Angus became best known for her industrial designs, tiles and wallpapers. Her significant achievements included a tile mural for the Susan Lawrence School in east London, a 'live exhibit' for the Festival of Britain, a tile mural at the British Pavilion at the 1958 Bruxelles Exhibition, and tile designs for Sir Frederick Gibberd at London Heathrow Airport Underground Station. She also designed a new form of marbling design for glass cladding for the original buildings at Gatwick Airport, which produced by the firm TW Ide was given the trade name 'Anguside'. The massive post-war increase in new public architecture led to a large number of commissions from F.R.S. Yorke of YRM (Yorke Rosenberg and Mardell) for tile designs, particularly for new schools and colleges. Her tile designs were produced commercially by Carter and Sons of Poole, Dorset. In 1952, she was made a member of the national Council of Industrial Design.