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in the button Options. Mussel-inspired hydrophobic polyimide brushes immobilized on screen-printed carbon electrodes.
Chemically modified screen-printed electrodes were prepared by anchoring layers of poly(epsilon-caprolactone) orpoly(4,4'-methylene diallyl diacrylate) [p(E-Cap)] brushes consisting of hyperbranched polymers on chemically functionalized
carbon-inked screen-printed electrodes. The influence of the grafting of polar or nonpolar brushes on the substrate's electronicand electrochemical properties was investigated by means of cyclic voltammetry (CV), electrochemical impedance spectroscopy(EIS), surface plasmon resonance (SPR) measurements, confocal scanning and transmission electron microscopy (TEM) andatomic force microscopy (AFM). Binding of the grafts was found to improve the electrochemical sensitivity toward ascorbic
acid in CV. While the grafted poly(epsilon-caprolactone) brushes showed a higher conductivity in the oxidized state, the numberof grafted poly(4,4'-methylene diallyl diacrylate) layers determined the better charge transport capability in the neutral state.
Thus, the electrochemical properties and the surface coverage of the polymers were confirmed by SPR measurements and TEMimages. It was also possible to apply the grafts in an electrochemical enzyme assay by using ascorbic acid as substrate andmonitoring the enzymatic reduction of this co- f678ea9f9e
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