From 1964 to 1977, Carlos Alberto was capped 53 times and scored 8 goals. He was included in the 44-man training squad for the 1966 FIFA World Cup but did not make the final 22. As it turned out, Brazil were knocked out at the Group stage in England, and when João Saldanha was tasked with restoring pride and passion to the "seleção", he recognised the leadership ability that Carlos Alberto was consistently demonstrating at Santos, and made him national captain. Thus, Carlos Alberto is remembered holding aloft the Jules Rimet trophy after Brazil secured the cup for good after an impressive victory over Italy in the 1970 FIFA World Cup Final in Mexico City. That squad also included Clodoaldo, Gérson, Jairzinho, Roberto Rivelino, Tostão and Pelé. Carlos Alberto's goal against Italy in the final is considered one of the best goals ever scored in the tournament. In 2002 the UK public voted the goal No. 36 in the list of the 100 Greatest Sporting Moments. 1970 would prove to be the only time he would play at that level. He was unable to participate in the 1974 World Cup due to a persistent knee injury. When he eventually regained match fitness, his speed had been compromised. However, his ability to read the game compensated for his loss of pace and when he moved to centre back, he found the form to warrant a recall to the national team. In 1977, he was selected by Claudio Coutinho to captain the national team for the first three qualifiers for the 1978 World Cup. He acquitted himself well despite those being the first competitive internationals he had played for almost seven years. He was approaching 33 years of age and retired from international football, immediately prior to joining New York Cosmos in the NASL. Today he is widely considered one of the finest Brazilian footballers of all time.