N incident on 37-CL. ORNL resonance param. evaluation.   Mar 2007    1 0  0    0
 1.703700+4 3.664830+1          1          0          0          21731 1451    1
 0.000000+0 0.000000+0          0          0          0          61731 1451    2
 1.000000+0 2.000000+7          9          0         10          71731 1451    3
 0.000000+0 0.000000+0          1          0        485        1571731 1451    4
 17-Cl- 37 ORNL,LANL  EVAL-OCT03 Sayer,Guber,Leal,Larson,Young+   1731 1451    5
                      DIST-DEC06                                  1731 1451    6
----ENDF/B-VII        MATERIAL 1731                               1731 1451    7
-----INCIDENT NEUTRON DATA                                        1731 1451    8
------ENDF-6 FORMAT                                               1731 1451    9
******************************************************************1731 1451   10
CL35,37 Resonance Parameter Evaluation Update, January, 2007.     1731 1451   11
R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson (ORNL)         1731 1451   12
                                                                  1731 1451   13
The updated ENDF format now permits the full generality of the    1731 1451   14
Reich-Moore theory, including charged particle exit channels.     1731 1451   15
Consequently, we have updated the ENDF evaluations by adding      1731 1451   16
resonance parameters (RPs) to File 2, MT=151, and by including    1731 1451   17
the corresponding RP covariance matrices in File 32, MT=151.      1731 1451   18
The Reich-Moore format with LRF=3 and LCOMP=1 was                 1731 1451   19
utilized for CL37.  The Reich-Moore Limited (LRF=7, LCOMP=2)      1731 1451   20
format was used for CL35 because the proton exit channel is open  1731 1451   21
(Q = +0.61522 MeV).  The applicable energy range is  0.00001 eV   1731 1451   22
to 1.2 MeV.  Above 1.2 MeV, cross sections from the February 2000 1731 1451   23
ENDF evaluation are used.                                         1731 1451   24
                                                                  1731 1451   25
The Cl evaluations [1,2] were based on fits of many data sets with1731 1451   26
the SAMMY code [3].  In ref [2] we give detailed discussions of   1731 1451   27
the analysis methods used to determine parameter values and       1731 1451   28
uncertainties.  For capture and neutron width uncertainties, for  1731 1451   29
example, for each resonance several SAMMY calculations with       1731 1451   30
different width values were overlaid with the data.  Both the     1731 1451   31
overlay plots and chi-squared changes with width variation were   1731 1451   32
used to determine final uncertainties that were, in most cases,   1731 1451   33
significantly larger than the SAMMY values.  The RADCOP code [4]  1731 1451   34
was used to generate both File 2 and File 32.                     1731 1451   35
                                                                  1731 1451   36
At the time of the Cl evaluation, SAMMY did not incorporate the   1731 1451   37
now available "Prior Uncertainty Parameter", or PUP procedure.    1731 1451   38
Thus, some normalization and background uncertainties were not    1731 1451   39
propagated properly through the sequential analysis of multiple   1731 1451   40
data sets.  Although uncertainties in resonance energies          1731 1451   41
and widths are felt to be realistic, the uncertainties in         1731 1451   42
computed cross sections in valleys between resonances were        1731 1451   43
underestimated.  Furthermore, since File 32 is limited by the     1731 1451   44
current ENDF format to RP uncertainties and correlations,         1731 1451   45
uncertainties in nuclear radii cannot be treated directly.        1731 1451   46
These "normalization/background/radius" effects were represented  1731 1451   47
approximately by adjusting the File 32 uncertainties for the      1731 1451   48
external RPs and for selected resonances in the energy range of   1731 1451   49
the evaluation.                                                   1731 1451   50
                                                                  1731 1451   51
Since the resonance parameter representation does not include the 1731 1451   52
direct capture (DC) part of the capture cross section, the DC     1731 1451   53
component was included as  a "background" 1/v cross section in    1731 1451   54
File 3, sections 1 and 102.   At E = 0.0253 eV, the CL35 (CL37) DC1731 1451   55
cross section is 0.16 (0.31) b, which is a small (large) fraction 1731 1451   56
of the overall capture cross section of 43.60 (0.433) b.          1731 1451   57
The upper energy limit for the DC cross section is estimated [2]  1731 1451   58
to be 10 (100) keV for CL35 (CL37).   Therefore, the "background" 1731 1451   59
1/v cross section was terminated at these energy values.          1731 1451   60
                                                                  1731 1451   61
REFERENCES                                                        1731 1451   62
----------                                                        1731 1451   63
[1] R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson,           1731 1451   64
    and T. Rauscher, ORNL/TM-2003/50, March, 2003.                1731 1451   65
[2] R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson,           1731 1451   66
    and T. Rauscher, Phys. Rev. C73, 044603 (2006).               1731 1451   67
[3] N. M. Larson, ORNL/TM-9179/R7 (2006), ENDF-364/R1.            1731 1451   68
[4] R. O. Sayer and D. Wiarda, Physor-2006, Vancouver, B. C.,     1731 1451   69
    Canada (2006).                                                1731 1451   70
                                                                  1731 1451   71
******************************************************************1731 1451   72
ORNL Resonance Parameter Evaluation, October, 2003.               1731 1451   73
R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson, T. Rauscher   1731 1451   74
                                                                  1731 1451   75
Our resonance parameter evaluation is described below.   File 3   1731 1451   76
total [MT 1], elastic [MT 2], and capture [MT 102] cross section  1731 1451   77
values for T=0K for  were computed from the resonance parameter   1731 1451   78
representation.   For the energy range 0.00001 eV to 1.2 MeV, the 1731 1451   79
pointwise File 3 cross sections are based on the resonance        1731 1451   80
parameter files.  Above 1.2 MeV, the current (February 2000) ENDF 1731 1451   81
cross sections are used.  The CL35 file also contains (n,p) [MT   1731 1451   82
103,600] cross sections for T = 0K.  For the energy range 0.00001 1731 1451   83
eV to 121 keV, the pointwise cross sections are based on the      1731 1451   84
resonance parameter file.   Above 121 keV, the current (February  1731 1451   85
2000) ENDF cross sections are used.   The last resonance with     1731 1451   86
non-zero proton width is at 103.5 keV.                            1731 1451   87
                                                                  1731 1451   88
We performed an evaluation [1] of Cl neutron cross sections in    1731 1451   89
the resolved resonance region with the multilevel Reich-Moore     1731 1451   90
R-matrix formalism. Resonance analyses were carried out with the  1731 1451   91
computer code SAMMY [3], which utilizes Bayes' method, a          1731 1451   92
generalized least squares technique.  A recent modification of    1731 1451   93
SAMMY enabled us to calculate charged particle penetrabilities    1731 1451   94
for the proton exit channel.  Our evaluation takes advantage of   1731 1451   95
recent high-resolution capture and transmission measurements at   1731 1451   96
the Oak Ridge Electron Linear Accelerator (ORELA) to extend the   1731 1451   97
resolved resonance energy range to 1.2 MeV with much more         1731 1451   98
accurate representation of the data than previous evaluations.    1731 1451   99
                                                                  1731 1451  100
The total cross section data include measurements by Guber, et    1731 1451  101
al. [2] and Good, et al. [4], on the 80-m flight path at ORELA;   1731 1451  102
Cierjacks, et al. [5], on a 57-m flight path at the Karlsruhe     1731 1451  103
Isochronous Cyclotron; Singh, et al. [6] on the 200-m flight      1731 1451  104
path at the Columbia synchrocyclotron; Brugger, et al. [7], who   1731 1451  105
utilized a crystal spectrometer and also the MTR fast chopper     1731 1451  106
with a flight path of 45 m; Kiehn, et al. [8], with the           1731 1451  107
Rockefeller generator; and Newson, et al. [9], at the Duke Van    1731 1451  108
de Graaff facility.                                               1731 1451  109
                                                                  1731 1451  110
Also included in the evaluation were the high resolution capture  1731 1451  111
cross section data (0.1 < En < 500 keV) of Guber, et al. [2] and  1731 1451  112
the older, low resolution capture data (0.02 < En < 1.0 keV) of   1731 1451  113
Kashukeev, et al. [10]. The 35Cl(n,p)35S cross section data of    1731 1451  114
Koehler [11] and Druyts, et al. [12] were also fit. The proton    1731 1451  115
widths are significant fractions of the total widths for          1731 1451  116
resonances at 398 and 4251 eV.                                    1731 1451  117
                                                                  1731 1451  118
In order to give a proper treatment for charged particles in an   1731 1451  119
exit channel, an algorithm to calculate charged particle          1731 1451  120
penetrabilities (CPP) and shifts was incorporated in the SAMMY    1731 1451  121
code. The methodology for CPP computation has been given          1731 1451  122
previously [13].  Routines based on the CPP algorithm have been   1731 1451  123
developed and incorporated in a development version of the        1731 1451  124
nuclear data processing code NJOY [14] for use in preparing data  1731 1451  125
for criticality safety benchmark calculations.  The nuclear       1731 1451  126
radii used for penetrabilities and shifts were computed           1731 1451  127
according to   R = 1.23A**0.33333 + 0.8 fm, where A is the        1731 1451  128
nuclide mass. These values were 4.8222 and 4.8974 fm for 35Cl     1731 1451  129
and 37Cl, respectively. In the SAMMY analysis the radii used to   1731 1451  130
compute hard sphere phase shifts were allowed to vary, and        1731 1451  131
different radii were allowed for s- and p-waves.  Final values    1731 1451  132
for 35Cl were R(L=0,1) = 3.6680, 4.8888 fm; final values for 37Cl 1731 1451  133
were R(L=0,1) = 3.3651,3.9565 fm.                                 1731 1451  134
                                                                  1731 1451  135
Capture Cross Section Analysis                                    1731 1451  136
------------------------------                                    1731 1451  137
Guber, et al. [2] measured the neutron capture of chlorine up to  1731 1451  138
500 keV using a natural LiCl sample of thickness 0.09812 atoms/b  1731 1451  139
and the ORELA capture system, which had been re-engineered [20]   1731 1451  140
to minimize the amount of structural material surrounding the     1731 1451  141
sample and detectors. To calculate accurate correction factors    1731 1451  142
for experimental effects of the neutron capture data, reliable    1731 1451  143
neutron widths are needed since the sample was fairly thick.      1731 1451  144
Initial neutron widths were obtained by  fitting the              1731 1451  145
transmission data; using these newly determined values,           1731 1451  146
corrections for self-shielding and multiple scattering were       1731 1451  147
calculated with SAMMY and used to determine capture widths.       1731 1451  148
Several iterations of fitting the transmission and capture data   1731 1451  149
were performed to obtain final resonance parameters for 0.1 < En  1731 1451  150
< 500 keV.   From their resonance parameters, Guber, et al. [2],  1731 1451  151
calculated average cross sections that were rather different      1731 1451  152
from ENDF/B-VI. This difference is very likely the result of      1731 1451  153
underestimated neutron sensitivity in the older measurements as   1731 1451  154
well as an improved calculation of the weighting function.        1731 1451  155
                                                                  1731 1451  156
In nuclides where the (n,gamma) cross section is small, the       1731 1451  157
direct capture (DC) is often a significant fraction of the cross  1731 1451  158
section. Guber, et al. [2] describe in detail the DC              1731 1451  159
calculations they performed for 35Cl and 37Cl using the code      1731 1451  160
TEDCA [21, 22]. They calculated that the effect of the DC         1731 1451  161
component was very small for 35Cl where the thermal capture       1731 1451  162
cross section is 43.6 b. However, for 37Cl approximately 0.31 b   1731 1451  163
of the thermal capture cross section of 0.433 b is due to direct  1731 1451  164
capture. We have deduced a set of resonance parameters,           1731 1451  165
including the external level parameters, that reproduce the       1731 1451  166
resonant part of the capture cross section. To this resonant      1731 1451  167
part, one must add the DC contribution to obtain the overall      1731 1451  168
capture cross section. The thermal value of the DC cross section  1731 1451  169
is 0.16 +- 0.05 b for 35Cl and 0.31 +- 0.16 b for 37Cl.           1731 1451  170
                                                                  1731 1451  171
Thermal and Integral Quantities                                   1731 1451  172
-------------------------------                                   1731 1451  173
The following table gives a comparison of our elastic, capture,   1731 1451  174
(n,p), and total cross sections for En = 0.0253 eV and T = 0K     1731 1451  175
with the corresponding ENDF/B-VI quantities, which are based      1731 1451  176
principally on the compilation of Mughabghab [15]. The capture    1731 1451  177
cross section values include the DC contribution.  Also given is  1731 1451  178
the resonance capture integral, I-gamma.                          1731 1451  179
                                                                  1731 1451  180
Cl Thermal Cross Sections and Resonance Integrals for T = 0K      1731 1451  181
Nuclide     Quantity  ENDF/B-VI (b)    Present Evaluation (b)     1731 1451  182
-------     -------   --------------   ----------------------     1731 1451  183
35Cl        total     64.70 +- 0.50           64.75               1731 1451  184
            elastic   20.60 +- 0.30           20.67               1731 1451  185
            capture   43.60 +- 0.40           43.60               1731 1451  186
            (n,p)      0.48 +- 0.14           0.480               1731 1451  187
            I-gamma   17.80 +- 2.00           18.19               1731 1451  188
                                                                  1731 1451  189
37Cl        total     1.583 +- 0.050          1.581               1731 1451  190
            elastic   1.150 +- 0.050          1.148               1731 1451  191
            capture   0.433 +- 0.006          0.433               1731 1451  192
            I-gamma   0.204 +- 0.040          0.198               1731 1451  193
                                                                  1731 1451  194
The new ORELA measurements and the older KFK measurements enabled 1731 1451  195
us to extend the resonance parameter representation to 1.2 MeV;   1731 1451  196
the ENDF/B-VI representation above 226 keV, based on calculations 1731 1451  197
utilizing Hauser-Feshbach statistical theory, is inadequate.      1731 1451  198
                                                                  1731 1451  199
SUMMARY AND CONCLUSIONS                                           1731 1451  200
-----------------------                                           1731 1451  201
The Cl data used in this evaluation include recent ORELA          1731 1451  202
high-resolution capture and transmission measurements as well as  1731 1451  203
several older data sets. Since the 35Cl(n,p)35S reaction yields   1731 1451  204
a significant contribution to the total cross section from        1731 1451  205
thermal energies up to about 10 keV, the 35Cl(n,p) data of        1731 1451  206
Koehler [11] and Druyts, et al. [12] were fit to obtain proton    1731 1451  207
width values for several resonances. The proton widths are        1731 1451  208
significant fractions of the total widths for resonances at 398   1731 1451  209
and 4251 eV. When uncertainties are considered, there is good     1731 1451  210
agreement between our resonance parameter calculations and        1731 1451  211
experiment for natCl total cross sections up to 1200 keV, for     1731 1451  212
35Cl(n,p) cross sections up to 100 keV, and for natCl capture     1731 1451  213
cross sections up to 500 keV. Our thermal elastic, capture,       1731 1451  214
(n,p), and total cross sections are in good agreement with the    1731 1451  215
corresponding ENDF/B-VI quantities, which are based primarily on  1731 1451  216
the compilation of Mughabghab [15].                               1731 1451  217
                                                                  1731 1451  218
Our evaluation fits the data much better than does ENDF/B-VI.     1731 1451  219
This new representation should be particularly applicable to      1731 1451  220
improvement of the reliability of criticality safety              1731 1451  221
calculations for systems where Cl is present.                     1731 1451  222
                                                                  1731 1451  223
The present ENDF format does not allow for a resonance parameter  1731 1451  224
representation of charged particle cross sections. A proposal is  1731 1451  225
in preparation for a new ENDF format which will permit the full   1731 1451  226
generality of the Reich-Moore theory, including charged particle  1731 1451  227
penetrabilities.   The parametric representation (File 2) will be 1731 1451  228
made available when the new ENDF format is approved.              1731 1451  229
                                                                  1731 1451  230
REFERENCES                                                        1731 1451  231
----------                                                        1731 1451  232
[1] R. O. Sayer, K. H. Guber, L. C. Leal, N. M. Larson,           1731 1451  233
    and T. Rauscher, ORNL/TM-2003/50, March, 2003.                1731 1451  234
[2] K. H. Guber, R. O. Sayer, T. E. Valentine, L. C. Leal,        1731 1451  235
    R. R. Spencer, J. A. Harvey, P. E. Koehler, and T. Rauscher,  1731 1451  236
    Phys. Rev. C65, 058801 (2002).                                1731 1451  237
[3] N. M. Larson, ORNL/TM-9179/R5 (2000).                         1731 1451  238
[4] W. M. Good, J. A. Harvey, and N. W. Hill, ORNL-4937,          1731 1451  239
    p. 198 (1973); J. A. Harvey, private communication.           1731 1451  240
[5] S. Cierjacks, P.Forti, D. Kopsch, L. Kropp, J. Nebe, and H.   1731 1451  241
    Unseld, "High Resolution Total Neutron Cross Sections for Na, 1731 1451  242
    Cl, K, V, MN and Co between 0.5 and 30 MEV",                  1731 1451  243
    KFK-1000, (1969).                                             1731 1451  244
[6] U. N. Singh, H. I. Liou, G. Hacken, M. Slagowitz, F. Rahn,    1731 1451  245
    J. Rainwater, W. Makofske, and J. Garg, "Neutron Resonance    1731 1451  246
    Spectroscopy: Chlorine", Phys. Rev. C10, 2138 (1974).         1731 1451  247
[7] R. M. Brugger, et al., Phys. Rev. 104, 1054 (1956).           1731 1451  248
[8] R. M. Kiehn, et al., Phys. Rev. 91, 66 (1953).                1731 1451  249
[9] H. W. Newson, et al., Phys. Rev. 105, 198 (1957).             1731 1451  250
[10] N. T. Kashukeev, Yu. P. Popov, and F. L. Shapiro,            1731 1451  251
     J. Nucl. Energy 14, 76 (1961).                               1731 1451  252
[11] P. E. Koehler, Phys. Rev. C44, 1675 (1991).                  1731 1451  253
[12] S. Druyts, C. Wagemans, and P. Geltenbort,                   1731 1451  254
     Nucl. Phys. A574, 291 (1994).                                1731 1451  255
[13] R. O. Sayer, ORNL/TM-2000/212 (2000).                        1731 1451  256
[14] R. E. MacFarlane and D. W. Muir, LA-12740-M (1994).          1731 1451  257
[15] S. F. Mughabghab, M. Divadeenam, N. E. Holden, Neutron Cross 1731 1451  258
     Sections, Vol. 1, Part A, Academic Press, Inc. (1981).       1731 1451  259
[16] G. H. E. Sims and D. G. Juhnke, Phys. Rev. 165, 1184 (1968). 1731 1451  260
[17] I. G. Schroder, M. McKeown, and G. Schar -Goldhaber,         1731 1451  261
     J. Inorg. Nucl. Chem. 31, 3721 (1969).                       1731 1451  262
[18] Y. M. Gledenov, V. I. Salatski, P. V. Sedyshev, P. J.        1731 1451  263
     Szalanski, J. Andrzejewski, and A. Zak, Proc. Int. Conf. on  1731 1451  264
     Nuclear Data for Science and Technology,                     1731 1451  265
     Trieste, p. 511 (1997).                                      1731 1451  266
[19] Y. M. Gledenov, L. B. Mitsina, M. Mitukov, Y. P. Popov, J.   1731 1451  267
     Rigol, V. I. Salatski, and F. Van Zuan, Joint Institute for  1731 1451  268
     Nuclear Research, Communications P3-89-351,                  1731 1451  269
     Dubna, USSR (1989).                                          1731 1451  270
[20] P. E. Koehler, et al., Phys. Rev. C54, 1463 (1996).          1731 1451  271
[21] H. Krauss, K. Grun, T. Rauscher, and H. Oberhummer, 1992,    1731 1451  272
     TU Wien (Vienna, Austria), code TEDCA (unpublished).         1731 1451  273
[22] T. Rauscher, R. Bieber, H. Oberhummer, K.-L. Kratz,          1731 1451  274
     J. Dobaczewski, P. Moller, and M. M. Sharma,                 1731 1451  275
     Phys.Rev. C57, 2031 (1998).                                  1731 1451  276
[23] R. L. Macklin, Phys. Rev. C29, 1996 (1984).                  1731 1451  277
[24] C. E. Porter and R. G. Thomas, Phys. Rev. 104, 483 (1956).   1731 1451  278
[25] E. P. Wigner, Can. Math. Congr. Proc., Toronto,              1731 1451  279
     p 174 (1957); Ann. Math 67, 325 (1958).                      1731 1451  280
****************************************************************  1731 1451  281
                                                                  1731 1451  282
 ENDF/B-VI MOD 1 Evaluation, February 2000, P.G. Young,           1731 1451  283
                 R.E. MacFarlane, L.C. Liu (LANL)                 1731 1451  284
                                                                  1731 1451  285
NEUTRON ENERGIES BELOW 202 keV ---------------------------------- 1731 1451  286
                                                                  1731 1451  287
  The resolved resonance parameter data of the JENDL3.2           1731 1451  288
evaluation by Watanabe (Wa94) was adopted.  The description of    1731 1451  289
those data in the JENDL3.2 evaluation is repeated below.          1731 1451  290
                                                                  1731 1451  291
MF=2  RESONANCE PARAMETERS(BELOW 202.0KEV)                        1731 1451  292
  MT=151 RESOLVED RESONANCE PARAMETERS                            1731 1451  293
    Resolved resonance parameters for MLBW formula with varying   1731 1451  294
  scattering radius. Negative energy level data were adjusted     1731 1451  295
  to reproduce 2200m/s cross sections.                            1731 1451  296
  Evaluation was mainly based on macklin's data [1] and           1731 1451  297
  Mughabghab's compilation [2].                                   1731 1451  298
                                                                  1731 1451  299
  Calculated 2200-m/s cross section and res. integrals (barns)    1731 1451  300
                     2200 m/s               Res. Integ.           1731 1451  301
      Total           1.583                    -                  1731 1451  302
      Elastic         1.15                     -                  1731 1451  303
      Capture         0.433                   0.204               1731 1451  304
                                                                  1731 1451  305
MF=12  PHOTON MULTIPLICITIES                                      1731 1451  306
  The spectrum of gamma rays from radiative capture is based      1731 1451  307
upon a new evaluation by A. Adams and S.C. Frankle [Ad98].        1731 1451  308
                                                                  1731 1451  309
NEUTRON ENERGIES ABOVE 202 keV ---------------------------------- 1731 1451  310
                                                                  1731 1451  311
SUMMARY                                                           1731 1451  312
   This evaluation is based primarily on a theoretical analysis   1731 1451  313
between neutron energies of 100 keV and 20 MeV that is optimized  1731 1451  314
to the somewhat limited available experimental data.  Elastic     1731 1451  315
and inelastic scattering angular distributions (through MT=76)    1731 1451  316
and the radiative capture cross section (MF=3, MT=102)            1731 1451  317
are taken from the JENDL3.2 evaluation [Wa94].                    1731 1451  318
   The theoretical calculations utilize Hauser-Feshbach           1731 1451  319
statistical theory with corrections for width fluctuations,       1731 1451  320
preequilibrium and direct reaction processes.  Spherical optical  1731 1451  321
model calculations are used to obtain the neutron total cross     1731 1451  322
section and neutron, proton, deuteron, triton, and alpha          1731 1451  323
transmission coefficients.                                        1731 1451  324
   Cross sections and spectra for individual reactions are        1731 1451  325
included for exiting neutron, proton, deuteron, alpha, and        1731 1451  326
gamma-ray reactions.  Multiplicities, angular distributions, and  1731 1451  327
emission energy spectra are given for gamma rays, particles, and  1731 1451  328
recoil nuclei emitted in the dominant reactions, utilizing File   1731 1451  329
6 of the ENDF/B-6 format [Ro91].  Energy-angle-correlated         1731 1451  330
spectra are given for all outgoing particles and photons, and     1731 1451  331
residual nuclei energy distributions are included.                1731 1451  332
                                                                  1731 1451  333
THEORY                                                            1731 1451  334
  HAUSER-FESHBACH STATISTICAL THEORY CALCULATIONS.  The GNASH     1731 1451  335
code [Yo92] was used for all Hauser-Feshbach statistical theory   1731 1451  336
calculations.  Preequilibrium corrections were performed in the   1731 1451  337
course of the GNASH calculations using the exciton model of       1731 1451  338
Kalbach [Ka77,Ka85].  Discrete level data from nuclear data       1731 1451  339
sheets were matched to continuum level densities using the        1731 1451  340
formulation of Gilbert and Cameron [Gi65] and pairing and shell   1731 1451  341
parameters from the Cook [Co67] analysis.  Neutron and charged-   1731 1451  342
particle transmission coefficients were obtained from the         1731 1451  343
optical potentials, as discussed below.  Gamma-ray transmission   1731 1451  344
coefficients were calculated using the Kopecky-Uhl model [Ko90].  1731 1451  345
  Calculations were performed for all significant reactions       1731 1451  346
producing neutrons, protons, deuterons, alpha particles, and      1731 1451  347
gamma rays for incident neutrons between 100 keV and 20 MeV.      1731 1451  348
  The angular distribution systematics by Kalbach [Ka88] were     1731 1451  349
used to describe the angular distributions for all continuum      1731 1451  350
particles.                                                        1731 1451  351
                                                                  1731 1451  352
  OPTICAL MODEL POTENTIALS.  For incident and exiting neutrons,   1731 1451  353
a phenomenological optical model potential by Arthur and Young    1731 1451  354
[Ar80], based on an analysis of n + Fe and p + Fe reactions, was  1731 1451  355
utilized for the neutron transmission coefficients, whereas the   1731 1451  356
potential of Watanabe [Wa94] was used to calculate the neutron    1731 1451  357
total cross section.  The two differenct potentials were used     1731 1451  358
because on the one hand the Watanabe potential agreed well with   1731 1451  359
total cross section measurements, whereas the Arthur potential    1731 1451  360
appears to give a better reaction cross section, which is very    1731 1451  361
important for Hauser-Feshbach calculations.  The SCAT2 optical    1731 1451  362
model code [Be92] was used for all calculations.                  1731 1451  363
   To obtain transmission coefficients for charged particle       1731 1451  364
reactions, the Beccetti-Greenlees potential [Be71] was used for   1731 1451  365
protons, the Perey and Perey [Pe63] potential for deuterons, the  1731 1451  366
Beccetti-Greenlees potential [Be69] for tritons,and the potential 1731 1451  367
of MacFadden [Mc66] was used for alpha particles.                 1731 1451  368
                                                                  1731 1451  369
  DIRECT REACTIONS:  Energy-dependent cross sections of           1731 1451  370
inelastic neutrons from 37Cl(n,n') direct reactions were          1731 1451  371
obtained using DWUCK calculations and deformation parameters      1731 1451  372
estimated from systematics using the compilations of Raman et     1731 1451  373
al. [Ra89] and Spear [Sp89].                                      1731 1451  374
                                                                  1731 1451  375
EVALUATED DATA                                                    1731 1451  376
                                                                  1731 1451  377
  CALCULATIONAL RESULTS.  The MF=3 cross sections and MF=6        1731 1451  378
energy/angle distributions that are based completely on           1731 1451  379
calculations are:                                                 1731 1451  380
                                                                  1731 1451  381
        MT =  16:     (n,2n) Reaction                             1731 1451  382
        MT =  17:     (n,3n) Reaction                             1731 1451  383
        MT =  22:     (n,nalpha) Reaction                         1731 1451  384
        MT =  28:     (n,np) Reaction                             1731 1451  385
        MT =  32:     (n,nd) Reaction                             1731 1451  386
        MT =  51-80:  (n,n') Discrete Level Reactions             1731 1451  387
        MT =  91:     (n,n') Continuum Reaction                   1731 1451  388
        MT = 103:     (n,p) Reaction                              1731 1451  389
        MT = 104:     (n,d) Reaction                              1731 1451  390
        MT = 105:     (n,t) Reaction                              1731 1451  391
        MT = 107:     (n,alpha) Reaction                          1731 1451  392
        MT = 649:     (n,p) Continuum Reaction                    1731 1451  393
        MT = 650-669: (n,d) Discrete Level Reactions              1731 1451  394
        MT = 699:     (n,d) Continuum Reaction                    1731 1451  395
        MT = 700-730: (n,t) Discrete Level Reactions              1731 1451  396
        MT = 749:     (n,t) Continuum Reaction                    1731 1451  397
        MT = 800-824: (n,alpha) Discrete Level Reactions          1731 1451  398
        MT = 849:     (n,alpha) Continuum Reaction                1731 1451  399
                                                                  1731 1451  400
   Additionally, (n,gamma) cross sections (multiplicities)        1731 1451  401
included in MF=12 and energy distributions in MF=15 are taken     1731 1451  402
from the GNASH calculations.  In addition to the usual Hauser-    1731 1451  403
Feshbach cross section component obtained using the Kopecky-Uhl   1731 1451  404
gamma-ray strength function, a semidirect component is included   1731 1451  405
in GNASH that enhances the cross section and hardens the          1731 1451  406
spectrum near En = 10-18 MeV.                                     1731 1451  407
   Discrete (n,n') cross sections and angular distributions were  1731 1451  408
calculated using a combination of the GNASH and COMNUC [Du70]     1731 1451  409
codes for compound nucleus reactions.  Preequilibrium components  1731 1451  410
were included in the (n,n') reactions at higher energies to       1731 1451  411
approximate direct reaction effects (in an average manner) for    1731 1451  412
discrete states not included in the DWUCK calculations.  Cross    1731 1451  413
sections for a total of 30 excited states are included for 37Cl.  1731 1451  414
Discrete gamma-ray cross sections that exceed 1 mb are included   1731 1451  415
explicitly in the MF=6 distributions for all reactions.  The      1731 1451  416
elastic angular distributions are included in in MF =4;  the      1731 1451  417
(n,n') angular distributions and (n,n'gamma) multiplicities are   1731 1451  418
included in MF=6.                                                 1731 1451  419
   Cross sections (MF=3) for approximately 20 or more discrete    1731 1451  420
states are included for charged-particle reactions.  Again,       1731 1451  421
multiplicities for (n,x gamma) reactions are included in MF=6.    1731 1451  422
   Kalbach systematics (Ka88) are used to specify all continuum   1731 1451  423
particle angular distributions in MF=6.  All continuum photon     1731 1451  424
angular distributions are assumed isotropic.  Residual nucleus    1731 1451  425
recoil energy spectra are included in MF=6 for all reactions.     1731 1451  426
                                                                  1731 1451  427
  USE OF EXPERIMENTAL DATA.  The available experimental data for  1731 1451  428
37Cl is somewhat limited.  Data that were useful for the          1731 1451  429
evaluation are measurements of the neutron total cross section    1731 1451  430
for natural Cl; measurements of (n,gamma) cross sections for      1731 1451  431
35Cl and 37Cl at lower energies;  and a few measurements above    1731 1451  432
12 MeV of (n,p) and (n,alpha) cross sections.                     1731 1451  433
  The only adjustment made to the calculated cross sections on    1731 1451  434
the basis of the experimental data was to fine tune the           1731 1451  435
normalization of the gamma-ray strength function calculations     1731 1451  436
using the radiative capture measurement.  The final               1731 1451  437
normalization that was determined is approximately a factor of 2  1731 1451  438
higher than the value we have established from systematics in     1731 1451  439
other analyses.                                                   1731 1451  440
                                                                  1731 1451  441
****************************************************************  1731 1451  442
                                                                  1731 1451  443
REFERENCES                                                        1731 1451  444
                                                                  1731 1451  445
[Ad98]  A. Adams and S.C. Frankle, LANL Group X-CI, personal      1731 1451  446
   communication (1998).                                          1731 1451  447
[Ar80]  E.D.Arthur and P.G. Young, "Evaluation of Neutron Cross   1731 1451  448
   Sections to 40 MeV for 54,56Fe," Proc. Sym Neutron Cross       1731 1451  449
   Sections from 10 to 50 MeV, BNL, 12-14 May 1980, p. 731.       1731 1451  450
[Be92]  O. Bersillon, "SCAT2 - A Spherical Optical Model Code,"   1731 1451  451
   in Proc. ICTP Workshop on Computation and Analysis of Nuclear  1731 1451  452
   Data Relevant to Nuclear Energy and Safety, 10 February-13     1731 1451  453
   March, 1992, Trieste, Italy, to be published in World          1731 1451  454
   |Scientific Press, and Progress Report of the Nuclear Physics  1731 1451  455
   Division, Bruyeres-le-Chatel 1977, CEA-N-2037 (1978) p.111.    1731 1451  456
[Be71]  F.D. Becchetti, Jr., and G.W. Greenlees in "Polarization  1731 1451  457
   Phenomena in Nuclear Reactions," (Ed: H.H.Barschall and        1731 1451  458
   W.Haeberli, The University of Wisconsin Press, 1971) p.682.    1731 1451  459
[Co67]  J.L. Cook, H. Ferguson, and A.R. Musgrove, Aust.J.Phys.   1731 1451  460
   20, 477 (1967).                                                1731 1451  461
[Du70]  C.L. Dunford, "A Unified Model for Analysis of Compound   1731 1451  462
   Nucleus Reactions," Atomics International report AI-AEC-12931  1731 1451  463
   (1970).                                                        1731 1451  464
[Gi65]  A. Gilbert and A.G.W. Cameron, Can.J.Phys. 43, 1446       1731 1451  465
   (1965).                                                        1731 1451  466
[Ka77]  C. Kalbach, Z.Phys.A  283, 401 (1977).                    1731 1451  467
[Ka85]  C. Kalbach, "PRECO-D2: Program for Calculating            1731 1451  468
   Preequilibrium and Direct Reaction Double Differential Cross   1731 1451  469
   Sections," Los Alamos National Laboratory report LA-10248-MS   1731 1451  470
   (1985).                                                        1731 1451  471
[Ka88]  C.Kalbach, Phys.Rev.C 37, 2350 (1988); see also           1731 1451  472
   C. Kalbach and F. M. Mann, Phys.Rev.C 23, 112 (1981).          1731 1451  473
[Ko90]  J.Kopecky and M.Uhl, Phys.Rev.C 42, 1941 (1990).          1731 1451  474
[Mc66]  L. McFadden and G.R. Satchler, Nucl. Phys. 84, 177 (1966).1731 1451  475
[Pe63a] F.G. Perey, Phys. Rev. 131, 745 (1963).                   1731 1451  476
[Pe63b] C.M. Perey and F.G. Perey, Phys. Rev. 132, 755 (1963).    1731 1451  477
[Pe72]  F.G. Perey, et al., Oak Ridge report ORNL-4823 (1972).    1731 1451  478
[Ra89]  S. Raman et al., At.Nucl.Data Tables 42, 1 (1989).        1731 1451  479
[Ro91]  P. Rose, "ENDF-102: Data Formats and Procedures for the   1731 1451  480
   Evaluated Nuclear Data File, ENDF-6," Brookhaven National      1731 1451  481
   Laboratory informal report BNL-NCS-44945 [ENDF-102, Rev. 10/91]1731 1451  482
   (1991).                                                        1731 1451  483
[Sp89]  R.H. Spear, At.Nucl.Data Tables 42, 55 (1989).            1731 1451  484
[Wa94]  T. Watanabe, JENDL-3.2 Evaluation (1994).                 1731 1451  485
[Yo92]  P.G. Young, E.D. Arthur, and M.B. Chadwick, Los Alamos    1731 1451  486
   report LA-12343-MS (1992).                                     1731 1451  487
                                                                  1731 1451  488
 ************************ C O N T E N T S *********************** 1731 1451  489
                                1        451        646          01731 1451  490
                                2        151        155          01731 1451  491
                                3          1         74          01731 1451  492
                                3          2         64          01731 1451  493
                                3          4         59          01731 1451  494
                                3         16         22          01731 1451  495
                                3         17          4          01731 1451  496
                                3         22         26          01731 1451  497
                                3         28         25          01731 1451  498
                                3         32          7          01731 1451  499
                                3         51         59          01731 1451  500
                                3         52         56          01731 1451  501
                                3         53         55          01731 1451  502
                                3         54         53          01731 1451  503
                                3         55         51          01731 1451  504
                                3         56         50          01731 1451  505
                                3         57         49          01731 1451  506
                                3         58         48          01731 1451  507
                                3         59         46          01731 1451  508
                                3         60         44          01731 1451  509
                                3         61         44          01731 1451  510
                                3         62         42          01731 1451  511
                                3         63         41          01731 1451  512
                                3         64         41          01731 1451  513
                                3         65         39          01731 1451  514
                                3         66         38          01731 1451  515
                                3         67         38          01731 1451  516
                                3         68         37          01731 1451  517
                                3         69         35          01731 1451  518
                                3         70         35          01731 1451  519
                                3         71         34          01731 1451  520
                                3         72         33          01731 1451  521
                                3         73         32          01731 1451  522
                                3         74         31          01731 1451  523
                                3         75         30          01731 1451  524
                                3         76         30          01731 1451  525
                                3         77         29          01731 1451  526
                                3         91         29          01731 1451  527
                                3        102         65          01731 1451  528
                                3        103         47          01731 1451  529
                                3        104         30          01731 1451  530
                                3        105         26          01731 1451  531
                                3        107         56          01731 1451  532
                                3        649         47          01731 1451  533
                                3        650         28          01731 1451  534
                                3        651         24          01731 1451  535
                                3        652         23          01731 1451  536
                                3        653         21          01731 1451  537
                                3        654         21          01731 1451  538
                                3        655         20          01731 1451  539
                                3        656         20          01731 1451  540
                                3        657         19          01731 1451  541
                                3        658         19          01731 1451  542
                                3        659         18          01731 1451  543
                                3        660         16          01731 1451  544
                                3        661         15          01731 1451  545
                                3        699         16          01731 1451  546
                                3        700         23          01731 1451  547
                                3        701         19          01731 1451  548
                                3        702         17          01731 1451  549
                                3        703         17          01731 1451  550
                                3        704         15          01731 1451  551
                                3        705         14          01731 1451  552
                                3        706         13          01731 1451  553
                                3        707         13          01731 1451  554
                                3        708         12          01731 1451  555
                                3        709         12          01731 1451  556
                                3        710         12          01731 1451  557
                                3        711         11          01731 1451  558
                                3        712         11          01731 1451  559
                                3        713         11          01731 1451  560
                                3        714         10          01731 1451  561
                                3        715          9          01731 1451  562
                                3        749         10          01731 1451  563
                                3        800         54          01731 1451  564
                                3        801         49          01731 1451  565
                                3        802         37          01731 1451  566
                                3        803         50          01731 1451  567
                                3        804         29          01731 1451  568
                                3        805         27          01731 1451  569
                                3        849         36          01731 1451  570
                                4          2        208          11731 1451  571
                                6         16       1034          11731 1451  572
                                6         17         64          11731 1451  573
                                6         22       1281          11731 1451  574
                                6         28       1439          11731 1451  575
                                6         32        253          11731 1451  576
                                6         51        206          11731 1451  577
                                6         52        200          11731 1451  578
                                6         53        162          11731 1451  579
                                6         54        186          11731 1451  580
                                6         55        185          11731 1451  581
                                6         56        152          11731 1451  582
                                6         57        153          11731 1451  583
                                6         58        181          11731 1451  584
                                6         59        152          11731 1451  585
                                6         60        181          11731 1451  586
                                6         61        148          11731 1451  587
                                6         62        171          11731 1451  588
                                6         63         31          11731 1451  589
                                6         64         31          11731 1451  590
                                6         65         29          11731 1451  591
                                6         66         31          11731 1451  592
                                6         67         31          11731 1451  593
                                6         68         35          11731 1451  594
                                6         69         29          11731 1451  595
                                6         70         31          11731 1451  596
                                6         71         29          11731 1451  597
                                6         72         29          11731 1451  598
                                6         73         31          11731 1451  599
                                6         74         29          11731 1451  600
                                6         75         29          11731 1451  601
                                6         76         33          11731 1451  602
                                6         77         22          11731 1451  603
                                6         91       1792          11731 1451  604
                                6        649       1400          11731 1451  605
                                6        650         13          11731 1451  606
                                6        651         22          11731 1451  607
                                6        652         22          11731 1451  608
                                6        653         22          11731 1451  609
                                6        654         22          11731 1451  610
                                6        655         22          11731 1451  611
                                6        656         24          11731 1451  612
                                6        657         22          11731 1451  613
                                6        658         24          11731 1451  614
                                6        659         22          11731 1451  615
                                6        660         24          11731 1451  616
                                6        661         24          11731 1451  617
                                6        699        523          11731 1451  618
                                6        700         13          11731 1451  619
                                6        701         22          11731 1451  620
                                6        702         22          11731 1451  621
                                6        703         22          11731 1451  622
                                6        704         26          11731 1451  623
                                6        705         26          11731 1451  624
                                6        706         30          11731 1451  625
                                6        707         26          11731 1451  626
                                6        708         34          11731 1451  627
                                6        709         32          11731 1451  628
                                6        710         34          11731 1451  629
                                6        711         34          11731 1451  630
                                6        712         26          11731 1451  631
                                6        713         36          11731 1451  632
                                6        714         24          11731 1451  633
                                6        715         28          11731 1451  634
                                6        749        338          11731 1451  635
                                6        800         13          11731 1451  636
                                6        801         22          11731 1451  637
                                6        802         22          11731 1451  638
                                6        803         24          11731 1451  639
                                6        804         24          11731 1451  640
                                6        805         30          11731 1451  641
                                6        849       1160          11731 1451  642
                               12        102        341          01731 1451  643
                               14        102          1          11731 1451  644
                               15        102        672          11731 1451  645
                               32        151      16842          11731 1451  646
 0.000000+0 0.000000+0          0          0          0          01731 1  099999
 0.000000+0 0.000000+0          0          0          0          01731 0  0    0
    17037.0 3.66483E+1          0          0          1          01731 2151    1
    17037.0 1.00000E+0          0          1          1          01731 2151    2
 1.00000E-5 1.20000E+6          1          3          0          01731 2151    3
        1.5 3.36510E-1          1          0          2          21731 2151    4
 3.66483E+1 3.36510E-1          0          0        204         341731 2151    5
-1000.000         -1.0 9.55569E+0 2.24585E-1                      1731 2151    6
8320.8168          2.0 7.87043E+1 1.96340E-1                      1731 2151    7
25579.301         -1.0 6.52216E+2 5.12780E-1                      1731 2151    8
46653.155          2.0 3.90486E+2 2.65280E-1                      1731 2151    9
93137.965          2.0 7.26630E+2 2.20590E-1                      1731 2151   10
97900.813         -1.0 1.44828E+0 7.06793E-1                      1731 2151   11
127757.07          2.0 3.91026E+2 2.67960E-1                      1731 2151   12
136284.67          2.0 1.39180E+3 2.62000E-1                      1731 2151   13
179861.20         -1.0 1.60978E+3 2.16000E-1                      1731 2151   14
186996.70          2.0 3.08529E+2 3.17500E-1                      1731 2151   15
190702.19         -1.0 1.11137E+3 4.64290E-1                      1731 2151   16
208346.42         -1.0 5.19418E+2 1.15010E-1                      1731 2151   17
221154.33          2.0 6.51564E+1 2.01470E-1                      1731 2151   18
226560.00         -1.0 4.30106E+0 4.77000E-1                      1731 2151   19
248454.69          2.0 1.33117E+2 2.67250E-1                      1731 2151   20
256783.00         -1.0 4.17880E+1 2.38430E+0                      1731 2151   21
281522.00         -1.0 1.31663E+2 3.17500E-1                      1731 2151   22
316614.00         -1.0 1.12460E+2 3.69050E-1                      1731 2151   23
334078.00         -1.0 1.03722E+3 3.65960E-1                      1731 2151   24
358378.83          2.0 7.64151E+2 2.17640E-1                      1731 2151   25
394434.66         -1.0 6.43706E+1 3.84240E-1                      1731 2151   26
431031.59          2.0 1.44137E+2 2.57810E-1                      1731 2151   27
434208.87          2.0 9.50321E+1 3.56120E-1                      1731 2151   28
493456.27          2.0 2.68702E+2 3.25210E-1                      1731 2151   29
507968.02         -1.0 3.12713E+3 8.32000E-1                      1731 2151   30
611811.00         -1.0 6.80704E+2 8.32000E-1                      1731 2151   31
627239.23          2.0 9.11936E+2 8.32000E-1                      1731 2151   32
649606.24          2.0 2.01671E+3 1.66400E+0                      1731 2151   33
670190.25          2.0 6.15710E+2 1.66400E+0                      1731 2151   34
747621.31          2.0 2.99169E+2 1.66400E+0                      1731 2151   35
789290.76          2.0 2.61745E+2 1.66400E+0                      1731 2151   36
1083306.4          2.0 1.64105E+3 1.66400E+0                      1731 2151   37
1482061.7          2.0 7.11829E+3 6.65600E+0                      1731 2151   38
1809579.4         -1.0 3.03262E+5 4.16000E-1                      1731 2151   39
 3.66483E+1 3.95652E-1          1          0        690        1151731 2151   40
27824.080         -2.0 5.53672E+0 7.88080E-2                      1731 2151   41
32187.017         -1.0 1.05349E+1 8.22790E-2                      1731 2151   42
42357.528         -1.0 2.78949E-1 2.60250E-1                      1731 2151   43
51547.653          3.0 3.32885E+0 7.84590E-2                      1731 2151   44
55145.856          0.0 3.92100E+0 7.00000E-2                      1731 2151   45
55440.455         -2.0 1.22796E+2 1.78840E-1                      1731 2151   46
66706.817         -2.0 2.59186E+1 1.07030E-1                      1731 2151   47
66837.404         -2.0 5.08838E+1 1.54030E-1                      1731 2151   48
86210.589         -1.0 1.10318E+0 2.51860E-1                      1731 2151   49
114740.00          0.0 2.50001E+2 3.30930E-1                      1731 2151   50
125259.29          3.0 3.11079E+1 6.00000E-3                      1731 2151   51
125508.33          3.0 2.63789E+1 6.00000E-3                      1731 2151   52
128224.65         -1.0 3.54931E+1 2.80900E-1                      1731 2151   53
135433.59          0.0 1.63916E+2 2.37990E-1                      1731 2151   54
143721.36          3.0 6.52968E+2 1.70610E-1                      1731 2151   55
144342.04         -1.0 6.40858E+1 1.54440E-1                      1731 2151   56
150084.40          1.0 8.96480E+1 5.14680E-1                      1731 2151   57
150672.36         -2.0 1.26628E+1 4.12480E-1                      1731 2151   58
157563.33         -2.0 1.48925E+2 1.65580E-1                      1731 2151   59
164953.72          0.0 2.14949E+2 1.17560E+0                      1731 2151   60
166468.76         -1.0 8.65883E+1 8.27230E-1                      1731 2151   61
167300.69         -1.0 5.15496E+1 2.85680E-1                      1731 2151   62
168957.98         -2.0 2.48027E+2 1.50990E-1                      1731 2151   63
176722.52          2.0 1.66176E+2 3.61310E-1                      1731 2151   64
177610.18          0.0 4.58508E+2 4.88030E-1                      1731 2151   65
179905.01         -1.0 1.16814E+2 2.15660E-1                      1731 2151   66
191133.97          1.0 1.84361E+2 3.91970E-1                      1731 2151   67
213225.38         -1.0 2.59126E+1 1.27690E+0                      1731 2151   68
214159.25          0.0 2.71190E+2 1.71820E+0                      1731 2151   69
217675.44          0.0 4.30707E+2 3.10410E+0                      1731 2151   70
218656.21          0.0 1.51040E+2 3.57580E-1                      1731 2151   71
219681.31          0.0 1.07211E+2 3.56340E-1                      1731 2151   72
227655.20          0.0 4.42782E+1 9.19090E-1                      1731 2151   73
229903.20          0.0 2.48750E+2 2.40640E-1                      1731 2151   74
244091.54          3.0 2.29533E+1 2.35090E-1                      1731 2151   75
254030.66         -2.0 6.94032E+2 3.65730E-1                      1731 2151   76
254781.56          1.0 6.39852E+1 5.47810E-1                      1731 2151   77
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