3

0.5 0.6 0.9 0.8 0.6 0.5 0.9 0.6 0.3

0.5 0.5 1.1 1.5 0.7 0.4 1.0 1.3 0.4

0.6 0.7 1.1 1.5 0.6 0.6 1.0 1.2 0.4

3.4 3.3 4.3 8.2 2.3 2.7 3.8 5.4 2.5

1.1 1.5 1.1 1.0 0.8 0.9 1.1 1.1 0.9

0.6 0.8 1.1 0.9 0.8 0.5 0.9 0.9 0.6

0.6 0.7 1.0 0.8 0.8 0.6 0.9 0.9 0.6

0.7 0.7 1.1 0.9 0.7 0.5 0.9 0.9 0.6

0.6 0.6 1.0 0.8 0.7 0.5 0.9 0.9 0.6

0.6 0.7 0.9 0.8 0.7 0.6 0.9 0.8 0.6

1.5 1.3 2.6 2.0 1.7 1.4 2.5 2.6 1.6
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

0.6 0.0 0.0 0.4 0.3 0.0 0.0 0.1 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.2 0.0 0.0 0.0 0.1 0.0 0.0 0.1 0.2

0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.1 0.0 0.0 0.1 0.1 0.0 0.0 0.1 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

1.1 0.0 0.0 0.7 1.1 0.0 0.0 0.3 0.1

0.7 0.0 0.0 0.4 0.6 0.0 0.0 0.4 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.2 0.2

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.1 0.0

0.9 0.0 0.0 0.2 0.4 0.0 0.0 0.3 0.6

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1 0.0

0.1 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.2 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.3 0.0 0.0 0.6 0.8 0.0 0.0 1.8 1.4

Nitrates

SANDWICHed*
0.1 0.0 0.0 0.0 0.1 0.0 0.0 0.1 0.1

0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.1 0.0 0.0 0.0 0.1 0.0 0.0 0.1 0.0

0.1 0.0 0.0 0.0 0.2 0.0 0.0 0.0 0.1

0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

1.4 0.1 0.0 1.0 1.4 0.1 0.0 0.3 0.6

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.3 0.0 0.0 0.2 0.1 0.0 0.0 0.0 0.0

0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.2 0.0 0.0 0.3 0.4 0.0 0.0 0.1 0.2

3.0 0.0 0.0 1.6 3.7 0.0 0.0 1.1 0.8

2.3 0.0 0.0 0.5 1.1 0.0 0.0 0.8 0.7

2.4 0.0 0.0 0.9 1.8 0.1 0.0 0.3 0.4

2.6 0.0 0.0 1.3 0.0

0.3 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.1 0.0 0.0 0.0

0.2 0.0 0.0 0.1 0.3 0.0 0.0 0.0 0.3

0.0 0.0 0.0 0.0 0.2 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.3 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.1 0.0 0.0 0.0 0.3 0.0 0.0 0.0 0.1

0.1 0.0 0.0 0.0 0.2 0.0 0.0 0.0 0.1

1.0 0.0 0.0 0.5 0.6 0.0 0.0 0.2 0.2

0.1 0.0 0.0 0.1 0.2 0.0 0.0 0.0 0.1

0.1 0.0 0.0 0.3 0.4 0.0 0.0 0.0 0.1

0.2 0.0 0.0 0.4 0.5 0.0 0.0 0.1 0.2

1.0 0.0 0.0 0.4 0.8 0.0 0.0 0.6 0.7

1.3 0.0 0.0 0.7 1.3 0.0 0.0 0.6 0.6

0.7 0.0 0.0 0.3 0.7 0.0 0.0 0.5 0.9

6.1 0.0 0.0 1.8 4.1 0.1 0.0 0.6 1.7

0.9 0.0 0.0 0.3 1.1 0.0 0.0 0.4 1.1

4.7 0.0 0.0 2.0 5.0 0.1 0.0 1.7 2.3

3.6 0.0 0.0 1.5 2.9 0.0 0.0 1.4 0.7

2.1 0.0 0.0 1.1 2.3 0.0 0.0 0.3 0.5

0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.2 0.0 0.0 0.2 0.5 0.0 0.0 0.8 0.2
0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

6.2 0.1 0.0 2.4 4.0 0.1 0.0 1.7 1.5

4.2 0.0 0.0 0.8

6.0 0.0 0.0 2.5 4.3 0.1 0.0 1.7 2.8

6.4 0.0 0.0 2.3 4.7 0.1 0.0 1.7 2.0

5.2 0.0 0.0 2.1 3.4 0.0

1.8 0.0 0.0 1.1 2.6 0.0 0.0 0.6 0.2

1.2 0.0 0.0 0.4 0.7 0.0 0.0 0.2 0.3

0.2 0.0 0.0 0.1 0.1 0.0 0.0 0.1 0.1

0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

2.4 0.0 0.0 0.7 1.8 0.0 0.0 0.3 1.0

0.6 0.0 0.0 0.1 0.2 0.0 0.0 0.0 0.2

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

1.7 0.0 0.0 1.0 1.2 0.0 0.0 0.4 0.9

1.8 0.0 0.0 0.5 1.0 0.1 0.0 0.3 0.5

2.5 0.0 0.0 0.8 1.3 0.1 0.0 0.8 0.7

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.1 0.2 0.0 0.0 0.0 0.2

0.5 0.0 0.0 0.1 0.4

1.3 0.0 0.0 0.6 1.2 0.0 0.0 0.1 0.4

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.4 0.0 0.0 0.3 0.1 0.0 0.0 0.8 0.3

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.2 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.5 0.0

0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

1.9 0.0 0.0 0.9 0.9 0.1 0.0 0.2 0.6

2.1 0.0 0.0 1.3 1.6 0.0 0.0 0.6 1.3

2.9 0.0 0.0 0.9 1.6 0.1 0.0 0.5 0.7

0.0 0.0 1.1 1.8 0.0 0.0 0.7 0.4

1.2 0.0 0.0 0.4 0.9 0.0 0.0 0.9 0.7

1.9 0.0 0.0 0.5 0.9 0.0 0.0 0.9 0.7

2.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0
0.1 0.0 0.0 0.1 0.2 0.0 0.0 0.1 0.1

0.1 0.0 0.0 0.1 0.8 0.0 0.0 0.2 0.0

1.3 0.0 0.0 1.2

1.7 0.0 0.0 1.1

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.9 0.0 0.0 0.2 0.6 0.0 0.0 0.0 0.2

0.7 0.0 0.0 0.2 0.6 0.0 0.0 0.1 0.2

0.3 0.0 0.0 0.1 0.1 0.0 0.0 0.0 0.1

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.2 0.0 0.0 0.0 0.0 0.0 0.0 0.3 0.1

0.7 0.0 0.0 0.0 0.3 0.0 0.0 0.1 0.0

0.1 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.3 0.0 0.0 0.0 0.0 0.0 0.0 0.1 0.0

0.1 0.0 0.0 0.1 0.2 0.0 0.0 0.0 0.3

0.6 0.0 0.0 0.1 0.9 0.0 0.0 0.1 0.3

0.8 0.0 0.0 0.1 0.4 0.0 0.0 0.1 0.1

0.7 0.0 0.0 0.3 0.8 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.1 0.0 0.0 0.3 0.3 0.0 0.0 0.0

0.9 0.0 0.0 1.1 0.6 0.0 0.0 0.3 0.3

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.6 0.0 0.0 0.2 0.4 0.0 0.0 0.2 0.1

0.5 0.0 0.0 0.1 0.5 0.0 0.0 0.1 0.5

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.1 0.0 0.0 0.0 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.2 0.0

0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0
2012 2012 2012 2010 2010 2010 2010 2011 2011

2 3 4 1 2 3 4 1 2

0.0 0.0 0.1 0.5 1.2 1.8 0.6 0.3 0.6

0.0 0.0 0.0 0.1 0.1 0.1 0.2 0.3 0.1

0.0 0.0 0.1 0.3 0.4 0.2 0.3 0.2 0.3

0.0 0.0 0.0 0.2 0.1

0.0 0.0 0.0 0.3 0.4 0.1 0.3 0.2 0.2

0.0 0.0 0.0 0.2 0.3 0.1 0.1 0.1 0.2

0.0 0.0 0.0 0.6 1.2 0.5 0.4 0.7 1.6

0.0 0.0 0.0 0.9 1.8 0.7 0.7 1.3 2.3

0.0 0.0 0.0 3.9 5.8 2.7 7.9 5.4 5.2

0.0 0.0 0.0 0.8 2.3 1.8 0.6 0.8 1.8

0.0 0.0 0.0 0.5 1.5 0.7 0.3 0.8 1.1

0.0 0.0 0.0 0.8 3.9 4.7 1.6 1.3 4.5

0.0 0.0 0.0 0.6 2.5 1.0 0.8 1.2 2.2

0.0 0.0 0.0 0.5 1.6 0.7 0.6 0.7 2.0

0.0 0.0 0.0 0.7 1.6 1.8 0.7 0.8 1.9

0.0 0.0 0.0 0.6 2.5 1.0 0.6 0.7 2.0

0.0 0.0 0.0 1.2 1.8 1.3 1.2 1.6 2.9

0.0 0.0 0.0 1.1 2.4 1.2 1.4 1.2 2.7

0.0 0.0 0.0 2.2 3.0 1.7 2.0 2.2 3.0

0.0 0.0 0.0 0.8 2.0 1.2 1.1 1.4 2.6

0.0 0.0 0.0 0.5 1.5 2.3 0.6 0.3 1.4

0.0 0.0 0.3 0.5 1.2 3.2 0.6 0.3 0.8

0.0 0.0 0.0 0.9 0.8 0.6 0.2 0.4 0.5

0.0 0.0 0.0 1.5 1.0 1.1 0.2 0.4 0.5

0.0 0.0 0.0 1.0 1.8 1.5 0.6 1.2 1.4

0.0 0.0 0.0 0.8 1.1 1.9 0.4 0.4 1.1

0.0 0.0 0.0 1.5 1.3 1.0 0.6 1.5 0.9

0.0 0.0 0.0

0.0 0.0 0.0 0.3 0.4 0.2 0.2 0.2 0.2

0.0 0.0 0.0 0.9 0.8 1.0 0.2 0.3 0.6

0.0 0.0 0.0 1.0 0.9 1.0 0.3 0.6 0.6

0.0 0.0 0.0 0.5 0.9 0.9 0.4 0.3 1.0

0.0 0.0 0.0 0.4 0.6 0.6 0.3 0.3 0.4

0.0 0.0 0.0 0.8 1.3 1.1 0.5 0.7 1.0

0.0 0.0 0.0 0.9 1.0 0.8 0.3 0.5 0.7

0.0 0.0 0.0 0.7 1.3 1.2 0.3 0.5 0.9

0.0 0.0 0.0 0.7 0.8 1.1 0.3 0.3 0.4

0.0 0.0 0.0 0.6 0.6 0.7 0.3 0.2 0.4

0.0 0.0 0.1 0.5 0.6 0.7 0.3 0.2 0.3

0.0 0.0 0.1 0.6 0.9 1.8 0.3 0.3 0.7

Crustal

SANDWICHed*
0.0 0.0 0.1 0.7 3.1 1.3 1.0 0.9 2.9

0.4 1.5

0.0 0.0 0.0 0.4 1.6 0.7 0.3 0.4 1.0

0.0 0.0 0.0 0.6 5.5 1.8 0.9 0.7 2.8

0.0 0.0 0.0 0.6 1.5 0.7 0.3 0.6 1.1

0.0 0.0 0.0 0.6 4.5 1.1 0.4 0.8 2.0

0.0 0.0 0.0 0.6 2.3 0.7 0.4 0.6 1.3

0.0 0.0 0.9 0.8 1.4 0.9 0.6 0.4 0.8

0.0 0.0 0.0 0.4 1.8 2.1 0.5 0.4 0.6

0.0 0.0 0.0 0.4 2.0 2.1 0.3 0.3 0.7

0.0 0.0 0.0 0.4 1.2 2.0 0.5 0.3 0.6

0.0 0.0 0.0 0.5 1.2 1.8 0.6 0.3 0.8

0.0 0.0 0.0 0.4 1.4 1.2 0.4 0.2 0.7

0.0 0.0 0.0

0.0 0.0 0.0 0.9 3.5 0.6 0.3 0.7 1.6

0.0 0.0 0.3 0.3 0.9 0.4 0.2 0.2 0.3

0.0 0.0 1.6 0.5 1.1 1.4 0.8 0.4 1.0

0.1 0.0 0.6 0.4 1.3 1.5 1.1 0.5 1.2

0.0 0.0 0.4 0.5 1.1 1.0 0.5 0.2 0.6

0.5 1.2 1.4 0.6 0.3

0.0 0.0 0.0 0.5 2.0 2.6 0.6 0.3 0.8

0.4 1.5 2.6 0.5

0.0 0.0 0.1 0.9 0.8 0.4 0.3 0.4 0.3

0.0 0.0 0.1 0.2 0.6 0.3 0.1 0.1 0.2

0.0 0.0 0.2 0.2 0.7 0.4 0.1 0.1 0.2

0.0 0.0 0.0 0.2 0.5 0.3 0.1 0.1 0.2

0.0 0.0 0.1 0.5 0.7 0.4 0.2 0.3 0.2

0.0 0.0 0.0 0.3 0.4 0.3 0.1 0.1 0.1

0.0 0.0 0.4 0.5 0.9 0.8 0.5 0.2 0.4

0.0 0.0 0.1 0.2 0.6 0.4 0.2 0.1 0.2

0.0 0.0 0.2 0.3 0.6 0.5 0.2 0.2 0.2

0.0 0.0 0.2 0.3 0.8 0.4 0.2 0.2 0.3

0.0 0.0 0.5 0.3 0.5 0.3 0.4 0.1 0.2

0.1 0.0 0.6 0.3 0.6 0.3 0.3 0.1 0.2

0.0 0.0 0.5 0.3 0.6 0.3 0.4 0.1 0.2

0.1 0.0 2.4 0.5 1.2 0.9 1.8 0.2 0.6

0.0 0.0 0.9 0.4 0.7 0.3 0.5 0.1 0.2

0.0 0.0 2.8 0.4 0.9 0.5 0.8 0.2 0.3

0.0 0.0 1.5 0.5 1.3 1.7 0.9 0.3 0.9

0.0 0.0 0.4 1.2 2.2 1.6 2.4 0.3 1.3

0.8 0.4 0.1 0.2

0.0 0.3 0.5 0.2 0.1 0.2 0.3

0.0 0.0 0.0 0.4 0.9 0.2 0.1 0.3 0.3

0.0 0.0 0.1 0.5 1.1 1.3 0.5 0.3 0.6
0.0 0.0 0.0 0.6 1.0 0.9 0.3 0.5 0.5

0.0 0.0 2.3 0.4 0.9 0.8 0.7 0.2 0.5

0.5 1.0 1.0 0.7

0.0 0.0 2.7 0.5 0.9 1.0 1.1 0.3 0.6

0.1 0.0 2.5 0.5 0.9 0.8 0.9 0.3 0.5

0.5 1.2 1.3 1.3 0.3 0.8

0.0 0.0 0.7 0.5 1.3 1.5 0.7 0.2 0.8

0.0 0.0 0.3 0.4 0.9 0.8 0.5 0.2 0.3

0.0 0.0 0.1 0.5 0.8 1.2 0.2 0.1 0.3

0.0 0.0 0.0 0.4 0.6 1.0 0.2 0.2 0.3

0.0 0.0 0.0 0.5 0.9 1.1 0.4 0.3 0.4

0.0 0.0 0.0 0.9 1.2 1.7 0.3 0.1 0.3

0.0 0.0 0.0 0.4 0.7 1.1 0.2 0.3 0.4

0.0 0.0 1.1 0.5 1.2 1.0 1.2 0.3 0.4

0.0 0.0 0.3 0.5 0.7 0.9 0.7 0.6 0.5

0.0 0.0 0.0 0.6 0.7 0.9 0.3 0.3 0.3

0.0 0.0 1.0 0.4 0.9 0.9 0.7 0.2 0.5

0.0 0.0 0.1 0.5 0.9 1.2 0.7 0.4 0.6

0.0 0.0 0.7 0.3 0.9 0.8 0.7 0.3 0.7

0.0 0.0 0.0 1.1 1.2 1.1 0.2 0.5 0.7

0.0 0.0 0.0 0.0 0.5 0.3 0.2 0.1 0.2

0.0 0.0 0.1 0.2 0.7 0.4 0.2 0.1 0.3

0.0 0.0 0.3 0.2 0.3

0.0 0.0 0.5 0.4 0.8 0.8 0.4 0.2 0.4

0.0 0.0 0.0 0.7 1.6 0.6 0.5 0.8 1.8

0.0 0.0 0.0 0.7 2.7 1.4 1.2 1.7 4.8

0.0 0.0 0.0 0.6 2.8 0.9 0.7 1.4 3.1

0.0 0.0 0.0 0.5 1.6 0.6 0.5 0.7 1.8

0.0 0.0 0.0 0.8 2.1 0.8 0.4 0.7 2.0

0.0 0.0 0.0 0.7 1.7 0.8 0.8 0.9 2.9

0.0 0.0 0.0 0.6 1.8 0.6 0.3 0.7 1.3

0.4 0.9

0.0 0.0 0.0 0.5 1.1 1.0 0.3 0.2 0.5

0.0 0.0 0.0 0.4 1.6 0.6 0.4 0.2 0.7

0.0 0.0 0.6 0.5 0.9 1.2 0.9 0.2 0.4

0.0 0.0 0.7 0.5 1.2 1.1 0.8 0.2 0.5

0.0 0.0 0.9 0.5 1.0 0.7 0.6 0.3 0.5

0.0 0.0 0.6 1.3 2.0 0.6 0.3 0.8

0.0 0.0 0.6 0.8 1.2 1.9 0.8 0.5 1.7

0.0 0.0 0.4 0.5 1.4 1.3 1.1 0.5 2.0

0.6 2.0

0.0 0.0 0.0 0.4 0.5 0.4 0.2 0.1 0.1

0.0 0.0 0.0 0.2 0.3 0.3 0.1 0.1 0.2

0.0 0.0 0.0 0.8 0.8 0.8 0.4 0.3 0.3
0.0 0.0 0.0 0.5 0.7 0.9 0.2 0.2 0.3

0.0 0.0 0.1 0.4 0.8 0.9 0.3 0.2 0.4

0.5 0.8 0.7 0.4

0.5 0.9 0.6 0.5

0.0 0.0 0.0 0.4 0.8 1.6 0.5 0.2 0.5

0.0 0.0 0.2 0.4 0.9 1.1 0.5 0.3 0.5

0.0 0.0 0.3 0.5 0.8 0.9 0.8 0.3 0.6

0.0 0.0 0.0 0.4 1.2 1.1 0.4 0.2 0.6

0.0 0.0 0.0 1.2 2.4 0.9 1.9 2.7 5.0

0.0 0.0 0.0 0.6 1.1 0.8 0.4 0.7 1.0

0.0 0.0 0.1 0.4 2.0 0.8 0.4 0.6 1.3

0.0 0.0 0.0 0.6 1.4 1.3 0.5 0.7 1.2

0.0 0.0 0.0 0.5 1.4 1.0 0.3 0.6 1.1

0.0 0.0 0.3 0.7 0.4 0.2 0.1 0.2

0.0 0.0 0.2 0.3 0.6 0.3 0.2 0.1 0.2

0.0 0.0 0.1 0.4 1.0 0.8 0.3 0.2 0.4

0.0 0.0 0.2 0.5 1.1 0.9 0.4 0.2 0.4

0.0 0.0 0.0 0.1 0.1 0.1

0.4 0.3 0.7 0.2

0.0 0.0 0.0 0.4 0.3 0.2 0.1 0.1 0.1

0.0 0.0 0.0 0.5 0.4 0.3 0.1 0.1 0.1

0.4 0.4 0.5 0.2 0.1 0.2

0.0 0.0 0.4 0.6 1.7 1.8 0.4 0.3 1.0

0.0 0.0 0.0 0.6 0.5 0.2 0.2 0.1 0.1

0.0 0.0 0.0 0.5 0.6 0.3 0.2 0.1 0.2

0.0 0.0 0.0 0.4 0.4 0.3 0.1 0.1 0.2

0.0 0.0 0.0 0.5 0.3 0.2 0.1 0.1 0.1

0.0 0.0 0.2 0.5 1.1 1.0 0.4 0.2 0.5

0.0 0.0 0.2 0.9 0.9 2.0 1.2 0.4 0.6

0.0 0.0 0.0 0.7 0.8 0.6 0.3 0.6 0.8

0.0 0.0 0.0 0.5 1.1 1.4 0.3 0.6 0.7

0.0 0.0 0.0 0.9 1.2 0.9 0.3 0.6 0.8

0.0 0.0 0.0 0.8 1.2 0.9 0.5 0.6 0.7

0.0 0.0 0.0 0.4 0.9 1.2 0.3 0.4 0.5

0.0 0.0 0.0 1.7 5.9 5.7 0.6 0.2 2.6
2011 2011 2012 2012 2012 2012 2010 2010 2010

3 4 1 2 3 4 1 2 3

0.5 0.3 0.4 0.5 1.1 0.4 1.3 3.3 2.9

0.1 0.1 0.1 0.2 0.1 0.1 0.7 0.6 0.7

0.1 0.1 0.1 0.4 0.3 0.1 0.2 0.7 0.9

0.0 0.2 0.1 0.1 0.0 0.2

0.1 0.1 0.1 0.3 0.0 0.5 0.0 0.4 1.3

0.0 0.1 0.1 0.2 0.0 0.1 0.4 1.5 3.1

0.7 0.5 0.9 1.8 0.7 0.5 0.2 0.5 0.8

1.2 0.7 1.3 2.1 0.9 0.8 0.2 0.3 0.5

2.5 2.9 5.6 5.5 3.0 5.0 1.3 0.7 0.8

1.1 0.6 1.0 2.8 1.1 0.9 0.2 0.6 1.0

0.8 0.4 1.0 1.9 0.8 0.5 0.1 0.4 1.9

3.2 1.3 2.2 6.3 5.3 3.3 0.5 0.4 0.9

2.2 0.7 1.5 3.3 1.2 0.8 0.5 0.8 1.0

1.1 0.4 0.9 2.8 0.9 0.8 0.7 0.8 0.7

1.6 0.8 1.1 2.6 1.2 0.9 0.2 0.6 0.8

1.0 0.5 1.2 2.3 1.0 1.0 0.5 0.7 1.2

2.7 0.9 1.8 2.4 1.2 1.2 0.4 0.7 0.2

1.8 1.2 1.6 2.8 1.5 1.4 0.4 0.7 0.6

3.0 1.8 4.1 4.9 2.7 2.9 0.8 0.6 0.4

3.6 0.8 2.1 3.3 1.4 1.4 0.4 0.7 0.5

0.9 0.3 0.5 1.0 2.0 0.7 1.6 2.1 2.3

0.9 0.3 0.6 0.8 2.6 0.5 1.2 2.1 2.5

0.3 0.2 0.3 1.0 0.5 0.4 0.5 0.5 1.2

0.6 0.4 0.5 1.4 1.1 0.5 0.1 1.1 2.8

1.1 0.8 1.6 2.4 2.2 1.1 0.2 0.6 1.2

1.1 0.5 0.5 1.8 1.6 0.9 0.8 1.8 4.7

1.1 1.1 1.2 1.7 1.1 0.7 0.6 0.6 0.8

0.4 0.4 0.6 1.5 0.6 0.4

0.1 0.2 0.2 0.3 0.1 0.2 2.3 3.0 2.0

0.6 0.4 0.4 1.2 1.1 0.4 0.2 0.9 2.5

0.5 0.4 0.4 1.3 0.9 0.4 0.0 0.3 1.5

0.6 0.6 0.6 0.8 0.7 0.5 1.4 2.2 2.2

0.5 0.4 0.3 0.7 0.5 0.3 1.5 1.9 1.7

0.9 0.7 1.0 1.8 1.4 0.6 0.8 1.5 1.4

0.6 0.3 0.7 1.4 0.7 0.4 1.1 2.5 1.9

0.9 0.6 0.5 1.4 0.7 0.4 1.0 1.8 2.1

0.5 0.2 0.2 0.8 0.7 0.4 0.2 0.5 2.7

0.6 0.2 0.3 0.8 0.7 0.7 0.3 0.4 1.7

0.5 0.1 0.2 0.7 0.6 0.4 0.6 0.5 1.6

1.3 0.5 0.4 1.3 1.9 0.7 1.1 2.8 5.3

Crustal

SANDWICHed*
0.8 0.6 1.1 2.5 0.8 1.0 0.3 0.4 0.9

0.7

0.4 0.3 0.6 1.2 0.5 0.3 0.0 0.4 0.8

1.1 0.8 0.8 3.4 1.5 2.1 0.1 0.2 0.7

0.6 0.4 0.7 1.7 0.6 0.4 0.3 0.5 1.3

0.9 0.6 1.1 2.9 0.8 0.8 0.2 0.2 0.7

0.7 0.4 0.8 2.0 0.4 0.4 0.0 0.2 0.6

0.5 0.6 0.6 0.6 0.6 0.5 2.4 2.8 2.2

0.9 0.2 0.3 0.6 1.9 0.4 2.3 2.1 1.4

1.5 0.2 0.2 1.6 4.1 0.2 1.4 1.1 1.1

0.7 0.2 0.2 0.6 1.9 0.4 2.2 2.3 2.1

0.9 0.2 0.3 0.6 1.5 0.3 2.2 2.6 1.9

0.3 0.2 0.3 0.5 1.3 0.3 0.9 2.8 2.9

0.4 0.9 1.6 0.7 0.5

0.5 0.5 0.9 2.3 0.5 0.5 0.1 0.3 0.8

0.2 0.2 0.2 0.3 0.2 0.2 0.9 2.2 2.1

1.2 0.5 0.8 1.2 1.9 1.0 0.6 2.5 1.9

1.3 0.6 1.1 1.8 2.6 2.1 0.7 1.3 1.6

0.4 0.3 0.4 0.5 1.0 0.4 0.8 2.3 2.8

1.8 3.3 3.3

1.2 0.2 0.3 0.9 3.5 0.5 2.0 2.1 1.6

1.7 2.8 3.4

0.2 0.3 0.5 0.4 0.3 0.3 1.0 3.1 2.3

0.1 0.1 0.2 0.3 0.1 0.1 0.7 2.0 2.3

0.2 0.1 0.1 0.2 0.1 0.2 1.3 2.5 2.3

0.1 0.1 0.2 0.2 0.2 0.1 0.4 1.8 1.9

0.2 0.2 0.4 0.3 0.2 0.2 1.3 2.4 2.1

0.1 0.1 0.2 0.2 0.1 0.1 0.3 1.9 1.6

0.3 0.2 0.3 0.5 0.5 0.2 0.9 1.4 1.6

0.1 0.2 0.2 0.3 0.2 0.2 1.5 1.8 2.3

0.3 0.2 0.2 0.3 0.2 0.2 1.7 2.9 2.3

0.2 0.2 0.2 0.3 0.2 0.2 1.0 2.2 2.2

0.2 0.2 0.2 0.4 0.3 0.1 0.5 1.5 2.3

0.2 0.2 0.2 0.4 0.3 0.1 0.5 2.1 1.9

0.2 0.3 0.2 0.5 0.4 0.2 0.4 1.0 2.7

0.9 1.3 0.4 1.2 2.1 1.2 1.2 1.3 1.6

0.3 0.3 0.2 0.5 0.4 0.2 0.5 1.0 2.7

0.5 0.5 0.3 0.8 1.0 0.4 1.3 1.6 2.3

1.6 0.7 0.7 1.5 2.9 1.7 1.4 1.9 2.2

1.2 0.9 0.8 1.9 1.6 1.0 2.5 2.2 3.2

0.6 0.3 0.1

0.1 0.1 0.2 0.6 0.3 0.7 0.7

0.1 0.1 0.5 0.4 0.1 0.1 0.0 0.1 0.1

0.9 0.3 0.8 1.1 0.9 0.5 0.1 0.2 1.2
0.5 0.2 0.4 0.9 0.9 0.3 0.3 0.4 2.0

0.6 0.4 0.3 0.6 1.0 0.4 1.5 2.0 2.4

2.0 2.4 3.1

0.9 0.8 0.6 1.1 1.8 0.9 1.7 2.1 2.3

0.7 0.5 0.3 0.8 1.5 0.5 1.9 2.1 2.3

1.2 2.0 2.2

0.9 0.3 0.5 0.8 1.6 0.6 1.6 2.1 2.3

0.9 0.4 0.4 1.3 1.9 0.3 0.3 0.5 1.6

1.1 0.2 0.2 0.5 1.4 0.1 1.5 0.9 2.5

0.7 0.1 0.2 0.5 1.1 0.2 0.4 0.6 2.0

0.6 0.2 0.4 0.8 0.7 0.2 0.1 0.2 1.4

1.1 0.1 0.3 0.6 3.7 1.2 0.4 0.4 1.8

0.5 0.1 0.3 0.6 0.6 0.3 0.2 0.4 1.9

1.1 0.6 0.5 0.9 1.5 0.2 0.0 0.6 2.5

0.8 0.3 0.4 1.0 1.4 0.3 0.1 0.5 1.4

0.8 0.2 0.2 0.6 0.9 0.3 0.3 0.6 2.0

1.3 0.8 0.7 1.3 2.4 0.3 0.1 0.8 2.4

0.8 0.8 0.6 1.0 1.3 1.1 0.3 0.9 1.7

0.9 0.7 0.8 2.1 2.1 1.1 0.3 1.1 1.8

0.8 0.4 0.8 1.6 0.6 0.4 0.0 0.2 0.6

0.1 0.1 0.2 0.3 0.1 0.1 0.0 1.5 2.2

0.2 0.2 0.2 0.3 0.2 0.2 0.5 1.8 1.9

0.2 0.2 0.2 0.3 0.4 0.2

0.3 0.3 0.2 0.5 0.4 0.2 1.6 2.1 2.2

0.7 0.7 1.5 2.6 0.7 0.6 0.1 0.7 1.1

1.9 1.0 1.4 2.3 2.0 1.8 0.8 0.5 0.8

1.2 0.7 1.7 2.2 1.0 0.9 0.1 0.5 0.8

0.7 0.4 0.9 1.7 0.8 0.8 0.3 0.5 0.9

0.9 0.9 1.1 2.1 0.8 0.9 0.1 0.3 0.8

1.3 0.7 1.5 2.2 1.4 1.5 0.4 0.3 0.5

0.6 0.4 0.7 1.7 0.6 0.6 0.0 0.7 0.7

0.8 1.6

0.2 0.2 0.3 0.5 0.7 0.2 1.1 2.7 3.2

0.3 0.4 0.3 0.4 0.6 0.2 0.8 2.3 2.9

1.2 0.9 0.5 1.1 1.7 0.4 0.1 0.8 1.9

1.5 0.7 0.8 1.2 2.8 0.7 0.0 1.0 2.7

0.4 0.3 0.3 0.7 0.6 0.4 1.1 1.7 2.1

1.1 0.4 0.5 0.9 2.4 0.9 2.4 2.4

1.6 0.4 1.2 1.3 2.6 0.7 1.1 1.9 2.0

2.0 0.6 0.7 1.4 2.5 1.2 0.8 1.1 1.5

0.9 3.5

0.4 0.1 0.2 0.6 0.8 1.5 0.2 0.3 1.6

0.3 0.1 0.1 0.3 0.3 0.1 1.3 1.4 2.4

0.4 0.2 0.3 0.8 0.5 0.7 0.2 0.3 1.4
1.3 0.2 0.3 0.6 1.3 0.6 0.3 0.4 1.9

0.8 0.3 0.4 0.9 1.4 0.5 0.6 0.4 2.0

1.3 2.5 2.6

1.7 2.2 3.1

0.8 0.2 0.3 0.5 1.2 0.3 2.4 2.5 1.9

0.8 0.3 0.6 1.3 1.3 0.5 0.2 0.4 1.3

0.7 0.6 0.5 1.0 1.3 0.8 0.1 0.6 1.6

0.3 0.2 0.4 0.5 0.8 0.2 0.9 3.0 3.3

1.9 1.2 2.6 2.3 1.8 1.7 0.5 0.5 0.3

0.6 0.3 0.9 1.6 0.7 0.4 0.1 0.4 1.0

0.7 0.4 1.0 2.1 0.8 0.6 0.1 0.3 0.9

1.0 0.5 1.0 2.0 0.8 0.7 0.2 0.6 1.2

0.6 0.4 1.0 1.7 0.6 0.5 0.4 0.2 0.8

0.1 0.2 0.2 0.3 0.2 0.5 1.7 1.8

0.1 0.1 0.2 0.3 0.1 0.2 0.7 1.9 2.3

0.3 0.2 0.2 0.4 0.5 0.2 0.6 2.1 2.8

0.3 0.3 0.4 0.5 0.6 0.3 2.3 2.2 2.9

0.1 0.0 0.1 0.2 0.1 0.1

3.0 1.9 1.6

0.1 0.1 0.1 0.2 0.1 0.1 0.7 0.8 1.4

0.2 0.1 0.2 0.3 0.3 0.1 0.4 0.5 1.9

0.4 0.2 1.0 1.1 1.8

1.8 0.5 0.1 0.3 1.7 0.6 0.9 0.7 2.3

0.2 0.1 0.3 0.5 0.4 0.2 0.2 0.2 1.5

0.4 0.1 0.2 0.5 0.4 0.2 0.3 0.4 2.1

0.3 0.1 0.1 0.3 0.3 0.1 0.5 0.9 1.9

0.2 0.0 0.1 0.3 0.2 0.1 0.1 0.5 2.5

0.3 0.2 0.3 0.6 0.5 0.2 1.2 1.5 1.9

1.4 1.0 0.7 1.6 2.7 0.8 0.6 0.2 1.2

0.6 0.3 0.8 1.0 0.7 0.3 0.1 0.4 1.4

0.6 0.2 0.5 1.0 1.3 0.4 0.1 0.2 1.2

0.5 0.2 0.6 1.4 0.6 0.4 0.1 0.2 1.1

0.5 0.3 0.6 1.3 0.7 0.4 0.1 0.2 0.9

0.4 0.2 0.6 0.9 0.6 0.3 0.1 0.2 1.5

3.1 1.4 0.7 4.6 6.1 0.5 1.0 0.9 1.3
2010 2011 2011 2011 2011 2012 2012 2012 2012

4 1 2 3 4 1 2 3 4

2.6 2.8 4.8 3.8 2.6 2.5 3.4 3.1 2.6

1.4 1.4 1.4 1.0 1.9 1.4 0.9 1.2 1.4

0.1 0.2 0.7 0.3 0.0 0.4 0.4 0.5 0.1

0.1 0.9 1.1 0.4 0.3 0.9 1.0 0.4

0.2 0.1 0.6 0.7 0.2 0.2 0.6 0.8 0.1

0.1 0.3 0.8 0.6 0.3 0.2 0.6 0.6 0.0

0.4 0.5 1.0 1.2 0.3 0.9 1.2 1.4 0.8

0.5 0.4 2.4 1.0 0.3 0.3 1.1 1.1 0.2

1.1 2.8 2.8 1.4 2.5 2.6 2.0 1.5 2.1

0.5 0.4 1.1 1.8 1.1 0.3 1.6 1.5 1.2

0.4 0.2 0.7 2.4 0.2 0.2 1.0 1.1 0.4

1.5 0.6 1.2 2.0 1.5 0.7 2.1 1.6 1.2

0.9 0.8 1.0 1.6 0.6 0.6 1.3 1.5 1.3

1.7 0.8 0.9 3.2 0.6 0.6 1.9 1.5 0.9

0.3 0.3 1.1 1.2 0.7 0.4 1.1 1.0 0.4

1.0 0.7 1.1 1.2 0.4 0.4 1.5 1.7 0.5

0.4 1.0 1.2 0.8 0.6 0.7 1.2 0.5 0.5

0.5 1.1 1.5 0.9 1.2 0.8 1.4 1.1 0.6

0.6 1.4 1.4 1.3 1.0 1.6 1.6 0.9 0.7

0.6 1.0 1.3 1.7 0.7 1.0 1.4 1.1 0.7

2.6 2.6 3.8 3.9 2.2 2.5 2.8 2.5 2.5

2.4 2.4 3.4 3.4 2.0 1.7 2.9 2.4 2.6

0.9 0.3 1.0 2.7 1.0 0.9 1.1 2.2 0.8

0.6 0.2 1.2 3.0 0.8 0.1 1.7 1.7 0.8

0.3 0.5 1.0 1.4 0.4 0.5 1.1 1.5 0.4

1.5 1.2 2.4 3.5 1.4 1.2 2.7 2.6 1.1

0.3 0.9 1.1 1.4 1.1 0.8 1.3 3.3 1.7

0.8 0.7 0.6 1.6 1.4 0.5

2.5 2.8 3.0 2.4 3.1 3.0 3.2 2.9 2.3

0.8 0.4 1.4 4.2 1.3 0.7 1.9 2.6 1.0

0.3 0.1 0.5 1.9 0.2 0.3 0.9 1.5 0.1

1.8 1.2 2.9 2.7 1.8 1.4 3.3 2.0 1.2

1.8 1.5 2.7 1.7 2.0 1.7 2.3 2.0 1.5

0.7 0.6 1.1 1.8 0.7 0.8 1.5 1.4 0.6

1.0 0.8 2.2 2.5 0.7 1.2 2.0 2.0 0.6

1.1 0.7 2.2 2.3 1.1 0.7 2.1 1.9 0.8

0.4 0.1 1.0 2.1 1.4 0.7 0.7 6.1 0.6

1.0 0.6 0.6 2.3 1.3 0.4 0.8 8.1 0.9

1.0 0.4 0.7 2.6 3.0 0.9 0.8 5.8 1.1

2.5 1.6 3.3 5.3 2.7 2.1 3.8 3.7 2.6

Organic Carbon

SANDWICHed*
0.4 0.3 2.0 1.4 0.5 0.3 1.1 2.2 0.5

0.0 0.9 1.0

0.4 0.1 0.6 1.0 0.2 0.1 1.0 4.0 0.9

0.4 0.5 1.2 1.3 0.5 0.3 2.6 2.3 0.3

0.3 0.2 1.1 1.4 0.2 0.2 1.7 3.5 0.4

0.4 0.3 0.8 1.0 0.3 0.3 1.0 2.0 0.3

0.3 0.1 1.0 0.9 0.1 0.1 0.6 2.6 0.3

2.4 2.2 3.9 3.4 3.2 2.8 2.2 2.7 4.2

2.5 3.3 2.2 2.9 2.7 3.0 2.9 1.7 3.2

1.3 1.6 3.7 2.3 2.1 1.8 1.5 2.1 2.1

3.5 4.4 3.1 3.3 2.4 2.5 2.1 1.8 2.7

2.9 4.0 5.4 4.8 2.5 3.4 2.7 2.3 2.5

2.1 2.7 5.1 3.1 1.7 1.9 2.8 2.6 2.2

0.1 0.2 1.1 3.4 0.3

0.4 0.2 0.6 1.2 0.2 0.2 1.4 2.3 0.3

0.8 1.0 1.9 3.3 1.1 1.4 1.7 2.4 1.4

1.2 1.8 4.1 2.7 1.5 1.8 2.6 2.3 1.8

1.0 1.0 2.3 2.1 0.8 0.7 1.9 2.5 1.4

1.8 1.4 3.6 3.8 1.9 1.8 2.7 3.1 2.2

2.7 0.9

2.8 2.4 2.9 2.5 2.4 2.0 2.4 1.3 3.1

3.5

1.0 1.5 1.5 3.0 1.5 1.9 1.4 2.2 2.2

1.0 1.2 1.5 3.4 1.3 1.9 1.5 2.5 1.6

1.5 2.0 1.8 4.6 2.4 2.4 2.3 2.8 2.7

0.9 1.1 1.4 2.8 1.2 1.4 1.4 2.2 1.5

1.9 2.4 1.5 2.7 2.5 2.9 1.5 1.9 2.8

0.7 0.7 1.5 2.4 1.4 1.1 1.0 1.7 1.5

1.0 1.2 2.6 2.2 1.3 1.3 1.8 1.8 1.4

2.0 2.1 2.2 3.2 2.1 2.2 2.7 2.5 1.7

2.4 2.5 2.8 3.9 2.2 2.6 2.3 2.9 1.7

1.3 1.4 1.6 3.1 1.4 1.7 1.4 2.2 1.5

0.6 0.5 1.9 3.6 0.9 0.6 1.4 2.7 0.6

0.6 0.3 1.6 2.6 0.9 0.6 1.2 2.3 0.6

0.7 0.3 1.6 4.3 1.7 0.3 1.1 2.7 1.3

2.1 1.7 2.4 2.1 2.3 1.8 1.7 3.0 2.7

1.3 0.6 1.1 2.5 1.4 0.6 1.1 2.9 0.8

1.6 1.4 2.0 2.7 1.6 1.4 1.7 2.6 1.3

1.9 2.7 3.0 3.0 2.2 2.4 2.8 2.7 2.4

4.2 2.3 3.7 3.6 3.5 2.8 2.9 2.9 3.2

0.1

0.4 0.5 1.0 1.0 0.7 0.5 1.0

0.1 0.3 0.2 0.1 0.0 0.1 0.2 0.1 0.1

0.5 0.1 0.3 2.6 0.7 0.3 0.6 12.2 1.0
0.9 0.3 0.5 3.4 0.8 0.5 0.6 15.2 2.4

2.3 2.2 3.4 3.2 2.2 2.2 2.4 3.1 2.9

2.6

1.4 1.9 2.8 3.0 2.2 2.3 2.4 3.0 2.5

2.0 2.2 3.3 3.2 2.2 1.9 2.4 2.9 1.9

2.2 2.1 3.2

1.9 1.6 3.4 3.1 2.0 2.9 2.5 2.5 2.3

0.6 0.3 0.7 1.9 0.8 0.2 0.9 4.2 0.5

2.0 1.0 1.3 3.4 2.6 1.0 1.4 5.5 2.5

1.4 0.2 0.7 2.8 1.6 0.3 1.0 6.0 1.4

0.8 0.0 0.3 2.1 0.6 0.1 0.5 8.0 0.7

2.5 0.2 0.5 3.2 1.9 0.3 0.8 7.7 3.1

0.7 0.1 0.4 6.3 0.6 0.1 0.8 25.7 3.4

0.7 0.2 1.0 1.7 1.0 0.1 1.1 2.7 0.2

0.5 0.3 0.6 3.3 0.5 0.1 1.7 10.0 0.2

1.7 0.2 0.6 2.3 1.8 0.3 0.9 4.6 1.9

0.3 0.1 1.0 1.6 0.9 0.1 1.1 3.7 0.3

0.7 1.0 1.8 1.8 0.5 0.6 1.4 3.3 0.5

0.5 1.0 1.6 1.9 0.7 0.5 1.9 3.2 0.8

1.9 0.1 0.5 1.3 0.1 0.2 0.6 2.3 0.4

0.9 0.6 1.8 4.4 0.9 0.9 1.4 2.8 0.9

0.9 0.9 1.2 2.9 1.1 1.3 1.5 2.1 0.8

2.5 2.2 4.1 2.6 2.8 2.0 3.0 2.7

1.7 2.1 4.1 3.0 2.3 2.1 2.2 2.6 2.1

0.4 0.3 3.3 1.4 0.4 0.4 2.8 1.6 0.4

1.3 1.4 3.4 1.8 1.3 1.2 2.0 1.8 1.3

0.5 0.6 2.9 1.9 0.4 1.0 2.3 1.8 0.6

0.7 0.5 2.8 2.4 0.7 0.4 1.1 2.0 0.7

0.5 0.2 2.3 2.3 0.2 0.2 1.0 1.5 0.3

0.7 0.9 1.9 1.1 1.1 0.6 5.2 1.9 1.0

0.2 0.2 1.7 1.2 0.1 0.2 0.9 1.9 0.2

2.1 1.8 3.9 3.5 1.8 2.4 2.9 3.0 2.4

1.1 0.9 3.4 2.8 1.0 1.1 2.5 2.5 0.9

0.7 0.3 1.4 1.7 0.9 0.2 1.0 3.2 0.4

0.5 0.4 1.7 1.8 1.0 0.4 1.3 2.2 1.1

1.8 1.3 2.2 2.6 1.4 1.1 2.3 2.6 1.8

3.1 4.1 4.2 3.8 3.3 3.1 3.2 2.7 3.5

1.6 2.6 3.4 3.0 1.3 1.5 2.4 2.3 1.5

1.0 1.9 3.5 2.1 0.8 1.0 2.1 2.5 1.4

0.6 0.1 0.5 3.9 1.1 0.2 0.8 4.4 1.8

2.1 1.6 1.3 1.9 2.9 1.6 1.5 2.2 1.8

0.6 0.1 0.3 2.0 1.0 0.1 0.5 3.0 0.7
1.5 2.1 0.8 2.6 1.2 0.4 0.8 5.5 1.1

1.7 0.6 0.7 2.4 1.6 0.4 0.9 7.2 2.2

1.5

2.5

4.1 3.7 5.3 3.6 2.0 3.1 2.4 2.6 2.8

2.5 0.3 0.9 2.0 0.3 0.2 0.7 3.7 0.6

0.6 0.2 1.2 2.1 0.6 0.2 1.1 3.1 0.3

1.8 1.8 4.3 3.8 1.7 1.6 3.0 2.8 1.9

0.8 1.5 3.7 1.6 0.8 1.1 1.5 1.3 0.9

0.5 0.2 0.7 1.6 0.2 0.2 0.8 1.8 0.3

0.5 0.1 0.6 0.9 0.3 0.3 0.5 2.6 0.4

0.5 0.3 0.8 1.1 0.4 0.3 0.9 1.5 0.4

0.4 0.3 0.6 1.2 0.3 0.3 1.2 2.6 0.3

0.6 0.4 1.4 2.5 0.8 0.9 1.3 2.0

1.0 1.2 1.4 3.3 1.2 1.5 1.4 2.3 1.3

0.9 1.1 2.9 3.6 1.3 1.2 2.5 2.9 1.1

2.9 2.2 3.3 3.9 3.2 2.9 3.1 3.1 3.8

1.1 0.7 0.7 0.8 1.7 0.7 0.8 1.4 1.2

3.8

1.2 0.6 0.9 1.4 1.5 0.7 1.0 1.8 1.0

1.0 0.5 0.6 2.0 0.8 0.4 0.7 5.6 1.8

2.5 1.1 1.6 2.3 3.1

1.8 0.8 0.7 2.8 2.3 3.6 1.8 4.0 2.2

0.3 0.1 0.4 1.5 0.4 0.0 0.5 5.9 1.2

1.3 0.1 0.6 1.7 0.9 0.1 0.4 5.7 1.4

1.0 0.9 1.1 2.6 1.6 0.6 1.1 4.5 1.3

0.9 0.1 0.6 1.9 0.8 0.1 0.6 3.4 1.0

1.3 2.0 2.4 2.3 1.2 1.2 2.0 1.9 1.3

0.3 0.4 0.6 2.4 0.6 0.3 1.4 5.8 0.2

0.4 0.1 0.2 2.5 0.3 0.1 1.1 5.4 0.3

0.4 0.1 0.5 2.2 0.4 0.1 0.5 7.5 0.3

0.4 0.1 0.4 1.6 0.3 0.2 1.8 5.2 0.6

0.3 0.2 0.4 1.6 0.3 0.1 1.4 5.0 0.5

0.4 0.2 0.4 3.5 0.6 0.2 0.7 8.5 0.8

1.5 2.1 2.4 3.0 1.7 2.1 3.5 2.8 1.5
2010 2010 2010 2010 2011 2011 2011 2011 2012

1 2 3 4 1 2 3 4 1

0.3 0.3 0.4 0.4 0.4 0.4 0.4 0.4 0.3

0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0 0.1

0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0 0.1

0.0 0.0 0.1 0.0 0.0

0.0 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.1

0.0 0.1 0.2 0.0 0.0 0.1 0.1 0.1 0.0

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1 0.1

0.4 0.2 0.2 0.3 0.3 0.2 0.2 0.4 0.3

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1

0.1 0.1 0.2 0.1 0.0 0.1 0.3 0.1 0.0

0.2 0.1 0.2 0.4 0.2 0.1 0.3 0.4 0.2

0.2 0.1 0.1 0.2 0.1 0.1 0.1 0.1 0.1

0.2 0.1 0.1 0.3 0.1 0.1 0.4 0.2 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.2 0.1 0.2 0.2 0.2 0.1 0.2 0.2 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.2 0.1 0.2 0.2 0.2 0.1 0.1 0.2 0.2

0.2 0.1 0.1 0.2 0.2 0.1 0.1 0.2 0.2

0.2 0.1 0.1 0.2 0.2 0.1 0.1 0.2 0.1

0.2 0.2 0.2 0.3 0.3 0.3 0.3 0.2 0.3

0.2 0.2 0.2 0.3 0.3 0.3 0.2 0.2 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.2 0.1

0.1 0.1 0.2 0.1 0.1 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.1 0.1 0.3 0.1 0.1 0.2 0.2 0.2 0.1

0.4 0.1 0.2 0.2 0.3 0.1 0.2 0.2 0.3

0.1 0.1 0.1

0.1 0.0 0.0 0.1 0.1 0.0 0.0 0.1 0.1

0.1 0.1 0.2 0.1 0.1 0.1 0.3 0.1 0.1

0.0 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.2 0.2 0.3 0.3 0.2 0.2 0.3 0.3 0.2

0.2 0.1 0.2 0.2 0.1 0.1 0.1 0.3 0.2

0.1 0.2 0.2 0.1 0.1 0.1 0.2 0.1 0.1

0.1 0.2 0.3 0.1 0.1 0.2 0.3 0.1 0.1

0.1 0.1 0.2 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.3 0.1 0.0 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.2 0.1

0.1 0.2 0.4 0.2 0.2 0.2 0.4 0.3 0.2

Elemental Carbon

SANDWICHed*
0.2 0.1 0.1 0.1 0.1 0.2 0.1 0.1 0.1

0.0 0.1 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.0 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.1

1.0 0.8 1.0 1.1 0.8 1.0 0.8 1.0 0.8

0.4 0.3 0.2 0.5 0.4 0.3 0.3 0.5 0.5

0.2 0.1 0.1 0.2 0.3 0.2 0.1 0.2 0.2

0.5 0.2 0.2 0.4 0.5 0.2 0.2 0.3 0.3

0.4 0.3 0.2 0.4 0.4 0.4 0.3 0.3 0.4

0.2 0.3 0.3 0.3 0.3 0.3 0.3 0.3 0.3

0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.2 0.3 0.3 0.2 0.2 0.2 0.3 0.3 0.3

0.2 0.3 0.2 0.2 0.3 0.4 0.2 0.2 0.3

0.1 0.1 0.2 0.1 0.1 0.2 0.2 0.2 0.1

0.3 0.3 0.4 0.4 0.3 0.4 0.3 0.3 0.3

0.3 0.4 0.3 0.4 0.1

0.4 0.3 0.3 0.5 0.4 0.3 0.3 0.4 0.3

0.3 0.3 0.2 0.4

0.2 0.2 0.2 0.2 0.3 0.2 0.2 0.2 0.3

0.1 0.2 0.2 0.2 0.2 0.2 0.3 0.2 0.3

0.3 0.3 0.4 0.3 0.3 0.2 0.4 0.4 0.4

0.1 0.2 0.2 0.1 0.1 0.1 0.2 0.2 0.2

0.3 0.3 0.3 0.3 0.5 0.2 0.2 0.4 0.5

0.1 0.1 0.2 0.1 0.2 0.1 0.1 0.1 0.1

0.3 0.3 0.3 0.3 0.3 0.3 0.3 0.3 0.3

0.2 0.2 0.2 0.1 0.1 0.2 0.2 0.2 0.2

0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.1

0.2 0.3 0.3 0.3 0.3 0.2 0.3 0.3 0.3

0.1 0.2 0.1 0.1 0.1 0.1 0.2 0.2 0.1

0.1 0.2 0.2 0.1 0.1 0.1 0.2 0.2 0.1

0.1 0.1 0.2 0.1 0.1 0.1 0.2 0.2 0.1

0.2 0.2 0.2 0.3 0.2 0.2 0.2 0.3 0.3

0.1 0.1 0.2 0.1 0.1 0.1 0.2 0.2 0.1

0.3 0.2 0.2 0.3 0.2 0.2 0.3 0.3 0.2

0.3 0.3 0.3 0.3 0.3 0.3 0.3 0.4 0.3

0.4 0.3 0.4 0.4 0.4 0.4 0.3 0.5 0.4

0.0 0.0 0.0 0.0

0.0 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.0

0.1 0.1 0.1 0.1 0.0 0.1 0.2 0.1 0.1
0.3 0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1

0.4 0.3 0.4 0.4 0.3 0.4 0.4 0.4 0.3

0.4 0.4 0.4 0.4

0.2 0.3 0.3 0.3 0.2 0.3 0.3 0.3 0.3

0.3 0.3 0.2 0.3 0.3 0.3 0.3 0.3 0.3

0.3 0.3 0.3 0.3 0.3 0.3

0.3 0.3 0.2 0.3 0.4 0.3 0.2 0.3 0.4

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.3 0.1 0.2 0.3 0.2 0.2 0.3 0.3 0.2

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.2 0.1

0.0 0.0 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.1 0.1 0.1 0.2 0.1 0.1 0.2 0.2 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.3 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.2 0.0 0.1 0.1 0.2 0.1

0.1 0.1 0.2 0.1 0.1 0.1 0.2 0.2 0.1

0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.0 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.2 0.1 0.1 0.2 0.2 0.2 0.1

0.2 0.2 0.2 0.1 0.2 0.1 0.2 0.2 0.2

0.4 0.3 0.4 0.4 0.5

0.3 0.3 0.4 0.4 0.3 0.3 0.3 0.4 0.3

0.1 0.1 0.1 0.1 0.1 0.3 0.1 0.1 0.1

0.1 0.1 0.1 0.2 0.1 0.2 0.1 0.2 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.2 0.1 0.3 0.2 0.2 0.1

0.1 0.1 0.1 0.1 0.1 0.2 0.2 0.1 0.1

0.2 0.1 0.1 0.2 0.2 0.2 0.1 0.2 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.2

0.2 0.3

0.3 0.3 0.4 0.3 0.2 0.3 0.3 0.3 0.3

0.2 0.3 0.3 0.2 0.1 0.2 0.2 0.1 0.1

0.2 0.1 0.2 0.2 0.1 0.1 0.2 0.2 0.1

0.2 0.2 0.3 0.2 0.2 0.2 0.2 0.3 0.2

0.4 0.4 0.4 0.5 0.3 0.3 0.3 0.3 0.3

0.2 0.3 0.4 0.4 0.4 0.3 0.4 0.4

0.2 0.2 0.2 0.2 0.3 0.2 0.2 0.2 0.2

0.2 0.2 0.2 0.2 0.2 0.3 0.2 0.2 0.2

0.2 0.5

0.0 0.1 0.1 0.1 0.1 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.2 0.2 0.1 0.1 0.2 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.2 0.2 0.1
0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.2 0.1 0.1 0.2 0.2 0.1

0.3 0.4 0.4 0.4

0.4 0.4 0.5 0.5

0.4 0.2 0.2 0.4 0.4 0.3 0.2 0.3 0.4

0.1 0.1 0.1 0.3 0.1 0.1 0.2 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.2 0.3 0.3 0.3 0.3 0.3 0.3 0.3 0.2

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.2 0.1 0.0

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.2 0.2 0.1 0.1 0.1 0.2 0.2 0.2

0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2

0.2 0.3 0.3 0.2 0.2 0.3 0.3 0.2 0.2

0.5 0.4 0.5 0.6 0.5 0.4 0.5 0.6 0.5

0.1 0.1 0.0 0.0 0.1 0.1

0.2 0.1 0.1 0.3

0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1 0.1

0.1 0.1 0.2 0.2 0.1 0.1 0.2 0.2 0.1

0.2 0.2 0.2 0.3 0.2 0.2 0.3 0.3

0.3 0.1 0.2 0.3 0.3 0.1 0.2 0.3 0.2

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.1

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.1 0.1 0.2 0.1 0.1 0.1 0.3 0.2 0.1

0.0 0.1 0.2 0.1 0.0 0.1 0.1 0.1 0.0

0.3 0.2 0.2 0.2 0.3 0.2 0.2 0.2 0.2

0.2 0.1 0.1 0.2 0.1 0.1 0.2 0.2 0.1

0.0 0.0 0.1 0.1 0.0 0.0 0.2 0.1 0.0

0.0 0.0 0.1 0.0 0.0 0.1 0.1 0.1 0.0

0.1 0.1 0.1 0.1 0.0 0.1 0.1 0.1 0.0

0.1 0.0 0.1 0.1 0.0 0.1 0.1 0.1 0.1

0.1 0.0 0.1 0.1 0.0 0.1 0.2 0.1 0.1

0.2 0.1 0.4 0.1 0.1 0.1 0.0 0.0 0.0
2012 2012 2012

2 3 4

0.4 0.3 0.3

0.2 0.1 0.0

0.1 0.1 0.1

0.0 0.1 0.0

0.1 0.1 0.0

0.1 0.1 0.0

0.1 0.1 0.1

0.1 0.1 0.1

0.2 0.2 0.3

0.1 0.1 0.1

0.1 0.1 0.1

0.2 0.2 0.3

0.1 0.1 0.2

0.2 0.2 0.2

0.1 0.1 0.1

0.2 0.2 0.2

0.1 0.2 0.1

0.1 0.1 0.2

0.1 0.1 0.2

0.1 0.1 0.2

0.3 0.2 0.3

0.3 0.2 0.2

0.1 0.2 0.1

0.1 0.2 0.1

0.1 0.1 0.1

0.2 0.2 0.1

0.1 0.4 0.1

0.1 0.2 0.1

0.0 0.0 0.1

0.1 0.2 0.1

0.1 0.1 0.0

0.2 0.3 0.2

0.1 0.1 0.1

0.1 0.2 0.1

0.2 0.3 0.1

0.1 0.1 0.1

0.1 0.5 0.1

0.1 0.4 0.1

0.1 0.3 0.1

0.2 0.3 0.2
0.1 0.1 0.1

0.1 0.2 0.1

0.2 0.2 0.1

0.1 0.2 0.1

0.1 0.1 0.1

0.1 0.2 0.1

0.6 0.7 1.1

0.3 0.2 0.5

0.1 0.1 0.2

0.2 0.1 0.3

0.2 0.2 0.3

0.2 0.2 0.2

0.1 0.2 0.1

0.1 0.2 0.1

0.2 0.3 0.2

0.3 0.2 0.3

0.2 0.2 0.1

0.3 0.3 0.3

0.3 0.2 0.4

0.2 0.2 0.3

0.2 0.2 0.2

0.2 0.3 0.4

0.1 0.2 0.1

0.2 0.2 0.3

0.1 0.1 0.1

0.3 0.3 0.3

0.1 0.2 0.2

0.1 0.2 0.2

0.2 0.3 0.2

0.1 0.1 0.1

0.1 0.2 0.1

0.1 0.2 0.1

0.2 0.2 0.2

0.1 0.2 0.1

0.2 0.3 0.3

0.3 0.2 0.3

0.3 0.3 0.4

0.1

0.0 0.0 0.0

0.1 0.7 0.1
0.1 0.8 0.1

0.3 0.4 0.3

0.3 0.3 0.3

0.3 0.3 0.3

0.3 0.2 0.3

0.1 0.2 0.1

0.2 0.4 0.3

0.1 0.3 0.1

0.1 0.4 0.1

0.1 0.4 0.2

0.1 1.5 0.2

0.1 0.2 0.1

0.2 0.5 0.1

0.1 0.2 0.1

0.1 0.3 0.2

0.1 0.2 0.1

0.1 0.2 0.1

0.1 0.2 0.1

0.1 0.2 0.1

0.2 0.2 0.2

0.3 0.3 0.4

0.2 0.3 0.3

0.2 0.1 0.1

0.2 0.2 0.2

0.1 0.1 0.1

0.1 0.2 0.2

0.1 0.1 0.1

0.4 0.1 0.2

0.1 0.2 0.0

0.3 0.2 0.3

0.2 0.2 0.1

0.2 0.3 0.2

0.2 0.2 0.2

0.4 0.4 0.3

0.3 0.2 0.4

0.2 0.2 0.2

0.2 0.2 0.2

0.1 0.3 0.1

0.1 0.1 0.1

0.1 0.2 0.1
0.1 0.3 0.1

0.1 0.3 0.1

0.2 0.2 0.3

0.1 0.2 0.1

0.1 0.2 0.1

0.3 0.2 0.2

0.1 0.1 0.1

0.1 0.2 0.1

0.1 0.2 0.1

0.1 0.1 0.1

0.1 0.2 0.1

0.1 0.2

0.2 0.2 0.2

0.2 0.3 0.2

0.4 0.4 0.6

0.0 0.1 0.1

0.1 0.1 0.1

0.1 0.5 0.2

0.1 0.3 0.3

0.1 0.3 0.1

0.1 0.3 0.1

0.1 0.4 0.1

0.1 0.2 0.1

0.2 0.2 0.2

0.2 0.3 0.1

0.1 0.3 0.1

0.1 0.4 0.0

0.2 0.3 0.1

0.1 0.3 0.1

0.1 0.4 0.1

0.0 0.0 0.0