Highly intensive cooling process and apparatus for the production of biaxially oriented films of high- and medium-molecular-weight thermoplastics

An apparatus for highly intensive cooling of biaxially oriented films from high- and medium-molecular weight thermoplastics using a long neck on a blown film line is described, including: a plastics extruder, a die for forming a tube neck from the extruded plastic, means positioned adjacent the die for externally cooling the tube neck, an expansion zone where the tube neck becomes a bubble, a drag mandrel positioned immediately before the expansion zone for internally contacting, stabilizing and guiding the tube neck, means for continuously providing cool air internally of the tube neck at the expansion zone immediately after the contact, the means including a first tube in communication with a cool air source, and means for continuously removing the cool air that has been heated. A related method includes the steps of: extruding plastic material through a die to form a tube neck, externally cooling the tube neck immediately after emergence of the tube neck from the die, internally contacting, stabilizing, and guiding the tube neck into a bubble, immediately before the expansion zone, by using a drag mandrel, continuously internally cooling the bubble in the expansion zone immediately after the tube neck contacts the drag mandrel, and continuously removing the cool air that has been heated by the thermoplastic.

BACKGROUND OF THE INVENTION 
The present invention relates to a highly intensive cooling process and an 
apparatus for the production of biaxially oriented films from high- and 
medium-molecular-weight thermoplastics. 
Conventional processes for production of biaxially oriented films from 
medium- and high-molecular-weight HEPE and LDPE polymers and LLDPE 
mixtures with the so-called "long-neck" procedure are old in the art. The 
"long-neck procedure" leads to improvement of the mechanical and physical 
film properties, enhancement of the drawdown of the polymers and 
achievement of better optical properties with LDPE and LLDPE polymer 
types. 
In what is known as the neck zone of devices of known construction, the 
tubular film is blown up to the desired diameter. Orientation of the film 
occurs in the transition zone from the neck to the tubular film. 
Furthermore, tests have been carried out in order to achieve higher 
extrusion outputs with better bubble stabilities, during which the 
specific die output can be increased only by intensifying the external 
cooling of the tubular film, i.e., by increasing the air velocity on the 
external surfaces of the neck and of the transition zone from the neck to 
the tubular film. 
However, the maximum air velocity and thus the maximum cooling effect are 
very rapidly limited by the stability of the bubble. If the cooling air 
streams are too large, the instability of the neck will cause considerable 
upward and downward movements of the bubble, leading to wide fluctuations 
and wrinkling of the film and ultimately to a break-off of the tubular 
film. The output limit in the conventional "long neck" process lies 
between 1.5 and 2.3 kg/cm depending on blow-up ratio, film thickness, type 
of polymer, and room temperature. 
Japanese Pats. No. 55/2180, 53/133,275 and 59/136,224 disclose processes by 
which the bubble stability was improved and the specific die output 
increased by the introduction of an internal drag mandrel in the neck 
zone. However, here the output limit is raised only 20% compared to the 
conventional process, approximately 1.8 to 2.75 kg/cm. 
Further output gains still with good bubble stabilities are achieved by the 
combination of an external cooling immediately after the melt's emergence 
from the die, a stabilization with an internal drag mandrel, and a second 
external cooling on the bubble or in the transition zone. 
Such processes are described in Japanese Pat. No. 59/171,620 and in U.S. 
Pat. No. 4,626,397. These processes, which use a second cooling annulus, 
are not quite operator-friendly, especially upon starting up the system 
and when converting the program. The second cooling annulus in the drag 
mandrel area gives rise to operating problems. 
West German Pats. No. 2,262,190, 2,306,831, 2,610,818 and 2,459,785, teach 
processes which are used for high-speed extrusion of LDPE and LLDPE with 
the conventional bubble shape or with a short neck. Because of the 
instability of the bubble, the process with the so-called "long neck", 
with a height of 6 to 10 times the die diameter, is possible only with 
restrictions. 
An improvement of bubble stability was achieved with U.S. Pat. No. 
4,606,879 and with West German Utility Model 85 25 622.6. But here, too, 
neither system is particularly operator-friendly, because of the second 
cooling annulus or because of the chambers with iris dampers. Also, the 
conversions of the production program are sensitive in both systems. A 
further disadvantage, especially in West German Utility Model 85 25 622.6, 
is the condensation of the monomers and of the additives to the polymers 
on the inner surfaces of the chambers and on the iris dampers. Frequent 
cleaning of the apparatus is necessary in order to ensure the operation of 
the system. 
Therefore, the present invention has as its object the provision of a 
highly intensive cooling apparatus for the production of biaxially 
oriented films from high-and medium-molecular-weight thermoplastics, which 
overcomes the disadvantages described above and features at the same time 
a combination of an intensive external cooling, which is effective 
immediately after the melt's emergence from the mold, a stabilizing 
mandrel positioned in the area of the neck immediately ahead of the 
expanding area of the bubble, and a highly intensive internal cooling 
system which is activated immediately after this drag mandrel in the 
expanding area of the bubble. 
This new apparatus results in a significant increase in the specific 
extrusion output of the die, substantial improvement of the mechanical and 
physical properties of the film, very close thickness tolerances, and the 
perfect bubble stability, the exact maintenance of the film width, and the 
absolute freedom from wrinkles of the lay-flat tubing are always ensured. 
Furthermore, the present invention is to provide an extremely 
operator-friendly apparatus, which is particularly flexible and can be 
used for a very wide range of applications, and which also permits in but 
a few minutes the startup of the system or a conversion of production. 
The invention achieves this object by leading the neck at the expansion 
zone: in two areas, on a conical contact surface of the drag mandrel and 
on point contact of air lips, both of which are inside the tube neck, and 
by activating the internal cooling system immediately after the point 
contact in the expansion zone of the bubble; or in three areas: on the 
conical contact surface, the point contact, and on a contact surface of 
guide rings, on the long-neck and by activating the internal cooling 
system immediately after the point contact in the expansion area of the 
bubble, by passing internal cooling air through a coaxial tube extending 
through the drag mandrel, to the air lips, and sucking the hot air from 
the internal cooling system centrally through the drag mandrel via another 
of the coaxial tubes. 
Furthermore, an apparatus for carrying out the method of the type mentioned 
in the introduction is characterized by the fact that it has a first tube 
mounted on a die, with an internal, second tube disposed therein and 
inserted into the die and in communication with an exhaust conduit, that 
it further has a conical drag mandrel disposed around the first external 
tube, and a terminal exhaust tube provided with air lips, that there is 
disposed in an end zone of the second tube a centering means that locates 
the second tube, there being formed in a main manifold at least one 
cooling channel which leads to a cooling channel that is formed by the 
first tube and by the second tube mounted on the air main manifold, that 
the lips of the have at least one cooling channel, that the outside 
diameters of the air lips are in congruent relationship with the outside 
diameter of the conical drag mandrel, or that the air lips have a portion 
that projects beyond the drag mandrel and forms a point contact, that 
channels that operate for pressure equalization are formed between the die 
and the main manifold, that there is formed between the drag mandrel and 
the first tube a gap which is in communication with vent bores disposed in 
the tube, as well as slots that operate for pressure equalization and are 
disposed near a centering means between the drag mandrel and the first 
tube, that a thermal expansion-compensation device in the form of a cup 
spring is disposed between the air lips and the terminal exhaust tube, 
that the apparatus is attached with a bayonet lock to a split ring and 
thus ensures rapid disassembly of the device, that the drag mandrel is 
covered with an insulating material, preferably of cotton, the drag 
mandrel is covered with an insulating ceramic coating, that the conical 
surface of the drag mandrel has a coarse thread or a wave-like profile in 
order to reduce the contact area, that at least one guide ring that forms 
a contact surface is disposed on the first tube, that the guide ring is 
provided with a coarse thread in order to reduce the contact area, and 
that the drag mandrel has a set screw for vertical adjustment.

DETAILED DESCRIPTION OF THE PREFERRED EMBODIMENTS 
FIG. 1 shows a complete extrusion system with the device incorporating the 
invention. 
The polyethylene granulate is fed into the hopper 43 and plasticized by the 
extruder 2, molded under high pressure by the screen pack changer 35 and 
the die 1 into a tube neck 44, which, after a length of approximately 4 to 
10 times the die diameter, expands across an expansion zone 45 to the 
tubular film 15. 
Directly above the die 1 is located a high-intensity external cooling 
annulus 5 with Venturi inserts 6, and which ensures optimum external 
cooling of the tube neck 44, the expansion zone 45 and the tubular film 
15. The die 1 is prepared for the internal cooling system. The cold-air 
supply is passed through a tube 3 to a manifold 22, then between coaxial 
tubes 24 and 23, and 7 and 8 to an internal cooling zone 46. The hot 
exhaust air is sucked through a central tube 14, tube 8, tube 24, from the 
manifold 22 and out the tube 4. 
The cold-air fan 29 delivers the cooling air through the manifold 36 both 
to the external cooling annulus 5 and to the internal cooling zone 46. The 
setting of the air flow rates is effected by the manually-controlled iris 
dampers 37 and 38. 
Additional conditioning of the cooling air is possible by means of a heat 
exchanger 39, which is attached immediately after the fan 29. The hot-air 
exhaust fan 33 sucks the hot air from the tubular film 15 through the 
tubes 14, 8, 24 and 4. The setting of the exhaust-air flow is effected by 
a manually-controlled iris damper 34. 
A vertically adjustable sizing cage 19 ensures the guidance and sizing of 
the blown tubular film 15. A feeler arm 20, by contacting the tubular film 
15, transmits the diameter variations changes of the bubble to an 
pneumatic sensor 16. The control of the diameter of the blown film tubing 
15 is effected by the control valve 17, which, with the air cylinder 18, 
is controlled by the sensor 16. If the bubble diameter is too large, the 
control valve 17 automatically throttles the internal air supply and, if 
the diameter is too small, the control valve 17 opens. This pneumatic 
control system is accurate to within around 0.1%. Thus, the widths of the 
lay-flat blown film tubing can be maintained with great precision. For 
example, the maximum variations observed for a width of 1000 mm are plus 
or minus 1 mm. 
FIG. 2 shows a practical embodiment of the invention wherein, in addition 
to a conical drag mandrel 9, internal air lips 10 and 11 are used, the 
outside diameters of which are congruent with the outside diameter of the 
internal drag mandrel 9. 
The contact between the tube neck 44 and the drag mandrel 9 is made by the 
conical surface 47, the height of which can be as much as 0.20 times the 
die diameter, depending on the film production. 
FIG. 3 shows an embodiment of the invention with a conical drag mandrel 9, 
but with much larger internal air lips 12 and 13. 
Here, the contact between the tube neck 44 and the parts of the tube neck 
occurs in two areas: 
1. on the conical contact surface 47, and 
2. with the point contact 48 of the internal air lip 12. 
The advantages of this version are better bubble stability because of the 
double contact between the tube neck 44 and the expansion zone 45 with the 
internal drag mandrel 9 and air lip 12, as well as better action of the 
internal cooling system as a result of the small distance between the 
internal air lips 12 and 13 and the expansion zone 45 of the tubular film 
tubing 15. 
The tube neck 44, shaped from the die 1 with a height of 4 to 10 times the 
die diameter, is blown up to the tubular film 15 across the expansion zone 
45. 
The external cooling occurs by means of the high-intensity cooling annulus 
5 with Venturi inserts 6, directly after the melt's emergence from the die 
1 along the entire height of the tube neck 44, the expansion zone 45 and 
to some extent even along the tubular film 15 as well. 
The internal cooling is supplied through the die 1 between the tubes 24 and 
2 and, between the tubes 7, 8, through the conical drag mandrel 9 to the 
internal air lips 10 and 11 or 12 and 13. 
The hot air is exhausted centrally via the tubes 14 and 24, through the die 
1. As shown in FIGS. 2 and 3, the conical drag mandrel 9 is seated on the 
external tube 7, centrally in the tube neck 44, at the expansion zone 45 
in which the tube neck 44 expands into the blown tubular film 15. 
Due to the highly turbulent rate of the air emerging from the air lips 10 
and 11 or 12 and 13, a very good coefficient of heat transfer to the 
inside of the expansion zone 45 is ensured, thus guaranteeing a highly 
intensive internal cooling. In the embodiment shown in FIG. 3, even better 
cooling is achieved with direct contact between the expanding tube neck 44 
and the lower air lip 12, due to the even shorter distance between the air 
lips 12 and 13 and the tube neck 44 becoming a bubble. As a result, the 
Reynolds number of the air flow in this zone is even greater, and thus the 
heat transfer is also more intensive. For the two versions illustrated in 
FIGS. 2 and 3, the internal cooling system requires less cooling air than 
in a conventional internal cooling system in order to achieve the same 
internal cooling effect. Put differently, given the same internal air flow 
rate, the device embodying the invention, as shown in FIGS. 2 and 3, is 
more efficient than the systems of known construction. 
As illustrated in FIGS. 2 and 3, the drag mandrel 9 is vertically 
adjustable. The drag mandrel 9 is attached by means of the set screw 49. 
This vertical adjustment is particularly important in order to be able to 
set different tube neck 44 heights. 
In the embodiment depicted in FIG. 3, the setting of the neck height can be 
effected only by replacing the tubes 8 and 7. A small vertical adjustment 
of the drag mandrel 9 permits adaptation of the distance between the 
conical contact surface 47 and the point contact 48, depending on the 
production program. It was chosen to allow the angle alpha, denoted by the 
reference numeral 50, of the internal air lips 10 and 13, to have a value 
between 90.degree. and 45.degree. relative to the vertical axis. 
Another feature of the invention is the guidance of the tube neck 44 by the 
conical contact surface 47 with the drag mandrel 9. This results in the 
stabilization of the tube neck 44 and of the tubular film 15. The tube 
neck 44, as well as the expansion zone 45, can no longer move up and down 
horizontally or vertically. An even better guidance of the tube neck 44 
and of the expansion zone 45 is achieved with the embodiment shown in FIG. 
3 in which a double contact with the parts internal of the tube neck 44 is 
present. The guidance of the tube neck 44 by the conical contact surface 
47 with the drag mandrel 9 is further supported by the point contact 48 
with the lower air lip 12. This results in the perfect width maintenance 
of the lay-flat tubing as well as the film web's absolute freedom from 
wrinkles. 
The conical shape of the drag mandrel 9 ensures a very universal use. All 
HDPE, LDPE and LLDPE mixtures can be extruded as single-ply film or 
coextruded as two-ply or three-ply film in a very broad processing range. 
Depending on the geometry of the parts 9, 10 and 11 or 9, 12 and 13, 
positioned internally of the tube neck a very large range of widths is 
made available, with blow-up ratios that can lie between 1:1.75 and 1:6 
and, depending on type of polymer, the range of film thickness can be 
adjusted between 5 and 75 micron. 
FIG. 4 shows an enlargement of the detail designated A in FIG. 2. 
Here, it can be seen that the internal air lips 10 and 11 have at least one 
cooling channel 32, which serves for the internal cooling of the tubular 
film 15. 
In this case, it is clearly evident that the tubular film 15 is in contact 
only on the conical surface 47 of the drag mandrel 9, since the outside 
diameters of the internal air lips 10 and 11 correspond approximately to 
the outside diameter of the conical drag mandrel 9. 
FIG. 5 shows an enlargement of the detail designated B in FIG. 3. 
In this case, internal air lips 12 and 13 are used which project beyond the 
outside circumference of the conical drag mandrel 9. The result is that a 
point contact 48 is established in addition to the conical contact surface 
47. 
The advantages of this embodiment have already been described hereinbefore. 
As can be seen in FIGS. 4 and 5, a thermal expansion-compensation device in 
the form of a cup spring 42 is dispersed between the central tube 14 and 
the nut 51 connecting the device and the internal air lip 11 or 13. 
FIGS. 6 to 8 show the details with which pressure equalization between the 
tube neck 44 and the external tube 7, as well as between the drag mandrel 
9 and the lower air lip 12, can be ensured. The pressure equalization 
takes place through the channels 21 of about 1 mm diameter between a main 
manifold 25 and a split ring 52, as well as through a 1 mm longitudinal 
gap 40 between the outer diameter of tube external tube 7 and the inner 
diameter of drag mandrel 9. Perpendicular vent bores 53 provide additional 
pressure equalization to the system via the gap 40. As can be seen in 
FIGS. 7 and 8, the gap 40 is provided over only 85% of the total height of 
the drag mandrel. A centering means 54 is disposed in the upper area of 
the drag mandrel 9. Several slots 41 are cut into the centering means 54 
for the pressure equalization in the device. As apparent from the diagram 
in FIG. 6, the centering of the parts 25 and 52 in is effected by three 
support points 55, which are spaced 120.degree. apart on the main manifold 
25. 
With this special construction, it is ensured that the tube neck 44 always 
remains very stable. Suction effects or inflations of the tube neck 44, 
depending on the production program, are therefore not possible. Vent gaps 
31 and the gap 40, the bores 53 and the slots 41 provide further 
advantages during the phase of startup of the extrusion system. The air 
flowing out of the gaps 31 and 40 expands the tube neck 44 during the 
startup phases and thus makes it easier to pull the same over the drag 
mandrel 9 and the die air lips 10 or 12. 
The air-guidance tubes 8 and 7 are centered exactly by the main manifold 25 
and the lower air lips 10 or 12. The cooling air flows through bores 56 
and 32a. The entire device is bolted together with the nut 51. The cup 
spring 42 equalizes the expansion differences which occur due to different 
temperatures in the tubes 8 and 7. 
The entire device is attached to the split ring 52 of the die 1 with a 
bayonet lock 57. Therefore, rapid disassembly of the device, as is 
necessary whenever the split ring 52 is cleaned, is ensured. 
Several provisions are necessary to prevent adhesion between the plastic 
melt and the drag mandrel 9 in the area of the conical contact surface 47: 
covering of the drag mandrel 9 by an insulating material of cotton, a 
possible alternative being to spray an insulating ceramic coating onto the 
surface of the drag mandrel 9, or reducing the contact area of the drag 
mandrel 9 by a coarse thread or by a wave-like profile cut onto the 
conical surface. 
An alternative version of the guidance of the tube neck 44 and of the shape 
of the tube 7 is illustrated in FIG. 9. A number of guide rings 60, with 
different diameters, which are attached to the external tube 7, ensure 
even better guidance of the tube neck 44 and, together with the point 
contact 48 and the conical contact surface 47, form a third contact 
surface 61. This special construction has proved effective especially when 
producing narrow tubular films with small die diameters and with reduced 
blow-up ratios. In such productions, e.g., during the production of a 
500-mm-broad tubular film with a thickness approximately 12 to 18 micron 
from HDPE, a considerable constriction of the tube neck 44 is observed as 
a result of the physical polymer properties and due to the process using a 
long neck. The diameter of the tube neck 44 can therefore decrease to 50% 
of the die diameter just ahead of the expansion zone of the bubble. In 
order not to influence the formation of the tube neck 44 too strongly, 
which process is determined by the laws of physics, the geometry of the 
device according to FIG. 9 is fashioned as follows: 
The diameter of the tube 7 is greatly reduced. 
The diameter of the rings 60 is chosen to become progressively smaller 
moving downstream, the bottom ring is equal in size as the die and the 
diameter of the top ring can be reduced to 0.8 times the die diameter. 
The number of rings varies according to die size and tube neck 44 height, 
but there is at least one ring. 
The minimum diameter of the drag mandrel is also greatly reduced. 
In order to reduce the surface area, the rings 60 are provided with a 
coarse thread 62 cut onto the outside diameter thereof. 
The apparatus incorporating the invention leads to advantages which are 
effective in particular when increasing the system output, to an 
improvement of the film quality, and to a process-related improvement when 
adjusting and converting the film-blowing system. 
A considerable increase in output is achieved when producing biaxially 
oriented films from HDPE, LDPE and LLDPE mixtures when employing the 
process with an extremely long neck of 4 to 10 times the die diameter and 
with very high die outputs of up to 4.5 kg/cm/hr or 25 lbs/inch/hr. 
A further advantage of the device according to the invention is that a 
considerable quality improvement is achieved when producing biaxially 
oriented films from HDPE, LIPE or LLDPE mixtures with particularly good 
physical and mechanical properties. These improvements of the film 
properties are attributable to optimum longitudinal and transversal 
stretching of the polymeric molecular chains. Because of the additional 
friction on the drag mandrel, greater longitudinal stretching of the films 
is achieved. Because of the intensive internal cooling of the film in the 
expansion, a much higher internal pressure in the bubble is needed in 
order to perform transversal stretching of the film. Both effects lead to 
a considerable shortening of the expansion zone between the beginning of 
the expansion zone and the frost line, and also the stretching in the 
longitudinal and transversal direction occurs progressively much more 
rapidly. Thus, the optimum biaxial orientation of the film is achieved, 
and more uniform film strengths in both the longitudinal and transversal 
directions are achieved, together with very high dart-test values and 
optimum tear propagation strengths of the film in both directions. This is 
true in particular for very large widths, which are produced with 
relatively large dies, for which the expansion zone becomes progressively 
longer. 
In addition, the production of biaxially oriented films from LDPE and LLDPE 
with particularly good optical properties and high drawdown of the 
polymers is possible as a result of the device incorporating the 
invention. 
Furthermore, the present invention enables the production of biaxially 
oriented films with good thickness distributions. Because of the 
stabilization of the bubble by the drag mandrel and the special shape of 
the internal cooling air lips, there are no differences in thickening of 
the film as a result of varying internal cooling effects. In conventional 
internal cooling systems, horizontal displacements of the neck have 
negative influences on the thickness distributions. 
Because of the surface contact between the tubular film and the drag 
mandrel according to FIG. 2, or because of the double contact between the 
neck, the expansion zone and the contact parts internal of the tube neck 
44 according to FIG. 3, a much better bubble stability is achieved. This 
leads to the exact width maintenance of the lay-flat tubing and thus to 
the perfect freedom from wrinkles of the film. Therefore, the production 
of exact laps, especially with regard to the geometry of the roll and to 
the flatness of the film, is always ensured. 
A further characteristic of the invention is the highly intensive internal 
cooling in the tubular film because of the short distance between the 
internal air lips and the expansion zone of the film. When compared to a 
conventional internal cooling system, the efficiency of the new device is 
much higher. 
An important advantage of the apparatus incorporating the invention also 
lies in the very wide processing range of the process which can be carried 
out with this device. For maximum extruder output and with the same 
apparatus, the following conversions can be effected extremely fast and 
without difficulty, often under one minute: 
Change of the reclining width in the range of blow-up ratios from 1 : 1.75 
to 1 : 6.0. 
Changes of the film thicknesses in the range from 5 to 75 micron. 
Changes of the take-off speeds in the range from 15 to 200 m/min. 
The final important advantage of the device incorporating the invention 
lies in the simple setting and conversion of the system, for which no 
skilled labor is needed.