In 2008 he signed a contract with and went on to finish second at the Volta a Catalunya and third at the Giro di Lombardia, a prestigious one-day classic. At the 2008 Summer Olympic Games, Urán competed in the road race but he did not finish. In 2009 he finished fifth overall at the Tour de Romandie and rode his first the Tour de France and finished 52nd. In 2010 he rode the Giro d'Italia and finished 7th overall in the 2010 Tour de Suisse. He also rode the Vuelta a España but suffered a fall that ended his options of a high overall placing while being eighth overall.