 )#%+& ⸘↹Direct disposal 100,000 y*䋨ో㊂⋥ធಣಽ䈱㪈ᐕ⋡䈱Ქᕈ㩿㪪㫍㪀䉕㪈䈫䈚䈢⋧ኻ୯䋩㪈Radiotoxicityof HLW per powerห䈛⊒㔚㔚ജ㊂䈮ኻ䈜䉎㜞䊧䊔䊦ᑄ᫈‛䈱᡼኿⢻䈮䉋䉎ẜ࿷⊛䈭᦭ኂᐲgeneration (relative value)㪈㪅㪜㪂㪇㪇

Pu recycling 8,000 y*(recovery rateᾉPu 99.5%, U 99.6%ὸ㪈㪅㪜㪄㪇㪈㪈㪇㪄㪈㪈㪇㪄㪉㪈㪅㪜㪄㪇㪉

㪈㪇㪄㪊㪈㪅㪜㪄㪇㪊

㪈㪇㪄㪋㪈㪅㪜㪄㪇㪋

㪈㪇㪄㪌㪈㪅㪜㪄㪇㪌

㪈㪇㪄㪍㪈㪅㪜㪄㪇㪍㪈㪇㪄㪎㪈㪅㪜㪄㪇㪎Pu and MA recycling 300 y*(recovery rate: Pu 99.9%,U 99.9%, MA 99.9%ὸNatural Uranium (requiredfor the same power generation)㪈㪇㪄㪏⊖ਁᐕంᐕ⊖ᐕਁᐕ㪈ᐕ010810410610210㪈㪅㪜㪄㪇㪏㪈㪅㪜㪂㪇㪇㪈㪅㪜㪂㪇㪈㪈㪅㪜㪂㪇㪉㪈㪅㪜㪂㪇㪊㪈㪅㪜㪂㪇㪋㪈㪅㪜㪂㪇㪌Year㪈㪅㪜㪂㪇㪍㪈㪅㪜㪂㪇㪎㪈㪅㪜㪂㪇㪏㪈㪅㪜㪂㪇㪐㪈㪅㪜㪂㪈㪇⊖ంᐕ1010/#ǿȸǲȃȈ/#ԃஊྙŴ൐஬Ჴэ҄ǦȩȳሁᲣౝ஥Ἱᔃ/#ǿȸǲȃȈᲢ/#ԃஊྙ᳸Ŵ൐஬/1:༓૰Უᄖ஥Ἱᔃ䉰䉟䉪䊦ᧃᦼ䉰䉟䉪䊦ೋᦼᵫᵟἑὊἄἕἚỉЈщ‫٭‬ѣầ‫ٻ‬Ἱਛᔃᓘᣇะဋ⾰ⵝ⩄

ᓥ᧪ᴺ䋨ಽᢔ㈩⟎䋩㕖ဋ⾰ⵝ⩄ᧄ⎇ⓥ‫ࠍ࠲࡯࠺ޠࠀߓࠎ߽ޟ‬ᵴ↪ߒߚ‫ࠍ࠲࡯࠺ޠࠀߓࠎ߽ޟ‬ᵴ↪ߒߚ/#/#ᩭᄌ឵ߩ⎇ⓥᩭᄌ឵ߩ⎇ⓥ ⢛᥊ߣ⋡⊛⢛᥊ߣ⋡⊛㗄䇭䇭䇭䇭⋡㪤㪘ဋ⾰ⵝ⩄ၮḰἹᔃ㔚᳇಴ജ㩷㪲㪤㪮㪼㪴㪎㪌㪇Ἱᔃᾲ಴ജ㩷㪲㪤㪮㫋㪴㪈㪎㪍㪌ૐ䊗䉟䊄෻ᔕᐲဳ䋨ゲᣇะ㕖ဋ⾰䇮㓏Ბဳ䇮䊅䊃䊥䉡䊛䊒䊧䊅䊛ઃ䈐䋩ἹᔃဳᑼἹᔃၮᧄ઀᭽ㆇォ䉰䉟䉪䊦㐳䈘㩷㪲䊱᦬㪴㪈㪏㪅㪍Άᢱ੤឵䊋䉾䉼ᢙ㩷䋨Ἱᔃ㪆ᓘᣇะ䍪䍼䍵䍻䍗䍍䍢䋩㪍㩷㪆㩷㪍Ἱᔃ㜞䈘㩷䋨ౝ஥Ἱᔃ㪆ᄖ஥Ἱᔃ䋩㩷㪲㪺㫄㪴㪍㪇㩷㪆㩷㪐㪇ౝㇱ䊑䊤䊮䉬䉾䊃ෘ䈘㩷㪲㪺㫄㪴㪉㪇ゲᣇะ䊑䊤䊮䉬䉾䊃ෘ䈘㩷䋨਄ㇱ㪆ਅㇱ䋩㩷㪲㪺㫄㪴䋭㩷㪆㩷㪊㪇䊅䊃䊥䉡䊛䊒䊧䊅䊛ෘ䈘㩷䋨ౝ஥Ἱᔃ㪆ᄖ஥Ἱᔃ䋩㩷㪲㪺㫄㪴㪋㪇㩷㪆㩷㪊㪇ἹᔃΆᢱ㓸ว૕ᢙౝ஥Ἱᔃ㪉㪋㪋ᄖ஥Ἱᔃ㪈㪇㪏ว⸘㪊㪌㪉ᓘᣇะ䊑䊤䊮䉬䉾䊃Άᢱ㓸ว૕ᢙ೙ᓮ᫔ᧄᢙ㩷㪎㪉ਥἹ஗ᱛ♽ᓟ஻Ἱ஗ᱛ♽㓸ว૕㈩೉䊏䉾䉼㩷㪲㫄㫄㪴㪍㪉㪇㪍㪅㪇Ἱᔃ╬ଔ⋥ᓘ㩷㪲㪺㫄㪴㪋㪉㪈Άᢱ⚵ᚑ㪫㪩㪬㩷㩿㪣㪮㪩㪍㪇㪞㪄㪊㪇㫐㪀ἹᔃΆᢱ㪟㪤⚵ᚑ䇭㩿ౝ஥Ἱᔃ㪆ᄖ஥Ἱᔃ㪀㩷㪲㫎㫋㩼㪴㪧㫌ንൻᐲ㩷㩿㪧㫌㪆㪟㪤㪀㪉㪍㪅㪏㩷㪆㩷㪉㪍㪅㪉㪫㪩㪬ንൻᐲ㩷㩿㪫㪩㪬㪆㪟㪤㪀㪊㪊㪅㪊㩷㪆㩷㪊㪉㪅㪍㪤㪘฽᦭₸㩷㩿㪤㪘㪆㪟㪤㪀㪍㪅㪌㩷㪆㩷㪍㪅㪋㓐઻㪝㪧฽᦭₸㩷䋨ౝ஥Ἱᔃ㪆ᄖ஥Ἱᔃ䋩䇭䇭㩷㩷㩷䇭㩷㪲㫍㫆㫃㩼㪴㩿㪝㪧㪆㪟㪤㪀㩷㩷㪲㫎㫋㩼㪴ข಴ᐔဋΆ὾ᐲ㩷㪲㪞㪮㪻㪆㫋㪴Ἱᔃਥⷐ․ᕈ㪉㪈㪇㪅㪉㩷㪆㩷㪇㪅㪉䋨㩷㪇㪅㪈㪋㩷㪆㩷㪇㪅㪈㪋㩷㪀Ἱᔃ㪈㪌㪇㪅㪈ౝㇱ䊑䊤䊮䉬䉾䊃㪍㪐㪅㪐ゲᣇะ䊑䊤䊮䉬䉾䊃㪈㪍㪅㪏ᓘᣇะ䊑䊤䊮䉬䉾䊃㪐㪅㪉ోἹᔃ㪎㪎㪅㪇Ά὾෻ᔕᐲ㩷㪲㩼㰱㫂㪆㫂㫂㩾㪴㪇㪅㪎㪋ჇᱺᲧ㪈㪅㪈㪉ቯᩰᤨ⸵ኈ✢಴ജ䇭䋨ౝ஥Ἱᔃ㪆ᄖ஥Ἱᔃ䋩㩷㪲㪮㪆㪺㫄㪴㪁㪈ᦨᄢ✢಴ജ 㩷䋨ౝ஥Ἱᔃ㪆ᄖ஥Ἱᔃ䋩㩷㪲㪮㪆㪺㫄㪴ᦨᄢ㜞ㅦਛᕈሶᾖ኿㊂㪁㪈㩷㩿㪜䋾㪇㪅㪈㪤㪼㪭䋩㩷㪲㪈㪇 㪉㪊㫅㪆㪺㫄㪉㪴䊅䊃䊥䉡䊛䊗䉟䊄෻ᔕᐲ㪁㪊䇭䇭䋨ᐔⴧᧃᦼ䋩㩷㪲㩻㪴䊄䉾䊒䊤ଥᢙ 㪁㪋䇭䇭䋨ᐔⴧᧃᦼ䋩㩷㪲㪈㪇 㪄㪊㪫㪻㫂㪆㪻㪫㪴㪋㪇㪇㩷㪆㩷㪊㪐㪐㪊㪏㪏㩷㪆㩷㪊㪐㪇㩷㩷㩿㪊㪏㪈㩷㪆㩷㪋㪇㪇㪀㪁㪉㪋㪅㪋Ἱᔃ㪋㪅㪍ౝㇱ䊑䊤䊮䉬䉾䊃㪈㪅㪌਄ㇱ䉧䉴䊒䊧䊅䊛䊶┵ᩖ㪄㪇㪅㪋䊅䊃䊥䉡䊛䊒䊧䊅䊛㪄㪉㪅㪇ว⸘㪊㪅㪍Ἱᔃ㪄㪉㪅㪋ౝㇱ䊑䊤䊮䉬䉾䊃㪄㪉㪅㪋ว⸘㪄㪋㪅㪏㪤㪘ᄌ឵㊂䇭㪲㫂㪾㪆㪞㪮 㪼㫐㪴㪈㪇㪌㪤㪘ข಴ᄌ឵₸䇭㪲㩼㪴㪊㪍㪁㪈㩷㩷㩷㪊ᰴర⸘▚⚿ᨐ㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㩷㪁㪉㩷㩷೙ᓮ᫔ᝌ౉ᤨ䋨㪧㪚㪩㩷㪋㪇㪺㫄ဋ╬ᝌ౉䋩㪁㪊㩷㩷㩷䊤䉾䊌▤㑆䉩䊞䉾䊒䈱಄ළ᧚䈲㕖䊗䉟䊄䇯Ἱᔃ෸䈶ౝㇱ䊑䊤䊮䉬䉾䊃ㇱ䈱㕖ဋ⾰ലᨐ⵬ᱜ㩷㪇㪅㪐㪎䋨ᥳቯ䋩䇮਄ㇱ䉧䉴䊒䊧䊅䊛䊶┵ᩖ䊶䊅䊃䊥䉡䊛䊒䊧䊅䊛ㇱ䈱ャㅍലᨐ⵬ᱜ㩷㪇㪅㪏䋨ᥳቯ䋩䉕⠨ᘦ䇯㪁㪋㩷㩷㕖ဋ⾰ലᨐ⵬ᱜ㩷㩷㪈㪅㪇㪌䋨ᥳቯ䋩䉕⠨ᘦ䇯Άᢱ⚵ᚑ

647 .94)[ ἹᔃΆᢱ */ ⚵ᚑ2W ንൻᐲ 2W*/ 

ౝ஥ᄖ஥ =YV?

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ᩭಽⵚਛᕈሶ㪤㪘䋺䊙䉟䊅䊷䉝䉪䉼䊉䉟䊄ᩭ⎕⎈䉺䊷䉭䉾䊃㜞ㅦਛᕈሶ㪘㪛㪪䈱․ᓽ䋺䊶ടㅦེ䉕ᱛ䉄䉏䈳ㅪ㎮෻ᔕ䈲஗ᱛ㸢 ᩭ෻ᔕ䈱᥸⿛䈱ᔃ㈩䈏ή䈇⍴ኼ๮䈱ᩭ⒳㐳ኼ๮䈱ᩭ⒳䊶㪤㪘Ớᐲ䈱㜞䈇Άᢱ䈏૶↪น⢻㸢 㪈ၮ䈪シ᳓Ἱ㪈㪇ၮಽ䈱㪤㪘䉕ᩭᄌ឵䊶㋦䊎䉴䊙䉴䈲ൻቇ⊛䈮ਇᵴᕈ䇯㵶 㓁ሶ䊎䊷䊛 㪑㩷㪈㪅㪌㪞㪼㪭㵶 ᩭ⎕⎈䉺䊷䉭䉾䊃 㪑㩷㋦䊎䉴䊙䉴㵶 ಄ළ᧚ 㪑㩷㋦䊎䉴䊙䉴౉䉍ญ䋺㪊㪇㪇㷄䇮಴ญ䋺㪋㪇㪎㷄㵶 ᦨᄢ 㫂㪼㪽㪽 㪔㩷㪇㪅㪐㪎㵶 ᾲ಴ജ 㪑㩷㩷㪏㪇㪇㪤㪮㫋㵶 㪤㪘ೋᦼⵝ⩄㊂ 㪑㩷㩷㪉㪅㪌㫋㵶 Άᢱ⚵ᚑ 㪑㩷㩿㪤㪘㩷㪂㪧㫌㪀㪥㩷㪂㩷㪱㫉㪥㵶 ᩭᄌ឵ല₸ 㪑㩷㪈㪇㩼㪤㪘㩷㪆㩷ᐕ㵶 Άᢱ੤឵ᴺ䋺㪍㪇㪇㪜㪝㪧㪛㪃㩷㪈㩷䊋䉾䉼㵶 ਥᓴⅣ䊘䊮䊒䋺㪉ၮ㵶 ⫳᳇⊒↢ེ䋺㪋ၮ㵶 ፣უᾲ㒰෰⸘䋺㪊♽⛔

 #&5 ߩࠛࡀ࡞ࠡ࡯ࡃ࡜ࡦࠬ㓁ሶ䊎䊷䊛಄ළ᧚䊘䊮䊒

⫳᳇⊒↢ེ

ౝ╴
䍩䍼䍎䍯䍞䍼䍖䍢䍩䍼䍎䍯⓹ἹኈེἹᔃᮏ13.5m䍔䍼䍎䍢䍼䍫䍼䍍䍜䍷Ἱᔃᡰᜬ᭴ㅧ

11.8m

㪤㪘Άᢱ䈱ή䈇㪘㪛㪪䈱ᛛⴚ䋨㋦䊎䉴䊙䉴Ἱᔃ䇮ടㅦེ䇮ㆇォ⚻㛎䋩಴ജⷙᮨታ㛎Ἱ⚖㪘㪛㪪㩷㹢࿖㓙౒ห䊔䊦䉩䊷䈱㪤㪰㪩㪩㪟㪘⸘↹㪉㪅㪋㪤㪮㪄㪹㪼㪸㫄㪃㩷㪌㪌 㪇䌾㪈㪇㪇㪤㪮㫋㪿䊶㪘㪛㪪ᛛⴚ䈱ታ⸽䈫Άᢱᾖ኿ታ↪㪘㪛㪪䊒䊤䊮䊃㪊㪇㪤㪮㪄㪹㪼㪸㫄㪃㩷㪏㪏 㪇㪇㪤㪮㫋㪿䊶シ᳓Ἱ㪈㪇ၮಽ䈱㪤㪘ᩭᄌ឵䊎䊷䊛⓹᧚ᢱ䈱㜞ᐲൻ㪤㪘Άᢱ䈱Ἱ‛ℂ䈫䉺䊷䉭䉾䊃᧚ᢱ㐿⊒㪡㪄㪧㪘㪩㪚ᩭᄌ឵ታ㛎ᣉ⸳ỶỼὅเᨗ‫܇‬ἥὊἲἑὊἄἕἚசᐮမఋ༓૰˳ኒᨠᩉࡰᾚᾤᾒᾐὼᾐ௚Өᾕᾕᾐᾖьᡮ֥ᩓᄬჽ㪉㪌㪇㫂㪮㪄㪹㪼㪸㫄䊶㋦䊎䉴䊙䉴䉺䊷䉭䉾䊃ᛛⴚ䊶ᩭᄌ឵䈱Ἱ‛ℂ•㪉㪇㪊㪇ᐕ㗃䉁䈪䈮䊂䊷䉺䈫⚻㛎䉕⫾Ⓧ䈚䇮ᰴ䈱Ბ㓏䈮ㅴ䉄䉎䈎䈬䈉䈎䉕್ᢿ䊦䊷䊒ታ㛎䇮㪢㪬㪚㪘ታ㛎䈭䈬䈱ၮ␆⹜㛎㪉㪇㪈㪇㪉㪇㪉㪇㪉㪇㪊㪇ᐕ㧹㧿㧲㧾 ṁⲢႮἹࡊ࡜ࡦ࠻ߩ᭎ᔨ⸳⸘ 㖧࿖ߩ⁁ᴫ߅ࠊࠅߦ⴫1㜞䊧䊔䊦ᑄᶧਛ䈱㐳ඨᷫᦼᩭ⒳䈫㊂[1]䋨シ᳓ἹUO2Άᢱ䋺Ά὾ᐲ43GWd/t䋩࿑1MA╬䈱ᩭᄌ឵䈮䈍䈔䉎㜞ㅦἹ䉰䉟䉪䊦೑↪ဳ䈫㓏ጀဳ䈱Ყセ[2]࿑2⟲ಽ㔌䊒䊨䉶䉴䈱৻଀[3]࿑3

TPDN䈮䉋䉎241Am,152Eu䈱ṁᇦ᛽಴⹜㛎⚿ᨐ[2]࿑6㊄ዻΆᢱੇᑼౣಣℂ䊐䊨䊷᭎ᔨ࿑7㔚⸃♖⵾䈱᭎ᔨ࿑8INL䈱㔚⸃ⵝ⟎HDEF䈱᭎ᔨ(Ꮐ)䈫EBRͲII૶↪ᷣΆᢱ䈱㔚⸃♖⵾⹜㛎䈮䉋䉎䉝䉪䉼䊆䊄䈫Ꮧ࿯㘃ಽ㔌ଥᢙ(ฝ)[6]࿑9

࿑10ᶧ૕Cd㒶ᭂ䈮䉋䉎䉝䉪䉼䊆䊄䈫ᮨᡆFP(Ꮧ࿯㘃)䈱ಽ㔌ଥᢙ [7]500͠䈮䈍䈔䉎LiCIͲKCl♽ṁⲢႮਛ䈱㊄ዻ䈫⓸ൻ‛䈱ᐔⴧ㔚૏[11]0.65 MDMDOHEMAin TPHAn + Ln extractionFeed3 M HNO30.1 M oxalic acid0.01 M HEDTARaffinateAn+Ln strippingAn + LnProductScrubbing3 M HNO30.2 M Oxalic acid0.015 M HEDTA

Organic waste0.1 MHNO3࿑࿑11Scrubbing

DIAMEX䊐䊨䊷䉲䊷䊃䈱৻଀䉲଀1.5 MHNO3CyMe4-BTBPCyMe4-BTPiPr-BTPiPr-BTP
DMDOHEMAIn n-octanolAn extractionAn
ProductSO3-Ph-BTP

ScrubbingRaffinate

FeedDIAMEX product0.5 M HNO3An strippingOrganic waste0.05 M HNO30.05 M N2H2pH4Glycolic acid࿑12

SANEXBTP䊐䊨䊷䉲䊷䊃䈱৻଀DMDOHEMA 0.6M +HDEHP 0.45M, TPH

Am/CmAm ExtractionCm ScrubbingFEED + TEDGAHNO 3 5-6 M

Cm, lightLn, Zr, RuTEDGAHNO3 5-6 MLa, Ce, Pr, Nd, Mo, Pd, Fe, Ru, TEDGAMo ScrubbingMo

NaOHCarboxylic acidpH 2.5-3.5

Am/Ln

Am StrippingAAm࿑13

DTPA +
Malonic acidpH 2.5Ln-Fe StrippingLn FeEXAmᴺ䈱䊐䊨䊷䉲䊷䊃଀[18]TEDGA+oxalic
HNO3 1 M࿑18ਛ࿖䈪䈱ಽ㔌䊒䊨䉶䉴᭎ⷐ[21]࿑19䉟䊮䊄䈮䈍䈔䉎MAಽ㔌䊐䊨䊷䈱଀[22]࿑࿑20㖧࿖䈪⎇ⓥ㐿⊒䈏ㅴ䉄䉌䉏䈩䈇䉎ੇᑼౣಣℂ䊒䊨䉶䉴᭎ᔨ[23]