Fundamental Carrier-Envelope Phase Noise Limitations during Pulse Formation and Detection

The difference between the positions of the maximum peak of the carrier wave of a laser pulse and the maximum of its intensity envelope is termed carrier-envelope phase (CEP). In the last decades, the control and stabilization of this parameter has greatly improved, which enables many applications in research fields that rely on CEP-stable pulses such as attosecond science and optical frequency metrology. Further progress in these fields depends strongly on minimizing the CEP noise that restricts stabilization performance. While the CEP of most high repetition-rate low-energy laser oscillators has been stabilized to a remarkable precision, some types of oscillators show extensive noise that inhibits precise stabilization. The CEP stabilization performance of low repetition-rate high peak-power amplified laser systems also remains limited by noise, which is believed to stem mainly from the CEP detection process. In this thesis, the origins of the CEP noise within four oscillators as well as the noise induced by the measurement of the CEP of amplified pulses are investigated. In the first part, the properties of the CEP noise of one Ti:sapphire oscillator and three different fiber oscillators are extracted by analyzing the unstabilized CEP traces by means of time-resolved correlation analysis of carrier-envelope amplitude and phase noise as well as by methods that reveal the underlying statistical noise properties. In the second part, investigations into the origin of CEP noise induced by the measurement of the CEP of amplified pulses are conducted by comparing several different CEP detection designs that are based on f -2 f interferometry. These detection setups differ in the employed sources of spectral broadening as well as frequency doubling media, both necessary steps to measure the CEP. The results in both parts of this thesis show that white quantum noise dominates most CEP measurements. In one particular fiber oscillator, the strong white noise is found to be a result of a correlating mechanism within the employed SESAM. During amplifier CEP detection, the CEP noise is found to be originating only to a marginal degree from the number of photons that are detected during the measurement, which excludes shot noise as a limiting source. Instead, the analysis reveals that the origin of the observed strong white noise can be interpreted as a loss of coherence during detection. This type of coherence is termed here intra-pulse coherence and describes the phase transfer within f -2 f interferometry. Its degradation is a result of amplitude-to-phase coupling during the spectral broadening process that leads to pulse-to-pulse fluctuations of the phases at the edges of the extended spectrum. Numerical simulations support the concept of intra-pulse coherence degradation and show that the degradation is substantially stronger during plasma-driven spectral broadening as compared to self-phase modulation-dominated spectral broadening. This difference in degradation also explains the much stronger CEP noise typically observed in amplified systems as compared to oscillators, as the former typically rely on filamentation-based and hence plasma-dominated spectral broadening for CEP detection. The concept of intra-pulse coherence constitutes a novel measure to assess the suitability of a spectral broadening mechanism for application in active as well as in passive CEP stabilization schemes and provides new strategies to reduce the impact of the CEP detection on the overall stabilization performance of most lasers.