ShantanuT01/DACTYL-Pretraining huggingface dataset:
Understanding the formation of metal-molecule contact at the microscopic level is the key towards controlling and manipulating atomic scale devices. Employing two isomers of bipyridine, $4, 4^\prime$ bipyridine and $2, 2^\prime$ bipyridine between gold electrodes, here, we investigate the formation of metal-molecule bond by studying charge transport through single molecular junctions using a mechanically controlled break junction technique at room temperature. While both molecules form molecular junctions during the breaking process, closing traces show the formation of molecular junctions unambiguously for $4, 4^\prime$ bipyridine via a conductance jump from the tunneling regime, referred as `jump to molecular contact', being absent for $2, 2^\prime$ bipyridine. Through statistical analysis of the data, along with, molecular dynamics and first-principles calculations, we establish that contact formation is strongly connected with the molecular structure of the electrodes as well as how the junction is broken during breaking process, providing important insights for using a single-molecule in an electronic device.
We propose a new structure suitable for quantum computing in a solid state environment: designed defect states in antidot lattices superimposed on a two-dimensional electron gas at a semiconductor heterostructure. State manipulation can be obtained with gate control. Model calculations indicate that it is feasible to fabricate structures whose energy level structure is robust against thermal dephasing.
The number of known PWNe has recently increased considerably, and the majority of them are now middle-age objects. Recent studies have shown a clear correlation of both X-ray luminosity and size with the PWN age, but fail in providing a thorough explanation of the observed trends. Here I propose a different approach to these effects, based on the hypothesis that the observed trends do not simply reproduce the evolution of a "typical" PWN, but are a combined effect of PWNe evolving under different ambient conditions, the leading parameter being the ambient medium density. Using a simple analytic approach, I show that most middle-age PWNe are more likely observable during the reverberation phase, and I succeed in reproducing trends consistent with those observed, provided that the evolution of the X-ray emitting electrons keeps adiabatic over the whole reverberation phase. As a direct consequence, I show that the X-ray spectra of older PWNe should be harder: also this is consistent with observations.
INTEGRAL detected on August 31, 2004, an unusual thermonuclear X-ray burst from the low-mass X-ray binary GX 3+1. Its duration was 30 min, which is between the normal burst durations for this source (<~10 s) and the superburst observed in 1998 (several hours). We see emission up to 30 keV energy during the first few seconds of the burst where the bolometric peak luminosity approaches the Eddington limit. This peculiar burst is characterized by two distinct phases: an initial short spike of ~6 s consistent with being similar to a normal type I X-ray burst, followed by a remarkable extended decay of cooling emission. We discuss three alternative schemes to explain its twofold nature: 1) unstable burning of a hydrogen/helium layer involving an unusually large amount of hydrogen, 2) pure helium ignition at an unusually large depth (unlikely in the present case), and 3) limited carbon burning at an unusually shallow depth triggered by unstable helium ignition. Though none of these provide a satisfactory description of this uncommon event, the former one seems the most probable.
The appearance of the world varies dramatically not only from place to place but also from hour to hour and month to month. Every day billions of images capture this complex relationship, many of which are associated with precise time and location metadata. We propose to use these images to construct a global-scale, dynamic map of visual appearance attributes. Such a map enables fine-grained understanding of the expected appearance at any geographic location and time. Our approach integrates dense overhead imagery with location and time metadata into a general framework capable of mapping a wide variety of visual attributes. A key feature of our approach is that it requires no manual data annotation. We demonstrate how this approach can support various applications, including image-driven mapping, image geolocalization, and metadata verification.
We examine the perennial quantum spin-liquid candidate $S=1/2$ Heisenberg antiferromagnet on the kagome lattice. Our study is based on achieving Lanczos diagonalization of the Hamiltonian on a $48$ site cluster in sectors with dimensions as a large as $5 \times 10^{11}$. The results reveal novel intricate structures in the low-lying energy spectrum. These structures by no means unambiguously support an emerging consensus of a $\mathbb{Z}_2$ spin liquid ground state, but instead appear compatible with several scenarios, including four-fold topological degeneracy, inversion symmetry breaking and a combination thereof. We discuss finite-size effects, such as the apparent absence of ETH, and note that while considerably reduced, some are still present for the largest cluster. Finally, we observe that an XXZ model in the Ising limit reproduces remarkably well the most striking features of finite-size spectra.
The diffusive epidemic process is a paradigmatic example of an absorbing state phase transition in which healthy and infected individuals spread with different diffusion constants. Using stochastic activity spreading simulations in combination with finite-size scaling analyses we reveal two qualitatively different processes that characterize the critical dynamics: subdiffusive propagation of infection clusters and diffusive fluctuations in the healthy population. This suggests the presence of a strong-coupling regime and sheds new light on a longstanding debate about the theoretical classification of the system.
Non-equilibrium phase transitions are studied theoretically for the two-dimensional Hubbard model subject to bias voltages from the electrodes coupled to the system. By combining the fluctuation exchange approximation with the Keldysh method for non-equilibrium, we have studied the properties of the non-equilibrium Fermi liquid phase and determined the phase diagram with transition to non-equilibrium magnetic and superconducting phases.
Text detection, the key technology for understanding scene text, has become an attractive research topic. For detecting various scene texts, researchers propose plenty of detectors with different advantages: detection-based models enjoy fast detection speed, and segmentation-based algorithms are not limited by text shapes. However, for most intelligent systems, the detector needs to detect arbitrary-shaped texts with high speed and accuracy simultaneously. Thus, in this study, we design an efficient pipeline named as MT, which can detect adhesive arbitrary-shaped texts with only a single binary mask in the inference stage. This paper presents the contributions on three aspects: (1) a light-weight detection framework is designed to speed up the inference process while keeping high detection accuracy; (2) a multi-perspective feature module is proposed to learn more discriminative representations to segment the mask accurately; (3) a multi-factor constraints IoU minimization loss is introduced for training the proposed model. The effectiveness of MT is evaluated on four real-world scene text datasets, and it surpasses all the state-of-the-art competitors to a large extent.
We review the progress in understanding the strange particle yields in nuclear collisions and their role in signalling quark-gluon plasma formation. We report on new insights into the formation mechanisms of strange particles during ultrarelativistic heavy-ion collisions and discuss interesting new details of the strangeness phase diagram. In the main part of the review we show how the measured (multi-)strange particle abundances can be used as a testing ground for chemical equilibration in nuclear collisions, and how the results of such an analysis lead to important constraints on the collision dynamics and space-time evolution of high energy heavy-ion reactions.
Multiple investigations support describing galaxy growth as a stochastic process with correlations over a range of timescales governed by a parameter, $H$, empirically and theoretically constrained to be near unity. Here, we show that the distribution of UV-slopes, $\beta$, derived from an ensemble of theoretical $H=1$ star formation histories (SFHs) is consistent with data at all redshifts $z\le 16$. At $z=0$, the median value $\langle\beta_{H=1}\rangle=-2.27$ agrees well with the canonical $\beta_0=-2.23$ for local starbursts \citep{meurer1999}. At $4\lesssim z\lesssim16$, JWST data span the model distribution's 2nd to 98th percentiles. Values of $-2.8\le \beta \le -2.5$ should be common in early galaxies without reference to exotic stellar populations -- arising solely from a null hypothesis of $H=1$ for the underlying diversity of galaxy growth histories. Future data should be interpreted with this fact in mind.
We show by numerical simulations that a purely stellar dynamical model composed of an exponential disc, a cuspy bulge, and an NFW halo with parameters relevant to the Milky Way Galaxy is subject to bar formation. Taking into account the finite disc thickness, the bar formation can be explained by the usual bar instability, in spite of the presence of an inner Lindblad resonance, that is believed to damp any global modes. The effect of replacing the live halo and bulge by a fixed external axisymmetric potential (rigid models) is studied. It is shown that while the e-folding time of bar instability increases significantly (from 250 to 500 Myr), the bar pattern speed remains almost the same. For the latter, our average value of 55 km/s/kpc agrees with the assumption that the Hercules stream in the solar neighbourhood is an imprint of the bar--disc interaction at the outer Lindblad resonance of the bar. Vertical averaging of the radial force in the central disc region comparable to the characteristic scale length allows us to reproduce the bar pattern speed and the growth rate of the rigid models, using normal mode analysis of linear perturbation theory in a razor thin disc. The strong increase of the e-folding time with decreasing disc mass predicted by the mode analysis suggests that bars in galaxies similar to the Milky Way have formed only recently.
The asymptotic solutions of cosmological topologically massive gravity (TMG) are analyzed for values of the mass parameter in the range $\mu\geq1$. At non-chiral values, a new term in the Fefferman-Graham expansion is needed to capture the bulk degree of freedom. The CDWW modes provide a basis for the pure non-Einstein solutions at all $\mu$, with nonlinear corrections appearing at higher order in the expansion.
Upper bounds on the secret-key-agreement capacity of a quantum channel serve as a way to assess the performance of practical quantum-key-distribution protocols conducted over that channel. In particular, if a protocol employs a quantum repeater, achieving secret-key rates exceeding these upper bounds is a witness to having a working quantum repeater. In this paper, we extend a recent advance [Liuzzo-Scorpo et al., arXiv:1705.03017] in the theory of the teleportation simulation of single-mode phase-insensitive Gaussian channels such that it now applies to the relative entropy of entanglement measure. As a consequence of this extension, we find tighter upper bounds on the non-asymptotic secret-key-agreement capacity of the lossy thermal bosonic channel than were previously known. The lossy thermal bosonic channel serves as a more realistic model of communication than the pure-loss bosonic channel, because it can model the effects of eavesdropper tampering and imperfect detectors. An implication of our result is that the previously known upper bounds on the secret-key-agreement capacity of the thermal channel are too pessimistic for the practical finite-size regime in which the channel is used a finite number of times, and so it should now be somewhat easier to witness a working quantum repeater when using secret-key-agreement capacity upper bounds as a benchmark.
When we watch a video, in which human hands manipulate objects, these hands may obscure some parts of those objects. We are willing to make clear how the objects are manipulated by making the image of hands semi-transparent, and showing the complete images of the hands and the object. By carefully choosing a Half-Diminished Reality method, this paper proposes a method that can process the video in real time and verifies that the proposed method works well.
We propose an efficient way to generate optical analogs of both even and odd Schrodinger cat states (SCSs) with high fidelity, large amplitude and reasonable generation rate. The resource consumed are a single-mode squeezed vacuum state (SMSV) and possibly a single photon or nothing. We report the generation of even (odd) SCS with amplitude 4.2, fidelity higher than 0.99 and reasonable generation rate by subtraction of 30(31) photons from SMSV by ideal photon number detection. In the case of inefficient detectors, maintaining SCS size and its fidelity at the same level as in the case of ideal detectors results in a dramatic decrease in the success probability. In order to have certain harmony between the three characteristics (large amplitude, high fidelity and acceptable success probability for the generation scheme) in the case of imperfect detection, highly transmitting beam splitters should not be used and number of the subtracted photons must be reduced to 10(11).
Our GHOSTS survey measures the stellar envelope properties of 14 nearby disk galaxies by imaging their resolved stellar populations with HST/ACS&WFPC2. Most of the massive galaxies in the sample (Vrot >200 km/s) have very extended stellar envelopes with Sersic law profiles or mu(r)~r^-2.5 power law profiles in the outer regions. For these massive galaxies we can fit the central bulge light and the outer halo out to 30 kpc with one and the same Sersic profile and the stellar surface density of the profiles correlate with Hubble type and bulge- to-disk ratio. This suggests that the central bulges and inner halos are created in the same process. Smaller galaxies (Vrot ~100 km/s) have much smaller stellar envelopes, but depending on geometry, they could still be more luminous than expected from satellite remnants in hierarchical galaxy formation models. Alternatively, they could be created by disk heating through the bombardment of small dark matter sub-halos. The halos we fit are highly flattened, with minor- over-ma jor axis ratios c/a=0.6. The halos are somewhat more compact than hierarchical model predictions. The halos show small metallicity gradient out to 30 kpc and the massive galaxies have typical [Fe/H]~-0.8. We find indications of halo substructure in many galaxies, but some halos seem remarkable smooth.
We study experimentally the electron transport properties of gated quantum dots formed in InGaAs/InP and InAsP/InP quantum well structures grown by chemical-beam epitaxy. For the case of the InGaAs quantum well, quantum dots form directly underneath narrow gate electrodes due to potential fluctuations. We measure the Coulomb-blockade diamonds in the few-electron regime of a single quantum dot and observe photon-assisted tunneling peaks under microwave irradiation. A singlet-triplet transition at high magnetic field and Coulomb-blockade effects in the quantum Hall regime are also observed. For the InAsP quantum well, an incidental triple quantum dot forms also due to potential fluctuations within a single dot layout. Tunable quadruple points are observed via transport measurements.
In the present paper, we have calculated the energy spectra for neutron rich $^{18-22}$N isotopes using no core shell model (NCSM).To calculate the energy spectrum we have used three different $NN$ potentials, inside non-local outside Yukawa (INOY), next-to-next-to-next-leading order (N3LO) from chiral effective field theory and charge-dependent Bonn 2000 (CDB2K). The INOY potential, which is a two body interaction but also have the effect of three body forces by short range and non local character present in it. The calculations have been done at $\hbar\Omega$=20 MeV, 14 MeV and 12 MeV using INOY, N3LO and CDB2K potentials, respectively. Apart from this, we have also performed shell model calculations with the YSOX interaction.The results with INOY interaction show good agreement with the experimental data in comparison to other three interactions. We have also shown the occupancy of different orbitals involved corresponding to the largest model space ($N_{max}$= 4) in the present calculations.
The ab initio calculation of quasiparticle (QP) energies is a technically and computationally challenging problem. In condensed matter physics the most widely used approach to determine QP energies is the GW approximation. Although the GW method has been widely applied to many typical semiconductors and insulators, its application to more complex compounds such as transition metal oxide perovskites has been comparatively rare, and its proper use is not well established from a technical point of view. In this work, we have applied the single-shot G0W0 method to a representative set of transition metal oxide perovskites including 3d (SrTiO3, LaScO3, SrMnO3, LaTiO3, LaVO3, LaCrO3, LaMnO3, and LaFeO3), 4d (SrZrO3, SrTcO3, and Ca2RuO4) and 5d (SrHfO3, KTaO3 and NaOsO3) compounds with different electronic configurations, magnetic orderings, structural characteristics and bandgaps ranging from 0.1 to 6.1 eV. We discuss the proper procedure to obtain well converged QP energies and accurate bandgaps within single-shot G0W0 by comparing the conventional approach based on an incremental variation of a specific set of parameters (number of bands, energy cutoff for the plane-wave expansion and number of k-points and the basis-set extrapolation scheme [Phys. Rev. B 90, 075125 (2014)]. In addition, we have inspected the difference between the adoption of norm-conserving and ultrasoft potentials in GW calculations. A minimal statistical analysis indicates that the correlation of the GW data with the DFT gap is more robust than the correlation with the experimental gaps; moreover we identify the static dielectric constant as alternative useful parameter for the approximation of GW gap in high-throughput automatic procedures. Finally, we compute the QP band structure and spectra within the random phase approximation and compare the results with available experimental data.
The space-borne missions CoRoT and Kepler have provided seismic data of unprecedented quality. Among the observed stars, red giants show a complex oscillation pattern exhibiting pressure modes as well as mixed modes. The latter carry information on the radiative region properties of these stars. The very high precision of Kepler data provide enough accuracy to decipher the complex structure of the mixed-mode pattern and, therefore, deduce precise information on the structure of the stellar core. In this work, we studied the precise influence of the core structural discontinuities on the mixed-mode pattern. These phenomena have indeed an influence on the gravity waves that propagate inside the core of the star and, therefore, on the mixed-mode pattern. In this study, we aim to investigate the impact of core structural discontinuities on the observed mixed-mode pattern and measure their properties for several red giants. We identified several objects showing evidence of deviations in their mixed-mode frequency pattern that are characteristic of core structural discontinuities. We fitted these deviations and showed that they likely correspond to the influence of the inner convective core of these stars.
A new type of gradient estimate is established for diffusion semigroups on non-compact complete Riemannian manifolds. As applications, a global Harnack inequality with power and a heat kernel estimate are derived for diffusion semigroups on arbitrary complete Riemannian manifolds.
The deliberate control over the spatial arrangement of nanostructures is the desired goal for many applications as e.g. in data storage, plasmonics or sensor arrays. Here we present a novel method to assist the self-assembly process of magnetic nanoparticles. The method makes use of nanostructured aluminum templates obtained after anodization of aluminum disks and the subsequent growth and removal of the newly formed alumina layer, resulting in a regular honeycomb type array of hexagonally shaped valleys. The iron oxide nanoparticles, 20 nm in diameter, are spin coated onto the nanostructured templates. Depending on the size, each hexagon site can host up to 30 nanoparticles. These nanoparticles form clusters of different arrangements within the valleys, such as collars, chains, and hexagonally closed islands. Ultimately, it is possible to isolate individual nanoparticles. The strengths of magnetic interaction between particles in a cluster is probed using the memory effect known from the coupled state in superspin glass systems.
We consider the response of a dynamical system driven by external adiabatic fluctuations. Based on the `adiabatic following approximation' we have made a systematic separation of time-scales to carry out an expansion in $\alpha |\mu|^{-1}$, where $\alpha$ is the strength of fluctuations and $|\mu|$ is the damping rate. We show that probability distribution functions obey the differential equations of motion which contain third order terms (beyond the usual Fokker-Planck terms) leading to non-Gaussian noise. The problem of adiabatic fluctuations in velocity space which is the counterpart of Brownian motion for fast fluctuations, has been solved exactly. The characteristic function and the associated probability distribution function are shown to be of stable form. The linear dissipation leads to a steady state which is stable and the variances and higher moments are shown to be finite.
We have studied the spin transport and the spin Hall effect as a function of temperature for platinum (Pt) and gold (Au) in lateral spin valve structures. First, by using the spin absorption technique, we extract the spin diffusion length of Pt and Au. Secondly, using the same devices, we have measured the spin Hall conductivity and analyzed its evolution with temperature to identify the dominant scattering mechanisms behind the spin Hall effect. This analysis confirms that the intrinsic mechanism dominates in Pt whereas extrinsic effects are more relevant in Au. Moreover, we identify and quantify the phonon-induced skew scattering. We show that this contribution to skew scattering becomes relevant in metals such as Au, with a low residual resistivity.
One of the most important problems in nanoelectronic device theory is to estimate how fast or how slow a quantum device can turn on/off a current. For an arbitrary noninteracting phase-coherent device scattering region connected to the outside world by leads, we have derived an exact solution for the nonequilibrium, nonlinear, and time-dependent current driven by both up- and down-step pulsed voltages. Our analysis is based on the Keldysh nonequilibrium Green's functions formalism where the electronic structure of the leads as well as the scattering region are treated on an equal footing. A model calculation for a quantum dot with a Lorentzian linewidth function shows that the time-dependent current dynamics display interesting finite-bandwidth effects not captured by the commonly used wideband approximation.
In this note, a diffusion approximation result is shown for stochastic differential equations driven by a (Liouville) fractional Brownian motion B with Hurst parameter H in (1/3,1/2). More precisely, we resort to the Kac-Stroock type approximation using a Poisson process studied in Bardina, Jolis and Tudor (2003) and Delgado and Jolis (2000), and our method of proof relies on the algebraic integration theory introduced by Gubinelli (2004).