In 2011, Smith competed in the FIFA World Cup, where she scored from the spot in England's quarterfinal match with France, to give England a 1–0 lead in the penalty shootout (England would go on to lose the shootout 4–3). Smith, hindered by an achilles injury, was dissatisfied with her own performances at the tournament: "I have to acknowledge that I didn't play well and I have to live with that." She returned to the England squad for a UEFA Women's Euro 2013 qualifying tie with Serbia after missing the first three matches of the campaign.